The effect of geometric modification on the performance of AC arc torch K. T. KIM, D. G. KIM, J. O. LEE, D. H. LEE, M. HUR and Y. H. SONG Environmental and Energy Systems Research Division, Korea Institute of Machinery & Materials 104 Sinseong-Ro, Yuseong-Gu, Daejeon 305-343, Korea Abstract: Design approach for the development of plasma torch with long lifetime by less erosion of electrode and volumetric generation of plasma has been carried. Plasma torch is based on the „rotating arc‟ design and the effect of different geometry of ground electrodes or step, linear and diverge types were compared. The application of the plasma torch is high temperature gasification process of waste to make synthesis gas and the process requires long lasting electrode and volumetric plasma. Both the shape of the ground electrode end tip and length affect generation of plasma volume. Comparison was done among selected geometries based on the size of the plasma volume generated, thermal efficiency, changes in electrical characteristics or I-V relation and erosion of electrode. In this study, diverge type was chosen to be best for the gasification process that was good at both volumetric generation of plasma and long lasting electrode. Keywords: plasma torch, gasification process, electrode lifetime, volumetric plasma 1. Introduction Requirement for the plasma reactor for an efficient gasification process can be listed as follows, 1) enhancement of thermally active volume, 2) enduring operation of electrode, 3) flexibility of diverse working gas, 4) high efficiency and so on [1, 2]. Most of current plasma torches used in the waste treatment are based on the DC torch technology and can be classified as rod type cathode and hollow type cathode as given in Figure 1. Rode type cathode sustains discharge by thermionic emission of electron in cathode and usually ThO2 embedded tungsten is used to maximize the thermionic emission. On the contrary, hollow type sustain arc discharge by field emission and for this reason, Cu that is good in thermal and electrical conductivity is commonly used as electrode material. Moreover, in view of application most important difference between rod type and hollow type is on working gas. In the case of rod type, working gas containing oxygen results in generation of WO that is formed by reaction of thermally dissociated oxygen and tungsten. Tungsten has high melting point of above 3,000 K but WO has rather low melting point of below 2,000 K compared to tungsten resulting in increased erosion of electrode. In the case of hollow type, using Cu as an electrode material, both Cu and CuO has melting point of below 2,000 K and not better than tungsten. However, arc point is not anchored or focused, different to the case of rod type, and can be moved both axial and radial direction, the drawbacks of relatively low melting point can be overcome [3-5]. In this study, arc plasma reactor with rod type electrode for waste gasification is developed as shown in Figure 2. Discharge gas is N2 that has high enthalpy and favorable for thermal decomposition of wastes. AC driven discharge is adopted to avoid imbalance of electrode erosion between cathode and anode that is often observed in DC driven discharges. Determining parameters of plasma volume are input voltage, geometry of ground electrode. In this study, 3 different type of ground electrode are considered for comparison. Step, linear and diverge are the three. With the same applied power condition, comparison of plasma flume and degree of electrode erosion has been done among these types. All of the results obtained are used for optimal design of the reactor. Figure 1. Type of conventional DC arc plasma torches used for hazardous waste treatment (rod and hollow types). 2. Experimental 2.1 Experimental apparatus Experimental set-up consisted of a plasma reactor, a power supply, flow controllers, and measurement systems as schematically shown in Figure 2. The reactor consists of an inner conical high voltage electrode and an outer cylinder electrode. Initially an arc will be ignited at the shortest distance between electrodes (A-B), and owing to the convective flow effect it stabilizes at the longest distance (C-D). Elongated arc reactor can make longer arc string than conventional DC arc torch resulting in higher voltage condition and reduced current levels and all of which are favorable for endurance of electrode. AC power supply, which can provide up to 8 kV in rms value with 5~20 kHz tunable frequency, was used for plasma generation. The flow rates of gases were controlled by mass flow controllers (Brooks, 5850E-series), and this mixture is supplied tangentially into the top-section of the plasma reactor. Electrical power delivered to the reactor is measured by oscilloscope (Tektronix TDS5054B) with 1000:1 high voltage probe and current probe with amplifier that can measure up to 50 A (Tektronix TCP 303 current probe and TCPA300 amplifier). Image of plasma flume is captured by direct photography (Canon EOS 50D). 2.2 Test conditions Once the available life of electrode is over, overhaul of the process is required to change the electrode. Thus increase of available life of the electrode is essential factor of consideration in commercial application as well as production of volumetric generation of plasma flume. Figure 2. Schematic of the experimental setup. As shown in Figure 3, all three types or step, linear and diverge shaped electrode are prepared and operated for 20 hours with the same condition of reactant flow rate of 70 L/min, input power of 10 kW. After the operation, each reactor is cut to cross sections to compare the degree of erosion. Also, for the comparison of reliability, voltage-current characteristics of each reactor are recorded. Flume image are used for the estimation of plasma volume generation. 3. Results and discussion 3.1 Comparison of step and linear type Determination of arc point in the ground electrode is closely related with the axial velocity of working gas. In the linear type, where the working gas flows toward the exit of the reactor, where the Lorentz force that is produced by cross product of gas dynamic drag force induced by axial velocity and magnetic field induced by arc current are balanced, the arc point is determined. At this stage, arc current, voltage, flow all has fluctuations of amplitude with time, the arc point can be moved and this movement prevents focusing of erosion. On the contrary, in the step type reactor, the flow confronts stagnant state at the point of step resulting in high possibility of focusing of arc point. Figure 3(a) and (b) show designed shape of step and linear types. In the case of linear type, it is not expected to have stagnant point. So, the arc string can have longer length and to make the arc point located within the reactor, length of the reactor is designed to have 2 times of that of step type (The diameter, D has the same dimension in both the cases). Figure 4 shows the comparison of voltage-current characteristics during 20 hours of continuous operation. All of the signals stabilized after initial spikes. Initial peaks are considered to be originated from the sensitive response of arc to non-eroded surface characteristics and after moderate erosion of electrode, the signals are stabilized. In the same input power condition, linear type has high voltagelow current state compared to step type and that is because linear type produces longer arc length. Figure 5. Comparison of electrode erosion shape between step and linear types. Figure 6. Comparison of plasma jet flame (a) step type (b) linear type. Figure 3. Shapes of grounded electrodes (a) step, (b) linear and (c) diverge types. 1.0 30 Voltage, Vrms [kV] 20 0.6 15 0.4 10 Linear(V) Linear(I) Step(V) Step(I) N2 flowrate: 70 L/min Discharge power: 10 kW 0.2 0.0 0 4 8 12 16 Current, I [A] 25 0.8 5 0 20 Figure 5 shows cross cut of the electrodes after 20 hours of operation. Step type has focused erosion point around step area but linear type has rather wide distribution of arc point after the length of L and as a result, no visible erosion is observed. Figure 6 compares the shape of plasma flume of the two cases. Linear type has rather smaller volume of plasma flume. With the results, linear type is evaluated to be better in view of endurance, but step type has better in generating reactive volume. 3.2 Comparison of linear and diverge type To overcome rather smaller plasma volume of linear type, diverge type that has diverging part in linear type reactor are proposed as shown in Figure 3(c). Operating time [hr] Figure 4. Comparison of voltage-current characteristics with operating time between linear (circle) and step (triangle) types. Erosion states after test of 20 hours are given in Figure 7 and plasma flumes are given in Figure 8. From figure 7, we can find that the diverge type still have the merits of wide distribution of arc point and Figure 8 shows that the effect of adding diverging part is favorable for larger plasma volume. It is suggested that more in detail optimization for enlargement of plasma volume should be followed. Figure 9 shows these optimization works to make larger plasma volume. Among the tested conditions, 40mm of exit diameter shows best performance for volumetric plasma generation and also reliability. Figure 7. Electrode erosion shape of diverge type. 4. Conclusions Optimization work for the development of plasma reactor for waste gasification process is presented. Step type shows best performance in generating volumetric plasma and efficiency. However for the focusing of arc point the type results in a severe erosion of electrode. In the linear type, both axial and tangential movement of arc point induces distributed erosion and thus good endurance. However, volumetric generation of plasma that is essential for the gasification process is not guaranteed. Finally, diverge type that has diverging part at the end of linear type is proposed. Test results of diverge type show that it has merits of both the linear and step type. It has distributed arc point and generates larger volume of plasma than linear type. In succession, optimization of design in diverging part is done. It is expected to have more efficient gasification process with developed plasma reactor. Acknowledgement This work is supported by basic research program (NK163B) of KIMM and research program of Small & Medium Business Administration (AI1600). References Figure 8. Comparison of plasma jet flame (a) Linear type (b) Diverge type. Figure 9. Influence of diameter of diverge part on the plasma jet flame. (1) R. Benocci, G. Bonizzoni and E. Sindoni, 1995, “Thermal plasmas for hazardous waste treatment”, World Scientific, London (2) L. Bin, M. Kikuchi, L. Heping, T. 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