Energy distributions of the secondary and backscattered electrons from polymethylmethacrylate irradiated by an electron beam. A Monte Carlo simulation Maurizio Dapor European Centre for Theoretical Studies in Nuclear Physics and Related Areas (ECT*-FBK), Trento, Italy and Trento Institute for Fundamental Physics and Applications (TIFPA-INFN), Trento, Italy [email protected] This work describes a Monte Carlo code which takes into account the stochastic behavior of electron transport in solids and treats event-byevent all the elastic and inelastic interactions between the incident electrons and the particles of the solid target [1]. It was recently demonstrated that the choice of the optical data model strongly influences the result of the simulation [2]. Extended Mermin theory [3,4] was utilized in this work, as extended Drude theory [5] is less accurate [2]. The code is used to simulate the energy distributions of the secondary and backscattered electrons from polymethylmethacrylate (PMMA) irradiated by an electron beam. Several values of the initial kinetic energy of the incident electrons are considered, and the evolution of the shape of the spectra is investigated. The simulation of the backscattered and secondary electron spectra also allows calculating the secondary electron yield of PMMA as a function of the initial energy of the incident electrons. Results of the simulation are compared with the available experimental data. Fig. 1.- Energy loss function (ELF) of PMMA as a function of the transferred energy, for several values of the momentum transfer. Symbols correspond to the experimental optical data from [6]. Solid (dashed) lines correspond to the extended Mermin [3,4] (extended Drude [5]) description of the ELF. Notice that at the optical limit (k=0) both ELF models are identical. From Ref. [2]. Fig.2. - Mermin differential inverse inelastic mean free path (DIIMFP) of electrons in PMMA as a function of the energy loss W for selected values of the incident electron kinetic energy E in the range 10-1000 eV. From Ref. [7]. Fig 3. - Monte Carlo simulated spectra of the secondary and backscattered electrons from PMMA for 200 eV (green line), 400 eV (red line), and 600 eV (black line) primary energy. Fig 4. - Monte Carlo simulated spectra of the backscattered electrons from PMMA for 200 eV (green line), 400 eV (red line), and 600 eV (black line) primary energy. Plasmon-loss peaks are located at about 20 eV from the elastic peaks (zero-loss peaks). References Fig 5. - Monte Carlo simulated spectra of the secondary electrons from PMMA for 200 eV (green line), 400 eV (red line), and 600 eV (black line) primary energy. Fig. 6.- Monte Carlo secondary electron yield of PMMA as a function of the primary electron kinetic energy obtained from the Mermin model (solid line). Symbols correspond to experimental data [8-10]. From Ref. [2]. [1] M. Dapor, Transport of Energetic Electrons in Solids, Springer Tracts in Modern Physics (Springer, Berlin, 2014), Vol. 257 [2] M. Dapor, I. Abril, P. De Vera, R. Garcia-Molina, Eur. Phys. J. D 69, 165 (2015) [3] N. D. Mermin, Phys. Rev. B 1, 2362 (1970) [4] I. Abril, R. Garcia-Molina, C.D. Denton, J.F. PerezPerez, N.R. Arista, Phys. Rev. A 58, 357 (1998) [5] R. H. Ritchie, A. Howie, Philos. Magazine 36, 463 (1977) [6] J. J. Ritsko, L. J. Brillson, R. W. Bigelow, T. J. Fabish, J. Chem. Phys. 69, 3931 (1978) [7] M. Dapor, Frontiers in Materials 2, 27 (2015) [8] T. L. Matskevich, Fiz. Tverd. Tela Adad. Nauk. 1, 277 (1959) [9] M. Boubaya, G. Blaise, Eur. Phys. J.: Appl. Phys. 37, 79 (2007) [10] E. I. Rau, E. N. Evstafeva, and M. V. Adrianov, Phys. Solid State 50, 599 (2008)
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