Bunched Beam Injection in a Plasma Accelerator S. Ya. Tochitsky1, P. Musumeci2, C. E. Clayton1, C. Pellegrini2, J.B. Rosenzweig2 and C. Joshi1 Department of Electrical Engineering, 2Department of Physics, University of California at Los Angeles, 405 Hilgard avenue, Los Angeles, CA 90025 Abstract An experiment on phase-locked injection of ~ 100 fs electron bunches in a plasma beat wave accelerator is presented. We consider using an IFEL microbunching technique to produce ultrashort electron bunches prebunched at the exact wavelength of the plasma wave 340 Jim (~lTHz). It is proposed to generate 100 MW of 1 THz radiation by difference frequency generation in a nonlinear crystal, mixing the same two CC>2 lines as used to drive the plasma accelerator. INTRODUCTION Laser -Plasma acceleration of particles is utilizing a relativistic plasma wave driven by a high-power laser beam. Plasma wave allows to couple energy of a transverse electromagnetic wave of laser field into a longitudinal electric field of the wave, thus making acceleration possible. The acceleration gradient has reached in experiments values from 3 to 100 GeV/m for the plasma density (no) 1016 cm"3 and 1019 cm"3, respectively [1]. So far all schemes of high gradient acceleration have shown 100 % energy spread. This is physically due to the experimental difficulties related to the generation and the injection of an electron beam in the high gradient accelerating field wave with a typical period of 10-300 jim. It is obvious that if the injected electron beam samples all the phases of the accelerating field, the energy spectrum at the output will be continuous. The goal of second generation experiments is to reduce the energy spread to make an electron beam produced by a plasma accelerator usable for different applications. There are two principle approaches to tackle this problem: optical injection of electrons in the plasma wave and injection of prebunched electrons in a plasma accelerator. For a 1019 cm"3 plasma density, which corresponds to a plasma wavelength 10 jim, perhaps the only way for a phased injection is production and injection of ultrashort electron bunches using different all-optical injection schemes: CP647, Advanced Accelerator Concepts: Tenth Workshop, edited by C. E. Clayton and P. Muggli © 2002 American Institute of Physics 0-7354-0102-0/02/$19.00 786 LILAC, LIP A, colliding beams (see these proceedings for more information). However, forlower plasma densities and, therefore, longer plasma wavelength it becomes possible to produce a high quality electron bunch (bunches) with a duration short compared to the plasma wavelength. Injection of prebunched electrons that are synchronized to the high gradient electric field wave is commonly called phase locking. Several methods have been considered for injection of a phase-locked ebeam in a plasma accelerating structure [2]. However this has not yet been experimentally demonstrated. In this paper we describe an experiment on phase-locked injection of ~ 100 fs electron bunches in a plasma beat wave accelerator proposed at Neptune Laboratory (UCLA). It is suggested to use an IFEL technique to produce ultrashort electron bunches prebunched at the exact wavelength of the plasma wave. For Neptune plasma accelerator the plasma wavelength is 340 jim (~lTHz). We propose to generate 100 MW of 1 THz radiation by difference frequency generation (DFG) in a nonlinear crystal, mixing two CO2 lines. Co-propagating the radiation with the electron beam inside a short undulator achieves the bunching at the required wavelength. Moreover, because the electromagnetic radiation is generated from the same laser that excites the relativistic plasma wave, phase-locking could be achieved. In the first part of the paper we describe the scheme and report preliminary experimental results on generation of THz radiation using noncollinear DFG in GaAs. Then we present results of modelling IFEL microbunching and address a beam loading problem. EXPERIMENT ON INJECTION OF PREBUNCHED ELECTRONS The Neptune Laboratory at UCLA is being used to explore advanced accelerator concepts including Plasma Beat Wave Acceleration (PBWA) of electrons. Here a plasma beatwave with acceleration gradient 1-3 GeV/m is driven by a 100 ps twowavelength TW CO2 laser pulse at 10.6 and lO.Sjim [3]. For PBWA, electrons from a photoinjector are injected in a plasma accelerating structure. The injected electron beam comes from an RF gun followed by a linac which can produce up to 0.5 nC in several ps at 12 MeV [4]. At present the PBWA experiment is operating and a long (>340 jim) electron bunch is injected in the plasma structure and accelerated with 100 % energy spread. Production of the monoenergetic beam require a bunch length of about 40 jim. In Fig.l we show a proposed scheme for phase-locked injection of electrons in the plasma beat wave accelerator. As shown in the picture, a high-power CO2 laser beam is focused by a F/5-F/18 optic at the interaction point (IP) and drives the relativistic plasma beatwave. A small fraction (~ 4%) of two-wavelength CO2 laser radiation is splitted by a NaCl beamsplitter, and then sent onto a nonlinear crystal. Here, by difference frequency generation, as discussed in the next section of this paper, we should generate up to 100 MW of 1 THz radiation. This 340 jim wave originates from the mixing of the same two wavelengths that drive the plasma beat wave, so that it 787 Electron Spectrometer has a well-defined phase relationship with the accelerating structure. The THz beam is made collinear with the electron beam and is sent through a planar undulator using a mirror with a hole. This off-axis off-axis parabolic mirror has also the function function of focusing THz radiation to a spot size of 7 mm located at the end of a 0.5 m long undulator. As IP NaCl BS µm + 10.3 |im µm 800 GW, 10.6 |im Final OAP f’=100 cm DFG OAP Focus f’=30cm =30cm Triplet THz THz IFEL buncher 100 fs e-bunches 1 THz, 340 µm Plasma wave From Neptune Laser 100 MW, 340 µm LINAC RF Gun 5 ps e-bunch, 12 12 MeV 1 THz, 340 µm urn Electromagnetic wave FIGURE 1. Experimental layout for THz Inverse Free Electron Laser microbunching. aresult of the IFEL interaction the electron beam propogating through the undulator magnetic field is microbunched on the scale of 340 µm; jim; then it is focused with the final focus triplet at the IP and finally it is accelerated by the relativistc plasma final beatwave. Absolute phase between electrons and the plasma wave can be adjusted simply by using a delay line. The distance between the end of the undulator and the possibility that debunching debunching effects, effects, taking place place in the the IP is up to 2 m. There is a possibility transport between the THz prebuncher and the plasma, will cause bunch lengthening. This issue is ought to be studied experimentally. Note that in the successful successful STELLA µm), experiment where tolerances are tighter because of the shorter wavelength (10 jim), the IFEL accelerator was located 2.3 m downstream of the IFEL prebuncher [5]. HIGH-POWER SOURCE OF THz RADIATION powerful source of optical The key element of a laser-driven IFEL prebuncher is a powerful difference frequency frequency mixing process in a nonlinear radiation. We propose to use difference crystal to produce high-power driving THz radiation (>100 MW) for the IFEL buncher. It is known that low DFG efficiency efficiency is a serious problem for the FIR 788 spectral range. The highest FIR power generated by now using this method is a few kW [6]. At the same time 100 ps, two-wavelength €62 laser pulses from the Neptune Lab system are naturally very well suited for producing high-power FIR radiation. Nonlinear frequency conversion efficiency increases significantly for short pulses: first owing to the power increase and second, this power can be coupled into a crystal because of the higher surface damage threshold for shorter pulses. According to the Manley-Rowe relations, the maximum power conversion efficiency can reach 3% for TW 10 (impulses. Three methods to generate high-power 340 jim radiation by CO 2 laser difference frequency mixing in a nonlinear crystal have been considered. They are: standard birefringent phase matching, quasi-phase matching with periodic structures, and noncollinear phase matching in isotropic materials. A comparative analysis shown that the later has the highest potential for FIR DFG [7]. Noncollinear mixing of two laser beams is possible in any crystal which possesses anomalous dispersion between the incident CO2 laser radiation and FIR difference frequency radiation. Zernike [8] and Aggarwal et al. [9] have demonstrated noncollinear mixing of two €62 laser beams in liquid helium cooled InSb and GaAs samples. Several reasons make GaAs a good candidate for generation of high-power 340 jim radiation. It has a relatively high value for the electro-optic nonlinear coefficient d=43 pm/V. GaAs with high resistivity (> 108 Qcm) is transparent in the FIR beyond 200 jim at room temperature as well as in the 10 jim region of the €62 laser [10]. High-quality, single crystals with a diameter of 15 cm and length up to 10 cm are commercially available. The expected surface damage threshold could reach 10 GW/cm2 for 100 ps €62 laser pulses. For noncollinear phase-matched mixing of two laser lines of frequencies GOi and 0)2 (coi>co2) to generate the difference-frequency radiation at 0)3, the conditions of photon energy and momentum conservation require that co3 =co1 -69 2 ;k 3 = k i - k 2 (i) where ki, k2 and ks are the respective vectors for radiation of frequencies GDI (10.3 jim), 0)2 (10.6 jim), 005 (340 jim). Fig 2a. shows the direction of propagation of the incident beams and that of the difference frequency radiation inside the crystal. Refractive indices for insulating GaAs are ni~n2=3.28 at 10 jim region, and n3=3.61 at 340 jim [10]. According to Aggarwal et al. [9], for these values of refractive index we obtain 0=0.72° and 9=21.64°. The corresponding external phase-matching angle is 2.38 degrees. The angle at which FIR radiation propagates inside the crystal is greater than the critical angle for total internal reflection. Therefore, as it shown in Fig.2b, the output face of the GaAs crystal has to be cut at 21 degrees to release the newborn radiation. Preliminary measurements of the DFG efficiency were done with a 3 cm long sample of (111) oriented GaAs. The measurements were performed with a two-wavelength output of a CO2 master oscillator which provided 50 mJ in a 200 ns pulse. Fig. 2b 789 presents a schematic diagram of the experiment. The laser beam was compressed to a spot size of 1 mm in order to increase the conversion efficiency. efficiency. By adjusting adjusting the distance between a ZnSe beamsplitter and a mirror we set the angle necessary for ω1 ϕ Θ ω2 ω3 a 10.3 +10.6 µm Filter llay Go l Cel GaAs b FIGURE 2. Schematic wave vector diagram for noncollinear noncollinear DFG DFG (a) (a) and optical scheme of an FIGURE FIR DFG DFG in GaAs(b). experimental set up for FIR produced was detected by a Gollay cell. The interaction length is limited by the length over which two crossed beams are overlapped and, according to calculations, was approximately 12 mm. We have observed FIR pulses with peak output power P340≈100 mW mW at peak input power Pio.3~20 P10.3≈20 kW and Pio.6~80 P10.6≈80 kW. It corresponds to a P340-100 -6 6 10 efficiency value. In order to compare the experimentally observed 10~ conversion efficiency from theory we used the following formula: FIR power output with that expected from 0.5 PFIR 2 µ 0 4d eff 2 ω FIR 2 P10.3 P10.6 Leff T1 T2 T3 − αL e = 0.5 S ε 0 n1n 2 n 3c2 (2) the area of the input beams, TI, T1, T2 T2 and TS T3 are the single surface where S denotes the transmission coefficients coefficients at the the frequencies frequencies GDI, ω1, 002, ω2, and 003 ω3 and aα is the absorption =50 coefficient of FIR radiation in GaAs. Theory predicts P coefficient Ps4o ff=50 340 =212 mW using deeff the only available in literature absorption coefficient coefficient for THz radiation radiation at pm/V and the room temperature of 0.2 cm" cm-11 . This is in a reasonable agreement with the observed value (uknown absorption may be a possible reason for this discrepancy), and allows us to estimate possible FIR power for amplified amplified pulses. Calculations have shown (see the pump intensity of 2-4 GW/cm22 and LLeeff =2.5 cm one can expect Fig. 3) that with the ff=2.5 the conversion efficiency efficiency up to 4xlO~ 4x10-33 . It means that for 100 ps ps pump pump growth of the 790 pulses the 100 100 MW level of power could be achieved for a beam diameter of 5 cm (82 10 MW/cm of the THz power density). 10 5 110" 0 4 11004 Projected wi h 100 Proje cted power with 100 ps ps pulses puls es L=2.5 L=2.5 cm 11 0 0 0 2 jfi FIR Power, kW/cm M o + ^/ S j^~———— 1100 00 10 0) I 1 0. 0.1 / 0.01 r with 200 200 ns n i pulses perimental power pov er with pulses ./* Experimental Ex L=1.2 L: ;1.2 cm 0 .001 1 11 0 11 0 0 11000 000 4 1100 4 22 Pump Pump Power, Power, MW/cm MW/cm FIGURE 3. Measured and calculated power at 340 340 µm Jim as as aa function function of of pump pump intensity. intensity. Due to high nonlinearity of GaAs interaction of a 10 10 µm jim beam beam of of GW GW power power with with the nonlinear material may result in spectral broadening, amplitude modulation, etc. [11] which could limit the allowed pump power besides the damage threshold. Moreover frequency mixing of different spectral components of a broadened pump pulse can cause generation of 3-5 mm radiation in aa collinear collinear geometry. geometry. A A detailed detailed experimental study of these issues is required. It is interesting that FIR power level could be scalable beyond 100 100 MW by increasing the beam diameter. A typical beam diameter of the Neptune TW two2 wavelength CO 2 laser system is 12 cm with an intensity †10 CO2 |10 GW/cm . This beam, in combination with available large-aperture GaAs crystals, opens possibility to create aa unique high-power ≥1 >1 GW source of coherent radiation in the range of 100 100 µm jim —10 mm (0.03 -3 THz) on the base of noncollinear frequency mixing of CO laser lines. of €622 laser lines. 791 MODELLING OF IFEL IFEL BUNCHING BUNCHING MODELLING OF ItIt isis known longitudinal lens lens and and microbunches microbunches the theelectrons electrons known that that an an IFEL IFEL acts acts as as aa longitudinal on the scale of the electromagnetic wavelength [12]. At the Neptune Laboratory, in on the scale of the electromagnetic wavelength [12]. At the Neptune Laboratory, in order to achieve efficient microbunching in the small experimental area available, we order to achieve efficient microbunching in the small experimental area available, we need Optimization was was done done using using standard standard need to to optimize optimize the the IFEL IFEL parameters. parameters. Optimization equations of the motion for a single electron moving in a plane linearly polarized equations of the motion for a single electron moving in a plane linearly polarized electromagnetic field [13]. [13]. For For 100 100 MW MWof ofTHz THzradiation radiation electromagnetic wave wave in in aa planar planar undulator undulator field and a magnetic field of 0.25 T, we achieve maximum bunching through the Inverse and a magnetic field of 0.25 T, we achieve maximum bunching through the Inverse Free Electron Laser interaction after 0.5m. It is important that having more Free Electron Laser interaction after 0.5m. It is important that having more electromagnetic power or a longer undulator doesn't increase the performance of the electromagnetic power or a longer undulator doesn’t increase the performance of the system, the efficiency of the IFEL buncher reaches a limit due to the effects of the system, the efficiency of the IFEL buncher reaches a limit due to the effects of the non-linearities emittance diluition. diluition. Detailed Detailed results results of of non-linearities and and the the longitudinal longitudinal emittance optimization [7]. Parameters Parameters of of aa permanent permanent magnet magnet optimization are are presented presented elsewhere elsewhere [7]. undulator undulator are are listed listed in in Table Table 1. 1. Table Table 1. 1. Undulator Undulator parameters___________ parameters Magnetic field Undulator wavelength Magnet gap K parameter Undulator length 0.6 T 10 cm 2 cm 2.2 0.5 m Simulations are shown shown in in fig. fig. 4. 4. The The Simulations confirm confirm well our estimates. The results are simulations [14], a 3d 3d Lienerd-Wiechert Lienerd-Wiechert based, based, 44ththorder order simulations are are performed performed using TREDI [14], Runge electrons through through the the undulator undulator Runge Kutta, Kutta, Lorentz Lorentz solver code to track the electrons magnetic electron beam beam has has the the parameters parameters magnetic field field and and the laser field. The input electron typically mm-mrad, 300 300pC. pC.The Theradiation radiation typically running running at Neptune laboratory, 4 ps long, 66 mm-mrad, isis assumed in vacuum vacuum to to aa 77 mm mm focal focal spot. spot. In In assumed to to be be a 100 MW THz wave, focused in Fig.4a phase space space at at the the end end of of the the Fig.4a there there is is aa snapshot of the electron longitudinal phase Bunching Bunching in in IFEL Histogram of of phase phase distribution distribution Histogram 0.1 p / p a t 0.05 l e d 0 0.05 0.2 0.2 % 0.1 0.002 00 z (m) z(m) 0 0.002 nnnn^nnnlLnl 0 1.57 1.57 lllllhlninljniii 3.14 3.144.71 4.716.28 6.28 phase phase bb a FIGURE 4. Simulation results for THz IFEL microbunching. FIGURE microbunching. 792 undulator. undulator.The The longitudinal longitudinal microbunches microbunches on on the the scale scale of of the the plasma plasma wavelength wavelength are are evident evidentwithin within the the 44 ps ps (rms) (rms) long long beam beam envelope. envelope. Fig.4b Fig.4b shows shows the the phase phase histogram histogram over over the the 340 340 µm jim wavelength. wavelength. The The microbunches microbunches have have aa width width of of ~~ 30 30 µm jim that that is is small small (1/10) (1/10) compared compared to to the the plasma plasma beat-wavelength. beat-wavelength. Since Since THz THz radiation radiation driving driving the the IFEL IFEL isis locked locked in in phase phase with with the the plasma plasma beatwave, beatwave, all all these these microbunches microbunches are are phase-locked phase-locked with with the the accelerating accelerating structure. structure. ItIt is is clear clear that that for for PBWA PBWA getting getting more more electrons electronswith withaasmaller smaller phase phase spread spread will will result result in in less less energy energy spread spread after after the the plasma plasma acceleration. acceleration. At At the the same same time time the the longitudinal longitudinal emmittance emmittance dilution caused by the nonlinearities nonlinearitiesisisaaprincipal principallimitation limitation of of the the IFEL IFEL microbuncher. microbuncher. Further Furtherimprovement improvement in inthis this respect respect could could be be achieved achieved by by driving driving the the same same rd undulator undulatorwith withboth both 340 340µm jimradiation radiation and and it’s it's 33rd harmonic harmonic as as suggested suggested recently recently by X.J. XJ. Wang Wang for for aa 11 µm jim IFEL IFEL buncher buncher [15]. [15]. As As oppose oppose to to the 11 µm jim beam, it is not rd durable durableto togenerate generate the the 33rd harmonic harmonic of of THz THz radiation. However one can generate 114 µm jimradiation radiationby by noncollinear noncollinear DFG DFG in in GaAs GaAs using using CO CO22 laser laser lines. lines. In In fact, fact, ifif we we take take the same asas forfor thethebeatwave, the10.6 10.6µm jimline line-the -the same beatwave,then thenthe the9.7 9.7µm jimline line(the (the9P(36) 9P(36)line) line) rd will willprovide provide the the difference difference frequency frequency equal equal to to the the 33rd harmonic harmonic of of beatwave beatwave with with aa negligible negligiblefrequency frequency off-set off-set of of ~1 ~1GHz. GHz. In In experiment experiment another another laser laser beam beam from from aa MW MW power, power,200 200ns nsCO CO22laser laser could could be be used used as as aa seed seed at at 9.7 9.7 µm jim in in combination combination with with aa TW TW 100 100ps pspulse pulseatat10.6 10.6µm. jim.3D 3Dmodelling modelling have have indicated indicated that that indeed indeed by by choosing choosing an an optimal optimalratio ratiobetween between114 114and and 340 340 µm jim radiation radiation (1.5/1) (1.5/1) one one can can significantly significantly increase number numberof ofelectrons electronstrapped trapped in in slightly slightly shorter shorter bunches bunches (~20 (~20 µm). jim). Preliminary Preliminary results are areshown shownin inFig.5. Fig.5. Histogram Histogramofofphase phasedistribution distribution 0.75 Bunching factor 0.3 0.2 0.2 % 0.1 0.1 0.65 0) 0.60 o c 0.55 D 0.50 CO 0 3rd Harmonic IFEL 0.70 0.45 0 1.57 1.57 3.14 3.14 phase phase 4.71 4.71 6.28 6.28 00.0 .0 b 00.5 .5 11.0 .0 11.5 .5 22.0 .0 22.5 .5 Line Line ratio ratio (3ω/ω) (3co/co) FIGURE5.5.Simulation Simulationresults resultsfor forthe the 33rdrd harmonic harmonic THz IFEL microbunching. FIGURE BEAM LOADING LOADING IN INAA PLASMA PLASMA ACCELERATOR ACCELERATOR BEAM Aswas wasshown shown in in the the previous previous section section THz THz IFEL IFEL microbunching microbunching can produce ~ 100 100 As fs electron bunches, which is ten times shorter than the plasma wavelength. Here we fs electron bunches, which is ten times shorter than the plasma wavelength. 793 examine analytically how many particles could be loaded in a plasma heatwave accelerator both longitudinally and transverse in order to obtain the small energy spread AE/E~0.1. It is known that when the electron beam and the plasma wave are much larger than c/cop, the beam-loading problem is approximately one-dimensional [16]. This condition is true for c/cop~50 jim for the case when the CO2 laser beam diameter is 400 jim (F/18 focusing). Longitudinal beam loading is limited by a wakefield production and the maximum number of beam electrons is given by (3) where 8 is the normalized plasma wave amplitude and S is the cross-sectional area of the plasma wave. In our conditions, for 10% wave, N0 equals to 6xl09 electrons. Therefore for AE/E~0.1 one can load up to 6xl08 electrons or 10 pC charge without significant dumping the plasma wave. In experiment we do not expect to exceed this charge per bunch. It is obvious that transverse variation of the longitudinal electric fields will result in a difference in energy gained by electrons or large energy spread. Typical size of the plasma wave seen in the 2D-PIC simulations is 170 pm (FWHM) for the laser field intensity 2xl014 W/cm2 [17]. Such an accelerating structure requires an e-beam size a^^SO jim. This is approximately 3 times larger what the Neptune photoinjector can provide at the moment and further work is needed to improve quality of the e-beam. SUMMARY THz driven IFEL microbunching is a promising scheme for a phase-locked injection of bunched electrons in a plasma accelerator. It is shown that for the Neptune PBWA experiment ~100 MW of 340 jim radiation is required to drive a THz buncher. Results of preliminary experiments on generation of THz radiation using noncollinear frequency mixing of €62 laser lines in GaAs are presented. ACKNOWLEDGEMENT This work was supported by the U.S. Department of Energy, grant DE-FG0392ER40727. REFERENCES 1. C. Joshi, and P.B. Corkum, Physics Today, 49, 36-42 (1996). 2. C.E. Clayton,and L. Serafmi, IEEE Trans. Plasma Science, 24, 400-408 (1996). 3. 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