Operator Generic Fundamentals Nuclear Physics - Fission © Copyright 2017 – Rev 3 Operator Generic Fundamentals 2 Terminal Learning Objectives At the completion of this training session, the trainee will demonstrate mastery of this topic by passing a written exam with a grade of 80 percent or higher on the following Terminal Learning Objectives (TLOs): 1. Describe neutron interactions with matter. 2. Describe the process of nuclear fission and the types of material that can undergo fission. 3. Explain the production of heat from fission. 4. Describe intrinsic and installed neutron sources and their contribution to source neutron strength over core life. 5. Explain the relationship between neutron flux, microscopic and macroscopic cross-sections, and their effect on neutron reaction rates. © Copyright 2017 – Rev 3 TLOs Operator Generic Fundamentals 3 Neutron Interactions TLO 1 – Describe neutron interactions with matter. 1.1 Describe the following neutron scattering interactions, including conservation principles: a. Elastic scattering b. Inelastic scattering 1.2 Describe the following reactions where a neutron is absorbed in a nucleus: a. Radiative capture b. Particle ejection c. Fission © Copyright 2017 – Rev 3 TLO 1 Operator Generic Fundamentals 4 Neutron Scattering Interactions ELO 1.1 – Describe the following neutron scattering interactions, including conservation principles: elastic scattering and inelastic scattering. • A neutron scattering reaction occurs when a nucleus, after having been struck by a neutron, emits a single neutron – In some cases the initial and final neutrons are not the same – Free neutron "bounced off," or scattered • Two categories of scattering reactions – Elastic – Inelastic • Important for thermal or low energy neutron availability © Copyright 2017 – Rev 3 ELO 1.1 Operator Generic Fundamentals 5 Elastic Scattering Figure: Elastic Scattering © Copyright 2017 – Rev 3 ELO 1.1 Operator Generic Fundamentals 6 Elastic Scattering • Conservation of momentum (𝑚𝑣) 𝑚𝑛 𝑣𝑛,𝑖 + 𝑚 𝑇 𝑣𝑇,𝑖 = 𝑚𝑛 𝑣𝑛,𝑓 + 𝑚 𝑇 𝑣𝑇,𝑓 • Conservation of kinetic energy 1 2 𝑚𝑛 𝑣𝑛,𝑖 2 + 1 2 𝑚 𝑇 𝑣𝑇,𝑖 2 = 1 𝑚𝑣 2 2 1 2 𝑚𝑛 𝑣𝑛,𝑓 2 + 1 2 𝑚 𝑇 𝑣𝑇,𝑓 2 ) • Where: 𝑚𝑛 = mass of the neutron 𝑚 𝑇 = mass of the target nucleus 𝑣𝑛,𝑖 = initial neutron velocity 𝑣𝑛,𝑓 = final neutron velocity 𝑣𝑇,𝑖 = initial target velocity 𝑣𝑇,𝑓 = final target velocity © Copyright 2017 – Rev 3 ELO 1.1 Operator Generic Fundamentals 7 Inelastic Scattering • Some KE transferred to target nucleus as excitation energy • Total KE outgoing neutron and nucleus is less than KE of incoming neutron Figure: Inelastic Scattering © Copyright 2017 – Rev 3 ELO 1.1 Operator Generic Fundamentals 8 Neutron Scattering Interactions Knowledge Check The difference between elastic and inelastic scattering where neutrons are concerned is elastic scattering involves no energy being transferred into excitation energy of the target nucleus. Inelastic scattering involves a transfer of kinetic energy into excitation energy of the target nucleus. A. True B. False Correct answer is A. © Copyright 2017 – Rev 3 ELO 1.1 Operator Generic Fundamentals 9 Neutron Absorption Reactions ELO 1.2 - Describe the following reactions where a neutron is absorbed in a nucleus: Radiative capture, Particle ejection, Fission. • Most absorption reactions result in: – The loss of a neutron – The production of charged particles – Gamma ray(s) – Fission fragments – The release of neutrons and energy • Three types of absorption reactions: radiative capture, particle ejection, and fission © Copyright 2017 – Rev 3 ELO 1.3 Operator Generic Fundamentals 10 Radiative Capture • Incident neutron interacts with the target nucleus forming a compound nucleus • Compound nucleus, with the neutron added - decays to its ground state via gamma emission 1 238 239 ∗ 239 0 𝑛+ 𝑈→ 𝑈 → 𝑈+ 𝛾 0 92 92 92 0 * Represents an excited nucleus © Copyright 2017 – Rev 3 ELO 1.3 Operator Generic Fundamentals 11 Particle Ejection • A compound nucleus is formed when the incident neutron interacts with the target nucleus • New compound nucleus, is excited to a high enough energy level for it to: – Eject a new particle with the incident neutron remaining in the nucleus – Ejected particles can be alpha particles, protons, etc • After the new particle is ejected, the nucleus may or may not exist in an excited state depending upon the mass-energy balance of the reaction 1 10 11 𝑛+ 𝐵→ 𝐵 0 5 5 © Copyright 2017 – Rev 3 ∗ 7 4 → 𝐿𝑖 + 𝛼 3 2 ELO 1.3 Operator Generic Fundamentals 12 Fission • The nucleus absorbs the incident neutron resulting in nucleus splitting into two smaller nuclei, called fission fragments • Fission reaction typically produces – Two fission fragments – 2 to 3 neutrons – Considerable amount of energy (e.g. kinetic and gamma rays) 1 236 ∗ 140 93 1 235 𝑛+ 𝑈→ 𝑈 → 𝐶𝑠 + 𝑅𝑏 + 3 𝑛 0 92 55 37 0 92 © Copyright 2017 – Rev 3 ELO 1.3 Operator Generic Fundamentals 13 Neutron Absorption Reactions Knowledge Check What type of neutron interaction has occurred when a nucleus absorbs a neutron and ejects proton? A. Fission B. Fusion C. Particle ejection D. Radiative capture Correct answer is C. © Copyright 2017 – Rev 3 ELO 1.3 Operator Generic Fundamentals 14 Neutron Fission TLO 2 – Describe the process of nuclear fission and the types of material which can undergo fission. 2.1 Define the following terms: a. Excitation energy (Eexc) b. Critical energy (Ecrit) 2.2 Explain the fission process using the liquid drop model of a nucleus. 2.3 Define the following terms: a. Fissile material b. Fissionable material c. Fertile material d. Thermal neutrons 2.4 Explain binding energy per nucleon 2.5 Explain the shape of the binding energy per nucleon versus mass number curve including its significance to fission energy. © Copyright 2017 – Rev 3 TLO 2 Operator Generic Fundamentals 15 Excitation Energy ELO 2.1 – Define the following terms: Excitation energy (Eexc), Critical energy (Ecrit). Excitation Energy • The measure of how far the energy level of a nucleus is above its ground state is called the excitation energy (Eexc) Critical Energy • The minimum excitation energy for a specific nuclide to fission © Copyright 2017 – Rev 3 ELO 2.1 Operator Generic Fundamentals 16 Critical Energy • Many neutron reactions can cause an increase in the excitation energy of a nucleus • When an incident neutron strikes a target nucleus, the reaction excites the target nucleus by an amount equal to the sum of – Binding energy of the neutron – The neutron’s kinetic energy (KE) • If the binding energy is less than the required critical energy for the nucleus – Additional energy is required to cause the nucleus to fission – Could be in the form of KE from the incident neutron • Neutrons of low KE cannot cause fission with some types of isotopes used in nuclear reactor fuels © Copyright 2017 – Rev 3 ELO 2.1 Operator Generic Fundamentals 17 Excitation Energy Knowledge Check Excitation must be at least equal to critical energy for fission to occur. A. True B. False Correct answer is A. © Copyright 2017 – Rev 3 ELO 2.1 Operator Generic Fundamentals 18 Fission Process ELO 2.2 - Explain the fission process using the liquid drop model of a nucleus. • In a fission reaction the incident neutron is absorbed in the heavy target nucleus • Creates a compound nucleus that is excited at a high-energy level (Eexc > Ecrit) • Nucleus "splits" (fissions) into two large fragments plus some neutrons • In addition a large amount of energy is released in the form of fragment kinetic energy and radiation © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 19 Fission Process • The nucleus is held together by the attractive nuclear force between nucleons – Resists the opposing electrostatic forces within the nucleus • Characteristics of the nuclear force are: – Very short range attractive force, with essentially no strength beyond nuclear scale dimensions (≈10-13 cm) – Stronger than repulsive electrostatic forces within the nucleus – Independent of nucleon pairing – Saturable – a nucleon can attract only a few of its nearest neighbors © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 20 Fission Process • One theory considers fission similar to the splitting of a liquid drop – Liquid drop is held together by molecular forces that tend to make the drop spherical in shape and resist deformation in the same manner as nuclear forces are thought to hold the nucleus together – By considering the nucleus as a liquid drop the fission process is better understood and visualized © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 21 Fission Process • The undisturbed nucleus in the ground state is undistorted Figure: Liquid Drop Model © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 22 Fission Process • When the incident neutron strikes the target nucleus and is absorbed an excited a compound nucleus is formed Figure: Liquid Drop Model © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 23 Fission Process • If the excitation energy is greater than the critical energy – oscillations may cause the compound nucleus to become dumbbell-shaped as it starts to come apart Figure: Liquid Drop Model © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 24 Fission Process • When the repulsive electrostatic forces exceed the attractive nuclear forces, nuclear fission occurs Figure: Liquid Drop Model © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 25 Fission Process Knowledge Check In the Liquid Drop Model of fission, the nucleus absorbs a neutron, becomes distorted into a “dumbbell” shape and splits into two nuclei. Which of the following forces is responsible for the nucleus splitting? A. Liquid drop force B. Gravitational force C. Electrostatic force D. Fission force Correct answer is C. © Copyright 2017 – Rev 3 ELO 2.2 Operator Generic Fundamentals 26 Fission Process ELO 2.3 - Define the following terms: Fissile material, Fissionable material, Fertile material, Thermal neutrons. Fissile Material • Fissile materials are nuclides for which fission is possible with neutrons of any energy level – Desired thermal reactors – Can fission with thermal neutrons – Change in binding energy (BE) from neutron alone is sufficient to exceed the critical energy • Thermal neutrons – very low KE levels, add essentially no KE to the reaction • Examples: – Uranium-235 – Uranium-233 – Plutonium-239 © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 27 Fissionable Material Fissionable Material • Nuclides for which fission is possible – All fissile nuclides fall into this category – And nuclides that fission only from high-energy neutrons • Change in binding energy causes excitation energy level insufficient to reach critical energy for fission • Examples (requiring high-energy neutrons): – Thorium-232 – Uranium-238 – Plutonium-240 © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 28 Fissionable Material Critical Energies Compared to Binding Energy (BE) of Last Neutron Target Nucleus Critical Energy Ecrit Binding Energy of Last Neutron BEn BEn - Ecrit 232 90Th 7.5 MeV 5.4 MeV -2.1 MeV 238 92U 7.0 MeV 5.5MeV -1.5 MeV 235 92U 6.5 MeV 6.8 MeV +0.3 MeV 233 92U 6.0 MeV 7.0 MeV +1.0 MeV 234 94Pu 5.0 MeV 6.6 MeV +1.6 MeV © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 29 Fertile Materials • Transmutation – all of the neutron absorption reactions that do not result in fission lead to the production of new nuclides • Nuclides can – Be transmuted again – Undergo radioactive decay to produce nuclides known as transmutation products • Some fissile nuclides do not exist in nature, only produced by nuclear reactions (transmutation) • Fertile materials are materials (nuclides) that can undergo transmutation to become fissile materials © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 30 Fertile Materials Figure: Transmutation Mechanisms © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 31 Thermal Neutrons • Thermal neutrons are neutrons with very low KE levels • Basically in equilibrium with the thermal energy of surrounding materials • Undergo scattering collisions where they are gaining and losing equal amounts of energy in successive collisions • Add essentially no KE to a neutron absorption reaction • In a commercial PWR, as a thermal reactor, the goal is to thermalize as many neutrons as possible © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 32 Thermal Neutrons • Thermal neutrons are standardized in table format for cross-section data at 68°F (20°C). • At 68°F, thermal neutron – Energy is 0.025 eV – Velocity of 2.2 X 105 cm/sec 𝐸𝑝 = 0.025 𝑒𝑉 𝑇 𝑇𝑜 1 2 𝑉𝑝 = 2.2 × 105 𝑐𝑚 𝑠𝑒𝑐 𝑇 𝑇𝑜 1 2 • Where: 𝐸𝑝 = Most probable energy (eV) 𝑉𝑝 = Most probable velocity (cm/sec) 𝑇𝑜 = Table temp 68°F (528°R) 𝑇 = New temperature in °R (°F + 460°) © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 33 Fission Process Knowledge Check What is the difference between a fissionable material and a fissile material? A. There is no difference between a fissionable and a fissile material, except for the number of protons and neutrons located in the nuclei of the particular materials. B. A fissionable material can become fissile by capturing a neutron with zero kinetic energy, whereas a fissile material can become fissionable by absorbing a neutron that has some kinetic energy. C. Fissile materials require a neutron with some kinetic energy in order to fission, whereas fissionable materials will fission with a neutron that has zero kinetic energy. D. Fissionable materials require a neutron with some kinetic energy in order to fission, whereas fissile materials will fission with a neutron that has zero kinetic energy. Correct answer is D. © Copyright 2017 – Rev 3 ELO 2.3 Operator Generic Fundamentals 34 Binding Energy per Nucleon ELO 2.4 - Explain binding energy per nucleon. • Binding energy per nucleon (BE/A) equals the average energy required to remove a nucleon from a specific nucleus • This is important from the standpoint of a thermal neutron’s ability to cause a fission © Copyright 2017 – Rev 3 ELO 2.4 Operator Generic Fundamentals 35 Binding Energy per Nucleon • Determined by dividing the total binding energy of a nuclide by the total number of nucleons in its nucleus. Example • Given that the total binding energy (BE) for a U-238 nucleus is 𝐵𝐸 1,804.3 MeV, calculate the binding energy per nucleon ( ) for U-238. 𝐴 Solution: 𝐵𝐸 1,804.3 𝑀𝑒𝑉 = = 7.6 𝑀𝑒𝑉 𝐴 238 © Copyright 2017 – Rev 3 ELO 2.4 Operator Generic Fundamentals 36 Binding Energy per Nucleon Knowledge Check Binding energy per nucleon is independent of the specific nuclide. A. True B. False Correct answer is B. © Copyright 2017 – Rev 3 ELO 2.4 Operator Generic Fundamentals 37 Binding Energy per Nucleon Curve ELO 2.5 - Explain the shape of the binding energy per nucleon versus mass number curve including its significance to fission energy. 𝐵𝐸 • The relationship of as the mass number changes is important for 𝐴 understanding how energy is released during fission • It also explains the theory of energy release from fusion • As the number of nucleons in a nucleus increases, – Total binding energy increases – Rate of BE increase is not linear as mass number increases • Variation in the binding energy per nucleon is seen when plotted against the atomic mass numbers (A) © Copyright 2017 – Rev 3 ELO 2.5 Operator Generic Fundamentals 38 Binding Energy per Nucleon Curve Figure: Binding Energy per Nucleon versus Mass Number © Copyright 2017 – Rev 3 ELO 2.5 Operator Generic Fundamentals 39 Binding Energy per Nucleon Curve Knowledge Check Generally, less stable nuclides have a higher ones. 𝐵𝐸 𝐴 than the more stable A. True B. False Correct answer is B. © Copyright 2017 – Rev 3 ELO 2.5 Operator Generic Fundamentals 40 Neutron Fission TLO 3 – Explain the production of heat from fission. 3.1 Describe the average total amount of energy released per fission event including: a. Energy released immediately from fission b. Delayed fission energy 3.2 Describe which fission products nuclides are most likely to result from fission. 3.3 Describe the energy released from fission by the following methods: a. Change in binding energy b. Conservation of mass – energy c. Decay energy 3.4 Describe how heat is produced as a result of fission. © Copyright 2017 – Rev 3 TLO 3 Operator Generic Fundamentals 41 Energy Release Per Fission ELO 3.1 – Describe the average total amount of energy released per fission event including: energy released immediately from fission and delayed fission energy. • Total energy released per fission varies, depending on what fission products are formed – Average total energy released from U-235 fission with a thermal neutron is approximately 200 MeV • The majority of this energy (approximately 83 percent) is from the KE of the fission fragments • Specific isotope undergoing fission has a small impact on the energy released – Thermal fission of U-235 and fast fission of U-238 yield nearly identical energy © Copyright 2017 – Rev 3 ELO 3.1 Operator Generic Fundamentals 42 Energy Release Per Fission Instantaneous Energy Kinetic Energy of Fission Fragments 165 MeV Kinetic Energy of Fission Neutrons 5 MeV Instantaneous Gamma Rays 7 MeV Capture Gamma Ray Energy 10 MeV Delayed Energy Kinetic Energy of Beta Particles 7 MeV Decay Gamma Rays 6 MeV Neutrinos 10 MeV* Total Energy Released 200 MeV © Copyright 2017 – Rev 3 ELO 3.1 Operator Generic Fundamentals 43 Delayed Fission Energy (Decay Heat) • Of the 200 MeV released per fission, about seven percent (13 MeV) is released sometime after the instant of fission • Decay heat – energy released from the decay of fission products after the reactor is shut down and fissions mostly cease – Represents about seven percent of reactor heat production during reactor operation – Once the reactor is shutdown decay heat production “decays” off but remains a significant source of heat for a very long time © Copyright 2017 – Rev 3 ELO 3.1 Operator Generic Fundamentals 44 Energy Release Per Fission Knowledge Check Which of the following statements correctly describes the amount of energy released from a single fission event? A. Approximately 200 MeV are released during fission. 13 MeV are released instantaneously, and 187 MeV are released later (delayed). B. Approximately 200 MeV are released during fission. 187 MeV are released instantaneously, and 13 MeV are released later (delayed). C. Approximately 200 eV are released during fission. 13 eV are released instantaneously, and 187 eV are released later (delayed). D. Approximately 200 eV are released during fission. 187 eV are released instantaneously, and 13 eV are released later (delayed). Correct answer is B. © Copyright 2017 – Rev 3 ELO 3.1 Operator Generic Fundamentals 45 Fission Fragment Yield ELO 3.2 - Describe which fission product nuclides are most likely to result from fission. • Fissions do not produce identical results on each occurrence – Both the number of neutrons and the resultant fission fragments vary • Scientific experiments have developed a yield curve of fission product probabilities © Copyright 2017 – Rev 3 ELO 3.2 Operator Generic Fundamentals 46 Most Probable Fission Fragments • Resultant fission fragments have masses that vary widely • Most probable pair of fission fragments for a thermal neutron fission of uranium-235 have masses of about 95 and 140 • Cesium-140 and rubidium-93 are very likely to result from fission • An example of one fission fragment yield is: 236 ∗ 235 𝑈+𝑛 → 𝑈 140 94 → 𝑋𝑒 + 𝑆𝑟 + 2𝑛 • 2 neutrons result from this fission © Copyright 2017 – Rev 3 ELO 3.2 Figure: Uranium-235 Fission Yield for Fast and Thermal Neutrons versus Mass Number Operator Generic Fundamentals 47 Most Probable Fission Fragments Isotope Average Neutrons released per fission (v) U-233 2.492 U-235 2.418 Pu-239 2.871 Pu-241 2.927 © Copyright 2017 – Rev 3 ELO 3.2 Operator Generic Fundamentals 48 Fission Fragment Yield Knowledge Check List the two most likely fission fragments resulting from fission of uranium-235. Correct answer is cesium and rubidium. © Copyright 2017 – Rev 3 ELO 3.2 Operator Generic Fundamentals 49 Energy Release Calculation ELO 3.3 - Describe the energy released from fission by the following methods: change in binding energy, conservation of mass – energy, and decay energy. • Nuclear fission releases enormous quantities of energy • Amount of energy release can be calculated • Consider a typical fission reaction: 1 236 235 𝑛+ 𝑈→ 𝑈 0 92 92 © Copyright 2017 – Rev 3 ∗ → 140 93 1 𝐶𝑠 + 𝑅𝑏 + 3 𝑛 55 37 0 ELO 3.3 Operator Generic Fundamentals 50 Change in Binding Energy Method 𝐵𝐸 • Use curve to determine the 𝐴 amount of energy released by a fission • An increase in total BE indicates greater stability by the release of the equivalent energy • In a fission process, the energy liberated is equal to the increase in the total BE of the system ∗ 1 236 235 𝑛+ 𝑈→ 𝑈 0 92 92 140 93 1 → 𝐶𝑠 + 𝑅𝑏 + 3 𝑛 55 37 0 © Copyright 2017 – Rev 3 ELO 3.3 Figure: Change in Binding Energy for Typical Fission Operator Generic Fundamentals 51 Change in Binding Energy Demonstration • Total BE for a nucleus is found by multiplying the BE/A by the number of nucleons ∆𝐵𝐸 = 𝐵𝐸𝑝𝑟𝑜𝑑𝑢𝑐𝑡𝑠 − 𝐵𝐸𝑟𝑒𝑎𝑐𝑡𝑎𝑛𝑡𝑠 = 𝐵𝐸𝑅𝑏−93 + 𝐵𝐸𝐶𝑠−140 − 𝐵𝐸𝑈−235 = 809 𝑀𝑒𝑉 + 1,176 𝑀𝑒𝑉 − 1,786 𝑀𝑒𝑉 = 199 𝑀𝑒𝑉 Nuclide BE per Nucleon (BE/A) Mass Number (A) Binding Energy (BE/A) x (A) 93 37Rb 8.7 MeV 93 809 MeV 140 55Cs 8.4 MeV 140 1,176 MeV 235 92U 7.6 MeV 235 1,786 MeV © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 52 Conservation of Mass-Energy Method • During fission a decrease in the system mass occurs equal to the energy liberated • This calculation method is more accurate than the change in BE method since it considers all mass changes – EInst, the instantaneous energy, is the energy released immediately after the fission process • This calculation includes: 1. Adding the nucleon masses of the fuel isotope including the incident neutron mass (reactants) 2. Adding the nucleon masses of the fission products and released neutrons (products) 3. Subtracting the mass of the products from the reactants 4. Multiple the mass calculated by 931.5 MeV to convert to energy © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 53 Conservation of Mass-Energy Demonstration Mass of the Reactants 235 𝑈 235.043924 amu 92 1 1.008665 amu 𝑛 0 Mass of the Products 93 92.91699 amu 𝑅𝑏 37 140 𝐶𝑠 139.90910 amu 55 1 3.02599 amu 3 𝑛 0 235.85208 amu Totals 236.052589 amu Mass Difference Energy Equivalent = 𝑀𝑎𝑠𝑠 𝑜𝑓 𝑡ℎ𝑒 𝑅𝑒𝑎𝑐𝑡𝑎𝑛𝑡𝑠 − 𝑀𝑎𝑠𝑠 𝑜𝑓 𝑡ℎ𝑒 𝑃𝑟𝑜𝑑𝑢𝑐𝑡𝑠 = 236.052589 𝑎𝑚𝑢 − 235.85208 𝑎𝑚𝑢 = 0.200509 𝑎𝑚𝑢 = 𝑀𝑎𝑠𝑠 × 931.5 𝑀𝑒𝑉/𝑎𝑚𝑢 = 0.200509 𝑎𝑚𝑢 × 931.5 𝑀𝑒𝑉/𝑎𝑚𝑢 = 186.8 𝑀𝑒𝑉 © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 54 Estimation of Decay Energy Decay energy • Additional energy released when the fission fragments decay by βemission • Added to the instantaneous energy release, • EDecay 𝛽− 𝛽− 𝛽− 𝛽− 93 93 93 93 93 𝑅𝑏 → 𝑆𝑟 → 𝑌 → 𝑍𝑟 → 𝑁𝑏 37 38 39 40 41 𝛽− 𝛽− 𝛽− 140 140 140 140 𝐶𝑠 → 𝐵𝑎 → 𝐿𝑎 → 𝐶𝑒 55 56 57 58 © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 55 Estimation of Decay Energy • The energy released during the decay for each chain is equivalent to: – The mass difference between the original fission product, and – The sum of the final stable nuclide and emitted beta particles • The total decay energy is the sum of both chains © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 56 Estimation of Decay Energy Demonstration • The energy released in the decay chain of rubidium-93 is: 𝐸𝐷𝑒𝑐𝑎𝑦 = 𝑚𝑅𝑏−93 − 𝑚𝑁𝑏−93 + 4 𝑚𝑒𝑙𝑒𝑐𝑡𝑟𝑜𝑛 931.5 𝑀𝑒𝑉 𝑎𝑚𝑢 = 92.91699 𝑎𝑚𝑢 − 92.90638 𝑎𝑚𝑢 + 4 0.0005486 𝑎𝑚𝑢 = 0.008416 𝑎𝑚𝑢 931.5 𝑀𝑒𝑉 𝑎𝑚𝑢 931.5 𝑀𝑒𝑉 𝑎𝑚𝑢 = 7.84 𝑀𝑒𝑉 © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 57 Estimation of Decay Energy Demonstration • The energy released in the decay chain of cesium-140 is: 𝐸𝐷𝑒𝑐𝑎𝑦 = 𝑚𝐶𝑠−140 − 𝑚𝐶𝑒−140 + 3 𝑚𝑒𝑙𝑒𝑐𝑡𝑟𝑜𝑛 931.5 𝑀𝑒𝑉 𝑎𝑚𝑢 = 139.90910 𝑎𝑚𝑢 − 139.90543 𝑎𝑚𝑢 + 3 0.0005486 𝑎𝑚𝑢 = 0.000202 𝑎𝑚𝑢 931.5 𝑀𝑒𝑉 𝑎𝑚𝑢 931.5 𝑀𝑒𝑉 𝑎𝑚𝑢 = 1.89 𝑀𝑒𝑉 • The total decay energy is the sum of the energies of the two chains, or 9.73 MeV © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 58 Energy Release Calculation Knowledge Check The change in binding energy per nucleon between the fissile nuclide and the fission products, is used to calculate _________. A. fission fragment speed B. decay heat C. energy released by fission D. increase in mass Correct answer is C. © Copyright 2017 – Rev 3 ELO 3.3 Operator Generic Fundamentals 59 Fission Heat Production ELO 3.4 – Describe how heat is produced as a result of fission. • Majority of the energy liberated in the fission process is released immediately after the fission occurs • This energy appears as – KE of the fission fragments and neutrons – Instantaneous gamma rays • Remaining energy is released over a period of time after the fission occurs and appears as KE of the decay products – Beta – Decay gammas © Copyright 2017 – Rev 3 ELO 3.4 Operator Generic Fundamentals 60 Fission Heat Production • All of the energy released in fission, with the exception of the neutrino energy, is transformed into heat • Fission fragments, with a positive charge and KE, cause ionization directly as they rip orbital electrons from the surrounding atoms – Provides biggest increase in fuel temperature • Beta particles and gamma rays also give up energy also through ionization • Fission neutrons interact and lose their energy through scattering – Primarily elastic scattering © Copyright 2017 – Rev 3 ELO 3.4 Operator Generic Fundamentals 61 Fission Heat Production Knowledge Check Which of the following is NOT a method by which heat is produced from fission? A. Fission fragments causing direct ionizations resulting in an increase in temperature. B. Beta particles and gamma rays causing ionizations resulting in increased temperature. C. Neutrons interacting and losing their energy through scattering, resulting in increased temperature. D. Neutrinos interacting and losing their energy through scattering and ionizations resulting in increased temperatures. Correct answer is D. © Copyright 2017 – Rev 3 ELO 3.4 Operator Generic Fundamentals 62 Neutron Fission TLO 4 – Describe intrinsic and installed neutron sources and their contribution to source neutron strength over core life. 4.1 Describe the purpose and importance of source neutrons. 4.2 Describe, including examples, of each of the following types of intrinsic neutron sources: a. Spontaneous fission b. Photo-neutron reactions c. Alpha-neutron reactions d. Transuranic elements 4.3 Describe the purpose and type of installed neutron sources. 4.4 Describe the primary source of intrinsic source neutrons in the reactor for the following conditions: a. At beginning and end of core life: b. Immediately following a reactor shutdown c. Several weeks after reactor shutdown © Copyright 2017 – Rev 3 TLO 4 Operator Generic Fundamentals 63 Source Neutrons Introduction ELO 4.1 – Describe the purpose and importance of source neutrons. • Sources neutrons – Non-fission produced neutrons • Help monitor the fission process during reactor startup • Ensure neutron population during shutdown conditions remains high enough for indication on source range nuclear instrumentation • Important during reactor shutdown and startup conditions: – To confirm instrument operability – Monitoring of the reactor’s neutron population changes – Subcritical multiplication • Source neutron sources are classified as either – Intrinsic – Installed neutron sources © Copyright 2017 – Rev 3 ELO 4.1 Operator Generic Fundamentals 64 Source Neutrons Knowledge Check Source neutrons are important because they: A. Extend the neutron lifetime allowing for a nuclear chain reaction to occur. B. Allow for visible indication of neutron level in a shutdown nuclear reactor. C. Shorten the neutron generation time allowing for operational control of a nuclear reactor. D. Contribute a larger percentage of the thermal neutron population than the fast neutron population in an operating nuclear reactor. Correct answer is B. © Copyright 2017 – Rev 3 ELO 4.1 Operator Generic Fundamentals 65 Intrinsic Neutron Sources ELO 4.2 - Describe, the following types of intrinsic neutron sources: spontaneous fission, photo-neutron reactions, alpha-neutron reactions, and transuranic elements. • Intrinsic neutron sources are neutron-producing reactions that occur in reactor core fuel related materials • The following types of neutron reactions are capable of producing source neutrons and transuranic contributions – Spontaneous fission – Photo-neutron reactions – Alpha-neutron reactions © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 66 Intrinsic Neutron Sources • A limited number of neutrons will be present, even in a reactor core that has never been operated • Due to spontaneous fission of some heavy nuclides present in the fuel. Examples: – Uranium-238 – Uranium-235 – Plutonium-239 • Later in core life the transuranic elements provide more spontaneous fission neutrons © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 67 Intrinsic Neutron Sources In a reactor that has been operated at power, source neutrons come from: • Photo-neutron reactions provide a significant source – Interaction of a gamma ray and a deuterium nucleus • Interactions between alpha particles and various isotopes in the reactor • Alpha particles from the decay of heavy nuclides, interacts with oxygen-18 and boron-11 in the core • Transuranic elements building in the core © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 68 Spontaneous Fission • The four isotopes that contribute most to the source neutron population via spontaneous fission are: – Uranium-235 – Uranium-238 – Curium-242 – Curium-244 • Uranium-235 and 238 from the core fuel load contribute approximately 1 x 106 neutrons per second (n/sec) to the source neutron population • Curium (a transuranic element) isotopes produced during reactor power operation are also a source of neutrons via spontaneous fission © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 69 Spontaneous Fission • Prior to a new core reactor startup, uranium spontaneous sources are significant contributors to the source neutron population • From startup to ≈ 20,000 MWD/MTU of core irradiation – curium-242 becomes a major producer of source neutrons from spontaneous fission • Beyond 20,000 MWD/MTU – curium-244 becomes a more predominant source neutron producer from spontaneous fission • As an example, one ton of spent nuclear fuel will contain on the order of 20 grams of curium © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 70 Photo-Neutron Reactions • In a reactor that has been operated at power, source neutrons from photo-neutron reactions become significant 1 2 1 𝛾+ 𝐻→ 𝐻+ 𝑛 1 1 0 • Referred to as a photo-neutron reaction because it is initiated by electromagnetic (gamma photon) radiation and results in the production of a neutron © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 71 Photo-Neutron Reactions • After the reactor has operated for a short time there is an abundant supply of high-energy gammas (2.22 MeV or greater) – Moderator/coolant has some deuterium present because the naturally occurring atom percentage of deuterium is 0.015 percent • This is sufficient deuterium for production of photo-neutrons following power operation • Quantity of gamma rays decreases with time after shutdown as gamma ray emitters decay off – Photo-neutron production rate decreases with reactor shutdown time © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 72 Alpha-Neutron Reactions • Alpha particles occur from the decay of heavy elements in the fuel • They interact with naturally occurring oxygen-18 and boron-11 • Transuranic elements produced during power operation also provide source neutrons via alpha-neutron reaction © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 73 Alpha-Neutron Reactions – Oxygen 18 This reaction does not contribute significantly to the source neutron population because • Uranium does not produce many alpha particles • Abundance of oxygen-18 in the reactor core is low 18 21 1 4 𝐻𝑒 + 𝑂 → 𝑁𝑒 + 𝑛 2 8 10 0 Nuclide © Copyright 2017 – Rev 3 t½ (Fission) t½ (α-decay) 235 92U 1.8 x 1017 years 6.8 x 108 years 238 92U 8.0 x 1015 years 4.5 x 109 years 239 94Pu 5.5 x 105 years 2.4 x 104 years 240 94Pu 1.2 x 1011 years 6.6 x 103 years ELO 4.2 Operator Generic Fundamentals 74 Alpha-Neutron Reactions – Boron 11 • Soluble boron is added to the reactor coolant system • Soluble boron contains boron-11 (80.1 percent of natural boron) • Boron 11 and alpha particles from heavy elements decay react to produce source neutrons 11 1 4 14 𝐻𝑒 + 𝐵 → 𝑁 + 𝑛 2 5 7 0 • The boron-11 must be in very close proximity to the fuel for this reaction because of the short travel path length of alpha particles © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 75 Alpha-Neutron Reactions – Transuranic Elements • Neutrons (transuranic) are produced from either spontaneous fission or alpha-neutron reactions • Curium and americium isotopes are the major transuranic elements of interest for source neutrons • Curium-242 production and neutron: 239 242 1 4 𝑃𝑢 + 𝐻𝑒 → 𝐶𝑚 + 𝑛 94 2 96 0 • Alpha production (163 day half-life): 242 238 4 𝐶𝑚 → 𝑃𝑢 + 𝐻𝑒 96 94 2 • In typical nuclear reactor core, transuranic neutron sources produce – About 100 neutrons per second for every gram of fuel in the core – Approximately 1 x 107 neutrons per second core wide © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 76 Alpha-Neutron Reactions – Transuranic Elements • One gram of curium-244 produces about – 5 x 105 neutrons per second due to alpha-neutron reactions – 1.2 x 107 neutrons per second due to spontaneous fission • One gram of curium-242 produces about – 2.5 x 107 neutrons per second from alpha-neutron reactions – 2.3 x 107 neutrons per second from spontaneous fission • One gram of americium-241 produces approximately – 4 x 103 neutrons per second from alpha-neutron reactions – No spontaneous fission © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 77 Intrinsic Neutron Sources Knowledge Check Select the three major contributors (types of reactions) to the intrinsic neutron source in a nuclear reactor. A. Photo-neutron B. Alpha-Neutron C. Spontaneous fission D. Oxygen-18 neutron Correct answers are A, B, and C. © Copyright 2017 – Rev 3 ELO 4.2 Operator Generic Fundamentals 78 Installed Neutron Sources ELO 4.3 - Describe, the purpose and types of installed neutron sources. • Because intrinsic neutron sources can be relatively weak or dependent upon the recent power history – Many reactors have additional neutrons sources installed to ensure a reliable and sufficient number of source neutrons – May be especially important with all new fuel in the core • Installed neutron sources ensure that shutdown neutron levels are high enough to be detected by the nuclear instruments at all times – Provides the operators with valid indication of the reactor’s status – Installed neutron sources are assemblies placed within the reactor for the sole purpose of producing source neutrons © Copyright 2017 – Rev 3 ELO 4.3 Operator Generic Fundamentals 79 Californium-252 • A strong source of neutrons • Artificial nuclide • Emits neutrons at the rate of about 2 x 1012 neutrons per second per gram from spontaneous fission • Not widely used as an installed neutron source in commercial PWRs because of its high cost and short half-life (2.65 years) © Copyright 2017 – Rev 3 ELO 4.3 Operator Generic Fundamentals 80 Alpha-Neutron Beryllium Source • Many installed neutron sources use an alpha-neutron reaction with beryllium • Composed of metallic beryllium (100 percent beryllium-9) with an alpha particle emitter, such as a compound of radium, polonium, or plutonium 13 ∗ 12 1 9 4 𝐵𝑒 + 𝛼 → 𝐶 → 𝐶+ 𝑛 4 2 6 6 0 • Is intimately (homogeneously) mixed with the alpha emitter and is usually enclosed in a stainless steel capsule © Copyright 2017 – Rev 3 ELO 4.3 Operator Generic Fundamentals 81 Photo- Neutron Beryllium Source • Beryllium-9 - stable isotope with weakly attached neutron with a binding energy of only 1.66 MeV • A gamma ray with greater energy than 1.66 MeV can cause neutrons to be ejected by the photo-neutron reaction 1 9 8 𝛾 + 𝐵𝑒 → 𝐵𝑒 + 𝑛 4 4 0 © Copyright 2017 – Rev 3 ELO 4.3 Operator Generic Fundamentals 82 Antimony-Beryllium Source • Most common secondary installed source • Antimony activated by absorbing neutron 123 1 124 𝑆𝑏 + 𝑛 → 𝑆𝑏 + 𝛾 51 0 51 • Radioactive antimony decays to Tellurium then emits high-energy gamma (60-day half-life) − 124 𝛽 124 0 𝑆𝑏 𝑇𝑒 + 𝑒+𝛾 51 52 −1 • Gamma ray has sufficient energy to interact with the beryllium to produce a neutron 1 9 8 𝛾 + 𝐵𝑒 → 𝐵𝑒 + 𝑛 4 4 0 © Copyright 2017 – Rev 3 ELO 4.3 Operator Generic Fundamentals 83 Installed Neutron Sources Knowledge Check Which of the following would be used to provide a source neutron population for a nuclear reactor core which has never been operated (newly installed core)? A. Photo-neutron source B. Transuranic source C. Startup source D. Installed source Correct answer is D. © Copyright 2017 – Rev 3 ELO 4.3 Operator Generic Fundamentals 84 Intrinsic Source Neutrons over Core Life ELO 4.4 - Describe the primary source of intrinsic source neutrons in the reactor for the following conditions; at beginning and end of core life: Immediately following a reactor shutdown, Several weeks after reactor shutdown. • Installed neutron sources provide a steady source of neutrons throughout core life – Over long periods their strength does decay • Intrinsic neutrons, however, do change in importance over core life © Copyright 2017 – Rev 3 ELO 4.4 Operator Generic Fundamentals 85 Photo-neutron Strength over Core Life • Changes significantly over core life • At BOL with no fission products present in the core (no high-energy gamma rays) little source neutron contribution – Deuterium concentration is also low BOL • Both factors change to increase source neutron production with increasing core life • After some power history - photo-neutron reactions are the largest contributor – Depending on amounts of new or reused fuel present – Exists for several days following shutdown from power operations © Copyright 2017 – Rev 3 ELO 4.4 Operator Generic Fundamentals 86 Transuranic Source Strength versus Core Life • Greater past middle-of-life (MOL) after several weeks of reactor shutdown from power operations – Transuranic alpha-neutron intrinsic neutron source tends to contribute the greatest number of source neutrons – Due to the photo-neutron source strength decaying off after a couple of weeks © Copyright 2017 – Rev 3 ELO 4.4 Operator Generic Fundamentals 87 Intrinsic Neutron Source Strength at Core BOL • Immediately following reactor shutdown from power: 1. Photo-neutron sources 2. Spontaneous fission sources 3. Alpha-neutron (transuranic) sources • Several weeks following reactor shutdown from power: 1. Spontaneous fission sources 2. Photo-neutron sources 3. Alpha-neutron (transuranic) sources © Copyright 2017 – Rev 3 ELO 4.4 Operator Generic Fundamentals 88 Intrinsic Neutron Source Strength at Core EOL • Immediately following reactor shutdown from power: 1. Photo-neutron sources 2. Alpha-neutron (transuranic) sources 3. Spontaneous fission sources • Several weeks following reactor shutdown from power: 1. Alpha-neutron (transuranic) sources 2. Spontaneous fission sources 3. Photo-neutron sources © Copyright 2017 – Rev 3 ELO 4.4 Operator Generic Fundamentals 89 Intrinsic Source Neutrons over Core Life Knowledge Check Which of the following reactions contributes the most to the source neutron population in a nuclear reactor core that is early in core life, shortly after the reactor is shutdown? A. Photo-neutron source B. Transuranic source C. Spontaneous fission source D. Californium source Correct answer is A. © Copyright 2017 – Rev 3 ELO 4.4 Operator Generic Fundamentals 90 Neutron Reaction Rates TLO 5 – Explain the relationship between neutron flux, microscopic and macroscopic cross-sections; and their affect on neutron reaction rates. 5.1 Explain the following terms, include any mathematical relationships: a. Atomic density b. Neutron flux c. Fast neutron flux d. Thermal neutron flux e. Microscopic cross-section f. Barn g. Macroscopic cross-section h. Mean free path 5.2 Define the following neutrons: a. Fast b. Intermediate c. Slow © Copyright 2017 – Rev 3 TLO 5 Operator Generic Fundamentals 91 Enabling Learning Objectives for TLO 5 5.3 Describe how the absorption and scattering cross-section of typical nuclides varies with neutron energies in the 1/v region and the resonance absorption region. 5.4 Given appropriate nuclei information, calculate the macroscopic cross-section and mean free path at various temperatures. 5.5 Describe radial and axial neutron flux distribution. 5.6 Describe how changes in neutron flux and macroscopic crosssection, affect reaction rates. 5.7 Describe the relationship between neutron flux and reactor power. © Copyright 2017 – Rev 3 TLO 5 Operator Generic Fundamentals 92 Neutron Reaction Terms ELO 5.1 - Explain the following terms, include any mathematical relationships: atomic density, neutron flux, fast neutron flux, thermal neutron flux, microscopic cross-section, barn, macroscopic cross-section, and mean free Path. Atomic Density • Atomic density is the number of atoms of a given type per unit volume of the material. 𝜌𝑁𝐴 𝑀 • Where: 𝑁 = Atomic density (atoms/cm3) 𝜌 = density (g/cm3) 𝑁𝐴 = Avogadro’s Number (6.022 x 1023 atoms/mole) 𝑀 = gram atomic weight or gram molecular weight 𝑁= © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 93 Atomic Density Example: • A block of aluminum has a density of 2.699 g/cm3. If the gram atomic weight of aluminum is 26.9815 g, calculate the atomic density of the aluminum. Solution: 𝜌𝑁𝐴 𝑁= 𝑀 𝑔 23 𝑎𝑡𝑜𝑚𝑠 6.022 × 10 𝑚𝑜𝑙𝑒 𝑐𝑚3 = 𝑔 26.9815 𝑚𝑜𝑙𝑒 𝑎𝑡𝑜𝑚𝑠 22 = 6.024 × 10 𝑐𝑚3 2.699 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 94 Neutron Flux • For calculations we need to know: – Number of neutrons existing in one cubic centimeter at any one instant – Total distance they travel each second while in that cubic centimeter • Neutron density (n) – Number of neutrons existing in a cm3 of material at any instant – Units of neutrons/cm3 • The total distance these neutrons travel each second is determined by the speed of the neutron © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 95 Neutron Flux • Number of neutrons passing through the unit area (cm2) per unit time – Total path length covered by all neutrons in one cubic centimeter during one second • Units are neutrons per square centimeter per second (n/cm2-sec) • Symbol Φ • Mathematically, Φ = 𝑛𝑣 • Where: Φ = neutron flux (neutron/cm2-sec) 𝑛 = neutron density (neutrons/cm3) 𝑣 = neutron velocity (cm/sec) © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 96 Neutron Flux • Since the atoms in a reactor do not have a preference for neutrons coming from any particular direction – All of the directional beams contribute to the total reaction rate – At any given point within a reactor, neutrons are traveling in all directions • In nuclear reactor, neutron flux is classified as either – Thermal flux – Fast flux © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 97 Thermal Neutron Flux • Thermal neutron flux (Φth) is the number of thermal neutrons crossing a unit area in the reactor in a given amount of time – Expressed in terms of neutrons (thermal) per square centimeter per second (n/cm2/sec) • Neutron flux is omni-directional – Neutrons can enter a particular square centimeter or reactor material from any direction • Therefore, Φth is viewed as the total distance of all thermal neutrons diffused (moved) in a particular unit volume in one second © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 98 Fast Neutron Flux • Fast neutron flux (Φf) is number of fast neutrons crossing a unit area in a given amount of time – Expressed in terms of neutrons (fast) per square centimeter per second (n/cm2/sec) • Fast neutron flux, Φf is viewed as the total distance that fast neutrons diffuse (move) in a particular unit volume in one second © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 99 Cross-Sections • The probability of a neutron interacting with a nucleus for a particular reaction is dependent on – The nucleus involved – The energy of the neutron • Absorption of a thermal neutron in most materials is much more probable than the absorption of a fast neutron • Probability of the neutron interaction varies with the type of reaction involved • Cross-section is based on the characteristics of the nucleus, not on the size of nucleus © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 100 Microscopic Cross-Section (σ) • Probability of a particular reaction occurring between a neutron and a nucleus varies with the energy of the neutron • May be regarded as the effective area the nucleus presents to the neutron for the particular reaction – Measured in barns – The larger the effective area, the greater the probability for reaction © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 101 Total Microscopic Cross-Section (σT) • A neutron interacts with an atom in two basic ways – Scattering – Absorption reaction • Probability of a neutron being absorbed is the microscopic crosssection for absorption (σa) • Probability of a neutron scattering is the microscopic cross-section for scattering (σs) • Sum of these two microscopic cross-sections is the total microscopic cross-section (σT) 𝜎𝑇 = 𝜎𝑎 + 𝜎𝑠 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 102 Microscopic Cross-Section for Scattering (σS) • Both the absorption and the scattering microscopic cross-sections can be further divided • Scattering cross-section is the sum of – Elastic scattering cross-section (σse) – The inelastic scattering cross-section (σsi) 𝜎𝑠 = 𝜎𝑠𝑒 + 𝜎𝑠𝑖 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 103 Microscopic Cross-Section for Absorption (σa) • Includes all reactions except scattering • For most purposes it is separated into two categories, – Fission (σf) and – Capture (σc) 𝜎𝑎 = 𝜎𝑓 + 𝜎𝑐 • The Chart of Nuclides uses two different conventions to represent microscopic cross-section for capture – If a gamma ray results, use σγ – If an alpha particle results, use σα © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 104 Barns • Microscopic cross-sections are expressed in units of area - square centimeters • 1 barn = 10-24 cm2 • Boron-10 – Has a relatively low mass with an absorption cross-section of 3838 barns that results in an ejected alpha particle – Presents a very large effective area for neutron interaction • Lead-208 – Relatively high mass and has an absorption cross-section of 8 microbarns (8 10-6 barns) for the same reaction – Presents a very small effective area for neutron interaction © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 105 Macroscopic Cross-Section (Σ) • Whether or not a neutron interacts with a certain volume of material depends – On its microscopic cross-section and – The number of nuclei within that volume (atomic density) • Macroscopic cross-section is the probability of a given reaction occurring per unit travel of the neutron – Related to microscopic cross-section (σ) by the following: Σ = 𝑁𝜎 • Where: Σ = macroscopic cross-section (cm-1) 𝑁 = atomic density (atoms/cm3) σ = microscopic cross-section (cm2) © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 106 Macroscopic Cross-Section (Σ) Microscopic Cross-Section Calculation • Most materials are composed of several elements, and most elements are composed of several isotopes; – Therefore, most materials involve many cross-sections, one for each isotope involved • To include all the isotopes for a material, each macroscopic crosssection is determined, then added together: Σ = 𝑁1𝜎1 + 𝑁2𝜎2 + 𝑁3𝜎3 + ⋯ … . . 𝑁𝑛𝜎𝑛 • Where: 𝑁𝑛 = the number of nuclei per cm3 of the nth element 𝜎𝑛 = the microscopic cross-section of the nth element © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 107 Macroscopic Cross-Section (Σ) Example Find the macroscopic thermal neutron absorption cross-section for iron, which has a density of 7.86 g/cm3. The iron microscopic cross-section for absorption is 2.56 barns and the gram atomic weight is 55.847 g. © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 108 Macroscopic Cross-Section (Σ) • Step 1: Using Equation for atomic density, calculate the atomic density of iron. 𝑔 23 𝑎𝑡𝑜𝑚𝑠 7.68 6.022 × 10 𝜌𝑁𝐴 𝑎𝑡𝑜𝑚𝑠 3 𝑚𝑜𝑙𝑒 𝑐𝑚 22 𝑁= = = 8.48 × 10 𝑔 𝑀 𝑐𝑚3 55.847 𝑚𝑜𝑙𝑒 • Step 2: Using the atomic density and given microscopic crosssection, calculate the macroscopic cross-section. Σ𝑎 = 𝑁𝜎𝑎 = 8.48 × 1022 𝑎𝑡𝑜𝑚𝑠 2.56 𝑏𝑎𝑟𝑛𝑠 3 𝑐𝑚 1 × 10−24 𝑐𝑚2 1 𝑏𝑎𝑟𝑛 Σ𝑎 = 0.217 𝑐𝑚−1 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 109 Microscopic versus Macroscopic CrossSection Review • Microscopic cross-section (σ) represents the effective target area that a single nucleus presents to a bombarding particle (neutron) – The units are in barns or cm2 • Macroscopic cross-section (Σ) represents the effective target area that is presented by all of the nuclei contained in 1 cm3 of the material – The units are 1/cm or cm-1 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 110 Mean Free Path • A neutron has a certain probability of undergoing a particular interaction in one centimeter of travel (Σ) in a material • The inverse of this probability describes how far the neutron will travel (average) before undergoing an interaction • Mean free path for interaction = average distance of travel by a neutron before interaction – Symbol λ 1 𝜆= Σ © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 111 Mean Free Path Mean Free Path Calculation Example An alloy is composed of 95 percent aluminum and 5 percent silicon (by weight). The density of the alloy is 2.66 g/cm3. Properties of aluminum and silicon are shown below. Element Gram Atomic Weight σa (barns) σs (barns) Aluminum 26.9815 0.23 1.49 Silicon 28.0855 0.16 2.20 Perform the following: 1. Calculate the atomic densities for aluminum and silicon. 2. Determine absorption and scattering macroscopic crosssections for thermal neutrons. 3. Calculate the mean free paths for absorption and scattering. © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 112 Mean Free Path Solution • Step 1: The density of aluminum is 95 percent of the total density. Using the formula for atomic density, calculate the atomic densities for aluminum and silicon. 𝑁𝐴𝑙 = 𝜌𝐴𝑙 𝑁𝐴 𝑀𝐴𝑙 𝑁𝑆𝑖 = 𝑔 23 𝑎𝑡𝑜𝑚𝑠 6.022 × 10 𝑚𝑜𝑙𝑒 𝑐𝑚3 = 𝑔 26.9815 𝑚𝑜𝑙𝑒 𝑎𝑡𝑜𝑚𝑠 = 5.64 × 1022 𝑐𝑚3 𝑔 23 𝑎𝑡𝑜𝑚𝑠 6.022 × 10 𝑚𝑜𝑙𝑒 𝑐𝑚3 = 𝑔 28.0855 𝑚𝑜𝑙𝑒 𝑎𝑡𝑜𝑚𝑠 = 2.85 × 1021 𝑐𝑚3 0.95 2.66 © Copyright 2017 – Rev 3 𝜌𝑆𝑖 𝑁𝐴 𝑀𝑆𝑖 0.05 2.66 ELO 5.1 Operator Generic Fundamentals 113 Mean Free Path Solution • Step 2: The absorption and scattering macroscopic cross-sections are calculated from the microscopic cross-sections and the combined atomic densities (95 percent aluminum and 5 percent silicon). Σ𝑎 = 𝑁𝐴𝑙 𝜎𝑎,𝐴𝑙 + 𝑁𝑆𝑖 𝜎𝑎,𝑆𝑖 = 5.64 × 1022 𝑎𝑡𝑜𝑚𝑠 𝑐𝑚3 0.23 × 10−24 𝑐𝑚2 + 2.85 × 1021 𝑎𝑡𝑜𝑚𝑠 𝑐𝑚3 0.16 × 10−24 𝑐𝑚2 1.49 × 10−24 𝑐𝑚2 + 2.85 × 1021 𝑎𝑡𝑜𝑚𝑠 𝑐𝑚3 2.20 × 10−24 𝑐𝑚2 = 0.0134 𝑐𝑚−1 Σ𝑠 = 𝑁𝐴𝑙 𝜎𝑠,𝐴𝑙 + 𝑁𝑆𝑖 𝜎𝑠,𝑆𝑖 = 5.64 × 1022 𝑎𝑡𝑜𝑚𝑠 𝑐𝑚3 = 0.0903 𝑐𝑚−1 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 114 Mean Free Path Solution • Step 3: Mean free paths are determined from the calculated absorption and scattering macroscopic cross-sections. 𝜆𝑎 = 1 Σ𝑎 1 0.01345 𝑐𝑚−1 = 74.3 𝑐𝑚 = 1 𝜆𝑠 = Σ𝑠 1 = 0.0903 𝑐𝑚−1 = 11.1 𝑐𝑚 © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 115 Neutron Reaction Terms Knowledge Check: _______________ is the total path length traveled by all neutrons in one cubic centimeter of material during one second. A. Mean free path B. Neutron flux C. Gamma flux D. Atomic density Correct answer is B. © Copyright 2017 – Rev 3 ELO 5.1 Operator Generic Fundamentals 116 Neutron Energy Terms ELO 5.2 - Define the following neutrons: fast, intermediate, and slow. • Neutrons are classified by energy levels: – Fast – Intermediate – Slow • Neutrons in energy equilibrium with their surrounding are called thermal neutrons. – These are in the slow category – Most important where thermal reactors are concerned © Copyright 2017 – Rev 3 ELO 5.2 Operator Generic Fundamentals 117 Neutron Energy Terms < 1 ev > 1 ev and < .1 Mev Born fast - > .1 Mev Figure: Neutron Energy © Copyright 2017 – Rev 3 ELO 5.2 Operator Generic Fundamentals 118 Neutron Energy Terms Knowledge Check Thermal neutrons are classified in the intermediate neutron energy range. A. True B. False Correct answer is B. © Copyright 2017 – Rev 3 ELO 5.2 Operator Generic Fundamentals 119 Neutron Energies versus Cross-Sections ELO 5.3 - Describe how the absorption and scattering cross-section of typical nuclides varies with neutron energies in the 1/v region and the resonance absorption region. • Neutron cross-sections, both absorption and scattering, are affected by neutron energies • In general, the higher the energy of the neutron the lower the probability of interaction • Resonance peaks at certain specific energies possess very high cross-sections © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 120 Neutron Energies versus Cross-Sections • Absorption cross-sections have three unique regions of probability related to neutron energy – 1/v region – Resonance region – Fast neutron region • Each with a different relationship to changing neutron energy • Neutron scattering cross-sections are different – Resonance elastic scattering and inelastic scattering crosssections do have resonance peaks smaller than absorption peaks – Potential elastic scattering cross-sections are not greatly affected by neutron energy © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 121 Neutron Scattering Cross-Section versus Incident Neutron Energy • With the exception of hydrogen, the elastic scattering cross-sections are generally small – Typically 5 barns to 10 barns – Close to the magnitude of the actual geometric cross-sectional area expected for atomic nuclei • In potential elastic scattering – Cross-section is essentially constant – Independent of neutron energy up to around 1 MeV © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 122 Neutron Scattering Cross-Section versus Incident Neutron Energy • Resonance elastic scattering and inelastic scattering exhibit resonance peaks similar to those for absorption cross-sections – Resonances occur at lower energies for heavy nuclei than for light nuclei – Variations in scattering cross-sections are very small when compared to the variations that occur in absorption cross-sections © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 123 Neutron Scattering Cross-Section versus Incident Neutron Energy • In the thermal reactor scattering reactions are primarily of concern in the moderator where neutrons are thermalized • Water (the moderator) are light nuclei, and elastic scatterings are most probable in light nuclei, therefore, σs = σselastic Figure: Elastic Scattering Cross-Section versus Neutron Energy © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 124 Neutron Absorption Cross-Section versus Incident Neutron Energy • Variation of absorption cross-sections with neutron energy is complex • Absorption cross-sections are small for many elements, ranging from a fraction of a barn to a few barns for thermal neutrons • For a considerable number of nuclides the variation of absorption cross-sections with incident neutron energy reveals three distinct regions: – 1/v region – Resonance peaks region – Fast neutron region © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 125 Neutron Absorption Cross-Section versus Neutron Energy - 1/v Region Figure: Typical Neutron Absorption Cross-Section versus Neutron Energy © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 126 Neutron Absorption Cross-Section vs. Neutron Energy - Resonance Region Figure: Typical Neutron Absorption Cross-Section versus Neutron Energy © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 127 Neutron Absorption Cross-Section versus Incident Neutron Energy Example • Assuming that uranium-235 has a nuclear quantum energy level at 6.8 MeV above its ground state, calculate the kinetic energy a neutron must possess to undergo resonant absorption in uranium235 at this resonance energy level. Solution 𝑀𝑒𝑉 𝐵𝐸 = 𝑀𝑎𝑠𝑠 𝑈 + 𝑀𝑎𝑠𝑠 𝑛𝑒𝑢𝑡𝑟𝑜𝑛 − 𝑀𝑎𝑠𝑠 𝑈 × 931 𝑎𝑚𝑢 𝑀𝑒𝑉 𝐵𝐸 = 235.043925 + 1.008665 − 236.045563 × 931 𝑎𝑚𝑢 𝑀𝑒𝑉 𝐵𝐸 = 0.007025 𝑎𝑚𝑢 × 931 = 6.54 𝑀𝑒𝑉 𝑎𝑚𝑢 6.8 𝑀𝑒𝑉 − 6.54 𝑀𝑒𝑉 = 0.26 𝑀𝑒𝑉 236 235 © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 128 Neutron Absorption Cross-Section versus Incident Neutron Energy Figure: Typical Neutron Absorption Cross-Section versus Neutron Energy © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 129 Neutron Energies versus Cross-Sections Knowledge Check At low neutron energies (<1 eV) the absorption cross-section for a material is ___________ proportional to the neutron velocity. (Fill in the blank). Correct answer is inversely. © Copyright 2017 – Rev 3 ELO 5.3 Operator Generic Fundamentals 130 Temperature Effects to Macroscopic Cross-Sections ELO 5.4 - Describe the macroscopic cross-section and mean free path at various temperatures. • Microscopic absorption cross-sections vary significantly as thermal neutron energy varies – Values given on most charts and tables are at an ambient temperature of 68°F – Equals a neutron velocity of 2,200 meters/second or 0.025 eV energy – At higher temperatures, microscopic absorption cross-sections must be corrected for the new temperature value • A temperature corrected microscopic cross-section allows corrected macroscopic cross-sections and mean free paths © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 131 Temperature Effects to Macroscopic Cross-Sections Note • Temperature corrections apply to any cross-section involving absorption (for example, σa, σc, σf) • However, they do not apply to scattering cross-sections, as neutron energies up to 1 Mev, have little effect on the predominant elastic scatterings occurring in the moderator © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 132 Temperature Affects to Macroscopic Cross-Sections • Determine the microscopic cross-section by obtaining the standard (at 68°F) table value • Convert temperatures to either Rankine or Kelvin absolute temperature scales – °R = °F + 460 or °K = °C + 273 1 • Calculate new microscopic cross-section using: 𝜎 = 𝑇 2 𝜎𝑜 𝑇𝑜 • Where: 𝜎 = microscopic cross-section corrected for temperature 𝜎𝑜 = microscopic cross-section at reference temperature (68°F or 20°C) 𝑇𝑜 = reference temperature (68°F) in degrees Rankine (°R) or Kelvin (°K) 𝑇 = temperature for which corrected value is being calculated © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 133 Temperature Affects to Macroscopic Cross-Sections • Calculate new macroscopic cross-section Σ = 𝑁𝜎 • Where: Σ = macroscopic cross-section (cm-1) 𝑁 = atomic density (atoms/cm3) 𝜎 = microscopic cross-section (cm2) • Calculate new mean free path (λ) 1 𝜆= Σ © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 134 Temperature Affects to Macroscopic Cross-Sections Example What is the fission macroscopic cross-section and mean free path for uranium-235 for thermal neutrons at 500°F? • Given: – Uranium-235 has a σf of 583 barns at 68°F. – Atomic density of uranium-235 is 7.03 x 1020 atoms/cm3 © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 135 Temperature Affects to Macroscopic Cross-Sections Solution • Steps 1, 2 and 3. Determine microscopic cross-section 𝜎𝑓 = 𝜎𝑓,𝑜 1 𝑇𝑜 2 𝑇 68℉ + 460 = 583 𝑏𝑎𝑟𝑛𝑠 500℉ + 460 1 2 = 432 𝑏𝑎𝑟𝑛𝑠 • Step 4. Determine macroscopic cross-section for fission 2 𝑎𝑡𝑜𝑚𝑠 𝑐𝑚 Ʃ𝑓 = 𝑁𝜎 = 7.03 × 1020 × 432 𝐵𝑎𝑟𝑛𝑠 × 1 × 10−24 3 𝑐𝑚 𝐵𝑎𝑟𝑛 Ʃ𝑓 = 0.304 𝑐𝑚−1 • Step 5. Determine the mean free path for fission 1 1 𝜆= = = 3.29 𝑐𝑚 Σ 0.304 𝑐𝑚−1 © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 136 Temperature Affects to Macroscopic Cross-Sections Macroscopic Cross-Section versus Temperature • Macroscopic cross-section is inversely proportional to temperature – As temperature increases, macroscopic cross-section decreases Mean Free Path versus Temperature • Mean free path shows that it is inverse to the macroscopic crosssection – Directly proportional to temperature – As temperature increases, the mean free path increases © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 137 Temperature Affects to Macroscopic Cross-Sections Knowledge Check If an isotope has an absorption microscopic cross-section of 5,000 barns at 68°F, what happens to its absorption microscopic crosssection if temperature is increased to 1,000°F? A. Increases B. Decreases C. No change D. Need more data to answer Correct answer is B. © Copyright 2017 – Rev 3 ELO 5.4 Operator Generic Fundamentals 138 Neutron Flux Distribution ELO 5.5 - Describe radial and axial neutron flux distribution. • Neutron flux distribution is very important and is monitored by not only the operators but also by reactor engineering • Limiting uneven flux distribution ensures fuel cladding integrity © Copyright 2017 – Rev 3 ELO 5.5 Operator Generic Fundamentals 139 Neutron Flux Distribution • Neutrons interact with all materials in a reactor, absorptions, scattering • The type of material found in particular locations of the core affects the neutron flux in that area • Examples: – Fast neutron flux in materials with large scattering cross-sections causes fast neutrons to slow down to lower energy levels more quickly – This reduces the fast neutron flux – Intermediate and thermal neutron flux increases as a larger percentage of fast neutrons slow down to these energy levels © Copyright 2017 – Rev 3 ELO 5.5 Operator Generic Fundamentals 140 Axial and Radial Neutron Flux Commercial PWR nuclear reactor cores are cylindrical in shape. • Axial and radial flux are used to describe neutron flux profiles from top to bottom and across the core. Figure: Axial and Radial Neutron Flux in a Reactor Core © Copyright 2017 – Rev 3 ELO 5.5 Operator Generic Fundamentals 141 Axial and Radial Neutron Flux • The axial and radial neutron flux distribution across a nuclear reactor is a spatial representation of neutron flux level throughout the core • Within the core boundaries, neutrons are – Being produced from fission – Slowed down by the moderator – Captured by core materials and fuel, and fissioned Figure: Axial and Radial Neutron Flux in a Reactor Core • These all affect the neutron flux distribution in the core © Copyright 2017 – Rev 3 ELO 5.5 Operator Generic Fundamentals 142 Axial and Radial Neutron Flux • Neutron flux distribution is generally highest in the center of the core and drops off toward the core boundaries (top and bottom, sides) • Neutrons produced near the edges of the core are more likely to leak out and not cause fission – Reducing thermal neutron flux in the outer boundaries of the core • Neutrons toward the center, have less leakage and greater probability of thermalizing to cause more fissions – Increasing neutron flux levels toward the center of the core © Copyright 2017 – Rev 3 Figure: Axial and Radial Neutron Flux in a Reactor Core ELO 5.5 Operator Generic Fundamentals 143 Self-Shielding • Neutron flux levels may be lower in some localized areas than in others – Known as self-shielding • For example, the interior of a fuel pin or pellet is exposed to a lower average neutron flux level than the outer surfaces – Caused by large fraction of neutrons having been absorbed in the outer layers of the fuel, reducing neutron availability to the pellet interior • Concept of self-shielding is also important relating to neutron poisons in the reactor core © Copyright 2017 – Rev 3 ELO 5.5 Operator Generic Fundamentals 144 Neutron Flux Distribution Knowledge Check The neutron flux that varies from the top to bottom of the core is called the ________ flux and the neutron flux that varies from across the top is ________. Correct answer is axial; radial. © Copyright 2017 – Rev 3 ELO 5.5 Operator Generic Fundamentals 145 Reaction Rate ELO 5.6 - Describe how changes in neutron flux and macroscopic crosssection, affect reaction rates. • Neutron flux [Φ] times macroscopic cross-section [Σ] equals the reaction rate – Denoted by the symbol R • The type of reaction rate calculated depends on the macroscopic cross-section used in the calculation • Normally, the reaction rate of greatest interest is the fission reaction rate © Copyright 2017 – Rev 3 ELO 5.6 Operator Generic Fundamentals 146 Neutron Reaction Rates • Fission neutrons are born at an average energy of about 2 MeV – Interact with reactor core materials in various absorption and scattering reactions – Scattering reactions are useful for thermalizing neutrons – Thermal neutrons absorbed for fission – Absorption in fertile material for production of fissionable fuel • Some neutrons are absorbed in structural components, reactor coolant, and other non-fuel materials – Resulting in the removal of neutrons from the fission process © Copyright 2017 – Rev 3 ELO 5.6 Operator Generic Fundamentals 147 Neutron Reaction Rates • To determine these neutron interaction rates, it is necessary to – Identify the number of neutrons available – The probability of interaction • To quantify neutron availability and reaction probabilities, terms including – Neutron flux – Microscopic cross-section – Macroscopic cross-section © Copyright 2017 – Rev 3 ELO 5.6 Operator Generic Fundamentals 148 Reaction Rate Calculation of the reaction rate: 1. Obtain the average thermal neutron flux in the reactor 2. Obtain the fuel macroscopic cross-section for the particular material and reaction of interest 3. Using the following formula for reaction rate, calculate the reaction rate 𝑅 = ΣΦ Where: 𝑅 = reaction rate (reactions/cm3 sec) Σ = macroscopic cross-section (cm-1) © Copyright 2017 – Rev 3 ELO 5.6 Operator Generic Fundamentals 149 Reaction Rate Demonstration Example • A reactor has a macroscopic fission cross-section of 0.1 cm-1, and thermal neutron flux of 1013 neutrons/cm2-sec, what is the fission rate in that cubic centimeter? Solution 𝑅𝑓 = ΦΣf 𝑛𝑒𝑢𝑡𝑟𝑜𝑛𝑠 = 1 × 10 𝑐𝑚2 – 𝑠𝑒𝑐 𝑓𝑖𝑠𝑠𝑖𝑜𝑛𝑠 = 1 × 1012 𝑐𝑚3 – 𝑠𝑒𝑐 13 © Copyright 2017 – Rev 3 0.1 𝑐𝑚−1 ELO 5.6 Operator Generic Fundamentals 150 Reaction Rate Knowledge Check Calculate the reaction rate (fission rate) in a one cubic centimeter section of a reactor that has a macroscopic fission cross-section of 0.2 cm-1, and a thermal neutron flux of 1014 neutrons/cm2-sec. neutrons cm2 –sec A. R = 2.0 × 1014 B. R = 0.2 × 1013 C. R = 2.0 × 1013 neutrons cm3 –sec D. R = 20 × 1013 neutrons cm3 –sec neutrons cm2 –sec Correct answer is C. © Copyright 2017 – Rev 3 ELO 5.6 Operator Generic Fundamentals 151 Reaction Rate Knowledge Check If the microscopic cross section for fission increases in a nuclear reactor, how will the reaction rate for fission be affected? A. R will decrease B. R will stay the same C. R change can not be determined based on information provided. D. R will increase Correct answer is D. © Copyright 2017 – Rev 3 ELO 5.6 Operator Generic Fundamentals 152 Neutron Flux and Reactor Power ELO 5.7 - Describe the relationship between neutron flux and reactor power. • Multiplying the reaction rate per unit volume by the total volume of the core equals the total number of reactions occurring in the core per unit time • If the amount of energy involved in each reaction is known, the rate of energy release (power) due to a certain reaction can be determined © Copyright 2017 – Rev 3 ELO 5.7 Operator Generic Fundamentals 153 Neutron Flux and Reactor Power • If average energy per fission is 200 MeV, the number of fissions to produce one watt of power equals: – 1 fission = 200 MeV – 1 MeV = 1.602 x 10-6 ergs – 1 erg = 1 x 10-7 watt-sec 1 𝑤𝑎𝑡𝑡 1 𝑒𝑟𝑔 1 × 10−7 𝑤𝑎𝑡𝑡– 𝑠𝑒𝑐 1 𝑀𝑒𝑉 1.602 × 10−6 𝑒𝑟𝑔 1 𝑓𝑖𝑠𝑠𝑖𝑜𝑛 𝑓𝑖𝑠𝑠𝑖𝑜𝑛 = 3.12 × 1010 200 𝑀𝑒𝑉 𝑠𝑒𝑐𝑜𝑛𝑑 • 3.12 x 1010 fissions release 1 watt-second of energy © Copyright 2017 – Rev 3 ELO 5.7 Operator Generic Fundamentals 154 Neutron Flux and Reactor Power Step 1. 2. © Copyright 2017 – Rev 3 Action Obtain the following reactor data: • Volume of core (cm3) 𝑅 = ΣΦ • Reaction rate OR • Fission macroscopic cross-section and average thermal neutron flux Calculate reactor power using the following equation, substitute reaction rate if known: Φ𝑡ℎ Σ𝑓 𝑉 𝑃= 𝑓𝑖𝑠𝑠𝑖𝑜𝑛𝑠 3.12 × 1010 𝑤𝑎𝑡𝑡– 𝑠𝑒𝑐 Where: P = power (watts) Φth = thermal neutron flux (neutrons/cm2 –sec) Σf = macroscopic cross-section for fission (cm-1) V = volume of core (cm3) ELO 5.7 Operator Generic Fundamentals 155 Relationship between Neutron Flux and Reactor Power • In an operating reactor the volume of the reactor is constant • Over a relatively short period of time (days and weeks), the number (density) of fuel atoms is also relatively constant • With a constant atomic density and microscopic cross-section, the macroscopic cross-section is also constant • If the reactor volume and macroscopic cross-section are constant, then reactor power and the neutron flux are directly proportional • If the fission macroscopic cross-section decreases from the reactor fuel burnup, neutron flux must increase to maintain power constant © Copyright 2017 – Rev 3 ELO 5.7 Operator Generic Fundamentals
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