22nd International Symposium on Plasma Chemistry July 5-10, 2015; Antwerp, Belgium Laser triggered discharge gap S.G. Davydov, A.N. Dolgov, V.O. Revazov, V.P. Seleznev and R.Kh. Yakubov Dukhov All_Russian Research Institute of Automatics, ul. Sushchevskaya 22, RU-127055 Moscow, Russia Abstract: Based on the data obtained in the experiment, an assumption about discharge development mechanism in laser trigged discharge gap was made. Initially, under the action of the laser pulse, a glow discharge in electrode erosion products is ignited. Then as the result of ionization-overheating instability the current channel undergoes contraction and glow discharge transforms into an arc. Keywords: vacuum gap, laser pulse, current delay, glow discharge, arc, instability 1. Introduction The aim of the presented work is to study physical processes, which occur during laser excitation of electrical discharge in a vacuum. The range of laser pulse intensity (q) used in experiments was between 3×106 and 3×109 W/cm2. In such a wide range of radiation intensity values a wide range of physical phenomena and processes is possible: from melting and evaporation to ionization of the vapor and absorption of incident radiation by the plasma. 2. Scheme of the experiment Pulsed solid-state LGI-60 laser in Q-switched mode generates radiation with a wavelength of 1.06 µm and time duration at the base of 20 ns. The discharge gap was placed in a glass vacuum chamber, which was evacuated to a residual gas pressure not higher than 10-1 Pa. Flat cathode target was at a zero potential with respect to a ground bus. The aluminium anode shaped as a flat ring before switching of a vacuum gap had a positive voltage of 3 kV. Laser radiation was focused on the surface of the cathode through the wall of the vacuum chamber so that the radiation beam passed through an opening with diameter of 2.5 mm in the anode center without losses. A focusing lens with a focal length of F = 50 mm was used in experiments. A focal spot with diameter of 0.8 mm was obtained on the cathode. The energy flux of the laser radiation incident on the cathode was regulated by a set of calibrated absorbing filters placed in front of the converging lens. The distance between the cathode and the anode was 1 mm. A circuit, switched by a discharge gap, consisted of a capacitor and a set of resistors. The current in the cathode-anode gap had an amplitude up to 100 A. The duration of the front edge of the current pulse was about 100 ns with a rise rate of the current dI/dt = (1-2)×109 A/s. Measurements of a current flowing through the gap during the discharge process were conducted with a calibrated Rogowski coil. The signal from the Rogowski coil was fed through a coaxial cable to the input of a high-speed oscilloscope. The signal from a high-speed photodetector was fed to the second input of the same oscilloscope. P-II-4-3 3. Results A wide range of laser radiation energy incident on the cathode surface was used, E LP = 2×10-6 - 2×10-3 J. The average intensity of the laser radiation on the surface of the cathode within the focal spot was calculated as: q= E LP , τS (1) where τ = 10 ns - laser pulse duration at half-height, S - area of the focal spot. The range of laser pulse intensity (q) used in experiments was between 3×106 and 3×109 W/cm2. In such a wide range of radiation intensity values a wide range of physical phenomena and processes is possible: from melting and evaporation to ionization of the vapor and absorption of incident radiation by the plasma [1]. In the course of these experiments, a minimum energy of the laser pulse radiation required to initiate a discharge in the studied vacuum gap was determined, and measurements of time parameters of the commutation process of discharge gap at a different energy of laser pulse radiation, constant pulse duration and constant area of a laser beam focal spot were conducted. Oscillograms of the discharge current were obtained and with a fixed value of E LP a distance on a time scale between specific points of discharge current oscillogram was determined (Fig. 1): 1 - start of the laser pulse; 2 - the time when the current with significant value occurs in a discharge circuit; 3 - feature (splash or fracture) on the oscillogram; 4 - moment when the maximum current in the circuit is achieved. Based on the data obtained, graphs of relation of duration of time intervals τ 1-2 , τ 1-3 , τ 1-4 to the E LP value were plotted for different cathode materials. Fig. 2 shows graphics of obtained experimental data for cathode made from Kovar (alloy 29NK). Note, that dependences τ 1-2 (E LP ), τ 1-3 (E LP ), τ 1-4 (E LP ) for mentioned materials (as well as for a variety of other materials that were tested, including aluminum, wolfram, stainless steel, copper , tantalum, titanium, graphite) have 1 almost identical shapes, which indicates the uniformity of the processes. 2 P-II-4-3 current pulse with increase of E LP , and the second branch, which corresponds to rapid changes of mentioned parameters with increase of E LP , and then the approximate position of intersection point of these lines was determined. For small values of E LP the current in the discharge circuit is not registered during 100 ÷ 200 ns after the end of laser pulse. For large E LP current in the discharge circuit is registered almost immediately after the start of cathode surface irradiation. Fig 1. Character oscillograms of vacuum gap commutation. Fig 2. Time parameters τ 1-2 , τ 1-3 , τ 1-4 as a function of laser pulse energy E LP for cathode of Kovar alloy. With relatively small E LP (below the threshold) in the range 2 ÷ 20 mJ (q = 3×106 ÷ 3×107 W/cm2) timeslots τ 1-2 , τ 1-3 , τ 1-4 vary slightly. For relatively large E LP (above the threshold) in the range of 200 ÷ 2000 mJ (q = 3×108 - 3×109 W/cm2) with increase of E LP the duration of the intervals τ1-2 and τ 1-3 decreases rapidly, and the duration of the interval τ 1-4 apparently reaches a plateau, which is defined by the parameters of the switching circuit. The threshold value of the E LP for each of mentioned materials was determined by finding the inflection point on the corresponding plot. For this purpose, an approximation of two branches of the graph was done, i.e., approximation of the first branch, which corresponds to slight changes of time parameters of the P-II-4-3 4. Discussion For relatively small values of E LP , i.e., less than the threshold, based on the intensity value of laser radiation incident on the cathode, proceeding from the fact that the current in the circuit, which is commutated by vacuum gap, is not registered during considerable period of time after the end of laser pulse, one can assume, that the weakly ionized vapor clot expands into the interelectrode space [2, 3]. Probably, a low-current glow discharge is ignited in the mentioned area and an external border of vapor clot, which is pointed at anode, plays the role of electrons emitter. The closure of the interelectrode gap by conducting medium and neutralization of space charge significantly increases the current registered on the oscillograms. Further, apparently, ionization-overheating instability of the glow discharge leads to the contraction of the current channel [4-6] and, respectively, leads to further heating of local region of cathode surface. This is followed by an increase in flux density of electrons produced by thermionic emission, in particular, due to the electric field intensity at the cathode surface and increase in flux density of ions from plasma to the cathode. The increase in density of evaporable or sublimated substance of electrode at its surface will lead to the decrease of electron's mean free path and, accordingly, to the decrease of the layers width of cathode potential drop, i.e., again electric field intensity and density of electron emission current from cathode will increase. The action continues till formation of the cathode spot, i.e., initiation of selfreproducing centers of explosive electron emission – the so called ectons [1]. Discharge transforms into an arc. The presence of bursts on the oscillogram (on the current pulse front) indicates, in our opinion, development of instability in a glow discharge, when it undergoes transformation from normal to abnormal form [7], and then transforms into an arc. For relatively large values of E LP , larger than the threshold, influence of laser radiation on the process of development of ionization-overheating instability in plasma of glow discharge, apparently, becomes a distinctive feature of the discharge. When E LP reaches the threshold value, an effective ionization of the cathode material vapors begins due to the breakdown of neutral gas in the field of electromagnetic wave with the further active absorption of laser radiation in produced plasma [8]. 3 In the presence of laser radiation flux development of instability happens faster, as local increase in temperature and degree of vapor ionization leads to increase of absorption of laser radiation and to further heating and, accordingly, to increase of ionization degree and conductivity of plasma, i.e., current contraction. Moreover, probably, the process of filling of interelectrode space by plasma develops faster. The result is acceleration of process of condition formation for arc ignition with the increase of E LP . Indeed, this assumption is in agreement with experimental data obtained in research [9] of scattering of laser-plasma torch by shadow photographing methods with pulsed laser as illuminator and with high-speed photographing. If our hypothesis is correct (we have glow discharge in the cathode material vapor on the first stage of a process), what parameters will turn out to be defining for the ELP value in the first approximation? Probability of molecule vapor ionization by electron impact will be determined by an average value of free electrons energy and the latter in turn will depend on the thermal energy of electrons, i.e., on the electrons temperature T and on the possibility of gaining the energy in electric field applied to the gap. The latter circumstance is determined by expansion rate of vapor formed during heating of the cathode by laser pulse. Energy is proportional to (Т∕μ)1/2. Further, influence of the initial density of vapor should be considered, which will be determined by the amount of vaporized substance, i.e., cathode heating depth by laser radiation, which, in turn, can be estimated as (τχ)1/2 , where τ – laser pulse duration, χ – coefficient of thermal diffusivity. By temperature we assume the melting temperature of cathode material as we are talking about the minimum value of required radiation energy. The diagram which demonstrates interconnection of (E LP ) min and designed parameter (Т3∕χμ)1/2 is presented in the Fig. 3. Fig. 3. Distribution diagram of cathode material for minimum value of radiation energy (E LP ) min dependence of parameter (Т3 ∕χμ)1/2. 4 The diagram shows the notable trend and can be used for preliminary search of the optimal cathode material for energy minimization of the laser pulse. The threshold value (E LP ) thre is determined by plasma expansion rate, which does not depend on the ion mass [10], according to experimental data, in condition of continuing laser pulse and is determined by electrons rate. The diagram which demonstrates interconnection of (E LP ) thre and designed parameter (Т∕χ) is presented in the figure 4, where T – boiling temperature of cathode material. Fig.4 Distribution diagram of cathode material for threshold value of radiation energy (E LP ) thre dependence of parameter (Т vap ∕χ). The major portion of researched materials fits into the scope of trend, the minor portion, aluminum and tungsten, do not fit in the scope. It can be assumed that this circumstance is tied with features of change of phase state dynamic of different materials under the action of highenergy laser radiation. Initially, under the influence of high-energy laser radiation on the surface of condensed matter, a thin surface layer of material heats up. This layer, in turn, through heat transfer mechanism becomes a source of heat wave, which spreads inside of the body. The heat wave rate in case of the constant heat conduction, density and specific heat of material decreases within time as t-1/2. On the other hand, at some moment of time the temperature on the material surface increases so much that the considerable evaporation begins. From this moment an evaporation wave will spread inside the matter and the wave rate will increase jointly with the temperature increase and will reach the stationary value of v evap ≈ q/ρr, where ρ – the density of condensed matter , r – specific heat of evaporation. At the moment of time t crit the evaporation wave rate will be equal of the heat wave rate. Provided that t crit < τ, where τ – laser pulse duration, the influence of laser radiation on the condensed matter practically comes down to the evaporation regime in which the heat conduction does not play a considerable role. The radiation intensity value should exceed q crit value, which is determined by expression [2]: P-II-4-3 χ 1 (2) τ The obtained data demonstrates that the regime of influence of laser radiation at intensity threshold value q thre for aluminium and tungsten radically differs from the regime for other researched materials. If the major part of researched materials is in conditions close to boundary conditions, then aluminum is in the conditions of heatconducting regime and tungsten – in evaporation regime. qχρiτ ≈ ρρ ( ) 2 , Table 1. material. Distribution q crit /q thre parameter of cathode Material W Al Kov Cu Mo q crit /q thre 1.8 0.017 0.2 0.11 0.2 Material Fe Ta Ti C q crit /q thre 0.07 0.2 0.3 0.5 [6] E.P. Velihov, A.S. Kovalev and A.T. Rahmanov. Physical phenomenon in the gas-discharge plasma. (Moscow: Nauka) 160 [in Russian] (1987) [7] S.K. Gdanov, V.A. Kurnaev, M.K. Romanovskii and I.V. Tsvetkov. Fundamentals of physical processes in plasma and plasma plans. (Moscow: MEPHI) 368 [in Russian] (2207) [8] Yu.P. Rayzer. Laser spark and diffusion of breakdowns. (Moscow: Nauka) 308 [in Russian] (1974) [9] N.B. Delone. Interaction laser radiation with matter. (Moscow: Nauka) 280 [in Russian] (1989) [10] V.S. Vorob’ev. “Plasma arising during the interaction of laser radiation with solids”. PhysicsUspekhi (Adv. Phys. Sci.) 36, 1129-1157 (1993) 5. Conclusions In the present paper it is demonstrated that the character of dependence of registered time parameters from radiation energy is the same for different cathode materials. For relatively small E LP (less than the threshold value (E LP ) thre ) in the range of 2 - 20 μJ (q = 3×106 - 3×107 W/cm2), registered time intervals change slightly or even remain constant within the random error interval. For relatively large E LP (larger than the threshold value E LP ) thre ) in the range of 200 – 2000 μJ (q = 3×108 - 3×109 W/cm2), the duration of time intervals, which characterize the speed of discharge gap commutation process by wellconducting medium, reduces with increase of E LP value. Value of the minimal laser pulse energy required for ignition of a vacuum gap (E LP ) min and threshold energy (E LP ) thre , from which the dependence of the registered time parameters of commutation process from laser pulse energy is observed, is determined by thermodynamic parameters of cathode material. 6. References [1] G.A. Mesyats. Ectons in Vacuum Discharges: Breakdown, Spark, and Arc. (Moscow: Nauka) [in Russian] 424 (2000) [2] O.B. Anan`in, Yu.V. Afanas`ev and O.N. Krohin. Laser plasma. Physics and application. (Moscow: MEPHI), 400 [in Russian] (2003) [3] D.A. Cremers and L.J Radziemski. Handbook of Laser Induced Breakdown Spectroscopy. (New York: Wiley) (2006) [4] L.M. Biberman, V.S. Vorob`ev and I.T. Yakubov. Kinetics of nonequilibrium low-temperature plasma. (Moscow: Nauka) 375 [in Russian] (1982) [5] Yu.P. Rayzer. Physics of gas discharge. (Moscow: Nauka, Moscow) 536 [in Russian] (1992) P-II-4-3 5
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