Flame initiation by nanosecond plasma discharges: Putting some new spark into ignition Paul D. Ronney University of Southern California, USA National Central University Jhong-Li, Taiwan, October 3, 2005 Research supported by U.S. AFOSR, ONR & DOE Travel supported by the Combustion Institute Faculty collaborator: Martin Gundersen (USC-EE) Research Associates: Nathan Theiss, Jian-Bang Liu Graduate students: Jason Levin, Fei Wang, Jun Zhao, Tsutomu Shimizu Undergraduate students: Brad Tallon, Matthew Beck Jennifer Colgrove, Merritt Johnson, Gary Norris University of Southern California Established 125 years ago this week! …jointly by a Catholic, a Protestant and a Jew - USC has always been a multi-ethnic, multi-cultural, coeducational university Today: 32,000 students, 3000 faculty 2 main campuses: University Park and Health Sciences USC Trojans football team ranked #1 in USA last 2 years USC Viterbi School of Engineering Naming gift by Andrew & Erma Viterbi Andrew Viterbi: co-founder of Qualcomm, co-inventor of CDMA 1900 undergraduates, 3300 graduate students, 165 faculty, 30 degree options $135 million external research funding Distance Education Network (DEN): 900 students in 28 M.S. degree programs; 171 MS degrees awarded in 2005 More info: http://viterbi.usc.edu Paul Ronney B.S. Mechanical Engineering, UC Berkeley M.S. Aeronautics, Caltech Ph.D. in Aeronautics & Astronautics, MIT Postdocs: NASA Glenn, Cleveland; US Naval Research Lab, Washington DC Assistant Professor, Princeton University Associate/Full Professor, USC Research interests Microscale combustion and power generation (10/4, INER; 10/5 NCKU) Microgravity combustion and fluid mechanics (10/4, NCU) Turbulent combustion (10/7, NTHU) Internal combustion engines Ignition, flammability, extinction limits of flames (10/3, NCU) Flame spread over solid fuel beds Biophysics and biofilms (10/6, NCKU) Paul Ronney Transient plasma ignition - motivation Multi-point ignition of flames has potential to increase burning rates in many types of combustion engines, e.g. Pulse Detonation Engines Reciprocating Internal Combustion Engines » (Simplest approach) Leaner mixtures (lower NOx) » (More difficult) Redesign intake port and combustion chamber for lower turbulence since the same burn rate is possible with lower turbulence (reduced heat loss to walls, higher efficiency) High altitude restart of gas turbines Lasers, multi-point sparks challenging Lasers: energy efficiency, windows, fiber optics Multi-point sparks: multiple intrusive electrodes How to obtain multi-point, energy efficient ignition? Transient plasma (“pulsed corona”) discharges Not to be confused with “plasma torch” Initial phase of spark discharge (< 100 ns) - highly conductive (arc) channel not yet formed Characteristics Multiple streamers of electrons High energy (10s of eV) electrons compared to sparks (~1 eV) Electrons not at thermal equilibrium with ions/neutrals Ions stationary - no hydrodynamics Low anode & cathode drops, little radiation & shock formation - more efficient use of energy deposited into gas Corona vs. arc discharge Corona phase (0 - 100 ns) Arc channel High voltage pulse Arc phase (> 100 ns) Images of corona discharge & flame Axial (left) and radial (right) views of discharge with rod electrode Axial view of discharge & flame (6.5% CH4-air, 33 ms between images) Characteristics of corona discharges For short durations (1’s to 100’s of ns depending on pressure, geometry, gas, etc.) DC breakdown threshold of gas can be exceeded without breakdown if high voltage pulse can be created and stopped quickly enough Breakdown strength (kV/cm) 100 90 Transient Steady 80 70 60 50 40 30 20 0 50 100 Time (ns) 150 200 Characteristics of corona discharges Voltage (KV) Energy 80 15 60 10 40 5 20 Current 0 -5 -50 0 50 100 150 Time (ns) 0 200 250 -20 300 20 150 Voltage 100 Energy 15 Current 10 50 5 0 0 -5 -50 Start of arc 0 50 100 150 Time (ns) 200 250 -50 300 Corona + arc Corona only If arc forms, current increases some but voltage drops more, thus higher consumption of capacitor energy with little increase in energy deposited in gas (still have corona, but followed by (relatively ineffective) arc) Current (amps) or Energy (mJ) Voltage Current (amps) or Energy (mJ) 20 25 100 Voltage (KV) 25 Corona discharges are energy-efficient Discharge efficiency d ≈ 10x higher for corona than conventional sparks P Volume Energy deposited in gas 1 d Electrical discharge energy IVdt Discharge efficiency 1 0.1 0.01 10 Corona, 1 pin, Cylindrical combustion chamber Corona, ring electrode IC engine like chamber Corona, Threaded rod electrode Cylindrical combustion chamber Spark, plain wire electrodes, gap = 1 mm Cylindrical combustion chamber Spark, Car spark plug IC engine like chamber 100 Energy (mJ) 1000 Objectives Compare combustion duration and ignition energy requirements of spark-ignited and corona-ignited flames in constant-volume vessel Determine effect of corona electrode geometry and ignition energy on combustion duration Determine if reduced combustion duration observed for corona ignition in quiescent, constant-volume experiments also applies to turbulent flames Integrate pulsed corona discharge ignition system into premixed-charge IC engines Compare performance of corona-ignited and spark-ignited engines Efficiency Emissions Experimental apparatus (constant volume) Pulsed corona discharges generated using thyratron or “pseudospark” gas switch + Blumlein transmission line 2.5” (63.5 mm) diameter chamber, 6” (152 mm) long Rod electrode (shown below) or single-needle Energy release (stoich. CH4-air, 1 atm) ≈ 1650 J energy release ≈ Discharge energy input for ignition is trivial fraction of heat release! Definitions Delay time: 0 - 10% of peak pressure Rise time: 10% - 90% of peak pressure 12 10 8 6 90% of total pressure rise Delay Time 14 Discharge trigger Pressure (atm., abs) 16 Rise Time 10% of total pressure rise 4 2 -0.02 0 0.02 0.04 Time (s) 0.06 0.08 0.1 Electrode configurations Rod electrode 1 ring with multi-pins (only 4 pins case is shown) Single pin electrode Multi-rings with 2 pins/ring (Only 4 rings case is shown) Insulation is indicated with shaded patern Pulsed corona discharges in IC engine-like geometry QuickTime™ and a Cinepak decompressor are needed to see this picture. Top view QuickTime™ and a Cinepak decompressor are needed to see this picture. Side view Minimum ignition energy vs. mixture 1 pin corona discharge vs. spark - ≈ same geometry MIE significantly higher (≈ 100x) for corona - more distributed energy deposition in streamers? Minimum spark kernel diameter ≈ 0.2 mm for stoich. CH4-air 1000 CH /Air Energy (mJ) 4 1 pin electrode 1 atm 100 Pulsed corona 10 Spark (Lewis and von Elbe) 1 0.1 0.6 0.7 0.8 0.9 1 1.1 Equivalence ratio 1.2 1.3 Pressure effects on MIE Energy (mJ) MIE for pulsed corona does NOT follow Emin ~ P-2 as spark ignition does; more like P-1 at low P, P0 at higher P Smaller chamber diameter enables ignition at higher P higher voltage gradient Ignited (2.5") Not Ignited (2.5") Ignited (1.1") Not Ignited (1.1") MIE (2.5") MIE (1.1") 100 CH -air, = 1 4 Single-pin electrode 10 0.1 1 P (atm) 10 Effect of geometry on delay time corona, 1 pin, 75 mJ spark, 75 mJ corona, 3.9 mm dia rod, 710 mJ corona, 2 ring x 2 pin, 170 mJ corona, 4 ring x 2 pin 170 mJ Delay Time (ms) 100 CH /Air 4 10 0.65 P = 1 atm 0.7 0.75 0.8 0.85 0.9 Equivalence ratio 0.95 1 1.05 Effect of geometry on delay time Delay time of spark larger (≈ 1.5 - 2x) than 1-pin corona (≈ same geometry) Consistent with computations by Dixon-Lewis, Sloane that suggest point radical sources improve ignition delay ≈ 2x compared to thermal sources More streamer locations (more pins, rod) yield lower delay time (≈ 3.5x lower for rod than spark) Suggests benefit of corona is both chemical (1.5 - 2x) and geometrical (≈ 2x) Effect of geometry on rise time corona, 1 pin, 75 mJ spark, 75 mJ corona, 3.9 mm dia. rod, 710 mJ corona, 2 ring x 2 pin, 170 mJ corona, 4 ring x 2 pin, 170 mJ Rise Time (ms) 100 CH /Air 4 P = 1 atm 10 0.65 0.7 0.75 0.8 0.85 0.9 Equivalence ratio 0.95 1 1.05 Effect of geometry on rise time Rise time of spark larger ≈ same as 1-pin corona (≈ same flame propagation geometry) More streamer locations (more pins, rod) yield lower rise time (≈ 3 - 4x lower for rod than spark), but multi-pin almost as good with less energy Peak pressures 6 CH /Air Peak P/P o 5.5 4 1 atm 5 4.5 4 corona, 1 pin, 75 mJ spark at center, 75 mJ corona rod, 710 mJ corona, 2 ring x 2 pin, 170 mJ corona, 4 ring x 2 pin, 170 mJ 3.5 3 0.65 0.7 0.75 0.8 0.85 0.9 0.95 Equivalence ratio 1 1.05 Peak pressures Peak pressures significantly higher for multi-point corona that one-pin corona or spark Improvement (for rod) nearly independent of mixture Probably due to change in flame propagation geometry, not heat losses Radial propagation (corona) vs. axial propagation (arc) Corona: more combustion occurs at higher pressure (smaller quenching distance) Corona: lower fraction of unburned fuel Consistent with preliminary measurements of residual fuel Energy & geometry effects on delay time What is optimal electrode configuration to minimize delay/rise time for a given energy? Delay time: 2-ring, 4-ring & plain rod similar (all are much better than spark) 35 corona, 1 ring x 2 pin corona, 2 ring x 2 pin corona, 4 ring x 2 pin corona, 3.9 mm dia. rod Spark Delay Time (ms) 30 25 20 CH /Air 15 = 1.0 P = 1 atm 4 10 5 00 100 200 300 400 500 Discharge energy (mJ) 600 700 Energy & geometry effects on rise time Rise time: 2-ring or 4-ring best Note “step” behavior for multi-point ignition at low energies - not all sites ignite Delay time doesn’t show “step” behavior 70 corona, corona, corona, corona, Spark Rise Time (ms) 60 50 1 ring x 2 pin 2 ring x 2 pin 4 ring x 2 pin 3.9 mm dia. rod 40 CH /Air 30 = 1.0 P = 1 atm 4 20 10 0 0 100 200 300 400 500 Discharge energy (mJ) 600 700 Energy & geometry effects (lean mixture) Delay time: same conclusion as stoichiometric mixture Delay Time (ms) 120 corona, 1 ring x 2 pin corona, 2 ring x 2 pin corona, 4 ring x 2 pin spark corona, 3.9 mm dia rod 100 80 60 40 CH /Air 4 = 0.7 P = 1 atm 20 0 0 100 200 300 400 Discharge Energy (mJ) 500 600 Energy & geometry effects (lean mixture) Rise time: 4-ring stands out corona, 1 ring x 2 pin corona, 2 ring x 2 pin corona, 4 ring x 2 pin spark corona, 3.9 mm dia rod 350 Rise Time (ms) 300 250 CH /Air 4 = 0.7 P = 1 atm 200 150 100 50 0 0 100 200 300 400 Discharge Energy (mJ) 500 600 Rod diameter effects File:030820 Plain rod: optimal diameter exists (≈ 0.15”), drod/dcyl ≈ 0.06 Large d: low field concentration, few streamers? Small d: Too many streamers, too much energy deposition? Delay or Rise Time (ms) 70 Delay T ime (ms) 60 Rise T ime (ms) CH4/Air Equivalence ratio: 1.0 P=1 atm. Rod-cylinder electrode Rod diameter: 0.09" 50 40 30 20 10 0 0 200 File:030813 Delay Time (ms) Rise Time (ms) 50 CH4/Air Equiv alence ratio: 1.0 P=1 atm. Rod-cy linder electrode Rod diameter: 0.155" 40 30 20 10 0 0 100 200 300 400 500 Energy (mJ/pulse) 600 600 800 700 1000 File:030818 100 Delay or Rise Time (ms) Delay or Rise Time (ms) 70 60 400 Energy (mJ/pulse) Delay Time (ms) Rise Time (ms) 80 CH4/Air Equiv alence ratio: 1.0 P=1 atm. Rod-cy linder electrode Rod diameter: 0.375" 60 40 20 0 0 100 200 300 400 Energy (mJ/pulse) 500 600 CH4/Air Equivalence ratio: 0.7 Delay Time (ms) P=1 atm. Rise T ime (ms) 1 ring x 1 pin electrode 180 Delay T ime (ms) File:030416 Rise T ime (ms ) Delay or Rise Time (ms) Delay or Rise Time (ms) Effect of number of pins on 1 ring 160 140 120 100 80 180 File:030509 160 140 120 100 80 60 60 80 90 100 110 120 130 140 40 150 60 Delay Time (ms) Rise Time (ms) Delay Time (ms) File:030515a Rise T ime (ms) Delay or Rise Time (ms) 200 CH4/Air Equiv alence ratio: 0.7 P=1 atm. 1 ring x 4 pin electrode 150 100 250 50 60 70 80 Energy (mJ) 90 100 110 100 120 140 CH4/Air Equivalence ratio: 0.7 P=1 atm. 1 ring x 8 pin electrode File:030516 200 150 100 50 0 120 50 40 80 Energy (mJ) Energy (mJ) Delay or Rise Time (ms) CH4/Air Equivalence ratio: 0.7 P=1 atm. 1 ring x 2 pin electrode 140 160 180 200 Energy (mJ) 220 240 Effect of number of pins on 1 ring MIE lower (!!) with more pins, optimal 4 More pins: Slightly beneficial effect on delay time, slightly adverse effect (!) on rise time More is not necessarily better! Energy (mJ) or time (ms) 250 Minimum ignition energy Maximum energy without arcing Average delay time Average rise time 200 CH /Air 4 = 0.7 P = 1 atm 150 100 50 0 0 2 4 6 Number of pins 8 10 Thyratron vs. pseudospark generator Little effect of discharge generator type (pseudospark: ≈ 1/2 discharge duration compared to thyratron) 20 20 Pseudo-spark generator 15 Thyratron-switched generator 10 5 0 400 Rise Time (ms) Delay Time (ms) Pseudo-spark generator CH /Air 4 600 700 Energy (mJ/pulse) 800 900 Thyratron-switched generator 10 5 = 1.0 1 atm Threaded electrode 500 15 0 400 CH /Air 4 = 1.0 1 atm Threaded electrode 500 600 700 800 Discharge energy (mJ) 900 Turbulent test chamber HV Anode Fan Grounded Cathode Turbulence effects Simple turbulence generator (fan + grid) integrated into coaxial combustion chamber, rod electrode Turbulence intensity ≈ 1 m/s, u’/SL ≈ 3 (stoichiometric) Benefit of corona ignition ≈ same in turbulent flames - shorter rise & delay times, higher peak P Note quiescent corona faster than turbulent spark! (Faster burn with less heat loss) 4 CH /Air 4 Pressure (atm) 3.5 = 1.0 1 atm 3 Quiescent, spark 2.5 2 Turbulent, spark Quiescent, corona 1.5 Turbulent, corona 1 -0.02 0 0.02 0.04 Time (s) 0.06 0.08 0.1 Turbulence effects Similar results for lean mixture but benefit of turbulence more dramatic - higher u’/SL (≈ 8) 0.6 CH /Air 0.55 Pressure (V) 0.5 4 = 0.7 1 atm Quiescent, corona 0.45 0.4 Quiescent, spark 0.35 Turbulent, spark 0.3 Turbulent, corona 0.25 0.2 -0.05 0 0.05 0.1 0.15 Time (s) 0.2 0.25 0.3 Engine experiments 2000 Ford Ranger I-4 engine with dual-plug head to test corona & spark at same time, same operating conditions National Instruments / Labview data acquisition & control Horiba emissions bench, samples extracted from corona equipped cylinder Pressure / volume measurements Optical Encoder mounted to crankshaft Spark plug mounted Kistler piezoelectric pressure transducer Electrode configuration Macor machinable ceramic used for insulator Coaxial shielded cable used to reduce EMI Simple single-point electrode tip, replaceable “Point to plane” geometry first step - by no means optimal On-engine corona ignition system Corona electrode and spark plug with pressure transducer in #1 cylinder Wired for quick change between spark and corona ignition under identical operating conditions ≈ 500 mJ/pulse (equivalent “wall plug” energy requirement of ≈ 50 mJ spark) Range of ignition timings for both spark & corona 3 modes tested Corona only Single conventional plug Two conventional plugs (results very similar to single plug) On-engine corona ignition system On-engine results Corona ignition shows increase in peak pressure under all conditions tested On-engine results Corona ignition shows increase in IMEP under all conditions tested IMEP at various air / fuel ratios Indicated mean effective pressure (IMEP) higher for corona than spark, especially for lean mixtures (nearly 30%) Coefficient of variance (COV) comparable 40 0.1 35 IMEP (psi) 30 IMEP (spark) IMEP (corona) 25 0.06 20 0.04 15 10 5 0 0.65 0.02 COV (spark) COV (corona) 0.7 0.75 0.8 0.85 0.9 Equivalence ratio 0.95 1 0 1.05 Coefficient of Variance 0.08 IMEP at various loads Corona showed an average increase in IMEP of 16% over a range of engine loads 40 0.4 3000 RPM, Phi = 0.7 0.35 30 0.3 25 0.25 Spark Corona Spark COV Corona COV 20 15 0.2 COV IMEP (psia) 35 0.15 10 0.1 5 0.05 0 0 0 5 10 15 Torque (ft-lb) 20 25 Burn rate Integrated heat release shows faster burning with corona leads to greater effective heat release 2900 RPM, = 0.7 Burn rates Corona ignition shows substantially faster burn rates at same conditions compared to 2-plug conventional ignition 2900 RPM, = 0.7 Emissions data - NOx Improved NOx performance vs. indicated efficiency tradeoff compared to spark ignition by using leaner mixtures with sufficiently rapid burning Emissions data - hydrocarbons Hydrocarbons emissions similar, corona vs. spark 100 BSHC (g/hp-hr) spark corona 10 1 0 0.1 0.2 Indicated Efficiency 0.3 0.4 Emissions data - CO CO emissions similar, corona vs. spark 1000 BSCO (g/hp-hr) spark corona 100 10 1 0 0.1 0.2 Indicated Efficiency 0.3 0.4 Conclusions Flame ignition by transient plasma or pulsed corona discharges is a promising technology for ignition delay & rise time reduction More energy-efficient than spark discharges Shorter ignition delay and rise times Rise time more significant issue » Longer than delay time » Unlike delay time, can’t be compensated by “spark advance” Higher peak pressures Benefits apply to turbulent flames also Demonstrated in engines too Higher IMEP for same conditions with same or better BSNOx Shorter burn times and faster heat release Improvements due to Chemical effects (delay time) - radicals vs. thermal energy Geometrical effects - (delay & rise time) - more distributed ignition sites Future work Improved electrode designs Solid-state discharge generators Multi-cylinder corona ignition Corona-ignited, low turbulence (thus low heat loss) engines??? Transient plasma discharges for fuel electrospray dispersion? Thanks to… National Central University Prof. Shenqyang Shy Combustion Institute (Bernard Lewis Lectureship) AFOSR, ONR, DOE (research support)
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