Solar radiation tidal forcing of radon signals in subsurface air Steinitz, G., Piatibratova, O., Kotlarsky, P. Geological Survey of Israel, Jerusalem [email protected] Monitoring sites The reasoning Geophysical background High temporal resolution monitoring of radon, using alpha & gamma detectors, is carried out at several arrays located in arid southern Israel. Monitoring, at a resolution of 15-minutes, is conducted at depths ranging from 1.5 to 120 meter. • Dominance of solar tidal frequencies of annual, and daily scale • Annual modulation of the amplitude and phase of daily and sub daily tidal frequencies • Systematic multi-year variation of signal and periodic characteristics • Occurrence different locations, at depth to >100 meter • Similar phenomena in laboratory experiments of radon in confined air And • Negation of climatic influences • [Lack of gravity tidal frequencies] Signal types, periodicity, Solar tide components Period 24-, 12-hours 1. Daily signals Temporal phenomena encountered differ among sites, but have similar fundamental characteristics. Radon monitoring arrays along the Dead Sea Rift (DSR) Tidal component S1, S2 2. Multi-Day (non-periodic) 3. Annual radon 4. Semi-annual radon 5. Ternary annual radon 365.2 days 182.6 days 121.7 days 6. Multi-Year (non-periodic?) Rn Acronym DR MD SA SSA STA AR SAR TAR • Array of stations, along a 20 km sector • 1.5 m deep in unconsolidated gravel Solar irradiance related components - S1, S2 dominate = solar tide Southern Arava Elat Granite 80 S1 80 S1 60 40 S2 20 • Array of stations, 20 km sector • In Precambrian basement rocks • Depth 2 to +100 meter Roded 19W Day 4100-4700 60 S2 40 0 1 20 1 Granite; Elat; 54m Cycle / day gamma radiation emitted from radon in the tank air varies spatially and temporally. A 4-year time series shows 1999 200 2001 2003 2005 and S3. Periodicities indicative for diurnal gravity tide (O1, M2; Lunar influence) are clearly lacking. Profound 100 10000 17W S2 0 1 external geophysical influence is further indicated by compounded relations that occur as annual modulation of 2007 N2 2 2 NW Gulf Elat, Rn in seawater Shore gravel; 2m deep, 130 days the amplitude and phase of the diurnal constituents S1, S2 and S3. Historgram of values (17W, Gamma detector) Further insight is derived from the long term variations in time series from the geological environment and from 1.5e+5 Cycle / day Granite; Elat; 54m are dominated by periodicities of 24-, 12-, and 8-hours which are attributed to the Solar tidal constituents S1, S2, The multi-year rising trend observed at Experiment, 17W and Amram sites. The temporal pattern is measured by alpha and gamma detectors in Amram and in the Experiment. M2 Cycle / day Gravel; NW Dead Sea; 1.5m radon, the latter diffusing into the upper air volume from U bearing ground phosphorite (376 Kg). Alpha and multi-year and multi-day signals and especially periodic signals of annual and daily scale. The diurnal variations 0 0 phenomena at depth. 300 0 2 meter. A component of solar irradiation tide was suggested (References) as the driver of these periodic • Periodicity is forced by solar tide • A component of solar radiation? O1 S1 0 in the arid desert of southern Israel demonstrated that the periodic variations, are observed to a depth of >100 recording radon within a confined volume of Air. The setup consisted of an isolated volume (640 L) of air with Bias Counts Amram Amplitude • Depth: 1.2 m & 90 meter • Massive syenite GAV 400 E-3; Days 4356-4441 100 – multi-year, annual to daily and sub-daily duration. Analysis of extensive data sets from key sites 200 km apart Gravity tide - rare Amplitude Intraplate temporal variations composed of periodic and non-periodic signals spanning several orders of magnitude in time IMPLIES Periodograms of the diurnal components of radon signals in subsurface air Amplitude 21W by alpha and gamma activity during the decay of radon and its progeny. Radon in geogas exhibits systematic The issue of external forcing of radon signals was tested experimentally using alpha and gamma detectors MY NW Dead Sea 17W Radon (Rn-222) occurs at highly varying levels as a trace component in subsurface air (geogas). It is measured the experiment. In addition to the annual periodicity clear semiannual and ternary annual signals are 5000 demonstrated. They are attributed to the solar tidal constituents Sa, SSa and STa. 1.0e+5 Experimental replication Gamma-C Alpha-H Alpha-L Cycles Name Period (hr) Principal lunar declinational O1 25.82 0.9295 Solar diurnal S1 24.00 1.0000 0 Principal lunar M2 12.42 1.9324 Principal solar S2 12.00 2.0000 Counts 1e+5 2008 2009 2010 2011 2008 2009 2010 3e+5 Measured Long-term bias Annual Radon (AR) Long-term (MY) 5.0e+4 Day 2e+5 2500 3000 3500 4000 4500 5000 Elat Granite: 5500 • Measured pattern • Smoothed time series - AR signal and SAR signal as an asymmetry • Modulation of the residual time series - AR and SAR signal Roded: Annual variation of amplitude of the diurnal periodicities S1, S2 2011 2.5e+5 2004 2006 2008 2010 1999 200 14000 AR Alpha (BGO) Alpha-H Alpha-L (Rn source) 2.2e+5 1000 5600 5800 6000 6200 6400 6600 5600 6800 5800 6000 6200 6400 6600 6800 Day since 1.1.1992 Day since 1.1.1992 2003 2004 8000 30 SAR 20 10 0 0.000 5e+9 .005 .010 .015 .020 500 MS MD AR DR Gamma (BGO) AR Cycle/day 50 0 100 Year 2005 400 40 Amplitude 1100 100 10000 Amplitude Phosphorite 2002 2009 100 12000 2.3e+5 2007 60 50 1200 2005 S1 Amram 1300 2003 Counts/15-minute 2.4e+5 2001 150 S2 400 200 300 200 0 100 4e+9 PSD SSA (air) 2002 Alpha (counts) Metal tank, tight Alpha 1400 Gamma (counts) Counts/15-min Gamma 0 6000 Counts/15-minute Main components (Day-1) 3e+9 0 50 2e+9 SAR -200 1e+9 -100 0 4000 1360 2008 27.0 2009 2010 26.2 1355 1345 1335 1340 26.1 5650 5660 5670 5680 5690 1330 5700 C 26.8 2.405e+5 2.430e+5 5640 o 2008 26.0 1335 2.400e+5 1330 6020 6030 6040 6050 6060 26.6 6070 Day since 1.1.1992 1400 27.4 2.428e+5 o 2009 26.2 2010 2.425e+5 1390 1300 1200 Gamma-C Alpha-H Alpha-L Temperature 2.3e+5 27.2 Alpha Gamma 2.435e+5 1400 Gamma Alpha C 2.4e+5 1385 27.0 2.423e+5 25 5750 6000 6250 6500 4000 5000 6000 o C 10 2008 Spectral analysis: SA. SSA, STA periodicities 6750 80 2009 2010 2008 Alpha H 2009 2010 75 4 gamma-C 6430 6750 6760 6770 6780 6790 Day since 1.1.1992 6800 6810 CWT analysis: Annual modulation of the amplitude of DR signal (S1 and S2) occurs as a compounded feature 2 20 2500 0 0.00 0.01 0.02 0.03 0.04 0.05 Cycle/day Mean of two alpha detectors 75 1 Gamma C 10 5 2 0 14 Alpha L 2005 2006 2007 2008 2009 S1 50 2001 2003 2005 2007 6 25 2 Cycle/day Spectra of alpha and gamma measurements (Experiment - 4yrs) show clear peaks characteristic for annual and semiannual periodicity (365.2 and 182.6 cycle/day). 0 5500 0 4800 5000 2004 2005 2006 S2 2007 2008 1000 500 0 6 GAV: Annual modulation of the amplitude of the diurnal periodicities S1 and S2 150 S2 3000 4000 5000 Days since 1.1.1992 6000 S1 100 50 15 0 2003 10 2004 2005 2006 2007 2008 REFERENCES 4500 0 6000 6500 Days since 1.1.1992 5500 S1 S2 S3 5000 5500 6000 6500 Days since 1.1.1992 0 0.05 S1 S2 0 2 4 0.04 4600 4 6 0.03 2 2 8 0.02 4400 5 10 25 2003 2009 4 0 6 12 0.01 4200 0 50 0.00 4000 7 Amplitude (x1000) Day since 1.1.1992 6420 2004 6 Phase (rad) 6410 3800 GAV: Daily averages at 1.2 meter 4 5 Amplitude (counts x103) 6400 1999 Phase 60 Day since 1.1.1992 3600 Days since 1.1.1992 6 Amplitude Amplitude 6390 26.8 3400 6000 Days since 1.1.1992 15 Amplitude 6380 1375 5000 diurnal periodicities S1, S2 40 2.420e+5 6740 4000 7000 Amplitude and phase are extracted by applying FFT windowing, where each point represents a (consecutive) 21-day time interval. 5000 26.0 3000 Roded: Multi-year variation of phase of the 20 1380 2.430e+5 6370 0 Spectra for alpha and gamma measurements (9 yrs) show clear peaks characteristic for annual and semi-annual periodicity (365.2 and 182.6 cycle/day). Smoothed pattern of • AR & SAR signals • (maxima of T – lags) 1100 o C Counts/15-min (alpha) 26.3 2.410e+5 Counts/15-min (gamma-C) 2.435e+5 C Day 30 1400 Alpha 1350 26.4 o Gamma 2007 Alpha Gamma 1355 .020 Cycle/day 2011 2.440e+5 .015 Daily mean (counts) 2.415e+5 26.5 .010 amplitude 30 days Semi-annual radon signals are superimposed on the annual signal recorded by alpha-L and gamma-C. A similar semi-annual pattern is absent in the ambient temperature. .005 phase (rad) Gamma-C Alpha-H Alpha-L Temperature Amplitude (x1000) Nuclear radiation - summer peak times of annual signal 0.000 6000 6500 Days since 1.1.1992 Annual modulation of the periodic components (amplitude & phase) of the DR signal in Experiment. • Annual variation of the amplitudes of the daily components is dissimilar for gamma and alpha time series - showing opposite temporal patterns! 21W: Annual and semi-annual modulation of the amplitude of the diurnal periodicities S1 and S2 1. Steinitz, G., O. Piatibratova, and S. M. Barbosa, 2007. Radon daily signals in the Elat Granite, southern Arava, Israel, J. Geophys. Res., 112, B10211, doi:10.1029/2006JB004817. 2. Steinitz, G., Piatibratova, O., 2010a. Radon signals in the Gavnunim intrusion, Makhtesh Ramon, Israel. Geophys. J. Int. 180, 651–665. 3. Steinitz, G. and Piatibratova, O., 2010. Radon signals at the Roded site, Southern Israel, Solid Earth, 1, 99-109, doi:10.5194/se-1-99-2010.
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