22nd International Symposium on Plasma Chemistry July 5-10, 2015; Antwerp, Belgium Electron density and temperature distributions in a supersonic dc plasma jet generated at reduced pressure J. Cao1,2, H. Huang1, W. Pan1 and C. Wu1 1 State Key Laboratory of High Temperature Gas Dynamics, Institute of Mechanics, Chinese Academy of Sciences, 100190 Beijing, P.R. China 2 Department of Nuclear Technology Application, China Institute of Atomic Energy, 102413 Beijing, P.R. China Abstract: In this paper, two dimensional distributions of electron density and electron temperature of a plasma jet produced by a fixed arc-length torch are diagnosed by electrostatic triple probes. Knot-like distributions of the electron density and correspondence electron temperature distributions are observed. Possible mechanisms of such kind of distribution are discussed. Keywords: electron density, electron temperature, dc plasma jet, fixed arc-length 1. Introduction Being able to generate high enthalpy plasma jet, nontransferred dc plasma torch has been widely used in thermal spraying and coating technology [1]. However, conventional dc plasma torch with turbulent jet has large amplitude of fluctuations, which limited its application in tailoring fine coating structure [2, 3]. A stepped structure plasma torch with fixed arc-length has been developed in our group, which facilitates generating stable laminar plasma jet in a wide range of operating parameters [4-10]. In this study, electron density and electron temperature distributions of the plasma jet generated at reduced pressure are diagnosed by an electrostatic triple probe system to understand the characteristics of the plasma better. 2. Experimental methods measurements start at Z=11mm when the arc current is 80A and 90A, and starts at Z=27mm when the arc current is 100A. 3. Results and discussion Measured distributions of the electron density are shown in Fig. 2. A knot-like structure is clearly shown in all the measured distributions. With the increase of the arc current, the high density domains expand. There are no noticeable position change of the “knots”. Numerical simulations of the plasma show that under the experimental conditions, the plasma jets are in supersonic state, which leads to Mach-disks because of compressible flow. Although the shock diamonds are hardly distinguished in normal photographs of the jet under the present experimental conditions, they could easily been detected by the sensitive electrostatic probes. 80A 90A 0 0 0 20 20 20 100A Ne (/m3) 40 40 60 Z (mm) Z (mm) Z (mm) 40 60 80 80 100 100 1.5E+20 1.4E+20 1.3E+20 1.2E+20 1.1E+20 1E+20 9E+19 8E+19 7E+19 6E+19 5E+19 4E+19 3E+19 2E+19 60 80 Fig. 1 Schematic diagram of diagnosing system. 100 0 10 20 r (mm) Fig. 1 shows the schematic diagram of the diagnosing system.The chamber pressure is kept at 200Pa during experiments. Pure Argon is used and the flow rate is 8.5 slm. The arc current varies from 80A to 100A. The axial (z direction) and radial (r direction) spatial intervals are 8mm and 4mm respectively. The anode exit locates at Z=0mm. To prevent over heating of the probe tip, the P-I-2-30 0 10 20 r (mm) 0 10 20 r (mm) Fig. 2 Distribution of electron density at 80A, 90A and 100A. The anode exit locates at Z=0, and r=0 is the center axis of the torch and the jet. Fig. 3 shows the distributions of the electron temperature with different arc current. Comparing Fig. 2 1 and Fig. 3, it is clearly seen that some areas along the center axis with higher electron density have relatively lower electron temperature, and vice versa. While the outer region of the jet has low electron density and electron temperature. Possible mechanisms causing such kind of distribution include: 80A 90A 0 100A 0 0 Te (eV) 20 40 40 40 60 80 80 100 100 0 Z (mm) Z (mm) 20 Z (mm) 20 60 10 20 r (mm) 0 2.4 2.2 2 1.8 1.6 1.4 1.2 1 0.8 0.6 60 80 100 10 20 r (mm) 0 10 20 r (mm) Fig. 3 Distributions of electron temperature at 80A, 90A and 100A. First, the deviation from LTE (Local Thermodynamic Equilibrium) state in the plasma jet causes the electron temperature decreasing at the positions with higher density where collisions between electrons and heavy particles are more frequent. Usually in non-LTE state, electron temperature is higher than that of heavy particle, which means the collision will decrease the electron temperature, which leads to “Collision Cooling”. The second mechanism is ambipolar diffusion. The net charge current in the jet is zero everywhere, so the electron diffusion flux must equal to ion diffusion flux. Since electrons move far faster than ions, an electric field is induced with opposite direction with electron density gradient. An electron diffusing along the density gradient will be cooled down gradually due to the electric field, which is called “Diffusion Cooling”. This effect was studied in [11], and it was shown that the electron 2 temperature could be cooler than heavy particle temperature if the collision is not frequent. According to the radial electron density distribution as demonstrated in Fig. 1, the “Collision Cooling” effect cools the regions near the center, while the “Diffusion Cooling” effect cools the peripheral regions. This combination of this two effects results in the distribution as shown in Fig. 3. 4. Acknowledgement This work is supported by the National Natural Science Foundation of China (No. 11175226). 5. References [1] P. Fauchais, Journal of Physics D-Applied Physics, 37, pp. R86-R108 ( 2004). [2] Z. Duan and J. Heberlein, Journal of Thermal Spray Technology, 11, pp. 44-51 (2002). [3] S. Ghorui, M. Vysohlid, J. V. R. Heberlein, and E. Pfender, Physical Review E, 76 (2007). [4] H. Huang, W. X. Pan, Z. Y. Guo, and C. K. Wu, Journal of Physics D:Applied Physics, 43, (2010). [5] H. J. Huang, Z. Q. Fu, W. X. Pan, and C. K. Wu, "Fast plasma sintering deposition of nano-structured silicon carbide coatings," 18th International Vacuum Congress (Ivc-18), 32, pp. 598-604 (2012). [6] H. J. Huang, W. X. Pan, Z. Y. Guo, and C. K. Wu, IEEE Transactions on Plasma Science, 36, pp. 10521053 (2008). [7] H. J. Huang, W. X. Pan, and C. K. Wu, IEEE Transactions on Plasma Science, 36, pp. 1050-1051, (2008). [8] H. J. Huang, W. X. Pan, and C. K. Wu, Chinese Physics Letters, 25, pp. 4058-4060 (2008). [9] H. J. Huang, W. X. Pan, and C. K. Wu, Plasma Chemistry and Plasma Processing, 32, pp. 65-74 (2012). [10] W. X. Pan, Z. Y. Guo, X. Meng, H. J. Huang, and C. K. Wu, Plasma Sources Science & Technology, 18, (2009). [11] M. A. Biondi, Physical Review, 93, pp. 1136-1140 (1954). P-I-2-30
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