Can we detect cirrus changes with remote sensing methods ? Bernd Kärcher DLR Institut für Physik der Atmosphäre with contributions from W. Haag, J. Ovarlez, J Ström CIRAMOSA and beyond Final project meeting CNES HQ, Paris, November 20/21, 2003 mesoscale gravity waves T(t) dehydration and denitrification HNO3 H2O liquid particles and ice nuclei cirrus Measurement strategy during INCA formation layer developed cloud, virga • When do cirrus clouds form ? • What are the freezing mechanisms ? Analysis of data taken inside and outside of clouds Freezing mechanisms in cirrus conditions A strong indirect effect of aerosols on cirrus clouds is possible if • liquid particles and IN are, at least in part, externally mixed • liquid aerosols and ice nuclei (IN) have distinct freezing thresholds (IN < 130% vs > 145%) Indirect aerosol effect on cirrus clouds Indirect aerosol effect on cirrus clouds The presence of IN may lead to • a suppression of ice crystal concentrations in cirrus clouds • a bimodal ice crystal size distribution, even at a constant cooling rate • differences in the vertical cloud structure and cloud cover • enhanced sedimentation fluxes through a small number of large crystals originating from IN The magnitude of the indirect aerosol effect depends on • spectrum (pdf) of updraft speeds or cooling rates • number densities and freezing relative humidities of ice nuclei • degree of external vs internal mixing of IN with liquid aerosol particles Ubiquitous mesoscale temperature fluctuations minimize the impact of heterogeneous IN. Distributions of RHI outside of cloud inside cloud Distributions of RHI outside of cloud inside cloud Lessons from RHI observations • homogeneous freezing controls cirrus formation in clean and polluted air masses • direct evidence for heterogeneous ice formation in cirrus clouds • number of IN (< 0.01 cm-3) too small to strongly alter cirrus properties (weak neg. Twomey effect) at the prevailing rapid cooling rates The combined effect of IN and small-scale fluctuations of temperature compared to synoptic cooling may lead to • high ice crystal concentrations even in the presence of IN • complex evolution of ice crystal size distributions Synoptic versus mesoscale waves Bimodality induced by IN and small-scale waves synoptic wave only (5 cm/s peak) Atmospheric modeling • Microphysical domain-filling trajectory simulations based on ECMWF wind fields with superimposed mesoscale temperature oscillations • Domain 25o-75oN, tropopause region (+1 km to –2 km around local TP), 3 month-averages Sep/Oct/Nov 2000 • H2O mixing ratio reinitialized every 6 hours at RHI < 95% and constant above to generate realistic supersaturation spectra (W. Haag, Ph.D. thesis) Cloud occurrence frequency / Cloud cover Cloud cover changes: add IN Cloud cover changes: alter wave prop‘s Do aerosol particles control the properties of cirrus clouds ? • Small-scale temperature oscillations and homogeneous freezing seem to be universal features of cirrus clouds • Regarding their impact on cloud, changes in aerosol may easily be masked by dynamical changes • IN may impact dehydration and seed lower level clouds, but would not alter overall cloud prop‘s at the observed concentration levels of O(0.01 cm-3) Cirrus changes quantified (prelimin. list) Changes in cloud cover caused by • vertical air motion variability: ± 5% • adding IN freezing @ 130%: ± 3% Changes in median cloud parameters caused by • vertical air motion variability: up to factor 3 (ni), ± 10-20% (ri and IWC), ± 15-50% (E), ± 10% (fsvc) • adding < 0.01 cm-3 IN freezing @ 130%: < factor 3 reduction (ni), < 15%increase (ri), < 25% reduction (IWC), < factor 2 reduction (E), < 60%increase (fsvc) Can we detect cirrus changes with remote sensing methods ? • Changes appear to be more pronounced for mean cloud parameters • Likely strong contrast induced by weak wave activity over the oceans vs intense orographic forcing • Aerosol-induced changes likely to be more pronounced for more abundant and/or more potent IN This is a discussion topic ..... A careful evaluation of dynamical changes in cloud formation is required • to assess cirrus cloud properties and trends in a future climate • before conclusions regarding the role of aerosol composition or other anthropogenic factors are made
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