PHYSICS OF FLUIDS VOLUME 10, NUMBER 12 DECEMBER 1998 Silo hiccups: Dynamic effects of dilatancy in granular flow Thierry Le Pennec Department of Physics, University of Oslo, P.O. Box 1048, Blindern, 0316 Oslo 3, Norway and Groupe Matiére Condensée et Matériaux, Université de Rennes 1, F-35042 Rennes Cedex, France Knut Jo” rgen Målo” y and Eirik G. Flekko” y Department of Physics, University of Oslo, P.O. Box 1048, Blindern, 0316 Oslo 3, Norway Jean Claude Messager and Madani Ammi Groupe Matière Condensée et Matériaux, Université de Rennes 1, F-35042 Rennes Cedex, France ~Received 4 December 1997; accepted 19 August 1998! The granular flow through an open silo is investigated experimentally. A mechanism based both on the dilation of the granular medium and an interaction with the interstitial gas causes the flow to stop at regular intervals. The experiments are carried out at different surrounding pressures P 0 , and it is found that the intermittent flow becomes continuous at sufficiently low P 0 , showing that the intermittency is linked to the interaction the gas. The scaling of the average flow rate with particle size further supports our view of the gas-grain interaction. © 1998 American Institute of Physics. @S1070-6631~98!00912-X# allow the grains to pass by each other.12 This expansion, or dilation, will create more void space between the grains, thus leaving more room for the interstitial fluid. Depending on the time scale of the process, this in turn will lead to a local lowering of the pressure, and when there is a granular flow, this pressure drop will couple back on the motion of the grains. This effect is expected to be general. The main mechanism, as it is realized in the present experiment, is illustrated in Fig. 1. The sand, which starts out with approximately constant density, moves down as a block through the upper pipe until it reaches the constriction or shear zone. Here the sand must dilate in order to accommodate the shear which is caused by the deformation. The dilation ~expansion! will create a local pressure drop in the shear zone which causes both a drag force on the moving sand and an air flow into hopper. In the present experiment we propose that the pressure drop ~together with wall friction, which is always present! entirely stops the flow at a regular time interval T, as long as the ambient pressure is above a certain threshold value. The flow intermittency is caused by a periodic sucking in of air, hence the term ‘‘silo hiccups.’’ I. INTRODUCTION Granular materials exhibit several flow properties which are qualitatively different from what is observed in simple fluids. These differences are linked to the fact that moving granular materials may continuously change their behavior from that of solids to that of liquids or highly compressible gases, thus making general descriptions in terms of continuum equations notoriously difficult. Recent research has focused on dynamic studies of granular materials in confined geometries, a field of broad industrial importance.1 Examples of the complex and intriguing phenomena arising from the granular nature of these systems2 include shocklike density waves in hoppers3 and tubes,4,5 1/f noise,6 and pattern formation in the density profiles of sand flowing out of a hopper.3,7–9 A fundamental understanding of the detailed mechanisms governing these granular flows is still mostly lacking. In recent experiments periodic intermittency in the mass flow rate have been observed in closed ‘‘ticking’’ hour glasses10,11 where gas-grain interactions are a dominant mechanism. Gas-grain interactions are generally important when grains are small or the interstitial fluid sufficiently viscous. In the present paper we investigate the intermittent flow of grains from an open model silo. In contrast to the ‘‘ticking’’ hour glass, which is governed by the ~nonlocal! increase of a pressure difference between two closed chambers, the key mechanism behind the intermittency in the present experiments is local and linked to the dynamic dilation of the granular medium. As such, it is another uniquely granular phenomenon which has no analogue in simple fluids. The term dilatancy was first introduced by Reynolds12 in 1885. It is the effect seen when one steps on a wet beach and the sand appears to dry around the foot. In general when a granular medium is subject to a local shear it must expand to 1070-6631/98/10(12)/3072/8/$15.00 II. EXPERIMENTAL SETUP The experiments are illustrated in Figs. 2 and 3. The silo consists of a cylindrical upper part, open to the surrounding pressure at the top, with a conical edge with an orifice at the bottom. In contrast to experiments in straight tubes,4 the present phenomenon is easily observed as the constriction in the silo geometry ~the hopper! serves to fix its location and scale. This allows for precisely controlled visual observations and pressure measurements. The silo was filled with spherical glass beads with diameters ranging from 35 mm to 1 mm. To obtain the same porosity f 0 50.3860.01 of the different powders, the silo 3072 © 1998 American Institute of Physics Downloaded 21 Jun 2006 to 129.240.250.104. Redistribution subject to AIP license or copyright, see http://pof.aip.org/pof/copyright.jsp Le Pennec et al. Phys. Fluids, Vol. 10, No. 12, December 1998 3073 FIG. 1. A sketch illustrating the proposed effect. The sand moves down as a block through the upper pipe until it reaches the shear zone. Here a local pressure drop caused by the dilation of the sand causes air to be sucked into the shear zone from the surroundings with an upward velocity relative to the moving grains. was tapped carefully on the sidewalls. The height of the silo is 600 mm, with an internal diameter of D t 516 mm, and 30 mm. Experiments were performed with silos of different conical angle 2 a 5180°, 19°, 14°, and 10°. The silos were made of brass, Plexiglas, and glass with a diameter of orifice D ranging from 2 to 15 mm. The silos made of brass have the advantage of preventing electrostatic charges. The importance of electrostatic interactions was further investigated by performing experiments with silver coated particles. No qualitative difference was observed in these experiments. The experiments were all done under dry conditions with a relative humidity within the range 20%–40%. In order to visualize the detailed movement of the sand in the vicinity of the orifice, a transparent glass silo with FIG. 3. Sequence of images which show the granular flow at the orifice within one oscillation. Images 1, 2, and 3 show an interface ~separation between the dense and dilute zone! which moves up. Images 4, 5, 6, and 7 show the the collapse of this interface followed by a strong increase in the flow rate. Images 8 and 9 show the flow just before it stops. conical angle 2a of 10° was used together with a video camera. III. INTERMITTENCY CYCLES FIG. 2. Drawing of the hopper with the laser and the photodetectors ~PD!. D is the orifice diameter, D t the diameter of the cylindrical part, h the height, and 2a is the opening angle of the conical part. We now describe one of the flow intermittency cycles which is shown in Fig. 3. The particles were observed to fall from the closely packed phase at the lower interface seen in Fig. 3. In image 1, when the interface is localized at the orifice, the absence of powder just below suggests that the flow is completely stopped for a short time. This is also easily seen in a direct video visualization, where a somewhat smeared video image of the grains becomes sharply con- Downloaded 21 Jun 2006 to 129.240.250.104. Redistribution subject to AIP license or copyright, see http://pof.aip.org/pof/copyright.jsp 3074 Le Pennec et al. Phys. Fluids, Vol. 10, No. 12, December 1998 FIG. 4. The intensity at the top ~a! and bottom ~b! photodetectors as a function of time. The integers correspond to the images in Fig. 3. trasted for about 0.05 s. Just after this stop the front between the falling particles and the closed packed region propagates upward in the conical part ~images 2 and 3! until it collapses ~image 4!. In general, the speed with which the front moves upward will depend on the force networks in the packing, the weights of the grains, and the hydrodynamic drag force acting on the particles. After the interface reaches the critical height were it collapse and suddenly falls down ~images 4 and 5!, a significant increase in the mass flow rate ~images 5, 6, and 7! is observed. The strong increase in the mass flow rate is followed by a decrease in the width of the powder beam which finally snaps off ~images 8 and 9!. The correlations between the movement of the sand in the vicinity of the orifice and at the top surface was studied using two 5-mW He–Ne lasers with expanded beams as shown in Fig. 2. The upper laser beam was partly screened by the upper granular surface, and the transmitted intensity, measured by photo-diode PD1 @see Fig. 4~a!#, is thus linearly related to the height of the interface of the sand. At the conical opening we measured the transmitted intensity of an expanded laser beam passing through the conical part of the silo @Fig. 4~b!#. Due to a more efficient screening of the light by the dense packing than from the free falling particles, the recorded intensity decreases when the interface moves down. The increase in the slope of curve ~a! starts at the same time as a fast decrease in curve ~b! in Fig. 4. This corresponds to image 4 in Fig. 3 and shows that the upper and lower interfaces start to move down simultaneously. The upper interface will continue to move quickly, with a corresponding outflow, for a short time after the lower interface has reached the height of the orifice ~images 6–8!. In this period the lower signal does not directly reflect the flow velocity, but rather the filling of the constriction. Just before the lower interface, which is observed in images 1–4 in Fig. 3, starts to move upward there is a short stop in the bulk movement as described above. This is too short to be observed in these measurements, but can be seen in the video visualization experiments. In the visualization experiments no bubble formation10 was observed in or above the conical part of the silo. After the stop the lower interface starts to move upward in the conical part until the interface again reaches a height where it collapses. In this part the upper interface is moving only slowly, as seen in the low slope of FIG. 5. The average flow rate ^W& ~s! and the period T ~d! of the intermittency as a function of the ambient pressure P 0 in units of the atmospheric pressure P a . curve ~a! in Fig. 4. The fluctuations in the high levels of curve ~b! in Fig. 4 reflect the fluctuations in the particle flow from the interface. IV. QUANTIFICATION AND DISCUSSION As will be seen below the intermittency is governed by internal pressure gradients which can only arise from variations in the density of the granular packing. In order to argue that the intermittency is really due to dynamic dilation, we need to rule out other mechanisms of interior expansion in the granular packing. The simultaneous motion of the upper and lower interfaces as deduced from Fig. 4, and the lack of observed bubbles, support the picture that the grain packing in the tube moves without expansion. Furthermore, the tube walls will exert a stronger vertical force per unit area on the granular packing in the constriction than above. Hence, there is no mechanical reason for the packing to open up or form bubbles as it moves down into the constriction. The final dilation due to shearing in the constriction cannot be avoided. A. The pressure evolution and the critical pressure To investigate the importance of the ambient pressure on the flow, we performed experiments in a chamber with a reduced ambient pressure P 0 . In these experiments we used d550 m m particles, and 2 a 5180°. As seen in Fig. 5, both the flow rate ^W&, averaged over the entire duration of the flow, and the period T between stops in the granular flow were roughly constant for pressures higher than 0.2 bar. When the pressure becomes lower than a critical pressure P c 50.1 bar, a transition from the intermittent to a continuous flow regime was observed. Correspondingly the period T diverges and the flow rate ^W& increases by nearly a factor of 2. In Fig. 5 both the remarkable constancy of the period and the flow rate over different pressures, and the pronounced transition from intermittent to continuous flow are striking, and in need of an explanation. To investigate the gas-grain interactions in more detail, the average pressure difference d P between the local pres- Downloaded 21 Jun 2006 to 129.240.250.104. Redistribution subject to AIP license or copyright, see http://pof.aip.org/pof/copyright.jsp Le Pennec et al. Phys. Fluids, Vol. 10, No. 12, December 1998 sure in the constriction and the ambient pressure was measured. The measurements were carried out using a pressure sensor connected to a small hole at a height D55 mm above the orifice of a hopper with opening angle 2 a 510°. The surrounding pressure was 1 bar. For small particles, as used here, the pressure drop building up between stops in the flow was measured as d P'0.001 bar' r gD, where r is the mass density of the granular packing and g is the acceleration of gravity. Hence, in the intermittent regime the pressure drop d P was observed to balance the weight of the particles occupying a region of linear dimension D above the orifice. In fact, for the observed halt of granular motion to take place, the pressure drop must be able to support the weight of the grains in the orifice for a short time. This can be used to estimate the critical pressure P c . The dilatancy, measured as the specific expansion d V/V, will cause a pressure drop that depends only on the compressibility of the gas. Lowering P 0 , the gas will eventually be so compressible that the pressure force resulting from the expansion of the gas inside the orifice is unable to balance the weight of the falling grains. Using the ideal gas law for isothermal gas expansion to get the pressure drop we can write 2 d P/ P 0 5 d V/V @an adiabatic expansion, would only lead to the replacement d V/V →(5/3) d V/V#. To obtain the critical value P 0 5 P c we set d P5 r gD in the above equation. This gives directly P c 5 r gD/( d V/V). To get an estimate of d V/V, as it results from the reconfigurations of the grains, we carried out an independent measurement. A funnel with the narrow pipe pointing up, closed on the wide bottom end with an elastic rubber membrane, was filled with grains. The funnel was then filled with water. Pushing the membrane from the bottom a dilatancy d V/V51% – 2% was obtained from the observation of the sinking water in the top pipe. Using this result in the above equation we get directly that P c '(100– 200) r gD'(0.1– 0.2) bar. This estimate is perhaps in better agreement with the observed value of P c ~Fig. 5! than could be expected. Note that the choice of the size of the volume, defined by D, over which the pressure falls is rather arbitrary. The above estimate of P c only considers the pressure force needed to balance the weight of the grains at the orifice, and not the forces needed to overcome the inertia of the grains. To understand the process that stops the granular outflow, one must consider the granular inertia and the time over which the pressure forces act. Moreover, as the granular medium is continuously deformed as it passes through the orifice, the dilatancy must also be considered as a dynamic process, as in the study of Lee et al.8 For this purpose we need a pressure evolution equation. Assuming that the gas is isothermal one may derive the following equation f S D S D ]P k 1u•¹ P 5¹• f P ¹ P 2 P¹•u. ]t m ~1! Here f is the local porosity, u the grain velocity, k the ~density dependent! permeability, and m the viscosity of the air. The above equation is derived from the mass conservation equations of the gas and the grains and a local Darcy law in 3075 the Appendix. The two terms on the left hand side taken together are simply the material derivative of the pressure ~multiplied by f!. They describe the time rate of change of the pressure in a local reference frame that moves with the sand. The first term on the right hand side is a diffusive term describing the Darcy flow. The second term on the right hand side is a source term that describes the pressure increase due to compression of the void space in the granular packing. The permeability k may be related to f by the so-called Carman Cozeny expression,13 which has the following form: k ~ r̂ s ! 5 f3 a2 . 45 ~ 12 f ! 2 ~2! This is the well-studied relation, which is known to hold relatively well for random packings of spheres, as long as the packing density is not too small. The effective diffusion coefficient D̂[ P k~ f ! P 0k~ f 0 ! ' , m m ~3! where f 0 '0.4 is the closed pack porosity, may thus be evaluated. Using the particle radius a525 m m and taking P to be the atmospheric pressure and m the viscosity of air, we find D̂'100 cm2/s. The different terms in Eq. ~1! may thus be evaluated when ¹ is replaced by an inverse characteristic distance, which we take to be D. This gives S ¹• f 0 D k0 D̂ ¹ P ' 2 P'1000 s21 P, m D u P¹•u'u•¹ P' P'10 s21 P, D ~4! where we used D50.3 cm and we have evaluated u from the measured values of the average flow rate W. The diffusive term is then seen to dominate the terms containing u in Eq. ~1!. By dropping these terms we are left with a simple diffusion equation describing the evolution of P. The characteristic diffusion time over a distance D, t D 5D 2 /D̂'0.5 ms is almost two orders of magnitude smaller than the time a grain spends in passing a distance D at the orifice. If one knew the instantaneous pressure drop D P inside the dilating regions, it would then be possible to check if the pressure forces alone were sufficient to stop the flow. This could be achieved by comparing the necessary momentum change r D 3 u with the impulse D PD 2 t D at the orifice. Taking D P as the measured value d P described above ~which is smaller than the real value since the measured value results from some diffusive smearing!, the impulse is too small to balance the momentum change by roughly a factor of 10. However, it is likely that a series of dilatancy events is responsible for the stopping of the flow. This is consistent with the picture of a series of discrete shear bands reported by Lee et al.8 In a radiographic study of hopper outflow ~with weak gas interaction! they observed that during the flow the dilating regions form in series of narrow bands. These bands, which form in the constriction, have an angle of 45 degrees to the flow direction. The fact that granular packings dilate and form shear bands when flowing out of a hopper has been Downloaded 21 Jun 2006 to 129.240.250.104. Redistribution subject to AIP license or copyright, see http://pof.aip.org/pof/copyright.jsp 3076 Le Pennec et al. Phys. Fluids, Vol. 10, No. 12, December 1998 FIG. 6. A qualitative picture showing how the various forces acting on the sand in the constriction are correlated with the velocity u there. Here f is the friction force from the walls, r g is the gravity force per unit volume and D P the pressure difference between the inside and the outside of the constriction. The integers correspond to the images in Fig. 3. observed by several authors.3,7–9 While these observations are all, in a way, concerned with dynamic effects of dilatancy, they did not include the coupling of hydrodynamics and granular dynamics studied here. While Eq. ~1! does not give a definite magnitude of the pressure impulse, it does indicate an explanation for the pressure independence of T and W in the intermittent regime. Assume that the stopping process is governed by a series of dilation events. Each such event will have a certain pressure drop D P depending on the local expansion of the packing, and D P will relax diffusively over a time t D . The impulse is proportional to D Pt D . The relaxation time t D }1/D̂}1/P 0 . The pressure drop D P, on the other hand, will be proportional to the relative granular density change in the dilatancy process, i.e., D P} P 0 D r / r if the process happens on a faster time scale than t D . In this case the impulse and the momentum change associated with each dilatancy event will be P 0 independent as the P 0 dependence in t D cancels the P 0 dependence in D P. When t D becomes too large, so that the impulse D Pt D is dominated by the impulse of gravity during the period T, the flow becomes continuous. This will eventually happen as P 0 is decreased. In principle this could be used to compute P c . However, t D goes as the square of the distance between the opening and the dilatancy event. This distance is not well known, and such a computation would therefore be highly unreliable. Figure 6 summarizes our picture of the forces acting on the granular material in the constriction and their correlation with the local average of the velocity u in the constriction. The forces are taken as forces per unit area, and they are the gravity ( r gD), the friction f from the walls, and finally the pressure drop D P. The latter is the most important force for the stopping of the flow. Due to the finite diffusive relaxation time t D , the pressure force will remain finite even as the velocity goes to zero. In the figure the dashed line shows how further relaxation of the pressure may have proceeded if the granular motion had not started again. The friction force f will, in general, fluctuate strongly and also depend on the density. It will, in general, have a larger static than dynamic value, and when the flow is at rest, arching effects between the grains will transfer friction forces over many grain diameters. These effects are illustrated by the steps in the friction force associated with vanishing u. However, this sudden increase cannot explain the stopping process of the flow since it does not set in before after the flow has stopped. Moreover, we have no reason to expect that r gD or f depends on the background pressure P 0 . The observation that the flow becomes continuous and never stops when P 0 is below its critical value thus indicates that the pressure force is crucial in stopping the flow. To test the dependence of the period T on the initial compactification, experiments were performed for two different porosities f 50.38 and f 50.44 ~using d551 m m particles!. A shorter period was observed for the more compactified than the less compactified powder. For the more compact powder T50.17 s while T50.24 s for the the less compact powder. This is in qualitative agreement with what we expect, since the compactified powder will have to expand more by dilatation than the less compact powder, thus creating a larger pressure drop. This means that fewer dilatency events should be required to stop the flow. However, the change in T is likely to also reflect changes in intergranular friction, grain-wall friction and changes in the location and magnitude of the pressure-dilatency coupling. Hence, while there is a basis for predicting the sign of the effect, a good quantitative theory appears out of reach. B. Possible effects of molecular discreteness An isothermal decrease in pressure could affect both the compressibility and the mobility k/m of the gas. The intergrain spacing is only about 20 times larger than the mean free path at the lowest pressures, and the hydrodynamic description will receive significant corrections due to the molecular nature of the gas.14,15 Klinkenberg modeled the correction due to the wall-slip gas flow in an idealized porous medium consisting of capillary tubes with random orientation, and found that the velocity wall-slip results in a correction term in the permeability14,15 k 8 5 k ~ 118cl/b ! . ~5! Here k is the permeability measured by liquid flow, where finite mean free path effects are supposed to be negligible, l is the mean free path of the gas, b is the pore size, and c is a constant, which is experimentally determined to be close to unity. As an estimate we will use b5d/3, where d is the particle size. The mean free path of the gas molecules is estimated to 0.08 mm at P 0 51 bar. This gives the correction term k 8 / k 51.04 at P 0 51 bar, and k 8 / k 51.4 at P 0 50.1 bar. It is possible that the crossover behavior of T near P c is governed by the effect that the impulse D Pt D decreases with increasing k 8 . The critical pressure P c is in the pressure range where the Klinkenberg effect Eq. ~5! is expected to be important. However, while t D should depend on the Klinkenberg effect, the pressure force resulting from a given dilatancy will not. Downloaded 21 Jun 2006 to 129.240.250.104. Redistribution subject to AIP license or copyright, see http://pof.aip.org/pof/copyright.jsp Phys. Fluids, Vol. 10, No. 12, December 1998 FIG. 7. The flow rate W5W a as a function of the particle diameter d on a log–log scale for the hopper angles 2 a 510°(s), 14°~n!, 19°~1!, 180°~h!. The insert shows the mass flow rate W as a function of the column height h for particle diameter d589 m m. Curve ~b! corresponds to a slight compactification of the packing relative to curve ~a!. This means that while molecular discreteness may affect the value of P c , it has no consequence for our interpretation that dilatancy created pressures stop the flow. C. Dependence on particle size and hopper opening diameter To investigate the particle size dependence of the flow, we used powders consisting of spherical glass beads with diameters ranging from 35 mm to 1 mm. To obtain the same porosity f 0 50.3860.01 of the different powders, the silo was tapped carefully on the side-walls. Figure 7 shows the asymptotic mass flow rate W a normalized with r as a function of particle size d. The insert in Fig. 7 shows how the average flow rate depends on the height of the granular column. The asymptotic flow rate W a is the time averaged flow rate corresponding to the h→` limit. The two curves in the insert correspond to slightly different initial states of the packing. For the upper curve the system was more loosely packed with a porosity f which is 8% larger than f 0 . As seen in the insert, the effect of this initial difference in compactification lasted almost throughout the experiments. This again indicates that the grains move coherently as a solid block relative to the smooth silo walls. To confirm this point, experiments with porosity f 0 were also performed with smaller initial filling heights. No changes in the subsequent mass flow rate W(h) were observed relative to the larger filling heights. This shows that the initial porosity is conserved in the packing as it moves down the main part of the tube. For flows of large particles that are not governed by interaction with the gas, the flow rate W is independent of the column height h until the upper interface reaches the conical part of the silo.16 In the present case, however, the small particle flow rate is observed to vary with h at much larger h values. This effect is assumed to be hydrodynamic. It is caused by the air coming in from the top, thus decreasing the pressure difference at the opening when h becomes sufficiently small. When the particle flow is controlled by inertia of the particles rather than drag forces, the flow rate is Le Pennec et al. 3077 d-independent.1,17 Figure 7, on the other hand, shows that in the intermittent (d,100 m m) regime the flow is consistent with W}d 2 , where d is the particle diameter. The data collapse observed for W a in the intermittent regime over different hopper angles is rather striking as it indicates that the gas-grain interactions are unaffected by the hopper angle a. It is well known from hopper experiments that stagnant zones will form near the outlet.3 In these zones which form along the inclined walls, there is no particle motion. It has been found that the distance d c from the opening to the stagnant zone scales as d c ; a 22.2. 3 The length of the inclined section measured from the hopper opening to the bottom of the vertical cylinder walls, l, goes as l;1/a for small a. At a sufficient small angle d c will become larger than l, and the stagnant zone will disappear. In the continuous flow regime, it is seen from Fig. 7 that the volume flow rate becomes constant for angles smaller than a 515°. This indicates pure ‘‘mass flow’’ with no stagnant zones. For larger angles the volume flow rate was found to decrease with increasing a as seen in Fig. 7. This decrease is probably due to the fact that the stagnant zones form boundaries that are effectively rough, whereas the walls are smooth. Hence a larger friction is felt from the boundaries of the stagnant regions than from the smooth walls. Our observations are consistent with the prediction by Rose and Tanaka.18 In the oscillatory, gas dominated regime the volume flow rate was found to be quite insensitive to the hopper angle. This is somewhat surprising, since a should affect both friction forces and the local volume over which the pressure may relax. However, for nonsteady flows little is known about the stagnant zones, and one must be careful in interpreting the nonsteady results in terms of the time-independent picture. For particles larger than 100 mm, a slight decrease in particle flux with particle size is observed. This decrease can be explained by an effective reduction in the orifice diameter D→(D2bd), where b is a dimensionless constant between 1 and 3.1 The W}d 2 behavior in the intermittent regime can be justified by the following argument. When the particles are small the drag forces will control the granular outflow. If the column is sufficiently high such that the main air flow takes place through the orifice, the slip velocity v a 2 v p between the speed of the air v a and the local speed of the particles v p will be proportional to v p . This follows under the assumption that the dilatancy expansion rate is proportional to the volume flux of grains. The particle velocity then follows from the local Darcy law v p } v a 2 v p 5 k ( f ) r g/ m , where k ( f ) is the permeability of the packing and m is the dynamic viscosity of the air. Since in general we have k}d 2 , we get the mass flow rate W} v p D 2 }d 2 D 2 , in agreement with the measurements of Fig. 7. The dependence of the mass flow rate on D 2 has been checked in separate small particle experiments using different diameters of the orifice D, as seen in Fig. 8. As seen in Fig. 8 the mass flow rate is consistent with D 2 dependence. Downloaded 21 Jun 2006 to 129.240.250.104. Redistribution subject to AIP license or copyright, see http://pof.aip.org/pof/copyright.jsp 3078 Le Pennec et al. Phys. Fluids, Vol. 10, No. 12, December 1998 ments and valuable input during the writing of the manuscript. This work has been in part supported by the CNRS and the NFR through a Programme International de Coopération Scientifique grant. APPENDIX: DERIVATION OF THE PRESSURE EQUATION Here we derive Eq. ~1! from the conservation of granular mass and gas mass, using the assumption of an isothermal gas to relate the gas density and gas pressure. The conservation of the granular mass density r s may be written ]r̂ s 1¹• ~ r̂ s u! 50, ]t FIG. 8. The dependence of W a / r on the diameter of the orifice. V. CONCLUSION In conclusion we summarize the essential argument of the paper. By enclosing the hopper, sketched in Fig. 2, in an airtight chamber where the pressure could be varied, we were able to observe that the granular flow exhibits a crossover from intermittent to continuous flow at a critical ambient pressure P c . This made it clear that the intermittency is governed by internal pressure gradients. In the absence of an externally imposed pressure differences ~the silo is open in both ends!, these pressure gradients can only arise from variations in the density of the granular packing. The question we addressed was if these density variations could be caused by any other effects than the dilatancy we know must take place in the constriction of the hopper. Spontaneous formations of air bubbles would represent such an alternative mechanism for density variations. However, our observations strongly support that prior to the stopping of the flow, the granular packing moves as a single rigid object with the exception of the deformation in the hopper region. Hence, no alternative mechanisms appear active, and we are left with the interpretation that it is the local pressure drop caused by the dilatancy that stops the flow. This argument has been substantiated by experimental measurements. By comparing terms in the pressure evolution equation ~1! it was found that relaxation of the pressure gradients was mainly diffusive. This was used to explain the observed pressure independence of the period T. From a practical point of view, the understanding of the flow of granular materials with interstitial gas is important for designing durable and efficient silos. Using a silo geometry we have examined the rather complex granular dynamics in the outflow of a model silo. Of possible practical utility is the data collapse of Fig. 7 which shows that the small particle flow rate is rather independent of hopper angle. Moreover, Fig. 5 demonstrates how the outflow of a hopper may be increased by roughly a factor of 2 by lowering the pressure. ACKNOWLEDGMENTS It is a pleasure to thank Bob Behringer, Daniel Bideau, Alex Hansen, Steve Pride, and Erik Skjetne for helpful com- ~A1! where u is the granular velocity and the density compacity r̂ s 5 r s / r g has been normalized by the density r g of the material in the grains. Hence r̂ s 512 f where f is the porosity. The conservation of the gas mass density r a may be written S F ]r a k ~ r̂ s ! 1¹• r a u2 ¹P ]t m GD 50. ~A2! Here the air current has both an advective term caused by the motion of the grains, and a diffusive term describing the Darcy flow in the local rest frame of reference for the sand. The permeability k is given as a function of f s in Eq. ~2!. By using the relation r̂ s 512 f in Eq. ~A1! we get 2 ]f 1¹• ~~ 12 f ! u! 50. ]t ~A3! Using the isothermal equation of state for an ideal gas, r a } f P, we can write Eq. ~A2! in the form S F ]~ f P ! k 1¹• f P u2 ¹ P ]t m GD 50. ~A4! Eliminating ] f / ] t between Eq. ~A4! and Eq. ~A3! gives P¹•u2 P¹• ~ f u! 1 f S D ]P k 1¹• ~ f Pu! 2¹• f P ¹ P 50. ]t m ~A5! The sum of the second and the fourth terms of Eq. ~A5! equals f u•¹ P, which gives f S D S D ]P k 1u•¹ P 5¹• f P ¹ P 2 P¹•u, ]t m ~A6! which is nothing but Eq. ~1!. This ends our derivation. R. M. Nedderman, Static and Kinematic of Granular Materials ~Cambridge University Press, Cambridge, 1992!. 2 D. Bideau and A. Hansen, Disorder and Granular Media ~Elsevier, Amsterdam, 1993!. 3 G. W. Baxter and R. P. Behringer, ‘‘Pattern formation in flowing sand,’’ Phys. Rev. Lett. 62, 2825 ~1989!. 4 T. Raafat, J. P. Hulin, and H. J. Hermann, ‘‘Density waves in dry granular media falling through a vertical pipe,’’ Phys. Rev. E 53, 4345 ~1996!. 5 G. Peng and H. J. Herrmann, ‘‘Density waves of granular flow using lattice gas automata,’’ Phys. Rev. E 47, 1796 ~1994!. 6 K. L. Schick and A. 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