Chapter4- Nuclear Chain Reaction CHAPTER 4 The Nuclear Chain Reaction A. Dokhane, PHYS487, KSU, 2008 1 Chapter4- Nuclear Chain Reaction 1. 2. 3. 4. 5. 6. 7. Review Neutron Reactions Nuclear Fission Thermal Neutrons Nuclear Chain Reaction Neutron Diffusion Critical Equation A. Dokhane, PHYS487, KSU, 2008 2 Chapter4- Nuclear Chain Reaction Lecture content: • Introduction • Neutroncycleandmultiplicationfactor • TheThermalutilizationfactor • Neutronleakageandcriticalsize • Nuclearreactorsandtheirclassification k∞ • Calculationofforhomogeneousreactor A. Dokhane, PHYS487, KSU, 2008 3 Chapter4- Nuclear Chain Reaction 5.1 Introduction Nuclear chain reaction is a central theme for reactor physics Question: What is Nuclear Chain Reaction? Answer: Answer self-sustained process that, one started, needs no additional agents to keep it going Goals of this chapter : 1. follow the life of a group of Neutrons and develop a numerical criterion for a nuclear chain reaction to be possible and 2. apply it to various types of nuclear reactors. A. Dokhane, PHYS487, KSU, 2008 4 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor Question: When a self-sustaining chain reaction is possible? Answer: Answer ifν , the number of neutrons released per fission, is sufficiently greater than 1 Why? to compensate for neutron loss due to a variety of causes A. Dokhane, PHYS487, KSU, 2008 5 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor However, However ν is a constant of nature for a given fissionable material and, therefore, It is beyond human control, the only alternative is to reduce the various causes which are responsible for the loss of neutrons in a given assembly. A. Dokhane, PHYS487, KSU, 2008 6 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor Consider now, a natural uranium assembly in which some fission reactions have been initiated Let us follow the life of a typical neutron from the instant of its creation as a fast fission neutron listing the various possible events that may occur during its lifetime. 1. Neutron may be absorbed by U238 while its energy is still greater than the threshold energy for U238 fission and it may cause a fission of a U238 nucleus. 2. It may be absorbed by U238 without leading to a fission (radiative capture). This most likely to happen for neutron whose energy has been reduced by elastic collisions to the epithermal region (from 1000 ev to 5 ev), where U238 has pronounced absorption resonance. A. Dokhane, PHYS487, KSU, 2008 7 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor 3. It may be absorbed by a U235 nucleus causing a fission. 4. It may be absorbed by U235 nucleus without causing fission. 5. It may be absorbed by other materials and impurities that are part of the assembly without causing a fission. 6. It may escape from the assembly and be lost by what is called “leakage”. A. Dokhane, PHYS487, KSU, 2008 8 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor Events (1) and (3) are positive contributions to the neutron economy Create new neutrons events (2), (4), (5), and (6) are negative contributions Remove available neutrons from the assembly A. Dokhane, PHYS487, KSU, 2008 9 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor Assume we start with n0 fast neutrons which have just been produced in a uranium assembly. A part causes fissions in U238 (event 1) consequent increase in the number of fast neutrons this small increase by means of a factor ε > 1 , called the fast fission factor. The number of neutron after this event is: A. Dokhane, PHYS487, KSU, 2008 n0 ⋅ ε 10 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor The energy of the fast neutrons is being reduced steadily by collisions with the other nuclei in the assembly until they eventually enter the epithermal energy region The epithermal energy region has strong U238 absorption resonances Some of the neutrons will be absorbed by U238 (event2), whereas most of them will escape resonance absorption. The number of neutrons that will pass through this region without being absorbed n0εp where p resonance escape probability A. Dokhane, PHYS487, KSU, 2008 11 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor These neutrons will then reach thermal energies They may be either absorbed by U235 (events 3 and 4) or absorbed in other materials (event 5) The fraction of thermal neutrons absorbed by the fuel as compared to all thermal neutron absorption in the assembly is called the thermal utilization factor f. the number of thermal neutrons that actually absorbed by the fuel: n0εpf A. Dokhane, PHYS487, KSU, 2008 12 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor the number of thermal neutrons that actually absorbed by the fuel: n0εpf This number of thermal neutron absorptions will yield a number of fast fission neutrons That is η times as large Starting with an initial number of fast neutrons n0, a new generation of fast neutrons is obtained whose total number is n0 εpfη reproduction or multiplication factor = A. Dokhane, PHYS487, KSU, 2008 Final number of fast neutrons = εpfη Initial number of fast neutrons 13 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor Final number of fast neutrons = εpfη reproduction or multiplication factor = Initial number of fast neutrons k ∞ = εpfη The expression fourfour-factor formula Final number of fast neutrons = εpfη Initial number of fast neutrons can be interpreted as the ratio of thermal neutrons created per second to the number of thermal neutrons destroyed per second A. Dokhane, PHYS487, KSU, 2008 14 Chapter4- Nuclear Chain Reaction 5.2 Neutron Cycle and Multiplication Factor n0 εpfη n0 n0 ⋅ ε n0εpf A schematic picture of the neutron cycle A. Dokhane, PHYS487, KSU, 2008 n0εp 15 Chapter4- Nuclear Chain Reaction 5.3 The thermal Utilization Factor When defining f, we conventionally consider uranium mixture as the fuel, although the thermal neutrons can produce fission with the U235 component only We must then also use the numerical value for η which applies to the uranium mixture For the natural mixture η = 1.34 Thus if σ stands for the thermal absorption cross sections and the suffix i referring to all non uranium materials and impurities and employing an obvious notation, we can write for a natural uranium fuel mixture that f ( nat ) = N 0 ( 235)σ ( 235) + N 0 ( 238)σ ( 238) N 0 ( 235)σ ( 235) + N 0 ( 238)σ ( 238) + N oiσ i the total number of thermal neutron absorptions in the assembly represents the thermal neutron absorptions by the two uranium isotopes only A. Dokhane, PHYS487, KSU, 2008 16 Chapter4- Nuclear Chain Reaction 5.3 The thermal Utilization Factor Also we have η ( nat ) σ f ( nat ) = ν ( 235) σ a ( nat ) = Multiplying f ( nat ) = N 0 ( 235)σ f ( 235)ν ( 235) N 0 ( 235)σ a ( 235) + N 0 ( 238)σ a ( 238) N 0 ( 235)σ ( 235) + N 0 ( 238)σ ( 238) N 0 ( 235)σ ( 235) + N 0 ( 238)σ ( 238) + N oiσ i η ( nat ) f ( nat ) = A. Dokhane, PHYS487, KSU, 2008 and = N 0 ( 235)σ f ( 235)ν ( 235) N 0 ( 235)σ a ( 235) + N 0 ( 238)σ a ( 238) N 0 ( 235)σ f ( 235)ν ( 235) N 0 ( 235)σ a ( 235) + N 0 ( 238)σ a ( 238) + N 0iσ i 17 Chapter4- Nuclear Chain Reaction 5.3 The thermal Utilization Factor Considering only the U235 portion of the natural uranium mixture as the fuel, we have f ( 235) = η ( 235) N 0 ( 235)σ a ( 235) N 0 ( 235)σ a ( 235) + N 0 ( 238)σ a ( 238) + N 0iσ i σ f ( 235) = ν ( 235 ) σ a ( 235) η ( 235) f ( 235 ) = N 0 ( 235)σ f ( 235 )ν ( 235) N 0 ( 235 )σ a ( 235 ) + N 0( 238 )σ a ( 238) + N 0iσ i η ( nat ) f ( nat ) = η ( 235) f ( 235) A. Dokhane, PHYS487, KSU, 2008 18 Chapter4- Nuclear Chain Reaction 5.4 Neutron Leakage and Critical Size In the preceding derivation of the multiplication factor we omitted completely the possibility of leakage from the assembly (event 6) we assumed zero leakage during the neutron cycle Question: When this assumption is valid? Answer: valid with an infinite size for the assembly, hence there will be no leakage of neutrons from the system That is why we denoted the multiplication factor by k∞ For an assembly of finite size, the effective reproduction constant k eff will be less than k ∞ by a factor L (L<1), which is determined by the neutron leakage from the system: k eff = k ∞ L A. Dokhane, PHYS487, KSU, 2008 19 Chapter4- Nuclear Chain Reaction 5.4 Neutron Leakage and Critical Size L = l f l th lf : fast neutron non-leakage factor lth : thermal neutron non-leakage factor This separation is suggested by the diffusion theory, which treats the diffusion of fast neutrons and that of thermal neutrons separately k eff = k ∞ l f l th keff is the ratio of the number of neutrons in successive generation This self-multiplication of neutrons is the essential feature of a nuclear chain reaction A. Dokhane, PHYS487, KSU, 2008 20 Chapter4- Nuclear Chain Reaction 5.4 Neutron Leakage and Critical Size Question: what does the magnitude of keff represent? Answer: the speed with which the number of neutrons builds up and the rate at which nuclear fissions occur in the assembly Example: in a nuclear bomb type assembly, this build-up must take place very rapidly in industrial and research reactors this self-multiplication must be slow enough to allow the fission rate to remain always under the control of the operator For k eff > 1 , the assembly continues to produce more neutrons than it consumes and is then said to be supercritical. For k eff < 1 , fewer neutrons are produced than are consumed. Such an assembly is said to be subcritical. For k eff = 1 , the rate of neutron production is exactly balanced by the rate of neutron consumption and, in this case, the assembly is called a critical one. A. Dokhane, PHYS487, KSU, 2008 21 Chapter4- Nuclear Chain Reaction 5.4 Neutron Leakage and Critical Size Question: What is the critical size of an assembly? Answer: If we start with an assembly for which k eff > 1 , we can decrease k eff by progressively reducing the reactor size, thereby increasing the neutron loss through leakage from the assembly. If this reduction in the dimensions of the assembly is continued until k eff = 1 , the reactor size of the assembly at that point is called its critical size the critical size of an assembly is that size for which the rate of neutron loss due to all causes is exactly equal to the rate of neutron production in the assembly. A. Dokhane, PHYS487, KSU, 2008 22 Chapter4- Nuclear Chain Reaction 5.4 Neutron Leakage and Critical Size The fundamental problem in the design of a nuclear reactor is to obtain an assembly with k eff > 1 . As a first step to this end, k ∞ must be calculated and then, by introducing the finite size and geometry of the reactor, k eff can be calculated from the layout and dimensions of the reactor. Although this plan of action is very straightforward, the actual mathematical work involved can be very complex. Of the four factors, η is a constant of nature for a given nuclear fuel (by changing the composition of the fuel, i.e. increasing the degree of enrichment, a higher value of η is achieved…) which must be obtained from experimental measurements. A. Dokhane, PHYS487, KSU, 2008 23 Chapter4- Nuclear Chain Reaction 5.4 Neutron Leakage and Critical Size The other three factors allow the nuclear engineer and designer some “choice”, as they depend on the physical properties of the fuel as well as on the size of the reactor, its geometry, fuel arrangement, moderator, as well as on the other materials incorporated in the reactor assembly. Question: is the neutron leakage desirable?? Answer: Although neutron leakage is generally not welcomed by the nuclear engineer, it is important to realize that the critical size requirement for a chain reaction to become possible is a consequence of neutron leakage. A. Dokhane, PHYS487, KSU, 2008 24 Chapter4- Nuclear Chain Reaction 5.5 Nuclear Reactors and Their Classification Question: How are the reactor classified? Answer: Reactors are classified based on a variety of characteristic features : 1) Type of fuel used 2) Average neutron energy at which the greater part of all fissions occur 3) Moderator materials used 4) Arrangement and spatial disposition of fuel and moderator 5) Purpose of the reactor صفحة( حول أنواع المفاعالت بناءا على الخصائص المذكورة أعاله20 )ال يزيد عن بحث صغير ال A. Dokhane, PHYS487, KSU, 2008 25 Chapter4- Nuclear Chain Reaction Homework • Problems: 4, 5 of Chapter 7 in Text Book, Pages 241 • اﱃ اﻟﻠﻘﺎء ﰲ اﳊﺼﺔ اﻟﻘﺎدﻣﺔ ان ﺷﺎء ﷲ A. Dokhane, PHYS487, KSU, 2008 26
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