Globalisation and Pollution: Tele-connecting Local Primary PM2.5 Emissions to Global Consumption Jing Meng1,2, Junfeng Liu1, * , Yuan Xu3, Dabo Guan4, Zhu Liu5, Ye Huang1,6, and Shu Tao† 1 Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China 2 School of Environmental Sciences, University of East Anglia, Norwich, NR4 7JT, UK 3 Department of Geography and Resource Management & Institute of Environment, Energy and Sustainability, the Chinese University of Hong Kong, Hong Kong, China 4 School of International Development, University of East Anglia, Norwich, NR4 7TJ, UK 5 Resnick Sustainability Institute, California Institute of Technology, Pasadena, California 91125, USA 6 Laboratoire des Sciences du Climat et de l’Environnement, Commissariat à l'Energie Atomique-Centre National de la Recherche Scientifique-Université de Versailles Saint-Quentinen- Yvelines, Centre d'Etudes Orme des Merisiers, 91191 Gif sur Yvette, France * Corresponding author: Email: [email protected] Tel.:+86 (0)10 6275 7852 Caption Table S1. Definition of regions. Table S2. Definition of sectors. Table S3. Produced, consumed and traded PM2.5 emissions. Table S4. Budget of average primary fine aerosol concentrations from inter-continental transport of aerosols from each source region to each receptor region, contributions of a region on itself (referred to ‘domestic’) are shown in bold: (a) induced by production of source region [Unit: μg∙m-3]; (b) induced by consumption of source region [Unit: μg∙m-3]; (c) the ratio concentrations induced by consumption to production. Figure S1. Distribution of consumption-based PM2.5 emissions (FCr) in 2007 by mass of emissions in the region. Figure S2. PM2.5 emissions embodied in imports and exports of the largest net importing/exporting countries/regions. Intermediate goods (gray) are those used by industries in the importing country to further processing and meet consumer demand for domestic goods. Supporting method Bridging PKU-inventory and GTAP classifications Table S1. Definition of regions. Number Code Description Member Countries 1 AUS Australia 2 3 NZL XOC New Zealand Rest of Oceania 4 5 6 7 8 9 10 CHN HKG JPN KOR MNG TWN XEA China Hong Kong Japan Korea Republic of Mongolia Taiwan Rest of East Asia 11 12 13 KHM IDN LAO 14 15 16 17 18 19 MYS PHL SGP THA VNM XSE 20 21 22 23 24 25 26 27 BGD IND NPL PAK LKA XSA CAN USA Cambodia Indonesia Lao People's Democratic Republic Malaysia Philippines Singapore Thailand Viet Nam Rest of Southeast Asia Bangladesh India Nepal Pakistan Sri Lanka Rest of South Asia Canada United States of America Australia, Cocos (Keeling) Islands, Christmas Island, Heard Island and McDonald Islands, Norfolk Island New Zealand American Samoa, Cook Islands, Fiji, Micronesia Federated States of, Guam, Kiribati, Marshall Islands, Northern Mariana Islands, New Caledonia, Niue, Nauru, Palau, Papua New Guinea, French Polynesia, Solomon Islands, Tokelau, Tonga, Tuvalu, Vanuatu, Wallis and Futuna, Samoa, Pitcairn, United States Minor Outlying Islands China Hong Kong Japan The Korea Republic of Mongolia Taiwan Macao, Korea Democratic Peoples Republic of Cambodia Indonesia Lao People's Democratic Republic Malaysia Philippines Singapore Thailand Viet Nam Brunei Darussalam, Myanmar, Timor Leste Bangladesh India Nepal Pakistan Sri Lanka Afghanistan, Bhutan, Maldives Canada United States of America Number Code Description Member Countries 28 29 MEX XNA 30 31 ARG BOL Mexico Bermuda, Greenland, Saint Pierre, and Miquelon Argentina Bolivia, the Plurinational Republic of 32 33 34 35 36 37 38 39 40 BRA CHL COL ECU PRY PER URY VEN XSM Mexico Rest of North America Argentina Bolivia, the Plurinational Republic of Brazil Chile Colombia Ecuador Paraguay Peru Uruguay Venezuela Rest of South America 41 42 43 44 45 46 47 CRI GTM HND NIC PAN SLV XCA 48 XCB Costa Rica Guatemala Honduras Nicaragua Panama El Salvador Rest of Central America Caribbean 49 50 51 52 53 54 55 56 AUT BEL CYP CZE DNK EST FIN FRA Austria Belgium Cyprus Czech Republic Denmark Estonia Finland France Brazil Chile Colombia Ecuador Paraguay Peru Uruguay Venezuela Falkland Islands (Malvinas), French Guiana, Guyana, Suriname, South Georgia and the South Sandwich Islands Costa Rica Guatemala Honduras Nicaragua Panama El Salvador Belize Aruba, Anguilla, Netherlands Antilles, Antigua & Barbuda, Bahamas, Barbados, Cuba, Cayman Islands, Dominica, Dominican Republic, Grenada, Haiti, Jamaica, Saint Kitts and Nevis, Saint Lucia, Montserrat, Puerto Rico, Turks and Caicos Islands, Trinidad and Tobago, Saint Vincent and the Grenadines, Virgin Islands British, Virgin Islands U.S. Austria Belgium Cyprus Czech Republic Denmark Estonia Finland, Aland Islands France, Guadeloupe, Martinique, Reunion Number Code Description Member Countries 57 58 59 60 61 62 63 64 65 66 67 68 69 70 71 72 73 74 75 76 77 78 79 80 81 82 83 84 DEU GRC HUN IRL ITA LVA LTU LUX MLT NLD POL PRT SVK SVN ESP SWE GBR CHE NOR XEF ALB BGR BLR HRV ROU RUS UKR XEE Germany Greece Hungary Ireland Italy Latvia Lithuania Luxembourg Malta Netherlands Poland Portugal Slovakia Slovenia Spain Sweden United Kingdom Switzerland Norway, Svalbard and Jan Mayen Iceland, Liechtenstein Albania Bulgaria Belarus Croatia Romania Russian Federation Ukraine The Moldova Republic of 85 XER Germany Greece Hungary Ireland Italy Latvia Lithuania Luxembourg Malta Netherlands Poland Portugal Slovakia Slovenia Spain Sweden United Kingdom Switzerland Norway Rest of EFTA Albania Bulgaria Belarus Croatia Romania Russian Federation Ukraine Rest of Eastern Europe Rest of Europe 86 87 88 KAZ KGZ XSU 89 90 91 92 ARM AZE GEO BHR Kazakhstan Kyrgyzstan Rest of Former Soviet Union Armenia Azerbaijan Georgia Bahrain Andorra, Bosnia, and Herzegovina, Faroe Islands, Gibraltar, Monaco, Macedonia the former Yugoslav Republic of, San Marino, Serbia, Guernsey, Isle of Man, Jersey, Montenegro, Holy See (Vatican City State) Kazakhstan Kyrgyzstan Tajikistan, Turkmenistan, Uzbekistan Armenia Azerbaijan Georgia Bahrain Number Code Description Member Countries 93 IRN The Iran Islamic Republic of 94 95 96 97 98 99 100 ISR KWT OMN QAT SAU TUR ARE 101 XWS The Iran Islamic Republic of Israel Kuwait Oman Qatar Saudi Arabia Turkey United Arab Emirates Rest of Western Asia 102 103 104 105 EGY MAR TUN XNF Egypt Morocco Tunisia Rest of North Africa 106 107 108 109 110 111 112 113 114 115 BEN BUF CMR CIV GHA GUI NGA SEN TOG XWF Benin Burkina Faso Cameroon Cote d'Ivoire Ghana Guinea Nigeria Senegal Togo Rest of Western Africa 116 XCF Central Africa 117 XAC South Central Africa 118 119 120 121 122 123 124 ETH KEN MDG MWI MUS MOZ RWA Ethiopia Kenya Madagascar Malawi Mauritius Mozambique Rwanda Israel Kuwait Oman Qatar Saudi Arabia Turkey United Arab Emirates Iraq, Jordan, Lebanon, Palestinian Territory Occupied, Syrian Arab Republic, Yemen Egypt Morocco Tunisia Algeria, Libyan Arab Jamahiriya, Western Sahara Benin Burkina Faso Cameroon Cote d'Ivoire Ghana Guinea Nigeria Senegal Togo Cape Verde, Gambia, Guinea-Bissau, Liberia, Mali, Mauritania, Niger, Saint Helena, Ascension and Tristan Da Cunha, Sierra Leone Central African Republic, Congo, Gabon, Equatorial Guinea, Sao Tome and Principe, Chad Angola, Congo the Democratic Republic of the Ethiopia Kenya Madagascar Malawi Mauritius Mozambique Rwanda Number Code Description Member Countries 125 TZA Tanzania United Republic of 126 127 UGA ZMB Tanzania United Republic of Uganda Zambia 128 129 ZWE XEC 130 131 132 133 134 BWA NAM ZAF XSC XTW Zimbabwe Rest of Eastern Africa Botswana Namibia South Africa Customs Union Rest of the World Zimbabwe Burundi, Comoros, Djibouti, Eritrea, Mayotte, Sudan, Somalia, Seychelles Botswana Namibia South Africa Lesotho, Swaziland Antarctica, French Southern Territories, Bouvet Island, British Indian Ocean Territory Uganda Zambia Table S2. Definition of sectors. Number Sector Category 1 Paddy rice Agriculture 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 Wheat Cereal grains nec Vegetables, fruit, nuts; Oil seeds Sugarcane, sugar beet Plant-based fibers Crops nec Cattle, sheep, goats, horses Animal products nec Raw milk Wool, silk-worm cocoons Forestry Fishing Coal Oil Gas Minerals nec Meat: cattle, sheep, goats, horses Meat products nec Vegetable oils and fats Dairy products Processed rice Sugar Food products nec Beverages and tobacco products Textiles Wearing apparel Leather products Wood products Paper products, publishing Petroleum, coal products Chemical, rubber, plastic products Mineral products nec Ferrous metals Metals nec Metal products Motor vehicles and parts Transport equipment nec Electronic equipment Machinery and equipment nec Mining Light Manufacting Petroleum, coal products Chemical, rubber, plastic productsproducts Mineral Metal products Equipment Manufacturing 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 Manufactures nec Electricity Gas manufacture, distribution Water collection, purification, and distribution Construction Trade Transport nec Sea transport Air transport Communication Financial services nec Insurance Business services nec Recreation and other services Public Administration, Defense, Health, Education Dwellings Power generation Construction Non-transport Services Transport Non-transport Services Table S3. Produced, consumed and traded PM2.5 emissions. Number Region 1 2 3 Australia New Zealand Rest of Oceania The mainland of China Hong Kong Japan Korea Mongolia Taiwan Rest of East Asia Cambodia Indonesia Lao People’s Democratic Republic Malaysia Philippines Singapore Thailand Viet Nam Rest of Southeast Asia Bangladesh India Nepal Pakistan Sri Lanka Rest of South Asia Canada United States of America Mexico Rest of North America Argentina Bolivia 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 Production based Emissions (Gg) Consumption based Emissions (Gg) Emission embodied in exports (Gg) Emission Embodied in imports (Gg) 114.5 12.4 22.9 173.4 24.5 16.8 48.6 4.2 11.2 107.5 16.4 5.1 9371.7 6947.7 2717.0 293.0 0.0 477.0 174.6 11.2 0.0 80.3 725.2 294.6 10.4 66.7 0.0 166.9 73.6 3.4 0.0 80.3 415.1 193.6 2.6 66.7 123.3 91.8 42.7 11.2 22.6 425.4 25.1 400.6 4.3 105.2 6.7 80.4 34.0 28.8 7.5 2.2 113.3 116.1 4.8 259.3 231.2 93.4 118.1 43.2 189.3 187.2 72.2 28.9 3.4 128.0 93.8 52.4 30.9 41.7 58.0 49.8 96.3 73.6 32.5 9.8 164.3 3060.3 29.8 251.7 20.0 179.6 2782.3 32.7 256.4 29.7 10.4 482.8 2.2 32.2 4.3 25.6 204.8 5.1 36.9 13.9 30.4 29.7 10.1 9.5 147.8 219.6 76.5 148.2 1217.2 2275.4 220.2 1278.5 183.1 221.3 54.6 92.8 19.6 12.3 10.4 3.1 253.1 14.0 98.3 13.7 183.0 3.2 28.2 3.0 32 33 34 35 36 37 38 39 678.0 40.0 53.4 21.0 27.3 36.3 10.0 72.0 567.6 43.4 64.4 27.6 18.3 43.6 8.5 78.1 211.2 21.8 13.6 4.2 13.0 9.4 6.3 22.2 100.8 25.2 24.5 10.8 4.0 16.8 4.8 28.2 26.4 21.4 6.4 1.3 6.0 11.3 7.1 3.9 4.5 6.3 7.6 14.5 9.2 5.2 8.4 9.3 3.2 3.8 1.8 1.3 0.7 1.6 4.8 7.0 3.9 2.6 4.7 4.6 0.4 0.6 0.2 0.4 48 49 50 51 52 53 54 55 Brazil Chile Colombia Ecuador Paraguay Peru Uruguay Venezuela Rest of South America Costa Rica Guatemala Honduras Nicaragua Panama EI Salvador Rest of Central America Caribbean Austria Belgium Cyprus Czech Republic Denmark Estonia Finland 211.7 28.0 32.6 2.8 34.6 16.6 11.3 28.4 211.8 50.0 104.6 8.8 41.9 48.5 13.1 47.3 43.2 16.8 24.1 0.7 19.7 8.5 4.5 14.3 43.4 38.8 96.2 6.6 27.0 40.4 6.4 33.2 56 France 141.0 318.6 53.3 230.8 57 58 59 60 61 62 63 64 65 66 67 68 69 70 71 72 Germany Greece Hungary Ireland Italy Latvia Lithuania Luxembourg Malta Netherlands Poland Portugal Slovakia Slovenia Spain Sweden 197.0 33.5 18.7 10.4 112.9 6.8 15.9 3.2 0.4 30.0 149.5 21.0 27.8 5.8 124.3 28.8 474.9 92.7 31.5 33.9 316.2 12.7 20.3 7.4 2.7 97.9 157.8 43.5 26.1 11.3 276.3 57.9 100.6 7.8 10.2 5.2 42.5 3.5 7.8 2.5 0.2 20.8 56.3 7.4 16.8 3.2 40.2 17.1 378.5 67.0 23.0 28.7 245.7 9.5 12.2 6.7 2.6 88.6 64.6 29.9 15.1 8.8 192.2 46.2 40 41 42 43 44 45 46 47 73 74 75 76 77 78 79 80 81 82 83 84 85 86 87 88 89 90 91 92 93 94 95 96 97 98 99 100 101 102 103 104 105 106 107 108 United Kingdom Switzerland Norway Rest of EFTA Albania Bulgaria Belarus Croatia Romania Russian Federation Ukraine Rest of Eastern Europe Rest of Europe Kazakhstan Kyrgyzstan Rest of Former Soviet Union Armenia Azerbaijan Georgia Bahrain Iran, the Islamic Republic of Israel Kuwait Oman Qatar Saudi Arabia Turkey United Arab Emirates Rest of West Asia Egypt Morocco Tunisia Rest of North Africa Benin Burkina Faso Cameroon 105.4 377.4 37.1 309.1 12.8 10.2 1.4 3.4 36.5 56.8 11.5 70.7 52.0 39.2 4.7 7.0 32.7 37.4 19.3 79.8 6.6 5.9 0.7 0.9 17.8 40.0 4.3 22.7 45.7 34.9 3.9 4.5 14.0 20.7 12.1 31.8 907.6 791.4 339.6 223.4 357.4 166.0 239.8 48.4 4.1 7.2 2.2 5.2 67.2 202.5 7.9 67.6 183.0 7.6 19.6 68.9 3.5 20.0 49.5 3.2 67.4 53.6 29.4 15.6 3.3 13.1 4.7 1.7 5.1 22.1 8.3 5.7 1.5 3.2 2.3 0.9 3.3 12.2 5.9 4.9 246.7 297.9 43.0 94.2 19.1 14.9 8.7 16.1 87.8 342.8 40.1 37.3 20.6 29.4 153.0 385.6 8.1 4.1 2.3 6.5 23.6 88.6 29.1 26.5 14.2 19.9 88.8 131.3 34.7 165.1 8.4 138.8 254.5 207.7 107.5 60.6 302.0 97.5 38.6 256.0 104.4 24.4 85.9 18.7 25.9 40.0 25.6 11.8 112.4 130.8 31.3 49.7 7.0 9.2 9.1 8.7 10.1 9.3 5.3 1.3 2.8 7.1 2.3 3.0 109 110 111 112 113 114 115 116 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 Cote d'lvoire Ghana Guinea Nigeria Senegal Togo Rest of Western Africa Rest of Central Africa Rest of South Central Africa Ethiopia Kenya Madagascar Malawi Mauritius Mozambique Rwanda Tanzania, the United Republic of Uganda Zambia Zimbabwe Rest of Eastern Africa Botswana Namibia South Africa Rest of South the African Customs Union Rest of the world Total 4.8 15.3 15.2 59.5 15.7 4.4 8.3 25.5 13.7 73.1 15.6 6.4 1.7 3.5 3.4 22.6 5.7 2.9 5.2 13.8 1.9 36.1 5.7 4.9 34.6 45.0 9.9 20.3 12.7 18.7 4.1 10.2 21.5 29.3 9.0 16.8 25.0 21.6 53.9 50.6 2.2 10.0 8.6 32.3 25.6 47.7 39.8 5.1 12.5 10.1 1.9 6.5 8.7 13.0 0.9 3.9 1.3 9.1 10.5 2.5 2.2 3.7 6.4 2.8 18.3 20.2 5.5 7.4 103.6 6.5 22.5 88.5 9.2 16.0 19.0 3.2 12.3 3.9 5.9 5.8 19.4 35.7 4.1 20.4 4.9 3.8 617.4 11.5 8.1 376.8 2.3 2.4 294.2 8.9 6.6 53.7 4.9 3.7 2.2 0.9 0.0 0.0 0.0 0.0 24002.4 24002.4 7236.3 7236.3 Table S4. Budget of average primary fine aerosol concentrations from intercontinental transport of aerosols from each source region to each receptor region, contributions of a region on itself (referred to ‘domestic’) are shown in bold: (a) induced by production of source region [Unit: μg∙m-3]; (b) induced by consumption of source region [Unit: μg∙m-3]; (c) the ratio concentrations induced by consumption to production. (a) induced by production of source region [Unit: μg∙m-3] Source Region NA EU IN EA NA 0.349 0.001 0.001 0.012 Receptor Region EU IN 0.007 0.002 0.005 0.773 0.001 2.931 0.004 0.019 EA 0.002 0.008 0.070 4.263 (b) induced by consumption of source region [Unit: μg∙m-3] Source Region NA EU IN EA NA 0.299 0.017 0.001 0.013 Receptor Region EU IN 0.034 0.097 0.121 0.631 0.004 2.469 0.019 0.057 EA 0.428 0.383 0.044 4.094 (c) the ratio concentrations induced by consumption to production. Source Region NA EU IN EA NA 0.9 14 1 1 Receptor Region EU IN 5 40 27 0.8 7 0.8 5 3 EA 223 50 0.6 1 Gg/y Tg/y 0.01 0.02 0.03 0.04 0.05 0.1 0.5 1 2 3 4 5 >5 Figure S1. Distribution of consumption-based PM2.5 emissions (FCr) in 2007 by mass of emissions in the region. Figure S2. PM2.5 emissions embodied in imports and exports of the largest net importing/exporting countries/regions. Intermediate goods (gray) are those used by industries in the importing country to further processing and meet consumer demand for domestic goods. Bridging PKU-inventory and GTAP classifications Bridging the two databases was done by setting up concordance matrices between the 78 emission sources and each of GTAP’s countries’ sectors. Let C be such a concordance matrix, holding Cij=1 if PKU-inventory class I corresponds to GTAP sector j, as shown in Table S1. The original primary fuel type in GTAP database covers coal, oil, coal and oil products, and gas. As the emission factors of various types of fuel vary significant, the coal, oil, coal and oil products were split into seven types of fuel according to the energy statistics from International Energy Agency [1-5]. The coal consumption was divided into Briquettes, coke; Brown coal, peat; Hard coal, coking coal. The consumption of coal and oil products was divided into Heavy fuel oil; Gasoline, aviation fuel, kerosene; Liquefied Petroleum Gas. For some developing countries without country-specific energy statistics, the average proportion of different types of fuels of NON-OECD countries were used. Then the emissions from power generation were split into 2 sectors (Sector 4344 in Table S5) according to the sectors’ fuel consumption. For example, the emissions from coke used in power generation were C, the coke consumption in Sector 43 and Sector 44 was E1 and E2, then the emissions from coke comsumption in Sector 43 and Sector 44 was C * E1 / (E1 E 2) and C * E 2 / (E1 E 2) , respectively. Reference (1). IEA (2010) Energy Statistics of Non ‐ OECD Countries 2010: (Complete Edition ‐ ISBN 9789264084117). Sourceoecd Energy volume 2010(16):i-770(770). (2). IEA (2012) Energy Statistics of OECD Countries 2012: Complete Edition - ISBN 9789264173736. Sourceoecd Energy volume 2012(8):i-426(426). (3) IEA (2007) Energy Statistics of Non‐OECD Countries: 2004/2005: 2007 Edition (Complete Edition ‐ ISBN 9264027688). Source OECD Energy 2007(15):i-786. (4) IEA 2010) Energy Statistics of OECD Countries 2010: (Complete Edition ‐ ISBN 9789264084087). Sourceoecd Energy volume 2010(16):i-398. (5) IEA (2010) Energy Statistics of OECD Countries 2010: (Edition complète ‐ ISBN 9789264084094 ‐ Fr. à paraître). SourceOCDE Energie 2010(26):i-398.
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