vii TABLE OF CONTENTS CHAPTER 1 2 TITLE PAGE DECLARATION ii DEDICATION iii ACKNOWLEDGEMENT iv ABSTRACT v ABSTRAK vi TABLE OF CONTENTS vii LIST OF TABLES x LIST OF FIGURES xi LIST OF SYMBOLS AND ACRONYMS xiv LIST OF APPENDICES xvi INTRODUCTION 1.1 Background of research 1 1.2 Historical Review of Neutron Radiography 3 1.3 Research Objectives 6 1.4 Rational for Research 6 1.5 Research Scope 7 1.6 Organization of Thesis 7 LITERATURE REVIEW 2.1 Neutron Radiography 8 2.1.1 Principle of neutron radiography 11 2.1.2 Neutron sources 12 viii 2.2 2.1.2.1 Accelerator 12 2.1.2.2 Radioisotopes 13 2.1.2.3 Nuclear reactor 14 The Monte Carlo N-Particle Code Version 5 15 2.2.1 The Monte Carlo Method 16 2.2.2 Neutron Physics in MCNP5 17 Transfer Function for Imaging System 18 2.3.1 Edge and Line Spread Function 18 2.3.2 Two Dimensional Fourier Transform 20 2.4 Modulation Transfer Function 21 2.5 Neutron Radiographic Facilities at the Malaysian 22 2.3 Nuclear Agency (Nuclear Malaysia) 2.6 3 Previous study on NUR-2 system 24 METHODOLOGY 3.1 Introduction to Sample 26 3.2 Geometry of Exposure 27 3.3 Monte Carlo Simulations 29 3.3.1 Input file 29 3.3.2 Output 30 3.3.3 Simulations in MCNP5 31 Experimental confirmation of the MCNP 32 3.4 simulation 4 3.4.1 Experimental Procedure 33 3.5 Edge Image Processing 37 3.6 MTF measurement and calculation 39 RESULTS AND DISCUSSION 4.1 4.2 MCNP simulation results 42 4.1.1 Cadmium without scattering material 43 4.1.2 Cadmium with scattering material 45 Experimental results 47 4.2.1 Cadmium without scattering material 47 ix 4.3 5 4.2.2 Cadmium with scattering material 51 Comparison of MCNP simulation and experiment 56 CONCLUSION AND RECOMMENDATION 5.1 Conclusion 59 5.2 Recommendation 61 REFERENCES 62 APPENDICES 65 x LIST OF TABLES TABLE NO. TITLE PAGE 2.1 Classification of neutron by energy 10 3.1 Radiographic image quality 35 4.1 Estimation of spatial frequency at MTF20% from simulation and experiment for each thickness of 58 cadmium 4.2 Estimation of FWHM from simulation and experiment for each thickness of cadmium 58 xi LIST OF FIGURES FIGURE NO. TITLE PAGE 2.1 Mass absorption coefficients for the elements for both thermal neutrons and X-rays 9 2.2 Schematic sketch for neutron radiography 11 2.3 Random history of a neutron incident on a slab of material that can undergo fission 17 2.4 A line input δ(x1) 19 2.5 Representation of an ideal edge profile 21 2.6 Derivation of the MTF from the edge response curve 2.7 22 Reactor TRIGA MARK II beamports and thermal column arrangements 23 2.8 Layout of NUR-2 facility 24 2.9 Neutron collimator arrangement 24 3.1 Cadmium foil 27 3.2 Diagram of knife-edge experiment 28 3.3 MCNP input file structure 29 3.4 The used Monte Carlo model for calculation of the ESF 3.5 Setup 32 for knife-edge measurement without scattering material 3.6 33 Neutron radiography setup in NUR-2 exposure room 34 xii 3.7 Characteristic of NUR-2 measured by measured ASTM beam purity indicator 35 3.8 DR3000 digital radiograph film digitisation system 36 3.9 Setup for knife-edge measurement with scattering material 3.10 36 (a) Surface plot of ESF profile direct from TECPLOT file 37 (b) Cropped ESF profile from TECPLOT file 37 3.11 Edge profile retrieval using Isee! Software 38 3.12 Cropped knife-edge image of cadmium 39 3.13 Operational framework of the MTF measurement and calculation 40 3.14 FWHM determination 41 4.1 Comparison of MCNP simulation result of (a) Edge spread function, (b) Line spread function and (c) Modulation transfer function for three different thickness of cadmium without scattering material 4.2 44 Comparison of MCNP simulation result of (a) Edge spread function, (b) Line spread function and (c) Modulation transfer function for three different thickness of cadmium with scattering material 46 4.3 Neutron radiography image for cadmium knife-edge 47 4.4 Cropped knife-edge image of cadmium 48 4.5 Comparison of experimental result of (a) Edge spread function and (b) Line spread function for three different thickness of cadmium without scattering material 4.6 49 Comparison of experimental result of (a) raw and (b) smoothed modulation transfer function for three different thickness of cadmium without scattering material 4.7 50 Neutron radiography image for cadmium knife-edge with scatterer 51 xiii 4.8 Cropped knife-edge image of cadmium with scatterer 4.9 52 Comparison of experimental result of (a) Edge spread function and (b) Line spread function for three different thicknesses of cadmium with scattering material 4.10 53 Comparison of experimental result of (a) Edge spread function and (b) Line spread function for three different thicknesses of cadmium with scattering material 4.11 55 MTF comparison of MCNP simulation and experiment for (a) 1 mm, (b) 2 mm and (c) 3 mm thick of cadmium for all cases 57 xiv LIST OF SYMBOLS AND ACRONYMS eV - Electron volt kW - Kilowatt R - Röentgen n - Neutron cm - Centimetre mm - Millimetre µm - Micrometre s - Second I - Transmitted intensity I0 - Incident intensity Ʃ - Macroscopic absorption cross section d - Thickness of the sample Sb-Be - Antimony Beryllium Am-Be - Americium Beryllium Cf-252 - Carlifornium-252 Gd - Gadolinium MCNP - Monte Carlo N-Particle FIR - Flux image radiograph PScF - Point scattered function l(x) - Line spread function (LSF) e(x) - Edge spread function (ESF) h(x,y) - Point spread function (PSF) M(u) - Modulation Transfer Function (MTF) f(x) - Input function F(u) - Fourier Transform xv σ - Standard deviation δ(x) - Delta function ROI - Region of Interest FWHM - Full Width at Half Maximum xvi LIST OF APPENDICES APPENDIX TITLE PAGE A Publications 65 B Material safety data sheet for cadmium 66 C Codes for MCNP simulation for 1 mm thick of cadmium without scattering material D 69 Codes for MCNP simulation for 1 mm thick of cadmium with scattering material 70
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