st 21 International Symposium on Plasma Chemistry (ISPC 21) Sunday 4 August – Friday 9 August 2013 Cairns Convention Centre, Queensland, Australia Graphical Analysis of LSD Wave Propagating Through a Diatomic Gas Using Thermal Non-equilibrium CFD Results H. Shiraishi1 1 Daido University, Nagoya, Japan Abstract: Laser-supported Detonation (LSD), one type of Laser-supported Plasma (LSP), is considered as one of the most important phenomena for laser propulsion systems; it can generate high pressure and high temperature, which are essential for propulsion, by absorbing a laser beam. In this study, p-v graphical analyses using the thermal-non-equilibrium and one-dimensional numerical results of LSD waves are performed for searching the detailed LSD structure propagating through a diatomic gas ,which are abundant in the atmosphere. Keywords: Numerical Analysis, Laser-supported Plasma (LSP), p-v Diagram Nomenclature D propagation velocity of detonation wave [m/s] I laser intensity [W/m3] I0 incident laser intensity [W/m3] h enthalpy per unit mass [J/kg] p pressure [Pa] p0 initial pressure of cold gas [Pa] t laser irradiation time [s] T temperature [K] u velocity in x direction [m/s] x x direction heat capacity ratio wavelength of incident laser beam density [kg/m3] 0 initial density of cold gas [kg/m3] Subscripts e 0 case of LSC, the shock front propagates almost adiabatically because the heat transfer from the laser absorption zone becomes much weaker. Therefore the transition from LSD to LSC is a very important theme for a laser propulsion system. For studying 1-dimensional (1-D) steady propagation of LSD, ZND (Zel’dovich-von Neumann-Doering) model, the classic 1-D distribution, is very important. Figure 1 and 2 show ZND model and p-v diagram of chemical detonation, non-dimensionalized by initial state, respectively. The point that both longitudinal axes indicate pressure makes easy to compare the two diagrams. electron initial cold gas 1. Introduction A beam (laser or microwave) propulsion system is one of the most promising next generation space propulsion systems. Laser-supported plasma (LSP) is essential for this system, because the laser energy is mainly absorbed by hot plasma and then converted to the kinetic energy that is necessary for propulsion. In this study, we investigate the use of laser supported detonation (LSD), a type of laser supported plasma (LSP), in a repetitively pulsed (RP) type laser propulsion system. LSD is also categorized as a type of hypersonic reacting flow, where exothermicity is supplied by laser absorption and not by chemical reaction. With the decrease in irradiative laser beam by LSD expanding, the detonation can be weaker and finally transform to LSC wave (Laser-supported Combustion- wave), in which the laser absorption zone detaches from the shock front. In the Fig. 1. ZND Mmodel for Cchemical Detonation. Fig. 2. p-v Diagram of Chemical Detonation. st 21 International Symposium on Plasma Chemistry (ISPC 21) Sunday 4 August – Friday 9 August 2013 Cairns Convention Centre, Queensland, Australia Fig. 3. Control Volume for Conservation Laws. In the diagram, three characteristic lines: Rayleigh, Poisson and Hugoniot curves exist. These lines derive from the Rankine-Hugoniot relation, which is composed by the conservation laws of mass, kinetic momentum and energy. The coordinate system in the conservation lows is shown in Fig.3. The difference between Poisson and Hugoniot lines is in the heat release value q[J/m3]. The Hugoniot line is calculated as follows: In the Poisson line, where q is equal to zero, therefore Poisson line indicates no-heat release case. Therefore von Nuemann state indicates the ignition delay where is no heat release by combustion as shown in Fig.1. As a practical case, Wang et al. [5] simulated LSD propagating in the inner geometry of a laser propulsion system, for example. Though some simulations for laser propulsions are studied, there had been no case which applies a detailed processes, such as multi-charged model [1], as far as I know. The objective of this study is to clarify the LSD propagation structure by applying p-v diagram to the simulation results. Especially, to evaluate the difference between the true distribution of LSD and the hypothetical ZND model shown in Fig. 4. , is important. 2. Numerical Model and Assumptions 2. 1. Analysis model Figure 5 shows the analysis model for the 1-dimensional study. The CO2 gasdynamic laser beam ( = 10.6μm) passes from the right to the left, and the LSD wave propagates through hydrogen gas at room temperature (T0 = 300K). In order to simulate the laser-supported plasma, a hot spot in which hot electrons are seeded, is set up to imitate the initial plasma. This hot spot model imitates the hot electrons, which are generated on a metal target by dielectric breakdown in an experiment [6]. In this study, the hot spot is placed at the center at x = 2 mm. The hot electron temperature is 30,000 K and the size of the hot spot is 2 mm (200 points 0.01 mm). Only 1% seeding rate is applied because the number of seeded electrons has little effect on the LSD propagation results; however, a high seeding rate is not good for the simulations. Fig. 4. Hypothetical ZND Model for LSD. Figure 4 shows the hypothetical ZND model for LSD. Though the frame zone is displaced by the laser absorption zone, the ionization delay is not clarified because the delay is remarkable only near the threshold condition in the conclusion of the previous work [1]. For simulating LSD propagation, 1-dimensional (1-D) steady and unsteady analyses [2] were performed at first, using a CO2 gasdynamic laser into argon gas, where the most important laser absorption mechanism for LSD propagation is Inverse Bremsstrahlung: The laser energy is transformed into the kinetic energy of free electrons by photon absorption during collisions of electrons with ions or neutral particles, which is re-distributed among heavy particles through collisions. As a numerical method, TVD scheme, which is taken into account of real gas effects, is applied. Though Quasi-1-dimenmsional analyses [3] were also performed, the dimension should be extended to axisymmetric 2-D model [4] for realistic cases. Fig.5. One-dimensional Analysis Model. 2. 2. Assumptions The assumptions for this analysis are the same as the previous work [1] except for the propellant gas. They are as follows: (1) The propellant gas is always electrically neutral. (2) Chemical reaction and laser absorption are considered. st 21 International Symposium on Plasma Chemistry (ISPC 21) Sunday 4 August – Friday 9 August 2013 Cairns Convention Centre, Queensland, Australia The chemical reactions considered in this model are as follows: 1500 1) H 2 H 2 H 2 2H Numerical Result Poisson 2) H 2 H 2H H (3) The thermal non equilibrium model is a p/p0 1000 3) H e H e e 500 two-temperature model. The electron temperature related to the electron-electronic excitation mode is separated 0 from the heavy particle temperature related to the other modes. (4)Transportation properties are considered. 2. 3. CFD method for graphical analyses In this study, CFD results are derived from one-dimensional Navier-Stokes solver using the Harten-Yee non-MUSCL modified flux-type TVD scheme, where the radiative energy transfer terms (Bremsstrahlung and Inverse Bremsstrahlung) are treated implicitly [7]. 2. 4. Laser absorption model In the presence of absorption, the local radiation intensity I(x, t) is governed by the following equation: dI ( x, t ) I ( x, t ) ( K ea K ei ) dx (7) 0.4 0.6 v/v0 (a) I0 = 60MW/cm2 1500 0.8 Numerical Result Poisson 1000 p/p0 With respect to the effective diffusion coefficient, the ambipolar diffusion is also considered. 0.2 500 0 0.2 0.4 0.6 v/v0 0.8 (b) I0 = 55MW/cm2 Fig. 7. p-v Diagram in LSD and LSC-LSD threshold. 3. Results and Discussion 3. 1. Initial conditions The physical conditions for analyses are shown in Table 1. Table 1. Initial Conditions for Analyses. Laser beam intensity Pressure of cool gas I0 = 50 - 65 MW/cm2 0.25atm 3. 2 Evaluation the difference between the LSD and LSC-LSD threshold Figures 7 shows the p-v diagrams in the case of (a) I0 = 5.5MW/cm2 , p0 = 0.2atm and (b) I0 = 4.9MW/cm2, p0 = 0.2atm. Here, we would like to emphasize again that the main object of this study is to evaluate the LSD structure by applying the simulation results, not simulation itself. In the case (a), the line from the numerical result gets into touch with the Poisson line except for the initial state. According to the p-v diagram of Fig. 2, this resembles the von Neuman state in the chemical detonation. This indicates the LSD propagation resemble the Hypothetical ZND Model for LSD in Fig. 4. On the other hand, the diagram of the case (b) intersects the Poisson line. As the laser absorption, which corresponds to the heat release in the chemical detonation, makes the line upper right, the energy loss in the case (b) excesses the laser absorption at the shock front. This energy loss is derived from dissociation and ionization. Therefore LSC-LSD threshold progagation will not be sustained in the weaker laser power. 4. Conclusions In order to studying the transition structure from LSD to LSC propagation, p-v diagraming from l-dimensional simulation is performed by applying the multiply-charged ionization model. The conclusions are as follows: st 21 International Symposium on Plasma Chemistry (ISPC 21) Sunday 4 August – Friday 9 August 2013 Cairns Convention Centre, Queensland, Australia (i) The p-v diagraming makes clarify the structure of laser absorption because the same discussion of the heat release as in the chemical detonation, which is induced by the Rankine-Hugoniot relation, is effective. (ii) The ionization delay length exposes in the typical LSD threshold in the diatomic gas. Therefore the LSD structure resembles the hypothetical ZND model for LSD, which is assimilated by that for chemical detonation, in the normal LSD propagation. (iii) In the LSC-LSD threshold, p-v diagram intersects the Poisson line. This differs from in the typical LSD case and indicates the energy loss derived from dissociation and ionization excesses the laser absorption at the shock front. Therefore LSC-LSD threshold propagation will not be sustained in the weaker laser power. 5. References [1] Shiraishi, H. and Kumagai. Y., Numerical Analysis of Threshold between Laser-Supported Detonation and Combustion Wave Using Thermal Non-Equilibrium and Multi-Charged Ionization Model, TRANSACTIONS OF THE JAPAN SOCIETY FOR AERONAUTICAL AND SPACE SCIENCES, AEROSPACE TECHNOLOGY JAPAN, Vol.10 iste28 (2012), pp.Pb_59-Pb_63. [2] Shiraishi, H., Fujiwara, T.: Thermal Nonequilibrium Analysis of 1-Dimensional Laser-supported Detonation Using a 2-Temperature Model, Proceedings of 22nd ISSW, July 18-23, 1999, pp.339-344. [3] Shiraishi, H.: Fundamental Properties of Non-equilibrium Laser-Supported Detonation Wave, Proceedings of 2nd Int. Symp. on Beamed Energy Propulsion, 2003, pp.68-79. [4] Shiraishi, H.: Numerical Analysis on Laser-Supported Plasma for Laser Propulsion Systems, The Journal of Space Technology and Science, 23 (2007), pp.20-29. [5] Wang, T.-S., Chen, Y.-S., Liu, J., Myrabo, L. N., and Mead, F. B., Jr.,: Advanced Performance Modeling of Experimental Laser Lightcraft, Journal of Propulsion and Power, 18 (2002), pp. 1129-1138. [6] Stuermer, E. and von Allmen, M.: Influence of laser-supported detonation wave on metal drilling with pulsed CO2 lasers, Journal of Applied Physics, 49 (1978), pp.5648-5654. [7] Numerical Analysis on Thermal Non-equilibrium and Multidimensional Laser-Supported Detonation Wave Propagating Through a Diatomic Gas, TRANSACTIONS OF THE JAPAN SOCIETY FOR AERONAUTICAL AND SPACE SCIENCES, SPACE TECHNOLOGY JAPAN, Vol. 7 (2009) , ists26 (ISTS Special Issue: Selected papers from the 26th International Symposium on Space Technology and Science), Pb_141-Pb_146, 2009.
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