Chapter 10. Laser Oscillation : Gain and Threshold Detailed description of laser oscillation 10.2 Gain <Plane wave propagating in vacuum> Consider a quasi-monochromatic plane wave of frequency n propagating in the +z direction ; A un z The rate at which electromagnetic energy passes through a plane of cross-sectional area A at z is In ( z ) A The flux difference ; z z+Dz [ In ( z Dz ) In ] A Nonlinear Optics Lab. ( In A)Dz z Hanyang Univ. This difference gives the rate at which electromagnetic energy leaves the volume ADz, (un ADz ) ( In A)Dz t z 1 In In 0 : Equation of continuity un In /c c t z <Plane wave propagating in medium> The change of electromagnetic energy due to the medium should be considered. => The rate of change of upper(lower)-state population density due to both absorption and stimulated emission. (7.3.4a) => energy flux added to the field : (n )( N 2 N1 )hn (n ) In ( N 2 N1 ) 1 In (n ) In ( N 2 N1 ) c t z Nonlinear Optics Lab. Hanyang Univ. (7.4.19) : (n )(hn /c) BS (n ) hn 1 In B ( N 2 N1 ) S (n ) In c c t z (no degeneracies) hn g B N 2 2 N1 S (n ) In c g1 (degeneracies included) 2 A g N 2 2 N1 S (n ) In 8 g1 g (n ) N 2 2 N1 In g1 Define, gain coefficient, g(n) 2 A g N 2 2 N1 S (n ) g (n ) 8 g1 g (n ) N 2 2 N1 g1 Nonlinear Optics Lab. Hanyang Univ. In 1 In g (n ) In z c t Temporal steady state : 0 t In ( z ) In (0)e g (n ) z * g>0 when N 2 * If N 2 g1 N1 , g2 dIn g (n ) In dz : valid only for low intensity ( saturation effect, g=g(I)) g1 N1 : population inversion g2 g g g N 2 2 N 1 2 N1 2 N g1 g1 g1 2 A g 2 g (n ) NS (n ) 8 g1 N g2 (n )a (n ) The gain coefficient is identical, except g1 for its sign, to the absorption coefficient. Nonlinear Optics Lab. Hanyang Univ. 10.3 Feedback In practice, g~0.01 cm-1 if the length of active medium is 1 m. => A spontaneously emitted photon at one end of the active medium leads to a total of e0.01 x 100=e1=2.72 photons emerging at the other end. => The output of such a laser is obviously not very impressive. => Reflective mirrors at the ends of the active medium : Feedback. 10.4 Threshold In a laser there is not only an increase in the number of cavity photons because of stimulated emission, but also a decrease because of loss effects. (Loss effects : scattering, absorption, diffraction, output coupling) In order to sustain laser oscillation the stimulated amplification must be sufficient to overcome the losses. Nonlinear Optics Lab. Hanyang Univ. <Threshold condition> Absorption and scattering within the gain medium is quite small compared with the loss occurring at the mirrors of the laser. => Consider only the losses associated with the mirrors. r t s 1 where, r : reflection coefficient t : transmission coefficient s : fractional loss At the mirror at z=L and 0 ; In( ) ( L) r2 In( ) ( L) In( ) (0) r1 In( ) (0) Nonlinear Optics Lab. Hanyang Univ. In steady state (or CW operation), g(n) : constant dIn( ) g (n ) In( ) dz dIn( ) g (n ) In( ) dz In( ) ( z ) In( ) (0)e g (n ) z In( ) ( z ) In( ) ( L)e g (n )( Lz ) Amplification condition : In( ) (0) after one round trip must be higher than the initial In( ) (0) In( ) (0) r1 In( ) (0) r1[e g (n ) L In( ) ( L)] r1e g (n ) L [r2 In( ) ( L)] r1r2 e g (n ) L [ In( ) (0)e g (n ) L ] r1r2e 2 gL 1 [r1r2 e 2 g (n ) L ]In( ) (0) In( ) (0) Nonlinear Optics Lab. Hanyang Univ. Threshold gain, gt gt 1 1 1 ln ln( r1r2 ) 2L r1r2 2L * In the case of high reflectivity, r1r2 1, and ln(1-x)-x gt 1 (1r1r2 ) (high reflectivi ties, r1r2 0.9) 2L * If the “distributed losses” (losses not associated with the mirrors) are included, g t 1 ln( r1r2 ) a 2L where, a : effective loss per unit length Nonlinear Optics Lab. Hanyang Univ. Example) He-Ne laser, L=50 cm, r1=0.998, r2=0.980 gt 1 ln[( 0.998)(0.980)]cm 1 2(50) 2.2 10 4 cm 1 Threshold population inversion ; 2 A g2 g (n ) N N1 S (n ) 2 8n 2 g1 g g 2 8n 2 gt DN t N 2 N1 2 t g1 AS (n ) (n ) A1.4106 sec 1 at 632.8 nm 1 T 1/2 T ~400K, M Ne 20 amu n D 2.1510 MHz 1500 MHz M 4 1 (8 )( 2.210 cm ) DN t (632810 8 cm) 2 (1.4106 sec 1 )(6.310 10sec) 6 1.6109 atoms /cm3 DN t 1.6 109 1 3 10 6 (very small !) 15 N 4.8 10 Nonlinear Optics Lab. Hanyang Univ. 10.5 Rate Equations for Photons and Populations Time-dependent phenomena ? 1) Gain term (stimulated emission or absorption) In( ) 1 In( ) g (n ) In( ) z c t In( ) 1 In( ) g (n ) In( ) z c t () () 1 () () ( In In ) ( In In ) g (n )( In( ) In( ) ) z c t () In many lasers there is very little gross variation of either In( ) or In with z. => d () ( In In( ) ) cg (n )( In( ) In( ) ) dt * l<L (l : gain medium length, L : cavity length) d () cl (10.5.4b) ( In In( ) ) g (n )( In( ) In( ) ) dt L Nonlinear Optics Lab. Hanyang Univ. 0 z 2) Loss term (output coupling, absorption/scattering at the mirrors) By the output coupling, a fraction 1-r1r2 of intensity is lost per round trip time 2L/c. d ( ) () c ( In In ) (1r1r2 )( In( ) In( ) ) dt 2L (10.5.8) From (10.5.4b), (10.5.8), and put In In( ) In( ) : total intensity dIn cl c g (n ) In (1 r1r2 ) In dt L 2L or photon number, qn In dqn cl c g (n )qn (1r1r2 )qn dt L 2L cl cl g (n )qn g t qn L L Nonlinear Optics Lab. Hanyang Univ. dIn cl 2 A c If g1=g2, ( N 2 N1 ) S (n ) In (1 r1r2 ) In dt L 8 2L cl c (n )( N 2 N1 ) In (1 r1r2 ) In L 2L Coupled equations for the light and the atoms in the laser cavity including pumping effect : dN1 1 N1 AN 2 g (n )n dt dN 2 (2 A) N 2 g (n )n K dt dn cl c g (n )n (1 r1r2 )n dt L 2L Nonlinear Optics Lab. Hanyang Univ. 10.7 Three-Level Laser Scheme 1) Two-level laser scheme is not possible. Neglecting 1, 2 in (7.3.2) => N 2 () N N : can’t achieve the population inversion A21 2 2 2) Three-level laser scheme (10.5.14) => P : pumping rate dN1 PN1 dt pumping dN1 PN1 21 N 2 n ( N 2 N1 ) dt dN 2 PN1 21 N 2 n ( N 2 N1 ) dt dn cl c g (n )n (1r1r2 )n dt L 2L dN dN 2 dN 3 1 PN1 dt pumping dt pumping dt pumping Nonlinear Optics Lab. Hanyang Univ. <Threshold pumping> for the steady-state operation i) Near threshold the number of cavity photons is small enough that stimulated emission may be omitted from Eq. (10.7.4) ii) Steady-state : N 1 N 2 0 P N 2 N1 21 And, N1 N 2 NT : total population is conserved N1 21 NT P21 P N2 NT P 21 N 2 N1 # Positive (steady-state) population inversion : P21 # Threshold pumping power : P 21 NT P 21 Pmin 21 h n P Pwr hn 31PN1 31 21 N T 12 21N T hn 31 V P 21 Nonlinear Optics Lab. Hanyang Univ. 10.8 Four-Level Laser Scheme Lower laser level is not the ground level : The depletion of the lower laser level obviously enhances the population inversion. Population rate equations : dN 0 PN 0 10 N1 dt dN1 10 N1 21N 2 (n )( N 2 N1 )n dt dN 2 PN 0 21N 2 (n )( N 2 N1 )n dt Nonlinear Optics Lab. Hanyang Univ. N 0 N1 N 2 constant NT Steady-state solutions : 1021 N0 NT 1021 10 P 21P Population inversion : 21P N1 NT 1021 10 P 21P N2 N 2 N1 10 P NT 1021 10 P 21P P(10 21 ) N T 1021 10 P 21P # Positive inversion : 10 21 lower level decays more rapidly than the upper level. If 10 21, P P N 2 N1 N 2 NT P 21 Nonlinear Optics Lab. Hanyang Univ. 10.9 Comparison of Pumping Requirements for Three and Four-Level Lasers 1) Threshold pumping rate, Pt (10.7.9) => ( Pt ) threelevel laser NT DN t 21 NT DN t (10.8.7), (10.8.6) => ( Pt ) four level laser DN t 1 ( Pt ) threelevellaser NT DN t ( Pt ) four levellaser DN t 21 NT DN t 2) Threshold pumping power, (Pwr)t 1 (Pwr )t hn 31NT 21 V threelevellaser 2 (10.7.15) => (Pwr )t hn 30DN t 21 V four level laser (( Pwr ) t /V ) four levellaser 2n 30DN t (( Pwr ) t /V ) threelevellaser n 31 NT Nonlinear Optics Lab. Hanyang Univ. 10.11 Small-Signal Gain and Saturation For the three-level laser scheme, steady-state solution including the stimulated emission term ; N 2 N1 ( P 21 ) NT P 21 2 n Gain coefficient (assuming g1=g2), g (n ) (n )( P21 ) NT 1 fn (n ) P21 2 (n )n : A large photon number, and therefore a large stimulated emission rate, tends to equalize the populations N1 and N 2 . In this case, the gain is said to be “saturated.” <Microscopic view of the gain saturation> As the cavity photon number increased, the stimulated absorption as well as the stimulated emission increased. => The lower level’s absorption rate is exactly equal to the upper level’s emission rate in the extreme limit. The gain is zero. Nonlinear Optics Lab. Hanyang Univ. <Small signal gain / Saturation flux> g (n ) (n )( P 21 ) NT P 21 1 1 [2 (n )n /( P 21 )] g 0 (n ) 1 n / nsat Where we define, Small signal gain as (n )( P 21 ) NT g 0 (n ) P 21 Saturation flux as nsat P 21 2 (n ) * The larger the decay rates, the larger the saturation flux. * The saturation flux Stimulated emission rate : The average of the upper- and lower-level decay rates. Nonlinear Optics Lab. Hanyang Univ. <Gain width> When the absorption lineshape is Lorentzian, 1 (n ) (n 21 ) (n 21 n ) 2 /(n 21 ) 2 1 * Small signal gain width : Dn g n 21 (10.11.3) => g (n ) g 0 (n 21 ) 1 (n 21 n ) 2 /(n 21 ) 2 1 (n / nsat21 ) where, g 0 (n 21 ) (n 21 )( P 21 ) NT P 21 : Line-center small signal gain * Power-broadened gain width : 1/ 2 n Dn g n 21 1 sat n 21 Nonlinear Optics Lab. Hanyang Univ. P21 4 2n 21 n 21 2 ( P21 ) n 21 2 (n 21 ) A sat : Line-center saturation flux is directly proportional to the transition linewidth. Nonlinear Optics Lab. Hanyang Univ. 10.12 Spatial Hole Burning In most laser, we have standing waves rather than traveling waves. => Cavity standing wave field is the sum of two oppositely propagating traveling wave fields ; E ( z, t ) E0 cos t sin kz 12 E0 [sin( kz t ) sin( kz t )] E ( z , t ) E ( z , t ) where, E ( z, t ) 12 E0 sin( kz t ) The time-averaged square of the electric field gives a field energy density : hn ( ) 0 2 n E0 c 8 => Total photon flux, n 2[n( ) n( ) ] sin 2 kz In hnn In 2[ In( ) In( ) ] sin 2 kz Nonlinear Optics Lab. Hanyang Univ. (10.11.3) => g (n ) g 0 (n ) 1 2[(n( ) n( ) ) / nsat ] sin 2 kz Nonlinear Optics Lab. Hanyang Univ.
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