QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY Q. J. R. Meteorol. Soc. (in press) Published online in Wiley InterScience (www.interscience.wiley.com) DOI: 10.1002/qj.84 Ice hydrometeor microphysical assumptions in radiative transfer models at AMSU-B frequencies A. M. Doherty,a * T. R. Sreerekha,b† U. M. O’Keeffea and S. J. Englisha a b Met Office, Exeter, UK University of Bremen, Bremen, Germany ABSTRACT: Comparisons between two radiative transfer models, ARTS and RTTOV, showed that results in the presence of scattering from ice hydrometeors are highly dependent on assumptions made about the ice microphysics, specifically the size distribution and the density of the ice particles. This paper presents the results of a comparison study between a number of different treatments for the ice microphysics in RTTOV. Of the approaches considered, the combination of a size-dependent density (larger ice particles are less dense) and a size distribution treatment based on the cloud temperature and ice water content give the best approximation for the cases examined. Further work is planned in other regimes to see if this approach can be applied more widely. Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd KEY WORDS satellite data; microwave; scattering; NWP Received 27 September 2006; Revised 21 March 2007; Accepted 28 March 2007 1. Introduction For many years, Numerical Weather Prediction (NWP) centres have been assimilating microwave radiances from satellites. However, the data used have been limited to clear fields of view because these cases are far simpler to model than cloudy cases. NWP requires an observation operator for each assimilated observation type to link the observed variable with physical atmospheric variables. In the case of satellite radiances, this operator is a Radiative Transfer Model (RTM). An RTM requires atmospheric profiles in order to model the upwelling radiation at the Top Of the Atmosphere (TOA). When the radiation observed is only absorbed and emitted by the atmosphere, as in the cloud free case, modelling is relatively straightforward. However, when thick cloud is present microwave radiation is also scattered and this proves far more difficult to model. The problem is partly the complexity of the calculation, which makes models solving the full scattering Radiative Transfer Equation (RTE) very expensive, and partly the lack of knowledge about the parameters on which scattering depends, namely the spatial distribution of cloud hydrometeors and the microphysics of those hydrometeors. In this paper we focus on ice hydrometeors, which have a strong scattering effect on microwave frequencies above ∼85 GHz. There are a number of methods of solving the RTE in an RTM, many of which employ approximations to reduce the cost and make models viable for NWP. These * Correspondence to: A. M. Doherty, Met Office, FitzRoy Road, Exeter, EX1 3PB. E-mail: [email protected] † Present address: Met Office, Exeter, UK. include the Eddington approximation (e.g. Kummerow, 1993), Monte-Carlo methods (e.g. Davis et al., 2005) and discrete ordinate techniques (Emde et al., 2004). Many comparisons between RTMs have been made, mainly at lower frequencies where scattering effects are less pronounced (e.g. Smith et al., 2002) but also more recently at higher frequencies in order to look at the effects of scattering (e.g. Kim et al., 2004). These show that given accurate inputs, different approaches to solving the equation of radiative transfer perform to a similar standard. Other studies such as Skofronick-Jackson et al. (2002) show that assumptions about microphysical parameters have a significant effect on the calculated TOA brightness temperature (BT). In scattering conditions RTMs calculate upwelling TOA microwave radiances using single scattering parameters (extinction, albedo and the asymmetry matrix) which are dependent on the ice microphysics, but the calculation of which is fundamentally independent of the radiative transfer problem itself. All RTMs contain assumptions about the microphysics of the cloud hydrometeors, and it is here that the main uncertainties in simulating TOA BT arise, rather than in the approach to radiative transfer. Parametrizations of microphysics should be as accurate as possible, but above all they should be consistent with the model providing the input profiles and the model calculating the single scattering parameters. This opinion is also given in the COST 712 report on microwave remote sensing in clouds and precipitation (Czekala et al., 2000). Atmospheric profiles, including those of cloud hydrometeors, can be obtained from an NWP forecast model. However, this rarely provides information on the bulk Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. A. M. DOHERTY ET AL. microphysical properties of clouds. If information is available it is diagnostic, not prognostic (Li et al., 2005). In the Met Office Mesoscale model, used in this case to generate inputs to the RTM, the prognostic variables are cloud ice and a liquid plus vapour variable; everything else is diagnostic. The shape, size distribution, permittivity and density of the particles within an ice cloud are unknown and must be parametrized or approximated. These have a significant impact on the results of the RT calculations (Hogan et al., 2000; Skofronick-Jackson et al., 2002). The bulk microphysics of clouds has been investigated by many measurement campaigns, both airborne (e.g. Baum et al., 2005) and ground-based (e.g. Shupe et al., 2005), and has been found to be highly variable both in time and space, from cloud to cloud and even within individual clouds (Hogan et al., 2000; Benedetti et al., 2003; Gayet et al., 2004). Czekala et al. (2000) concluded that knowledge of bulk microphysical hydrometeor properties and their relation to individual hydrometeor optical properties is one of the key areas where effort is required in this field. Aircraft measurement campaigns have been the most common approach for investigating ice cloud microphysics. Many parametrizations have been developed using data sets from such campaigns which link atmospheric variables to the unknown microphysical parameters. For instance, McFarquhar and Heymsfield (1997) used temperature and ice water content to parametrize the size distribution of ice particles in tropical cirrus and Field et al. (2005) carried out a similar analysis to obtain particle size distribution (PSD) parametrizations for midlatitude stratiform cloud. However, in many RTMs and NWP centres, less flexible PSDs are still in use, such as those of Marshall and Palmer (1948) and Sekhon and Srivastava (1970). The need for variability is addressed by dividing hydrometeors into a number of categories (rain, snow, hail, graupel, cloud liquid and cloud ice) and applying a different size distribution and maximum and minimum size to each type. There is no consensus in the literature as to which approach is best. Ice hydrometeor density has generally been approximated as a constant in radiative transfer and cloud resolving models. Variability has been introduced by categorizing ice hydrometeors into different types, each with its own constant density. This is a crude approximation as the density of a snow or ice particle is not independent of its size (Heymsfield et al., 2004). Density relations have been extensively studied through the use of aircraft data, with mass–size parametrizations being developed by Heymsfield et al. (2004), Brown and Francis (1995) and others. Hogan et al. (2000) examined some of these density relations and investigated the effect of a 40% error in density on retrieval of frozen hydrometeor diameter and ice water content (IWC) using dual frequency radar. They found that the density assumption is a larger source of error in retrieving diameter than either crystal habit or the shape of the size distribution. However, they did not reach a conclusion about which mass–size relation best parametrizes density for any particular situation and stress the importance of resolving this issue for remote sensing applications in precipitating cloud. It should be noted that one set of parametrizations is not going to be appropriate for all situations and the microphysical information available from operational models is not currently sufficient to allow a choice to be made between available schemes. In this paper a number of parametrizations of the density and size distribution of ice hydrometeors is examined. Investigation is undertaken of their effect on scattering RT calculations at microwave frequencies (the frequencies of the channels of the Advanced Microwave Sounder Unit B (AMSU-B) instrument, i.e. 89–183 GHz) in the RTTOV model (Saunders et al., 1999). The assumption is made that at frequencies below 200 GHz ice particles can be approximated by spheres, allowing the application of Mie theory. Although the assumption of spheres will introduce errors to the calculations, these are thought to be smaller than those associated with the other uncertainties. This approximation is widely used in other work recorded in the literature (e.g. Brown et al., 1995; Hogan et al., 2000; Bennartz and Petty, 2001). Hogan et al. (2000) quote an error of less than 15% in calculations of scattering parameters using a T-matrix code by assuming spherical particles compared to using more realistic shapes such as hexagonal columns and plates or dendritic snowflakes. The expense of using these more complex scattering models precludes their use in NWP, and no prior information is available about which shape would be more suitable. Given that Hogan et al. (2006) quote an error of roughly 40% in the derivation of IWC from radar due to the uncertainty in the shape of the size distribution, the error introduced by the assumption of spherical particles is of secondary importance. Section 2 describes the AMSU-B instrument. The RTMs are described in Section 3. Section 4 presents one of the case studies used in the comparisons. Section 5 describes the density and PSD models used in this study. Section 6 presents the results of the comparisons using different microphysics in RTTOV and Section 7 gives the summary and conclusions. 2. AMSU-B AMSU-B is a side-scanning nadir-viewing instrument, which is part of the Advanced Television Infrared Observation Satellite (TIROS) Operational Vertical Sounder (ATOVS) suite carried on the NOAA polar orbiting satellites NOAA 15–18. It has five channels numbered as AMSU channels 16–20, with AMSU channels 1–15 belonging to the AMSU-A instrument. The AMSU-B channels are sensitive to atmospheric water vapour and hydrometeors and their weighting functions peak at different altitudes throughout the atmosphere. In standard atmospheric conditions, AMSU channel 16 (89 GHz) is a surface channel and channel 17 (150 GHz) peaks low in the atmosphere with a large contribution from the surface. The other channels peak successively higher in the Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. Q. J. R. Meteorol. Soc. (in press) DOI: 10.1002/qj ICE HYDROMETEOR MICROPHYSICS FOR RADIATIVE TRANSFER atmosphere starting with channel 20 (183 ± 7 GHz) at a water vapour burden of about 10 kg m−2 , then channel 19 (183 ± 3 GHz) and channel 18 (183 ± 1 GHz) at the highest altitude, at a water vapour burden of about 0.8 kg m−2 (Staelin, 1987). AMSU-B has a field of view of 1.1° corresponding to a nadir resolution of 16 km (Muller et al., 1994). Each AMSU-B scan line takes 2.67 s to complete with 90 fields of view per line. The maximum scan angle of AMSU-B is 48.3° , and the innermost scans are at 0.55° . AMSU-B is a total power radiometer and measures the combined horizontal and vertical polarization of the incoming radiation. The proportion of the measured radiation that is vertically polarized is 100% at nadir and decreases with increasing scan angle (Saunders et al., 1995). The cross-track scanning nature of the AMSU-B instrument means that it records measurements with variable polarization along the scan. There is also a representation of spatial cloud variability along the scan and off-nadir effects due to the slant path of the observation. These effects are assumed to be of secondary importance to the signals presented in this paper from variations in the ice microphysical assumptions. 3. Radiative transfer models 3.1. RTTOV Radiative Transfer (RT) for the Television infrared observation satellite Operational Vertical Sounder (TOVS) (RTTOV) is a fast RTM developed by the EUMETSAT Satellite Application Facility for NWP (http://www. metoffice.gov.uk/research/interproj/nwpsaf/index.html) for use with nadir viewing instruments such as AMSU (Saunders et al., 1999). RTTOV 8.7 (http://www. metoffice.gov.uk/research/interproj/nwpsaf/rtm/index. html) was released in November 2005. It includes the ability to model microwave scattering in the presence of snow and ice cloud (Bauer et al., 2006). RTTOV assumes a plane parallel atmosphere and spherical hydrometeors, allowing the use of Mie Theory. The scattering calculations are solved using the delta-Eddington approximation (Wu and Weinman, 1984; Bauer, 2002) and surface emissivity is calculated using FASTEM-3 (English et al., 2003). The Maxwell-Garnett approach (Maxwell-Garnett, 1904) is used to account for the fraction of an ice particle comprising ice, liquid water or air and to calculate the refractive index. RTTOV 8.7 requires temperature, pressure and humidity profiles plus profiles of four hydrometeor types: rain, snow, liquid cloud and ice cloud. A Marshall-Palmer size distribution (Marshall and Palmer, 1948) is assumed for the precipitating hydrometeors and a modified gamma distribution for the cloud hydrometeors. The density of the ice hydrometeors is constant and set to 0.9 g cm−3 for ice and 0.1 g cm−3 for snow. In the work presented in this paper, RTTOV 8.7 was modified to allow the use of different size distributions and densities. 3.2. The Atmospheric Radiative Transfer System (ARTS) ARTS is an RTM developed by the University of Bremen for use with upward, downward and limb viewing instruments. It deals with scattering by solving the full vector radiative transfer equation using a multi-stream solution, so it is a slower model than RTTOV but more exact in its calculations (Sreerekha et al., 2002). ARTS uses spherical Earth geometry and in the version used here is run in one-dimensional mode using the discrete ordinate iterative method (Emde et al., 2004). For the ARTS results shown in this paper, FASTEM was implemented to calculate surface emissivity over the ocean (English and Hewison, 1998) and the McFarquharHeymsfield PSD was adopted for ice hydrometeors (McFarquhar and Heymsfield, 1997). Ice density was a constant at 0.91 g cm−3 . Ice hydrometeor refractive indices were calculated using data from Warren (1984). Liquid cloud hydrometeors were also considered in the RT calculations, although precipitating hydrometeors were not. As a result, the liquid hydrometeors input to ARTS differed from that used in RTTOV as rain was not included. However, ice inputs were identical as RTTOV was also adjusted to accept only one frozen hydrometeor type. In a separate study (Courcoux et al., 2006), ARTS and RTTOV have been compared using identical microphysics. The comparisons showed very close agreement between the two RTMs (∼1 K) when identical assumptions were made. 4. Case study A number of case studies over the UK were chosen for the purposes of investigating the effect of ice hydrometeor microphysical assumptions in RTTOV. The case study from 25 January 2002, 13 UTC, when a frontal system with thick ice cloud and heavy rain was present over the UK, is presented here. The input profiles for the RTMs were obtained from the Met Office Mesoscale model, which has a horizontal resolution of 12 km. The forecast fields were for a 13 UTC forecast and the NOAA 16 overpass was at 13:32, so there is a discrepancy of 32 min between model and observation times. Figure 1 shows the Advanced Very High Resolution Radiometer (AVHRR) infrared (IR) image for this case. As error analysis of the Met Office model forecast fields is not an aim of this paper, we make the assumption that these fields can be assumed to be without bias in the following. 5. Ice microphysical assumptions There are a number of treatments for size distribution and density of ice hydrometeors available in the literature. Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. Q. J. R. Meteorol. Soc. (in press) DOI: 10.1002/qj A. M. DOHERTY ET AL. Figure 1. AVHRR IR image for case study showing a strong frontal system across the UK. However, we have no information about separate ice hydrometeor types in the input files used from the Met Office Mesoscale model, and consider all ice hydrometeor types together. In this paper, there is no distinction between, for example, cloud ice, snow, graupel and hail. 5.1. ρ = 8.74×10−4 exp (−0.625 D 2 )+4.5×10−5 . (2) 3. A density treatment from Brown and Francis (1995) based on aircraft data from midlatitude cirrus: Density treatments Constant ice hydrometeor density is often used in cloud resolving models, and is used in the released versions of RTTOV and ARTS (Section 3). However, atmospheric ice hydrometeors can be aggregates comprising ice, air and liquid in differing quantities. Generally, the density of ice hydrometeors decreases with increasing size (Heymsfield et al., 2004). To account for this, a number of expressions for density ρ as a function of particle diameter D have been developed. Three are considered here. All of the following equations are in SI units (ρ in kg m−3 , D in m). 1. The parametrization used in the Unified Model at the UK Met Office: ρ = 0.132 D −1 . 2. A parametrization based on aircraft data from stratiform precipitating mixed phase cloud (Jones, 1995): (1) ρ = 0.035 D −1.1 . 5.2. (3) Particle size distributions (PSD) As outlined in Section 3, RTTOV 8.7 uses a MarshallPalmer size distribution for snow and a modified gamma distribution for ice. For the purposes of this paper, snow and ice are treated as a single hydrometeor type with a single size distribution. A number of PSD parametrizations are investigated for use with this single ice hydrometeor type. PSDs examined include the modified gamma distribution and a new treatment developed by Field et al. (2005). This new treatment is based on aircraft data gathered over the UK and calculates the size distribution of the ice hydrometeors using the IWC and temperature within the cloud. Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. Q. J. R. Meteorol. Soc. (in press) DOI: 10.1002/qj ICE HYDROMETEOR MICROPHYSICS FOR RADIATIVE TRANSFER 6. Comparison of different ice microphysical assumptions Table I outlines the microphysical assumptions used in RTTOV for the purposes of this paper. The histogram in Figure 2 shows the frequency of each BT bin in the case study for ARTS and RTTOV simulations and for observations. ARTS and RTTOV both agree well with observations for BTs greater than ∼250 K. However, RTTOV does not agree so well with observations at lower temperatures where the scattering signal from ice hydrometeors is found. The lowest RTTOV BT is 245 K, while the observations and ARTS simulations fall as low as 220 K. BT maps for channel 20 (183 ± 7 GHz) of the output from RTTOV experiment 1 and from ARTS for the case study are shown in Figure 3. Three points can be noted from Figure 3: 1. Both RTMs reproduce the broad structure seen in the observations. The frontal system across the British Isles is clearly visible in both simulations. 2. The smaller scale features seen in the observations are not reproduced exactly by either model. This is probably due to discrepancies in the forecast fields, which may not be accurate on smaller scales and which are 32 min before the ATOVS overpass. 3. There is greater agreement in structure between the two models than compared to observations, but there Table I. RTTOV configurations. Experiment 1 2 3 4 5 6 Density Size distribution 0.1 g cm−3 0.5 g cm−3 0.5 g cm−3 8.74 × 10−4 exp (−0.625 D 2 ) +4.5 × 10−5 0.132 × D −1 0.132 × D −1 Modified Gamma Modified Gamma Field et al. (2005) Modified Gamma Modified Gamma Field et al. (2005) 800 Frequency 600 400 solid line=RTTOV dotted line=ARTS dashed line=obs 200 0 200 220 240 260 280 300 Brightness Temperature (K) Figure 2. Histogram of experiment 1: RTTOV, ARTS and observed channel 20 BTs. is a significant difference in the magnitude of the scattering signal. This difference in the model outputs may come from either the approach to radiative transfer or from the basic microphysical assumptions. We cannot comment on the agreement between the models until we know how much these assumptions affect the results of the radiative transfer. The effective radius is an input parameter to ARTS. This can be varied to effectively tune ARTS to agree closely with observations, as seen in Figure 2, or to agree closely with RTTOV, simply by using a smaller assumed effective radius. Since agreement between modelled results and observations is better at higher BTs (<5 K difference), it is likely that the problem arises from the ice microphysical assumptions in RTTOV and not from the method of solving the radiative transfer equation. Choosing a realistic size distribution and density for ice hydrometeors is difficult as these quantities differ from cloud to cloud and even within clouds (Korolev et al., 2001). The effect of the assumptions is demonstrated by the BT plots in Figure 4 which show the difference between channel 20 RTTOV BT for experiments 2 and 3 (same density but different size distribution) and between experiments 2 and 4 (same size distribution but different density). The top two panels in Figure 4 show that BT variablity due to changes in microphysical assumptions is very high. The maximum difference between experiments 2 and 3 (same density, different PSD) is of the order 20 K and for experiments 2 and 4 (same PSD different density) it is of the order 50 K. It is often larger than the signal seen from cloud itself (∼15 K for channel 20). This sensitivity to assumed microphysics was also seen by SkofronickJackson et al. (2002) in their comparison of microwave BTs in different cloud parametrizations for convective situations. In the bottom panel of Figure 4, the difference between simulated and observed BT for experiment 6 is shown. Some of the differences are due to the time offset between the AMSU-B overpass and the forecast fields used in the models (32 min). Errors in the forecast fields themselves will also generate errors in the simulated BT, no matter how well the RTM performs. Figure 5 shows a histogram of the frequency of occurrence of each BT for each of the six RTTOV experiments at the lower end of the BT range. This BT range has been magnifed as this is where the scattering signal for ice hydrometeors is seen and where the greatest differences exist between the experiments. This plot depicts how, of all the parametrizations considered here, experiment 6 matches observations most closely. There is still a discrepancy of more than 10 K at the lowest BTs, showing that this parametrization does not completely reproduce the observed ice scattering signal. At the highest BTs, experiment 6, in common with all the RTTOV experiments, overestimates the BT by about 1 K (not shown). Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. Q. J. R. Meteorol. Soc. (in press) DOI: 10.1002/qj A. M. DOHERTY ET AL. Obs Channel 20 experiment 2 – experiment 3 ARTS −21 −18 −15 −12 −9 −6 −3 0 RTTOV Channel 20 experiment 2 – experiment 4 −59 −49 −40 −30 −20 −10 0 channel 20 BT (K) 220 228 236 244 252 260 268 276 Figure 3. Observed, ARTS and RTTOV experiment 1 BT, for channel 20. Observed minus simulated BTs were calculated for each point in the case study for each experiment. The data were then sorted into nine categories defined by the ice water path (IWP) and liquid water path (LWP) as outlined in Table II. The mean and standard deviation were calculated for each bin. These are shown in Figure 6 for channels 16, 17 and 20 for bins 1, 3, 7 and 9. Figure 6 shows that, as expected, all experiments perform similarly when the IWP is below 25 g m−2 (cross and star symbols). However, the bins with IWP >500 g m−2 (triangle and diamond symbols) show Observed – Experiment 6 RTTOV BT channel 20 −26 −17 −9 0 8 16 25 Figure 4. Top panel: difference between RTTOV channel 20 simulations for experiments 2 and 3. Middle panel: difference between RTTOV channel 20 simulations for experiments 2 and 4. Bottom panel: difference between observed channel 20 BT and RTTOV simulations for experiment 6. large variations between experiments. Experiments 2 and 3, with the ice particle density of 0.5 g cm−3 show the largest difference from observations, confirming that this density is an unreasonably large assumption if applied to Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. Q. J. R. Meteorol. Soc. (in press) DOI: 10.1002/qj ICE HYDROMETEOR MICROPHYSICS FOR RADIATIVE TRANSFER comparison of ch 20 TBs 250 Frequency 200 150 100 50 0 180 RTTOV expt 1 RTTOV expt 2 RTTOV expt 3 RTTOV expt 4 RTTOV expt 5 RTTOV expt 6 Observation 200 220 240 Brightness Temperature (K) 260 Figure 5. Histogram of RTTOV channel 20 BTs for all experiments and the observations. all ice hydrometeors. Figure 6 shows that experiment 6 has comparable mean and standard deviation to experiments 1, 4 and 5. Noting evidence from Figure 5, it can be concluded that experiment 6 fits the observed behaviour most closely. 7. Figure 6. Mean and Standard Deviation of observed minus simulated BT from the case study for each of 4 IWP and LWP bins. Results are shown for channels 16, 17 and 20 for each experiment. Summary and conclusions A number of different parametrizations for the ice hydrometeor microphysics were implemented in RTTOV. The resulting simulated BTs were compared with observations and with ARTS output for a number of case studies using input fields from the Met Office Mesoscale model. The results for one of the case studies are presented in this paper. The comparisons highlight the sensitivity of the RTMs to the assumptions made about the density and size distribution of the ice hydrometeors. Of the parametrizations examined, a density of ρ = 0.132 D −1 and the Field size distribution (experiment 6) was identified as the best fit to observations across a range of measures. When comparisons of the mean and standard deviation of differences were examined, experiments 1, 4, 5 and 6 performed well and consistently. When comparisons were made in the form of histograms of BT to overcome mislocation problems, experiments 3 and 6 provided the closest approximations to observations. Given these results, experiment 6 was identified as the best of the parametrizations examined. However, none of the experiments fully captures the natural variation of BT seen in the observations. It is possible that some errors are introduced through the use of forecast model fields as input. While we have made the assumption throughout this work that a forecast model can be taken as a biasfree reference, the profiles may include errors. Both the density and PSD treatments used in experiment 6 have the benefit that they are dependent on other cloud parameters, namely temperature and IWC for the PSD and particle size for the density. This makes them more flexible and, if the relations between the known and unknown parameters are valid for the conditions in which they are used, more realistic. When using the experiment 6 parametrization, Table II. LWP and IWP bins. Bin number IWP limits LWP limits 1 2 3 4 5 6 7 8 9 <25 g m−2 <25 g m−2 <25 g m−2 25 g m−2 < IWP <500 g m−2 25 g m−2 < IWP <500 g m−2 25 g m−2 < IWP <500 g m−2 >500 g m−2 >500 g m−2 >500 g m−2 <25 g cm−2 25 g m−2 < LWP < 500 g m−2 >500 g m−2 <25 g m−2 25 g m−2 < LWP < 500 g m−2 >500 g m−2 <25 g cm−2 25 g m−2 < LWP < 500 g m−2 >500 g m−2 Crown Copyright 2007. Reproduced with the permission of Her Majesty’s Stationery Office. Published by John Wiley & Sons, Ltd. Number of points 1850 874 103 1204 1584 584 159 1478 164 Q. J. R. Meteorol. Soc. (in press) DOI: 10.1002/qj A. M. DOHERTY ET AL. no particle size is required from the forecast model: only temperature and IWC. The parametrizations presented here have been tested for case studies over the UK only. Comparisons under other meteorological conditions should be made to ensure assumptions are valid in a range of situations and climatological zones. 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