SPECTROSCOPIC STUDY OF THE IONIZATION DYNAMICS IN A CO2 LASER-PRODUCED PLASMA OF HELIUM J. Gauthier, J. Geindre, N. Grandjouan To cite this version: J. Gauthier, J. Geindre, N. Grandjouan. SPECTROSCOPIC STUDY OF THE IONIZATION DYNAMICS IN A CO2 LASER-PRODUCED PLASMA OF HELIUM. Journal de Physique Colloques, 1979, 40 (C7), pp.C7-735-C7-736. <10.1051/jphyscol:19797355>. <jpa-00219350> HAL Id: jpa-00219350 https://hal.archives-ouvertes.fr/jpa-00219350 Submitted on 1 Jan 1979 HAL is a multi-disciplinary open access archive for the deposit and dissemination of scientific research documents, whether they are published or not. The documents may come from teaching and research institutions in France or abroad, or from public or private research centers. L’archive ouverte pluridisciplinaire HAL, est destinée au dépôt et à la diffusion de documents scientifiques de niveau recherche, publiés ou non, émanant des établissements d’enseignement et de recherche français ou étrangers, des laboratoires publics ou privés. JOURNAL DE PHYSIQUE CoZZoque C7, suppZ6ment au n07, Tome SO, JuiZZet 1979, page C7- 735 SPECTROSCOPIC STUDY OF THE IONIZATION DYNAMICS IN A C02 LASER-PRODUCED PLASMA OF HELIUM J.C. Gauthier, J.P. Geindre and N. Grandjouan. Groupe drEZectroniwue dans Zes Gaz. I n s t i t u t drEZectronique Fondamentale, k b o r a t o i r e associe' au C.N. R.S,, Universitg Paris-XI- BEt. 220, 91405 Orsay Cedex, France. This paper r e p o r t s on a spectroscopic study of HELlA 760 TORR - t h e i o n i z a t i o n dynamics of C02 l a s e r induced plasmas m - A - i n medium p r e s s u r e helium gas. Previous s t u d i e s have shown /1-3/ t h a t t h e v a r i o u s mechanisms of plasma evolution i n space and time a r e n o t f u l l y elucidated and may vary s t r o n g l y with experimental conditions. I n t h i s experiment, a W preionized TEA C02 l a s e r d e l i v e r e d approximately 1 J i n a p u l s e which c o n s i s t s of a n i n t e n s e s p i k e % I 0 0 n s wide, followed by a weaker emission about 20% o f t h e peak of some 1QQQ n s duration. The p u l s e g e p e t s t i o n r a t e $5 3 p u l s e s p e r second. Plasma d i a g n o s t i c s were c a r r i e d F i q . 1 ~Time r e s o l v e d s p e c t r a a t lmm above f o c u s . S t a r k broadened He1 l i n e s a r e prominent above t h e continuum. The 4686 o u t with a high degree o f p r e c i s i o n and r e l i a b i l i t y by t a k i n g advantage o f t h e good shot-to-shot repro- d u c i b i l i t y and of t h e high r e p e t i t i o n r a t e of t h e - ' L B'i 3, -- ? -- 15 32 3 z - E l a s e r . Spectroscopic measurements were made with a > -temporal r e s o l u t i o n of 8 ns and a s p a t i a l resolutiion b e t t e r than 0.1 mm i n both t h e a x i a l ( z ) and t h e r a d i a l ( r ) d i r e c t i o n , using a computer c o n t r o l l e d data a c q u i s i t i o n system a l r e a d y described /4/. A t y p i c a l time resolved spectrum taken a t 1 atm. about Imm above t h e focus i s shown on Fig.1. Time ~lDiE1440 and space-resolved measurements taken along t h e l a s e r a x i s a r e shown on Figs.2a-c. They g i v e r e s p e c t i - I, cxF-it- IP d SE76.BZ 1132 - v e l y t h e i n t e n s i t y of t h e continuum i n a s p e c t r a l region f r e e from atomic and i o n i c l i n e s , t h e i n t e n 9 3 3 s i t y of t h e 3 D-2 P (5876 A) He1 t r a n s i t i o n , a n d t h e i n t e n s i t y o f t h e n=4 t o n=3 (4686 A) He11 t r a n s i t i o n both c o r r e c t e d from t h e i r underlying continuum. The time s c a l e o r i g i n corresponds t o t h e beginning of t h e l a s e r p u l s e . R e s u l t s obtained over t h e range Article published online by EDP Sciences and available at http://dx.doi.org/10.1051/jphyscol:19797355 8. He11 l i n e a p p e a r s by 300 n s . C7- 736 0.7-2.5 atm. were q u a l i t a t i v e l y t h e same. A break- 3/ E.V.GEORGE, Fluids down plasma c o n s i s t i n g mainly of ~ e i+o n s (only t h e G-BEFEKI and B.YAIAKOBI 14,2708 (1971) - Phys. . 4/ N. GRANDJOUAN, J-C.GAUTHIER and J-P-GEINDRE continuum and He1 s p e c t r a a r e observed) appears near C.R. Ac. S c i . 284, 437 - (1977). t h e f o c a l plane (z=O) during t h e r i s i n g edge o f t h e pulse. An expansion f r o n t w i t h a n i n i t i a l v e l o c i t y of 5x10 6 cm/s i s observed t o move i n a d i r e c t i o n op- p o s i t e t o t h a t o f t h e i n c i d e n t l a s e r beam. By 300 ns t h e plasma v e l o c i t y d e c r e a s e s while t h e t r a i l i n g edge of t h e luminous f r o n t moves toward t h e focus.ThiS p e r i o d i s dominated by a s h a r p r i s e of HeII emission ( F i g . 2 ~ )and a s t r o n g decrease of both continuum and He1 emissions (Fig.2a-b). These r e s u l t s confirmed t h e time-resolved spectrum o f Fig.1. The e l e c t r o n temperature i n c r e a s e c h a r a c t e r i z e d by t h e a p p a r i t i o n of HeII r a d i a t i o n was found t o be d i r e c t l y proport i o n a l t o t h e f r a c t i o n of l a s e r energy contained i n - Time r e s o l v e d i n t e n s i t i e s a l o n g z . L a s e r from t e f t t o o r i g h t a ) continuum (4750 i) ; b ) He1 emiss i o n (5876 A) ; c ) HeII emission (4686 i). Fig.2 - t h e hil. I n a d d i t i o n , t h e i n i t i a l speed o f t h e plasma f r o n t and t h e time of HeII r a d i a t i o n appearance were a l s o found t o be p r o p o r t i o n a l t o t h e g a s p r e s s u r e . This r u l e s o u t a r a d i a t i o n d r i v e n d e t o n a t i o n mecha- nism /1/ of expansion under t h e p r e s e n t c o n d i t i o n s . Also, p h o t o i o n i z a t i o n of t h e unheated g a s ahead of t h e plasma f r o n t i s u n l i k e l y t o occur s i n c e t h e el e c t r o n temperature deduced from t h e i o n i z a t i o n s t a t e i n t h e i n i t i a l plasma i s too low (4 eV). I n s t e a d , plasma e v o l u t i o n i s governed by l a s e r d r i v e n i o n i z a t i o n dynamics. Radial o b s e r v a t i o n s shown i n Figs.3a -b f u r t h e r s u b s t a n t i a t e t h i s hypothesis. The h b t plasma c o r e (800 ns on Fig.3b) b u i l d s up from t h e bulk o f t h e c o l d plasma through absorbed IR r a d i a t i o n from t h e l a s e r t a i l . Indeed, experiments with a C02 p u l s e f r e e from tail e m i s s i o n d i s p l a y a consider a b l e r e d u c t i o n o f t h e hot c o r e s i z e and temperature The b l a s t wave mechanism s t a t e d i n Ref.3 4 s t h u s t o b e rejected. Further studies of plasma ,parameters mder &mi. l a r conditions a r e presented in the following paper. 1/ Yu.P. RAIZER - Sov. Phys. Uspekhi 2/ N. AHMAD, B.C.GALE A310, 231 (1969). and M.H.KEY 8, 650 (1966). - PrOc. ROy.Soc. Fig.3 - Time r e s o l v e d * n t e n s i t i e s aloong r a t 1 mm above f o c u s . a ) oHeI emission (5876 A) ; b) HeII ,-I., e m i s s i o n (4686 A ) . i
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