Imaging of charge transport in CVD diamond

Detector Research at the University of Surrey
Dr Paul Sellin
Centre for Nuclear and Radiation Physics
Department of Physics
University of Surrey, Guildford
Paul Sellin
High-Z materials for room temperature gamma ray detectors
CdTe/CdZnTeX-ray
are the
most
mature efficiency
high-Z bulk materials for X-ray and gamma ray detectors:
photon
detection
Detection Efficiency (%)
100
Calculated for 500m thick material
single crystal HgI2
Si
GaAs
CdTe
HgI2
TlBr
10
www.realtimeradiography.com
1
50
100
150
200
250
300
350
400
450
500
Photon energy (keV)
CdTe and CdZnTe offer good spectroscopic performance
for X-rays and gammas
For higher photon energies very high-Z materials such as
mercuiric iodide (HgI2) are actively being developed
Paul Sellin
Cadmium Zinc Telluride for X-ray/gamma spectroscopy
CdZnTe material quality has improved recently, with various new suppliers in the
US/Canada, Europe and Japan:
 wafers of large single-crystal areas are available, with excellent charge transport
 High resistivity r=3x1011Wcm, and te=1.8x10-2 cm2/V
4x4 pixellated devices
have shown very good
resolution
 1.35% FWHM at
662 keV
Paul Sellin
‘Hexitec’ Basic Technology project
Surrey is one of the major members of the recent Hexitec Basic
Technology project – a £3M 4 year project
Project aim – development of CdZnTe pixel detectors for X-ray imaging




Manchester – detector applications
Durham – CdZnTe material growth
Surrey – Material and detector characterisation and prototyping
CCLRC RAL – Pixel detector fabrication
Paul Sellin
Synthetic diamond for detector applications
Single-crystal natural diamonds have been studied in the past for
detector applications – excellent electronic properties are seen in a tiny
number of gem stones.
P. Bergonzo et al, Dia Rel Mat 10 (2001) 631-638
Paul Sellin
Single-crystal CVD diamond detectors
Specialist applications of diamond detectors:
 as tissue-equivalent rad-hard detectors, eg megavoltage
therapy beams, neutrons
 detectors for very high temperature, high radiation environments
True single-crystal material removes charge trapping associated with grain boundaries:
 100% CCE demonstrated from alpha particles
 Extreme radiation hardness
 High mobility  very fast signals (~10ps timing resolution)
silicon detector
diamond detector
Paul Sellin
Ref: M. Pomorski et al, phys stat sol a 203 (2006) 3152-3160
Semiconducting polymer – a new radiation detector material?
Various candidate semiconducting polymers are of interest for radiation
detection applications, eg:
 Poly-acetylene
 PPV (poly-phenylene-vinylene)
These materials have the following properties:
 A ‘band gap’ energy low enough to give semiconducting properties
(eg. ~1.5 eV)
 High resistivity combined with reasonable charge transport:
 Electron and hole mobilities are low
 Carrier concentrations are low (<1014cm-3)  good depletion
thickness
 Sufficient radiation hardness
Potential Benefits:
 large area, low cost sensor technology
 fabrication onto flexible, complex geometry, substrates
 tissue equivalent for dosimetry applications
Paul Sellin
X-ray response from the PFO detector
X-ray response photocurrent was measured from the PFO device for dose
rates up to 18.5 mGy/s
Photocurrent (nA)
-50
-40
-30
-20
-10
0
0
0
-1
-1
-2
-2
-3
-3
-4
-4
No Dose
0.99 mGy/s
1.92 mGy/s
3.79 mGy/s
7.52 mGy/s
13.16 mGy/s
18.5 mGy/s
-5
-6
-5
-6
-7
-7
-50
-40
-30
-20
-10
Applied Voltage (V)
0
Corrected Photocurrent (nA)
Photocurrent vs dose rate gives the
detector sensitivity. For a 10m thick device:
~0.06 nC/mGy @ -10V
~0.24 nC/mGy @ -50V
Photocurrent vs bias voltage shows
an approximately linear increase
Dark current is ~0.8 nA @ -50V
4
-50V
3
2
1
-10V
0
0
4
8
12 Paul
16 Sellin 20
X-ray
Dose
Rate
(mGy/s)
X-ray
Dose
(mGy/s)
Other plastic dosimetry materials
Various organic and plastic bulk materials have been investigated since
Fowler’s work in the 1950’s
Early measurements investigated
X-ray induced photocurrents, and
showed long time transients
Recent data at Surrey on newer
material have studied dosimetry
response of thick (~mm) plastic
layers to 50 kV X-rays:
 signal-background ratio of
~500x
 ‘fast’ X-ray response of <100 ms
Paul Sellin
New MSc course in Radiation Detection and Instrumentation
A new MSc programme for September 2008 – exploring the operation,
characterisation and development of radiation detectors and
instrumentation
Application areas will include medical physics, dosimetry, particle physics,
synchrotrons, space science and homeland security
Core programme modules:
 Radiation Physics and Laboratories
 Radiation Measurement
 Detector Instrumentation
 Interfacing and Signal Processing
 Imaging and Remote Sensing
Applications modules:
 Particle Physics Detector Technology
 Astronomy Detector Technology
 Radiation Protection
 Medical applications of Ionising Radiation
www.ph.surrey.ac.uk/msc/rdi
Paul Sellin