Quasi-uniform planar plasma jet generated by using an atmospheric pressure DBD configuration Qing Li 1,2, Hidemasa Takana 1, Yi-Kang Pu 2, and Hideya Nishiyama 1 1 Institute of Fluid Science, Tohoku University, 2-1-1, Katahira, Aoba-ku, Sendai, 980-8577, Japan 2 Department of Engineering Physics, Tsinghua University, Beijing, 100084, China Abstract: A stable non-thermal quasi-uniform planar plasma jet, originating from a planar dielectric duct with a rectangular exit and injecting into ambient air at atmospheric pressure of room temperature, is reported in the present work. Current-voltage characteristics, one discharge current pulse per sinusoidal half voltage cycle, show that the discharge is not filamentary. Its spatial uniformity in the transverse direction is shown to be excellent by monitoring optical emission spectra in the jet core region other than jet boundaries. These observations are a challenge to the explanation of the traditional single streamer model for the propagation of non-thermal plasma jets. Keywords: atmospheric pressure plasma jets, dielectric barrier discharge, nonthermal plasma, planar plasma jets, uniform discharge 1. Introduction Homogeneous plasmas with large scale and low temperature have a great potential for applications, such as the uniform biological treatment and large industrial scale process by using the configuration of dielectric barrier discharge (DBD) at atmospheric pressure [1, 2]. This kind discharge has been observed in atmospheric pressure chambers [3, 4], but has not been obtained as atmospheric pressure plasma jets (APPJs), which are free of the vacuum system. Recently the non-thermal APPJ of several centimeter length, originating from a DBD tube wrapped with power electrode and injecting into ambient air, has made it possible for the plasma direct treatment in the discharge region [5 - 8]. However, the APPJ cross sectional emission pattern typically covers only a few mm2, which is too small for large scale applications. To generate large scale plasmas, arraying up of many DBD APPJs in parallel was designed [9]. Its uncontrolled interaction between plasma jets resulted in unstable and non-uniform discharge [9]. In this work, we report an attempt study of plasma jets generated in a planar DBD duct with a rectangular exit, which can generate a large scale quasi-uniform discharge in the transverse direction in the jet core region. Fig. 1 (a) Schematic of the experimental setup; and (b) photo of the planar DBD plasma jet in the case of 7.3 kV applied voltage. 2. Experimental setup Figure 1(a) shows the schematic of the experimental setup. The origin is located at the exit of the rectangular duct on central axis. The helium gas flows through a planar quartz duct, 3.1 mm × 50.0 mm × 300 mm (inner) and 6.1 mm × 53.0 mm × 300 mm (outer). A copper strip of 30 mm × 312 mm worked as a power electrode is wrapped around the duct and the separator is made of Teflon block. A copper plate of 40 mm × 150 mm as a grounded electrode is attached only one side of the duct. The two electrodes were fixed at z = 7.0 cm and z = 1.0 cm upstream from the rectangular exit, respectively. In experiment, the applied sinusoidal voltage of 10.0 kHz and the discharge current were recorded by a digital oscilloscope (Tektronix TDS 2024C, bandwidth 200 MHz) with a high voltage probe and a high current probe, respectively. Gas flow rate was fixed at 20.0±0.2 L/min, controlled by a mass flow controller. Optical emission spectra, used to investigate the discharge processes and to monitor the discharge uniformity, were recorded at different locations along z-axis using a spectrometer (Ocean optics MAYA 11127). Its fiber probe was placed at 2 cm and perpendicular to the duct outer surface. The discharge photo was taken by a digital camera, as shown in Fig. 1(b). The luminescent jet length is about 4 cm in the case of 7.3 kV applied voltage. 3. Experimental Results Figure 2 shows typical waveforms of the instantaneous applied voltage on the electrode and the discharge current, i.e., the total current subtracted the displacement current. The discharge is characterized by one current pulse per half cycle of the applied voltage. The amplitudes of the sinusoidal applied voltage presented in Fig. 2(a) and (b) are 6.5 kV and 7.3 kV, respectively. The current pulse peak values presented in Fig. 2 are 7.6 mA and 7.9 mA in the positive half cycles, while they are 5.2 mA and 5.5 mA in the negative cycles, respectively. The first current pulses increase to their peak values at about 3 μs and 7 μs as shown in Fig. 2(a) and (b), respectively. These characteristics suggest that the Fig. 2 Typical waveforms of the applied voltage (red dashed line) and the discharge current (blue solid line). The amplitudes of the applied voltages on the gas flow are (a) 6.5 kV and (b) 7.3 kV, respectively. plasma tends to be a continuous DBD discharge [4], instead of a filamentary discharge whose current is characterized by multiple current pulses of a series of microdischarges per half cycle of the applied voltage with a typical microdischarge current pulse width of 100 ns [11]. Comparative analysis of Fig. 2(a) and (b) can also suggest that the current slowly increases with applied voltage, and this is consistent with glow-like discharge [12]. Figure 3 shows the spectra at different plasma locations from upstream to downstream along z-axis with the applied voltage of 7.3 kV. Spectra (a)-(d) are corresponding to z = - 9.0 cm, z = - 4.5 cm, z = 0.5 cm, and z = - 0.5 cm, respectively. Spectra (a) and (b) show the continuous emissions, the helium lines, and the bands from residue gases of H2O and O2 in the upstream region. Spectrum (c) shows weak emissions from He, H2O, and N2. Spectrum (d) shows that bands from the N2 (C 3∏u – B 3∏g) bands. These spectra characteristics are consistent with the optical emission colors in different locations of Fig.1(b): blue in the downstream region (mainly from nitrogen) and dark between the power electrode and the exit. The high concentration of helium in the upstream region results in the formation of He2 [13, 14], and the high electron concentration and temperature, due to the requirement of the high helium excited energy. These effects are responsible for the presence of the bands from OH and He2 in the spectra (a) and (b), and the continuum radiations, which are possible from the recombination of electrons and positive ions, such as H2O+, O+, He+, and He2+. decreases in the downstream region, possibly since the high collision cross section between electrons and Figure 4 shows the distributions of 337 nm emission intensities from N2 and the gas flow velocities in the transverse direction (i.e., x direction) with difference distances downstream the exit (i.e., different z values). The gas velocities are uniform in jet core and non-uniform in the jet boundary due to the development of thick boundary layers, where the helium flow mixes with entrained ambient air. The 337 nm emission intensities show similar characteristic, and the non-uniform in the jet boundary are possibly due to that the different mixing ratios of air in helium plasma can result in different reaction possibilities between helium and entrained air [15]. The quasi-uniform distribution (in the jet core region) of the emission 337 nm intensities (representing the discharge emissions) is consistent with the distribution of the gas flow velocities (representing the gas compositions). 4. Discussion Comparing with single tube plasma jets [14, 16], our discharge current pulse is several times wider. This electrical characteristic is consistent with spectra in Fig. 3. The high intensity discharge between two electrodes generates high concentrations of charged particles and metastable helium states, which could result a high preionization level to ignite a quasiuniform planar jet [4]. The electron temperature Fig. 3 Relative optical emission spectra (left) from 290 to 385 nm and (right) from 390 to 900 nm. The pink (a), green (b), red (c), and blue (d) spectra are corresponding to z = - 9.0 cm (the center of grounded electrode), z = - 4.5 cm (the space center between two electrodes), z = - 0.5 cm (the space center between the power electrode and the exit), and z = 0.5 (0.5 cm downstream away from the exit), respectively. The base lines are shifted in order to distinguish these spectra. The voltage amplitude is 7.3 kV. in-Aid for Challenging (No.22656004). Exploratory Research References Fig. 4 Distributions of emission 337 nm intensities and gas flow velocities along the transverse direction (x direction) with different z locations. The voltage amplitude is 7.3 kV. diatom molecules such as entrained N2 and O2. However, its large scale in the transverse direction and its rectangular cross-section direction could not be explained by the traditional single streamer model [16, 17], which propose that the plasma jet is a streamer propagation with a cylindrical symmetry channel. Its optical emission and discharge current suggest that it is a continuous discharge with large scale and non-cylindrical channel, and tend to sustain our previous proposed streamer-coupling model [18], which explains that the formation of plasma jets is the propagation of many simultaneous streamers coupling with each other. Comparing with small tube plasma jets, the long planar DBD jet is more important for its applications [19]. 5. Summary A non-thermal planar plasma jet is obtained by using a planar dielectric duct. Electrical and optical characterizations of the planar APPJ have been used to demonstrate its stability and spatial quasiuniformity of the DBD plasma jet in the transverse direction. 6. 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