SPECIAL FEATURES IN RADIOGRAPHY ACCESSED BY 3D MONTE CARLO MODEL Gerd-RUdiger Tillack and Carsten Bellon Federal Institute for Materials Research and Testing (BAM), Unter den Eichen 87, 12205 Berlin, Germany ABSTRACT. Standard radiography simulators are based on the attenuation law complemented by built-up-factors (BUF) to describe the interaction of radiation with material. The assumption of BUF implies that scattered radiation reduces only the contrast in radiographic images but does not image object structures itself. This simplification holds for a wide range of applications like weld inspection as known from practical experience. But only a detailed description of the different underlying interaction mechanisms is capable to explain effects like mottling or others that every radiographer has experienced in practice. The application of the N-Particle Monte Carlo code MCNP is capable to handle primary and secondary interaction mechanisms contributing to the image formation process like photon interactions (absorption, incoherent and coherent scattering including electron-binding effects, pair production) and electron interactions (electron tracing including X-Ray fluorescence and Bremsstrahlung production). Additionally it opens up possibilities like the separation of influencing factors and the understanding of the functioning of intensifying screen used in film radiography. The paper intends to discuss the opportunities in applying the Monte Carlo method to investigate special features in radiography in terms of selected examples. It is important to note that the use of Monte Carlo methods is a laboratory type of technique for basic investigations because of the enormous computing power that is needed. For in-field applications such as for inspection planing simplified models are of much greater importance and increasingly in use. INTRODUCTION In recent years the availability of computing power on PC-platforms allows the modeling of complex processes and physics that control the X-ray image formation. This development in computer hardware allows the implementation of NDE measurement models that are capable to predict the signals seen in NDE inspections and that can be used to quantitatively study the effects of various parameters on those signals. The link between NDE models and CAD provides the ability to quantitatively evaluate complex inspection procedures. Depending on the formulated inspection problem or the influencing factor that should be accessed by modeling an appropriate physical model has to be chosen to handle the underlying interaction mechanisms. Scattered radiation generated by a specimen can significantly influence the flaw sensitivity by reducing the relative contrast of the flaw indication [1]. This statement holds if the scattered radiation produces a uniform intensity distribution in the film or detector plane, i.e. it is non-image forming while contributing to the radiographic projection. The CP657, Review of Quantitative Nondestructive Evaluation Vol. 22, ed. by D. O. Thompson and D. E. Chimenti © 2003 American Institute of Physics 0-7354-0117-9/03/S20.00 537 introduction of built-up factors yields a sufficient description of the reduction of the relative contrast in the radiographic image [1]. Accordingly radiography simulators are widely used that are based on the attenuation law to describe the primary radiation and a BUF model to count for scattered radiation. These models have a wide application range as known from practice. But if the specimen covers a large range of material thickness (e.g. castings) this simplification can not been used any more because the distribution of the scattered radiation becomes non-uniform, i.e. it is influenced by the object structure itself. In this case the underlying physical mechanisms have to be treated as an X-ray or photon transport problem based on a Boltzmann type equation. There are several attempts known to solve this problem for X-ray NDE applications such as moment approximation methods [2,3], solution of the integral transport equation [4,5], and the Monte Carlo method [6-8]. The Monte Carlo approach is capable to count for primary and secondary interaction mechanisms contributing to the image formation process like photon interactions (absorption, incoherent and coherent scattering including electron-binding effects, pair production) and electron interactions (electron tracing including X-Ray fluorescence and Bremsstrahlung production). It is a powerful tool to separate different influencing factors and to understand special features of detector systems, e.g. the functioning of intensifying screen used in film radiography. On the other hand this approach is restricted applicable due to the required computing time or the need of using parallel computing capabilities. This paper intends to discuss exemplary the use of standard Monte Carlo packages like MCNP [9] to derive fast empirical models counting for the contribution of scattered radiation and to analyze the impact of lead screen on the image formation in industrial radiography. PHYSICAL BACKGROUND The Monte Carlo code MCNP [9] used for the investigations presented here includes neutron, photon, and electron interactions. For the studies elaborated here photon and electron interactions have to be considered as shown in Fig. 1. The physics treatment for the photon transport includes the photoelectric effect, coherent and Compton scattering, and pair production. In detail it accounts for fluorescent photons after photoelectric absorption. Additionally form factors are used with coherent and incoherent scattering to account for electron binding effects. The photoelectric effect consists of the absorption of the incident photon with energy £, with the consequent emission of fluorescent photons and the ejection or excitation of an orbital electron of binding energy e<E, giving the electron a kinetic energy of E-e. Up to two fluorescent photons are emitted. Only emitted photons with energy greater than 1 keV are considered. Each fluorescent photon born is assumed to be emitted isotropically and transported. To model Compton scattering the angle 6 of scattering, the new energy £" of the photon, and the recoil kinetic energy of the Compton electron E-E' are determined. The differential cross section is assumed as product of the Klein-Nishina cross section and the scattering form factor counting for electron binding effects. The coherent scattering involves no energy loss. It is only a photon process that cannot produce electrons for further transport. Only the scattering angle 6 is computed. The differential cross section includes the form factor to modify the energy-dependent Thompson cross section. This investigation includes only photons with energy smaller 1 MeV such that pair production does not occur. 538 incident photon scattering Rayleigh scattering Compton electron scattered photon electron escape photon escape I photoelectric absorption incident photon scattering I photoelectric absorption photo electron X-ray fluorescence production of conduction band electrons phonons photon escape light photons electron escape FIGURE 1. Photon and electron interaction mechanisms. The transport of electrons or other charged particles is fundamentally different from the transport of uncharged particles like neutrons or photons. The long-range Coulomb force, resulting in a large number of possible interactions, dominates the transport of the electrons. The energy loss of the electron by multiple interaction is considered such as the production of Bremsstrahlung, K-shell electron impact ionization, Auger transition, and scattering of an electron by an electron. The trace of the electrons is only used for the investigation of the lead screens. APPLICATION OF MONTE CARLO METHOD Contribution of Scattered Radiation to the Image Formation The contribution of scattered radiation to the image formation is discussed here in terms of two examples. The first example (see Fig. 2) shows the distribution of scattered 539 FIGURE 2. Scattered photon flux for (a) steel and (b) Aluminum plate (thickness 10 mm, 80 keV photons). radiation for a plate of 100x100 mm with a thickness of 10 mm made of steel (Fig. 2a) and Aluminum (Fig. 2b) using a monochromatic source with 80 keV. In case of steel the mean free path of the photons is 7.1 mm, i.e. smaller than the thickness of the plate. It is assumed that the main contribution to a point in the detector plane is given by photons being scattered in within a half sphere of radius equal to the mean free path / of the photons. As a result three regions can be distinguished. If an arbitrary position is chosen with a distance larger than / from the edge of the plate the integration volume is constant yielding a uniform distribution of the scattered photons in this region. If coming closer to the edge the corresponding integration volume is reduced up to a factor of 4 yielding a reduction of the scattered flux. For positions outside the area covered by the plate the morphology of the problem is changed. Here angle-selective contributions to the scattered scalar flux are found. The smaller the angle of the photon path relative to the edge of the plate the more it contributes to the flux in the film plane because the total path length of the photon through the material is decreased. This results in an increase of the flux that is overlaid by the divergence of the beam yielding a maximum as shown in Fig. 2a. If the material is changed to Aluminum the mean free path of the photons is 21.7 mm, i.e. / is larger than the thickness of the plate. In this case no increase of the photon flux is found for positions outside the plate because the integration volume does not change here. Here only a decrease of the flux is found due to beam divergence (see Fig. 2b). The second example investigates the distribution of scattered radiation in case of projection radiography for pipes. Fig. 3 shows the geometrical setup together with two profiles of the scattering contribution for two different wall thicknesses. As seen in the figure, the Lorentz function fits the scattered distribution over a range of about two orders of magnitude. This function can be used as an empirical model to describe the contribution of scattered radiation for pipes. The Monte Carlo calculations are used to determine the parameters a and b of the Lorentz function over the expected application range of this projection technique. By introducing this approximation to standard X-ray simulators instead of the simple BUF model, the accuracy of these simulators is considerably increased without increase of calculation expenses. A comparison of the BUF model and the Lorentz approximation is shown in Fig. 4. The total photon flux is given by the primary radiation calculated from the attenuation law plus the contribution of scattered radiation. 540 (b) (a) io-9 io-1 -200 ——H 0 position [mm] 400 FIGURE 3. Geometrical setup for projection radiography (a) and profile of scattered radiation in the detector plane (b) together with Lorentz fit. 2.5 >> 2.0 1 •9 <d 0 ^.^ —— ^ /^/^ !'5 U 1.0 "^NTX N .......... I / y BUF \\ l^^^ 0.5 0.0 . — —- Lorentz approximation ^—— Built up Factor approximation 3.0 Lorentzfit primary radiation -100 -50 0 50 100 position [mm] FIGURE 4. Comparison BUF and empirical scattering model. Heavy Metal Intensifying Screens Radiographic screens are employed to utilize more fully the X- or gamma ray energy reaching the film. When an X- or gamma ray beam strikes a film, usually less than one percent of the energy is absorbed. Since the formation of the radiographic image is primarily governed by the absorbed radiation, more than 99 percent of the available energy in the beam performs no useful photographic work. Any means of utilizing this unused energy without complicating the technical procedure is highly desirably. Two types of radiographic screens are in use to achieve this goal: lead and fluorescence screen. For radiography in the range 150 to 400 kV, lead screens in direct contact with both sides of the film are used. Lead screen has three principle effects: (i) it increases the photographic action on the film mainly by reason of the electrons emitted and partly by the secondary radiation generated in the lead (see Fig. 5), (ii) it absorbs the longer wavelength scattered radiation more 541 incident photons photoelectric f absorption ft film FIGURE 5. Principle of intensification by lead screens. than the primary, and (Hi) it intensifies the primary radiation more than the scattered radiation. The aim of this investigation was to understand the intensification effect of lead screens because of the production of electrons and to study the influence of the screen thickness on the intensifying factor. Additionally the effect of secondary radiation produced in the screen is evaluated. As shown in Fig. 5, two interaction mechanisms are to be considered here that produce electrons, namely the photoelectric absorption and the Compton scattering. If these electrons reach the film emulsion they will be absorbed and contribute to the formation of the latent image. The secondary radiation, i.e. the Compton photon and the X-ray fluorescence radiation, also reaches the film and contributes to the latent image. But again more than 99 percent of its energy stays unused. Fig. 6 gives the distribution of scattered photons and fluorescence photon for a monochromatic photon source of 310 keV producing a pencil beam. Here lead screens of 0.027 and 0.100 mm thickness are investigated as commonly used in Europe. Comparing the photon flux reaching the film it turn out that the fluorescence flux is about one order of magnitude smaller than the Compton scattered flux. Additionally these results can be used to determine the contribution of scattered photons to the inner unsharpness, i.e. to determine a point spread function. As the thickness of the screen increases the more scattering occurs and the distribution becomes wider. The distribution of electrons produced in the lead screen is shown in Fig. 7. The width of the electron distribution is not very much influenced by the thickness of the 2.5 310 keV monochromatic X-i needle beam I 310 keV monochromatic X-rays needle beam 1.0 t 0.0 6** -0.10 -0.05 0.00 position [mm] 0.05 0.10 0.10 FIGURE 6. Distribution of scattered (left) and fluorescence (right) photons for monochromatic source and pencil beam. 542 310 keV monochromatic X-rays needle beam 0.027 mm Pb 0.100 mmPb 10 T3 5 -0.05 0.00 position [mm] 0.05 0.10 FIGURE 7. Distribution of electron flux in the film plane. 30 1.40 100 keV monochromatic X-rays needle beam 7cd 300 keV monochromatic X-rays needle beam 25 T? 1-35 1 20 1.30 15 1.25 13 1 10 0.00 0.02 0.04 0.060.08 1.20'— 0.00 0.05 0.10 0.15 thickness of lead screen [mm] thickness of lead screen [mm] FIGURE 8. Total electron yield as function of screen thickness for 100 keV (left) and 300 keV (right) incident photons. screen. The total electron yield can be used as a measure for the intensification. A series of calculation have been carried out to study the influence of the screen thickness on the total electron yield for various incident photon energies. As an example the results for 100 keV and 300 keV incident photons are given in Fig. 8. A clear maximum of the total electron yield can be found. This maximum is shifted to greater screen thicknesses as the energy of the photons is increased. Additionally it can be seen from the plots, that the form of the curve is changed. With increasing photon energy the tail of the distribution becomes longer and does not decrease as fast as for smaller energies. The reason for this behavior is the increased kinetic energy of the produced electrons such that their mean free path in the screen material is also increased. The conclusion can be drawn that for higher energy photons the correct choice of the optimal screen thickness is not that important as for lower energy photons. If the total electron yield is taken as a measure for the effect of intensification its maximum can be chosen as optimal screen thickness. The results are plotted in Fig. 9. As a result follows, that with increasing photon energy thicker screens are preferable as it is suggested by the European standards for film radiography. 543 0.25 monochromatic X-rays needle beam 0.20 0.15 0.10 0.05 0.00 0 150 300 450 600 photon energy [keV] FIGURE 9. Screen thickness as function of incident photon energy. CONCLUSIONS State-of-the-art radiography simulators have a broad application range. These simulators are based on the attenuation law to describe the primary radiation. The BUF is used to simulate the contribution of the scattered radiation yielding a reduction of the radiographic contrast. Empirical detector models based on transfer functions are implemented to describe the recording of the radiation in the film or detector plane. To handle inner unsharpeness and detector noise a point spread function and Gaussian distributed white noise is introduced. In cases where a detailed description of the radiation physics is required, Monte Carlo packages can be applied. These models include the interaction mechanisms for photons and electrons. With the help of Monte Carlo models complex problems can be simulated like the intensifying effect of heavy metal screens. On the other hand these models can be used to derive empirical models for the contribution of scattered radiation to the image forming process to increase the accuracy of simplified radiographic simulators. REFERENCES 1. Halmshaw, R., Industrial Radiology, Chapman & Hall, London, 1995 2. Tillack, G.-R., Bellon, C, and Nockemann, C., in Review of Progress in QNDE9 Vol. 14, eds. D. O. Thompson and D. E. Chimenti, Plenum Press, New York, 1995, pp. 665-672 3. Tillack, G.-R., Artemiev, V. M., and Naumov, A. O., JNDE 20 4, 153 (2001) 4. Inane, F. and Gray, J. N., in Review of Progress in QNDE, Vol. 10, eds. D. O. Thompson and D. E. Chimenti, Plenum Press, New York, 1991, pp. 355-362 5. Inane, F. and Gray, J.N., Applied Radiation and Isotopes 48 10-12, 1299(1997) 6. Bell, Z. W., in Review of Proggress in QNDE, Vol. 10, eds. D. O. Thompson and D. E. Chimenti, Plenum Press, New York, 1991, pp. 347-353 7. Aerts, W., De Meester, J. R., and Bollen, R., Mat. Eval. 40 9, 1071 (1982) 8. 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