22nd International Symposium on Plasma Chemistry July 5-10, 2015; Antwerp, Belgium Threshold electric fields for the inception of a primary streamer and a secondary streamer in water H. Fujita1, S. Kanazawa2, K. Ohtani1, A. Komiya1, T. Kaneko3 and T. Sato1 1 Institute of Fluid Science, Tohoku University, Sendai, Japan Department of Electrical and Electronic Engineering, Oita University, Oita, Japan 3 Department of Electronic Engineering, Tohoku University, Sendai, Japan 2 Abstract: The influence of gap distance, capacitance, and water conductivity on the inception electric fields of a primary streamer and a secondary streamer was investigated when a single-shot pulsed positive voltage with a duration of 10 µs was applied to a needle electrode in water. As the inception electric fields were estimated to be constant regardless of the discharge parameters, it was suggested that there are threshold electric fields for the inceptions of a primary streamer and a secondary streamer. Keywords: underwater discharge, electric field, primary streamer, secondary streamer 1. Introduction Streamers in water are pre-breakdown phenomena, mainly observed as the development of luminous filaments from a needle electrode submerged in water. We have investigated the initiation process [1], the propagation process of a primary streamer [2] and a secondary streamer [3] through the highly spatiotemporal visualization of streamer discharges in ultra-pure water. Initiation process is the time lag process between the beginning of voltage application and the streamer inception. During the initiation process, Joule heating increases the water temperature at the tip of a needle electrode and results in the formation of a gaseous region by evaporation. Weak discharges occur in the gaseous region. Protrusions are formed on the surface of the gaseous region and then an electric field is concentrated at the tip of the protrusion. Streamers are initiated from the tip of the protrusion. Generally, a primary streamer with a semi-spherical brush-like structure appears at a lower voltage level and a secondary streamer with a filamentary structure appears at a higher voltage level. However, the influence of discharge parameters on the appearance tendency of a primary streamer and a secondary streamer has not been clarified. In this study, the influence of the discharge parameters such as gap distance, capacitance, and water conductivity on the inception electric fields of a primary streamer and a secondary streamer were investigated. 2. Experimental methods Figure 1 shows a schematic of the experimental setup. A single-shot pulsed high voltage with a duration of 10 µs was generated through a high voltage circuit. A DC power source charged up the ceramic capacitor, the capacitance of which was changed in 666 pF, 2 nF, and 6 nF. The charged electrons were transferred to a discharge part when a MOS-FET switch was turned on. The discharge part was composed of a needle-to-wire electrode system, P-I-3-23 High voltage probe Pulsed power source Current probe Electrodes High speed camera Water Fig. 1. Schematic of experimental setup. the gap distance of which was changed in the range of 2 – 10 mm [1-3]. The pulsed high voltage was applied to the needle electrode with a tip radius of around 40 µm. The wire electrode was grounded. Both electrodes were made of a platinum wire with a diameter of 500 µm and were covered with insulation tubes except for their tips. The discharge reactor was filled with 3 ml of ultrapure water (Milli-Q water) and its typical electrical conductivity was 0.8 µS/cm after exposure to atmospheric air. Water conductivity was adjusted in the range of 0.8 µS/cm to 1 mS/cm by adding sodium chloride to ultra-pure water. Inception voltage is defined as the applied voltage level at which a streamer appears with a probability of 20%. This is because 20% would be the minimum appearance rate to eliminate the influence of the individual variability of the needle electrodes. Actual inception voltage V ai is the inception voltage considering the voltage decay during the initiation time. Inception electric field E i is estimated by the actual inception voltage as follows [4]: , (1) 1 electric fields of a primary streamer and a secondary streamer in water with various conductivities. The water conductivity also had little influence on the inception electric fields. The inception fields of a primary streamer Fig. 2. Inception electric field estimated by the equation (1) at rtip = 1 µm vs. gap distance. (σ = 0.8 µS/cm, C = 666 pF) Fig. 5. Threshold electric fields for the inception of a primary streamer and a secondary streamer in water. Fig. 3. Inception electric field estimated by the equation (1) at rtip = 1 µm vs. capacitance. (d = 6 mm, σ = 0.8 µS/cm) and a secondary streamer were estimated to be constant, respectively, regardless of the discharge parameters. This result shows that there are threshold electric fields for the inceptions of a primary streamer and a secondary streamer. The threshold field of a primary streamer is estimated to be 23 MV/cm and that of a secondary streamer is estimated to be 34 MV/cm. That is, if the local electric field at the tip of a protrusion exceeds 23 MV/cm, a primary streamer can propagate from the protrusion. If the local electric field exceeds 34 MV/cm, there is the possibility of secondary streamer propagation in addition to primary streamer propagation as shown in Fig. 5. 4. Conclusion It was suggested that there are threshold electric fields for the inceptions of a primary streamer and a secondary streamer, respectively. This is because the inception fields were estimated to be almost constant when the gap distance, the capacitance, and the water conductivity changed. Fig. 4. Inception electric field estimated by the equation (1) at rtip = 1 µm vs. conductivity. (d = 6 mm, C = 666 pF) where r tip is the tip radius of a protrusion on the gaseous region, and d is the gap distance. Here, the inception field is calculated assuming r tip = 1 µm [1, 5]. 3. Results and Discussion Figure 2 shows the inception electric fields of a primary streamer and a secondary streamer at each gap distance. The gap distance had little influence on the inception electric fields. Figure 3 shows the inception electric fields of a primary streamer and a secondary streamer at each capacitance. The capacitance had little influence on the inception electric fields. Figure 4 shows the inception 2 Acknowledgements This study was partly supported by a Grant-in-Aid for Scientific Research from JSPS, by a grant from the Collaborative Research Project of the Institute of Fluid Science, Tohoku University, and by a grant from Tohoku University International Advanced Research and Education Organization. The author wishes to thank Tomoki Nakajima, Tohoku University, for technical support. References [1] H. Fujita et al., J. Appl. Phys., 116, 213301 (2014). [2] H. Fujita et al., J. Appl. Phys., 113, 113304 (2013). [3] H. Fujita et al., EPL, 105, 15003 (2014). [4] P. Gournay and O. Lesaint, J. Phy. D: Appl. Phys., 26, P-I-3-23 1966 (1993) [5] H. Fujita et al., IEEE Trans. Plasma Sci., 42, 2398 (2014)
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