Segregation Effects in Granular Collapses Joshua Caplan Supervisors: Stuart Dalziel and Nathalie Vriend Abstract In this essay we consider the collapse of a cylindrical column comprised of two layers of differently sized ballotini. We vary the initial mass of the column and compare the two orientations of the layers with the case of a column of a single material. The use of differently sized particles leads to so-called granular segregation, with the larger particles rising towards the surface of the flow. Remarkably this does not affect the macroscopic flow dynamics and other properties, such as the final run-out distances, are consistent with previous work. 1 Introduction Granular materials are ubiquitous in both geophysical and industrial situations and exhibit a wide variety of complex behaviours. Despite much recent research they remain poorly understood. One particular problem, as illustrated in figure 1, is that of the collapse of a column of granular material under its own weight, and the resulting spreading flow. Such situations occur in, for example, cliff collapses and industrial accidents, and can be extremely dangerous and destructive. ℎ 𝑟 ℎ∞ 𝑟∞ Figure 1: Illustration of the column collapse problem. The problem of granular collapse was first considered by Lube et al. (2004) and Lajeunesse et al. (2004) who independently considered the case of a monodisperse column 1 and varied the initial column height ℎ , the initial column radius 𝑟 , the granular medium and the base roughness. Both papers found that the key variable was the aspect ratio, 𝑎 ≡ ℎ /𝑟 , of the initial column and that the actual mass (or volume) of the column was unimportant. Using this they found that there were two main regimes depending on whether the aspect ratio was greater or less than a critical value 𝑎 , although they disagreed on the exact value. For small 𝑎, only the edge of the column collapsed, leaving a truncated cone. For larger 𝑎, the collapse reached the centre, leaving a steep central cone which tapered towards the edges. Lajeunesse et al. refer to this as a ‘Mexican hat’ profile. In both regimes there was an undisturbed region of material in the centre of the deposit. Lube et al. (2004) found power laws for the non-dimensional run-out distance 𝑟̃ ≡ ⎧1.24𝑎 𝑟∞ − 𝑟 =⎨ / 𝑟 ⎩1.6𝑎 𝑎 < 1.7 𝑎 > 1.7 . In contrast Lajeunesse et al. (2004) derived semi-empirical laws ⎧ 𝑟∞ = 𝑟̃+ 1 = ⎨ 𝑟 ⎩ 𝑎 + 4 tan 𝜃 − 𝑎 < 0.74 , 𝑎 > 0.74 where 𝜃 was the angle of repose of the material. These two sets of laws are, however, similar over the range of aspect ratios considered. Both groups found that the final nondimensional height of the deposit followed power laws ⎧𝑎 ℎ 𝑎<1 ℎ̃ = ∞ = ⎨ (Lube et al., 2004) / 𝑟 𝑎 > 1.7 ⎩0.88𝑎 ⎧𝑎 𝑎 < 0.74 =⎨ (Lajeunesse et al., 2004), ⎩0.74 𝑎 > 0.74 where the differences appear to be in the interpretation of very similar data. In addition, both groups found that, for large aspect ratios, the deposit spread outwards at a constant velocity proportional to 𝑔𝑟 , with only a short acceleration and deceleration phase. Lube et al. also found that the time taken for the full collapse was 𝑡∞ = 3.0 ℎ , 𝑔 which they note is approximately twice the free-fall time for a particle dropped from height ℎ , i.e. 𝑡∞ ≈ 2(2ℎ /𝑔) / . Neither group found that the choice of material had any significant effects on the flow, although later work by Trepanier & Franklin (2010) showed that extremely non-spherical grains (particle aspect ratio > 4) behave very differently. The choice of base roughness 2 also had little effect on the run-out distance, but Lajeunesse et al. found that it did affect the final profile shape at large aspect ratios. Both groups also found that there was little mixing between adjacent horizontal slices of the initial monodisperse column. These experiments have also been extended to quasi-two-dimensional collapses along rectangular channels (Lube et al., 2005; Balmforth & Kerswell, 2005; Lajeunesse et al., 2005; Lube et al., 2007). As with axisymmetric collapses, two regimes were found depending on the aspect ratio, but the behaviours for large 𝑎 followed a different power law that, due to the effects of friction at the walls, depended on the width of the channel. A semi-circular geometry was also considered by Lajeunesse et al. (2005), which behaved the same as the axisymmetric case but allowed more of the internal structure of the collapses to be observed. Various systems involving sloped beds have also been considered (Hogg, 2007; Mangeney et al., 2010; Lube et al., 2011; Maeno et al., 2013). Collapses have also been successfully modelled numerically using discrete element methods (DEM) (Staron & Hinch, 2005, 2006; Zenit, 2005), using shallow-water-like systems of equations (Mangeney-Castelnau, 2005; Kerswell, 2005; Larrieu et al., 2006; Doyle et al., 2007; Hungr, 2008), and using the non-Newtonian 𝜇(𝐼) rheology (Lagrée et al., 2011). All of this previous work has focused on monodisperse materials, whereas real systems typically feature significant amounts of polydispersity. This leads to segregation, with the larger and less dense particles rising to the surface of the flow, and the smaller and denser particles sinking towards the bottom (Drahun & Bridgwater, 1983). This can then cause so-called segregation-mobility feedback, which can have dramatic effects on the flow dynamics (e.g. Pouliquen et al., 1997). For the collapse problem this could lead to changes in the run-out distance and other flow properties. Tunyasuvunakool (2011) considered columns of a fixed size composed of large pearl barley and small glass ballotini collapsing onto a smooth base. He found that columns with large particles initially on the bottom (normally stratified columns) typically had larger run-outs than the reverse (inversely stratified columns). In particular the normally stratified columns had their longest run-out when they comprised around 80% ballotini by volume. Inversely stratified columns only had longer run-outs for columns with around 10% ballotini, which Tunyasuvunakool attributed to the smaller particles forming rollers for the barley to slide along. Tunyasuvunakool also found that, for certain combinations of layer orientation and height ratio, a region of barley would separate from the deposit to give what he termed a ‘detached ring’. In Caplan (2012), I instead considered the same materials but varied the column height for a fixed ratio (50%) of the two materials. Overall, I found that inversely stratified columns behaved almost identically to the monodisperse columns considered by Lajeunesse et al. (2004) and Lube et al. (2004), albeit with a slightly reduced run-out distance due to the large barley grains sinking into the ballotini layer beneath them. In contrast, normally stratified columns behaved significantly differently due to the smaller ballotini falling through the barley layer and pushing a ring of barley outwards. At lower aspect ratios this gave rise to a detached ring, whereas it remained attached to the main 3 deposit for larger columns. In addition, I found that the collapse edge became unstable leading to asymmetric deposits, most likely due to a fingering instability of the form discussed in Pouliquen et al. (1997) and Pouliquen & Vallance (1999). 2 Experimental Method Figure 2: Photograph of the experimental setup. The cylinder used to construct the columns can be seen in the centre of the image. The laser scanner is the metal box to the right of the cylinder; the red line on the deposit is the image of the laser. The high-speed camera can be seen in the background to the left of the cylinder. The apparatus used in this experiment can be seen in figure 2. In all the experiments we used spherical ballotini. For the small particles we used colourless ballotini with diameters between 300 µm and 425 µm, and for the large particles we used red ballotini with diameters between 1000 µm and 1300 µm. We considered columns with layers of equal mass of the two particle types in both the inversely stratified (large ballotini on top) and normally stratified (small ballotini on top) orientations. In addition, we considered monodisperse columns comprised solely of the smaller ballotini. The columns were constructed in a plastic cylinder of internal diameter 32 mm and ranged in total 4 initial mass from 200 g to 1200 g. At the start of the experiment the cylinder was lifted using a pneumatic piston, thereby allowing the column to collapse over a flat base covered with sandpaper. The collapses were filmed with a high-speed camera recording at 1000 frames per second, and the height profiles were measured using a laser scanner operating at 100 profiles per second. The high-speed camera footage was then digitally processed to automatically measure the radius of the final deposit. 3 Results 3.1 Collapse dynamics The dynamics of all three column types were very similar over the range of aspect ratios (1.3 to 8.0) considered, as shown in figure 3. As the column collapses it spreads axisymmetrically outwards at the base, with the upward regions falling straight down. When the upper layer reaches the base of the collapse it spreads outwards over the lower layer. At this stage no segregation can be observed in any initial stratification. As the collapse progresses, the upper layer moves outwards faster than the lower layer, reaching the deposit edge as the collapse ends. During the very end of the collapse, some large ballotini can be seen rising to the surface of the normally stratified columns due to segregation. In figure 4 we can see the height profiles taken during the collapse of a typical inversely stratified column; the other column types are qualitatively and quantitatively similar at the same aspect ratios. This shows how the deposit only spreads at the base, rather than along its whole height. We can also see how material moves from the centre of collapse to the deposit edge as the collapse occurs and the deposit thins. An example of the surface radial velocities during a collapse can be seen in figure 5. As with the height profiles this does not vary significantly between collapses of different types with the same aspect ratio. As the collapse begins, the deposit accelerates outwards before reaching a roughly constant spreading velocity. Material that was initially higher in the column moves outwards faster than the front, as was seen in figure 3. When the column of material has completely collapsed (at 𝑡 ≈ 400 ms in this example), the flow begins to decelerate before stopping. This leads to a region of stationary material, which can be seen expanding from the centre of the deposit towards the edge. Figure 6 shows the deposit radius against time for the full range of collapses considered. In this the constant spreading speed can be clearly seen along with shorter acceleration and deceleration phases. In particular, the spreading velocity is independent of the initial height of the column and the composition of the column. For the initial column radius used in these experiments, the spreading velocity is approximately 0.5 m s− . Figure 7 shows the run-out against time for the columns of largest aspect ratio after 5 (a) Inverse (𝑎 = 7.9) (b) Monodisperse (𝑎 = 8.0) (c) Normal (𝑎 = 7.9) Figure 3: Images for column collapses of different types. Images are taken 200 ms, 300 ms, 400 ms and 600 ms after the start of the collapse. These correspond to non-dimensional times of approximately 0.33, 0.95, 1.6 and 2.8. 6 60 0.25 s 0.35 s 0.37 s 0.39 s 0.41 s 0.45 s 0.55 s 50 h/mm 40 30 20 10 0 −40 −20 0 20 40 60 80 100 x/mm Figure 4: Deposit profiles taken at various times during the collapse of an inversely stratified column of aspect ratio 𝑎 = 7.9 as measured using the laser scanner. t/ms 500 0.8 400 0.6 300 0.4 200 0.2 100 0 50 100 150 200 Radial velocity/ms−1 1 600 0 250 r/mm Figure 5: Plot of the radial velocity at the surface of the flow throughout the collapse for the same collapse as in figure 4. non-dimensionalising by 𝑟̂ = 𝑟̃ 𝑎 / = 𝑟∞ − 𝑟 , 𝑟 𝑡̃= 𝑡−𝑡 , ℎ /𝑔 where 𝑡 is the time at the start of the constant speed phase. As can be seen, all the data collapses onto a single curve thereby showing that these scalings are appropriate. In particular, the time scaling is that for a freely falling object (free fall time = (2ℎ/𝑔) / ), demonstrating that the flow is controlled by the influx of new material as the column collapses. For smaller aspect ratios the acceleration and deceleration phases dominate (as can be seen in figure 6) and the scalings break down. 7 250 Inverse Monodisperse Normal r/mm 200 150 100 50 0 0 100 200 300 400 500 600 700 t/ms Figure 6: Measurements of deposit radius 𝑟 against time 𝑡 for a range of collapses. Collapses of the same type range in initial mass from 200 g to 1200 g, with the larger columns travelling a further distance. 2.5 2 r̂ 1.5 1 Inverse Monodisperse Normal 0.5 0 0 0.5 1 1.5 2 t̃ 2.5 3 3.5 4 Figure 7: Graph showing the modified non-dimensional run-out distance 𝑟 ̂ = 𝑟𝑎̃ − / against the non-dimensional time 𝑡 ̃ for collapses with large aspect ratio (𝑎 > 5). 3.2 Deposit details Figure 8 shows the interiors of an inversely and a normally stratified collapse. Both types of collapse feature a central cone where the initial orientation is preserved. As expected, there is negligible mixing anywhere in the inversely stratified column as the stable stratification prevents any segregation and, as shown in the work on monodisperse collapses, there is no other mechanism for mixing. In contrast, the normally stratified collapse shows some signs of segregation but this process is incomplete. For segregation to occur there needs to be shearing across the interface between the layers. The experimental set-up means that this can only occur for a short period of time and the amount of shearing is too weak to allow complete segregation. Figure 9 shows the central height of the deposit, as measured using the laser scan- 8 (a) Inversely stratified column. (b) Normally stratified column. Figure 8: Cross-sections of the final deposit for typical examples of the two types of column. Photograph was taken by rapidly inserting a piece of clear plastic and removing the material from one side of it. 32 Inverse Monodisperse Normal h∞ /mm 30 28 26 24 22 20 1 2 3 4 a 5 6 7 8 Figure 9: Graph of the final deposit height ℎ∞ against the initial aspect ratio 𝑎. ner, against the initial aspect ratio of the column. Monodisperse columns appear to be slightly taller than either type of stratified column. In addition, inversely stratified columns appear to be slightly shorter at larger aspect ratios. The cause of this is not fully understood and is likely, in part, to be a measurement issue. The deposit height appears to decrease slightly at larger aspect ratios but the trend is unclear. Figure 10 shows a log-log plot of the final non-dimensional radius for the collapses 9 r̃ 8 7 6 5 4 Inverse Monodisperse Normal 3 2 1 1 2 3 4 5 6 7 8 9 10 a Figure 10: Log-log plot of non-dimensional run-out 𝑟 ̃ against initial aspect ratio 𝑎. The solid line is 𝑟 ̃ = 2.1𝑎 / and the dashed line is 𝑟 ̃ = 1.25𝑎. considered. In addition, the best fitting half-power laws ⎧1.25𝑎 𝑟̃ = ⎨ / ⎩2.1𝑎 𝑎<2 𝑎>4 , have been plotted which are consistent with those previously found for monodisperse columns. While all three types of column have very similar final run-outs, the monodisperse columns travel slightly further. In addition, the inversely stratified columns travel a slightly shorter distance than the normally stratified ones. The exact cause of this is unclear and may just be due to differences in how the radius measurement program detected the edge of the deposit. 3.3 Effect of ratio of particle types In addition we also considered a range of columns with varying proportions of small particles Π . These were all of total mass 2000 g and of initial radius 47 mm. Only normally stratified columns were considered: inversely stratified columns should not be affected by column make-up due to their stable initial stratification. Although figure 11 appears to show that columns with a large proportion of small ballotini go further, this is misleading. The main difference is due to the type of particles present at the edge of the collapse when it begins to decelerate. As this happens, particles at the edge are able to separate from the bulk and spread out as discrete objects. If these are small particles then they cannot get very far due to the surface roughness, whereas large ballotini are able to bounce across the surface. This means that the large particles are not included in the final deposit, causing it to appear smaller. Figure 12 shows the final deposits for these collapse, showing the different edge behaviour. 10 300 Π =0 r/mm s 250 Πs= 0.25 200 Πs= 0.5 Πs= 0.75 150 Πs= 1 100 50 0 0 100 200 300 400 t/ms 500 600 700 800 Figure 11: Measurements of the deposit radius 𝑟 against time 𝑡 for a range of collapses of differing proportions of small particles Π . This behaviour at the edge also causes problems when measuring the deposit radius. When the edge becomes disperse it is hard to determine the edge in a consistent manner. This means that the radius measurement becomes inaccurate at late times, with the level of inaccuracy depending on the choice of particle type ratio. 4 Conclusions The key finding of my work is that, contrary to expectations, segregation is surprisingly unimportant in the macroscopic dynamics of the systems considered: the bidisperse columns behaved almost identically to the monodisperse ones previously considered. While segregation does occur, it is incomplete and has no effect on the flow dynamics. The few differences present between the collapses considered can be adequately explained by the different behaviour of the two sizes of grain when they act as discrete particles, as opposed to changes in the behaviour of the bulk flow. It is also important to reconcile these findings with those of Caplan (2012) and Tunyasuvunakool (2011) who found significant differences between their columns. The significant difference in experimental methods is that we both used barley grains for the larger grained material. Barley has a lower density than the ballotini and means that columns of the same height no longer have the same potential energy. We can compensate for this by rescaling the initial height to that of a column comprised purely of the material in the lower layer with the same initial potential energy. As seen in figure 13, this causes the differences in run-out to mostly disappear. The increased run-out from the ‘outside’ measurement can be explained in a similar 11 (a) Π = 1 (b) Π = 0.75 (c) Π = 0.5 (d) Π = 0.25 (e) Π = 0 Figure 12: Final deposits for normally stratified columns of mass 2000 g, initial radius 47 mm and a range of different proportions of small particles Π . 12 7 6 5 r̃ 4 3 Inverse Monodisperse Normal (inside) Normal (outside) 2 1 0 0 1 2 3 4 5 a (a) Graph showing the non-dimensional run-out 𝑟 ̃ against the non-rescaled aspect ratio 𝑎. 7 6 5 r̃ 4 3 Inverse Monodisperse Normal (inside) Normal (outside) 2 1 0 0 1 2 3 ã 4 5 6 (b) Graph showing the non-dimensional run-out 𝑟 ̃ against the rescaled aspect ratio 𝑎.̃ Figure 13: Graphs showing effect of rescaling the aspect ratios of the collapses considered by Caplan (2012) in order to take into account the differing initial potential energies. For the distinction between the two normal measurements see the original paper. manner to the discussion in section 3.3. In the normally stratified collapses a region of barley detached from the edge of the deposit and, due to the smooth base, was able to slide a significant distance. In contrast, the other collapses had ballotini at the edge which could slide a much shorter distance. As the outer measurement includes this sliding distance it is not surprising that it fails to collapse onto the same curve. The ‘detached rings’ observed are likely due late stage separation of barley from the edge of the collapse. Due to the smooth base the barley slides as opposed to the bouncing observed in the set of experiments discussed earlier. This is a less random process and so a distinct ring is formed as opposed to the diffuse edge. This sliding is likely why Tunyasuvunakool found that, for normal columns, there 13 was a peak in run-out at roughly 80% ballotini. 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