Nature of low-energy dipole states in exotic nuclei Xavier Roca-Maza Università degli Studi di Milano, Via Celoria 16, I-20133, Milano SPES One-day Workshop on "Collective Excitations of Exotic Nuclei" December 9, 2013, Milano 1 Motivation Giant Resonances are collective excitations of atomic nuclei. The measurement of such (high-energy) excitations has allowed us to constraint many properties of the nuclear equation of state Giant Monopole Resonance → K0 [G. Colò, N. Van Giai, J. Meyer, K. Bennaceur and P. Bonche, Phys. Rev. C 70, 024307 (2004)] Giant Dipole Resonance → S2 (ρ = 0.1 fm−3 ) [Luca Trippa, Gianluca Colò, and Enrico Vigezzi, Phys. Rev. C 77, 061304(R) (2008)] Giant Quadrupole Resonance → m∗ [“Nuclear Structure”, Bohr & Mottelson → Ex = p 2m/m∗ hω] Experiments on Giant Resonances constitute a basic tool for the study of fundamental properties of the nuclear strong interaction. 2 Motivation What is the Pygmy Dipole Strength (PDS)? Giant Dipole Resonance neutron-capture rates in the r−processes† since the energy window for both observables is similar if collective, it may be correlated with the slope of the symmetry energy (L): a basic property of the nuclear EoS that impacts on a variety of physical systems: from the very big (neutron stars) to the very small (neutron skin) Pygmy dipole ◮ Low-energy peak in the dipole response of neutron rich (exotic) nuclei It might be relevant in ... ◮ The PDS seems to appear in certain models as a coherent excitation (resonance), and not in others (shell effect) † β−decay rates and radiative neutron capture. In the latter, σ may increase due to the low-energy E1 enhancement when approaching the neutron drip line. [A. C. Larsen and S. Goriely, PRC 82, 014318 (2010)] 3 Motivation What is the Pygmy Dipole Strength (PDS)? Low-energy peak in the dipole response of neutron rich (exotic) nuclei Equation of state for It uniform might benuclear relevantmatter in ... Giant Dipole Resonance neutron-capture rates in the r−processes† since the energy window for both observables is similar if collective, it may be correlated with the slope of the symmetry energy (L): a basic property of the nuclear EoS 2 e(ρ, δ) =on e(ρ, δ = 0) + + Osystems: δ4 withfrom the that impacts a variety ofS(ρ)δ physical ρn − ρp very big (neutron stars) δ = to the very small (neutron skin) Pygmy dipole ◮ ◮ ρn + ρp 2 The PDS seems toρ − appear in certain as a coherent ρ0 ρ − ρ0models 3 + K + O (ρ − ρ ) S(ρ) = J + L sym 0 excitation (resonance), (shell effect) 3ρ0 and not in others 3ρ0 † β−decay rates and radiative neutron capture. In the latter, σ may increase due to the low-energy E1 enhancement when approaching the neutron drip line. [A. C. Larsen and S. Goriely, PRC 82, 014318 (2010)] 3 Motivation What is the Pygmy Dipole Strength (PDS)? Giant Dipole Resonance Low-energy peak in the dipole response of neutron rich (exotic) nuclei It might be relevant in ... neutron-capture rates in the r−processes† since the energy window for both observables is similar ◮ if collective, it may be correlated with the slope of the symmetry energy: a basic property of the nuclear EoS that impacts on a variety of physical systems: from the very big (neutron stars) to the very small (neutron skin) The PDS seems to appear in certain models as a coherent excitation (resonance), and not in others (shell effect) Pygmy dipole † ◮ β−decay rates and radiative neutron capture. In the latter, σ may increase due to the low-energy E1 enhancement when approaching the neutron drip line. [A. C. Larsen and S. Goriely, PRC 82, 014318 (2010)] 4 Motivation: experimentally, the PDS splits into two parts ... Alpha-gamma coincidence experiments allow the separation of E1 excitations in ... J. Endres et al. Phys. Rev. Lett. 105, 212503 (2010) ◮ one part excited via (α, α′ γ) [dominant isoscalar excitation where the probe mainly interacts with the nuclear surface] and (γ, γ′ ) ◮ and the other only via (γ, γ′ ) [dominant isovector excitation where the probe interacts with the whole nucleus] 5 Motivation: bibliography (non-exhaustive list) There is a great interest on the PDS .... ... on experiment ◮ Experimental Studies of the Pygmy Dipole Resonance by D. Savran, T. Aumann and A. Zilges, Prog. Part. Phys. and Nucl. 70 210-245 (2013). ◮ Evidence for Pygmy and Giant Dipole Resonances in 130 Sn and 132 Sn by P. Adrich et al., Phys. Rev. Lett. 95, 132501 (2005). Concentration of electric dipole strength below the neutron separation energy in N=82 nuclei by A. Zilges et al., Phys. Lett. B542, 43 (2002). ◮ ◮ ◮ The photoresponse of stable N=82 nuclei below 10 MeV by S. Volz et al., Nucl. Phys. A779, 1 (2006). ◮ Search for the Pygmy Dipole Resonance in 68 Ni at 600 MeV/nucleon by O. Wieland et al., Phys. Rev. Lett. 102, 092502 (2009). Nature of Low-Energy Dipole Strength in Nuclei: The Case of a Resonance at Particle Threshold in 208Pb by N. Ryezayeva et al., Phys. Rev. Lett. 89, 272502 (2002). ... and theory ◮ Multiphonon excitations and pygmy resonances in tin isotopes by E.G. Lanza, F. Catara, D. Gambacurta M.V. Andres and Ph. Chomaz, Phys. Rev. C 79 054615 (2009) and Pygmy dipole resonances in the tin region by N. Tsoneva and H. Lenske, Phys. Rev. C 77 024321 (2008). ◮ Exotic modes of excitation in atomic nuclei far from stability by Nils Paar, Dario Vretenar, Elias Khan and Gianluca Colò, Rep. Prog. Phys. 70 691 (2007). ◮ Constraints on the symmetry energy and neutron skins from pygmy resonances in 68 Ni and 132 Sn by Andrea Carbone, Gianluca Colò, Angela Bracco, Li-Gang Cao, Pier Francesco Bortignon, Franco Camera, and Oliver Wieland, Phys. Rev. C 81, 041301 (2010). ◮ Nuclear symmetry energy and neutron skins derived from pygmy dipole resonances by A. Klimkiewicz et al., Phys. Rev. C 76, 051603(R) (2007). ◮ Low-lying dipole response: Isospin character and collectivity in 68 Ni, 132 Sn, and 208 Pb by X. Roca-Maza, G. Pozzi, M. Brenna, K. Mizuyama, and G. Colò, Phys. Rev. C 85, 024601 (2012). ◮ Pygmy resonances and neutron skins by J. Piekarewicz, Phys. Rev. C 83, 034319 (2011). 6 Contents Microscopic analysis of the PDS: model dependence and sensitivity to the symmetry energy We study the PDS within the self-consistent HF+RPA approach in the exotic 68 Ni and 132 Sn and the stable 208 Pb nuclei. For that, we use three Skyrme interactions with very different isovector properties (L ranges from 40 MeV to 100 MeV). We focus on: ◮ RPA and unperturbed dipole strength. ◮ the transition densities. ◮ the isoscalar or isovector nature. ◮ the most relevant p-h contributions. X. Roca-Maza, G. Pozzi, M.Brenna, K. Mizuyama and G. Colò, Phys. Rev. C 85 024601 (2012) 7 Contents Microscopic analysis of the PDS: model dependence and sensitivity to the symmetry energy We study the PDS within the self-consistent HF+RPA L estimates approach in the exotic 68 Ni and 132 Sn and the stable 208 Pb nuclei. For that, we use three Skyrme interactions with very different isovector properties (L ranges from 40 MeV to 100 MeV). We focus on: χ Lagrangian and Q. Montecarlo Neutron-Star Observations p & α scattering charge ex. Antiprotonic Atoms Neutron Matter Kebeler et al. PRL105 (2010) 161102 and Gandolfi et al. PRC85 (2012) 032801 (R) Mass-Radius (Neutron Star) Steiner et al. Astrophys. J. 722 (2010) 33 Lie-Wen Chen et al. PRC 82 (2010) 024321 Neutron Skin Neutron Skin Mass Nuclear Model Fit Kortelainen et al. PRC 82 (2010) 024313 Mass Danielewicz NPA 727 (2003) 233 Empirical Heavy Ion Collisions n−p Emission Ratio Isospin Diffusion IVGQR Agrawal et al. PRL109 (2012) 262501 Famiano et al. PRL 97 (2006) 052701 Tsang et al. PRL 103 (2009) 122701 Roca-Maza et al. PRC 87 (2013) 034301 Dipole Polarizability ◮ Centelles et al. PRL 102 (2009) 122502 Warda et al. PRC 80 (2009) 024316 Neutron Skin Roca-Maza et al. in preparation (2013) RPA and unperturbed dipole strength. Giant Resonances Trippa et al. PRC 77 (2008) 061304(R) GDR Klimkiewicz et al. PRC 76 (2007) 051603(R) PDR PDR Carbone et al. PRC 81 (2010) 041301(R) ◮ the transition densities. ◮ the isoscalar or20isovector 40 60 80 nature. 100 120 ◮ the most relevant p-h contributions. N−A scattering Charge Ex. Reactions Energy Levels Parity Violating e-scattering Optical Potential Parity Violating Asymmetry Xu et al. PRC 82 (2010) 054607 PREX Collab. PRL 108 112502 (2012) L (MeV) X. Viñas et al. EPJA special volume on the symmetry energy X. Roca-Maza, G. Pozzi, M.Brenna, K. Mizuyama and G. Colò, Phys. Rev. C 85 024601 (2012) 7 Contents Microscopic analysis of the PDS: model dependence and sensitivity to the symmetry energy We study the PDS within the self-consistent HF+RPA approach in the exotic 68 Ni and 132 Sn and the stable 208 Pb nuclei. For that, we use three Skyrme interactions with very different isovector properties (L ranges from 40 MeV to 100 MeV). We focus on: ◮ RPA and unperturbed dipole strength. ◮ the transition densities. ◮ the isoscalar or isovector nature. ◮ the most relevant p-h contributions. X. Roca-Maza, G. Pozzi, M.Brenna, K. Mizuyama and G. Colò, Phys. Rev. C 85 024601 (2012) 8 Dipole strength functions (IV) 50 7 SGII SkI3 SLy5 0 9 10 11 68 Ni 12 3 30 5 10 20 15 25 SGII SkI3 SLy5 80 −1 10 9 132 10 Exp. 9.8 MeV [2] Sn 8 9 208 10 Pb 20 15 Energy [MeV] 15 20 SGII L = 37.6 MeV SLy5 L = 48.3 MeV SkI3 L = 100.5 MeV Exp. 7.37 MeV [3] 10 10 Isovector properties of the interactions: 2 7 0 5 A. Carbone et. al., PRC81 (2010) 041301. 5 0 IV 8 larger L → larger PDS peak Exp. 13.43 MeV [3] 15 0 5 20 Energy [MeV] 100 40 1 0 10 Energy [MeV] 60 2 IV IV Exp. 11 MeV [1] 5 4 2 2 1 0 B (E1) [fm MeV ] 40 −1 15 10 SGII SkI3 SLy5 6 B (E1) [fm MeV ] 3 2 −1 B (E1) [fm MeV ] 20 20 Experiment: [1] O. Wieland et. al., PRL 102 (2009) 092502. [2] P. Adrich et. al., PRL 95 (2005) 132501. [3] N. Ryezayeva et. al., PRL 89 (2002) 272502. 9 Microscopic analysis of the PDS RPA versus unperturbed strength 40 35 40 SGII SkI3 SLy5 68 35 Ni 30 30 25 25 20 20 15 15 10 10 5 5 IV 2 −1 B (E1) [fm MeV ] Unperturbed 0 0 10 20 0 10 20 0 10 20 0 Energy [MeV] - No low energy peak in the unperturbed response. - Indications that the PDS may show some coherency depending on the model. (RPA peaks do not coincide in energy with the unperturbed peak) 10 Microscopic analysis of the PDS the transition densities (∼ amplitude of neutron and proton transition probabilities as a function of r-coordinate) r [fm] 0 2 r [fm] 6 4 rp rn 0.004 8 10 0 neutrons protons E = 9.77 MeV -0.004 SkI3 E = 10.45 MeV -0.008 0.004 E = 9.77 MeV 0.005 0 -0.005 SkI3 -0.01 E = 10.45 MeV 0.005 0 0 68 -0.004 -0.008 0 SGII -0.01 0 10 isovector isoscalar 0 −3 -0.008 0.004 8 -0.005 δρ(r) [fm ] −3 δρ(r) [fm ] SGII 6 4 rp rn 0.005 0 -0.004 2 Ni 2 4 6 r [fm] -0.005 SLy5 8 68 Ni -0.01 E = 9.30 MeV 10 0 2 4 6 SLy5 E = 9.30 MeV 8 10 r [fm] Around the nuclear surface: all models clearly isoscalar. In the interior: not clear nor definite trends in the studied models. 11 Microscopic analysis of the PDS Isoscalar or isovector? BIV (E1) = X Z Z ν A drr3 δρn ν (r) − 30 −1 B (E1) [fm MeV ] Z p drr3 δρν (r) 30 68 SkI3 IS 70% [0,R] 25 N A Ni IS 70% 25 [R/2,R] IS 70% [0,R/2] 20 15 15 10 10 5 5 IV 2 20 0 10 15 20 25 10 15 20 25 10 15 20 0 25 Energy [MeV] [N. Paar et. al., PRL103 (2009) 032502] IS nature of the PDS due to outermost nucleons (neutrons in a neutron-rich nucleus). The ∆rnp is correlated with I and L. 12 2 2 neutrons protons 68 1f7/2 1g9/2 2d3/2 1f5/2 1g9/2 1f7/2 1g9/2 1f7/2 1g9/2 1f7/2 1g9/2 A -1 2 Aq ph (E1) | ph,q 1f7/2 2p3/2 2d5/2 (E1) [e fm] 0 1f7/2 1g9/2 X B(E1) ≡| 1 0 q ph The most relevant p-h excitations in the IS and IV dipole response 1 2p1/2 2d3/2 Ni Microscopic analysis of the PDS SGII SkI3 SLy5 E = 9.77 MeV E = 10.45 MeV E = 9.30 MeV -2 8 10 12 14 8 10 12 14 8 10 12 -1 14 -2 Eph [MeV] 25 Ni (E1) [e fm] 20 1f5/2 1f7/2 2p1/2 2p3/2 15 10 2p1/2 2p3/2 1f5/2 2d3/2 1g9/2 2d3/2 2d5/2 1f7/2 2d3/2 3s1/2 2d3/2 1g9/2 25 20 1f5/2 1f7/2 2p1/2 2d3/2 1g9/2 3s1/2 15 2p3/2 2d5/2 10 5 5 A q ph neutrons protons 68 0 0 -5 E = 10.45 MeV E = 9.77 MeV 10 15 SLy5 SkI3 SGII 20 10 15 Eph [MeV] E = 9.30 MeV 20 10 15 -5 20 The largest neutron p-h contributions (around 8 with BIS > 1) are coherent and all of them (except one) correspond to transitions of the outermost neutrons → indicates that the ISPDS is a collective mode that may be correlated with N − Z. 13 Collectivity: Coherence of the different contributions cumulative sum cumulative sum 132 Sn 1 -2 0 SGII π SkI3 π ν 10 20 30 nph 0 SLy5 π ν 10 20 30 nph 0 IS ph 0 -1 80 132 3 2 (E1) [e fm ] 100 20 SGII π ν SkI3 π ν SLy5 π ν 0 10 20 30 40 0 10 20 30 40 0 10 20 30 40 50 nph nph nph 10 20 30 40 nph The largest p-h contributions are: 40 0 ν Sn 60 A A IV (E1) ph [e fm] 3 ◮ coherent in the IS channel, ◮ less coherent in the IV channel. 14 2 1 0 8 9 10 8 9 10 E [MeV] 8 9 10 16 12 SkI3 SLy5 132 8.64 MeV 8.64 MeV 9.23 MeV 3 Sn SGII 9.23 MeV 132 5 4 20 SLy5 8.52 MeV SkI3 B(E1;IS) [s.p. units] 7 6 SGII 8.52 MeV B(E1;IV) [s.p. units] Single particle units: qualitative indications Sn 8 4 0 8 9 10 8 9 10 E [MeV] 8 9 10 If different p-h states are contributing coherently to the PDS, B(E1) in single-particle units should be clearly larger than 1. 15 Dipole strength functions (IS) 10 10 20 30 E (MeV) Sn 4 10 20 E (MeV) 30 The response of the low-energy pygmy state to an isoscalar probe is comparable to the high-energy states corresponding to the ISGDR 20 3 6 −1 B(E1;IS) (10 fm MeV ) 132 (b) pygmy region 208 10 10 8 0 40 30 (b) pygmy region 3 Ni 0 −1 6 68 0 B(E1;IS) (10 fm MeV ) 20 2 6 12 (b) pygmy region −1 B(E1;IS) (10 fm MeV ) 30 20 E (MeV) 30 Pb 40 16 Conclusions: PDS in 68 Ni, 132 Sn, 208 Pb: 1 The IV (and IS) dipole response show a low-energy peak in the strength function for all studied nuclei and models. 2 Such an IV peak (and also IS) increases in magnitude with increasing values of L [in agreement with other works]. 3 The collectivity associated with the RPA states giving rise to the PDS show up depending on the nature of the probe used for exciting the nucleus: there is systematically more collectivity in the IS than in the IV transitions. 4 The low-energy IV and IS responses are basically due to the outermost neutrons. 5 The isoscalarity displayed by the RPA states giving rise to the PDS may probe isoscalar properties. 17 Conclusions: Therefore, ◮ IS probes interacting with the surface of the nucleus seem to be more suitable for the study of the low-energy dipole response in nuclei far from the stability valley. ◮ The properties of the PDS may display an involved correlation with the parameters of the nuclear EoS that it is not clear enough yet ◮ This puzzle may be solved by performing more studies on neutron-rich systems ◮ For that, we miss some systematic scattering experiments (in inverse kinematics) that can excite predominantly IS states like (α,α′ ) or (16 O,16 O′ ) [See next talk from Prof. Lanza] 18 I would like to kindly thank my collaborators: Giacomo Pozzi, Marco Brenna, Kazhuito Mizuyama and Gianluca Colò 19 Thank you for your attention! 20
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