22nd International Symposium on Plasma Chemistry July 5-10, 2015; Antwerp, Belgium Shadowgraphy investigations of a filamentary atmospheric plasma jet M. Teodorescu, E.R. Ionita and G. Dinescu2 National Institute for Laser, Plasma and Radiation Physics, Magurele, PO Box Mg36, Bucharest, 077125, Romania Abstract: A long and thin filamentary plasma jet was generated at atmospheric pressure via radiofrequency power. The behaviour of the plasma jet was investigated by means of shadowgraphy, at different gas flow rates and applied RF powers, in order to determine the operation domains for which the flow is stable. The turbulent behaviour was also investigated and its dependence with the applied power and gas flow. Keywords: atmospheric pressure, filamentary plasma jet, shadowgraphy 1.Introduction Low temperature atmospheric pressure plasma jets are a practical means of processing materials that require either controlled atmosphere and low treatment temperatures or a large surface area treatment. The complex shape of some substrates represents a problem that can be solved with localized treatments employing long and thin plasma jets. Usually this kind of jets can be generated in Helium but the treatment temperatures may be too high, and thus damage the substrate (like for example for polymeric foils). The requirements of such specific plasma jets can be resolved partially via the device described in the following presented work. The results here focus on the gas interaction with the ambient air and can lead to conclusions regarding the optimum discharge parameters and nozzle-to-substrate distance for direct use in treatment procedures. 2.Experimental The investigated plasma source consists of a glass tube of 6.5mm outer diameter and 3.5mm inner diameter. The discharge is initiated and maintained inside the tube, while the plasma column exits the glass tube as a plasma jet. electrode is absent altogether. The discharge configuration uses a single-electrode geometry, placed on the outside of the glass tube, and thus the tube itself acts as a dielectric barrier [1]. The power to the discharge is supplied via a computer controlled AD-TEC AX-600 III radiofrequency generator (13.56MHz) and an automatic matching network. An additional movable electrode is used for initiating the discharge by placing it inside the glass tube near the RF electrode. After ignition it is retracted from the tube. The experiments were performed in open atmosphere using argon as the discharge gas. The experimental parameters are as follows: forwarded RF power in the range of 50-130W and argon gas flow in the range of 500 – 3000sccm. In order to investigate the dependence of the filament’s length with the gas flow, a simple yet effective shadowgraphy investigation setup was designed, using a He-Ne laser, a beam expander and an imaging lens (Figure 2). The lens has a 500mm focal length and the Focusing Laser beam Expanding Laser beam He-Ne Laser Beam expander Collimating lens Plasma source DSLR Camera Fig. 2. Setup for shadowgraphy measurements Fig. 1. Image of the filamentary plasma jet. Discharge parameters: RF power- 100W, 3000sccm Argon 5.0. The plasma jet itself has a dual nature: a filamentary discharge is surrounded by a diffuse one (Figure 1). The jet can have lengths in the range of 30 to 60mm, depending on the operating parameters. The aluminium RF electrode is of a cylindrical shape, while the ground P-I-2-13 diameter of the lens is 65mm, such that it can cover the entire filament and also a large part of the outward gas flow. The plasma jet was placed immediately after the lens, and at 700mm a DSLR camera without the objective was used to image the object. Due to the designed setup, the RAW images were of low contrast, so a digital subtract method was used in order to enhance the final data. The RAW images were all corrected using an initial no-plasma source image (in which only the laserilluminated field of view was imaged) which was 1 afterwards subtracted from the data, leaving only the gas flow images. 3.Results and discussion The difference between the no-plasma laminar flow and plasma-on images are shown in Figure 2. There is also a normal image of the mono-filament at the same scale, showing that the turbulence zone of the gas flow actually starts about half-way from the jet outwards. This observed that the turbulence start point gets closer to the nozzle with the increase of the gas flow (Figure 3). The power increase also plays a major role in the turbulence evolution in the flow range of 1500-3500 sccm. Increasing the RF power also moves the turbulence starting point towards the nozzle but this is less obvious then for the gas flow change (Fig. 4). Also the stability of the discharge filament deceases with the power increase. This is important, again, for the precise localization in the case of substrate treatments. However, it seems that except for the higher RF powers and gas flows, the two parameters do not actually influence greatly the stability of the monofilament, as in the flow domain of 500-1500sccm and throughout the entire range of the applied power values, the filamentary discharge remains largely unaffected. 48 36 24 12 Distance from nozzle [mm] 60 0 0W Fig. 2. Images showing shadowgraphy and normal imaging aspects of the filamentary plasma: Leftgas flow without discharge; Center-gas flow with discharge; Right- discharge filament in normal operation. Operating parameters: gas flow 1800sccm Ar, RF power 130W. 70W 80W 90W 100W ] [W er ow P 110W 120W 130W 500 1000 1500 2000 2500 3000 3500 Gas flow [sccm] Fig. 4. Turbulence dependence with the gas flow and the forwarded RF power. Fig. 3. Turbulence evolution with the gas flow increase in NO-plasma mode (first row) and with plasma (second row) at 130W forwarded RF power. sequence shows just how important this type of investigation is for determining the optimum distance from the glass tube end at which a substrate can be placed in order to get a uniform treatment by using the laminar flow characteristics of the discharge. The turbulence start point was investigated for different RF forwarded powers and different gas flow rates. It was 2 4.Conclusions One of the advantages of our device compared to other plasma sources is the possibility to generate a plasma jet with lengths of more than 40mm, and also the narrowness of the discharge column, which can be very useful for fundamental studies or highly localized plasma treatments. The shadowgraphy measurements showed that despite the apparent stable discharge aspect, the gas turbulence is present on at least half of the plasma jet. The starting point of the turbulence shift with the two main parameters, getting closer to the nozzle with the power increase, and also with the increase of the gas flow rate. The measurements allow for the optimization of the treatment setup in the case where a laminar gas flow is needed. 5.Acknowledgements: The financial support of the Ministry of National Education National Authority for Scientific Research Financing contract: PN-II-RU-PD-2012-3-0583 44/30.04.2013 is gratefully acknowledged. 6.References [1] M. Teodorescu, M. Bazavan, E. R. Ionita, G. Dinescu, Plasma Sources Science and Technology, Submitted. P-I-2-13
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