Effect of Voltage transfer Curve on Pattern Formation in Dielectric Barrier Glow Discharge Xiaoxi Duan, Feng He, and Jiting Ouyang* School of science, Beijing Institute of Technology, Beijing 100081, China (*Author to whom correspondence should be addressed; [email protected]) Abstract: The voltage transfer curve reveals the important relationship between the voltage transfer in a pulsed discharge and the initial voltage across the gas gap in dielectric barrier glow discharge. Based on its bifurcation characteristic and considering the coupling term as a short-range activator and long-range inhibitor, a discrete one-component coupled-map model is developed to study the pattern formation in barrier discharge system. The stability of spatially structures and the bifurcation condition are investigated. The initial uniform discharge evolves to the eventual patterned discharge in one- and two- dimensional simulations. The evolution processes show that, the wavelike patterns firstly form near the boundary of the electrode and then occupy the whole space of the electrode. The results of this model are well consistent with the pervious experimental and fluid modeling results, and provide a new method to investigate the pattern formation in discharge systems. Keywords: Dielectric barrier discharge, coupled-map model, voltage transfer curve, lateral inhibition, pattern formation 1. Introduction Dielectric barrier discharge (DBD) is an excellent pattern forming system which shows interesting phenomena such as self-generated oscillation, stable pattern formation or chaotic behavior under different conditions [1, 2]. Especially in glow mode, the discharge develops generally synchronously in the whole space, with a single current pulse in each half period [2]. This allows one to achieve a favorable observation for the pattern formation in experiments. The voltage transfer curve is an important characteristic in glow DBD systems [3]. It is well used to define the stable operating conditions in plasma display panel (PDP). It has been verified that the distribution of the wall charge density is in good accordance with the discharge structure both in experiments and simulations [4]. Therefore a dynamic model taking the wall voltage as the sole parameter is helpful to simplify the discharge model. In this work, we employ a simple coupled-map model [5] based on the voltage transfer theory. The processes of the pattern formation in glow DBD systems are achieved from this model. 2. Description of the coupled-map model In this model, the spatio-temporal evolution of DBD is governed by the total voltage across the gas gap (i.e., the sum of the applied voltage and the wall voltage) at position x before each pulsed discharge, written as the general form of V i +1 (x) = f (V i (x);VS (x)) + c(x, V i ) . (1) Where Vi(x) denotes the voltage across the gas gap at position x before the ith breakdown. Reaction term f represents the ideal voltage transfer caused by voltage V(x) at an applied voltage VS(x). The function c is a coupling term that specifies the interaction of the voltage at different position x. The bold V refers to the gas gap voltage at the positions around x. To simplify, we consider a square-wave driven DBD system in which the voltage is a constant during any discharge pulse. Then, the reaction term f can be written as follows: f (V i (x);VS (x)) = 2VS (x) − V i (x) + g (V i (x)) . (2) Where g(Vi(x)) represents the function of the voltage transfer curve for DBD systems. It is defined as the change of the wall voltage during a discharge pulse at a given voltage. The typical voltage transfer curve for an infinity plate DBD system can be obtained by the fluid model. Figure 1 shows a voltage transfer curve for DBD in 3 KPa Ne (parallel electrodes structure, two 1 mm-wide dielectric layers are spaced by a 3 mm-wide gas gap, the relative permittivity of the dielectric layer is 10). This curve can be well fitted by the following polynomial expression V ≤ 150 ⎧0 ⎪ −4 3 2 ⎪-1.66 × 10 V +0.104V g (V ) = ⎨ 150 < V ≤ 280 . (3) − 18.9 V + 1050.5 ⎪ ⎪⎩V V > 280 voltage transfer g(V) (V) 300 250 voltage transfer Polynomial fitting curve 200 The coupling term c is derived from the fluid modeling of discharge in a non-uniform electric field, as shown in figure 2. This figure shows that at the positions where there are obvious voltage gradients along the dielectric surface, the voltage transfer deviates from the ideal value calculated from the voltage transfer curve. The coupling term c can be considered as a short-range activator and long-range inhibitor from the deviation curve. The edge area of the higher voltage gradient is the source of this effect. The modeling also indicates that the strength of the coupling term c(x) relates to the voltage difference closed to position x. Hence, the coupling term c can be described as follows: c ( x, V i ) = Δx ⎧⎪ ⎫⎪ (4.1) − i 2σ 2 γ 1 ∑ ⎨Vm (x + Δx)e [ a − V i ( x + Δx)]⎬, 0 ≤ Δx ≤ r ⎪ ⎩ ⎭⎪ 2 c ( x, V i ) = Δx ⎧⎪ ⎫⎪ − 2 −γ 2 ∑ ⎨Vm i ( x + Δx)e 2σ [V i ( x ) − b]⎬. Δx > r ⎪ ⎩ ⎭⎪ 2 100 50 150 200 V (V) 250 300 (4.2) Where Δx is the deviation vector from x, Δx is the distance between (x+Δx) and x. γ1 and γ2 are constant coefficients. A symmetrical exponential distribution is assumed and the parameter σ determines standard deviation. The amplitude Vm(x) is defined as the difference between the value of the voltage at position x and the average voltage at x Vm (x) = V (x) − V (x + Δx) . 150 0 100 the wall voltage before each pulsed discharge would be just equal to the applied voltage. (5) In equation (5) only the positive value is considered and we set Vm(x) = 0 when Vm(x) < 0. The last term ( a − V(x +Δx )) in function (4.1) is included Figure. 1 The voltage transfer curve of an infinite plate DBD system (obtained from 2-D fluid model in 3 KPa Ne), and its fitting curve. because the effect of the activate effect decrease when the voltage increase and is close to the completed voltage transfer value. While the factor (V (x) − b) in (4.2) indicates that the effect of the This curve indicates that the breakdown voltage of the DBD system is 150 V. When the total voltage V is above 280 V, the voltage transfer is complete and lateral inhibition is more obvious when the voltage is higher which could result from the transverse field becoming stronger due to the localized discharge. 200 Voltage (V) 160 120 80 40 0 0 8 16 24 Position (mm) 32 40 V: initial voltage across the gas gap g1(V): caculated voltage transfer from voltage transfer curve g2(V): simulated voltage transfer by fluid model g2(V)-g1(V) Figure 2. Voltage transfer from a non-uniform initial voltage distribution. 300 150 0 80 V S=152 V V S=160 V i=2 20 0 A B 150 -20 D C 200 250 300 i=4 Voltage (V) i+1 δV=V i=0 40 i -V (V) 60 initial voltage is constructed and out of the electrode boundary the voltage decreases exponentially. The disturbance to the uniformity status firstly forms at the edge region because the obvious voltage grads at these places provide a bigger value Vm(x). Due to the effect of lateral inhibition the voltage at the sites near the boundary decrease and a new boundary forms in the inner of the electrode. In the same mechanism the maximum of the voltage forms one by one towards the central of the electrode and finally the wavelike patterns form in the whole electrode. 350 i V (V) i=6 i=8 i = 10 -40 Figure 3. Typical phrase diagrams of equation (1) at VS = 152 V / VS = 160 V. The arrows indicate the direction of the discharge evolution at given voltages. The stability of this model is plotted at given applied voltages VS for a uniform system (i.e., the coupling term c is not considered in the variation term of δV), as shown in figure 3. One sees that for an applied voltage slightly higher or lower than the breakdown voltage, (e.g. VS = 152 V), the discharge shows a bistability property and the points “A” and “D” are the two stable states for the DBD. The characteristic is well discussed in Ref [3]. For a higher voltage (e.g. VS = 160 V), there is only one stable point (i.e., the point “D”) and the variation of the voltage δV is always above zero. Under this condition, the patterned structures, once formed, must satisfy the bifurcation condition at some positions δ V + c(x,V i ) ≤ 0 . (6) 3. Results and discussion Based on the model described above, the evolution of the patterned DBD can be observed. The typical evolution of a 1D pattern is shown in figure 4. In these results, a finite-width electrode with a uniform i = 12 -r r i = 14 Figure 4. Time evolution of the patterned discharge in a onedimensional model. Parameters: γ1=2.07×10-4, γ2=1.33×10-3, a=480, r=3, σ=5, b=150. When we decrease the effect of the lateral inhibition (i.e., reduce the value of σ or γ2), different stable states of the DBD can be observed,as shown in figure 5. One can see that strong lateral inhibition is important for the pattern formation because the coupling term has a low absolute value at the inhibited positions and the bifurcation condition is easy to be satisfied. Furthermore, the places near the boundary are more unstable than the inner places. It results from that the system has a lower value of δV from the phrase diagram during the first few breakdowns. It is helpful to satisfy the bifurcation condition at the positions near the boundary of the electrode where the initial voltage gradient forms. The evolution of the pattern in the 2D model under the same condition as in figure 4 (only the radius of the electrode is set to a half value) is achieved, as shown in figure 6. One sees that the initial uniformity transits to the concentric ring structure after about 10 breakdowns and then the rings become unstable and some spots appear. Eventually, the stable hexagonal patterns are achieved. Comparing with the previous results obtained from experiments and fluid modeling, the discrete onecomponent model shows well-matched spatiotemporal evolution of the patterned discharge. Although in a real DBD system, the discharge development are much more complicated and many input parameters such as the gases, the pressure, and the characteristics of the power source must be considered, the process of the discharge and effect of all the parameters can be involved in our model in a phenomenological way. This simplified model will be helpful to discuss the formation and behavior of the patterns. 4. Conclusions Figure 5. Stable structures of the DBD in a one-dimensional model for (a) different γ2, σ = 5.0 and (b) different σ, γ2 =1.33× 10-3. The other parameters are the same as in figure 4. A discrete one-component model based on the voltage transfer curve and the effect of lateral inhibition in a glow DBD system is developed. The bifurcation condition for the pattern formation is discussed from the phase diagram. The one- and two- dimensional pattern evolution from the initial uniform voltage distribution are observed. The wavelike patterns evolve from the edge of the electrode to the center. During this process, the strong effect of the lateral inhibition plays a major role in pattern formation. Acknowledgement This work was supported in part by the National Science Foundation of China under Grant No. 10875010. References Figure 6. Time evolution of the patterned DBD in a twodimensional model. The time t at which the figures are taken are as follows: (a) i = 10; (b) i = 20; (c) i = 40; (d) i = 60. The evolution of the pattern structures in our model has the similar processes as the reaction-diffusion systems [6]. But differently, the voltage across the gas gap can be considered playing the both roles of activator and inhibitor. [1] H. G. Purwins, H. U. Bodeker, and S. Amiranashvili, Adv. Phys. 59, 485 (2010) [2] X. X. Duan, J. T. Ouyang, X. F. Zhao, and F. He, Phys. Rev. E 80, 016202 (2009) [3] J. P. Boeuf, J. Phys. D: Appl. Phys. 36, R53 (2003) [4] L. Stollenwerk, S. Amiranashvili, J. P. Boeuf, and H. G. Purwins, Phys. Rev. Lett. 96, 255001 (2006) [5] G. L. Oppo and R. Kapral, Phys. Rev. A 33, 4219 (1986) [6] M. C. Cross and P. C. Hohenberg, Rev. Mod. Phys. 65, 851 (1993)
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