22nd International Symposium on Plasma Chemistry July 5-10, 2015; Antwerp, Belgium Numerical study on the gliding behaviour of a DC argon arc root along the electrode surface under gas blast and externally applied magnetic field W. Wang1,2 and A. Bogaerts1 1 2 Research Group PLASMANT, Department of Chemistry, University of Antwerp, 2610 Antwerpen-Wilrijk, Belgium Qian Xuesen Laboratory of Space Technology, China Academy of Space Technology, No.104 Youyi Road, CN-100094 Beijing, P.R. China Abstract: This paper focuses on the numerical investigation of the gliding behaviour of a DC argon arc under gas blast and externally applied magnetic field. A three-dimensional simulation model of an argon arc generated between two diverging electrodes is built, based on magneto-hydro-dynamic (MHD) theory. Besides the coupled electromagnetic and gas dynamic interactions, the arc motion is described in detail by the temperature distribution, and its gliding mechanism along the electrode surface, under the gas blast and externally applied magnetic field, is discussed. Keywords: numerical investigation, arc simulation, arc root, low voltage, applied magnetic field 1. Introduction A GlidArc is an auto-oscillating periodic discharge between at least two diverging electrodes with gas blast. A plasma column connecting the electrodes is formed by self-initiation in the upstream narrowest gap. Subsequently, this column is dragged by the gas flow toward the diverging downstream section. Besides the gas blast, an externally applied magnetic field can also provide a driving force of arc root gliding phenomena along the electrode surface [1]. The GlidArc, which can produce a large density of highly reactive species, has great potential in many industrial applications, such as the conversion of greenhouse gases (mainly CO 2 , CH 4 ) to value-added chemicals or renewable fuels [2, 3]. However, due to the complexity of the GlidArc, i.e., unsteady behaviour in time and space, detailed investigations on gliding arc behaviour are rare in the literature. As the GlidArc is a kind of transitional plasma from thermal to non-thermal state and can be assumed as equilibrium plasma at the shortest electrode separation [4], it is meaningful to first investigate the arc gliding behaviour along the electrode surface under equilibrium conditions where the discharge current is usually above 1 A. Besides the GlidArc applications, the arc root gliding phenomenon is also quite common in thermal plasma applications such as switching devices [5]. Therefore, we here preform a numerical modelling of the gliding behaviour of an argon arc root along the electrode surface based on the assumption of local thermodynamic equilibrium and we intend to provide an insight in the gliding mechanism along the electrode surface under the gas blast and externally applied magnetic field, respectively. P-II-12-18 2. Model geometry and numerical model 2.1. Model geometry The model geometry of the argon arc reactor between two diverging electrodes is shown in Fig. 1. Only half of the geometry is presented, considering the symmetry. The cathode and anode with a thickness of 5 mm in the x direction which are found at the left and right side of the geometry (see figure caption). The current is fed into the plasma from the anode and flows out from the cathode. Fig. 1. Structure of the arc reactor (units: mm), the symmetry plane: A 1 B 1 C 1 D 1 E 1 F 1 G 1 H 1 , the anode surface: the cathode surface: B1C1D1E1E2D2C2B2, A 1 H 1 G 1 F 1 F 2 G 2 H 2 A 2 , gas inlet: A 1 A 2 B 2 B 1 , gas exit, E1E2F2F1. 2.2. Hypotheses To reduce the complexity of the simulation, a few assumptions and simplifications are adopted as follows: (a) The plasma is assumed as a laminar flow in a state of local thermodynamic equilibrium (LTE). (b) The arc 1 restrike process is not included in the simulation. (c) The electrode erosion is not considered in the model. (d) The Eddy current in the arc and metal part is not included in this model. 2.3. Equations The mathematical description of the arc plasma includes nine coupled transport equations. The laws of the compressible gas are described by Navier–Stokes equations considering different sources of energy generation and loss. The magnetic flux density is determined through calculating the magnetic vector potential. All the equations included in the arc model can be written in a general formulation as follows: ∂ ( rΦ ) ) div(Γ Φ grad Φ ) + SΦ (1) + div( rΦV= ∂t where Φ is the field variable. For each equation, Γ Φ is the corresponding property coefficient of the arc plasma and S Φ is the source term. The variables and parameters for the nine second-order partial differential equations are given in Table 1. Table 1. Equation variables and parameters. Equations Mass conservation equation Momentum conservation equation Φ ΓΦ SΦ 1 0 0 u h Su v h Sv w h Sw Energy conservation equation h λ/c p Sh Electrical field equation φ σ 0 Ax 1 S Ax Magnetic field equation Ay 1 S Ay Az 1 S Az For the source terms in the above equations ∂p − + ρ g i + ( J × B )i Si = ∂xi (2) where I = u, v, w, Sh=σ E 2-qrad + qh (3) where q rad is the radiative loss, which is calculated by Lindmayer’s empirical model [7] considering the complexity of the arc radiation mechanism, q h is the heat lost due to viscous dissipation, and S Ai = − µ0 ji The electrical field is obtained using E = − gradφ 2 (4) (5) The current density is defined by J =σE (6) According to Maxwell’s equation, we can obtain the magnetic flux density from B = ∇× A (7) In the above equations, r is the density, σ is the electrical conductivity, c p is the specific heat, h is the dynamic viscosity, λ is the thermal conductivity, µ 0 is the argon magnetic permeability, t is time, p is pressure, φ is the electrical potential, S i is the momentum source term (S u , S v , S w ), S h is the enthalpy source term, S Ai is the magnetic potential source term, h is the enthalpy, V is the velocity vector, u, v, w are the velocity components in the x, y, z directions, j i are the current density components (j x , j y , j z ) and A is the magnetic vector potential. The argon plasma physical properties (σ, r, λ, h, c p ) described above, which depend on the temperature and pressure, are taken from the literature [8]. 2.4. Boundary conditions According to the standard method to deal with the velocity in the computational fluid dynamics method, a non-slip boundary condition is imposed on the wall-plasma interfaces. At the interfaces between the electrodes and the plasma, the heat is transferred from the plasma to the electrodes according to the energy transfer conservation law [7]. Thus, the temperature of the elements on each side of the electrode-arc interface is coupled during the calculation. The electrode surface temperature is set below the melting temperature of the electrode material, which was set to 2500 K for copper metal in the current calculation. The magnetic vector potential, described in Table 1, is used to calculate the self-magnetic field produced by the currents in the electrodes and arc column. We set the boundary condition of the magnetic vector potential to zero at a large distance from the arc. A current density is imposed on the interface between the cathode and the arc plasma by Lindmayer’s methods [9] in which the arc root commutation is described by the “thermally driven model” based on the electrode temperatures deduced from a heat flux balance. In this model, Richardson’s equation is used to define the current density at the cathode-plasma interface, i.e., the electron current from the cathode is assumed to be produced by thermionic emission. Thus, the current density at this boundary is mainly dependent on the temperature of the interface elements and the total arc current. We take the anode–arc interface as a collector for negative particles. Thus, a Dirichlet condition is used to define the potential boundary condition, i.e., a zero electrical potential is imposed on the anode-arc interface in our simulation work. If not specially mentioned, the inlet and exit pressure is set as 1atm in the computation. In the symmetry plane, the P-II-12-18 gradients of all the physical quantities are set zero. The calculation begins with a stationary temperature distribution between the two electrodes without gas blast and externally applied magnetic field. In order to investigate the influence of gas blast on the arc gliding behavior, we give a mass flow rate of 0.005 kg/s during the transient computation. The equations mentioned above are solved by the adapted commercial code Ansys FLUENT [10], which is based on the finite volume method. 3. Results and Discussion Fig. 2 shows the steady temperature distribution on the symmetry plane of an argon arc with a current of 100 A. As we can see, the relatively low temperature of the electrode leads to an arc column constriction near the electrodes. Besides, the self-induced magnetic field generated by the arc current can also contribute to the arc column constriction by the Lorenz force. Therefore, due to the large current density and hence the joule heating effects, the arc column temperature near the electrodes is relatively high. density, is influenced more intensely by the external magnetic field and brings a more swift movement along the surface. Because the magnetic field can only be effectively applied to the high temperature gas by the Lorenz force, in which the current density passes through, the gas below 10000 K has a low electrical conductivity and does not move apparently. This leads to an arc tailing phenomenon behind the arc column with temperatures of several thousand kelvins, as clearly indicated in Fig. 3. Its length increases as the arc column moves along the electrodes. Similar results were also presented in literature [11]. Fig. 3. Transient temperature distribution of an argon arc with a current of 100 A under an external magnetic field B y0 = 10 mT. Fig. 2. Steady temperature distribution of an argon arc with a current of 100 A. We can separately investigate the influence of externally applied magnetic field and gas blast on the arc gliding behaviour along the electrode surface, which is illustrated in Figs. 3 and 4, respectively. In Fig. 3, a 10 mT magnetic field is employed in the y direction at the starting time of 0 ms. In the initial period of 0.071 ms, the arc gliding velocity is low and the arc does not move apparently. After that, the arc which is driven under the applied magnetic field glides along the electrode surface with continuously increasing velocity and a great change in the arc column’s shape is observed. Compared to the anode spot, the cathode spot, which has a larger current P-II-12-18 Similarly, after the gas blast is imposed at the inlet plane at the time of 0 ms, the arc gliding velocity is not increasing until 0.009 ms when the gas blow reaches the arc column. Compared with the conditions under the external magnetic field, the gas blast does not bring an arc tailing phenomenon and can easily drag the column toward the diverging downstream section in a quite thin shape due to the strong cooling effects. The arc plasma near both the anode and cathode moves slowly compared with the arc column which can easily be influenced by the coming gas blast, especially when the arc root moves into the diverging section of the electrodes. We can also find that although the arc root near the anode and cathode has almost the same moving velocity, there exists a slight deviation. For example, the arc gliding velocity near the anode surface is slightly larger than that near the cathode 3 surface in the initial stage of constant electrode separation. However, after the arc root comes into the diverging section of the electrodes, the arc root near the cathode surface glides faster. We believe this is mainly caused by the different boundary conditions for the electric field. Fig. 4. Transient temperature distribution of an argon arc with a current of 100 A under a mass flow rate of 0.005 kg/s. electrode surface should be quite dependent on the critical parameter of the current value and this should be carefully treated in future modelling of low current GlidArc behaviour. 5. Acknowledgements This research was supported by the Marie SkłodowskaCurie Individual Fellowship. 6. References [1] A. Fridman, A. Gutsol, S. Gangoli, Y.G. Ju and T. Ombrellol. J. Propul. Power, 24, 1216 (2008) [2] C.S. Kalra, A.F. Gutsol and A.A. Fridman. IEEE Trans. Plasma Sci., 33, 32 (2008) [3] A. Indarto, D.R. Yanga, J. Choib, H. Leeb and H.K. Song. J. Hazard. Mater., 146, 309 (2007) [4] I.V. Kuznetsova, N.Y. Kalashnikov, A.F. Gutsol, A.A. Fridman and L.A. Kennedy. J. Appl. Phys., 92, 4231 (2002) [5] Y. Wu, M.Z. Rong, A.B. Murphy, et al. IEEE Trans. Plasma Sci., 36, 2831 (2008) [6] M.Z. Rong, F. Yang, Y. Wu, et al. IEEE Trans. Plasma Sci., 38, 2306 (2010) [7] F. Karetta and M. Lindmayer. IEEE Trans. Comp. Trans. Packag. Manufact. Technol., 21, 96 (1998) [8] W.Z. Wang, M.Z. Rong, A.B. Murphy, et al. J. Phys. D: Appl. Phys., 44, 355207 (2012) [9] M. Lindmayer, E. Marzahn, A. Mutzke, T. Ruther, and M. Springstubbe. IEEE Trans. Compon. Packag. Technol., 29, 310 (2006) [10] Ansys Fluent v12.0 user guide; ANSYS Inc. (2009) [11] Y. Wu, M.Z. Rong, X.W. Li, et al. IEEE Trans. Plasma Sci., 36, 2831 (2008) 4. Conclusions The gliding behaviour of a DC argon arc under the gas blast and externally applied magnetic field is studied in this paper using a 3-D MHD model based on the assumption of local thermodynamic equilibrium. It is found that the current density can greatly influence the magnetic force under the condition of externally applied magnetic field and hence an arc tailing phenomenon occurs behind the arc column with temperatures of several thousand kelvins. Moreover, the gas blast can drag the column toward the diverging downstream section in a quite thin shape due to the strong cooling effects. A thermal arc with a relatively high current, as considered in our current work, can strongly heat the electrode and influence the thermionic electron emission processes of the cathode. Therefore, the energy interaction between the arc and electrode should have a great influence on the arc root current density distribution and hence on the gliding behaviour. For a low current GlidArc, there is no significant heating of the cathode surface and the discharge is sustained by field electron emission from the cathode, accompanied by the formation of a cathode spot. Therefore, the plasma and electrode interaction and hence the gliding behaviour along the 4 P-II-12-18
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