Topics: Particulate matter Variation Characteristics of Particles Mass Concentration in Urban Air of Changsha Wang Qi* Shanghai Research institute of Building Sciences(Group) Co,Ltd., Shanghai, China * Corresponding email:[email protected] Keywords: particulate matter, mass concentration, PM10, PM2.5 1 Introduction 2 Methods As the rapid developing of urbanization, atmospheric pollution is very serious especial particulate matter. Scientists and governments pay more attention to particles all over the world, as it would have the potential impacts on the global climate change and the effect on the health to human beings. Many epidemiological studies showed that there was strong correlation between the level of particle and human health. The rise of particle concentration has lead to a significant increase of morbidity and mortality in respiratory and cardiovascular diseases. ( Brunekreef and Holgate, 2002; Samet et al., 2000 ) The mass concentrations of particles were measured in urban air of Changsha from November 2007 to October 2008. The real-time mass concentrations of PM10 were measured using a TEOM monitor (50℃, R&P 1400a). The TSI Model 8520 DustTrak aerosol monitor with a 2.5μm inlet was used to measure the real-time approximation of PM2.5 concentration. The PM2.5 values obtained using this instrument which operates based on a light scattering technique were not actual gravimetric values. In order to obtain values close to true PM2.5 from the data collected by the DustTrak, an additional experiment was conducted under laboratory conditions to compare the DustTrak data with the data of TEOM. Based on the results of this additional experiment, the following liner regression equation was obtained: The communique of environment in Hunan province 2007 reported re-suspension of particles was main atmospheric pollutant especially PM10, the average annual concentration of PM10 was higher than the limit Ⅱof National Air Quality Standard in Changsha. The main aim of this study was to investigate variation characteristics of particles mass concentration in urban air of Changsha. PM2.5 (TEOM) = 0.367 PM2.5 (DustTrak) 8.428 (1) (with R2 = 0.90) Morawska et al. (2003) also conducted the same comparison study. All statistical analyses were conducted using a statistical analysis software package-SPSS 13.0. 3 Results and Discussion PM10 was primary atmospheric pollution in Changsha and the concentration of PM10 was high. Average diurnal concentrations of PM10 were 116.4±42.6μg/m3 122.3±46.1μg/m3 125.0±57.4μg/m3 in summer, autumn and winter in Fig 1. Average diurnal concentrations of PM10 were higher in autumn and winter than concentration in summer. This can be explained by the domestic use of coal fuels in autumn and winter. There was a correlation between indoor and outdoor PM10 without indoor source and correlation coefficients varied from 0.84 to 0.93 (p<0.01), showing that outdoor levels influenced indoor concentrations. Finally, the relationship between PM10 and PM2.5 was investigated. PM10 concentration was strongly associated with PM2.5 (p<0.01), as showed in Fig3. It was suggested that PM2.5 was main part in PM10. Fig.3. Relationship between PM10 and PM2.5. Fig.1. Particle concentrations at different seasons. Average diurnal variations of PM10 presented two peaks in Fig 2. The morning peak hour was at about 8-10 a.m. and the evening peak hours at 5-7 p.m. The phenomena mainly attributed to traffic emission and meteorological parameters. Mönkkönen et al., 2004 also found the similar effect in New Delhi. 4 Conclusions In the past ten years, particulate pollution was mainly caused by coarse particle. The government focused on PM10 and established Ambient air quality standard. However, recent years, PM2.5 has been received more attention because of local traffic. Much future research on PM2.5 will be essential. 5 References Brunekreef B., Holgate S.T., Air pollution and health. Lancet, 2002, 360: 1233-1242. Samet J.M., Dominici F., Curriero F.C., et al. Fine particulate air pollution and mortality in 20 US cities. 1987-1994, New England Journal of Medicine, 2000, 343: 1742-1749. Morawska L., He C., Hitchins J., et al. 2003. Characteristics of particle number and mass concentrations in residential houses in Brisbane, Australia. Atmospheric Environment, 2003, 37(30), 4195-4203. Fig.2. Average diurnal variation of PM10 concentrations. Mönkkönen P, Uma R, Srinivasan D, et al. Relationship and variations of aerosol number and PM10 mass concentrations in a highly polluted urban environment – New Delhi, India. Atmospheric Environment,2004,38(3): 425-433.
© Copyright 2024 Paperzz