Contents Page Acknowledgements Certificate 1 2-3 Journal publications 4 Conference proceedings 5 Summary 6 List of figures Chapter 1: Introduction 11 16-51 1.1 Development of lasers 17 1.2 Nonlinear phenomena arising through laser-plasma interaction 23 1.2(a) Self-focusing of laser beams in plasma 23 1.2(b) Wakefield generation 30 1.2(c) Laser pulse compression 34 1.3 Propagation of a laser beam in a plasma channel 40 1.4 Variational technique 46 1.5 Approach 48 1.6 Aim 50 Chapter 2: Simultaneous evolution of spot-size and length and induced chirping of short laser pulses in a plasma channel 52-81 2.1 Evolution of spot-size and pulse length 52 2.2 Analytical solution for laser spot-size and pulse length 63 2.3 Numerical solution for simultaneous evolution of laser spot-size and pulse length 69 2.4 Group velocity dispersion and self-phase modulation induced chirping of short laser pulses in a plasma channel 74 Chapter 3: Propagation of ultrashort chirped laser pulses in a plasma channel 82-102 3.1 Analysis of wave equation 82 3.2 Effect of chirp on matched laser pulse propagation 90 3.3 Variation of laser frequency across chirped laser pulses 96 Chapter 4: Wakefield effects on the evolution of symmetric laser pulses in a plasma channel 103-122 4.1Wave dynamics 103 4.2 Density perturbation 106 4.3 Evolution of laser spot-size and pulse length 111 4.4 Graphical description 118 2 Chapter 5: Conclusions 123-128 5.1 Conclusions 123 5.2 Recommendations for future work 127 References 129 3 Acknowledgements First and foremost it is my pleasure to thank my supervisor, Prof. Pallavi Jha, Department of Physics, University of Lucknow, for all her support and enthusiasm during the course of my Ph. D. She is an inspirational teacher and tireless campaigner for the cause of scientific rigour. She has been a fantastic supervisor, who maintains an overwhelming energy throughout her work and carries that through to all around her. I am very fortunate to have had the chance to work with her so closely. I express my gratitude to Prof. U.D. Misra, Head, Department of Physics, University of Lucknow, for being supportive. My special thanks to Dr. Ajay Kumar Upadhyay, Dr. Gaurav Raj and Dr. Rohit Kumar Mishra for their enthusiastic help and timely advice towards completion of the thesis. I am thankful to Mr. Ram Gopal Singh, Mr. Vijay Singh, Ms. Akanksha Saroch and Mrs. Anjani Singh for creating a congenial work environment in our Plasma Electrodynamics Group at the University. I am specially indebted to my Parents Mrs. Pratima Malviya and Mr. Ram Krishna Malviya, brother Mr. Anand Malviya and entire family for their unflinching and whole-hearted support throughout the endeavour. The thesis in the present form would not have been possible without the blessings of my grand parents Mr. Ram Shankar Malviya and Late Mrs. Chanda Malviya. 4 Journal Publications 1. Simultaneous evolution of spot-size and length of short laser pulses in a plasma channel Pallavi Jha, Amita Malviya, Ajay K. Upadhyay and Vijay Singh Plasma Phys. Control. Fusion, vol. 50, 015002 (2008). 2. Propagation of chirped laser pulses in a plasma channel Pallavi Jha, Amita Malviya and Ajay K. Upadhyay Physics of Plasmas, vol. 16, 063106 (2009). 3. Wakefield effects on the evolution of symmetric laser pulses in a plasma channel Pallavi Jha, Amita Malviya and Ajay K. Upadhyay Laser and Particle Beams, vol. 28, 245 (2010). 5 Conference Proceedings 1. Simultaneous evolution of pulse length and spot of laser beam in homogeneous plasma Amita Malviya, Ajay K.Upadhyay, and Pallavi Jha 22nd National Symposium on Plasma Science and Technology-2007 (Ahmdabad). 2. Group velocity dispersion and self-phase modulation induced chirping of short laser pulses in a plasma channel Amita Malviya, Ajay K. Upadhyay and Palllavi Jha 24th National Symposium on Plasma Science and Technology-2009 (Hamirpur). 6 Summary Chirped-pulse amplification technique has permitted the production of laser pulses with peak powers ranging from 100 terawatt (TW) to 1 petawatt (PW) by stretching, amplifying and then recompressing. High power is achieved due to very short pulse duration. Shorter pulses would be of interest because they could lead to higher peak powers without increasing the size and cost of the laser system. These pulses find applications in ultrahigh intensity laser-plasma interaction such as particle acceleration, high harmonic generation and X-ray lasers. For all these applications long distance propagation of intense lasers in plasma is desirable. However, since diffraction will spread the laser beam after the focus, the effective interaction length is limited by the Rayleigh length Z R k r 2 0 0 2 , where k0 and r0 are the laser wavenumber and beam waist respectively). A plasma channel having a parabolic radial density variation prevents diffraction of the laser pulse. While propagating in a plasma channel the laser spot undergoes betatron oscillations which allows the pulse to remain confined close to the channel axis. For a moderately intense laser pulse propagating in a pre-formed plasma channel, focusing will be brought about due to the channel as well as relativistic selffocusing. On account of focusing of the laser beam, its pulse length is affected as the laser pulse propagates in plasma. Thus the evolution of the spot-size and pulse length are coupled. Therefore it is important to study the simultaneous evolution of the laser spotsize and pulse length for most laser-plasma applications. Also for short laser pulses, wakefields will be generated and will affect the propagation characteristics in plasma. 7 The variation of pulse length and spot-size of the laser beam in turn affects the wakefield generation. The present thesis is a theoretical analysis of the evolution characteristics of short laser pulses propagating in a plasma channel. The effects of group velocity dispersion, induced chirp, as well as relativistic and ponderomotive nonlinearities have been considered, to study the evolution dynamics. The wave equation for the laser field amplitude is set up and an appropriate Lagrangian is defined. A variational technique is used to analyze the laser-plasma system. Chapter 1 presents the basic properties of plasma and condition required for the propagation of electromagnetic waves inside the plasma. A brief summary of the development of lasers and the properties of laser beams is presented. Nonlinear phenomena such as self-focusing of a laser beam in plasma, wakefield generation and laser pulse compression dynamics arising due to interaction of laser pulses with plasma have been discussed briefly. The utility of a plasma channel for the purpose of guiding laser beams has been shown. The method of using the variational technique as a mathematical tool for describing the evolution of laser pulses in plasma has been presented. This technique has been used for all analyses presented in the thesis. In Chapter 2, nonparaxial, nonlinear propagation of an intense, short, Gaussian laser pulse in a plasma channel is studied in a particular regime in which relativistic nonlinearity dominates over ponderomotive effects. Also the parameters are limited to a regime in which the group velocity dispersion effect dominates over finite pulse length effect. Using the variational technique, simultaneous equations describing the evolution of the laser spot-size and pulse length have been set up. An analytical solution is obtained 8 for the spot-size (pulse length) by considering the pulse length (spot-size) to be constant. Further, numerical solutions for simultaneous evolution of the laser spot-size and pulse length are obtained and graphically analyzed and the condition for achieving pulse compression has been highlighted. Simultaneous solutions show a higher rate of compression of pulse length as compared with the constant spot-size case. Also, the focusing effect increases for the evolving pulse length case. It is seen that the presence of the channel leads to compression of the pulse length whereas in the absence of the channel, a broadening effect is observed. It is also observed that a laser spot satisfying the beam matching condition, when pulse compression effects are neglected, does not remain matched when the laser spot and pulse length evolve simultaneously. The chirp induced over the laser pulse due to group velocity dispersion and self-phase modulation is evaluated. These studies point towards the possibility of generating high intensity laser pulses via pulse compression and production of chirped laser pulses. The present study reveals that an unchirped pulse becomes chirped as it propagates in plasma. This is due to group velocity dispersion and self-phase modulation. The propagation of an initially chirped ultrashort laser pulse in a pre-formed plasma channel is presented in Chapter 3. For ultrashort laser pulses, relativistic and ponderomotive nonlinearities cancel each other, hence a linear analysis can approximately describe the propagation dynamics. Evolution of the laser spot-size and phase shift with propagation distance of the laser pulse is analyzed. The effect of initial chirp on the laser pulse length and intensity of a matched laser beam propagating in a plasma channel has been presented. The effective pulse length and chirp parameter of the laser pulse due to its interaction with plasma have been obtained and graphically 9 depicted. It is observed that for a positively chirped laser, the pulse length is compressed up to a certain distance and then starts to broaden. However, the length of a negatively chirped pulse broadens continuously and broadening is more rapid in comparison to an unchirped pulse. For a positively chirped pulse, intensity of the matched beam increases in the region where pulse compression occurs. The intensity of a negatively chirped pulse is damped in comparison to its initial value. Also, after the pulse has traversed a certain critical distance, the positively chirped laser pulse becomes unchirped. Beyond this critical distance, chirp reversal occurs for a positively chirped laser pulse. This reversal occurs because the group velocity induced negative chirp and its coupling with initial chirp becomes more effective in comparison to the initial positive chirp. If the distance traversed by the laser pulse is less than the critical distance, reversal of chirp does not occur. Also chirp reversal does not occur for negatively chirped pulses. The resultant variation in the laser frequency across the laser pulse is evaluated. Chapter 4 deals with the combined effect of wakefields (inside the laser pulse) and relativistic nonlinearity on the propagation of a laser pulse in a parabolic plasma channel. Quasi-static approximation is used to obtain density perturbations. Considering a wide channel, the radial dependence of the plasma frequency has been neglected. The variation in density of the transverse and axial ponderomotive nonlinearity is evaluated and coupled equations describing the evolution of the laser pulse length and spot-size are set up. In the presence of wakefields, the evolution equation for pulse length and spotsize exhibit singularity if the pulse length approaches the plasma wavelength. Therefore in this limit, the density perturbation is obtained using l’ Hospital’s rule and the evolution equations for the pulse length and spot-size of the laser are derived separately. The laser 10 propagation characteristics have been analyzed with the help of numerical solutions of these equations. The present study shows that the laser propagation dynamics is extremely sensitive to the ratio of pulse length and plasma wavelength and show contrary behavior for ( L0 P where L0 and P are the initial pulse length and plasma wavelength) less than or greater than unity. This result will be significant for operation of laser-plasma based accelerator systems. Conclusions from the present research and recommendations for future work are presented in Chapter 5. 11 List of figures Page Fig 1.1: Chirped pulse amplification concept. 19 Fig.1.2: History of light sources over the last century. Each advance in laser intensity enables a new regime of optics. 20 Fig.1.3: Normalized pulse length ( L L0 ) against normalized propagation distance ( z Z R ) in the absence of nonlinearity. 38 Fig.1.4: Normalized pulse length ( L L0 ) against normalized propagation distance ( z Z R ) in the presence of nonlinearity. 39 Fig.1.5: Evolution of normalized spot size versus normalized propagation distance for a) vacuum diffraction b) homogeneous plasma c) a plasma channel. Fig.2.1: Variation of 45 normalized pulse length L L0 with propagation distance z Z R in the absence of (curve a) and in the presence (curve b) of the plasma channel for f 02 0.03, 1m, r0 33m, L0 14m, P 10m, n 2 1017 and rch 50m . Fig.2.2: Simultaneous variation of normalized spot size rs r0 (curve a) 12 70 and the normalized pulse length L L0 (curve b) with normalized propagation distance z Z R . Evolution of the spot-size keeping the pulse length constant (curve c). Evolution of the pulse length keeping the spot size constant (curve d) for f 02 0.03, 1m, r0 33m, L0 14m, P 10m, n 2 1017 cm 3 and rch 50m . 72 Fig.2.3: Simultaneous variation of normalized spot-size rs r0 (curves a, b and c) and the normalized pulse length L L0 (curves d, e and f ) with normalized propagation distance z Z R , f 02 0.03 , nc 1.7 1017 cm 3 , 0.04 nc 1.4 1017 cm 3 and 0.05 nc 1.2 1017 cm 3 , 1m , r0 33m, L0 14m, P 10m and rch 50m . Fig.2.4: Variation n n of intensity for the initial values f 02 0.03 0.04 n 1.4 10 cm . Other laser plasma parameters c 1.7 1017 cm 3 , c 1.2 1017 cm 3 17 73 3 c and 0.05 are 1m , r0 33m, L0 14m , P 10m and rch 50m. 75 Fig.2.5: Variation of normalized frequency 0 with z Z R . Solid (dotted) curve a (curve d) , curve b (curve e ), curve c (curve f ) are due SPM, GVD and combined effect of SPM and GVD at front (back) 0.5 - 0.5 of the pulse for f 02 0.03, 1m, r0 33m, L0 14m, P 10m, n nc 1.7 1017 cm -3 and rch 50m. 13 77 Fig 2.6: Variation of normalized chirp 0 across the laser pulse after traversing distance z Z R 3 (curve a) and z Z R 6 (curve b) for f 02 0.03, 1m, r0 33m , L0 14m, P 10m, rch 50m and n nc 1.7 1017 cm -3 . Fig.2.7: Variation of intensity f 2 79 z, with after pulse has traversed a distance z Z R 0 (curve a), z Z R 3 (curve b) and z Z R 6 (curve c) r0 33m, 1m, f 02 0.03, for L0 14m, P 10m , n nc 1.7 1017 cm -3 and rch 50m . Fig.3.1: Variation of effective pulse length Le0 L0 with 80 propagation distance z Z D 0 for a positively chirped pulse ((curve a), 0.3 ), unchirped pulse (curve b) and negatively chirped pulse ((curve c), 0.3 ). 94 Fig 3.2: Variation of normalized intensity a 2 f 02 with L 0 for the initial laser pulse z Z D 0 0 , dotted curve) and after the laser pulse has traversed a distance z Z D0 0.275 (critical distance) for chirp parameter 0.3 (curve a), 0 (curve b) and 0.3 (curve c). Fig.3.3: Variation of normalized frequency 0 97 with L 0 at z Z D 0 0.1 for chirp parameters 0.3 (line a), 0 (line b) and -0.3 (line c) for r0 25m , L0 10m , 1m and p 40m. 14 99 Fig.3.4: Variation of normalized z Z D 0 0.275 frequency for chirp parameters 0 with L 0 at 0.3 (line a), 0 (line b) and 0.3 (line c) for r0 25m , L0 = 10 m , 1m and p 40m. 100 Fig. 3.5: Variation of normalized frequency z Z D 0 0.45 for chirp parameters 0 with L 0 at 0.3 (line a), 0 (line b) and 0.3 (line c) for r0 25m , L0 = 10 m , 1m and p 40m. Fig.4.1: Variation when 101 of normalized pulse length with propagation distance 1 curve a, 1 curve b and 1 curve c for L0 16m , 9m and 11m , r0 25m, 1m , f 02 0.015 P 11m , rch 40m and n nc 4.3 1017 cm 3 . 120 Fig.4.2: Variation of normalized spot-size with propagation distance when 1 curve a, 1 curve b and 1 curve c for L0 16m , 9 m and 11m , r0 25m, f 02 0.015 , 1m , P 11m , rch 40m and n nc 4.3 1017 cm 3 . 121 Fig.4.3: Variation of laser pulse intensity with propagation distance when 1 curve a, 1 curve b and 1 curve c for L0 16m , 9 m and 11m , r0 25m, f 02 0.015 , 1m , P 11m , rch 40m and n nc 4.3 1017 cm 3 . 15 122 Chapter 1 Introduction Plasma is a quasi-neutral gas of charged and neutral particles which exhibits collective behaviour. It is a phase of matter distinct from solids, liquids and normal gas. Since plasma electrons are of very small mass, their motion controls the plasma 16 behaviour in fast processes. In fully ionized plasma, electron-electron collisions are negligible and ionic thermal motion is also negligible. In plasma only electrons are mobile, ions provide a neutralizing background of positive charges. Irving Langmuir, the Nobel laureate who pioneered the scientific study of ionized gases, gave this fourth state of matter, the name plasma. Any ionized gas cannot be called plasma. For an ionized gas to be categorized as plasma, the existence of the following conditions must be fulfilled: (i) the Debye length ( D k B T 4n0 e 2 where k B , T , n0 , and e represent the Boltzman constant, absolute temperature, plasma electron density and electronic charge respectively), must be smaller than the plasma size, (ii) the number of electrons within a sphere which has volume 43D 3 must be greater than unity 43D 3 1 , and (iii) quasi-neutrality of plasma implies that the ion density must be equal to the electron density. If the quasi-neutrality of plasma is disturbed by some external force, the charge separation between ions and electrons gives rise to electric fields and the flow of plasma electrons gives rise to current and magnetic fields. These electrons begin to accelerate in an attempt to restore the charge neutrality. Due to their inertia they will move back and forth about the equilibrium position, resulting in fast collective oscillations around the more massive ions. The frequency of these oscillations is known as plasma frequency P 4n0 e 2 m 12 where m is the electron mass . The propagation of electromagnetic waves through pre-ionized plasma is governed by the dispersion relation c 2 k 02 02 P2 , where 0 and k 0 ( 2 0 , 0 being the radiation wavelength) are the wave frequency and wavenumber. An electromagnetic wave can propagate through plasma if its propagation constant is real i.e. its frequency is greater than the plasma frequency. Such a plasma is known as underdense 17 plasma. As the plasma density increases P becomes equal to 0 and the plasma is said to be critically dense. With further increase in density, the wavenumber becomes imaginary and the electromagnetic wave is unable to propagate. This plasma is known as overdense plasma. The interaction of electromagnetic waves with matter becomes interesting as well as important if the intensity of the wave becomes high such that the index of refraction becomes nonlinear i.e. it becomes a function of the radiation intensity. 1.1 Development of lasers Since 1960, lasers [1-5] have evolved in peak power by a succession of leaps, each three orders of magnitude. These advances were produced each time by decreasing the pulse duration accordingly. Initially laser sources emitted a peak power in the kilowatt (KW) range. In 1962, modulation of the laser cavity quality factor enabled the same energy to be released on a nanosecond (ns) timescale, a thousand times shorter, to produce pulses in the megawatt (MW) range. In 1964, locking the longitudinal modes of the laser (mode locking) enabled the laser pulse duration to be reduced by another factor of a thousand down to the picosecond (ps) level, thus increasing the peak power to the gigawatt (GW) level. Presently, chirped pulse amplification (CPA) [6-10] technique has led to the production of femtosecond (fs) laser pulses generating multiterawatt (TW) and even petawatt (PW) of power. In CPA, the pulse is first stretched by a factor of a thousand to a hundred thousand. This step does not change the input pulse energy (input fluence), and 18 therefore the energy extraction capability, but it does lower the input intensity by the stretching ratio. The pulse is then amplified by 6 to 12 orders of magnitude i.e. from the nanojoule (nJ) to the millijoule-kilojoule (mJ-kJ) level and is finally recompressed by the same stretching ratio back to a duration close to its initial value. The power production through CPA is 10 3 10 4 times more than that produced by dye or excimer systems of equivalent size. (Fig. 1.1) At present, about fifteen petawatt lasers are being built around the world and plans are afoot for new, even higher power lasers reaching values of exawatt (EW) or even zetawatt (ZW) powers. Fig. 1.2 illustrates the increase in achievable laser intensity since 1960. High-intensity laser radiation may now be applied in many traditional areas of science usually reserved to nuclear accelerators and reactors. Fig. (1.1) Chirped pulse amplification concept 19 Fig.(1.2) History of light sources over the last century. Each advance in laser 20 intensity enables a new regime of optics. (Ledingham and Galster New J. Phys. 12, 045005, (2010)). As the laser intensity and associated electric field is increased the electron quiver energy, (the energy a free electron has in the laser field) increases accordingly as illustrated in Fig.1.2. When the laser radiation is focused onto solid and gaseous targets at intensities 1018 W cm -2 , electron quiver with energies greater than their rest mass energy (0.511MeV) are achieved, creating relativistic plasma. In most laser applications it is necessary to know the propagation characteristics of the laser beam. The simplest and most appropriate type of beam provided by a laser source is a Gaussian beam. It is the lowest order ( TEM 00 ) mode of the laser optical resonator. The mathematical function that describes the Gaussian beam is a solution to the paraxial form of the Helmholtz equation. The amplitude of a fundamental Gaussian laser beam as a function of the transverse and axial coordinates propagating along the zdirection is given by ik 0 r 2 r2 E r , z E0 exp i z 2 2 R z rs z 21 (1.1) where rs z is defined by the transverse distance at which the field amplitude drops to 1 e of its axial (peak) value. Rz and z are the radius of curvature and phase shift of the laser beam respectively. The characteristic laser beam parameters (evolving with propagation distance) are therefore given by rs z , R z and z [11]. In vacuum the evolution of the spot-size along the direction of propagation z is given by z rs z r0 1 ZR 2 12 (1.2) where Z R k 0 r02 2 is the Rayleigh length. It is the distance at which the laser spot becomes 2 times the beam waist r0 . At the beam waist the wavefront is planar, R0 . As the beam propagates outwards, the wavefront gradually becomes curved and the radius of curvature Rz drops down to finite values. For distances well beyond the Rayleigh length, the radius increases again. The analytical form of the radius of curvature Rz of the wavefront is given by, Z2 R z z R z for z Z R 2 Z R for z Z R z for z Z R . (1.3) The third beam parameter, z is known as the Guoy phase shift and is given by 22 z ZR z tan 1 . (1.4) This factor should be taken into account when the exact knowledge of the wavefront is needed for involved applications. 1.2 Nonlinear phenomena arising through laser-plasma interaction With the advent of high intensity laser systems, studies based on nonlinear laserplasma interaction became a frontier field of Physics. The rapid progress in the technology of high power lasers based on chirped pulse amplification makes possible, the exploration of relativistic Plasma Physics in the laboratory. In this regime, plasma electrons oscillate at relativistic velocities leading to nonlinear interaction dynamics. Nonlinear propagation of laser pulses in underdense plasma can change its temporal, spatial and spectral properties. These changes give rise to various interesting phenomena such as self-focusing, pulse compression, self-phase modulation and wakefield generation. In this context, the possibility of development of a wide range of applications, such as high energy particle acceleration [12-16], inertial confinement fusion [17-19], and harmonic generation [20-24], are being explored. 1.2(a) Self-focusing of laser beams in plasma A primary phenomenon that occurs when a laser beam having a Gaussian radial profile (intensity peaked on-axis) passes through plasma, is self-focusing [25-33]. When 23 intense laser beams interact with plasma, the refractive index is modified and is given by r 1 P2 nr 02 n0 r . The change in refractive index occurs due to relativistic 12 mass correction r and the radial variation nr of plasma electron density due to ponderomotive effects. Since the laser intensity is peaked on-axis, plasma electrons are expelled radially outward, leading to decrease (increase) in on-axis density (refractive index). Also, the relativistic factor is maximum on the axis. This contributes to a maximum value of refractive index at the laser axis. Therefore, the phase velocity of the laser wavefront increases with the radial distance causing them to curve inwards and the laser focuses towards the axis. Consider the propagation of a linearly polarized laser beam in homogeneous plasma. The vector potential of the radiation field is given by Ar , z , t A xˆ exp ik 0 z i 0 t c.c. 2 (1.5) where Ar, z, t is the field amplitude and k0 ( 0 ) is the wavenumber (frequency). The wave equation governing the propagation of the laser field in plasma can be obtained from Maxwell’s time dependent equations [34] and is given by, 2 1 2 4J 2 2 A c c t (1.6) 24 where J nev is the plasma current density. In deriving Eq. (1.6), Coulomb gauge .A 0 has been used. The current density may be obtained with the help of the Lorentz force equation, 1 2 1 a v a v . p mc c t c t (1.7) and the continuity equation given by n .nv 0 t (1.8) where p mv is the momentum of plasma electrons. Eq. (1.7) shows that the fast response of the plasma electrons to the laser field gives rise to the electron velocity 12 2 v v 1 v ca where 1 a 2 is the relativistic factor, a eA mc 2 is the normalized laser strength parameter and e mc 2 is the normalized scalar potential. Thus the lowest order quiver velocity of the plasma electrons is given by 2 v 1 ca and the perturbed part of plasma electron velocity is given by v ca a 4 in the mildly relativistic regime a 1, 1 a 2 2 4 . Substituting the value of the plasma current density J (= e n0 v 1 n0v v 1n where n is the higher order density perturbation) into Eq. (1.6), gives the wave equation describing the evolution of the vector potential driven by relativistic and ponderomotive nonlinearities, as, 25 a 2 n 2 2 1 2 2 a 2 2 2 a k P 1 4 n0 z c t (1.9) where k P P c is the plasma wavenumber. Substituting Eq. (1.5) into Eq. (1.9) and transforming independent variables z, t to z , ( z g ct , where g ck 0 0 is the normalized group velocity of the laser pulse) gives 2 2 2 2 2 2 ik 2 1 0 g ar , z, z z 2 z 2 2 a n k 1 ar , z, k 02 P2 1 ar , z, 4 n0 2 P (1.10) where P 0 ck 0 and g P 1 . If the laser pulse length L is sufficiently greater than the plasma wavelength P and the laser beam is broad k P r0 1 and L r0 , the electron density response n may be neglected in comparison to the relativistic effect (Sec.1.2b). Thus Eq. (1.10) reduces to 2 2 2 2 2 2 ik 2 1 0 g ar , z, z z 2 z 2 2 a k 1 ar , z, k 02 P2 1 ar , z, . 4 2 P 26 (1.11) Eq. (1.11) describes the nonparaxial wave equation governing the evolution of the laser pulse amplitude. The first term on the left side of this equation represents transverse amplitude variation, the second term shows the first order diffraction effect, the third term represents finite pulse length effects, while the fourth and fifth terms represent higher order finite pulse length (group velocity dispersion) and diffraction effects respectively. Neglecting finite pulse length and higher order diffraction effects in Eq. (1.11) the paraxial wave equation is given by 2 a 2 2 2 2 2ik 0 z ar , z , k P 1 4 ar , z, k 0 P 1 ar , z, . (1.12) In order to study the evolution of the laser spot-size rs z , several methods, such as, the heuristic method [35-36], Variational method [37-51] or source dependent expansion (SDE) method [52-56] may be used. For any of these techniques, a trial function for the amplitude of the radiation field is assumed. For a Gaussian beam a suitable trial function can be assumed as ik r 2 r2 a f z exp i z 0 2 . 2 Rz rs z (1.13) Considering the heuristic method, the trial function (Eq. 1.13) is substituted into the paraxial wave equation (1.12) to give 27 4r 2 k 02 r 2 4ik 0 r 2 2ik 0 4 2 4 a 2 2 rs z R z rs z Rz rs z Rz 1 f z z 2r 2 rs z ik 0 r 2 Rz i 3 2ik 0 a z rs z z 2R 2 z z f z z k2 P 4 f 2 z 1 2r 2 k P2 k 02 P2 1 a . 2 rs z (1.14) Comparing imaginary and real parts and equating coefficients of r 2 and r 0 on both sides of Eq. (1.14) gives the evolution of curvature, amplitude, spot-size and phase shift of the laser as R z rs rs z , (1.15) f 02 r02 f z 2 , rs 2 2 rs 4 2 3 2 z k 0 rs (1.16) k P2 f 02 r02 1 , 8 (1.17) and k P2 z 2k 0 f 2 z k 0 2 2 1 P 1 2 rs k 0 4 2 28 (1.18) where r0 is the beam waist and f 0 ( eA0 mc 2 where A0 is the initial vector potential) is the laser strength parameters. The first term on the right hand side of Eq. (1.17) represents vacuum diffraction, whereas the second term leads to relativistic self-focusing. The solution to Eq. (1.17) with initial condition rs z 0 at z 0 , is given by rs2 P 1 1 2 r0 Pc where z2 2 ZR (1.19) 2r 2c5 P k P2 r02 f 02 0 . The laser power is given by P 4 Pc 8 e2c Pc 2 0 2re P 2 e2 GW where re in practical units 2 mc m f0 e0 2 GW and is the critical power for relativistic self focusing of the laser beam. Eq. (1.19) shows that the spot-size diffracts for P Pc , remains guided or matched rs r0 for P Pc and for P Pc it focuses initially but predicts catastrophic focusing after a certain value of z . This is due to the approximation 1 a 2 2 1 2 1 a 2 4 in the a 1 limit. In a relativistic situation, 2 however, higher-order nonlinearities will prevent the laser from focusing indefinitely. For short laser pulses (pulse lengths less than a plasma wavelength) relativistic optical guiding is significantly diminished even when the laser power exceeds the critical power P Pc . This is due to the fact that the index of refraction becomes modified by the laser pulse on the plasma frequency time scale, not the laser frequency time scale. 29 1.2(b) Wakefield generation When the laser pulses interacting with plasma are short k P L 1, L c 1 ps , density perturbations become important. The laser pulse will exert a significant radial and axial ponderomotive force on the plasma electron. The radial ponderomotive force expels electrons radially outward, while the front (back) of the laser pulse exerts a forward (backward) axial force on the electrons. The ponderomotive force exerted by the laser pulse on the plasma electrons can be obtained from the slow components of the Lorentz force equation (1.7), as 2 2 v 1 v 2 c t 2 (1.20) where v represents the second order slow velocity. The first term on the right of Eq. (1.20) is the space charge force while the second term represents the generalized v 1 force FP m mc 2 2 . 2 2 ponderomotive This ponderomotive force is responsible for generation of plasma waves. In order to analyze the excitation of plasma waves, perturbation technique is used to expand the Lorentz force, continuity and Poisson’s equations in various orders of the laser field amplitude. The zeroth order describes the equilibrium plasma n n0 , 0 1 and 0 0 . The first order is the electron quiver motion of the plasma electron in the laser field v 1 ca and 30 n 1 1 1 0. The higher order expansion of the momentum, continuity and Poisson’s equations yields 2 1 v 2 a 4 c 2 t (1.21) n n0 .v 0 t (1.22) 4e 2n . mc 2 (1.23) and 2 2 Differentiating Eq. (1.22) with respect to time and substituting Eq. (1.21) and Eq. (1.23) gives the equation governing the evolution of the slow density perturbation as, 2 a 2 n 2 2 k P2 2 . 4 c t n0 (1.24) In order to solve Eq. (1.24), the quasi-static approximation [57-61] is used. Under the quasi-static approximation (QSA) it is assumed that the electron transit time (distance) through the laser pulse is short in comparison with the characteristic laser pulse evolution time (distance). This implies that, QSA is valid if L E L Z R , where L L c 31 is the laser pulse duration and E is the laser pulse evolution time, which is on the order of Rayleigh time Z R c . Transforming independent variables z ct and t (or z z ) in the plasma fluid equation (1.24) and neglecting the derivative with respect to ( z ) (under QSA) gives, 2 2 2 2 n 2 k P 2 n0 2 a . 4 (1.25) Eq. (1.25) represents the governing equation for the generation of plasma waves (wakefields) [62-71]. It has been shown [72] that if the laser pulse duration is approximately equal to the plasma wave period a large amplitude plasma wave (wakefield), with phase velocity close to the speed of light, is generated. This large amplitude wakefield can be used for acceleration and/or focusing of electron bunches. Accelerating gradients as high as a few tens of GV/m have been measured in experiments. These gradients are approximately three orders of magnitude higher than those achieved in conventional radio frequency linear accelerators. The evolution of the density perturbation can be reduced under two separate conditions viz 1) long pulse, and 2) ultrashort pulse regimes. For a sufficiently long laser pulse such that 1 P and L r0 , Eq. (1.25) reduces to n 2 1 a . 2 2 n0 k P r0 4 (1.26) 32 It may be noted that for a broad beam k P r0 1 , the right side of Eq. (1.26) will be much less than a 2 4 . Since a 2 4 represents the contribution of relativistic nonlinearity in Eq. (1.9), it may be concluded that for a broad beam, relativistic nonlinearity will dominate over pondermotive effects. However for a narrow beam k P r0 1 ponderomotive effects will dominate over relativistic effects. For an ultrashort laser pulse L P Eq. (1.25) reduces to 2 n 2 2 2 n0 2 2 a . 4 (1.27) Further, if the laser spot is broad r0 L the transverse ponderomotive effect is negligible and n a 2 4 . In this regime the effect of relativistic nonlinearity is exactly cancelled by the axial ponderomotive effect n n0 a 2 4 in Eq. (1.9) [73]. Hence the laser amplitude of an ultrashort pulse is driven by a linear source. However for narrow laser beams r0 L the transverse ponderomotive effect becomes significant and affects the propagation dynamics [74]. 1.2(c) Laser pulse compression In order to analyze the compression dynamics of short laser pulses in plasma, it becomes important to study its nonparaxial propagation since finite pulse length and group velocity dispersion effects [75-79] become significant. Relativistic and 33 ponderomotive nonlinearity arising due to laser-plasma interaction provides the source for laser pulse compression. Theoretical and simulation studies have shown that two colliding laser beams in plasma lead to laser pulse compression [80-88]. Theoretical and experimental work has also shown the possibility of obtaining pulse compression in plasma using a single laser pulse. The interplay of relativistic self-phase modulation (SPM), group velocity dispersion (GVD) and the presence of high amplitude nonlinear plasma waves can lead to laser pulse self-compression. Considering the nonparaxial wave equation (1.11) and assuming ar , z, to be slowly varying with propagation distance, the higher order diffraction term 2 z 2 is neglected in comparison to 2k 0 z . Also in the limit L Z R 1 c 2 k 02 02 2 the mixed derivative term 2 2 z is neglected in comparison to 1 g2 2 2 . With these approximations, the one-dimensional form of Eq. (1.11) is given by 2 a 2 2 2 2 2 a . 2 ik 1 a k 1 k 1 g P 0 P 0 z 4 2 (1.28) While deriving Eq. (1.28), density perturbations have been neglected since it is assumed that r0 L p . In order to solve Eq. (1.28), a trial function for the laser amplitude is assumed as 2 i 2 a f z exp i 2 L (1.29) 34 where f z and are the amplitude and chirp parameter of the laser pulse respectively. The evolution of the laser pulse length may be analyzed with the help of the heuristic method. In this context, the trial function (Eq. 1.29) is substituted into the Eq. (1.28) to give 1 f z i 2 2 L i 2 2ik 0 3 a z L z 2 z f z z 4 2 4 2 8i 2 2 2i 1 g2 4 2 2 2 a L L L k P2 f 2 z 2 2 1 2 a k P2 k 02 P2 1 a . 4 L (1.30) Comparing imaginary and real parts and equating coefficients of 2 and 0 on both sides of Eq. (1.30), the chirp, amplitude, length and phase of the laser pulse respectively evolve as 1 k0 L , 2 2 L 1 g z (1.31) L0 , L (1.32) f z f 0 2 2L 4 1 g z 2 L3 k 02 1 k 2 2 g 2 P f 02 L0 2k 02 L2 , 35 (1.33) and 1 g2 k P2 f 2 z 1 k P2 k 02 P2 1 . 2 z 8 k 2 k k0 L 0 0 (1.34) The first term on the right side of Eq. (1.33) leads to pulse broadening on account of group velocity dispersion whereas the second term leads to compression due to effect of relativistic nonlinearity. Figs. 1.3 and 1.4 respectively show the variation of normalized pulse length L L0 with propagation distance z Z R in the absence and in the presence of nonlinearity for f 02 0.05, r0 20m, L0 15m and P 10m . It is seen that in the absence of nonlinearity the laser pulse broadens slightly (Fig. 1.3) with propagation distance while in the presence of nonlinearity pulse length compression is observed (Fig. 1.4). 36 1.005 1.004 1.003 L L0 1.002 1.001 1 0.999 0 1 2 3 z ZR 4 5 6 Fig. 1.3 Normalized pulse length ( L L0 ) against normalized propagation distance ( z Z R ) in the absence of nonlinearity. 37 1.1 1 L L0 0.9 0.8 0.7 0 1 2 3 4 5 6 z ZR Fig. 1.4 Normalized pulse length ( L L0 ) against normalized propagation distance ( z Z R ) in the presence of nonlinearity. 1.3 Propagation of a laser beam in a plasma channel For most laser-plasma applications it is necessary that the laser beam should propagate several Rayleigh lengths in plasma. Since short laser pulses do not self-focus in 38 homogeneous plasma (Sec.1.2a), pre-formed plasma channels have been proposed [8994] as a means for allowing extended propagation distances for short pulses. There are several techniques for creating a plasma channel. In the hydrodynamic expansion [95-96] approach, a laser pulse having energy ~100 mJ and length ~100 ps, is focused with an axicon to generate a line focus in a gas at an ambient pressure of about 100 mbar. The intensity at the line focus 1013 1014 Wcm 2 , ionizes the gas and heats the resulting plasma by inverse bremsstrahlung (IB). The hot plasma column so formed then expands on a nanosecond time scale, driving a shock wave into the surrounding cold gas and leaving a plasma channel behind the shock front. The plasma channels formed by this method are not fully ionized, and so may only be used below the intensity at which substantial further ionization of the channel would occur. In the heater-ignitor method, [97-98] a short (<100fs), intense 5 1014 Wcm 2 ignitor pulse produces initial ionization by optical field ionization (OFI). This initial plasma is then heated and further ionized by a long (~100ps) “heater” pulse of relatively low intensity. This approach is implemented by overlapping the line foci produced by focusing the ignitor and heater beams with cylindrical mirrors. Cylindrical channels are formed if the ignitor and heater beams propagate perpendicular to each other and common line focus. This technique has been used to guide laser pulses with a peak input intensity as high as 1019 Wcm 2 over 4mm. Plasma channels have also been formed by the opposite process i.e. hydrodynamic compression, [99-100] using fast capillary discharges. In this approach a capillary of a few millimeters diameter is filled with gas at low pressure and ionized by a discharge current with a rise time of 10-50 ns, and a peak current of 5-20 kA. Since the 39 current rises rapidly, the skin effect ensures that the ionization occurs close to the capillary wall. The large magnetic field generated by the current then compresses the plasma through the J B force to drive a strong shock towards the capillary axis. A plasma channel is formed just before the rapidly collapsing annulus of plasma reaches the axis. Plasma channels have also been formed in slow capillary discharges [101-102]. In this technique, a discharge pulse with a rise time of the order of 100 ns and a peak current of a few hundred amperes is passed through an initially evacuated capillary formed in a soft material such as polypropylene. This discharge current ablates and ionizes the wall material to fill the capillary with plasma and forms a plasma channel by radiative and collisional heat transfer to the capillary wall. This causes the temperature of the plasma to be greater on axis and since the pressure across the capillary is uniform, an axial minimum in the plasma density is achieved. In order to study the evolution of the laser spot in a plasma channel, consider a laser beam propagating in a pre-formed plasma channel. The paraxial wave equation (Eq. (1.12)) describing the evolution of the laser beam amplitude in a parabolic plasma density channel modifies to a 2 nr 2 2 2 2 2 2ik 0 z a k P 1 4 n r 2 a k 0 P 1 a 0 ch 40 (1.35) where n and rch are the channel depth and radius respectively. Using the same procedure as described in Sec. (1.2a), the evolution of the laser spot in a plasma channel is described by, 2 rs 4 k P2 f 02 r02 rs4 4 1 8 z 2 k 02 rs3 rM (1.36) where rM rch2 re n , re e 2 mc 2 is the classical electron radius. The third term on 14 the right side of Eq. (1.36) represents the channel focusing effect. It may be noted that the laser spot-size remains matched 2 rs z 2 0, rs r0 as it propagates in the plasma channel if the depth of the channel n is kept equal to a certain critical value given by nc 4n0 r ch2 k P2 r04 k P2 f 02 r02 1 . 8 (1.37) The laser spot evolution equation (1.36) can be analytically solved by assuming an oscillatory solution of the form rs2 A1 cos 2 k M 2 z A2 sin 2 k M 2 z (1.38) 41 where k M 2 Z RM is the betatron wave number and Z RM k 0 rM2 2 . A1 and A2 are constants which can be obtained with the help of initial conditions. Differentiating Eq. (1.38) gives 2r r A A2 2 2 s 2rs 2s 1 k M cos k M z . z 2 z 2 (1.39) Substituting Eq. (1.36) into Eq. (1.39) gives 8 r 2 s 2 2 k 0 rs z 2 k P2 f 02 r02 rs4 A A2 2 1 4 1 k M cos k M z . 8 rM 2 (1.40) Assuming that at z 0, rs r0 and rs z 0 Eq. (1.38) gives A1 r02 . (1.41) Substituting Eq. (1.41) into Eq. (1.39) and applying the same initial conditions, gives rM4 A2 2 r0 k P2 f 02 r02 1 . 8 (1.42) Now substituting Eq. (1.41) and Eq. (1.42) into Eq. (1.38) leads to 42 r02 r 2 2 s 4 rM 1 4 r0 4 k P2 f 02 r02 r 1 1 M4 8 r0 k P2 f 02 r02 1 cos k M z . (1.43) 8 The variation of spot-size with propagation distance is shown in Fig. 1.5. The laser and plasma parameters are f 02 0.15, 1m, P 10m, r0 10m , n 2 1018 cm 3 and rch 20m. Curve a represents the linear evolution of the laser spot (vacuum diffraction) while curve b represents the spot-size variation in homogeneous plasma in the presence of relativistic effects which reduce the diffraction of the beam. Curve c shows the spot-size evolution in a plasma channel in the presence of relativistic effects. It is seen that laser spot focuses and undergoes oscillation and thus remains confined within the channel. 43 2.5 a 2 b 1.5 rs r0 c 1 0.5 0 0 2 4 z ZR 6 8 10 Fig.1.5 Evolution of normalized spot-size versus normalized propagation distance for a) vacuum diffraction, b) homogeneous plasma and c) a plasma channel. 1.4 Variational technique Interest in nonlinear properties of short pulses propagating in plasma has grown tremendously during the last few years. The two main reasons for this interest are the (a) 44 possibility of undistorted laser pulse propagation over large distances for applications based on laser-plasma interaction such as particle acceleration and (b) the possibility of extreme compression of laser pulses resulting in pulse widths lying well into the femtosecond domain. Therefore, it is important to obtain differential equations for the evolution of the macroscopic quantities that characterize the laser profile. The laser parameters that undergo simultaneous evolution as the laser pulse propagates in plasma are its spot-size, amplitude, phase, pulse length, radius of curvature and centroid. One of the most powerful techniques for establishing the simultaneous evolution equations is the variational method. The variational structure for dissipationless dynamical equation relies on the existence of a Lagrangian density. The Lagrangian density for the wave equation (1.10) is written as a a a a a a a a 1 g2 l a . a ik 0 a a z z z z a a a 2 a 2 n k P2 aa aa k 02 P2 1 aa . z z 8 n0 (1.44) The correctness of this Lagrangian density, can be verified by using the Euler-Lagrange equation given by l l n k 1 x k x k l t t 0 45 (1.45) where a or a is the dependent variable. For independent variables x r, z, , k Eq. (1.45) reduces to l l n k 1 xk xk 0. (1.46) Replacing by a and x k by the independent variables z, and r in Eq. (1.46) gives l l a z a z l l 0 . a a (1.47) The wave equation is recovered when the value of l (Eq. (1.44)) is substituted into Eq. (1.47). This verifies the correctness of the Lagrangian density given by Eq. (1.44). Further, a system of partial differential equations is recast in terms of Hamilton’s principle according to which an action integral S ( d n rldt , where n is the number of spatial co-ordinates on which the variational field depends), is stationary with respect to independent, first-order variations of the dependent variables. Substituting the Lagrangian density into the action 0 r and performing explicit integrals ld dr across the transverse and axial coordinates yields a reduced action (reduced Lagrangian density) with only z as the independent variable. Thus with the help of the Euler- 46 Lagrange equation the evolution of the laser parameters with propagation distance is obtained. 1.5 Approach The present study deals with the nonlinear, nonparaxial propagation of short laser pulses in a parabolic plasma channel. The wave dynamics of laser pulses interacting with plasma has been described with the help of Maxwell’s, Lorentz force and continuity equations. A wave equation for the laser field is set up. Considering the mildly relativistic regime a perturbative approach is used to obtain the source driving the laser field amplitude. All independent variables describing the laser field amplitude are transformed into the pulse frame in order to include the role of finite pulse length and group velocity dispersion effect. Further, in this thesis a regime has been defined in which the group velocity dispersion effect dominates over the finite pulse length effect. An appropriate Lagrangian density has been obtained for the wave equation. Suitable trial function for the laser pulse amplitude is assumed and substituted into the Lagrangian density. This density is used to obtain the action integral. Integrating over r and leads to the reduced Lagrangian density. In this reduced form of the action integral the parameters of the trial function represent a set of dependent variables. With the help of the Euler-Lagrange equation, variation of the action with respect to the dependent variables yields a set of coupled differential equations for the evolution of the laser parameters with propagation distance. An analytical solution for the spot-size (pulse length) by considering the pulse length (spot-size) to be constant is derived. Further, 47 numerical methods are used to graphically analyze the simultaneous evolution of the laser spot-size and pulse length. The propagation dynamics of an initially chirped ultrashort laser pulse in a preformed plasma channel is studied. For ultrashort laser pulses, relativistic and ponderomotive nonlinearities cancel each other. Hence the source driving the laser amplitude becomes linear. In this limit, the evolution of the laser spot-size and phase shift has been obtained using the Variational technique. The variation in amplitude and frequency have been derived for a matched laser beam propagating in a plasma channel. A graphical analysis is presented for the effective pulse length and chirp parameter of the laser pulse due to its interaction with plasma. For short laser pulses, radial and axial ponderomotive forces acting on the plasma electron become significant. This leads to density perturbations which in turn generate electric and magnetic wakefields. The density perturbation has been derived with the help of second order expansion of Lorentz force, continuity and Poisson’s equations. The plasma response in the nonlinear regime has been examined within the quasi-static approximation (QSA) according to which the plasma fluid equation is a function of alone (Sec.1.2b). Assuming a wide channel the radial dependence of the plasma frequency has been neglected. Evolution equation for laser spot-size, pulse length and intensity have been obtained using the variational technique. As the pulse length approaches the plasma wavelength a singularity occurs. In this regime l’Hospital’s rule is used to derive the maximum L P density perturbation. Using this density perturbation the evolution equation for the laser spot, pulse length and intensity of the laser have been obtained in this regime. For a matched laser pulse numerical methods are 48 used to graphically analyze the evolution of the pulse length and intensity of the laser for the cases when the pulse length is greater than less than and equal to the plasma wavelength. 1.6 Aim The present study will be significant for applications such as laser plasma based accelerators where the laser intensity and pulse length have to be optimized with respect to the plasma wavelength. Since the laser pulse length and spot-size vary with propagation distance, it becomes important to study the simultaneous variation of both these parameters. Further, the possibility of compressing the laser pulse length for obtaining enhanced intensities can also be explored. The present work is aimed at a detailed theoretical analysis of the simultaneous evolution of the spot-size and length of a laser pulse propagating in a parabolic plasma channel. The effects of finite pulse length, group velocity dispersion, chirping and relativistic as well as ponderomotive nonlinearities have been taken into account. 49 Chapter 2 Simultaneous evolution of spot-size and length and induced chirping of short laser pulses in a plasma channel In this chapter, nonlinear, nonparaxial propagation of intense, short, Gaussian laser pulses in a pre-formed plasma channel having a parabolic radial density profile has been studied [103]. Taking into account the effect of group velocity dispersion, the wave equation describing the evolution of the laser field amplitude driven by relativistic nonlinearity has been set up. Chirping of the laser pulse induced due to propagation in plasma is analyzed and a comparison of group velocity dispersion and self-phase modulation induced chirp is presented. Variational technique is used to obtain equations describing the simultaneous evolution of the laser spot-size and pulse length in the plasma channel. Numerical methods are used to study the simultaneous evolution of the laser spot and pulse length. 2.1 Evolution of spot-size and pulse length 50 Consider the propagation of a linearly polarized laser pulse in a pre-formed plasma channel having a parabolic density profile of the form n(r ) n0 (nr 2 rch2 ) , where n0 is the ambient plasma density and n and rch are the channel depth and radius respectively. The vector potential of the radiation field is given by, A A xˆ (r , z , t ) exp( ik 0 z i 0 t ) c.c. 2 (2.1) where A( r , z , t ) , k 0 and 0 are the amplitude, wavenumber and frequency of the laser field respectively. The wave equation governing the evolution of the vector potential of the radiation field is given by 2 1 2 4 nr ev. 2 2 A c c t (2.2) While deriving Eq. (2.2), Coulomb gauge . A 0 has been used. Also considering the limits r0 L, k P L 1 , where k P 4n0 e 2 mc 2 12 is the plasma wavenumber, the ponderomotive nonlinearity has been neglected (Sec.1.2(b)). In this limit, only the relativistic nonlinearity will drive the laser field. In Eq. (2.2), the relativistic plasma electron velocity v ( eA mc , where is the relativistic factor) is obtained with the help of Lorentz force equation (1.7). Substituting the value of plasma electron density and relativistic electron velocity into Eq. (2.2) the wave equation reduces to 51 nr 2 a 2 nr 2 a 2 2 1 2 2 a , ( 2 2 2 )a k P 1 4 z c t n0 rch2 n0 rch2 4 2 (2.3) where a eA mc2 1 is the normalized vector potential. The second, third and fourth terms on the right side of Eq. (2.3) are due to plasma channel, relativistic nonlinearity and coupling of relativistic nonlinearity with the plasma channel (channel coupling). Substituting Eq. (2.1) into Eq. (2.3) and transforming independent variables z, t to z, ( z g ct where g v g c the normalized is group velocity of the pulse) gives, ( 2 2ik 0 2 2 2 2 2 (1 g2 ) 2 20 k 02 k P2 2 )a(r , z, ) z z c z a 2 nr 2 k 4 n0 rch2 2 P a 2 1a(r , z, ). 4 (2.4) Assuming ar , z, to be slowly varying with z, the higher order diffraction term 2 z 2 may be neglected in comparison with 2k 0 z . The mixed derivative term 2 2 z is neglected in comparison with the term describing the group velocity dispersion effect (1 2 g ) 2 2 in the limit k 0 L 1 k P2 r02 4. Thus Eq. (2.4) reduces to 2 02 2 ( 2ik 0 (1 g ) 2 2 k 02 k P2 )a(r , z, ) z c 2 a 2 nr 2 k n0 rch2 4 2 P a 2 1a(r , z, ). 4 52 (2.5) The Lagrangian density for Eq. (2.5) is written as, * * 02 a * * a 2 a a l a . a ik 0 (a a ) (1 g ) 2 k 02 k p20 aa z z c 2 a 2 a *2 a 2 a *2 nr 2 * nr k aa . 8 n0 rch2 n0 rch2 8 2 P (2.6) In order solve the wave equation (2.5), a trial function is assumed as, i z 2 2 i z r 2 r2 a f ( z ) exp i z 2 2 2 2 , L z L z rs z rs z where (2.7) f , rs , L , , and k 0 rs2 2 Rz represent the laser amplitude , spot-size, pulse length, phase, chirp and curvature respectively. In Eq. (2.7) the radial beam as well as axial pulse profiles of the laser are assumed to be Gaussian. Substituting Eq. (2.6) into the action integral 0 r ld dr yields the reduced Lagrangian density, f lˆ 2 z L1 2 2 2 k 0 f 2 z Lrs2 2 2 f 2 z rs2 1 g2 1 2 4 2L 1 2 L 1 2 rs z 4 z L z 2 r z z s f 2 z rs2 L 02 2 k 02 k P2 c 4 2 f 4 z rs2 L f 4 z rs4 Ln f 2 z rs4 Ln k P2 . 128 512n0 rch2 8 2n0 rch2 53 (2.8) The Euler-Lagrange equation for various laser parameters j j 1, 2,.......6 , , rs , , L and f 2 is given by lˆ z j z ˆ l 0 . j (2.9) Substituting the reduced Lagrangian density (Eq. (2.8)) into Eq. (2.9) for each value of j leads to equations relating various laser parameters with each other and a set of coupled differential equations describing the evolution of the laser parameters. Thus for 1 , Eq. (2.9) gives, ˆ l lˆ 0. z z (2.10) Substituting Eq. (2.8) into Eq. (2.10) leads to 2 2 f rs L 0 z (2.11) Eq. (2.11) shows the conservation of energy of the laser pulse. Therefore, 54 f 2 rs2 L f 02 r02 L0 constant M (2.12) and f z f 0 r0 L0 (2.13) rs L where f 0 , L0 , r0 are the initial values of amplitude, pulse length and spot-size respectively. For 2 , Eq. (2.9) gives, lˆ lˆ 0. z z (2.14) Substituting Eq. (2.8) into Eq. (2.14) yields, 1 2 k 0 rs 0. rs2 rs z (2.15) Solving Eq. (2.15) gives the evolution of with propagation distance as k 0 rs rs . 2 z (2.16) 55 In order to obtain the evolution equation for the laser spot-size, consider 3 rs . Thus Eq. (2.9) gives lˆ z rs z ˆ l 0 . rs (2.17) Substituting Eq. (2.8) into Eq. (2.17) gives, 1 rs 2 1 2 2M nrs r k0 2 k 0 2 s k P2 0. 3 3 2 z rs 32 r L 2 n r r rs z rs z s 0 ch s (2.18) The evolution equation for the laser spot-size is obtained by substituting Eq. (2.16) into Eq. (2.18) as, 2 rs 4 2 3 2 z k 0 rs where P rs4 1 4 Pc rM P Pc 2 f 02 r02 L0 k P2 64L represents the laser power normalized by critical Pc 2 2cLe 202 L0 re2P2 GW (2.19) power for self-focusing, rM4 rch2 re n and re e 2 mc 2 is the classical electron radius. The first term on the right side of Eq. (2.19) represents vacuum diffraction, the second term representing relativistic self-focusing effect is a function of the pulse length and the third term leads to channel focusing. The matching condition of the laser spot as it propagates in the plasma channel is obtained by 56 assuming that rs r0 , 2 rs z 2 0 and that the pulse length remains constant L L0 with propagation distance. With these conditions, Eq. (2.19) gives n nc 4rch2 n0 k P2 r04 2 f 02 r02 k P2 1 64 . (2.20) The critical density nc [104-105] represents the density gradient for which the laser spot-size remains matched rs r0 as it propagates in the plasma channel, when the evolution of the pulse length is ignored. Similarly substituting 4 into Eq. (2.9) gives, lˆ z z lˆ 0. (2.21) Substitution of the Lagrangian density leads to 1 g2 1 2 k 0 L 0. L z L2 (2.22) Solving Eq. (2.22) gives the evolution of chirp with propagation distance as k 0 L L . 2 1 g2 z (2.23) 57 In order to obtain the evolution of the laser pulse length, 5 L is substituted into Eq. (2.9). Thus, lˆ lˆ 0, z L L z (2.24) and 2 2 1 L k 0 L 2 1 g 1 k0 2 2 L3 L z L z L z 2k P2 M 2k P2 Mn 32rs2 L2 128n0 rch2 L2 (2.25) Substituting the value of chirp parameter from Eq. (2.23) into Eq. (2.25) gives 2 2 2 (1 g2 )k P2 M nrs2 1 2 L 4(1 g ) 1 ( 1 ) . z 2 k 02 L3 16k 02 rs2 4n0 rch2 L2 58 (2.26) The first term on the right side of Eq. (2.26) represents the linear contribution due to group velocity dispersion while the second term consists of the terms due to relativistic nonlinearity and its coupling with the plasma channel. The shift of central wave number k z of the laser pulse can be obtained from Euler-Lagrange equation (2.9) by substituting 6 f lˆ z f 2 z 2 z , as ˆ l 0 , f 2 (2.27) or 1 L Lr 2 1 2 L 1 2 rs r2 1 g2 1 2 s k L z 2 rs z z 2L z 4 z 2 s 0 f 2 rs2 L f 2 rs4 Ln rs2 L 02 nrs4 L 2 k 02 k P2 2k P2 0. 2 c 128n0 rch2 4 2n0 rch2 32 (2.28) Substituting Eqs. (2.16) and (2.23) into Eq. (2.28) gives 2 2 k 0 L 2 L k 0 rs 2 rs 1 g rs rs2 L 02 2 k 02 k P2 L Lr k 2 z 8 1 2 z 2 4 z 2L 2 c g 2 s 0 f 2 rs2 L f 2 rs4 Ln nrs4 L 2k P2 0. 128n0 rch2 4 2n0 rch2 32 59 (2.29) Further, substituting Eqs. (2.19) and (2.26) into Eq. (2.29) gives 2k P2 f 02 r02 L0 2 1 1 1 g 2 2 z k 0 r0 rs k 0 L2 128k 0 rs2 L 2 5nrs2 7 . 4n0 rch2 (2.30) The third and fourth terms on the right side of Eq. (2.30) represent the phase shift induced by GVD and relativistic nonlinearity respectively. 2.2 Analytical solution for laser spot-size and pulse length The laser spot evolution equation (2.19) can be analytically solved by assuming the pulse length to remain constant L L0 . Multiplying Eq. (2.19) by 2rs z and integrating with respect to z gives, r2 4 4 P rs s2 A 2 2 2 2 k 0 rs k 0 rs Pc 0 Z RM z 2 (2.31) where P Pc 0 2 f 02 r02 k P2 64 and Z RM k 0 rM2 2. The constant A is determined with the help of the initial condition rs r0 , rs z 0 at z 0 as 60 r02 4 4 P A 2 2 2 2 2 . k 0 r0 k 0 r0 Pc 0 Z RM (2.32) Substituting Eq. (2.32) into Eq. (2.31) yields 4 rs 2 2 k 0 rs z 2 P 4 1 2 2 Pc 0 k 0 r0 r2 P rs2 1 2 02 . Pc 0 Z RM Z RM (2.33) Multiplying both sides of Eq. (2.33) by rs2 gives 2 2 1 4 Z 2 P 2 2 4Z RM rs r0 rs r 2 2 RM2 1 Z RM k 0 r0 Pc 0 k 02 z 2 s P 4 1 rs Pc 0 (2.34) or rs 1 z Z RM rs 2 4Z RM 2 2 k 0 r0 2 P 2 2 4Z RM 1 r0 rs 2 k0 Pc 0 12 P 4 1 rs . Pc 0 (2.35) Integrating Eq. (2.35) with respect to z gives rM4 2 r0 rs rs P 2 2 P 4 1 r0 rs rM4 1 rs P P c0 c0 12 Substituting rs2 t , 2rs rs t in Eq. (2.36) gives 61 1 Z RM z . (2.36) 1 2 r 4 M2 r0 t P 2 P 2 1 r0 t rM4 1 t Pc 0 Pc 0 12 1 Z RM z . (2.37) Solving Eq. (2.37) gives 1 2 4 1 rM 4 r02 t P 2 1 rM4 1 r0 t 2 Pc 0 2 r0 2 P 2 1 r0 Pc 0 2 12 1 Z RM z . (2.38) Solving the integrals in Eq. (2.38) gives 1 rM4 P 2 r0 t 2 1 2 P r 1 1 c0 0 z B . sin 4 2 1 rM 1 P r 2 Z RM 2 r 2 P 0 c0 0 (2.39) Since rs r0 at z 0 the constant of integration is given by 2 1 rM4 P 2 r0 r 1 0 2 r02 Pc 0 1 1 . B sin 4 2 4 1 rM 1 P r 2 2 r2 P 0 c0 0 62 (2.40) Therefore Eq. (2.39) leads to 2 1 rM4 P 2 r0 rs 2 1 2 r0 Pc 0 cos 2 z 4 Z RM 1 rM 1 P r 2 2 r2 P 0 c0 0 (2.41) or rs2 r02 rM4 1 2 r04 P rM4 1 1 4 P c 0 r0 P 1 cos k M z Pc 0 (2.42) where k M 2 Z RM is the wavenumber describing the oscillation of the laser spot-size. Similarly the pulse length evolution equation (2.26) can be analytically solved by assuming the spot-size to remain constant rs r0 . Multiplying both sides of Eq. (2.26) by 2L z and integrating with respect to z gives U 2V L C1 2 L L z 2 where U 4 1 g2 k 02 and V (2.43) 2 1 k 2 g 2 P M 16k 02 rs2 1 nrs2 4n0 rch2 . C1 is the constant of integration which can be determined by applying the initial condition dL dz 0 , L L0 at z 0 . Thus, 63 C1 U 2V . L20 L0 (2.44) Substituting Eq. (2.44) into Eq. (2.43) gives U 2VL0 L2 2VL20 L UL20 . L L20 L2 z 2 (2.45) Assuming U 2VL0 Q, 2VL20 D and UL20 E , Eq. (2.45) reduces to QL2 DL E L . z L0 L (2.46) Integrating both sides of Eq. (2.46) with respect to z and multiplying by 2Q gives 2QL QL2 DL E L 1 2Qz . L0 (2.47) Substituting QL2 DL E x, 2QL DL x into the first term on the left side of Eq. (2.47) gives x x D QL DL E 2 L 1 2Qz . L0 64 (2.48) Solving Eq. (2.48) gives 2 QL 2VL L UL 2 2 0 2 0 VL20 2VL20 L UL20 2 log L L . Q Q Q Q 2VL20 2Q z C2 . L0 (2.49) The constant C2 is obtained with the help of the initial condition that at z 0, L L0 . Therefore, C2 UL VL0 log 0 . Q U 2VL0 2VL20 (2.50) Substituting Eq. (2.50) into Eq. (2.49) gives 2U 2VL0 z 2VL20 2 2 2 2 (U 2VL0 ) L 2VL0 L UL0 L0 U 2VL0 UL VL 0 log 0 U 2VL0 VL20 2VL20 UL20 2 log L L U 2VL0 U 2VL0 U 2VL0 . (2.51) The evolution of the laser spot-size and pulse length as given by Eqs. (2.19) and (2.26) are graphically depicted in Fig. (2.2) of Section (2.3). 2.3 Numerical solution for simultaneous evolution of laser spot-size and pulse 65 length The simultaneous evolution of the laser spot and pulse length in homogeneous as well as inhomogeneous plasma is studied numerically by solving equations (2.19) and (2.26), using the fourth order Runge Kutta method, with the assumption that at z 0, rs z 0, rs r0 33m, L z 0, L L0 14m. The other laser and plasma parameters are f 02 0.03, 1m and p 10m. Fig. 2.1 shows a comparison between the evolution of the normalized pulse length L L0 with propagation distance z Z R for a laser pulse propagating in homogeneous plasma curve a and in plasma channel with n 2 1017 cm 3 and rch 50 m 1.002 1 0.998 0.996 L L0 0.994 a 0.992 b 0.99 0.988 0 0.2 0.4 z Z R 0.6 66 0.8 1 1.2 a Fig.2.1 Variation of normalized pulse length L L0 with propagation distance z Z R in the absence of (curve a) and in the presence (curve b) of the plasma channel for f 02 0.03 , 1m, r0 33m, L0 14m P 10m, n 2 1017 and rch 50m . (curve b). It is seen that compression of the laser pulse length occurs for both cases. However, in the presence of the channel compression is enhanced in comparison to the homogeneous case. This is due to the combined effects of relativistic nonlinearity and plasma channel. Fig. 2.2 depicts the simultaneous evolution of the spot-size (curve a ) and pulse length (curve b ) of a laser pulse propagating in a plasma channel. Curve c (curve d) shows the variation of the spot-size (pulse length) when the pulse length (spot-size) is non-evolving. All the parameters are the same as in Fig. 2.1. It is seen that the laser pulse length compresses for both cases due to the dominance of relativistic nonlinearity over GVD effects. However, curve b shows more compression in comparison to curve d due to the evolution of the spot-size. Curve a shows that the focusing of the spot-size improves since its amplitude of oscillation decreases, while the spot-size is seen to oscillate with constant amplitude in curve c . In the former case the evolution of the pulse length leads to a reduction of the spot-size. 67 The simultaneous variation of the normalized spot-size rs r0 and normalized pulse length L L0 with the normalized propagation distance, keeping the channel density gradient equal to the critical density ( n nc 0.238 1018 1 9.4 f 02 cm 3 , Eq. (2.20)), is plotted in Fig. 2.3. The set of curves a, b and c (d, e and f) variation represent of the laser spot size (pulse length) for 1.1 1 c a 0.9 rs L r0 L0 0.8 d b 0.7 0.6 0 1 2 3 4 5 6 7 z ZR Fig.2.2 Simultaneous variation of normalized spot size rs r0 (curve a) and the normalized pulse length L L0 (curve b) with normalized propagation distance z Z R . Evolution of the spot-size keeping the pulse 68 the length constant (curve c). Evolution of the pulse length keeping the spot size constant (curve d) for f 02 0.03, 1m, r0 33m, L0 14m, P 10m, rch 50m and n 2 1017 . 1.1 a b c 1 rs L r0 L0 0.9 d e 0.8 f 0.7 0 1 2 z ZR 3 4 5 Fig.2.3 Simultaneous variation of normalized spot-size rs r0 (curves a, b and c) and the normalized pulse length L L0 (curves d, e and f ) with normalized propagation distance 69 f 02 0.03 n c 1.7 1017 cm 3 , 0.04 n c 1.4 1017 cm 3 and 0.05 n c 1.2 1017 cm 3 , 1m , r0 33m, L0 14m, P 10m and rch 50m . . different laser intensities f 02 0.03, 0.04 and 0.05 respectively. All other parameters are the same as in Fig. 2.1. The critical density represents the density gradient for which the laser spot-size remains matched rs r0 as it propagates in the plasma channel, without considering the evolution of the pulse length. Consideration of the pulse length evolution in the present study leads to mismatched propagation of the spot-size. Also when the initial laser intensity is increased, mismatching and compression of the laser pulse increases with propagation distance. Fig. 2.4 shows a plot of the evolution of laser intensities corresponding to the parameters used in Fig. 2.3. It is seen that for higher initial laser intensities, the rate of increase in intensity enhances due to rapid compression of the laser pulse and decrement in the spot-size with propagation distance. 2.4 Group velocity dispersion and self-phase modulation induced chirping of short laser pulses in a plasma channel Consider a matched n nc laser beam propagating in the plasma channel. The variation of frequency across the laser pulse may be obtained by writing the resultant phase of the laser pulse as, 2 2 . L (2.52) 70 0.08 c 0.07 0.06 b 0.05 f 2 z 0.04 a 0.03 0.02 0.01 0 0 1 Fig. 2.4 Variation of 2 intensity z ZR for the 3 initial 4 5 values f 02 0.03 n c 1.7 1017 cm 3 , n c 1.2 1017 cm 3 . Other laser plasma parameters are 1m , 0.04 n c 1.4 1017 cm 3 r0 33m, L0 14m , P 10m and rch 50m. The frequency shift across the laser pulse (chirp) is given by 71 and 0.05 . t t (2.53) Combining Eqs. (2.52) and (2.53) and substituting t v g gives 2v g L2 . (2.54) Eq. (2.54) indicates that if 0 ( 0) the laser pulse will be positively (negatively) chirped i.e. the frequency increases (decreases) from the front to the back of the pulse [106]. Further, substituting the value of ( Eq. (2.23)) into Eq. (2.54) leads to v g k 0 L 1 2 g L . z (2.55) Eq. (2.55) shows that the frequency chirp is a function of propagation distance and varies with the laser pulse length evolution. Since the pulse length evolves (Eq. (2.26)) primarily on account of GVD and SPM [107-108], therefore GVD as well as SPM are also responsible for inducing chirp of the laser pulse. In Fig. 2.5, solid 72 0.05 0.04 d 0.03 f 0.02 0.01 0 b 0 0 1 2 3 4 5 z ZR 6 e -0.01 -0.02 c -0.03 a -0.04 -0.05 Fig. 2.5 Variation of normalized frequency 0 with z Z R . Solid (dotted) curve a (curve d) , curve b (curve e), curve c (curve f) are due to SPM, GVD and combined effect of SPM and GVD at front (back) 0.5 (-0.5) of the pulse for f 02 0.03, 1m, P 10m , r0 33m, L0 14m, rch 50m and n nc 1.7 1017 cm -3 . curves (dotted curves) a, b and c d , e and f show the variation of frequency induced chirp due to SPM, GVD and combined effect of both, respectively at the front (back) of the laser pulse. All laser and plasma parameters are considered to be the same as in Fig. 73 2.3 for f 02 0.03 . Curve a (d) shows that due self-phase modulation the frequency at the front (back) of the pulse decreases (increases). Group velocity dispersion leads to a converse frequency variation as seen in curves b and e. It may be noted that when both effects are taken into account SPM dominates over GVD since curve c (f) follows curve a (d) with a lesser magnitude. Therefore GVD effects tend to reduce the chirp generated by self-phase modulation of the laser pulse. Frequency variation of the pulse at a given normalized propagation distance z Z R is shown in Fig. 2.6. Curves a and b show frequency variation at z Z R 3 and z Z R 6 respectively, all other parameters being the same as in Fig. 2.5. It is seen that the laser frequency varies linearly over the pulse. The variation of the normalized induced chirp 0 is negative (red shifted) near the leading edge and becomes positive (blue shifted) near the trailing edge of the pulse. Since the instantaneous frequency increases linearly from the leading to the trailing edge, the laser pulse is positively (up) chirped. Fig. 2.7 shows the variation of the intensity f z, f 2 2 0 L0 L exp 2 2 L2 across the matched laser pulse. Curve a shows the initial intensity distribution at z Z R =0 while curves b and c depict the intensity variation after the pulse has propagated a distance z Z R 3 and 74 0.06 0.04 0 0.02 0 -1 -0.5 0 0.5 L0 1 -0.02 a -0.04 b -0.06 Fig. 2.6 Variation of normalized chirp 0 across the laser pulse after traversing distance z Z R 3 (curve a) and z Z R 6 (curve b) for f 02 0.03, 1m, P 10m, L0 14m, r0 33m, rch 50m . 75 n nc 1.7 1017 cm -3 and 0.045 c 0.04 0.035 b 0.03 a 0.025 0.02 f 0.015 2 z, 0.01 0.005 0 -1.5 -1 Fig.2.7 Variation -0.5 of intensity f 0 2 z, 0.5 with after pulse 1 1.5 has traversed a distance z Z R 0 (curve a), z Z R 3 (curve b) and z Z R 6 (curve c) for f 02 0.03, 1m, P 10m, L0 14m, n nc 1.7 1017 cm -3 r0 33m, and rch 50m. 76 z Z R 6 respectively. All other laser-plasma parameters being the same as in Fig. 2.5. It is seen that the intensity increases with respect to the initial intensity as the propagation distance increases. Chapter 3 Propagation of ultrashort chirped laser pulses in a plasma channel 77 In this chapter, propagation of an initially chirped, Gaussian laser pulse in a preformed parabolic plasma channel is analyzed [109]. The pulse is considered to be ultrashort, so that relativistic and ponderomotive nonlinearities cancel each other and the source driving the laser amplitude becomes linear. Evolution of the laser spot-size and phase shift, with propagation distance of the laser pulse is obtained using a variational technique. The effect of initial chirp on the laser pulse length and intensity of a matched laser beam propagating in a plasma channel has been analyzed. Also the variation of the initial chirp parameter of the laser pulse, as it propagates in plasma, has been obtained and graphically depicted. 3.1 Analysis of wave equation Consider a linearly polarized, ultrashort laser pulse propagating in a pre-formed plasma channel of the form nr n0 nr 2 rch2 where n and rch are the channel depth and radius respectively. The vector potential of the laser field is given by Ar , z , t A xˆ exp ik 0 z i 0 t c.c. 2 (3.1) where Ar, z, t , k 0 and 0 are the amplitude , wavenumber and frequency of laser field respectively. For ultrashort ( L p , r0 ) laser pulses, relativistic and pondermotive nonlinearities cancel each other (Sec.1.2 b). Therefore, the wave equation governing the evolution of the normalized vector potential of such laser pulses is given by 78 nr 2 2 1 2 a 2 2 a k P2 1 c t n0 rch2 (3.2) 12 where a eA mc 2 and k P 4n0 e 2 mc 2 is the on-axis plasma. Substituting Eq. (3.1) into Eq. (3.2) and transforming independent variables z, t to z , ( z g ct , where g ( v g c) is the normalized group velocity) leads to 2 2 2 2 2 ik ( 1 ) ar , z, g 0 z 2 z 2 nr 2 = k P2 1 n0 rch2 k 02 P2 1 ar , z , (3.3) where p ( 0 ck 0 ) is the phase velocity of the laser pulse. The terms 2 2 z and 1 2 g 2 2 on the left side of Eq. (3.3) represent finite pulse length and GVD effects respectively. Assuming ar , z, to be slowly varying with z , the higher order diffraction term 2 z 2 on the left side of Eq. (3.3) is neglected in comparison to 2k 0 z . Thus Eq. (3.3) reduces to 2 2 2 2 ik ( 1 ) a(r , z, ) g 0 z 2 79 nr 2 k P2 1 n0 rch2 k 02 ( P2 1) a(r , z, ) . (3.4) Considering a chirped Gaussian laser pulse, the solution of Eq. (3.4) may be written in the form of a trial function given by i z, r 2 r2 ar , z, bz, exp i z, 2 2 rs z, rs z, where b( z , ) ( f ( z, ) exp( 2 (1 i ) L20 ), f ( z, ), L0 and (3.5) being the pulse amplitude, constant length and constant chirp parameter respectively), ( z , ) , ( z, ) and rs ( z, ) represent the phase, radius of curvature and spot-size of the laser beam respectively. Taking the Fourier transform of Eq. (3.4) with respect to gives 2 nr 2 2 2 2 2 2 ˆ ˆ 2 ik a k 1 k ( 1 ) k ( 1 ) k p 0 p g ak , z n0 rch2 (3.6) where k k 0 k , k is the spread in laser wavenumber and the Fourier transform of a( ) is given by aˆ k 1 2 d exp( ik )a( ). (3.7) 80 In order to obtain the Fourier transform of the trial function, Eq. (3.5) is substituted into Eq. (3.7). Thus i z, k r 2 r2 f z, k exp i z, k 2 2 rs z, k rs z, k 2 1 aˆ k 2 exp 2 1 i ik d . L0 (3.8) 2 2 4 p where p 1 i L20 and q ik , Eq. Since exp px qx dx p exp q (3.8) gives aˆ k f z, k L0 2 1 i 12 k 2L20 i z, k r 2 r2 , exp i z, k 2 2 4 1 i r z , k r z , k s s (3.9) or aˆ k f z, k L0 1 i 1 2 1 2 12 2 k 2L20 ir 2 r2 . exp 1 i i z , k 2 2 2 4 1 r z , k r z , k s s (3.10) Assuming 1 i r cos1 i sin 1 r exp i1 where r 1 2 and 1 tan 1 , Eq. (3.10) leads to, i z, k r 2 r2 aˆ k bk z, k exp i z, k 2 2 rs z, k rs z, k 81 (3.11) where the beam amplitude in k - space is given by bk z , k f z , k L0 1 2 1 4 2 k 2 L20 1 i i tan 1 . exp 2 2 4 1 (3.12) Applying a variational technique, the Lagrangian density of Eq. (3.6) is given by aˆ a l aˆ k . aˆ k ik aˆ k k aˆ k k z z nr 2 + k P2 1 n0 rch2 k 02 ( p2 1) k 2 (1 g2 ) aˆ k aˆ k 0. (3.13) Substituting Eq. (3.11) into Eq. (3.13) and taking action integral 0 rdrl yields the reduced Lagrangian density f 2 rs2 L20 1 2 lˆ 4 k P2 2 r 2 n 1 s 2 2n r 0 ch 1 2 k 2 L20 exp 2 2 1 1 2 1 rs k 2 z 2 z rs z rs 1 k 2 1 g2 k 02 P2 1 . 2 82 (3.14) Proceeding lˆ z j z as in ˆ l 0 j Chapter 2, the Euler–Lagrange equation, where j j 1, 2,.......4 , , rs and f 2 define various laser parameters, is considered. Now substituting 1 and using the Lagrangian density (Eq. (3.14), the Euler–Lagrange equation gives 2 2 bk rs 0 , bk2 rs2 bk20 r02 z where (3.15) L0 k 2 L20 i 2 1 4 1 bk 0 f 0 (1 ) exp ( 1 i ) tan 2 2 2 4(1 ) is the expression for bk (Eq. 3.12) at z 0. Eq. (3.15) shows the power conservation relation. For 2 the Euler-Lagrange equation gives f 2 rs2 L20 1 2 z 8 1 2 k k 2 L20 exp 2 2 1 f 2 L2 2 1 2 0 4 f 2 L2 r 1 2 0 s 4 1 2 k 2 L20 exp 2 2 1 1 2 k k 2 L20 exp 2 2 1 rs 0. z (3.16) On account of the power conservation relation, the first term on the left side of Eq (3.16) vanishes. Thus 83 krs rs . 2 z (3.17) For 3 rs , the Euler-Lagrange equation gives k 1 2 k rs k P2 rs2 n 0. z rs rs rs2 rs z 4n0 rch2 (3.18) With the help of Eq. (3.17) the evolution of the laser spot-size is described by 2 rs 4 k P2 nrs4 1 . z 2 k 2 rs3 4n0 rch2 (3.19) Assuming rs r0 and 2 rs z 2 0 in Eq. (3.19) the critical channel depth is given by nc ( rch2 re r04 where re e 2 mc 2 is the classical electron radius). If the channel depth is equal to the critical channel depth the laser beam propagates with a constant spot-size which is equal to its beam waist (matched beam). For a matched laser beam, Eq.(3.19) reduces to 2 rs nrs4 4 1 z 2 k 2 rs3 nc r04 (3.20) 84 Eq. (3.20) shows the evolution of the laser spot-size in a parabolic plasma channel and is the same as that obtained in Ref. [110]. The Euler–Lagrange equation for amplitude of the laser pulse 4 f 2 z is given by f 2 k P2 2 f 2 r 2 L2 1 2 s 0 4 r 2 n 1 s 2 2n r 0 ch 1 2 k 2 L20 exp 2 2 1 1 2 1 rs k 2 z 2 z r z r s s 1 2 k 1 g2 k 02 P2 1 0 . 2 (3.21) Solving Eq. (3.21) gives, krs 2 rs k P2 rs2 rs2 n 1 1 kr 4 z 2 2 2n0 rch2 z 2 s rs2 k 2 1 g2 k02 p2 1 0 . 2 (3.22) Substituting Eq. (3.19) into Eq. (3.22) and using the linear dispersion relation 2 0 c 2 k 02 k P2 4 r02 gives the equation governing the evolution of the phase of the laser amplitude as 2 1 1 (k ) 2 2 2 (1 g2 ) . z k rs r0 2k 3.2 Effect of chirp on matched laser pulse propagation 85 (3.23) In order to study the effect of chirp on the length and intensity of the laser pulse, consider a matched ( rs r0 , n nc ) laser pulse propagating in a plasma channel. For a matched laser beam, Eqs.(3.15), (3.17) and (3.23) yield bk bk 0 , 0 k 2 (1 g2 ) z . Hence the Fourier transform of the trial function as given by and 2k Eq. (3.11) reduces to r 2 k 2 ˆak bk 0 exp 2 i (1 g2 ) z . 2k r0 (3.24) The second term in the exponent (proportional to k 2 ) on the right side of Eq. (3.24) arises due to group velocity dispersion (GVD) effects. Taking the inverse Fourier transform of Eq. (3.24) gives the laser field amplitude as a f 0 L0 1 2 1 4 2 i r2 exp tan 1 2 r0 2 L20 1 i i 1 g2 z 2 k exp ikdk . exp 4 1 2 2 k 0 (3.25) While deriving Eq. (3.25) it is assumed that k ~ 1 L << k 0 , so that k 2 k k 2 k 0 . The integral on the right side of Eq. (3.25) may be solved as before (Eq. 3.8) to give 86 12 1 2 z 1 i Z D 0 i r2 2 1 4 1 a f0 1 exp tan 2 12 r0 2 1 2 z 2 2z 1 Z D0 Z D2 0 2 1 2 z 1 i 2 Z D 0 L0 exp 1 2 z 2 2z 1 Z D2 0 Z D0 where Z D0 k 0 L20 2 1 g2 k 03 L20 r02 8 1 k P2 r02 4 1 2 z r exp i 2 Assuming 1 i Z D 0 (3.26) 12 where is the dispersion length.. 2 1 2 z 1 2 z , 2 tan 1 , Eq.(3.26) reduces to, Z D0 Z D 0 z2 2 z a f 0 1 (1 2 ) 2 Z D0 Z D0 1 4 z 2 1 i ( 1 ) 2 Z D0 r i z 2 . (3.27) exp 2 tan 1 (1 2 ) 2 2 r 2 Z D 0 L0 z 2 z 2 0 1 (1 ) 2 Z Z D 0 D 0 Comparing Eq. (3.5) and (3.27) shows that the effective pulse length is modified to 12 z2 2z . Le 0 L0 1 (1 2 ) 2 Z Z D 0 D 0 87 2 2 2 1 z 2 r 1 2 Z D0 (3.28) The second term on the right hand side of Eq. (3.28) tends to broaden the pulse length while the third term leads to compression (broadening) for a positively (negatively) chirped laser pulse. Variation of the effective normalized pulse length Le 0 L0 with propagation distance z Z D 0 is presented in Fig. 3.1. Curves a and c show the variation in pulse length for positively 0.3 and negatively 0.3 chirped pulses respectively, while curve b has been plotted for an unchirped pulse. For a positively chirped laser pulse, the pulse length initially compresses with propagation distance. Maximum compression occurs at a critical distance z Z D 0 1 2 where the effective pulse length becomes L0 1 2 1 2 . When z Z D 0 exceeds the critical distance, 12 the pulse length starts to broaden. The effective pulse length becomes equal to the initial pulse length after the laser beam has traversed a distance equal to twice the critical distance. Beyond this distance, broadening of the laser pulse length occurs. Unchirped as well as negatively chirped pulses are seen to broaden with propagation distance. Apart from changes in pulse length, comparison of Eq. (3.5) with Eq. (3.27) shows that the effective chirp parameter becomes 88 1.8 b 1.6 c 1.4 a Le 0 1.2 L0 1 0.8 0.6 0 0.2 0.4 z 0.6 0.8 1 Z D0 Fig.3.1 Variation of effective pulse length Le 0 L0 with propagation distance z Z D 0 for a positively chirped pulse ((curve a), 0.3 ), unchirped pulse (curve b) and negatively chirped pulse ((curve c), 0.3 ). (1 2 ) z Z D0 . 2 (1 ) z 2 2 z 1 Z D0 Z D2 0 e0 (3.29) 89 Eq. (3.29) shows that if the laser pulse is positively chirped, the effective chirp becomes zero at the critical distance z Z D 0 (1 2 ) . This implies that the initially (positively) chirped pulse becomes unchirped. When z Z D 0 exceeds the critical distance, the positively chirped laser pulse becomes negatively chirped (chirp reversal). This reversal occurs because the group velocity induced (negative) chirp and its coupling with initial chirp becomes more effective in comparison to the initial (positive) chirp. If z Z D 0 is less than the critical distance, reversal of chirp does not occur. Also, negatively chirped pulses do not undergo chirp reversal. 2 The matched pulse intensity ( a ) can be obtained with the help of Eq. (3.27) and is given by a f 02 2 2r 2 2 2 L0 exp 2 2 . Le 0 Le 0 r0 (3.30) Eq. (3.30) shows that the on-axis intensity of the laser pulse increases as the effective pulse length ( Le0 ) decreases. For a positively chirped pulse, maximum intensity will be obtained at the critical distance where compression of the pulse length is maximum. Fig. 3.2 shows the variation of normalized on axis r 0 intensity a 2 f 02 across the laser pulse. The dotted curve represents the initial z Z D 0 0 intensity spread for chirped as well as unchirped laser pulses. Curve a has been plotted for a positively chirped 0.3 laser pulse after it has traversed a distance z Z D0 0.275 (critical distance). It is seen that 90 after traversing the critical distance the peak intensity (at the pulse centroid) of the positively chirped laser pulse increases by about 4% in comparison to the initial peak intensity. Curves b and c respectively show the intensity variation of an unchirped 0 and negatively 0.3 chirped laser pulse after traversing the same distance. The maximum intensity of a negatively chirped laser pulse is damped by about 10.5% as compared to its initial value. The intensity of the unchirped pulse also shows a slight decrease due to GVD effects. 3.3 Variation of laser frequency across chirped laser pulses In order to study the variation of frequency across the laser pulse, the resultant phase of the laser pulse is obtained by comparing Eqs. (3.5) and (3.27) as, 2 2 1 2 1 (1 ) z 2 tan 2 e0 . 2 Z L L0 D0 0 91 (3.31) 1.2 a b c 0.8 a 2 f 02 0.4 0 -1.5 -1 -0.5 Fig 3.2 Variation of normalized L0 0 intensity a 0.5 2 f 02 1 1.5 with L 0 for the initial laser pulse z Z D 0 0, dotted curve and after the laser pulse has traversed a distance z Z D0 0.275 (critical distance) for chirp parameter 0.3 (curve a), 0 (curve b) and 0.3 (curve c). The z v g t dependence of the phase ( ) implies that the instantaneous frequency varies across the pulse from the central value 0 . The frequency shift ( ) is given by the time derivative of the phase t as 92 2 e0 v g L20 2 4c 2 where v g c1 P2 2 2 0 0 r0 (3.32) 12 is the group velocity of the pulse. It may be noted that the frequency at the pulse centroid ( 0 ) remains unaffected by propagation of the pulse in the plasma channel, while the frequency shift across the pulse tends to zero after a positively chirped pulse has traversed a distance equal to the critical distance where the pulse becomes unchirped e 0 0 . Figs. 3.3-3.5 show the variation of the normalized frequency shift 0 with L 0 after the pulse has propagated a normalized distance z Z D 0 0.1, 0.275 and 0.45 respectively for 0.3 (line a) 0 , (line b) -0.3 (line c). The laser and plasma parameters are r0 25m, L0 10m, 1m and p 40m . Fig. 3.3 shows that the frequency increases (decreases) linearly from the front to the back of a positively (negatively) chirped laser pulse. It may be noted that an 93 Fig.3.3 Variation of normalized frequency 0 with L 0 at z Z D 0 0.1 for chirp parameters 0.3 line a , 0 line b and -0.3 (line c ), for r0 25m , L0 10m , 1m and p 40m. 94 Fig. 3.4 Variation of normalized frequency 0 with L 0 at z Z D 0 0.275 for chirp parameters 0.3 line a , 0 line b and -0.3 (line c) for r0 25m , L0 10m , 1m and p 40m. 95 Fig. 3.5Variation of normalized frequency 0 with L 0 at z Z D 0 0.45 for chirp parameters 0.3 line a, 0 line b and -0.3 (line c) , for r0 25m , L0 10m , 1m and p 40m. unchirped laser pulse attains a slight negative chirp due to GVD effect. This induced negative chirping will superimpose upon initial chirping and will result in decrease (increase) in effective chirp of a positively (negatively) chirped pulse. After 96 propagating a distance z Z D0 0.275 , the frequency variation of the laser pulse is shown in Fig. 3.4. The negative chirping of the unchirped and negatively chirped laser pulse increases in comparison to Fig. 3.3 due to increase in propagation distance. However, the frequency variation of the positively chirped pulse reduces to zero, since at this critical distance a positively chirped pulse becomes unchirped. Fig.3.5 shows that with increase in propagation distance beyond the critical value, the positively chirped pulse becomes negatively chirped (chirp reversal). This reversal occurs because the group velocity induced chirp and its coupling with the initial chirp becomes more effective in comparison to the initial (positive) chirp. However for unchirped and negatively chirped pulses, the effective chirp becomes more negative in comparison to Figs. 3.3 and 3.4. The study shows that the length as well as the chirp of an ultrashort laser pulse changes due to propagation in a plasma channel. A positively chirped pulse may be compressed after propagating a certain critical distance, thus leading to a shorter pulse length laser source. It is important to note that there is a possibility of unchirping a positively chirped laser pulse by allowing it to propagate a given distance in plasma. CHAPTER 4 Wakefield effects on the evolution of symmetric laser pulses in a plasma channel The present chapter deals with the study of the combined effects of wakefields (inside the laser pulse) and relativistic nonlinearity on the propagation of a short laser pulse in a parabolic plasma channel [111]. The density variation of plasma electrons 97 produced by the combined effect of transverse and axial ponderomotive nonlinearity have been obtained. The wave equation describing the evolution of the laser amplitude driven by relativistic and ponderomotive nonlinearities has been set up. Further, the reduced Lagrangian density is obtained and variational technique is used to derive the coupled equations governing the evolution of the pulse length and spot-size of the laser. Numerical methods are used to graphically analyze the evolution of the laser pulse length and intensity. 4.1 Wave dynamics Consider a linearly polarized, short laser pulse propagating in a pre-formed plasma channel of the form nr n0 nr 2 rch2 where n and rch are the channel depth and radius respectively. The vector potential of the radiation field is given by Ar , z , t A xˆ exp ik 0 z i 0 t c.c. 2 (4.1) where Ar, z, t , 0 and k 0 are the field amplitude, frequency and wavenumber respectively. The wave equation describing the evolution of the vector potential driven by relativistic and ponderomotive nonlinearities is given by 98 nr 2 a 2 n nr 2 a 2 2 1 2 2 a 2 2 a k P 1 2 2 4 n 4 c t n r n r 0 0 ch 0 ch a (r , z , t ) ( eA(r , z , t ) mc 2 ) where k P 4n0 e 2 mc 2 12 is the normalized (4.2) vector field and is the plasma wavenumber. The second, third, fourth and fifth terms on the right side of Eq. (4.2) represent the contributions due to the plasma channel, relativistic nonlinearity, ponderomotive effect and coupling of the relativistic nonlinearity with the channel (channel coupling). Substituting Eq. (4.1) into Eq. (4.2) and transforming independent variables z, t to z , ( z g ct , where g ck 0 0 is the normalized group velocity of the laser pulse) gives, 2 0 2 2 2 2 2 2 2 k k 2 ik 2 1 0 P 0 g 2 2 2 c z z z 2 n nr 2 a k 4 n0 n0 rch2 2 P a2 1 ar , z, 0 . 4 (4.3) Neglecting the higher order diffraction effect 2 z 2 in comparison to the terms 2 2 z 2k 0 z , and 1 L2 r02 1 k P2 r02 4 k P2 r02 f 02 16 2 g 2 2 in the limit k 0 r0 >1, L 2Z R and respectively, the Lagrangian density of the wave equation (4.3) is given by 99 a a a a a a * l a. a * ik 0 a a * z z z z 1 g2 a a * 02 2 k02 k P2 aa * c a 2 a 2 n nr 2 2 2 nr 2 k P2 aa a a aa . n0 8n0 rch2 n0 rch2 8 (4.4) Considering a sinusoidal laser pulse the trial function for its amplitude may be represented by r 2 a f exp i 1 i 2 sin rs L (4.5) where f ( z ), ( z ), ( z ), rs ( z ) and Lz are the amplitude, phase shift, curvature, spotsize and length of the laser pulse respectively. 4.2 Density perturbation In order to determine the density perturbation (wakefield) inside the laser pulse, its evolution equation (Sec.1.2b) is written as 2 2 c 2 k P2 1 nr 2 n0 rch2 t n c 2 2 2 ( a ). 4 n0 100 (4.6) Transforming independent variables z, t to z, z g ct in Eq. (4.6) gives 2 k P2 1 nr 2 n0 rch2 2 2 g nn 0 1 4 g2 2 ( a ) 2 2 2 ( a ). (4.7) 2 2 4 g 1 While deriving Eq. (4.7) the quasi-static approximation (Sec.1.2b) has been used. In this approximation the laser does not evolve significantly as it transits a plasma electron. Thus plasma electrons experience a laser field which is a function of and r variables only (independent of z ). The solution of Eq. (4.7) is obtained by first writing the corresponding homogeneous equation as 2 k P2 1 nr 2 n0 rch2 2 2 g nn 0 . (4.8) 0 Eq. (4.8) has a solution of the form n n0 C1 cos k P C 2 sin k P (4.8a) where C1 and C2 are constants. For obtaining the particular solution, C1 and C2 are replaced by u and v respectively. Thus 101 n n0 u cos k P v sin k P . (4.8b) Differentiating Eq. (4.8b) with respect to gives n n0 u v cos k P sin k P k P v cos k P u sin k P . (4.9) In order to obtain the value of u and v , it is assumed that cos k P u v sin k P 0. (4.10) Therefore, Eq. (4.9) reduces to n n0 k P v cos k P u sin k P . Second differentiation of Eq. (4.11) with respect to gives 2 n n0 v u k P cos k P sin k P 2 102 (4.11) k P2 u cos k P v sin k P . (4.12) Substituting Eqs. (4.8b) and (4.12) into Eq. (4.7), and assuming a wide channel k P rch 1 and g2 1 , gives v u 1 2 2 1 2 2 k P cos k P sin k P a . a 2 4 4 (4.13) Multiplying Eq. (4.10) by sin kP and Eq. (4.13) by cos kP and adding gives v 1 4k P 2 2 2 2 a a cos k P . 2 (4.14) Similarly multiplying Eq. (4.10) by cos k P and Eq. (4.13) by sin kP and subtracting gives u 1 2 2 2 2 a 2 a sin k P . 4k P (4.15) Integrating Eqs (4.14) and (4.15) yields v 1 2 2 a 4k P L 2 2 2 L 2 a cos k P d and 103 (4.16) u 2 1 2 2 2 a a sin k P d 2 2 L 4k P L (4.17) respectively. Substituting the values of u and v into Eq. (4.8b) gives the density perturbation as, n n0 1 4k P L 2 a sin k P d 2 2 2 L 2 a sin k P d . 1 4k P (4.18) Substituting the trial function (Eq. (4.5)) into Eq. (4.18) gives f 2 z 2 2 2 n0 k P r0 rˆs n 2 ˆ2 2r 2 1 ˆ L cos 2 1 2 2 1 cos 2 L 2 ˆ2 1 2 Lˆ2 L0 Lˆ r0 rˆs p 1 L z 2r 2 2 ˆ 2 2 cos 2 L cos exp r rˆ ˆ 8 1 2 Lˆ2 L L P 0 s 0 f 2 (4.19) where Lˆ L L0 and rˆs rs r0 are the normalized laser pulse length and spot-size ( L0 , r0 represent the initial values of the pulse length and spot-size respectively), P is the plasma wavelength and L0 P . The first and second terms on the right side of Eq. (4.19) respectively arise due to transverse and longitudinal ponderomotive effects. Since 104 L̂ varies with propagation distance, Eq. (4.19) becomes invalid if Lˆ 1 . Hence in this limit the l’Hospital’s rule is applied to give the maximum density perturbation as f 2 z n0 k P r02 rˆs2 n 2r 2 1 2 2 r rˆ 0 s 1 cos k P P sin k P k 2 kP P 2 f 2 z 4k P L0 L 2r 2 . 2 2 r0 rˆs P sin k P exp 2 ˆ2 (4.20) 4.3 Evolution of laser spot-size and pulse length Inserting Eqs. (4.5) and (4.19) into the Lagrangian density (Eq. (4.4)) and using L lˆ r ld dr yields the reduced Lagrangian density as 0 0 f lˆ 2 z L0 Lˆ 4 1 f 4 2 g rˆs 2 rˆs2 Lˆ ˆ ˆ 2 r 2 r s s zˆ zˆ zˆ k 0 L0 Lˆ2 zˆ 2 2 02 k P2 r04 rˆs4 n 2 2 r0 rˆs k0 k P 4n0 rch2 2 L20 Lˆ2 c 2 2 2 r02 rˆs2 z L0 Lˆ 32 2 1 rˆs 3k P2 r02 rˆs2 3k P2 r04 rˆs 4 n 1 2 2 1 2 64n0 rch 16 Lˆ 1 k P2 r02 rˆs2 Lˆ sin 2Lˆ r02 rˆs2 k P sin 2Lˆ 8 2 2 Lˆ2 1 4 L0 Lˆ 2 Lˆ2 1 . sin 2Lˆ 2 Lˆ2 2Lˆ 2 (4.21) L ˆ l r ld Similarly, substituting Eq. (4.5) and (4.20) into Eq.(4.4) and using 0 0 dr gives the reduced Lagrangian density in the limit L P as, 105 f 2 z L0 Lˆ 2 lˆ 1 rˆs 4 1 3f 4 2 g 2 r02 rˆs2 2 L20 Lˆ2 z L0 Lˆ 256 5 rˆs 2 rˆs2 Lˆ ˆ ˆ 2 r 2 r s s zˆ zˆ zˆ k 0 L0 Lˆ2 zˆ 2 2 02 ˆs k P2 r04 rˆs4 n 2 2 r0 r 2 k0 k P 4n0 rch2 c 2 k p2 r02 rˆs2 2 k p2 r04 rˆs4 n 8n0 rch2 2 r02 rˆs2 . L20 Lˆ2 (4.22) The evolution of various laser parameters may be described with the help of the Euler-Lagrange ˆ j lˆ j 0 l z z equation, where j j 1, 2,.......4 , L , and rs . Using the reduced Lagrangian density given by Eq.(4.21) and substituting 1 and 2 L gives, 2 2ˆ f rˆs L 0 zˆ (4.23) and 1 2 g 4 L30 Lˆ3 2 f 02 3 2 f 02 2 3 2 nf 02 r02 2 128L30 rˆs2 Lˆ2 512n0 rch2 L30 Lˆ2 32r02 L0 rˆs4 Lˆ2 106 f 02 L20 16r02rˆs4 f 02 2 64r02 L0 rˆs4 f 02 2 2 3 2 Lˆ2 1 2 64 L3 2 Lˆ2 1 rˆ 2 Lˆ2 s 3 2 Lˆ2 1 sin 2Lˆ ˆ cos 2L 0 2 2 Lˆ2 1 Lˆ 32 2 Lˆ2 1 L30 Lˆ2 rˆs2 f 02 cos 2Lˆ Lˆ sin 2Lˆ f 02 2 2 Lˆ2 1 2 2 2 2 2 4 2 ˆ2 2 ˆ 2 Lˆ2 1 ˆ L 1 16 r L r L 1 0 0 s 0 2 2 Lˆ2 1 sin 2Lˆ cos 2Lˆ 2 3 3 3 ˆ2 2 ˆ2 2 2 ˆ2 ˆ 2L0 L L 1 2 L 1 L0 L (4.24) respectively. Differentiating Eq. (4.24) with respect to propagation distance z gives the equation describing the evolution of the laser pulse length as, 3 2 1 g2 3 2 f 02 2 3 2 nf 02 r02 2 f 02 4 L40 Lˆ4 64 L40 Lˆ3 rˆs2 256n0 rch2 L40 Lˆ3 16r02 L20 rˆs4 Lˆ3 f 02 2 2 Lˆ2 1 cos 2Lˆ ˆ sin 2L 16r02 L20 2 Lˆ2 1 rˆs4 Lˆ2 Lˆ 2 Lˆ2 1 f 02 2 2 Lˆ2 1 cos 2Lˆ 2 16 2 Lˆ2 1 r 2 L2 rˆ 4 Lˆ3 0 0 s f 02 4 Lˆ 2 32r 2 L2 2 Lˆ2 1 rˆ 4 0 0 f 02 sin 2Lˆ 2 16r02 L20 2 Lˆ2 1 rˆs4 Lˆ4 s 2 6 2 Lˆ2 1 2 2 2 Lˆ2 1 2 ˆ2 2 L 1 2 2 Lˆ2 1 1 2 ˆ2 L 1 107 sin 2Lˆ Lˆ cos 2Lˆ f 02 3 2 2 2 2 ˆ2 4 2 2 Lˆ2 1 ˆ 8r0 L0 L 1 rs sin 2Lˆ Lˆ cos 2Lˆ 3 2 Lˆ2 sin 2Lˆ f 02 3 3 8 8 2 Lˆ2 1 r02 L20 rˆs4 2 Lˆ2 1 16 f 02 2 2 2 32 L20 2 Lˆ2 1 rˆs2 2 2 3 sin 2Lˆ 3 Lˆ 1 cos 2Lˆ Lˆ 3 2 Lˆ2 1 cos 2Lˆ ˆ sin 2 L Lˆ 2 Lˆ2 1 1 rˆ Lˆ f 02 1 f 02 cos 2Lˆ 3 3 5 2 2 2 8L0 r0 rˆs Lˆ 8r0 L0 Lˆ 1 f 02 2 3 16 L40 2 Lˆ2 1 Lˆ2 rˆs2 2 3 2 Lˆ2 1 3 2 2 ˆ 2 ˆ3 2 ˆ2 L0 L L0 L L 1 f 02 2 3 2 16 L40 2 Lˆ2 1 rˆs2 Lˆ2 2 3 f 02 2 2 Lˆ2 1 sin 2Lˆ 2 2 8r03 L0 2 Lˆ2 1 5 s 2 Lˆ2 1 2 2 2 2 Lˆ Lˆ 1 2 1 rˆ 5 Lˆ3 s f 02 2 2 Lˆ2 1 f 02 2 cos 2Lˆ 3 f 02 2 2 f 02 3 Lˆ sin 2Lˆ 2 3 2 3 3 2 8r03 L0 2 Lˆ2 1 rˆs5 64r0 L0 rˆs Lˆ 4L0 r03 rˆs5 2 Lˆ2 1 16L0 r03 rˆs5 2 Lˆ2 1 f 02 2 2 3 2 Lˆ2 1 f 02 2 2 cos 2Lˆ f 02 3 2 Lˆ2 1 sin 2Lˆ 2 2 3 32r0 L30 rˆs3 Lˆ2 2 Lˆ2 1 16r0 L30 2 Lˆ2 1 rˆs3 Lˆ2 16r0 L30 2 Lˆ2 1 rˆs3 Lˆ3 r0 rˆs L0 zˆ where Lˆ zˆ (4.25) ẑ propagation z Z R , Z R k 0 r02 2 is the Rayleigh length distance. Eq. (4.23) representing 108 the is the normalized conservation of energy f 2 rs2 L f 02 r02 L0 constant w here f 0 is the initial laser field amplitude , has been used while deriving the evolution equation for the pulse length. The first, second and third terms on the left side of Eq. (4.25) arise due to group velocity dispersion (GVD), relativistic nonlinearity and its coupling with the plasma channel respectively. The remaining terms are due to the presence of wakefields. When the laser pulse length approaches the plasma wavelength, Eq. (4.22) is used to obtain the evolution of the laser pulse length with the help of the Euler-Lagrange equation as 3 2 1 g2 3 2 2 f 02 r02 n 3 2 f 02 2 15 f 02 9 2 f 02 Lˆ 4 4 256n0 rch2 L40 Lˆ3 64 L40 rˆs2 Lˆ3 128r02 L20 rˆs4 Lˆ3 64 L40 rˆs2 Lˆ5 zˆ 4 L 0 Lˆ 3 2 f 02 2 15 f 02 9 2 f 02 r0 rˆs . 3 3 2 64r03 L0 rˆs5 Lˆ2 128r0 L30 rˆs3 Lˆ4 L0 zˆ 64r0 L0 rˆs Lˆ (4.26) Substituting 3 and the reduced Lagrangian density (Eq.4.21) into the EulerLagrange equation gives rˆs rˆs . zˆ (4.27) The evolution of the laser spot-size is described by substituting 4 rs into the EulerLagrange equation as 109 2 4 2 2 2 2 rˆs 1 k p r0 rˆs n 3k p f 0 r0 zˆ 2 rˆs3 4n0 rch2 128Lˆ rˆs3 sin 2Lˆ 2 Lˆ sin 2Lˆ 1 ˆ 2 ˆ2 ˆ2 2 2 Lˆ2 1 2 2 Lˆ2 1 2 L 2 L 1 L 2 2 2 ˆ kP f 0 r0 sin 2L 2 . 2 ˆ2 3 ˆ 2 Lˆ2 1 4 16 L 1 Lˆ rˆs L L 0 f 02 5 4rˆs (4.28) In deriving the Eq. (4.28), Eqs. (4.23), (4.27) and (4.21) have been used. The first term on the right side of Eq. (4.28) shows vacuum diffraction, the second term represents channel focusing, the third term leads to relativistic self-focusing and is a function of pulse length. The fourth and fifth terms arise due to the transverse and axial ponderomotive effects, respectively. When the laser pulse length approaches the plasma wavelength, singularity arises in Eq. (4.21). In this limit Eq. (4.22) is used along with the Euler-Lagrange equation to obtain the evolution of the laser spot-size as, 2 rˆs 1 k P2 r04 rˆs n 3k P2 f 02 r02 15 f 02 3 2 f 02 r02 . zˆ 2 rˆs3 4n0 rch2 128Lˆ rˆs3 32rˆs5 Lˆ 64 L20 rˆs3 Lˆ3 (4.29) In order to obtain the usual matching condition (Sec. 1.3) of the laser spot as it propagates in the plasma channel with the effect of wakefields neglected and the pulse length kept constant L L0 , the right hand side of Eq. (4.28) or Eq. (4.29) is considered to be zero. Thus the laser beam will propagate with a constant spot-size (matched beam) if the channel density gradient is equal to a certain critical value given by 110 nc 4rch2 n0 k P2 r04 3 f 02 r02 k P2 1 . 128 (4.30) The intensity of the laser pulse is dependent upon both the spot-size and pulse length of the laser. Simultaneous evolution of the spot-size and pulse length enhances the laser intensity with propagation distance if the laser compresses and focuses. Thus, the intensity of the laser pulse, after it has propagated a given distance, is represented by f 2 f 02 . rˆs2 Lˆ (4.31) 4.4 Graphical description Maximum wakefields are obtained when the laser pulse length tends to the plasma wavelength 1 . Therefore, numerical studies for three cases 1 , 1 and 1 have been presented. Figs. 4.1, 4.2 and 4.3 respectively depict the evolution of the laser pulse length, spot-size (considering matching condition) and intensity. Curves a, b and c are plotted for 1, 1 and 1 respectively. Curves a and b are plotted with the help of Eqs. (4.25) and (4.28) while curve c 1 has been plotted by simultaneously solving Eqs. (4.26) and (4.29). The channel depth nc is considered to be equal to a certain critical value (Eq. (4.30)) for which a laser beam (assuming a constant pulse length and neglecting wakefields) propagates with a constant spot-size. The laser and plasma parameters for all these figures are L0 16m (curve a), 111 9 m (curve b) and 11m (curve c), r0 25m, f 02 0.015 P 11m , rch 40m and n nc 4.3 1017 cm -3 . Fig 4.1 shows that due to the presence of wakefields, the laser pulse length tends to compress when 1 (curve a) while the pulse length broadens when 1 (curve b). It is interesting to note that the results obtained for both cases are contrary to each other. For the case 1 (maximum wakefield), compression of pulse length is slow. Fig 4.2 shows the evolution of the laser spot-size with propagation distance. It is seen that for all three cases the laser spot becomes mismatched (even though n nc ) and tends to focus due to the presence of wakefields. For 1 (curve a) focusing is greater than the other two cases. Consequently, in Fig.4.3 the peak intensity of the laser pulse (Eq. 4.31) increases with propagation distance for all the three cases (curves a, b and c). Since both compression and focusing of the laser pulse occurs when 1 , the enhancement in intensity is more rapid (curve a) in comparison to the cases when 1 and 1. When 1, the increase in laser intensity is small due to broadening of the laser pulse. These results will be extremely useful for optimization of laser and plasma parameters for applications such as laser-plasma based accelerators and intense radiation generation. 112 1.005 b 1 0.995 L L0 0.99 c 0.985 a 0.98 0.975 0 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 z ZR Fig.4.1 Variation of normalized pulse length with propagation distance when 1 curve a , 1 curve b and 1 curve c for L0 16m , 9m and 11m r0 25m, 1m , f 02 0.015 P 11m , rch 40m and n nc 4.3 1017 cm 3 . 113 1.005 1 0.995 0.99 rs r0 b 0.985 c 0.98 0.975 a 0.97 0 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 z ZR Fig.4.2 Variation of normalized spot-size with propagation distance when 1 curve a, 1 curve b and 1 curve c for L0 16m , 9 m and 11m , r0 25m, f 02 0.015 , 1m P 11m , rch 40m and n nc 4.3 1017 cm 3 . 114 0.0164 a 0.0162 c 0.016 0.0158 f 2 z 0.0156 0.0154 b 0.0152 0.015 0.0148 0 0.2 0.4 0.6 z Z R 0.8 1 1.2 1.4 1.6 Fig.4.3 Variation of laser pulse intensity with propagation distance when 1 curve a, 1 curve b and 1 curve c for L0 16m , 9 m and 11m , r0 25m, f 02 0.015 , 1m , P 11m , rch 40m and n nc 4.3 1017 cm 3 . CHAPTER 5 Conclusions 5.1 Conclusions 115 The present thesis is a significant contribution towards understanding the evolution dynamics of short laser pulses in a pre-formed plasma channel. The study shows that the evolution characteristics of laser pulses are affected by group velocity dispersion as well as relativistic and ponderomotive nonlinearities. The possible important applications arising from this study are in the fields of laser wakefield acceleration and ultrashort laser pulse generation. Considering the mildly relativistic regime, the wave equation describing the evolution of the laser field amplitude in a plasma channel has been set up, taking into account relativistic nonlinearity and group velocity dispersion effects. The Lagrangian density for the wave equation is obtained and the variational technique is used to derive equations describing the evolution of various laser parameters. Numerical techniques are used to study the spot-size (pulse length) evolution, considering the pulse length (spotsize) to be constant. Further, simultaneous evolution of the laser spot-size and pulse length has been studied. A higher rate of compression of the pulse length occurs when the spot-size and pulse length evolve simultaneously as compared to the constant spot-size case. Also, the focusing effect increases when the spot-size evolves simultaneously with the pulse length in comparison to the case when the pulse length is considered to be constant. Thus the enhancement in intensity of the laser pulse is more when the spot-size and pulse length evolve simultaneously as compared to the case when either the spot-size or the pulse length is considered to be constant. In order to study the effect of the presence of the plasma channel, the simultaneous evolution of the laser spot-size and pulse length in the channel is compared with the evolution in homogeneous plasma. It is 116 seen that the presence of the plasma channel enhances the compression of the pulse length. This is due to the combined effect of relativistic nonlinearity and its coupling with the plasma channel. An important advantage of using a plasma channel for applications based on laser-plasma interaction is that the channel allows the propagation of the laser beam with constant spot-size (matched beam). This can be achieved by choosing a certain critical value of the channel density gradient nc . The evaluation of the critical channel depth is independent of the laser pulse length. The present study shows that when a laser spot satisfying the beam matching condition propagates in a plasma channel it does not remain matched when the pulse length evolution is taken into account. Since the laser pulse length undergoes compression the laser spot-size reduces (focuses), instead of remaining constant. It is also shown that if the initial laser intensity is increased, compression as well as focusing of the laser spot increases. It is shown that, an initially unchirped laser pulse becomes chirped as it propagates in a plasma channel, due to group velocity dispersion (GVD) as well as selfphase modulation (SPM). For a matched rs r0 , n nc laser pulse the frequency at the front (back) of the pulse decreases (increases) due to SPM effect whereas it increases (decreases) due to GVD effect. However, when both effects are taken into account SPM dominates over GVD leading to an increase in frequency from front to back of the pulse (positive chirping). Since SPM depends upon the intensity of the laser pulse, a reduction in intensity causes the GVD and SPM induced chirp to approximately cancel each other so that the initially unchirped laser pulse remains nearly unchirped. 117 The propagation of an ultrashort chirped laser pulse in a parabolic plasma channel has been analyzed. For such pulses, relativistic and ponderomotive nonlinearities nearly cancel each other. The effect of initial chirp on the laser pulse length and intensity of a matched laser beam propagating in a plasma channel is studied. The pulse length and chirp parameter of the laser pulse are modified due to its interaction with plasma. The effective values of these parameters have been obtained. It is shown that the pulse length of a positively chirped laser pulse length, compresses with propagation distance. Maximum compression occurs at a certain critical distance which depends on the chirp parameter. When the propagation distance exceeds the critical value, the pulse length starts to broaden. The effective pulse length becomes equal to the initial pulse length after the laser beam traverses a distance equal to twice the critical distance. However, the pulse length of a negatively chirped pulse broadens continuously. Consequently, it is seen that at the critical distance, the peak intensity (at the pulse centroid) of a positively (negatively) chirped laser pulse maximizes (decreases) in comparison to its initial peak intensity. It is seen that the chirp parameter of an initially chirped laser pulse changes due to propagation in plasma. Also, after the pulse has traversed a certain critical distance, the positively chirped laser pulse becomes unchirped. Beyond this critical distance, chirp reversal occurs and the laser pulse becomes negatively chirped. This reversal occurs because the group velocity induced (negative) chirp and its coupling with the initial chirp becomes more effective in comparison to the initial (positive) chirp. If the distance traversed by the laser pulse is less than the critical distance, reversal of chirp does not occur. Also chirp reversal does not occur for negatively chirped pulses. 118 The effect of wakefields, generated inside the pulse, on the propagation characteristics of the laser beam has been studied. The density variation of plasma electrons produced by the combined effect of transverse and axial ponderomotive nonlinearity is obtained. Since the density perturbation exhibits a singularity when the laser pulse length approaches the plasma wavelength (maximum wakefield condition), source term driving the laser amplitude for this case is obtained using l’Hospital rule. Using the variational technique, coupled equations describing the evolution of the laser pulse length and spot-size are obtained for the case when (i) the plasma wavelength P is not equal to the pulse length L and when (ii) L P . It is seen that for a matched laser beam the pulse length tends to compress (broaden) when it is initially greater (less) than the plasma wavelength. When the plasma wavelength is equal to the laser pulse length the rate of compression of the pulse length is slow. It is important to note that in the regime where maximum wakefields are obtained the propagation characteristics of the laser pulse are extremely sensitive to the ratio of the pulse length to the plasma wavelength and show contrary behaviour when the laser pulse length is slightly increased or decreased. These results will be extremely useful for optimization of laser and plasma parameters for various applications, for example, in laser wakefield accelerators, generation of maximum wakefield amplitude is essential but at the same time, matched beam propagation is equally important. Therefore the regime 1 may be more appropriate as compared to 1. On the other hand for generating high intensity laser beams (via compression), the regime 1 will be suitable. 5.2 Recommendations for future work 119 The thesis presents a comprehensive study of the simultaneous evolution of the spot-size and pulse length of a laser, as it propagates in a pre-formed plasma channel. With appropriate choice of laser and plasma parameters it has been shown that focusing of the laser spot-size and compression of its pulse length can be achieved. The possibility of further pulse compression could be explored by tapering the plasma density along the direction of propagation of the laser pulse. Therefore, the study of simultaneous evolution of the laser spot-size and pulse length in a tapered plasma channel can be an interesting proposal for future work. In the presence of a plasma channel, the study of propagation characteristics of initially chirped ultrashort laser pulses in the linear regime is presented. 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