Basic Elements of Static RTG's Load Energy Conditioning Control Energy Conversion Radioisotope Fuel Energy Transfer Heat Rejection Shielding Power Generated by Radioisotopic Heat Sources Power (t) = Initial # of Radioisotopes No ln 2 Decay Rate, s-1 l= t 1/2 Energy Released Per Decay MeV E Number of Radioisotopes Left After t Years Power (t) = No • E • ln 2 t1/2 exp -( exp -( t•ln 2 ) t1/2 t•ln 2 t1/2 ) Important Characteristics of Radioisotopic Heat Sources Physical Properties • Isotope • Type of Radiation • Energy of Decay • Half Life • Curies/gram • Curies/Watt • Watts/gram • Total kWh Realizable Commercial Properties • Form of Compound • Melting Point • Isotopic Purity • % Isotope in Compound • Watts/g (compound) • Watts/cm3 (comp.) Production Properties • Recovery From Power Reactor Fuel • Production Rate in Power Plants • Availibility • Price Most Commonly Used Isotopes for Radioisotope Heat Sources Co-60 Sr-90 Ru-106 Cs-137 Cm-242 Ce-144 Cm-244 Pm-147 Tm-170 Po-210 Pu-238 Main Decay Mode Of Most Favored Radioisotopes MAINLY GAMMA Co-60 MAINLY BETA Sr-90 Ru-106 Pm-144 Tm-170 GAMMA & BETA Cs-137 Ce-144 MAINLY ALPHA Po-210 Pu-238 Cm-242 Cm-244 Half Life of RTG Fuels 87.4 Pu-238 30 Cs-137 28 Sr-90 18.1 Cm-244 5.24 Co-60 2.6 Pm-147 1 Ru-106 0.78 Ce-144 0.45 Cm-242 0.38 Po-210 0.35 Tm-170 .1 1 10 Half Life-Yr 100 1000 Decay Energy of Radioisotopes Cm-244 Cm-242 Pu-238 Isotope Po-210 Tm-170 Pm-147 Ce-144 Cs-137 Ru-106 Gamma Ray Beta Alpha Sr90 Co-60 0 1 2 3 4 5 6 Particle Energy-MeV 7 8 Specific Activity of RTG Fuels Pu-238 17 Cm-244 81 Cs-137 87 Isotope Sr-90 Pm-147 Co-60 142 928 1130 3180 Ce-144 Cm-242 3320 Ru-106 3394 4500 Po-210 6048 Tm-170 0 2000 4000 Curies/gram 6000 8000 Power Density in RTG Isotopes 141 Po-210 120 Cm-242 33.1 Ru-106 25.6 Isotope Ce-144 Co-60 Tm-170 Cm-244 17.4 13.6 2.65 Sr-90 0.96 Pu-238 0.56 Cs-137 0.42 Pm-147 0.33 0 2 0 4 0 6 0 8 0 100120140160180200 Watts/gram Isotope Comparison of Specific Activity and Activity Required to Produce a Watt Pu-238 30 17 Cm-244 29 81 Cs-137 207 87 Sr-90 148 142 2788 Pm-147 928 65 Co-60 Curies/Watt Curies/gram 1130 124 Ce-144 3180 28 Cm-242 3320 102 Ru-106 3394 32 Po-210 4500 445 Tm-170 6048 0 2000 4000 6000 Curies/gram or Curies/Watt 8000 Total Energy Content in RTG Fuels For Reasonable Mission Times 575 Co-60 350 (0.4) Po-210 310 Cm-242 210 Ru-106 Isotope (5) (1) (10) 190 Cm-244 (0.4) 150 (1) Ce-144 74 (10) Sr-90 (10) 47 Pu-238 Tm-170 33 Cs-137 33 Pm-147 0 6 (0.4) (10) (3) 100 200 300 400 500 600 Total kWh/g for Stated Time (Y) Period 700 Commercial Fuel Form (% Isotope in the Metallic Element) Co-60 (10 %) Metal Sr-90 (55 %) SrTiO 3 Ru-106 (3.3 %) Metal Cs-137 (35 %) Ce-144 (4. 5%) Pm-147 (95 %) Tm-170 (10 %) Po-210 (95 %) Metal Pu-238 ( 80 %) Pu O Cm-242 ( 0.45 %) Cm-244 ( 18.1 %) CsCl Ce 2O 3 Pm 2O 3 Tm 2O 3 2 Cm 2O 3 Melting Point of Commercial RTG Fuel Compound 2375 Tm-170 2310 Ru-106 2250 Pu-238 2190 Isotope Ce-144 2130 Pm-147 Cm-242 1950 Cm-244 1950 1910 Sr-90 1480 Co-60 646 Cs-137 Po-210 0 255 500 1000 1500 2000 Melting Point °C 2500 3000 Concentration of Active Radioisotopes 95 Po-210 86 Isotope Cm-244 Cm-242 82 Pm-147 82 70 Pu-238 28 Cs-137 23 Sr-90 Co-60 10 Tm-170 8.8 Ce-144 3.8 Ru-106 3.3 0 10 20 30 40 50 60 70 % Active Isotope 80 90 100 Commercial Specific Power Level of RTG Iostopes 134 Po-210 98 Cm-242 2.27 Cm-244 1.74 Isotope Co-60 Tm-170 1.2 Ru-106 1.1 Ce-144 1 0.39 Pu-238 Pm-147 Sr-90 Cs-137 .1 0.27 0.22 0.12 1 10 100 Watts/g compound 1000 Specific Power Density of Leading Radioisotopes 1210 Po-210 882 Cm-242 20.4 Cm-244 15.8 Isotope Co-60 13.7 Ru-106 9.6 Tm-170 6.2 Ce-144 3.9 Pu-238 1.8 Pm-147 1.01 Sr-90 Cs-137 .1 0.38 1 10 100 Watts/cm3 1000 10000 Production of Radioisotopes in Commercial Power Plants 36 Cs-137 16 Sr-90 15 Isotope Pu-238 Ce-144 3.8 Pm-147 3.6 2.3 Ru-106 Cm-244 0.4 Po-210 0 Cm-242 0 Co-60 0 Tm-170 0 0 10 20 30 40 Production Rate in Power Reactor- kg/1000 MWeY Future Cost of RTG Fuels 2800 Po-210 2000 Isotope Cm-242 Pu-238 300 Co-60 280 Cm-244 170 Tm-170 136 Ru-106 120 Pm-147 75 Ce-144 50 Sr-90 20 6.5 Cs-137 0 500 1000 1500 2000 2500 3000 3500 Cost $ per Gram (pure) Energy Cost For Fuel Only For Reasonable Missions 350 Pm-147 235 Po-210 138 Isotope Pu-238 125 Tm-170 Ru-106 23 (1) Cm-244 22 (10) Co-60 15 (5) Ce-144 11 (1) Sr-90 6 (10) Cs-137 4 (10) 0 100 200 (0.4) (0.4) 180 Cm-242 (3) (10) (0.4) 300 400 Cost/kWh for Stated Mission (Y) 500
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