2005 International Nuclear Atlantic Conference - INAC 2005 Santos, SP, Brazil, August 28 to September 2, 2005 ASSOCIAÇÃO BRASILEIRA DEENERGIA NUCLEAR - ABEN ISBN: 85-99141-01-5 THE USE OF NUCLEAR TECHNIQUES FOR THE QUANTIFICATION OF SEDIMENT TRANSPORT AND BULK DENSITY OF DEPOSITS – APPLICATION TO DREDGING AND DUMPING OPERATIONS OPTIMISATION AND ENVIRONMENTAL IMPACT STUDIES Jefferson V. Bandeira 1 , Lécio H. Salim1 , Pedro E. Aun1 1 Centro de Desenvolvimento da Tecnologia Nuclear (CDTN / CNEN- MG) Serviço de Meio Ambiente e Técnicas Nucleares - TR-1 Rua Prof. Mário Werneck s/n Cidade Universitária – Pampulha – CP 941 30123-970 Belo Horizonte, MG [email protected]; [email protected]; [email protected] ABSTRACT Nuclear techniques are used, since the 1950’s and 1960’s, for studying the transport, in water environment (rivers, estuaries, bays and open coast) [1, 2], of sandy bottom sediment and fine sediment (silt and clay) in suspension, through the labelling of sediments with γ emitters radioactive tracers of a suitable half-life. The labelling is followed by injection and subsequent in situ detection, by means of scintillation detectors sliding on the bottom or transported at suitable depths, by positioned boats. These kinds of studies associated with the knowledge of the hydrodynamic agents, e.g.: river, tidal, wind and wave currents, are powerful tools for the understanding and quantification of the sediment transport and also for its response to human interventions. Some of these interventions, are: construction of dams and training walls in rivers; dredging of reservoirs, access channels and harbours and dumping of the dredged material, in water environment. A recent improvement for the utilisation of radioactive tracers in labelling fine sediment was the development of the methodology for the use of 99mTc [3, 4, 5, 6, 7], broadly applied in Nuclear Medicine [11]. Another important application of nuclear techniques is the use of sealed sources of γ emitters radioisotopes (e.g. 241 Am; 137 Cs) for measuring vertical density profiles of fine sediments in reservoirs, access channels, turning basins and berthing areas in harbours, and in the well of trailing suction hopper dredgers (TSHD) [1, 14, 19]. The use of these techniques contributes for the optimisation of the dredging works and allows the evaluation of dumping sites and also the physical environmental impacts of the dumping. Furthermore, they allow calibrating mathematical models for different aspects of sediment movement. Some examples of applications of these techniques are shown for harbours in Santos-SP; São Luiz-MA and for the Pampulha reservoir in Belo Horizonte-MG, and the watercourses downstream. 1. INTRODUCTION: NUCLEAR TECHNIQUES IN SEDIMENTOLOGY 1.1. Artificial Tracers When dealing with various aspects of the behaviour of sediments in water environment, tracers are usually a quite pragmatic approach to many engineering and environmental questions. They provide responses for the long-term interaction between the sediment and the flow processes that act over it, since they are able to integrate all the actions suffered by the sediment during the observation period. Since most applications are concerned with a well-defined site, it would be a very lucky circumstance to find some natural tracer that would provide information about the sediment behaviour at the area of interest. More generalised utilisation of tracers only became possible with the advent of artificial tracers in the 1950's and 1960's. From this time on, sediment labelled with material having radioactive or fluorescent properties (named tracers), have been used to study sediment movement, provided they were able to accurate matching the properties of the natural sediment. Also activatable tracers (activated in a nuclear reactor after the sediment sampling) were considered. Radioactive tracers (γ-emitters) of a suitable half-life are used in sediment movement studies in water environment (rivers, estuaries, bays and open coast) [1]. The steps for these studies are labelling of the sediment; injection; detection and analysis of the results. The radioactive tracers have the advantage of versatility: they can be used for gravel, sand, and fine sediment (silt and clay) transport studies. Moreover, they enable direct in situ detection of the material, which means that the scanning of the tracer cloud is always done with open eyes, a great help in planning the detection strategy. The in situ detection is performed by means of scintillation detectors (towed by positioned boats – Lagrangean detection), sliding on the bottom or transported at suitable depths, for sand bottom or for fine sediment in suspension transport studies, respectively [1, 2]. For narrow watercourses, the detectors could be hanged in bridges or poles (Eulerian detection) [3]. In relation to fluorescent (suitable only for labelling sand) and activatable tracers, the problem is the blind detection, performed by sampling and subsequent analysis in laboratory, which means that no feedback is being received when performing the field detection works. During the sediment labelling with radioactive tracers, one has to pursue mass labelling, in order to allow reliable quantitative results in the detection, that is: the counts must be proportional to the sediment mass and not to the sediment surface. In this way, for sand studies, ground glass (same density as sand) in the suitable grain-size distribution and doped with an activatable element (e.g. 191 Ir, 197Au, 50 Cr, 45 Sc) to be irradiated in a nuclear reactor previously to the injection, is almost universally used. The resultant radioactive elements have the following half- lifes (T1/2 ) and the main γ radiation energy: 192 Ir (T1/2 = 74.4 days, γ = 0.32-0.47-0.30-0.31-0.61MeV); 198 Au (T1/2 = 2.7 days, γ = 0.41MeV); 51 Cr (T1/2 = 27.8 days, γ = 0.32MeV) and 46 Sc (T1/2 = 84 days, γ = 0.891.12MeV). The mass of ground glass for each injection and the activity utilised does not surpass, respectively, 1kg and 2Ci (74GBq), taking into account the statistical aspects of the in situ detection [4] and the radiological safety standards [1, 5]. For silt and clay studies, the labelling is performed in the natural sediment (generally electronegative) through its capacity to adsorb cations of radioactive tracers (e.g. 198 Au, 51 Cr, 46 Sc) [6]. This aspect makes necessary the irradiation of the chosen element for each experiment. A few grams of the chosen radioactive tracer are necessary to label a considerable mass of fine sediment. The radioactive is the unique tracer suitable for reliable labelling of fine sediments, considering they allow mass labelling and the same behaviour of the labelled and not labelled sediment, in hydrodynamic conditions [6, 10]. The time scale of the experiment determines the type of radioisotope to be chosen: short halflife isotopes for short time scales (e.g. study of fine sediment transport in suspension) and the opposite for large scales (e.g. slow bottom sand sediment transport). INAC 2005, Santos, SP, Brazil. 1.1.2. Development of 99m Tc as a tracer for fine sediment in suspension A recent improvement for the utilisation of radioactive tracers in labelling fine sediment was the development of the methodology for the use of 99m Tc (technetium meta-stable) [3, 7, 8, 9, 10], broadly applied in Nuclear Medicine [11]. The 99m Tc has the following properties: (T½ = 6.02 hours; γ = 0.14MeV), and it comes from the parent nuclide 99 Mo (T½ = 66 hours; β = 1.2MeV; γ = 0.74; 0.18....MeV) through a metastable transition [11, 12]. Technetium generators, known as “milk generators” or “cows”, are then supplied to Nuclear Medicine laboratories. These generators, due to the convenient halflife of the 99 Mo, make possible to obtain 99m Tc for one week or more, by its elution through an ion-exchange column, using 6mL of a solution of NaCl (9mg/mL) passing through the column. After each elution, the generator continues to produce the 99m Tc and in 24 hours, due to its growth rate and considering the radioactive decay of the 99 Mo, it is possible to extract about 88.5% of the activity previously extracted. The low γ radiation energy and the portability aspect are two of the reasons for its broad use in Nuclear Medicine. The 99m Tc is eluted as an anion TcO 4 - (pertechniate). In this form it is injected in the veins of patients, in Nuclear Medicine applications. It should be worthy if 99m Tc could also be used for labelling fine sediment and applied to dynamic sedimentology studies, because of its characteristics, such as: 1. Short half-life adequate for short time scales of the studies of fine sediment in suspension; 2. Low γ energy (0.14MeV), implying moderate shielding and ease of manipulation in field conditions; 3. Portability of the tracer when compared with 198 Au, for example, obtained by irradiation in nuclear reactor for each experiment; 4. Availability even in places where there are no nuclear facilities, due to its widespread application in Nuclear Medicine, making also possible its use in dynamic sedimentological applications that can be performed daily, for more than one week, in field studies, using only one portable generator. As the 99m Tc is eluted as an anion, in order to be adsorbed by the fine sediment (generally electronegative), studies were performed [7, 8] to transform it in an electropositive form. Several reductors were tested for this purpose. It was selected and used the SnCl2 .2H2 O. The reduction of Tc(VII) with Sn(II) is produced according to the following equations [13]: 3 Sn (II) + 2 Tc (VII) = 3 Sn (IV) + 2 Tc (IV) (1) In aqueous solution, a colloidal compound is formed after reduction. TcO2+ + 2 H2 O = TcO(OH)2 + 2H+ (2) Most probably this is the chemical specie which is adsorbed in sediments after reduction of the pertechniate. The labelling of the fine sediment with this colloid was studied considering the effect of: a) mass of the reducing agent; b) pH; c) concentration of sediment; d) contact time; e) INAC 2005, Santos, SP, Brazil. possibility of release as a function of water turbulence [7, 8]. Only the labelling of the fine sediment with a radioactive tracer is not enough for its correct application in field studies. It is necessary to prove first that the hydrodynamic behaviour of the labelled and the not labelled sediment are the same. In this way, the settling behaviour, in still water, of both sediments were compared, through sedimentation tests relating the cumulative % of mass in function of the fall velocity of the particles [9, 10]. The results obtained were very good. Afterwards, the tracer was used for studying the physical behaviour (advection, dispersion, sedimentation rate) and the corresponding environmental impacts (increase of concentration and possibility of deposition) of the fine sediment dredged in the accreted Pampulha reservoir and dumped in the watercourses downstream [3]. It is expected that the 99m Tc, with its new use for labelling fine sediment, can be applied for studies in estuarine and coastal environments, as the ones already performed using 198 Au [1], some of them being briefly presented in Chapter 3 (Case Studies) of this paper. 1.2. Nuclear Gauges for the Determination of Bulk Density of Fine Deposited Sediment The absorption (photoelectric effect) and scattering (Compton effect) of electromagnetic radiation (X or γ) emitted by an artificial radioactive source are a function of the concentration or the bulk density of the mixture sediment-water. In this way it is possible to construct nuclear gauges based on these principles, provided that the system is calibrated for known concentrations. The gauges use sealed sources and scintillation detectors. The gauges based on the photoelectric effect and the Compton effect are, respectively, the transmission and the backscattering gauges (figures 1a and 1b). They are normally equipped with depth sensors and inclinometers for the underwater unit and are used as point measuring systems being lowered on a suspension cable to sink into the soft bed by gravity. In this way, bulk density profiles between 1.0 and 1.5 ton/m3 may be determined. Figure 1a. Transmission gauge After Salim et al. [14] INAC 2005, Santos, SP, Brazil. Figure 1b. Backscattering gauge After Meyer et al. [15] 2. PRACTICAL USES OF ARTIFICIAL TRACERS AND NUCLEAR GAUGES 2.1. Sand Bottom Sediment Transport Bed-load transport studies present different effectiveness in function of the environment in which they are performed. Sand bottom sediment transport studies applying tracers are important if the information provided is worthwhile. In the case of rivers, bed-load is only a fraction of the sediment transported by the river, most of which (~90%) occurs in suspension. Nevertheless, in some cases, such as the artificial deepening (e.g. dredging) or construction of training walls with navigation purposes, the bed-load transport knowledge is very useful. In the cases of estuaries and open sea this knowledge is important: 1. For monitoring sedimentation, by sand, in existing dredged areas (e.g. access channels) or predicting the maintenance in future ones; 2. For design harbour inlet by-passing schemes, location and dredging of sand traps; 3. For the construction of coastal structures, such as: groins, jetties, detached breakwaters and sea walls and for artificial beach nourishment. The associated sedimentological studies related to the response (accretion or erosion) of the shoreline to the coastal structures and the artificial beach nourishment require, respectively, a knowledge of the littoral-drift and the cross-shore sand transport in the nearshore region; 4. For the temporary excavation below natural depths for the burial of pipelines and cables; 5. For the reclamation works in estuaries and the influence of the loss of tidal volume on the sedimentary regime. A detailed description of the methodology applied for the study of sandy bottom sediment transport, applying radioactive tracers, can be seen in [2, 16 and 17]. 2.2. Suspended Transport of Fine Sediment The study of the dynamics of suspended sediment with tracers is of capital interest in problems of civil engineering, mostly for the definition and optimisation of dumping sites for dredged material (the nearest place environmentally suitable for the dumping) and in water pollution problems. In such cases, it has to be known how a given pollutant adsorbed to fine sediment or the sediment itself is dispersed. The most important results obtained from such experiments are: 1. The path and drift caused by currents; 2. The mean velocity of transport; 3. The turbulent dispersion coefficients that characterise the dispersion of the sediment by the water body; 4. The dilution of the sediment (maximum concentration in function of time); 5. The sedimentation rate; 6. The area over which the sediment is deposited. The methodology for the study of fine sediment in suspension applying radioactive tracers can be seen in [2, 17 and 18]. Results obtained for the bottom and suspended transport allows calibrating mathematical models for different aspects of sediment movement and known hydrodynamic conditions. INAC 2005, Santos, SP, Brazil. 2.3. Nuclear Gauges for Measuring Bulk Density The nuclear gauges can be employed for measuring the bulk density in vertical profiles of fine sediments deposited in: 1. Reservoirs, generally near the dam, when studying sedimentological balance of the system lake catchment basin-reservoir; 2. Access channels, turning basins and berthing areas of harbours, in estuarine and coastal regions, and in the well of dredgers, being these measurements related to the optimisation of dredging works and environmental studies. In harbours submitted to heavy fine sediment siltation, such as Rotterdam and Zeebrugge, in Europe, and in some harbours in South America and Indonesia it exists, in certain parts, a lower density layer above the more consolidated bed sediment, named fluid mud, which can attain several metres. The top interface between the fluid mud layer and the water above is detected by the echosounder of 210kHz frequency, normally employed for surveying nautical depths. It was demonstrated, by ship manoeuvring and laboratory studies, that the fluid mud is not an obstacle to navigation, provided its bulk density is equal to 1.2ton/m3 or less (Figure 2). In this way, since the late seventies, radioactive gauges have been operated at spot locations in Rotterdam waterway, in conjunction with echo sounding surveys, allowing to produce nautical charts showing the 1.2ton/m3 density depth contours. They are used for navigation (addition of the loose silt layer to the keel clearance) and for improving dredging efficiency (positioning of the dredger suction tube below the loose silt layer, when dredging). Figure 2. Scheme of keel clearance. After Caillot et al [20] A transmission gauge (Figure 1a) was used in Brazil, in the access channel to Alumar harbour and in its turning basin and berthing area (Figure 6), between 1983 and 1994, and also in the well of a trailing suction hopper dredger (TSHD), with good technical and economical results [14, 19]. This last use allows evaluating the load efficiency of a particular dredging practice (Figure 3). Loading curves of the dredger, according to the percentage of sand dredged (related to the total amount of sand, silt and clay), are drawn. For a fixed travel and dumping time (same dredged region and same dumping site), and for each loading curve, there is an optimum time for dredging with overflow (t3 - t2), in order to get the optimum dredging INAC 2005, Santos, SP, Brazil. cycle time (tangent to the specific loading curve). Suspended sediment studies labelling the full load of TSHD or barges (see case studies in Chapter 3) could promote the optimisation of the dumping sites with a consequent reduction of the travel and dumping time (Figure 3), shortening, even more, the optimum dredging cycle and increasing the dredging efficiency. Figure 3. Dredging cycle for a trailing suction hopper dredger. After De Heer [21] 3. CASE STUDIES 3.1. Santos Bay, Santos, SP - Brazil [1, 22] The shape of Santos Bay, in São Paulo State, Brazil, 60km far from São Paulo city, is roughly quadrangular, limited at E and W by two rocky points, Ponta Grossa and Ponta de Itaipu (Figure 4), with an area of about 36km2 . Two estuaries, Santos at E, and São Vicente at W open into the bay, the contribution of Santos estuary to the overall flow in the bay being more important. The most important Brazilian port facilities are installed at Santos estuary. Adequate depths are kept at the harbour and access channel through permanent maintenance dredging. Due to the importance of Santos harbour, several sedimentological studies were performed at Santos Bay and surroundings, from 1973 to 1985, using a combination of hydraulic measurements, physical movable bed models and radioactive tracer studies. Bottom sediments in the bay cover all the range between fine sand and clay (Figure 5). The material dredged in the harbour is mainly silt and clay, including also fine sand in the access channel. INAC 2005, Santos, SP, Brazil. Studies performed in 1973/74 [23] had the objective of evaluating several dumping sites to reduce the distance from the dredging region to the disposal areas. In the first study it was determined, by labelling the full load of barges (600m3 capacity) with 198Au, that the disposal area near Ponta de Itaipu, at W, was inadequate, since the material could return, by the action of hydrodynamic circulation, to the bay-estuary system (Figure 4). A new alternative site outside the bay and at E was chosen, near Ilha da Moela. Its use, implemented immediately after the studies, resulted in a sensible reduction on maintenance dredging costs. Figure 4. Key map, Santos Bay and estuary. After Aun & Bandeira [1] In 1985, another dumping site, also eastward to the bay entrance, near Ponta da Munduba rocky point was defined (Figure 4), with the objective of reducing, even more, the transportation distances [24]. Again, the technique used was the labelling, with 198 Au, of the dredged material transported by barges. The new dumping site is being used since 1986. Hydraulic measurements and tracer studies performed in 1980/81 [25], using ground glass labelled with 192Ir, were intended to define the behaviour of the bottom fine sandy sediment that is found in some regions of the bay, on behalf of physical movable bed model studies. Six injections were performed in different regions of Santos Bay, three in the winter of 1980 and three in the summer of 1981 (Figure 5). Before the injections in summer, the bottom was surveyed in order to detect the remaining of the radioactive clouds from the winter experiments. It was still possible to find activities of more than twice the background, in the INAC 2005, Santos, SP, Brazil. regions inside the dotted lines, having origin in PI1 WINTER and PI3 WINTER. In this way, the summer tracer injections were made outside these regions. Figure 5. Santos Bay: tracer injection points (PI). Clouds near PI’s (Injection Points) are related to the last complete detection performed. After Aun & Bandeira [1] Both, in summer and winter, bottom sediment movement has an onshore resultant, being more important in winter conditions. Transportation rates were quantified in both regimes (Table 1). Waves, associated with tidal currents inside the bay, are the main transport agents, the direction of movement being compatible with the prevailing wave incidence direction. It was also determined that, when the depth of 7m is attained, bottom material under movement tends to inflect towards Santos estuary entrance. This is indicated by the two sets of dotted lines (having origin in the injection performed at 03/Aug./80 in PI1 WINTER ), obtained in the detections dated 07/Feb./81 and 08/Apr./81 (Figure 5). It is also possible to observe, from the successive positions of these dotted lines, the movement of the bottom sediment towards the coast and also a smaller shift towards W of the western portion of the lines limiting an activity equal to twice the natural bottom sand background. The current circulation pattern inside the bay, mainly tidal influenced, was determined by intensive field measurements at three levels (1.0m below water surface, mid depth and 1.0m above the bottom) employing manned and recording currentmeters [26]. They demonstrated that, for the eastern part of the bay, where the injections PI2 WINTER and PI2 SUMMER were performed, the currents are always, in flood and ebb tide, and for the three levels, INAC 2005, Santos, SP, Brazil. directed to N, flowing towards the interior of the bay. This is due to a counterclockwise circulation inside the bay, during ebb flow. Table 1. Main results obtained with sandy bottom sediment transport studies in Santos Bay using ground glass labelled with 192Ir Injection Points (Figure 5) Time interval considered Depth related to hydrographic Datum (m) Bottom sediment transport rate Azimuth of the sediment transport cloud axis (kg/m/day) PI1 WINTER PI2 WINTER PI3 WINTER PI1 SUMMER PI1 SUMMER PI2 SUMMER PI2 SUMMER PI3 SUMMER 03/08/80 to 22/09/80 08/08/80 to 18/09/80 06/08/80 to 19/09/80 09/02/81 to 08/04/81 08/04/81 to 20/06/81 21/02/81 to 07/04/81 07/04/81 to 19/06/81 19/02/81 to 02/04/81 7.9 270 342° 12.3 350 335° 10.0 200 14° 7.6 10 350° 7.6 20 350° 10.9 40 339° 10.9 40 339° 9.3 10 349° As a consequence, in spite of the greater depths relatively to the other regions, the bottom sediment transport rate for the eastern region is also higher, both in winter and summer regimes (Table 1). This could be the reason for not finding remaining activities in the region of PI2 WINTER radioactive injection, before the injection performed in the summer season. From this Case Study it is possible to evaluate how powerful radioactive tracers can be in answering bottom and suspended sediment movement questions, provided a good knowledge of the hydrodynamic conditions of the site under study is available. 3.2. Alumar harbour, São Luis, MA - Brazil [1, 22] Alumar harbour (Figure 6) has been built to serve a huge aluminium factory near São Luis City, capital of Maranhão State, in the north of Brazil. The access channel in Estreito dos Coqueiros, linking the terminal to São Marcos Bay, the turning basin and the berthing area were dredged in a region between two islands: Taua Mirim and São Luis. The currents in the region are mainly tidal influenced and can reach values above 2.0m/s during spring tides. The tide is semidiurnal presenting spring tidal amplitude of about 7.0m. The natural sediment encountered on the bottom of São Marcos Bay is mainly sand. INAC 2005, Santos, SP, Brazil. Figure 6. Key map, Alumar harbour. After Aun & Bandeira [1] Due to the high natural suspended sediment concentration (about 600mg/L), being silt and clay its main constituent, a strong sedimentation occurs in the artificially enlarged and deepened dredged regions. Thus, the dredged material is mainly silt and clay, except when certain parts of the access channel, nearer to São Marcos Bay are dredged. Adequate natural INAC 2005, Santos, SP, Brazil. depths are kept at this bay due to the high tidal currents, being this region the natural dumping site for the disposal of the dredged material. In order to improve dredging works, various studies employing nuclear techniques together with hydraulic measurements, were performed. Labelling full charges of a trailing suction hopper dredger and dumping the material in São Marcos Bay showed that the conditions for the dispersion of the dredged material, dumped into the bay, were very favourable [27]. Very little of the fine material discharged by the dredger remained on the sandy bottom at the site of disposal, being resuspended by the high-speed currents. Besides that, the concentration of the discharged particulates remaining in suspension soon reached the concentration level naturally present in the bay. Consequently, the chosen disposal area could be changed to a site closer to the entrance of Estreito dos Coqueiros, care being taken to avoid disposal shortly before or after tide reversal, while currents are not strong enough. Other studies were made at the harbour region [28] in an attempt to implant some sort of agitation dredging in this area where the sediment deposition is quite important. In this case, the fate of the dredged spoil depends on the position of the discharge site and the stage of the tide. During flood tide the suspended material is carried either to the stretch of the Estreito dos Coqueiros south of the harbour or to Rio dos Cachorros, which opens in the harbour region (Figure 6), and most of it settles down to the bottom. When the dumping is performed during ebb tide, the position of the discharge site makes a great difference. Tests were made near the western and the eastern extremity of the harbour terminal. The trajectories of the sediment are quite different in both cases, but the material tends to move to sites of preferential sedimentation. When discharge is done through a pipeline from a hydraulic suction dredger operating near the berth, a considerable part of the dredged spoil sinks directly to the bottom due to the influence of the initial downwards momentum and negative buoyancy of the slurry jet. If the discharge is made parallel and just below to the surface water, the slurry remains in suspension for a long time (figures 7 and 8). Since the tidal stage is of utmost importance for the behaviour of the dredged spoil which remains in suspension after the disposal, much can be gained in terms of abatement of sedimentation in the berthing area and in the turning basin, by matching the discharge regime to the tidal stages. Six suspended sediment injections of fine material labelled with 198Au were performed in different points of the Estreito dos Coqueiros and the harbour turning basin (Figure 9). The labelled material was discharged into the jet of a suction dredger (injections 3 and 4) or directly, parallel and just below the water surface (injections 1, 2, 5 and 6). Due to the small depths in some parts of the studied region, two scintillation detectors were placed at one metre below the water surface, in a rigid pole fixed to the detection boat. It was possible to compute the advection velocity u, the longitudinal DL and transversal DT dispersion coefficients, the dilution, the sedimentation rate SR, the necessary time for the sedimentation of half of the cloud T1/2 and L1/2 = u.T1/2 , for the clouds of all the experiments. Table 2 presents the results of some of these parameters, where the dispersion values are calculated for the T1/2 instant. INAC 2005, Santos, SP, Brazil. Figure 7. Sketch of the set-up for tracer injection in the dredger jet. After Moreira & Bandeira [28] Figure 8. Behaviour of fine sediment dumped in the ebb phase. After Moreira & Bandeira [28] INAC 2005, Santos, SP, Brazil. Figure 9. Injection points of suspended sediment labelled with After Moreira & Bandeira [28] INAC 2005, Santos, SP, Brazil. 198 Au. Table 2. Main results of suspended sediment transport studies in Alumar Harbour region using mud labelled with 198 Au Injection Gauge number 1 2 3 4 5 6 1 2 1 2 1 2 1 1 2 1 Tidal ampl (m) and stage 6.6 ebb 5.8 flood/ ebb 3.9 ebb 3.2 flood 3.4 ebb 5.4 ebb/flood Average Advect. velocity (m/s) 0.75 0.22-0.63 0.32 0.38 0.55 Longitudinal dispersion DL (m2 /s) 2.15 2.76 0.88 0.19 0.10 3.27 Transversal Sedimendispersion tation rate DT (m2 /s) SR (g/ton/s) 0.23 431 0.18 361 0.28 532 0.30 306 0.11 2289 0.10 2257 233 1.10 2.89 0.08-0.28 1.12 3.43 0.53 449 371 917 L1/2 (m) 896 1069 290 449 94 95 1123 794 961 68 It can be inferred from Table 2 and Figure 9 that the higher sedimentation rates correspond to injections (3 and 6) being performed in situation of ebb flow, in the sheltered region of the turning basin, relatively to the ebb flow coming from the southern reach of Estreito dos Coqueiros. For this situation, in this region, there is the composition of the ebb flows coming from Rio dos Cachorros and from the southern reach of Estreito dos Coqueiros, producing a gyre of the cloud from an E-W movement to a S-N one, in a kind of vortex, facilitating the sedimentation. Furthermore, the third injection, resulting in the higher sedimentation rate (Table 2), was performed into the jet of the suction dredger operating in the berthing area. Current measurements made during the rainy season [29] showed the existence of a null-drift point in the lower water layer in the vicinity of the harbour, at spring tides, which strongly enhances sedimentation. This is unlikely to occur during dry seasons since fresh-water contribution to the system is very low at that time. In-situ density measurements, using a nuclear transmission gauge developed in Brazil (Figure 1a), allowed an evaluation of the thickness of the fluid mud layer up to the bulk density of 1.3ton/m3 . The variations in this thickness clearly showed a preferential sedimentation in the turning basin and a still stronger tendency to deposition in the berthing area, halfway from its centre, towards its eastern extremity. These measurements were performed, in a monthly basis, from 1983 to 1994, to control depth variations and to optimise dredging operations at Alumar harbour [14, 19]. 3.3. Pampulha reservoir, Belo Horizonte, MG - Brazil [3] The Pampulha reservoir, in Belo Horizonte, Brazil, is in an accelerated process of decrease of its liquid volume and water surface, due to an accretion of the order of 400,000m3 /year, mainly caused by fine sediment [3]. As the reservoir is located in an urban area, there is no suitable place to dump the dredged material on land, on a permanent basis. In this way, one reliable possibility is the implementation of the transposition, by dredging (e.g. using a INAC 2005, Santos, SP, Brazil. hydraulic suction dredger), of the sediments to the rivers downstream the dam, their natural way in the absence of the dam. This problem was the main motivation for the pioneer studies to labelling the fine sediment with 99m Tc [7, 8, 9 and 10]. Field experiments, with simultaneous and instantaneous injections of sediment and water, labelled, respectively, with 99m Tc and Rhodamine WT, were performed, in dry season, to measure the hydrotransport capability in a stretch of 25km, since Pampulha creek until Rio das Velhas, inclusive (Figure 10). Figure 10. Key map of the studied region. Pampulha Hydrographic Basin and Velhas River. After Bandeira [3] A recent mathematical model was applied and calibrated to the data obtained and, through convolution, the sediment dumping using the hydraulic suction dredger system was simulated (Figure 11), calculating also, the physical environmental impacts: increase of sediment concentration and its decrease by subsequent dilution and the possibility of deposition. Through the measurement of physical-chemical parameters of the water, the possibility of desorption of the metals adsorbed in the sediment to be dredged, was evaluated. It was concluded that, from the studied aspects, there is no impediment for the dumping of the dredged fine sediment in the watercourses downstream Pampulha reservoir. INAC 2005, Santos, SP, Brazil. D1 1,00 D3 0,90 D4 0,80 D5 0,70 D6 0,60 FOZ 0,50 D7 D8 0,40 D9 0,30 DP 0,20 Concentration attenuation 0,10 DPRS DJEQ 0,00 0 100 200 300 400 500 600 700 Time interval (10 min.) Figure 11. Temporal variation of the concentration downstream the Pampulha reservoir, in function of the dredging dumping lasting 9 hours, in D1 (Figure 10). After Bandeira [3] 4. CONCLUSIONS The use of artificial tracers and nuclear gauges contributes for the optimisation of the dredging works and allows the evaluation of the dumping sites and also the physical environmental impacts of the dumping. Furthermore, artificial tracers allow calibrating mathematical models for different aspects of sediment movement. The nuclear gauges for measuring bulk densities can be used in various applications, such as: • In reservoirs, allowing the improvement of the sedimentological balance of the lake catchment/basin-reservoir system; • In access channels, turning basins and berthing areas in harbours, allowing the addition of the fluid mud layer, up to the bulk density of 1.2ton/m3 , to the keel clearance of the ships, reducing the amount of sediment to be dredged; • In the well of trailing suction hopper dredgers, allowing the evaluation of the load efficiency of a particular dredging practice. It is expected that the 99m Tc, broadly used in Nuclear Medicine could also be applied for studies in continental, estuarine and coastal environments, such as those mentioned in Chapter 3. This is due to its new use for labelling fine sediment [3] and its advantages in relation to the use of 198 Au, as mentioned in the Item 1.1.2. Besides that, the concentration of the 99m Tc activity (Bq/mL of water) is of the order of 10-7 of the concentrations used in medical applications (Bq/mL of blood). The reason is that, for medical applications, the detector is placed outside the patient while for environmental use the detector is placed inside the water, in a “4π Geometry”, and this allows an enormous gain in counting efficiency. INAC 2005, Santos, SP, Brazil. REFERENCES 1. P. E. Aun, J. V. Bandeira, “The Role of Nuclear Techniques in Sedimentological Studies and Some Applications in Latin America”, Use of Nuclear Techniques in Studying Soil Erosion and Siltation, Vienna, 26-29 April 1993, IAEA-TECDOC-828, pp. 29-97 (1995). 2. F. Tola, “The Use of Radioactive Tracers in Dynamic Sedimentology”, Regional Seminar on the Use of Isotope Techniques in Water Resources Development, Athens, Greece 1981, IAEA, Vienna (1981). 3. J. V. Bandeira, Development of Nuclear and Correlate Techniques for Studies in Urban Hydrology - Aplication in Pampulha Hydrographic Basin and in Velhas River, MG. Doctorate Thesis in Sanitation, Environment & Water Resources - Escola de Engenharia, UFMG, Belo Horizonte, Brasil (2004). (In Portuguese) 4. G. Sauzay, G. Courtois, “The Quantity of Sediment to be Deposited in a Radioactive Tracer Experiment on Dynamic Sedimentology”, CEA Report S.A.R. S 68-8, Saclay, France (1968). (In French) 5. A. Plata, A. Moser, Guide to the Safe Handling of Radioisotopes in Hydrology, Reproduced by the IAEA,Vienna, Austria, (1990). 6. H. Bougault, Étude de la sorption de quelques radioéléments artificiels par les sédiments pélitiques en vue de son application au marquage radioactif de ces matériaux. Thèse (Doctorat) - Faculté des Sciences , l´Université de Paris, France, 1970. (In French) 7. J. V. Bandeira, et al., “The Use of 99m Tc as an Adsorbable Tracer for Studying the Dynamics of Fine Sediments in Suspension”, International Symposium on Isotope Techniques in Water Resources Development and Management, Vienna, 10-14 May 1999, Proceedings…1 CD-rom. 8. J. V. Bandeira, et al., “The Use of the 99m Tc as an Adsorbable Tracer for Studying the Dynamics of Fine Sediments in Suspension”, Simpósio Brasileiro de Recursos Hídricos, 13, Belo Horizonte, 1999, Anais...São Paulo: ABRH, 1999. 1 CD-rom. (In Portuguese) 9. J. V. Bandeira, “The Use of the 99m Tc as an Adsorbable Tracer for Studying the Dynamics of Fine Sediments”. Final Report. Belo Horizonte: [s.n.], 2001. (IAEA Research Contract BRA-10891). 10. J. V. Bandeira, et al., “Development of a Technique for Using 99m Tc as an Adsorbable Tracer for Hydrodynamic Studies of Fine Sediments in Suspension”. Journal of Applied Radiation and Isotopes, Volume 57, pp.85-92 (2002). 11. M. P. Sandler, et al., Diagnostic Nuclear Medicine. 3 ed. Williams & Wilkins, Baltimore, USA (1996). v.1 12. Radiological Health Handbook, U.S. Department of Health, Education and Welfare – Public Health Service. Washington D.C., USA: USGPO (1960) 13. T. Sekine, et al., “Complexation of technetium with humic acid”. Radiochimica Acta 63, pp. 87-90 (1993). 14. L. H. Salim, et al., “Report of the First Survey of the Bottom at the Turning Basin and Access Channel to Alumar Harbour - São Luis, Maranhão State”, NUCLEBRAS/CDTN Rep. DERL.PD-016/83, Belo Horizonte, Brazil (1983). (In Portuguese) 15. G. Meyer, et al., “Use of nuclear density gauges for studying and measuring silt deposit formation and concentration in the laboratory and in situ”, Proceedings Symposium on Use of Isotopes in Hydrology, Vienna 1983. IAEA, pp. 741-752 (1984). (In French). 16. G. Sauzay, Méthode du Bilan des Taux de Comptages d'Indicateurs Radioactifs pour la Détermination du Débit de Charriage des Lits Sableux, Thèse d'Ingénieur Docteur, Faculté des Sciences de Toulouse, CEA R. 3431 (1967). (In French) INAC 2005, Santos, SP, Brazil. 17. P. E. Aun, V. L. Mendes, “Radioactive tracers in the study of the movement of sediments”, Regional Training Course on the Use of Isotope Techniques in Environmental Studies of the Hydrosphere and the Atmosphere, Piracicaba and Belo Horizonte, Brazil 1992, IAEA (1992). (In Portuguese) 18. A. Caillot, et al., “Étude au laboratoire et in situ du comportement hydrodinamique des fines particules en suspension, à l'aide de traceurs radioactifs”, Technical Co-operation Project BRA/8/018, Belo Horizonte, Brazil 1978. IAEA (1978). (In French) 19. L. H. Salim et al. “Bottom survey of turning basin and access channel to Alumar harbour – São Luis/MA”. Technical Reports NUCLEBRÁS/CDTN/DERL.PD e CDTN/CNEN to ALUMAR, between 1983 & 1994. 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Bandeira, “Study of the Dumping of Spoils from Maintenance Dredging of Alumar Harbour into Estreito dos Coqueiros, Maranhão State”, NUCLEBRAS/CDTN, Belo Horizonte, Brazil. Rep. DERL.PD-019/84 (1984). (In Portuguese) 29. L. H. Salim, “Hydraulic and Sedimentological Measurements at Estreito dos Coqueiros and Rio dos Cachorros, in the Surroundings of the Alumar Harbour”, NUCLEBRAS/CDTN, Belo Horizonte, Brazil. Rep. DERL.PD-022/84 (1984). (In Portuguese) INAC 2005, Santos, SP, Brazil.
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