Frequency dependencies of phase velocity and attenuation coefficient in a water-saturated sandy sediment from 0.3 to 1.0 MHz Kang Il Lee Department of Physics, Kangwon National University, Chuncheon 200–701, Republic of Korea Victor F. Humphrey Institute of Sound and Vibration Research, University of Southampton, Southampton SO17 1BJ, United Kingdom Byoung-Nam Kim and Suk Wang Yoona兲 Department of Physics and Institute of Basic Science, Sungkyunkwan University, Suwon 440-746, Republic of Korea 共Received 24 March 2006; revised 19 January 2007; accepted 9 February 2007兲 The frequency-dependent phase velocity and attenuation coefficient for the fast longitudinal wave in a water-saturated sandy sediment were measured over the frequency range from 0.3 to 1.0 MHz. The experimental data of phase velocity exhibited the significant negative dispersion, with the mean rate of decline of 120± 20 m / s / MHz. The Biot model predicted the approximately nondispersive phase velocity and the grain-shearing 共GS兲 model exhibited the slightly positive dispersion. In contrast, the predictions of the multiple scattering models for the negative dispersion in the glass-grain composite were in general agreement with the experimental data for the water-saturated sandy sediment measured here. The experimental data of attenuation coefficient was found to increase nonlinearly with frequency from 0.3 to 1.0 MHz. However, both the Biot and the GS models yielded the attenuation coefficient increasing almost linearly with frequency. The total attenuation coefficient given by the algebraic sum of absorption and scattering components showed a reasonable agreement with the experimental data for overall frequencies. This study suggests that the scattering is the principal mechanism responsible for the variations of phase velocity and attenuation coefficient with frequency in water-saturated sandy sediments at high frequencies. © 2007 Acoustical Society of America. 关DOI: 10.1121/1.2713690兴 PACS number共s兲: 43.30.Ma 关RAS兴 Pages: 2553–2558 I. INTRODUCTION The Biot model 共Biot, 1956a, b, 1962兲 for elastic wave propagation in porous media has been applied to sediment acoustics with varying degrees of success. It was originally applied to the analysis of ultrasound geophysical test data for porous rock samples. In 1970, the model was applied by Stoll and Bryan 共1970兲 in a form more suitable for watersaturated sediments. Recently, Buckingham 共1997, 2000, 2005兲 developed the grain-shearing 共GS兲 model for wave propagation in saturated, unconsolidated granular materials, including marine sediments. Since the mineral grains are unbonded, it is assumed that the shear rigidity modulus of the medium is zero, implying the absence of a skeletal elastic frame. The GS model has been successfully applied to predict the relationship between mechanical properties, such as grain size and porosity, and acoustic properties of marine sediments. Chotiros and Isakson 共2004兲 also proposed a new theoretical model based on the grain-to-grain contacts in unconsolidated granular materials. Dispersion of phase velocity has been extensively investigated in marine sediments by a number of authors 共Hamp- ton, 1967; Wingham, 1985; Turgut and Yamamoto, 1990; Stoll, 2002; Tang et al., 2002; Williams et al., 2002; Chotiros and Isakson, 2004兲. Most of the studies have been performed over various frequency ranges from a few hundreds of hertz up to a few hundreds of kilohertz, where the propagation of interest occurs over ranges that are sufficiently long to include bottom interactions. The fast longitudinal wave in marine sediments has been known to exhibit the positive dispersion of phase velocity at frequencies lower than about 200 kHz, which is predicted by theoretical models such as the Biot and the GS models. In contrast, an interesting highfrequency experimental study demonstrated that the fast wave velocity in water-saturated sandy sediments shows the negative dispersion from 0.2 to 1.2 MHz 共Moussatov et al., 1998兲. However, the velocity dispersion predicted by the Biot model has been reported to be very weak, but positive at frequencies higher than 0.2 MHz 共Moussatov et al., 1998兲, and the GS model also tends to predict the slightly positive dispersion in this frequency range 共Buckingham, 1997兲. These results may imply that the underlying mechanism responsible for the velocity dispersion in the high frequency range is different from that in the low frequency range. Thus, a兲 Electronic mail: [email protected] J. Acoust. Soc. Am. 121 共5兲, May 2007 0001-4966/2007/121共5兲/2553/6/$23.00 © 2007 Acoustical Society of America 2553 both the Biot and the GS models may only have validity in a limited range of frequency for the dispersion of phase velocity in water-saturated sediments. As extensively discussed by Buckingham 共2005兲 and Ohkawa 共2006兲, the frequency dependence of attenuation coefficient in marine sediments has been argued for many years. The Biot model predicts an attenuation coefficient increasing as the half power of frequency, which is due to the fluid viscosity only. Nolle et al. 共1963兲 found the f 1/2 dependence of attenuation coefficient in water-saturated sands at frequencies of 0.2, 0.5, and 1.0 MHz. In contrast, most data exhibit a linear scaling of attenuation coefficient with frequency over a wide range of frequencies 共Wingham, 1985; Hamilton, 1987兲, which is consistent with the prediction of the GS model based on grain-to-grain shearing mechanisms 共Buckingham, 1997兲. In fact, the GS model yields an attenuation coefficient that is almost but not quite linear in frequency. On the other hand, Ohkawa 共2006兲 demonstrated that the frequency dependence of attenuation data collected during the sediment acoustics experiment in 1999 共SAX99兲 follows f 1/2 at frequencies below 50 kHz, as the Biot model predicts, and the deviation of attenuation from the Biot model at frequencies higher than 200 kHz is due to effects of scattering. This suggests that the scattering is likely to be the principal mechanism responsible for the attenuation in the ultrahigh frequency range. The present study aims to provide an insight into the frequency dependencies of phase velocity and attenuation coefficient for the fast longitudinal wave in a water-saturated sandy sediment over the frequency range from 0.3 to 1.0 MHz. The frequency-dependent phase velocity and attenuation coefficient in the water-saturated sandy sediment were measured using two different matched pairs of transducers with a diameter of 25.4 mm and center frequencies of 0.5 and 1.0 MHz. They were compared with the predictions obtained from the Biot and the GS models. FIG. 1. Schematic diagram of the experimental setup for ultrasonic measurements in through-transmission geometry. B. Ultrasonic measurements Figure 1 illustrates the schematic diagram of the experimental setup for ultrasonic measurements in throughtransmission geometry. A sediment specimen and transducers were immersed in a water bath with the dimensions of 650 mm⫻ 750 mm⫻ 1500 mm at room temperature. Two different matched pairs of unfocused, broadband transducers with a diameter 共D兲 of 25.4 mm and center frequencies of 0.5 MHz 共Panametrics V301兲 and 1.0 MHz 共Panametrics V302兲 were used in order to cover the wide range of frequencies of interest. The opposing faces of coaxially aligned transducers were separated by a distance of 150 mm, greater than the near-field distances 共D2 / 4兲 of 53 and 108 mm for the 0.5 and the 1.0 MHz transducers. A 200 MHz pulser/ receiver 共Panametrics 5900PR兲 was used to generate pulses and to receive signals. Received signals were averaged over 100 pulses in time domain using a 500 MHz digital storage oscilloscope 共LeCroy LT342兲 and stored on a computer for off-line analysis. In order to measure the phase velocity, the received signals were recorded with and without the sediment specimen in the acoustic path. The frequency-dependent phase velocity c p共兲 was determined by II. MATERIALS AND METHODS A. Sandy sediment The sandy sediment used in the present study was composed of clean medium sand with a porosity of 0.408± 0.013 and a mean grain diameter of 425± 84 m spanned from 250 to 500 m. The grain sizes of the sediment were much smaller than the ultrasonic wavelength 共兲 over the bandwidth investigated. The sediment was boiled for 1 h to remove air bubbles and to saturate it with water. The watersaturated sediment was then poured into a small rectangular container immersed in water with one aperture at its top. The sediment container has the dimensions of 100 mm ⫻ 100 mm⫻ 50 mm. The thickness of 50 mm was chosen to optimize the measurement of velocity dispersion and to avoid excessive attenuation of ultrasonic pulses. In order to minimize the transmission losses at the surfaces of the container perpendicular to wave propagation, its front and back walls 共i.e., the faces which measured 100⫻ 100 mm2兲 were made from thin plastic films 100 m thick. 2554 J. Acoust. Soc. Am., Vol. 121, No. 5, May 2007 c p共 兲 = cw , 1 − 关cw⌬共兲/d兴 共1兲 where is the angular frequency of the wave, d is the thickness of the specimen, and ⌬共兲 is the difference in unwrapped phases of the received signals with and without the specimen. The unwrapped phase difference ⌬共兲 was calculated by taking the fast Fourier transform 共FFT兲 of the digitized received signal, as follows 共Wear, 2000兲. The phase of the signal at each frequency was taken to be the inverse tangent of the ratio of the imaginary to real part of the FFT at that frequency. Since the inverse tangent function yields principal values between − and , the phase had to be unwrapped by adding an integer multiple of 2 to all frequencies above each frequency where a discontinuity appeared. The temperature-dependent speed of sound in distilled water, cw, is given by 共Kaye and Laby, 1995兲 Lee et al.: Acoustic properties of a water-saturated sediment cw = 1402.9 + 4.835T − 0.047016T2 + 0.00012725T3 , 共2兲 where T is the temperature in °C. The estimates of Eq. 共2兲 were consistent with the measured values in the water bath given the precision of the digital thermometer used. Measurements of phase velocity were also repeated with the specimen reversed. A total of 10 measurements 共5 measurements in each direction兲 were obtained for a mean value, repositioning the specimen after each measurement. The sound speed in the sediment, ranging approximately from 1590 to 1680 m / s, is sufficiently close to that in fresh water at room temperature, 1483 m / s, that potential diffraction-related errors in this substitution method caused by the disparity in speeds between the two media may be ignored 共Verhoef et al., 1985; Xu and Kaufman, 1993兲. The attenuation coefficient was determined by using the same signal acquired for phase velocity measurements, as follows. The FFT was taken to obtain the amplitude spectrum of the signal. The signal loss as a function of frequency was obtained by subtracting the logarithm of the amplitude spectrum of the signal through the sediment specimen from that through water only, and divided by the thickness of the specimen to determine the attenuation coefficient in units of dB/cm. Finally, the attenuation coefficient was corrected by taking into account the transmission losses at each interface, water/sediment and sediment/water, over the range of frequencies of interest. Ten measurements of attenuation coefficient in the specimen were averaged to obtain a mean value. FIG. 2. 共a兲 Temporal signals and 共b兲 pressure spectra measured with and without the sediment in the acoustic path for the pair of 0.5 MHz transducers. III. RESULTS AND DISCUSSION A. Temporal signals and pressure spectra B. Frequency dependence of phase velocity Figures 2 and 3 show the temporal signals and their corresponding pressure spectra measured with and without the sediment in the acoustic path, using the two different pairs of transducers with the center frequencies of 0.5 and 1.0 MHz. The temporal signals observed in the sediment correspond to the fast longitudinal wave. In the present study, no attempt was made to measure the slow wave in the sediment. As shown in Figs. 2 and 3, each sediment signal exhibits an earlier arrival time than that observed in water. This is because the sound speed in the sediment is greater than that in water. It is notable that the sediment signal for the pair of 1.0 MHz transducers in Fig. 3共a兲 exhibits pulse elongation with the higher frequencies arriving later, characteristic of negative dispersion. As can be seen in spectra, the center frequencies of the pulses were clearly shifted to lower frequencies, resulting from increasing attenuation with frequency. This is more pronounced for the pulse centered at 1.0 MHz than that at 0.5 MHz. The usable frequency bandwidths were taken to be from 0.3 to 0.7 MHz for the pair of 0.5 MHz transducers and from 0.5 to 1.0 MHz for the pair of 1.0 MHz transducers. The frequency-dependent phase velocity in the watersaturated sandy sediment was experimentally measured and theoretically predicted by the Biot and the GS models. The experimental results were plotted as a function of frequency in Fig. 4, over the usable frequency bandwidths of the transducers, i.e., from 0.3 to 0.7 MHz for the 0.5 MHz transducer measurements 共circles兲 and from 0.5 to 1.0 MHz for the 1.0 MHz transducer measurements 共asterisks兲. The error bars denote the standard deviations of ten measurements and represent the random uncertainties of the measurement procedure. It should be noted that there is some overlap of the two frequency bandwidths, i.e., from 0.5 to 0.7 MHz, where the phase velocities for the two sets of transducers agree within the experimental uncertainty. As clearly seen in Fig. 4, the average of measurements of phase velocity exhibits the significant negative dispersion, with the velocity ranging from 1680± 5 m / s at 0.3 MHz to 1590± 4 m / s at 1.0 MHz. The mean rate of decline in phase velocity was 120± 20 m / s / MHz between 0.3 and 1.0 MHz. This negatively sloped trend is similar to that measured in watersaturated sandy sediments from 0.2 to 1.2 MHz by Moussatov et al. 共1998兲 共1760– 1680 m / s兲. J. Acoust. Soc. Am., Vol. 121, No. 5, May 2007 Lee et al.: Acoustic properties of a water-saturated sediment 2555 TABLE I. Input parameters of the Biot model for a water-saturated sandy sediment. FIG. 3. 共a兲 Temporal signals and 共b兲 pressure spectra measured with and without the sediment in the acoustic path for the pair of 1.0 MHz transducers. The solid and the dashed curves in Fig. 4 represent the phase velocities predicted by the Biot and the GS models, respectively. The input parameters of the Biot and the GS models for a water-saturated sandy sediment are summarized Parameter Value Density of sand grain 共s兲 Density of fluid 共 f 兲 Bulk modulus of sand grain 共Ks兲 Bulk modulus of fluid 共K f 兲 Bulk modulus of frame 共Kb兲 Shear modulus of frame 共b兲 Bulk log decrement 共␦k兲 Shear log decrement 共␦兲 Viscosity of fluid 共兲 Permeability 共兲 Pore size parameter 共a兲 Tortuosity 共␣兲 Porosity 共兲 2650 kg/ m3 1000 kg/ m3 36.9 GPa 2.2 GPa 66.3 MPa 24.9 MPa 0.15 0.2 0.001 Pa s 1 ⫻ 10−10 m2 58.2 m 1.73 0.408 in Tables I and II. A large amount of information can be found in the literature about the determination of the parameters required for these two models 共Chotiros, 1995; Buckingham, 1997, 2000, 2005; Williams et al., 2002兲. The sediment depth parameter, d = 0.063 m, in Table II was determined by curve fitting the prediction of the GS model to the experimental data of phase velocity at 0.3 MHz. As seen in Fig. 4, the Biot model predicts the approximately nondispersive phase velocity over the frequency range from 0.3 to 1.0 MHz and the GS model exhibits the slightly positive dispersion. This suggests that both of these models may not be suitable at very high frequencies for the dispersion of phase velocity in water-saturated sediments. Multiple scattering models have shown to be useful in gaining an insight into wave propagation in unconsolidated granular composites saturated with fluid. Schwartz and Plona 共1984兲 reported success in applying multiple scattering techniques 共Nicholson and Schwartz, 1982; Tsang et al., 1982兲 to the dispersion of phase velocity and attenuation in the glassand the Plexiglas™-grain composites from 0.3 to 2.0 MHz. They used suspensions comprised of water-saturated, roughly monosized spherical grains with a porosity of 0.380. Especially, the glass grain had similar acoustic properties 共 TABLE II. Input parameters of the GS model for a water-saturated sandy sediment. FIG. 4. Experimental and theoretical phase velocities plotted as a function of frequency for the fast longitudinal wave in the water-saturated sandy sediment. 2556 J. Acoust. Soc. Am., Vol. 121, No. 5, May 2007 Parameter Value Density of grain 共s兲 Density of fluid 共 f 兲 Bulk modulus of grain 共Ks兲 Bulk modulus of fluid 共K f 兲 Longitudinal coefficient 共␥ p0兲 Shear coefficient 共␥s0兲 Strain-hardening index 共n兲 rms grain roughness 共⌬兲 Reference depth in sediment 共d0兲 Reference grain diameter 共u0兲 Reference porosity 共0兲 Depth in sediment 共d兲 Grain diameter 共ug兲 Porosity 共兲 2650 kg/ m3 1000 kg/ m3 36.9 GPa 2.2 GPa 388.8 MPa 45.9 MPa 0.0851 4.55 m 0.3 m 1000 m 0.377 0.063 m 425 m 0.408 Lee et al.: Acoustic properties of a water-saturated sediment FIG. 5. Experimental and theoretical velocity shifts plotted as a function of frequency for the fast longitudinal wave in the water-saturated sandy sediment and in the glass-grain composite. s = 2480 kg/ m3, cs = 5850 m / s兲 and a mean diameter 共545 m兲 to those of the sand grain of the sediment used here. They compared the model predictions with the experimental data and concluded that, at high frequencies, the Plexiglas-grain composite exhibits the stronger scattering effects than the glass. It is notable that both unconsolidated composites showed the significant negative dispersion of phase velocity and the multiple scattering models, such as the familiar quasicrystalline approximation 共QCA兲 and the self-consistent effective medium approximation 共EMA兲, could successfully explain the negative dispersion 共Schwartz and Plona, 1984兲. Figure 5 compares the predictions of these multiple scattering models for the glass-grain composite against the experimental data for the water-saturated sandy sediment measured here. It can be seen that the experimental results for the water-saturated sandy sediment presented in this study are also in general agreement with their predictions for the negative dispersion in the glass-grain composite. Future studies will apply the multiple scattering techniques to elucidate the characteristics of dispersion in the watersaturated sediment in more depth. C. Frequency dependence of attenuation coefficient Figure 6 shows the experimental and theoretical attenuation coefficients plotted as a function of frequency for the fast longitudinal wave in the water-saturated sandy sediment over the same frequency range as shown in Fig. 4. The error bars denote the standard deviations of ten measurements. It is shown that the experimental measurements are in good agreement with each other over the overlapped frequency bandwidth 共from 0.5 to 0.7 MHz兲. The solid and the dashed curves in Fig. 6 represent the attenuation coefficients predicted by the Biot and the GS models, using the input parameters in Tables I and II, respectively. As seen in Fig. 6, the attenuation data increase nonlinearly with frequency whereas both the Biot and the GS models yield the attenuation coefficient that is almost linear in frequency from 0.3 to 1.0 MHz. It can also be seen that the Biot model consistently underestimates the experimental measurement of atJ. Acoust. Soc. Am., Vol. 121, No. 5, May 2007 FIG. 6. Experimental and theoretical attenuation coefficients plotted as a function of frequency for the fast longitudinal wave in the water-saturated sandy sediment. tenuation. This is because the Biot model predicts absorption due to the viscous dissipation of the pore fluid only. In contrast, the prediction obtained from the GS model is larger than the measurement over most of the frequency range. Ohkawa 共2006兲 found an excellent agreement between the SAX99 attenuation data and the calculated attenuation coefficient given by the algebraic sum of absorption and scattering components. The absorption attenuation corresponds to the viscous dissipation of the pore fluid following the f 1/2 dependence, as the Biot model predicts, and the scattering attenuation is given by the empirical f 2 dependence obtained by curve fitting to the experimental data for watersaturated fine sands with a mean grain diameter of 230 m measured by Seifert et al. 共1999兲. The dotted curve in Fig. 6 represents the total attenuation coefficient, ␣, in units of dB/ cm, calculated using ␣ = ␣a + ␣s , 共3兲 where ␣a is the absorption of the Biot model and ␣s is the scattering obtained by curve fitting to the experimental data of attenuation coefficient for the water-saturated sandy sediment measured here, expressed as ␣s = 0.28 ⫻ 10−10 ⫻ 20 log共e兲f 2 , 共4兲 where f is the frequency of the wave in hertz. As found in Fig. 6, the total attenuation coefficient shows a reasonable agreement with the experimental data for overall frequencies. These findings underpin the fact that the scattering is the dominant cause of attenuation in the water-saturated sandy sediment with a mean grain diameter of 425 m from 0.3 to 1.0 MHz. However, the scattering attenuation becomes weaker at lower frequencies and effects of the fluid viscosity may become more important. The role of absorption and scattering in attenuation at low and high frequencies provides an explanation for the difference observed when comparing in situ and laboratory measurements. Lee et al.: Acoustic properties of a water-saturated sediment 2557 IV. CONCLUSIONS We have investigated the frequency dependencies of phase velocity and attenuation coefficient for the fast longitudinal wave in a water-saturated sandy sediment over the frequency range from 0.3 to 1.0 MHz. The experimental data of phase velocity exhibited the significant negative dispersion, with the mean rate of decline of 120± 20 m / s / MHz. The Biot model predicted the approximately nondispersive phase velocity and the GS model exhibited the slightly positive dispersion. In contrast, the predictions of the multiple scattering models, such as the familiar QCA and the selfconsistent EMA, for the negative dispersion in the glassgrain composite were in general agreement with the experimental data for the water-saturated sandy sediment measured here. The experimental data of attenuation coefficient was found to increase nonlinearly with frequency from 0.3 to 1.0 MHz. However, both the Biot and the GS models yielded the attenuation coefficient increasing almost linearly with frequency. The total attenuation coefficient given by the algebraic sum of absorption and scattering components showed a reasonable agreement with the experimental data for overall frequencies. This study suggests that the scattering is the principal mechanism responsible for the variations of phase velocity and attenuation coefficient with frequency in water-saturated sandy sediments at high frequencies. ACKNOWLEDGMENTS This work was supported by the Korea Research Foundation Grant funded by the Korean Government 共MOEHRD兲 共KRF-2005-214-C00060兲. The authors thank the referees for their cogent and insightful comments. Biot, M. A. 共1956a兲. “Theory of propagation of elastic waves in a fluidsaturated solid. I. Low-frequency range,” J. Acoust. Soc. Am. 115, 168– 178. Biot, M. A. 共1956b兲. “Theory of propagation of elastic waves in a fluidsaturated solid. II. Higher frequency range,” J. Acoust. Soc. Am. 28, 179– 191. Biot, M. A. 共1962兲. “Generalized theory of acoustic propagation in porous dissipative media,” J. Acoust. Soc. Am. 34, 1254–1264. Buckingham, M. 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