JLAB-TN-06-022 Suitability of High Power Beam Dumps in Hall A and Hall C for use at 14.5 GeV Operation Erik Abkemeier, Radiation Control Department The purpose of this technical note is to summarize and update information concerning operability of the High Power Beam Dumps (HPBDs) located in Experimental Halls A and C at an energy of 14.5 GeV, and an operating beam power envelope of 900 kW (e.g. an operating beam current of 62 microamps at an energy of 14.5 GeV) and a safety envelope of 1 MW. An important fundamental concept to grasp is that all aspects within the realm or radiological protection (e.g., dose rate produced) essentially scale with operating beam power, particularly for accelerators operating at energies above 3 Ge, as shown in Figure 1. (Thomas, 2003; Sullivan 1992). The proposed operating and safety envelopes for 14.5 GeV operation to either Experimental Hall A or C is identical to the current operating envelope of 900 kW and a safety envelope of 1 MW for Experimental Halls A and C with operation a approximately 6 GeV, which is the current physical accelerator operating limit at the time of this technical note. In order to explain how operating either Experimental Hall A or C at 14.5 GeV would affect the surrounding groundwater, it is helpful to summarize how the shielding for the HPBD shielding was developed during the initial construction. The principal factors include: (1) the radioisotopes potentially created, leached into groundwater, and the groundwater standards to which Jefferson Lab was to be held; (2) the assumed average beam power operating envelope; (3) the groundwater flow rate; (4) the dose created from impinging typical beam power on the beam coupled with a conversion to neutron flux at energies necessary to create the radioisotopes. Each of these factors will briefly be discussed and compared as to the impact for the proposed energy upgrade versus the original shielding design criteria. As to the driving concern (i.e., radionuclides produced in the groundwater outside of the HPBD shielding enclosure), the only long-lived radionuclides of concern capable of being produced in soil and leached into water, or produced directly in groundwater continue to be H-2 and Na-22. (Stapleton, 1989). An increase in beam energy will not introduce the potential for more radionuclides of concern. The groundwater standards at the time of the original design of the HPBD shielding enclosures were such that the total dose to a person not exceed 1 mrem per year if ingesting the water at a rate of 2.2 liters a day. This correlated to a concentration of 2800 pCi/l for H-3, and 100 pCi/ for Na-22. These standards have not changed since that time. The only peripheral point of note is that Jefferson Lab currently is issued a permit from the Commonwealth of Virginia Department of Environmental Quality that references a number of groundwater wells in three concentric rings varying from 3 to 5 meters from the accelerator ring and experimental halls, and to the site boundary (VPDES, 2001). For the closest wells (in the “A” ring), an “action limit” of 5000 pCi/l for H-3 is enacted such that if during the mandatory quarterly sampling which is required to be submitted to the DEQ. Additionally, the “C” ring wells located at the site boundary have a limit of 1000 pCi/l for H-3 and 61 pCi/l for Na-22. As a note, during the conduct of mandatory sampling and JLAB-TN-06-022 analysis by a third party radiochemical analysis lab, no detectable concentrations of H-3 or Na-22 have been detected at any groundwater well site at any time since the inception of the sampling protocol in 1989( Virginia Commonwealth 1989-2006). As the CEBAF accelerator has been operating since 1994, this would indicate that the HPBD shielding enclosure (as well as other groundwater shielding) has performed more than adequately. Concerning the assumed average beam power operating envelope, the constraints on maximum normal beam power operations will remain in effect. That being the case, the power assumptions from the initial design of the HPBD shielding enclosure remain valid. The groundwater flow is a critical piece in determining concentrations of radionuclides in the groundwater because the build-up of radionuclides in the groundwater is directly proportional to the residence time that the water remains in the neutron flux field that creates the radionuclides. In other words, the slower the groundwater movement rate, the greater the radionuclide concentration in the groundwater. At design time for the the HPBD shielding enclosures, the estimated groundwater flowrate was assumed to be zero, i.e., the water would remain around the surfaces exposed to neutron flux so that the water would reach a saturation concentration. (Stapleton 1989). Post accelerator construction and start up hydrogeological survey performed by Malcolm Pirnie indicates that the groundwater flow rate in the area of the HPBD at Hall A averages 68 meters per year for the period from 1996 to 2001 (Malcolm Pirnie 2001). This same study shows an average groundwater flow in the area of the HPBD for Hall C of 142 meters per year for the same period. To date, this flow has not been considered in the groundwater activation calculations. Because the experimental halls have been constructed below the water table, in order to maintain structural integrity of the halls, it is necessary to continuously pump groundwater around the experimental halls to the surface at a rate of approximately 12,000 to 24,000 gallons per day (Malcolm Pirnie, 1995). These dewatering operations cause the elevated groundwater flow rates in the areas surrounding the experimental halls. (As a note, the de-watering consists of water collecting in the End Station Dewatering Sump that is monitored for radionuclide concentration prior to discharge to the surface). The radionuclide production mechanism in groundwater at 14.5 GeV is the same as that at 6 GeV, i.e., it is based upon the neutron fluence rate into the soil/groundwater surrounding the concrete shielding surrounding the HPBDs for neutrons above the energy of approximately 20 MeV. This number is obtained conservatively by converting an assumed neutron dose rate based upon empirical shielding calculations developed at SLAC from an accelerator operating at 15 GeV, into a neutron flux rate using a selected dose to neutron flux conversion factor (Jenkins, 1979). As stated previously and shown in the SHIELD 11 coded exposure rate formula, the dose rate is proportional to power envelope (Nelson, 2005). As this power envelope remains the same at 14.5 GeV as it is at current operating energy of 6 GeV, the calculated dose rate will remain the same. The dose rate to neutron flux conversion rate used for the original 6 GeV calculation was based on a conservative approximation of 2.3 n/cm2sec per 1 mrem/hr which continues to be valid to energies up to 28 GeV(Gilbert 1968). Additionally, the simplified conservative model for the initial calculations was predicated on all of the neutron JLAB-TN-06-022 production emanating at a single point within the middle of the proposed HPBD. A more complex modeling was undertaken that showed the H-3 and Na-22 concentration levels anticipated would be approximately a factor of 10 lower than calculated under the original method (Thomas 1989). This is further borne out in that no groundwater well in any of the rings around the accelerator and experimental halls has ever had any detectable concentration of H-3 or Na-22. For H-3, this is approximately 700 pCi/l. For Na-22, this is approximately 30 pCi/l. The past 4 years indicated that actual experimental power for the year was on the order of 100 kW for the entire year (Degtiarenko 2002, 2003, 2004, 2005). For an exercise in conservatively scaling radionuclide concentration to power deposited in the beam dumps based on radioanalytical results, we can assume that the water levels were actually at the highest Minimum Detectable Concentrations, and scaled power up to 750 kW in each hall (which is highly unlikely given that Scheduled Accelerator Downs occur for at least 2 months out of any given year, and in order to average 750 kW, the Halls would need to be operating at maximum capacity for the remaining 10 months of the year.) Even given that entirely unrealistic set of conditions, this would scale to a concentration approximately 5250 pCi/l for H-3, and 225 pCi/l for Na-22. Again this assumes an unrealistic extended run of maximum power accelerator beam delivered to a hall, coupled with the assumption that water surrounding the HPBDs is stationary and at saturation activity (which is clearly not the case), and the radionuclide concentration in the water is just beneath the MDC. Even under this extremely conservative scenario the concentrations projected are not entirely inconsistent with limits for the EPA. The derivation of the concentration limits is described more fully in previous tech notes, but is based upon one quarter of the EPA limit of 4 mrem/year assuming ingestion of the groundwater in question. This correlates to a limit of 2800 pCi/l for H-3 and 100 pCi/l for Na-22 in order to receive a dose of 1 mrem in a year. For the purposes of obtaining more accurate (yet conservative) numbers, now that information of groundwater flow data is more readily available, the calculation will be performed utilizing the SHIELD 11 code formula, with only the high energy and mid energy neutron components, as these are the only components active in activation of soil and water. The formula for this is: 100t 100t c 120 c 3 2 1 55 MIDe 2.3x10 n cm s Where φ = activating neutron fluence rate HEN = 22.5 rem h-1 kW-1 m2 MID = 225 rem h-1 kW-1 m2 t = thickness of concrete = 4.5 meters at 90 degrees ρc = density of concrete = 2.35 g/cm3 HENe at one meter This results in an activating neutron fluence rate for a saturation activity in the water normalized to power of 7.7 n cm-2 s-1 per m2/kW. The assumed conservative power envelope (as described previously) is 750 kW averaged throughout the year. JLAB-TN-06-022 Additionally, the distance at 90 degrees from the point of beam interaction with the beam dump which includes the thickness of the concrete and air space between the dump and the concrete is approximately 5.5 meters. Using these numbers yields a neutron fluence of 190 n cm-2 s-1. However, this number assumes that the water remains static in the regions adjacent to the HPBDs (i.e., the water does not move.) We know from hydrogeologic studies that this is not the case (Malcolm Pirnie 2001). In fact, due to the continuous pumping action necessary to maintain structural integrity of the Experimental halls, water moves rapidly in that area. By inspection of Fig. 2 which is a simulated spectrum of neutrons traveling through the concrete dimensions of the HPBD shielding enclosure using GEANT modeling, one can see that only approximately half of the surface area is exposed to the neutron activating flux. In other words, groundwater cannot be activated unless it comes in contact with this region. For the sake of conservatism, we can assume a worst case scenario in which groundwater flows along the lateral surface of one side of the HPBD shielding enclosure and down to a point under the center of the experimental hall where the groundwater is collected in the end station dewatering sump. We will also assume that (contrary to modeling), the entire surface of the HPBD shielding enclosure has an activating neutron flux of energy greater than 20 MeV, such that groundwater can be activated during the entire time that it is in the region of the shielding wall until the water reaches the groundwater dewatering sump. We will then assume that the water flow in the region of the HPBD shielding is the average from the lower of the two halls (68 meters/year), and use that to determine the actual build-up of activity, and concentration as the water passes through that area. We can use the formula for determining activity at time t, which can be adjusted for neutron activating flux by canceling out like terms such that the following correction factor is used. ( 1 e t )( e t ) to account for building up activity as well as decay in the water, and hence concentration (Bevelacqua, 1999). In the case of H-3: λ = 0.693/(12.3 years)] t = (60 m) / (68 m/year) Which results in a correction factor of: 0.046. This, in turn, results in a scaled down neutron flux of 8.7 n cm-2 s-1 In the case of Na-22: λ = 0.693/[(2.6 years) t = (60 m)/(68 m/year) which results in a correction factor of 0.165. This, in turn results in a scaled down neutron flux of 31.3 n cm-2 s-1 From previous calculations determining radionuclide concentration in groundwater, the limit for neutron fluence rate to prevent groundwater activation that would cause greater JLAB-TN-06-022 than 1 mrem/year dose is 35 n cm-2 s-1 (Stapleton, 1997). As one can see, the neutron fluence rates are again beneath those necessary to maintain the H-3 and Na-22 concentrations beneath one quarter of the EPA limits. In conclusion, production of radionuclides of concern in groundwater (H-3 and Na-22) is proportional to beam power. As the beam power operating envelope will not change in the course of running 6GeV operations to 14.5 GeV operations, radionuclide production should not vary significantly. Additionally, design of the original High Power Beam Dump shielding enclosure did not take credit for the rapid groundwater flow rates in the areas adjacent to the Experimental Halls, which is a parameter that significantly affects radionuclide production. Furthermore, quarterly sampling of installed groundwater wells since the beginning of accelerator operations has not shown any detectable concentrations of H-3 or Na-22. JLAB-TN-06-022 References Bevelacqua, J. 1999. “Basic Health Physics”, John Wiley and Sons Degtiarenko, P. 2002. “Radiation Dose Rates Resulting from the Experimental Program at Jefferson Lab, July-December 2002” RCG Note 02-03, Newport News, Virginia Degtiarenko, P. 2003. “Radiation Dose Rates Resulting from the Experimental Program at Jefferson Lab, October-December 2003” RCG Note 03-04, Newport News, Virginia Degtiarenko, P. 2004. “Radiation Dose Rates Resulting from the Experimental Program at Jefferson Lab, October-December 2004” RCG Note 04-04, Newport News, Virginia Degtiarenko, P. 2005. “Radiation Dose Rates Resulting from the Experimental Program at Jefferson Lab, July-December 2005” RCG Note 05-02, Newport News, Virginia Gilbert, W.S. et al. 1968. CERN-LRL-RHEL Shielding Experiment at CERN, Lawrence Radiation Laboratory Report UCRL-17941, Sept. 1968 Jenkins, T. 1979. “Neutron and Photon Measurements Through Concrete from a 15 GeV electron Beam on a Target – Comparison with Models and Calculations”, Nuclear Instruments and Methods 159. Malcolm Pirnie, Inc. 1995. CEBAF Hydrogeologic Review, Newport News, Virginia, September. Malcolm Pirnie, Inc. 2002. Groundwater Flow Directions and Velocities at Jefferson Lab, Newport News, Virginia, February. Nelson, W. et al. 2005. SLAC-Report-737 “The SHIELD11 Computer Code”, February 2005. Stapleton, G. 1987. “The Production of Radionuclides in the Groundwater”, Jefferson Lab Tech Note, TN-0062, Newport News, Virginia Stapleton, G. 1989. “Design of Shielding to Ensure Maximum Concentrations of H-3 and Na-22 in the Groundwater Remain Within Standards”, Jefferson Lab Tech Note TN-0155, Newport News, Virginia Stapleton, G. et al. 1997. “Occupational and Environment Aspects of the Radiation Control Provisions at Jefferson Lab,” Jefferson Lab Tech Note, JLAB TN 97-017, Newport News, Virginia. JLAB-TN-06-022 Sullivan, A. H. 1992. “A Guide to Radiation and Radioactivity Levels Near High Energy Particle Accelerators,” Nuclear Technical Publishing, Ashford, Kent, TN23 1JW, England, Chap 4. Thomas R., et al. 1989. “Review of the Radiological Aspect of the Conceptual Design Report for the CEBAF End Station and Switchyard, August 15-17, 1989”, Jefferson Lab Tech Note TN-0174, Appendix 4 “Consideration of the Use of the EGS/FLUKA Monte Carlo Code to Determine the Activity of H-3 and Na-22 in the Groundwater”. Thomas R., et al., 2003. NCRP (National Council on Radiation Protection and Measurement) No. 144, “Radiation Protection for Particle Accelerator Facilities”. Virginia Commonwealth Department of Environmental Quality (DEQ) VPDES Monitoring Reports 1989-2006. VPDES (Virginia Pollutant Discharge Elimination System) Permit No. VA0089320. Thomas Jefferson National Accelerator Facility/U.S. Department of Energy, Newport News, Virginia. Effective July 16, 2001 to July 16, 2006 JLAB-TN-06-022 Figure 1 JLAB-TN-06-022 Figure 2
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