Journal of Contaminant Hydrology 30 Ž1998. 79–100 Influence of fracture truncation on dispersion: A dual permeability model Paige Stafford a , Laura Toran a a,) , Larry McKay b EnÕironmental Sciences DiÕision, Oak Ridge National Laboratory 1, Oak Ridge, TN 37831-6400, USA b Department of Geological Sciences, UniÕersity of Tennessee, KnoxÕille, TN 37996-1410, USA Received 27 September 1996; revised 3 April 1997; accepted 3 April 1997 Abstract Simulations with a dual permeability model show that a few discrete fractures can have a major influence on plume geometry. A limited number of truncated fractures Ž1–4. within a permeable matrix can create nearly circular plumes, with about the same degree of spreading in the direction transverse to the average hydraulic gradient as in the longitudinal direction. By comparison, continuous fractures in the direction of flow tend to produce elongated plumes, similar to those typically seen in granular materials. Both types of plumes have been observed in tracer experiments in fractured porous media on the Oak Ridge Reservation. Understanding the influence of fracture geometry is important in planning field characterization and subsequent remediation in fractured porous media. q 1998 Elsevier Science B.V. 1. Background and purpose Shales are typically considered adequate barriers against migration of contaminants. However, on the Oak Ridge Reservation ŽORR. the upper portion of these deposits Žusually less than 10 m depth. are highly weathered and fractured, which substantially increases the hydraulic conductivity and potential for contaminant migration ŽSolomon et al., 1991.. For example, tritium migration from shallow low-level radioactive waste ) Corresponding author. Current address: Dept. of Geology, Temple University, Philadelphia, PA 19022, USA. Tel.: q1-215-2048227; fax: q1-215-2043496. 1 Oak Ridge National Laboratory is managed by Lockheed Martin Energy Research Corp. for the U.S. Department of Energy under contract No. DE-AC05-96OR22464. 0169-7722r98r$19.00 q 1998 Elsevier Science B.V. All rights reserved. PII S 0 1 6 9 - 7 7 2 2 Ž 9 7 . 0 0 0 3 7 - 5 80 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 trenches within the weathered shales has been observed at a number of sites on the ORR ŽOlsen et al., 1986; Wickliff et al., 1989; Solomon et al., 1991; Shevenell et al., 1994; Sanford and Solomon, 1995; McKay et al., in press.. Investigations in fractured clay-rich glacial deposits ŽKeller et al., 1986; D’Astous et al., 1989; Thompson, 1990; Balfour, 1991, Ruland et al., 1991; McKay et al., 1993a., which are similar to the weathered shales, have also shown that contaminant migration can occur at environmentally significant rates. Numerical modeling of groundwater flow and solute migration in the weathered and fractured shale poses special challenges because it is not clear whether the material can be considered as a continuum or equivalent porous media ŽEPM., or whether it must be modeled on the scale of individual fractures Ždiscrete fracture or DF approach.. The EPM approach defines a fractured system as a single continuum, or series of continua, where the parameter values are affected by the presence of fractures, but the fractures are not modeled explicitly. The advantage of this approach is that just a few parameters, such as hydraulic conductivity, hydraulic gradient, effective porosity and dispersivity, are necessary for simulations. They are either measured in the field or laboratory, or are obtained from fitting simulations to data from tracer experiments. This approach can still have a high degree of uncertainty because of problems with ‘fitting’ parameters, such as dispersivity and effective porosity, that may vary with time and scale. Many studies exist that examine the applicability of EPM Žor continuum. models to idealized fractured systems Že.g., Long et al., 1982; Berkowitz et al., 1988; Maloszewski and Zuber, 1993.. Long et al. Ž1982. determined which characteristics of a fractured system increase the likelihood of the EPM approach being appropriate. Some of these characteristics are: Ži. high fracture density, which creates connected fractures and therefore connected flow paths, Žii. relatively constant fracture aperture, to prevent only a few fractures from controlling most of the flow and Žiii. random orientation of fractures so that flow is not unidirectional. In addition, it must be possible to define a representative elemental volume ŽREV. where: Ži. heterogeneity is negligible, Žii. the REV is large relative to the fracture lengths to represent complete flow paths and Žiii. the REV is small compared to the system being modeled. These factors, particularly fracture density and orientation, can be used to provide a preliminary indication of whether an aquifer will behave as an EPM, but there are insufficient well-documented field examples to say in which settings an EPM approach should be effective. The limited number of field studies available has provided important information to help conceptualize these systems Že.g. Bibby, 1981; Pankow et al., 1986; Cacas et al., 1990; McKay et al., 1993a,b; Sanford et al., 1996; Cook et al., 1996.. On the other hand, a discrete fracture approach requires information about both the fractures and the blocks of soil or rock between fractures. Some of these parameters, particularly fracture aperture and degree of fracture interconnection, are difficult to measure and may contain a high degree of uncertainty. Discrete fracture models typically require considerably more computer memory than an EPM model; computer memory is often a limitation on the size and detail of the region modeled. The matrix between discrete fractures is treated differently depending on the modeling approach. Modeling studies conducted in the 1980’s ŽLong et al., 1982; Schwartz et al., 1983; Endo et al., 1984; Long and Witherspoon, 1985. described the importance of P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 81 effective porosity Žwhich they define as the porosity contributed by fractures alone. and fracture orientation, but matrix transport parameters were considered insignificant and were not included in these models. Other studies ŽFoster, 1975; Day, 1977; Sudicky and Frind, 1982; Maloszewski and Zuber, 1985, 1993; Harrison et al., 1992; Sudicky and McLaren, 1992; Zuber and Motyka, 1994. established the importance of matrix diffusion in fractured, high porosity materials by indicating its effect on delaying solute breakthrough. Sudicky and Frind Ž1982., in simulating solute migration Žtritium. in a fractured porous material, showed that matrix diffusion acts as a dynamic storage mechanism. The process was sufficient to retard the overall migration rate of the plume by several orders of magnitude, as compared to advective transport rates in fractures alone, where no diffusion is assumed. An alternate approach to selecting either EPM or a discrete fracture approach is to consider a dual permeability approach. In this model, there is an EPM, resulting from intergranular flow or from flow through a network of closely-spaced fractures, and a few interconnected larger aperture fractures within it. This scenario is likely to be common in fractured deposits, with the larger aperture fracture sets resulting from later tectonic activity, or intersecting fracture sets. The importance of considering hydraulically connected fractures as an important subset of fractures has been noted by a number of researchers using field and modeling data Že.g., Cacas et al., 1990; Clemo and Smith, 1989, cited in Smith and Schwartz, 1993; Renshaw, 1996; Therrien and Sudicky, 1996; Parney and Smith, 1995.. The fractures within a system that are hydraulically connected can influence flow directions and flow rates, but be part of a limited network. Parney and Smith Ž1995. used particle tracking in network models Žfractures only. to show that particles tend to have longer flow paths in higher aperture pathways, and that these select pathways need to be incorporated into EPM approaches. Rubin et al. Ž1996. found that in fractured permeable formations, longer injection times lead to closer approximations with EPM. One further consideration in comparing EPM and DF approaches is whether dispersion within a fracture network can be modeled adequately. Dispersion in fracture networks Žno block permeability. has been studied by Schwartz et al. Ž1983. and Smith and Schwartz Ž1984.. They found that the longitudinal and transverse dispersivity of mass varied for different realizations of fracture networks, and that both flow direction and fracture geometry were important. Significant longitudinal dispersion and long tails for solute breakthrough were observed in some fracture networks. Although an EPM approach to characterizing dispersion has been formulated ŽVan der Kamp, 1992., the information needed to calculate an equivalent dispersivity Že.g., fracture spacing. requires characterization that could be used to better identify pathways if used explicitly, and does not account for geometry of fracture configuration. Rubin and Buddemeier Ž1996. evaluated the effects of fracture orientations and relative fracture permeability in a permeable matrix, and found that transverse dispersivity may exceed longitudinal dispersivity when fracture permeability is high and orientations approach a direction 908 to flow. They studied continuous fracture networks. This paper examines how fracture geometry can influence dispersion in a hypothetical plume. The study of dispersion in discrete fractures presented here differs from previous studies by examining Ž1. the effect of the geometry of fracture intersections, 82 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 and Ž2. the influence in a dual permeability media. The dual permeability media consists of a few larger aperture, hydraulically active fractures set within a matrix of small fractures that act as a porous medium. The results of the modeling study are compared with two existing plumes in fractured shale saprolite on the Oak Ridge Reservation in Tennessee. 2. Example plumes 2.1. Broad plume: the burial ground 4 site Although the modeling presented here is hypothetical, the problem is based on a tritium plume observed on the Oak Ridge Reservation. The plume exhibited an Fig. 1. Contours of tritium concentrations in log scale of pCirml at three different times after initial injection. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 83 unusually large transverse spreading, with the width of the plume approximately equal to its length ŽFig. 1.. The plume developed from a long term tritium tracer test that was carried out in the fractured, highly weathered shale of the Conasauga group at Oak Ridge National Laboratory ŽWebster, 1996. near burial ground 4 ŽBG4.. The experiment is unique due to the high levels of tritium injected Ž50 curies. and the long monitoring period Ž16 years to date.. This test is one of the few controlled field-scale tracer experiments in a fractured media containing significant matrix porosity Ž10 to 40%. and permeability Ž; 10y2 mrd.. The study site is adjacent to low level radioactive waste disposal sites on the ORR, and hence should be relevant to assessing contaminant migration and behavior at this and other waste sites in the same geologic deposits. Seven monitoring wells were constructed in a semi-circle 3.7 m down-slope from the injection well ŽFig. 1.. The depth of the monitoring wells ranges from 8.3 m to 9.4 m, and the depth of the injection well is 6.3 m. Slug tests were carried out in each well at Fig. 2. Contours of 10 ppb rhodamine from the West Bear Creek Valley tracer experiments at two different times. 84 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 the experiment site to determine bulk hydraulic conductivity, K b . The K b values range from 1.2 = 10y2 to 3.0 = 10y3 mrd, with a geometric mean of 7.2 = 10y3 mrd. The water table gradient from the injection well to monitoring well 7 Ždirectly downslope. averages 0.15. The migration of the plume is characterized by a fast moving, low concentration front Ž10’s of cm per day., a slower moving center of mass Ž- 1 cmrday., a very long Žup to 16 years. low concentration tail, and an unusually large degree of transverse spreading. 2.2. Narrow plume: West Bear Creek Valley site A second example is presented here that was not explicitly modeled, but used to contrast plume shape and orientation. A rhodamine dye tracer experiment ŽLee et al., 1989, 1992; Brown et al., 1992. was conducted at the West Bear Creek Valley ŽWBCV. site on the ORR. The geologic material at this site is similar to that at the BG4 site in terms of porosity, hydraulic conductivity, and fracture spacing and orientation. However, the shape of the plume was very narrow ŽFig. 2. as compared to the wide shape of the BG4 plume ŽFig. 1.. The major difference between the two sites is that the average water table gradient direction at the WBCV site is approximately parallel to strike of the bedding plane, and at the BG4 site it is nearly perpendicular to strike ŽFigs. 1 and 2.. The orientation of the water table gradient with respect to the fracture planes likely contributed to the difference in plume shapes. The hydraulic conductivity is expected to be higher in the direction of strike at both locations due to bedding plane partings or fractures ŽSolomon et al., 1991.. With this in mind, transverse spreading at the WBCV site, where there is a strike-parallel gradient, would not be strongly influenced by fluctuating water table direction and secondary fractures perpendicular to strike because of the lower hydraulic conductivity in the transverse direction. Conversely, at the BG4 site, where the average hydraulic gradient is in the direction of the lower hydraulic conductivity Žperpendicular to strike. fluctuating water table direction and fractures perpendicular to bedding are expected to have more of an influence on transverse spreading. It is likely that at other locations, where water table slope is neither parallel or perpendicular to bedding strike, the shape of the plumes would be intermediate between these two extremes. 3. Modeling approach In this study, the discrete fracture approach was combined with the EPM approach ŽDF-EPM. to investigate the influence of a few widely-spaced larger-aperture fractures in a highly fractured matrix. These widely-spaced fractures, if present, could have a large influence on transverse spreading of a plume. The fracture networks chosen are hypothetical and may not be the cause of transverse spreading at the BG4 site. Other factors, such as seasonal variations in the elevation and direction of slope of the water table are expected to be significant at the site, but were not incorporated in the 2D steady-state approach. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 85 The highly fractured network was assumed to act as an EPM. A transverse dispersivity of zero was used with an implicit hypothesis that the transverse spreading can be modeled using fractures. Different scenarios were then run with a few widely-spaced fractures superimposed on the EPM to see if transverse spreading could be reproduced by these fractures. Fracture aperture values for the widely-spaced fractures were set at either 150 or 250 m m, based on estimates from hydraulic tests ŽMoore and Toran, 1992.. Other parameters used in the simulations are listed in Table 1. The water table gradient from the injection well to the downgradient well averaged 0.15 at the BG4 site. The matrix porosity in the shallow subsurface was estimated to be about 0.4. Using the calculated velocity of 0.01 mrd from EPM modeling ŽStafford, 1996; McKay et al., in press. resulted in a hydraulic conductivity of 0.03 mrd, which is close to the geometric mean value measured in slug tests at the site Ž0.01 mrd.. Other combinations of hydraulic conductivity and porosity could have been used, preserving the observed velocity, with only minor effect on the transport calculation. The longitudinal dispersivity of 0.8 m was obtained from the EPM model fitting ŽStafford, 1996; McKay et al., in press.. The longitudinal fracture dispersivity was based on literature derived values on the order of 0.1 m. The duration of the input function was 40 days. This was chosen based on the time necessary for the concentration in the injection well to decline to half of its initial value, so that the area under the input function was approximately the same as the area under the measured relative concentration Ž CrCo . versus time plot for the injection well. For tritium, the half life is 12.4 y, the diffusion coefficient is 5.18 = 10y5 m2rd, and the retardation factor is 1. The EPM parameters for hydraulic conductivity, porosity, and longitudinal dispersivity were used to describe the matrix for the DF-EPM model. These parameters were not varied in this study because this was not a calibration exercise. Table 1 Parameters used for FRAC3DVS DF-EPM simulations Parameters Used Values Flow velocity Žmrd. Hydraulic gradient Matrix porosity Longitudinal dispersivity Žm. Transverse dispersivity Žm. Effective diffusion coefficient Žm2 rd. Retardation Solute half-life Žd. Source concentration Duration of source Žd. Longitudinal fracture dispersivity Žm. Transverse fracture dispersivity Žm. Fracture aperture Ž2 b . Ž m m. Fracture retardation 0.01 0.15 0.40 0.8 0 5.18=10y5 1.0 4.53=10 3 1.0 40.0 0.10 0 150, 250 1.0 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 86 3.1. FRAC3DVS The model used was FRAC3DVS, a discrete fracture numerical model where advective transport and diffusion are accounted for in the matrix ŽTherrien and Sudicky, 1996.. The matrix is represented in three dimensions, and fractures are represented by two-dimensional planes. The model employs a time marching Galerkin finite element technique which is used to discretize the solute transport equation with either finite element or by mimicking a finite difference discretization. The solution for the flow equation is solved by the control volume finite element approach and a preconditioned ORTHOMIN solver. The fracture elements are common to nodes comprising the porous matrix elements which ensures the continuity of hydraulic head at the fracture-matrix interface. The governing equation for solute transport in the matrix is R dc dt d s d xi ž Di j dc d xj / dc y Õj d xi y R l c i , j s 1, 2 where Di j ŽL2 Ty1 . is dispersion defined as q1 q 2 Di j s Ž a L y a T . q a T < q < d i j q D )d i j < q< i , j s 1, 2, Ž 1. Ž 2. where a L ŽL. is the longitudinal dispersivity, a T ŽL. is the transverse dispersivity, < q < is the magnitude of the Darcy flux, defined as d qs d xi ž Ki j d ŽCqz . d xj / i , j s 1, 2 where c ŽL. is the pressure head, z ŽL. is the elevation head. Fig. 3. Model domain for FRAC3DVS simulations. Ž 3. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 87 For transport in the fracture, the governing equation is 0s2 b R f d cf dt d y d xi ž Df i j d cf d xj / q qf d cf d xj q R f l cf y V n < Iyq V < Iq i , j s 1, 2, Ž 4. where the terms V n represents the advective–dispersive loss or gain of solute mass across the fracture-matrix interfaces Iy and Iq due to fluid leakage and hydrodynamic dispersion and 2 b is the fracture aperture. The Darcy flux in the fracture is d d Ž cf q zf . qf s i , j s 1, 2, Ž2 b. Kf Ž 5. d xi d xj where c f ŽL. is the pressure head in the fracture, z f ŽL. is the elevation head in the fracture, and qf is the fluid flux in the fracture ŽLrT.. The fracture dispersivity is defined in the same way as matrix dispersivity where dispersivity coefficients and fluxes correspond to the fracture. Fig. 4. Fracture effects on head distribution using an aperture of 250 m m for the domain shown in Fig. 3, with Õ s 0.01 mrd Žbefore addition of fractures.. Direction of flow is from top to bottom. 88 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 3.2. Model grid The two-dimensional modeling in this study was performed with the FRAC3DVS code for a 10 m = 10 m plan view region as shown in Fig. 3. The same model grid used for the EPM modeling to determine matrix parameters was used for the DF-EPM model. The flow system was assumed to be at steady-state and fully saturated, with the medium Žbefore addition of fractures. homogeneous and isotropic. A uniform, constant head along the top and bottom of the grid was used to establish an overall hydraulic gradient of 0.15. The bulk hydraulic conductivity for the medium was assumed to be isotropic, even though it may be anisotropic at the field site, because of fractures parallel to bedding strike. However, strike-parallel fractures were represented explicitly in the DF-EPM model. The source term used was a step-function with a relative concentration of 1.0 for 40 days. Fig. 5. Simulation results for two-dimensional DF-EPM model, case A, using 2 bs 250 m m. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 89 3.3. Discrete fracture-EPM (DF-EPM) simulation Simulations were carried out with very simple networks typically with one to four fractures. Isolated fractures which did not penetrate a boundary or another fracture were not considered because they are expected to have less influence than interconnected fractures. To create transverse spreading, fracture patterns which are truncated by a fracture parallel to the direction of spreading are considered. Truncation of fractures with a perpendicular fracture set is a common style of fracturing because stress relief in an alternate direction will cause a fracture to terminate at fracture intersections ŽHancock, 1985; Pollard and Aydin, 1988.. The influence of different styles of fractures ŽFig. 4. is compared by examining both the head and the concentration contours. Then some variations on fracture aperture, fracture density and source location are also examined. Fig. 6. Simulation results for two-dimensional DF-EPM model, case B, using 2 bs 250 m m. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 90 4. Results 4.1. EPM modeling to determine matrix parameters An EPM model was fit to the BG4 plume using velocity and longitudinal dispersivity as fitting parameters ŽStafford, 1996; McKay et al., in press.. In the EPM model, a high transverse dispersivity is needed to represent the broad shape of the plume ŽFig. 1.. The best fit to the shape of the plume was for a transverse dispersivity of approximately 0.8 m, which contrasts with the commonly seen assumption that transverse dispersivity will be about an order of magnitude smaller than longitudinal. Although a variety of factors can contribute to the broad plume at BG4, the one explored here is the affect of fracture flow on plume spreading. Fig. 7. Simulation results for two-dimensional DF-EPM model, case C, using 2 bs 250 m m. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 91 4.2. Fracture geometry In the DF-EPM model, the transverse dispersivity is set to zero, and instead fractures are used to spread the plume. The degree of spreading varied depending on fracture geometry. The initial cases A through F are described first. ŽA. A single fracture which fully penetrated the system and was perpendicular to flow direction had no effect on the head distribution, and no effect on transport ŽFig. 5.. The simulated plume was identical to the plume generated for the case with no fractures and no transverse dispersivity. This case represents a setting where the flow direction is perpendicular to the dominant fracture orientation, and there is no secondary fracture set. Fig. 8. Simulation results for two-dimensional DF-EPM model, case D, using 2 bs 250 m m. 92 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 ŽB. A single fracture which fully penetrated the system and was aligned parallel to the direction of flow had no influence on hydraulic head. There was relatively little influence on transverse spreading ŽFig. 6.. There was somewhat faster transverse spreading at early times, but about the same amount of spreading as case ŽA. at later times. However, the fracture, which intersected the source well, caused longitudinal transport rates to increase, as seen by the faster arrival of breakthrough at the lower boundary Ž85 days.. This case represents a setting where the flow direction is oriented along the dominant fracture orientation, and there is no secondary fracture set. ŽC. Two orthogonal fractures which fully penetrate the system and intersect downgradient of the source well had no effect on head distribution, and had the same effects Fig. 9. Simulation results for two-dimensional DF-EPM model, case E, using 2 bs 250 m m. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 93 on transport ŽFig. 7. as described in ŽB. above, i.e., an increase in longitudinal transport at early times. This case illustrates that fractures orthogonal to a fully penetrating fracture do not create significant transverse spreading, and why the plume at WBCV would not be influenced by perpendicular fractures. The fully penetrating fracture oriented parallel to the flow direction represents the dominant fracture set. Fractures perpendicular to both the gradient and the fully penetrating fracture are not an important influence. Thus, a relatively narrow plume develops. ŽD. A single fracture parallel to the direction of flow which passed through the tracer injection well and penetrated the up-gradient constant head boundary, but did not reach the other end of the system, influenced the hydraulic head distribution, causing radial flow away from the terminus of the fracture ŽFig. 8.. The radial flow caused solute Fig. 10. Simulation results for two-dimensional DF-EPM model, case F, using 2 bs 250 m m. 94 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 spreading in the transverse direction ŽFig. 8.. At 85 days, the outer contour interval Ž CrCo s 10y8 . is about three times wider for the case with the truncated fracture than for the systems with continuous fractures ŽFigs. 5–7.. As the plume dissipates, the shape remains broad. This case is an example of fracture geometry of a subdominant fracture set that can broaden plume geometry. The truncation of the fracture makes it a subdominant fracture set in contrast to fully penetrating, or longer fractures. ŽE. Two fractures, one perpendicular to the direction of flow and the second parallel to flow but terminating at the intersection with the other fracture, disrupted the head distribution and increased the amount of transverse spreading ŽFig. 9. even more than a single terminated fracture. This case illustrates that the presence of a second fracture set, where a dominant fracture transverses the model domain, is an important influence on plume development. This secondary set intersects the primary set providing connectivity. ŽF. When the fracture orientation described in ŽE. was repeated such that there was a regular brickwork of fractures, hydraulic heads were disrupted and a large degree of transverse spreading of the plume occurred ŽFig. 10.. In this case, there was now a continuous network of fractures in the direction of flow and the rate of longitudinal migration of the plume increased. The truncated fractures represent a secondary fracture Fig. 11. Simulation results for two-dimensional using 2 bs 250 m m and varying fracture spacing. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 95 set because the fractures in the direction of the flow field are shorter than the fracture perpendicular to the flow field. 4.3. Fracture density Increasing the density of the fracture brickwork Ži.e., increasing the number of fractures. further increased both the transverse and longitudinal spreading ŽFig. 11.. Although the contours are not smooth even for the dense network, the broad outline of the contours becomes more convex, approaching an EPM appearance, as the network density increases. 4.4. Fracture aperture Increasing the fracture aperture from 150 m m to 250 m m increases transport in the fracture and broadens the plume in the transverse direction for a fracture truncated by a Fig. 12. Simulations for case E with different aperture Ž2 bs150 m m.. 96 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 perpendicular fracture ŽFig. 12.. The effects of increase transport in wide fractures is seen even at early times Ž85 days.. 4.5. Location of the source term The location of the source term with respect to the fracture affects the symmetry of the plume. When the fracture is located 0.4 m from the injection well, the head gradient is offset and there is slightly less up-gradient spreading ŽFig. 13.. The asymmetry is more pronounced at early times, then at later times the plume moves away from the source more slowly than the case where the source intersects a fracture. Fig. 13. Simulation results for two-dimensional DF-EPM model, case D, using 2 bs 250 m m and varying fracture placement from source. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 97 5. Discussion 5.1. Implications for remediation Tritium migration through the fractured porous material at the experiment site is strongly influenced by matrix diffusion. If this was not so, tritium would have rapidly flushed out through the fractures under natural gradient conditions, rather than persisting for at least 16 years, as was observed. It is likely that tritium removal by pump-and-treat or drainage methods would be a very slow process due to ‘storage’ effects created by matrix diffusion. Thus, it is important to distinguish plume spreading which is influenced by fracture patterns rather than hydraulic affects. Furthermore, although a variety of fracture networks could reproduce the present plume, they may behave very differently when simulated remediation efforts, such as pumping from wells, are added to the system. If flow rates are increased by lowering the water table, such as could occur for remediation purposes, this would affect predictions of the effectiveness and required duration of remediation. These precautions are valid for any site with a dual permeability system or extreme variations in hydraulic conductivity. 5.2. Implications for field inÕestigations Evaluation of field-scale systems is still problematic because of the cost and difficulty in sampling fractured systems. Modeling studies, such as the one presented here, can be used to determine the types of fracture geometry that can influence observable plume features such as spreading and long term behavior. Although a few large aperture fractures Žas shown in this study. can greatly affect plume behavior, they could be very difficult to detect by hydraulic testing. Instead, the plume geometry could be used to indicate behavior caused by major fractures. For example, in the two field experiments presented here, there was a large contrast in plume shape. At BG4, the plume was very broad, and transverse fractures may have been important in spreading the plume. At the WBCV site, the plume was narrow, and transverse fractures are not believed to be important because the dominant fracture set was in the direction of flow, not perpendicular to flow. The large aperture fracture set contributed not only to transverse spreading, but also increased longitudinal spreading as seen in cases D–F with increased downgradient plume concentrations. Because this was not a calibration exercise, the matrix EPM dispersivity value was not adjusted to account for the influence of the discrete fractures. However, this could be a future exercise to understand the relationship between EPM parameters and DF-EPM parameters. The EPM parameters would need to account for all fracture sets, and lumped fracture and ‘matrix’ dispersivity and conductivity values tend to be higher. In contrast, the DF-EPM model the matrix parameters only describe the small scale fractures and values tend to be lower. Simulations show that it may not be necessary to characterize all of the minor fractures, but instead focus on finding the major fractures, fracture orientations, and network patterns. By understanding the influence of fracture geometry on plume shape, modeling may assist the difficult task of detecting the influential fractures in the field. 98 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 6. Conclusions The large transverse spreading observed in the tritium tracer test near Burial Ground 4 on the Oak Ridge Reservation could be reproduced with the DF-EPM approach using a few larger aperture truncated fractures superimposed on an EPM. This does not imply that truncated fractures are responsible for the spreading, but merely identifies them as a possible cause. The combined discrete-fracturerequivalent porous media ŽDF-EPM. approach is useful for looking at possible causes of features such as the observed transverse spreading, but in the absence of detailed data on the fracture network, it is likely that it would be no more effective than the EPM approach in predicting future behavior of the plume. Because this was a dual permeability model, transport occurred in both the fracture and the matrix. This model represents a fractured field site where the matrix permeability is either due to primary permeability or due to a network of closely spaced fractures acting an EPM. Superimposed on the closely spaced fractures are some large-aperture fractures. When these fractures have deadends or truncate at a perpendicular fracture, they can influence transport in the matrix by spreading the plume in the transverse direction, followed by continuing transport in the matrix along the spread-out front. Although the narrow plume at the WBCV site was not modeled, it provides further evidence of the importance of fracture geometry. At this site, the flow direction is the same as the dominant fracture orientation. Without the truncation of fractures in this direction, the plume was not spread in the transverse direction. A variety of fracture networks could result in similar plumes under a given set of hydraulic boundary conditions, but might behave differently from one another when these conditions are changed. The model is not yet valid as a predictive tool. Nonetheless, the contrast in plume geometry at the two sites discussed, and the modeling of BG4 with the broad plume, indicates the importance of fracture geometry in plume development through effects usually attributed to dispersivity. Thus, the simulations show that studies focussed on characterizing the major fractures provide important information for understanding plume behavior in fractured porous media. Acknowledgements These numerical simulations were an outgrowth of the extensive tracer test conducted by David Webster of the U.S. Geological Survey, and we gratefully acknowledge his efforts and willingness to share the results of his experiment. We also thank D. Kip Solomon and Dale Huff for bringing the data to our attention and for their assistance in the early stages of the project. References Balfour, D.J., 1991. Evaluation of lateral solute migration in surficial weathered clayey till. M.Sc. thesis, Univ. of Waterloo, Waterloo, Ontario, Canada. P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 99 Berkowitz, B., Bear, J., Braester, C., 1988. Continuum models for contaminant transport in fractured porous formations. Water Resour. Res. 24, 1225–1236. Bibby, R., 1981. Mass transport of solutes in dual-porosity media. Water Resour. Res. 17, 1075–1081. Brown, T., Toran, L., Solomon, D.K., Shropshire, R., Lee, R., Ketelle, R., 1992. Contaminant migration at a fractured test site on the Oak Ridge Reservation. American Geophysical Union Fall Meeting, San Francisco, Dec. 7–11, 1992. Cacas, M.C., Ledoux, E., de Marsily, G., Barbreau, A., Calmels, P., Galaillard, B., Margritta, R., 1990. Modeling fracture flow with a discrete network model: Calibration and validation 2. The transport model. Water Resour. Res. 26, 479–489. Clemo, T.M., Smith, L., 1989. Solute transport in fractured media: Dual permeability modes. EOS, 70Ž43.. Cook, P.G., Solomon, D.K., Sanford, W.E., Busenberg, E., Plummer, L.N., Poreda, R.J., 1996. Inferring shallow groundwater flow in saprolite and fractured rock using environmental tracers. Water Resour. Res. 32, 1501–1509. D’Astous, A.Y., Ruland, W.W., Bruce, J.R.G., Cherry, J.A., Gillham, R.W., 1989. Fracture effects in the shallow groundwater zone in weathered Sarnia-area clay. Can. Geotech. J. 26, 43–56. Day, J.J., 1977. Analysis of movement and hydrochemistry of groundwater in the fractured clay and till deposits of the Winnipeg area, Manitoba. M.Sc. thesis. Dep. of Earth Sci., Univ. of Waterloo, Waterloo, Ontario, Canada. Endo, H.K., Long, J.C.S., Wilson, C.R., Witherspoon, P.A., 1984. A model for investigating mechanical transport in fracture networks. Water Resour. Res. 20, 1390–1400. Foster, S.S.D., 1975. The chalk groundwater tritium anomaly: A possible explanation. J. Hydrol. 25, 159–165. Hancock, P., 1985. Brittle microtectonics: Principles and practice. J. Struct. Geol. 7, 437–457. Harrison, B., Sudicky, E.A., Cherry, J.A., 1992. Numerical analysis of solute migration through fractured clayey deposits into underlying aquifers. Water Resour. Res. 28, 515–526. Keller, C.K., van der Kamp, G., Cherry, J.A., 1986. Fracture permeability and groundwater flow in clayey till near Saskatoon, Saskatchewan. Can. Geotech. J. 23, 229–240. Lee, R.R., Ketelle, R.H., Bownds, J.M., Rizk, T.A., 1989. Calibration of a groundwater flow and contaminant transport computer model: progress toward model validation. ORNLrTM-11294. Oak Ridge National Laboratory. Lee, R.R., Ketelle, R.H., Bownds, J.M., Rizk, T.A., 1992. Aquifer analysis and modeling in a fractured, heterogeneous medium. Ground Water 30, 589–597. Long, J.C.S., Remer, J.S., Wilson, C.R., Witherspoon, P.A., 1982. Porous media equivalents for network of discontinuous fractures. Water Resour. Res. 18, 645–658. Long, J.C.S., Witherspoon, P.A., 1985. The relationship of the degree of interconnection to permeability in fracture networks. J. Geophys. Res. 90B, 3087–3098. Maloszewski, P., Zuber, A., 1985. On the theory of tracer experiments in fissured rocks with a porous matrix. J. Hydrol. 79, 333–358. Maloszewski, P., Zuber, A., 1993. Tracer experiments in fissured rocks: Matrix diffusion and the validity of models. Water Resour. Res. 29, 2723–2735. McKay, L.D., Cherry, J.A., Gillham, R.W., 1993a. Field experiments in a fractured clay till. 1. Hydraulic conductivity and fracture aperture. Water Resour. Res. 29, 1149–1162. McKay, L.D., Gillham, R.W., Cherry, J.A., 1993b. Field Experiments in fractured clay till. 2. Solute and colloid transport. Water Resour. Res. 29, 3879–3890. McKay, L.D., Stafford, P.L., Toran, L.E., in press. EPM modeling of a field-scale tritium tracer experiment in fractured, weathered shale. Ground Water. Moore, G.K., Toran, L.E., 1992. Supplement to a hydrologic framework for the Oak Ridge Reservation, Oak Ridge, Tennessee. ORNLrTM-12191. Oak Ridge national Laboratory. Olsen, C.R., Lowry, P.D., Lee, S.Y., Larsen, I.L., Cutshall, N.H., 1986. Geochemical and environmental processes affecting radionuclide migration from a formerly used seepage trench. Geochim. Cosmochim. Acta 50, 593–607. Pankow, J.F., Johnson, R.L., Hewetson, J.P., Cherry, J.A., 1986. An evaluation of contaminant migration patterns at two waste disposal sites on fractured porous media in terms of the equivalent porous medium ŽEPM. model. J. Contam. Hydrol. 1, 65–76. 100 P. Stafford et al.r Journal of Contaminant Hydrology 30 (1998) 79–100 Parney, R., Smith, L., 1995. Fluid velocity and path length in fractured media. Geophys. Res. Lett. 22, 1437–1440. Pollard, D.D., Aydin, A., 1988. Progress in understanding jointing over the past century. Bull. Geol. Soc. Am. 100, 1181–1204. Renshaw, C.E., 1996. Influence of subcritical fracture growth on the connectivity of fracture networks. Water Resour. Res. 32, 1519–1530. Rubin, H., Soliman, A.M., Birkohozer, J., Rouve, G., 1996. Transport of a tracer slug in a fractured permeable formation. J. Hydrol. 176, 153–180. Rubin, H., Buddemeier, R.W., 1996. Transverse dispersion of contaminants in fractured permeable formations. J. Hydrol. 176, 133–151. Ruland, W.W., Cherry, J.A., Feenstra, S., 1991. The depth of active groundwater flow in a clayey till plain in southwestern Ontario. Ground Water 29, 405–417. Sanford, W.E., Solomon, D.K., 1995. Noble gas solute tracer experiment in a fractured, weathered shale near Oak Ridge, TN. Presented at the International Association of Hydrogeologists Congress, Edmonton, Alta., June 5–10. Sanford, W.E., Shropshire, R.G., Solomon, D.K., 1996. Dissolved gas tracers in groundwater: Simplified injection, sampling, and analysis. Water Resour. Res. 32, 1635–1642. Schwartz, F.W., Smith, L., Crowe, A.S., 1983. A stochastic analysis of macroscopic dispersion in fractured media. Water Resour. Res. 19, 1253–1265. Shevenell, L.A., Moore, G.K., Dreier, R.B., 1994. Contaminant Spread and flushing in fractured rocks near Oak Ridge Tennessee. Ground Water Monit. Rev. 14, 120–129. Smith, L., Schwartz, F.W., 1984. An analysis of the influence of fracture geometry on mass transport in fractured media. Water Resour. Res. 20, 1241–1252. Smith, L., Schwartz, F.W., 1993. Solute Transport through fracture networks. In: Flow and Contaminant Transport in Fractured Rock. Academic Press, San Diego, CA, pp. 129–167. Solomon, D., Moore, G.K., Toran, L.E., Dreier, R.B., McMaster, W.M., 1991. Status report: A hydrologic framework for the Oak Ridge Reservation. ORNLrTM-12026. Oak Ridge National Laboratory. Stafford, P.L., 1996. Simulation of a field scale tritium tracer experiment in a fractured, weathered shale using discrete-fracturermatrix-diffusion and equivalent porous medium models. M.Sc. thesis, University of Tennessee, Knoxville. Sudicky, E.A., Frind, E.O., 1982. Contaminant transport in fractured porous media: Analytical solutions for a system of parallel fractures. Water Resour. Res. 18, 1634–1642. Sudicky, E.A., McLaren, R.G., 1992. The Laplace Transform Galerkin technique for large-scale simulation of mass transport in discretely fractured porous formations. Water Resour. Res. 28, 499–514. Therrien, R., Sudicky, E.A., 1996. Three-dimensional analysis of variably-saturated flow and solute transport in discretely-fractured porous media. J. Contam. Hydrol. 23, 1–44. Thompson, D., 1990. Hydraulic evidence of Wisconsinan-aged open fractures in a deep clayey till. M.Sc. thesis, University of Waterloo, Waterloo, Ontario, Canada. Van der Kamp, G., 1992. Evaluating the effects of fractures on solute transport through fractured clayey aquitards. Int. Assoc. of Hydrogeologists Congress, Hamilton, Ont., May 11–12, pp. 468–476. Webster, D.A., 1996. Results of Ground-Water Tracer Tests Using Tritated Water at Oak Ridge National Laboratory, Tennessee. U.S.G.S Water-Resources Investigations Report 95–4182. Wickliff, D.S., Gregory, S.M., Larsen, I.L., Clapp, R.B., 1989. Contaminant transport during storms near solid waste storage areas 4 and 5. ORNLrRAPrLTR-89r20. Oak Ridge National Laboratory. Zuber, A., Motyka, J., 1994. Matrix porosity as the most important parameter of fissured rocks for solute transport at large scales. J. Hydrol. 158, 19–46.
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