Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems (ACRIDICON) Project Outline for a HALO Demo Mission DLR Oberpfaffenhofen (Atmospheric Physics, Flight Operations) FU Berlin (Space Science) HU Jerusalem (Atmospheric Physics) IFM-GEOMAR at University of Kiel (Marine Meteorology) IfT Leipzig (Physics) MPIC Mainz (Air Chemistry, Biogeochemistry, Cloud Physics & Chemistry) MPIM Hamburg (Climate Processes) University of Mainz (Atmospheric Physics/Meteorology) University of Frankfurt (Atmospheric Physics/Meteorology) University of Darmstadt (Electron Microscopy) University of Bonn (Meteorology) University of Heidelberg (Environmental Physics) University of München (Meteorology) ACRIDICON Motivation General scientific questions to be addressed by ACRIDICON: 1) Does interaction of aerosols with clouds and precipitation influence the formation & dynamics of convective cloud systems and influence the vigor of heavy weather events? 2) What are the effects of convective cloud systems on the solar & terrestrial radiation budget and how important is the micro structure of the clouds? 3) Can these effects induce substantial changes in the global circulation of the atmosphere, the Earth’s energy budget, and climate? ACRIDICON Objectives Specific scientific questions to be answered by ACRIDICON: 1) Can we achieve comprehensive in-situ characterization of the microphysical & chemical properties of aerosol, cloud, and precipitation particles in convective cloud systems with the deployed scientific instrumentation? 2) Do the deployed aircraft remote sensing instruments (radar & lidar) allow to determine reliable microphysical profiles of convective clouds? 3) What are characteristic particle properties in the convective cloud inflow, updraft, and outflow, and how do they change in the course of cloud evolution? 4) Can we observe characteristic differences in the microphysical properties, dynamics, and radiative effects of convective cloud systems in polluted & unpolluted air? ACRIDICON Measurement Region & Time ¾ Measurements region, where intense convective activity can be expected and where clean background air is polluted by regional sources. ¾ Example: Iberian Peninsula, which can be easily reached by HALO. Alternative or complementary locations: Western Europe (France, British Isles) and around the Alps. ¾ Flights probing the interior of convective clouds as well as their inflow and outflow regions should be conducted in clean and polluted air masses. ¾ The mission would be scheduled for summer (maximum convection), but the planned experiments should also be feasible in late spring/early fall. ACRIDICON Flight Pattern ¾ For vertical documentation of the microphysical evolution of the convective clouds, flights shall start by probing the aerosols below cloud base, and then ascend through the young cloud in the growing stages of the convective cloud, to the level of the anvil. ¾ The penetrations should be such that ambient air and aerosols will be sampled as well, including air detrained from the cloud. ¾ The vertical cross section should take an hour. Several profiles shall be taken with similar thermodynamic conditions but contrasting aerosol content. ACRIDICON Aircraft Measurements ¾ In-situ characterization & remote sensing of aerosol, cloud, and precipitation particle properties, cloud dynamics, and radiative properties shall be accompanied by trace gas measurements to identify the extent and sources of air pollution influencing the investigated convective cloud systems. ¾ We distinguish between core aircraft instrumentation & measurement parameters which appear to be most important for achievement of the aims, and of optional instruments & parameters which would be desirable but less important (subsequent Tables). ACRIDICON Core Instrumentation 1 Measurement Parameters Instruments/Packages Volume (Racks) Operating Partners updraft velocity, turbulence & precipitation intensity 3-D wind sensors, p, T, RH, weather radar, drop sondes 2 DLR aerosol & cloud residual number concentration, size distribution, volatility, absorption coefficient aerosol inlets & counterflow virtual impactor 1-2 (CVI); condensation & optical particle counters (CPC, OPC, PSAP), thermodenuder, filter collection, Lyman-α hygrometer, dewpoint mirror IfT aerosol & cloud particle number concentration, size distribution, shape, phase, chemical composition condensation & optical particle counters (COPAS, CIP, FSSP, CIP), aerosol mass spectrometer (Q/TOF-AMS, SPLAT), holographic system (HALOHOLO) 2-3 MPIC-C, Uni Mainz aerosol particle number concentration, size distribution, volatility, absorption coefficient optical particle counters (OPC, PCASP, FSSP); multi-channel condensation particle counters (CPC); thermal denuder; mobility analyzer (DMA); multi-angle absorption photometer (MAAP) 1 DLR cloud condensation nuclei concentration, aerosol absorption & scattering coefficients cloud condensation nuclei counter (CCNC), optical analyzers (SP2, PAS, nephelometer); particle collectors (filter/impactor) 1 MPIC-B ACRIDICON Core Instrumentation 2 Measurement Parameters Instruments/Packages Volume (Racks) Operating Partners ice nuclei concentration ice nuclei counter (INC) 1 Uni Frankfurt CO, O3 optical spectrometer 0-1 DLR, MPIC-A liquid water path microwave radiometer 1 Uni München cloud base and density cloud radar 1 MPIM aerosol particle vertical distribution, cloud top height cloud lidar (POLIS) 1 Uni München irradiance, radiance, actinic flux densities spectral radiometer, imaging spectrometer (polarization) 1-2 IfT ACRIDICON Optional Instrumentation Measurement Parameters Instruments/Packages Volume (Racks) Operating Partners vertical distribution of aerosol particles, water vapor, and optically thin clouds cloud lidar 6 DLR NO, NOy, O3 chemiluminescence, UV absorption 1 DLR NO, NOx, O3 chemiluminescence 1 MPIC-A CO, CO2, HCHO, H2O2 optical spectrometer 0-1 MPIC-A carbon monoxide, volatile organic compounds (VOC) mass spectrometry (PTR-MS) 1 MPIC-A O3, NO2, BrO, HCHO, IO, OIO, OClO, H2O vapour, O2, O4, UV/vis/near IR skylight radiances DOAS 0-1 Uni Heidelberg ACRIDICON Complementary Activities ¾ Satellite remote sensing: aerosol optical depth, Angstrom coefficient, particle size & type (sulfates, dust, smoke, sea salt); cloud & precipitation effective radii, phase, optical depth, liquid water path; trace gas distributions for CO, CH4, O3, NOx, etc. (FU Berlin, HU Jerusalem, IFM-GEOMAR, Uni Heidelberg) ¾ Ground-based remote sensing: evolution of the various types of hydrometeors in the clouds investigated by the aircraft (conventional and polarimetric radars, DLR). ¾ Off-line particle analysis: aerosol and cloud residual particle composition & structure (electron, atomic force, and optical microscopy; laser desorption ionization and secondary ion and mass spectrometry; biochemical assays; evolved gas analysis; Uni Frankfurt, Uni Darmstadt, MPIC-B). ¾ Data assimilation and numerical simulations: convective cloud properties, processes, and effects at a hierarchy of scales, from the individual particle through the individual cloud scale, the regional scale to the global circulation and climate scales (HU Jerusalem, IFM-GEOMAR). ACRIDICON Status ¾ Many instruments for ACRIDICON are already operational and has been applied successfully on the Falcon and other research aircrafts. ¾ Several new and improved instruments are currently under development. ¾ Depending on the progress of these developments, the actual volume of individual instruments and instrumentation packages may still undergo some change.
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