EUM�CO�96�430�SAT E�ect of Thin Cirrus Clouds on Meteosat Second Generation �MSG� Observations Final Report Matthias Wiegner, Peter Seifert, and Peter Schl�ussel Universit�at M�unchen, Meteorologisches Institut Theresienstra�e 37, D-80 333 M�unchen Germany 2 Final Report for EUM�CO�96�430�SAT Page left intentionally blank 3 Final Report for EUM�CO�96�430�SAT Contents 1 Introduction and Background 9 2 SEVIRI channels 11 3 Scattering Properties of Ice Crystals 13 3.1 3.2 3.3 3.4 3.5 3.6 Theoretical Approach . . . . . . . . . . . . . . . . . Selection of Particles . . . . . . . . . . . . . . . . . Selection of Size Distributions . . . . . . . . . . . . Phase functions . . . . . . . . . . . . . . . . . . . . Asymmetry Parameter and Single Scattering Albedo Wavelength Dependence in SEVIRI Channels . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 13 15 16 17 26 29 4 Comparison with Mie-Calculations 35 5 Radiative Transfer Calculations �IR-Channels� 41 5.1 Discrete ordinate method . . . . . . . . . . . . 5.2 Expansion of the phase function . . . . . . . . 5.3 Radiances at Top of Atmosphere . . . . . . . . 5.3.1 Dependence on Cloud Optical Depth . . 5.3.2 Dependence on Size Distribution . . . . 5.3.3 Dependence on Cloud Height . . . . . . 5.3.4 Dependence on Satellite Zenith Angle . 5.3.5 In�uence of Phase Function Expansion . 5.4 Justi�cation of scattering . . . . . . . . . . . . 5.5 Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 6 Radiative Transfer Calculations �VIS-Channel� . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 41 42 46 46 48 50 51 51 53 54 56 6.1 Method of Successive Order of Scattering . . . . . . . . . . . . . . . . . . . 56 6.2 Radiances at the Top of the Atmosphere . . . . . . . . . . . . . . . . . . . . 57 7 Summary and Conclusions 64 4 Final Report for EUM�CO�96�430�SAT 8 Acknowledgments 66 9 References 67 Final Report for EUM�CO�96�430�SAT 5 List of Figures 1 Number densities of hexagonal crystals as derived from Heyms�eld and Platt's size distributions HP1 and HP7. . . . . . . . . . . . . . . . . . . . . 18 2 Phase function vs. scattering angle � for wavelength ��0.635 �m. The curves show di�erent particle sizes as indicated, cf. Tab. 3 . . . . . . . . . . 19 3 Same as Fig. 2, but ��3.8 �m. . . . . . . . . . . . . . . . . . . . . . . . . . 19 4 Same as Fig. 2, but ��8.7 �m. . . . . . . . . . . . . . . . . . . . . . . . . . 20 5 Phase function vs. scattering angle � for wavelength ��0.635 �m. The curves show di�erent particle size distributions as indicated, cf. Tab. 4 . . . 21 6 Same as Fig. 5, but ��3.8 �m. . . . . . . . . . . . . . . . . . . . . . . . . . 21 7 Same as Fig. 5, but ��8.7 �m. . . . . . . . . . . . . . . . . . . . . . . . . . 22 8 Phase function vs. scattering angle � for ��0.635 �m for size distributions HP1 and HP1ST. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 24 9 Phase function vs. scattering angle � for ��3.8 �m for size distributions HP1 and HP1ST. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 24 10 Same as Fig. 9, but size distributions HP7 and HP7ST. . . . . . . . . . . . 25 11 Phase function vs. scattering angle � for ��8.7 �m for size distributions HP1 and HP1ST. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 25 12 Same as Fig. 11, but size distributions HP7 and HP7ST. . . . . . . . . . . 26 13 Real part of the refractive index as a function of wavelength . . . . . . . . . 31 14 Imaginary part of the refractive index as a function of wavelength . . . . . . 31 15 Phase function vs. scattering angle � for several wavelengths between 3.4 �m and 4.2 �m and size distribution HP1ST . . . . . . . . . . . . . . . . . 32 16 Same as Fig. 15, but size distribution HP7ST . . . . . . . . . . . . . . . . . 33 17 Phase function vs. scattering angle � for several wavelengths between 8.3 �m and 9.1 �m and size distribution HP1ST . . . . . . . . . . . . . . . . . 33 18 Same as Fig. 17, but size distribution HP7ST . . . . . . . . . . . . . . . . . 34 19 Comparison of phase functions of spherical �dashed line� and non-spherical particles �full line�; size distribtion is HP1ST, ��0.635 �m. . . . . . . . . . 36 20 Same as Fig. 19, but size distribtion HP7ST . . . . . . . . . . . . . . . . . . 36 6 Final Report for EUM�CO�96�430�SAT 21 Comparison of phase functions of spherical �dashed line� and non-spherical particles �full line�; size distribtion is HP1ST, ��3.8 �m. . . . . . . . . . . 22 Same as Fig. 21, but size distribtion HP7ST . . . . . . . . . . . . . . . . . . 23 Comparison of phase functions of spherical �dashed line� and non-spherical particles �full line�; size distribtion is HP1ST, ��8.7 �m. . . . . . . . . . . 24 Same as Fig. 23, but size distribtion HP7ST . . . . . . . . . . . . . . . . . . 25 Phase function of size distribution HP1ST for 8.7 �m �full line� and reconstructed from a Legendre expansion with 1000 coe�cients . . . . . . . . . . 26 Phase function of size distribution HP1ST for 8.7 �m �full line� and reconstructed from a Legendre expansion with 1800 coe�cients . . . . . . . . . . 27 Phase function of size distribution HP1ST for 8.7 �m �dashed line� and the reconstructed �full line, Delta-M-Method, M �100�. . . . . . . . . . . . . . . 28 Phase function of size distribution HP1ST for 8.7 �m �dashed line� and the reconstructed �full line, Delta-M-Method, M �50�. . . . . . . . . . . . . . . . 29 Change of brightness temperature with �c �3:8�m�; size distribution HP1ST, ��3.8 �m �dashed line�, ��8.7 �m �full line�. . . . . . . . . . . . . . . . . 30 Change of brightness temperature as a function of cloud optical depth for di�erent size distributions as indicated; ��3.8 �m. . . . . . . . . . . . . . . 31 Same as Fig. 31, but ��8.7 �m. . . . . . . . . . . . . . . . . . . . . . . . . . 32 Error in brightness temperature as a function of �c when Mie-phase functions are used; ��3.8 �m �see text�. . . . . . . . . . . . . . . . . . . . . . . 33 Same as Fig. 32, but ��8.7 �m. . . . . . . . . . . . . . . . . . . . . . . . . . 34 Vertical pro�le of brightness temperature for di�erent cloud heights; ��3.8 �m. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 35 Vertical pro�le of brightness temperature for di�erent cloud heights; ��8.7 �m. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 36 Change of brightness temperature with satellite zenith angle; �c �0.1. . . . . 37 Anisotropy function � ��; '� for size distribution HP1 �KRIPO model�; �o �30� . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 38 Same as Fig. 37, but �o �60� . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 Anisotropy function � ��; '� for size distribution HP1 �Mie calculations�; �o �30� . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 37 37 38 39 43 44 45 46 47 49 49 50 51 52 52 53 60 60 61 Final Report for EUM�CO�96�430�SAT 7 40 Same as Fig. 39, but �o �60� . . . . . . . . . . . . . . . . . . . . . . . . . . . 62 41 Anisotropy function � ��; '� for size distribution HP7ST �KRIPO model�; �o �30� . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 62 8 Final Report for EUM�CO�96�430�SAT List of Tables 1 List of wavelengths of SEVIRI channels, spectral interval ��1 , �2 � and central wavelength ��c � in �m . . . . . . . . . . . . . . . . . . . . . . . . . . . 11 2 Refractive index, nr and ni being real and imaginary part, respectively, for selected wavelengths within SEVIRI channels . . . . . . . . . . . . . . . . . 12 3 Dimensions �in �m� of particles of the eight selected classes: c and a are the large and small half-axes, respectively, rc is the radius of a sphere with same cross section. cl and cu are the lower and upper boundaries of c for each class. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 15 4 Selected size distributions from Heyms�eld and Platt and the corresponding temperature range. �'s and � 's are parameters describing the size distribution �see text, Eq. 2�. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 16 5 Single scattering albedo and asymmetry parameter for eight size distributions HP1 to HP8 for ��0.635 �m. . . . . . . . . . . . . . . . . . . . . . . 27 6 Single scattering albedo for di�erent size distributions and six wavelengths from SEVIRI channel IR 3.8. . . . . . . . . . . . . . . . . . . . . . . . . . . 28 7 Asymmetry parameter for di�erent size distributions and six wavelengths from SEVIRI channel IR 3.8. . . . . . . . . . . . . . . . . . . . . . . . . . . 28 8 Single scattering albedo for di�erent size distributions and �ve wavelengths from SEVIRI channel IR 8.7. . . . . . . . . . . . . . . . . . . . . . . . . . . 29 9 Asymmetry parameter for di�erent size distributions and �ve wavelengths from SEVIRI channel IR 8.7. . . . . . . . . . . . . . . . . . . . . . . . . . . 30 10 Asymmetry parameter for size distribution HP1ST and HP7ST: Mie and KRIPO calculations. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 11 Single scattering albedo for size distribution HP1ST and HP7ST: Mie and KRIPO calculations. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 12 E�ective radii for di�erent size distributions. . . . . . . . . . . . . . . . . . 13 Planetary albedo in percent for a cirrus cloud �9.5 � 11 km�. ��0.635 �m, �0 �30� . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 14 Same as Tab. 13, �0 �60� . . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 40 48 58 59 Section 1: Introduction and Background 9 1 Introduction and Background The use of data from operational meteorological satellites requires the development of retrieval techniques for the interpretation of satellite-measured radiances in terms of geophysical parameters. Usually, the algorithm development is done by means of radiative transfer simulations. In the frame of these simulations the interaction of atmospheric parameters with the radiation �eld must be described. In the visible and near infrared spectrum the radiative transfer is signi�cantly controlled by clouds. Clouds re�ect solar radiation to the satellite's sensors and modify the radiation leaving the surface and the lower atmosphere on its way to the satellite. Even thin cirrus clouds can modify upwelling radiance �elds to an extent that may not be neglected. Otherwise, interpretation of satellite images with respect to properties of the surface or the lower atmosphere can be erroneous. As a consequence, one of the key tasks in using data from present, but in particular of future instruments like the Spinning Enhanced Visible and Infra-Red Imager �SEVIRI� to be �own as part of Meteosat Second Generation �MSG� programme, is cloud detection and classi�cation. Many scene identi�cation schemes have been successfully applied to detect and characterize clouds in visible and infrared satellite imagery, however, it is still an unsolved problem to adequately detect optically thin clouds. Especially, thin ��subvisible"� cirrus clouds are di�cult to detect. This de�ciency is a severe drawback. Therefore, it is necessary to thoroughly describe the interactions between cirrus clouds and the radiation �eld by means of radiative transfer simulations. This �nally leads to the development of mathematical models which allow the retrieval of properties of the troposphere and the Earth's surface. In the past cirrus clouds have not been adequately described in radiative transfer simulations due to numerical de�ciencies in modelling the non-spherical particle shapes which are typical for ice crystals in cirrus clouds. Commonly spherical particles were assumed and the Lorenz-Mie theory was applied to determine the single scattering properties. One main reason was unavailable computing power for the calculation of scattering properties of ice crystals. Early attempts to consider hexagonal structures as scattering particles were made in the 1970'ties. �e.g., Wendling et al., 1979�. However, only with the recent availability of enhanced computing power more complete calculations including absorption and polarization were possible �Hess and Wiegner, 1994; Hess et al., 1996�. These studies have shown that the non-spherical particle shapes cause optical properties that drastically di�er from those known from spheres. In particular, the shape of the scattering function of ice crystals di�ers from that of spheres. This in turn will likely be important in cases where 10 Section 1: Introduction and Background the single scattering of radiation plays the major role, which is true for thin cirrus clouds. Therefore, the detection of thin cirrus clouds by radiometers like SEVIRI will critically depend on the knowledge about the impact of nonspherical particles on the atmospheric radiation �eld. It is the objective of this study to contribute to the development of an improved identi�cation of cirrus clouds by the SEVIRI radiometer. In this context two issues are discussed in detail: the �rst deals with radiative properties of ice clouds, the second concerns the induced modi�cations of radiative transfer. 11 Section 2: SEVIRI Channels 2 SEVIRI channels To determine the e�ect of cirrus clouds on satellite measurements it is su�cient to restrict oneself to the consideration of the spectral bands of the radiometer. The current de�nition of SEVIRI is based on the outcome of the MSG Phase-A-Study and includes 12 channels. The spectral bands are listed in Tab. 1. Channel VIS 0.6 VIS 0.8 IR 1.6 IR 3.8 IR 8.7 IR 10.8 IR 12.0 WV 6.2 WV 7.3 IR 9.7 IR 13.4 HRV �1 �c �2 0.560 0.635 0.710 0.740 0.830 0.880 1.500 1.615 1.780 3.400 3.800 4.200 8.300 8.700 9.100 9.800 10.800 11.800 11.000 12.000 13.000 5.350 6.260 7.150 6.850 7.350 7.850 9.460 9.700 9.940 13.040 13.400 13.760 0.500 0.900 Table 1: List of wavelengths of SEVIRI channels, spectral interval ��1 , �2 � and central wavelength ��c � in �m �c denotes the central wavelengths, �1 and �2 gives the lower and upper limit of the channels, respectively. All numbers in Tab. 1 are given in �m. Within this study we consider all channels below 10 �m with focus on channels IR 8.7 and IR 3.8. It is discussed in Sec. 3.6 whether the wavelength dependence of the optical properties within the channel requires a subdivision into several spectral intervals or not. If the latter is true the calculation of one wavelength for each channel su�ces. In Tab. 2 the refractive indices of ice �Warren, 1984� are listed for the central wavelengths of the SEVIRI channels. Furthermore, the refractive index is given for those wavelengths which are used to investigate the variability of optical properties within certain channels �cf. above�. 12 Section 2: SEVIRI Channels Channel �c 0.560 VIS 0.6 0.635 0.710 0.740 VIS 0.8 0.830 0.880 1.500 IR 1.6 1.615 1.780 3.400 3.500 3.600 IR 3.8 3.800 4.000 4.200 5.350 WV 6.2 6.260 7.150 6.850 WV 7.3 7.350 7.850 8.300 8.500 IR 8.7 8.700 8.900 9.100 IR 9.7 9.700 IR 10.8 10.800 IR 12.0 12.000 IR 13.4 13.400 nr 1.311 1.308 1.307 1.306 1.304 1.304 1.292 1.289 1.283 1.505 1.455 1.422 1.384 1.422 1.347 1.319 1.318 1.319 1.319 1.318 1.315 1.301 1.292 1.284 1.275 1.267 1.231 1.089 1.280 1.522 ni �3.29�10,9 �1.13�10,8 �3.44�10,8 �4.92�10,8 �1.45�10,7 �3.35�10,7 �5.88�10,4 �3.32�10,4 �1.15�10,4 �3.87�10,2 �1.64�10,2 �8.97�10,3 �6.72�10,3 �9.62�10,3 �1.36�10,2 �1.62�10,2 �6.65�10,2 �5.51�10,2 �5.77�10,2 �5.21�10,2 �4.91�10,2 �3.75�10,2 �3.91�10,2 �4.00�10,2 �4.18�10,2 �4.41�10,2 �4.46�10,2 �1.83�10,2 �4.13�10,1 �3.44�10,1 Table 2: Refractive index, nr and ni being real and imaginary part, respectively, for selected wavelengths within SEVIRI channels Section 3: Scattering Properties of Ice Clouds 13 3 Scattering Properties of Ice Crystals 3.1 Theoretical Approach Several methods have been proposed for the simulation of optical properties of nonspherical particles. They can be classi�ed in discrete dipole approximation �DDA�, extended boundary condition method �EBCM�, method of anomalous di�raction �MAD�, method of suppression of resonances �MSR�, statistical approach �STA�, and geometrical optics approach �GOA�. DDA �Draine, 1988; Draine and Flateau, 1994� is suitable for particles of arbitrary shape but limited to very small size parameters x � 2�r��. r is the particle radius and � is the wavelength of the incident radiation. It is used where � � a, i.e., it can be utilized for describing the interaction of millimetre and sub-millimetre waves with cirrus particles �Evans and Vivekanadan, 1990�. In principle, it can also be used in the visible or near infrared spectral range. However, for cirrus clouds size parameters larger than 100 frequently occur, resulting in an extremely large number of dipoles to be considered in the model. As a consequence the requirements on computing resources �memory, time� are far beyond any reasonable limit. A realistic upper limit of the application of DDA is about x�5 �several hours to one day on a cluster of 20 RISC workstations�. The EBCM, also referred to as T-matrix approach, covers the radiation-particle interaction where the wavelength is of the same order as the particle size �Mugnai and Wiscombe, 1986; Mishchenko, 1991; Mishchenko and Travis, 1994; Mishchenko et al., 1996�. It has been shown that it agrees well with results obtained from GOA up to size parameters of approximately 60 �Macke et al., 1996�. However, it should be noted that the T-matrix method can only be applied to particles which are rotationally symmetric; i.e., �relatively smooth" particles such as spheroids or so called Chebychev particles. Thus, most of the natural particles cannot be precisely modelled. The MAD was developed by Van de Hulst �1957� for cases where jm , 1j � 1 and x is large. Comparisons with the EBCM made by Latimer and Barber �1978� for ellipsoids of m � 1:05 and m � 1:20 with x � 2:37 and x � 4:31 generally agreed well but disagreed at large scattering angles. The results obtained for m � 1:05 were better than those obtained for m � 1:20. The MSR followed the detection by Chylek �1976, 1977� that resonances in the Mie coe�cients an and bn are responsible for the ripples superimosed on the general curve of extinction e�ciency versus size parameter of spherical particles. According to Van de Hulst �1957� the resonances are due to waves travelling along the surface of the sphere 14 Section 3: Scattering Properties of Ice Clouds and spewing o� energy which interferes with the forward di�racted wave. Chylek et al. �1976� conjectured that surface waves do not exist on aspherical particles. Hence, a good approximation of non-spherical particles would be the removal of all resonances in the Lorenz-Mie theory. Good agreement between this theoretical attempt and measurements were obtained for the range of size parameter 3 � x � 30. The method does not work at x � 30. The STA was described by Nevitt and Bohren �1984� for randomly oriented anisotropic oscillators named Rayleigh ellipsoids. This method is only adequate for x � �. For particles being large compared to the wavelength only GOA gives reliable results �Macke et al., 1995�. This is the size range relevant for cirrus clouds. Another advantage of this approach is that there are no limitations with respect to the particle shape. Finally it should be noted that the numerical resources required for GOA are reasonable � the typical time scale for one run �one particle size, one wavelength� is in the order of a few minutes on a typical desktop computer �DEC Alpha 255�. The selection of a suitable method is governed by the wavelength of the radiation and typical particle sizes and shapes. As already stated the spectral range is between 0.5 �m and 10 �m �SEVIRI channels�, particle sizes are between approximately 10 �m and a few millimetre, and typical shapes are hexagonal crystals. As a consequence, GOA seems to be the best choice for modelling scattering processes in cirrus clouds. We are aware that using GOA for small ice crystals at wavelengths near 10 �m might be critical. However, errors caused by GOA at this size parameter range can hardly be quanti�ed. On the one hand reference models do not exist, on the other hand comparisons between di�erent approaches su�er from inconsistent particle shapes �either the shapes are not exactly the same or the non-sphericity is only idealized�. Consequently, only some rough estimates on the accuracy are available. For example, Macke et al. �1995� state that GOA certainly is a better solution than Mie theory. They also found that the single scattering albedo � being one of the most important parameters govering radiation transfer � agrees within about one percent when T-matrix and GOA are compared, even at size parameters as small as x�10 �spheroids�. The asymmetry parameter seems to be overestimated by 5 � at maximum for x�20. For this reason a GOA model �`KRIPO'� has been developed on the basis of ray-tracing and Fraunhofer di�raction �Hess and Wiegner, 1994; 1995�. The model includes multiple refraction, absorption, di�raction and polarization of radiation at hexagonal plates and columns. Results from the KRIPO model have already been included in radiative transfer sim- 15 Section 3: Scattering Properties of Ice Clouds ulations for a comparison of modelled and groundbased radiance measurements. Good agreement has been obtained �Hess, 1996�. 3.2 Selection of Particles For this study hexagonal columns have been selected as typical particle shape for modelling the optical properties of ice crystals; they represent the most fundamental crystal shape relevant for ice clouds. This is true in particular for large particles which occur in `warm' cirrus clouds �T � ,20� C� Eight classes of columns are de�ned covering the full range of particle sizes. The classes are de�ned by logarithmic intervals of the large axis of the crystal c as described in Tab. 3. cl cu Class 2 6 6 20 20 40 40 90 90 200 200 400 400 900 900 2000 1 2 3 4 5 6 7 8 c a rc 3.5 1.4 1.77 10.0 4.0 5.07 30.0 10.0 13.6 60.0 22.0 28.8 130.0 41.0 56.9 300.0 60.0 100.0 600.0 80.0 159.9 1300.0 110.0 270.7 Table 3: Dimensions �in �m� of particles of the eight selected classes: c and a are the large and small half-axes, respectively, rc is the radius of a sphere with same cross section. cl and cu are the lower and upper boundaries of c for each class. Parameters c and a represent the length of the c-axis and the half-length of the a-axis of the crystals, respectively. The parameter c is a mean value representative for each class de�ned by its lower boundary cl and upper boundary cu . Dimension a is calculated from prescribed aspect ratios �c��2a�� published by Auer and Veal �1970�; note that they vary with size. The equivalent radius rc is the radius of a sphere with the same cross section as the hexagonal column when averaged over all randomly distributed orientations. All dimensions in Tab. 3 are given in �m. The equivalent radius rc can be calculated from a and c by v �p u 2 u 3 3 a t rc � � c + 4 2a ! �1� 16 Section 3: Scattering Properties of Ice Clouds Size Dist. Tmin Tmax �1 HP1 �20 �25 1.85�107 HP2 �25 �30 1.83�107 HP3 �30 �35 3.42�106 HP4 �35 �40 9.50�106 HP5 �40 �45 7.35�107 HP6 �45 �50 2.79�107 HP7 �50 �55 3.20�108 HP8 �55 �60 2.52�108 �1 �2.56 �2.51 �2.21 �2.29 �3.23 �3.15 �3.83 �3.85 �2 5.39�1010 7.67�1012 1.59�1011 1.67�1012 �2 c12 �3.74 �4.49 �3.94 �4.37 860 690 500 330 Table 4: Selected size distributions from Heyms�eld and Platt and the corresponding temperature range. �'s and � 's are parameters describing the size distribution �see text, Eq. 2�. Large particles �c � 300 �m� frequently exist in horizontal orientation. This results in phase functions which are not rotationally invariant with respect to the direction of the incident radiation, i.e., p��; �� in lieu of p��� with � being the scattering angle and � the scattering azimuth. In this case the scattering also depends on the solar zenith angle. However, these two-dimensional phase functions cannot be used in present state radiative transfer codes. For this reason it is assumed throughout this study that all particles are randomly oriented in space. 3.3 Selection of Size Distributions In real clouds always an ensemble of particles of di�erent sizes and shapes exist. In this study we assume all particles to be hexagonal columns. The particle size spectra are taken from measurements of Heyms�eld and Platt �1984� who introduced a classi�cation of size distributions � referred to as HP1 till HP8 � in terms of the ambient air temperature. It is given in Tab. 4. The size distributions HP1 - HP4 are described by one power law each for small and large particles according to N � �j c� j for j � 1; 2 �2� while for HP5 - HP8 one equation su�ces �j �1�. c is the largest dimension �length of the c-axis� of the crystal. Parameters �1 ; �1 and �2 ; �2 are given in Tab. 4. They were derived by Heyms�eld and Platt by �tting the measured size distributions for the given temperature ranges separately below and above a threshold value c12 which is de�ned by Section 3: Scattering Properties of Ice Clouds � �1���1 ,�2 � c12 � ��2 1 17 �3� Note that Heyms�eld and Platt's measurements do not include particles with c � 20 �m because no reliable measurements were available. HP1 and HP7 are the most interesting distributions with respect to the natural variability and the sensitivity of cirrus cloud optical properties: for HP1 �`warm cloud', �20� C to �25� C� the relative contribution of small particles to the total particle number is the smallest of all distributions, while for HP7 �`cold cloud', �50� C to �55� C� the relative number of small particles is largest. A graphical display of the size distributions HP1 and HP7 is given in Fig. 1. Note, that the number densities for the �rst two classes �cf. Tab. 3� are amended according to measurements published by Strauss �1994�. To distinguish these `more complete' size distribution from the original ones they are marked as HP1ST and HP7ST, respectively. The in�uence of these small crystals on the phase functions is discussed in Sec. 3.4. To easily describe the size distributions by one parameter it is common to de�ne an e�ective radius reff . It is given by reff � P � Qi �3�2 Ni � P � Qi � � Ni with Qi being the mean cross section of the crystal, Ni the number density of the particle and i denoting the number of the particle class as given in Tab. 3. The e�ective radii of HP1 and HP7 are reff �91.7 �m and reff �30.7 �m, respectively. 3.4 Phase functions Phase functions of a size distribution of cirrus ice crystals are calculated by superposition of phase functions of eight columns according to p�� � � 8 X Qi i�1 � N i p i �� � �4� The phase functions are normalized to unity, i.e., 1 Z 2� Z 1 p��� d cos � d� � 1 4� 0 ,1 or �5� 18 Section 3: Scattering Properties of Ice Clouds Figure 1: Number densities of hexagonal crystals as derived from Heyms�eld and Platt's size distributions HP1 and HP7. Z 1 ,1 p��� d cos � � 2 with � being the scattering angle and � the azimuth angle. Note, that all phase functions are rotationally invariant, that means, they only depend on �. For the individual particles described in Sec. 3.2, Qi and phase functions p��� are calculated utilizing the ray-tracing model KRIPO, the size distributions are taken from Tab. 4. With this input, realistic phase functions of cirrus clouds are calculated with Eq. �4�. In the following we show a few typical examples of phase functions and discuss their main features. First, p��� for individual particles are shown �Figs. 2-4� then phase functions of di�erent size distributions are presented �Figs. 5-7�. As just mentioned, Figs. 2-4 show as examples the phase functions for ��0.635 �m, ��3.8 �m and ��8.7 �m of all eight ice column classes as de�ned in Tab. 3. It can be seen that in the visible spectral range �Fig. 2� the di�erences of the scattering characteristics are relatively small. The two well known haloes are clearly visible near 22� and 46� , also the pronounced forward scattering peak and the enhanced backward Section 3: Scattering Properties of Ice Clouds 19 Figure 2: Phase function vs. scattering angle � for wavelength ��0.635 �m. The curves show di�erent particle sizes as indicated, cf. Tab. 3 Figure 3: Same as Fig. 2, but ��3.8 �m. 20 Section 3: Scattering Properties of Ice Clouds Figure 4: Same as Fig. 2, but ��8.7 �m. scattering. In general, the forward scattering peak is the larger and narrower the larger the particles are � curve labelled `8' denotes the largest crystal. For the 3.8 �m wavelength �Fig. 3�, the haloes are much less pronounced. The position of the �rst halo is shifted towards larger scattering angles and the second one has almost disappeared. This is caused by the strong absorption and the slightly greater real part of the refractive index at ��3.8�m when compared to the visible spectral range. The smooth parts of the small-particle-curves ��1 and �2� for 5� � � � 30� are caused by di�raction; this contribution becomes less important when the particle size increases. The general pattern of the phase function is similar for all crystals, however, the di�erences with particle size are larger than in the case of the short wavelength. The height of the forward scattering peak in general is smaller compared to p��; � � 635�m� as expected due to the smaller size parameter x. For the third wavelength of interest, 8.7 �m �Fig. 4�, the general shape of phase functions reveals features which are already known from the two previous cases. The position of the haloes is similar to the visible case while the magnitude of the forward scattering peak is reduced because of the reduced sizeparameter. As the particles become large, haloes vanish due to absorption and the phase functions remains almost unchanged. In Figs. 5-7 phase functions of the eight HP-size distributions �Tab. 4� are shown, the Section 3: Scattering Properties of Ice Clouds 21 Figure 5: Phase function vs. scattering angle � for wavelength ��0.635 �m. The curves show di�erent particle size distributions as indicated, cf. Tab. 4 Figure 6: Same as Fig. 5, but ��3.8 �m. 22 Section 3: Scattering Properties of Ice Clouds Figure 7: Same as Fig. 5, but ��8.7 �m. wavelengths are again 0.635 �m, 3.8 �m and 8.7 �m. Note that these size distributions do not include ice crystals smaller than 20 �m. In view of the discussions concerning the implementation of phase functions into the radiative transfer model �Sec. 5� it is worthwhile to have a closer look at some details of the phase functions. Fig. 5 �0.635 �m� shows only a very small in�uence of the size distributon on the phase function; they can hardly be distinguished in the plot. The zero-angle scatting value � lying between 8980 sr,1 � p�0� � 66000 sr,1 for HP7 and HP3, respectively � shows large variations, however, for all cases the peak is extremely narrow and the di�erences become smaller. At ��90� the phase function varies only within � 12�. Fig. 6 reveals a somewhat larger in�uence of the size distribution: the forward scattering peak p�0� varies between 2900 sr,1 for HP3, and 669 sr,1 for HP7, and the width of the peak is also changing. From the eight phase functions, four can be clearly distinguished. According to the lowest forward peak, HP7 is the uppermost curve in the sideward scattering range, followed by almost identical curves for HP5, 6, and 8. The next �coinciding� curves represents HP1, 2, and 4, while HP3 is the lowest which is in agreement with the quite large p�0�-value. The variability at ��90� is approximately � 50�. For 8.7 �m, shown in Fig. 7, the results for the di�erent size distributions are the same as in Fig. 6. Again, neither HP5, 6, and 8 nor HP1, 2, and 4 can be distinguished. HP3 exhibits Section 3: Scattering Properties of Ice Clouds 23 the lowest sideward scattering and the most dominating forward scattering �p�0��590 sr,1 �, whereas HP7 shows just the opposite behaviour �p�0��196 sr,1�. The variability of the phase function at 90� is again in the order of � 50�. The general pattern re�ects the special features of the phase functions of individual particles discussed above. The most prominent properties can be summarized as follows: The magnitude of the forward scattering peak decreases with wavelength while the width of the peak increases. The haloes are present at all wavelengths but most pronounced in the visible spectral region. And the sensitivity of the phase functions to variations in the size distributions is large in the infrared domain but negligible at 0.635 �m. As already mentioned in Sec. 3.3 it is interesting to investigate the role of small ice crystals which often have been neglected because of measurement problems. For this purpose we have compared HP-size distributions with the corresponding size distributions when small crystals according to Strauss' measurements were added. A few typical results are brie�y discussed. Fig. 8 shows the in�uence of small particles on the phase function at ��0.635 �m. Phase functions HP1 and HP1ST are compared. It is obvious that the e�ect is almost negligible; as a consequence, further size distributions are not discussed here. However, in the infrared spectral region this is not true as is demonstrated by the following �gures. Fig. 9 shows the comparison assuming HP1 with or without small particles �referred to as HP1ST and HP1� for ��3.8 �m. Fig. 10 shows the corresponding comparison for size distributions HP7 and HP7ST. Both �gures elucidate signi�cant di�erences. The general shape of the phase functions did not change, but adding small particles results in larger p��� for any scattering angle larger than approximately 10� �full lines�. Accordingly, the forward scattering peak is somewhat reduced. For ��3.8 �m, p�0� is reduced from 2840 sr,1 to 2370 sr,1 �HP1� and p�0� from 669 sr,1 to 533 sr,1 �HP7�. For a second wavelength, the overall e�ect of small particles is the same, however, the di�erences are even larger �Figs. 11-12� since particle size and wavelength are of the same order of magnitude. In particular, the forward scattering peak is considerably reduced by including the small particle fraction: from 590 sr,1 to 534 sr,1 �HP1� and from 196 sr,1 to 29 sr,1 �HP7�. As a conclusion, small ice crystals signi�cantly in�uence the scattering function of cirrus clouds: forward scattering is reduced whereas scattering in the backward hemisphere increases. The variability of the phase function with the particle size is also enlarged when compared to Figs. 6 and 7. 24 Section 3: Scattering Properties of Ice Clouds Figure 8: Phase function vs. scattering angle � for ��0.635 �m for size distributions HP1 and HP1ST. Figure 9: Phase function vs. scattering angle � for ��3.8 �m for size distributions HP1 and HP1ST. Section 3: Scattering Properties of Ice Clouds 25 Figure 10: Same as Fig. 9, but size distributions HP7 and HP7ST. Figure 11: Phase function vs. scattering angle � for ��8.7 �m for size distributions HP1 and HP1ST. 26 Section 3: Scattering Properties of Ice Clouds Figure 12: Same as Fig. 11, but size distributions HP7 and HP7ST. Consequently, changes of the asymmetry parameter are also expected. 3.5 Asymmetry Parameter and Single Scattering Albedo The single scattering albedo !0 and the asymmetry parameter g are two optical properties relevant for radiative transfer. The single scattering albedo is the ratio of the scattering coe�cient and the extinction coe�cient. The smaller !0 the stronger is the absorption. The asymmetry parameter is derived from the phase function and can be interpreted as the expectation value of the cosine of the scattering angle. It is de�ned as Z1 1 g�2 p��� cos � d�cos �� �6� ,1 In many radiative transfer calculations g replaces the full information inherent in the phase function p���. This reduces computing time signi�cantly at the expense of an information loss on the angular distribution of the radiances. Nevertheless, comparison of g for di�erent particle ensembles is a good indicator for the variability of the scattering characteristics of the medium. Asymmetry parameters and single scattering albedoes are listed for selected wavelengths in the following tables. Tab. 5 gives the values for the eight HP-size distributions �partcles 27 Section 3: Scattering Properties of Ice Clouds Size Dist. HP1 HP2 HP3 HP4 HP5 HP6 HP7 HP8 ��0.635�m !0 g 0.999 983 0.999 984 0.999 982 0.999 985 0.999 990 0.999 989 0.999 994 0.999 990 0.797 0.796 0.801 0.792 0.780 0.782 0.773 0.780 Table 5: Single scattering albedo and asymmetry parameter for eight size distributions HP1 to HP8 for ��0.635 �m. larger than 20 �m� for the central wavelength of a SEVIRI channel in the visible spectral range, ��0.635 �m. It can be seen, that absorption is extremely low, i.e., !0 �1 and that g is in the range between 0.77 and 0.80, i.e., the variability of g is very small. This result could already be anticipated from visual inspection of Fig. 5. In the following we want to focus on the central wavelengths of the IR 3.8 and IR 8.7 � the wavelength dependence within each channel which is of interest for the radiative transfer calculations will be discussed later. For the center of channel IR 3.8, single scattering albedoes and asymmetry parameters are given in Tabs. 6 and 7, �fth column. Compared to the visible spectral range, !0 is smaller and g is larger. The variability with the size distribution is considerable for both parameters: 0.60 � !0 � 0.77, and 0.85 � g � 0.93. This example shows that a simple relationship between p�0� �which was considerably larger in the visible; see above� and g does not exist. The reason for this variation is that di�erent particle sizes contribute in a di�erent way to the total scattering and extinction properties of the particle-ensemble according to their relative number. Both HP-ST size distributions reveal signi�cant di�erences compared to their corresponding counterparts. !0 is larger, g is smaller than in case of the original HP distributions. The e�ect is particularly strong if the amount of relatively small particles is already large �HP7ST�. Note that the e�ect of regarding or disregarding small particles �e.g., HP1 vs. HP1ST� is larger than the variability between the di�erent HP distributions �e.g., HP1 vs. HP2 vs. HP3 etc.�. For the central wavelength of SEVIRI channel IR 8.7, single scattering albedoes !0 and 28 Section 3: Scattering Properties of Ice Clouds Size Dist. HP1 HP1ST HP2 HP3 HP4 HP5 HP6 HP7 HP7ST HP8 ��3.4�m 0.551 0.567 0.551 0.551 0.551 0.554 0.554 0.558 0.629 0.555 ��3.5�m 0.563 0.596 0.563 0.557 0.561 0.584 0.581 0.602 0.733 0.585 ��3.6�m !0 0.592 0.632 0.592 0.580 0.590 0.633 0.628 0.667 0.809 0.635 ��3.8�m 0.617 0.659 0.618 0.602 0.616 0.671 0.664 0.771 0.846 0.672 ��4.0�m 0.594 0.635 0.594 0.581 0.592 0.639 0.633 0.675 0.817 0.640 ��4.2�m 0.576 0.616 0.576 0.566 0.574 0.612 0.608 0.642 0.786 0.613 Table 6: Single scattering albedo for di�erent size distributions and six wavelengths from SEVIRI channel IR 3.8. Size Dist. HP1 HP1ST HP2 HP3 HP4 HP5 HP6 HP7 HP7ST HP8 ��3.4�m ��3.5�m ��3.6�m 0.943 0.923 0.943 0.945 0.943 0.937 0.938 0.933 0.856 0.937 0.940 0.905 0.940 0.945 0.941 0.924 0.926 0.911 0.796 0.923 0.925 0.884 0.925 0.943 0.927 0.895 0.899 0.873 0.759 0.895 g ��3.8�m ��4.0�m ��4.2�m 0.914 0.874 0.914 0.926 0.916 0.879 0.883 0.855 0.749 0.878 0.930 0.890 0.930 0.939 0.932 0.902 0.905 0.881 0.767 0.901 0.941 0.902 0.941 0.948 0.943 0.919 0.922 0.902 0.785 0.918 Table 7: Asymmetry parameter for di�erent size distributions and six wavelengths from SEVIRI channel IR 3.8. 29 Section 3: Scattering Properties of Ice Clouds Size Dist. HP1 HP1ST HP2 HP3 HP4 HP5 HP6 HP7 HP7ST HP8 !0 ��8.3�m ��8.5�m ��8.7�m ��8.9�m ��9.1�m 0.561 0.598 0.560 0.552 0.558 0.588 0.585 0.612 0.753 0.589 0.560 0.597 0.560 0.552 0.558 0.588 0.584 0.611 0.753 0.588 0.560 0.597 0.560 0.552 0.558 0.588 0.584 0.612 0.754 0.589 0.560 0.597 0.559 0.551 0.557 0.587 0.584 0.611 0.754 0.588 0.558 0.596 0.558 0.550 0.556 0.586 0.582 0.609 0.751 0.587 Table 8: Single scattering albedo for di�erent size distributions and �ve wavelengths from SEVIRI channel IR 8.7. asymmetry parameters g are given in Tabs. 8 and 9, fourth column. The single scattering albedo is even lower and the asymmetry parameter is larger than at ��3.8 �m. Again, di�erences among the eight size distributions occur, however, they are not as pronounced as in the previous case. Typical values for g are 0.93, for !0 0.56. Concerning the e�ect of particles smaller than 20 �m, the conclusions drawn from the calculations at ��3.8 �m are con�rmed. Summarizing, we strongly recommend to apply size distributions which include the full spectrum of ice crystal sizes though small particles are di�cult to be detected. The uncertainty in estimating asymmetry parameters and single scattering albedoes for a speci�c cloud due to the unknown size distribution certainly introduces errors, however, using optical parameters calculated from uncomplete measurements of the size spectrum will introduce even larger errors. 3.6 Wavelength Dependence in SEVIRI Channels To investigate the variability of optical properties of cirrus clouds, we have calculated phase functions p���, single scattering albedoes !0 and asymmetry parameters g for di�erent wavelengths within selected channels. This answers the question about the number of wavelengths for which optical properties should be provided for the radiative transfer calculation. In this section the 3.8- and 8.7-�m-channels are discussed in more detail. 30 Section 3: Scattering Properties of Ice Clouds Size Dist. HP1 HP1ST HP2 HP3 HP4 HP5 HP6 HP7 HP7ST HP8 g ��8.3�m ��8.5�m ��8.7�m ��8.9�m ��9.1�m 0.947 0.905 0.947 0.953 0.948 0.927 0.929 0.911 0.780 0.926 0.948 0.907 0.948 0.954 0.949 0.928 0.930 0.913 0.782 0.927 0.948 0.907 0.949 0.955 0.950 0.929 0.931 0.913 0.782 0.928 0.949 0.908 0.949 0.955 0.950 0.929 0.923 0.914 0.783 0.929 0.950 0.909 0.950 0.956 0.951 0.931 0.933 0.916 0.784 0.930 Table 9: Asymmetry parameter for di�erent size distributions and �ve wavelengths from SEVIRI channel IR 8.7. A �rst indication of the spectral variability can be derived from the wavelength dependence of the refractive index within the SEVIRI channels. Figs. 13 and 14 show the real nr and imaginary part ni of the refractive index, respectively. The spectral windows of the SEVIRI channels mentioned above are indicated by the dashed lines. It can be clearly seen that the variation of both, nr and ni , is signi�cant in the 3.8 �m region whereas it is much less pronounced around 8.7 �m. Accordingly, !0 and g also vary with the spectral band of the SEVIRI channels. Let us �rst consider the asymmetry parameter and the single scattering albedo. In Tabs. 6 and 7 g and !0 for six wavelengths within this channel are shown. The wavelengths correspond to the lower limit of the channel �3.4 �m�, the central wavelength �3.8 �m� and the upper limit �4.2 �m�. The additional wavelengths 3.5 �m, 3.6 �m and 4.0 �m have been included to allow for the strong variation of the spectral properties in the 3.7-�m-window. The corresponding numbers for the IR 8.7-channel are given in Tabs. 8 and 9. For this channel, �ve wavelengths su�ce. Tab. 6 reveals that the !0 varies considerably within the spectral band of the SEVIRI �lter. This is caused by the wavelength dependence of the refractive index in this spectral range which shows a non-monotonic behaviour �cf. Tab. 2�. There is also a variability with the size distribution. This is a consequence of the di�erent relative contributions of Section 3: Scattering Properties of Ice Clouds Figure 13: Real part of the refractive index as a function of wavelength Figure 14: Imaginary part of the refractive index as a function of wavelength 31 32 Section 3: Scattering Properties of Ice Clouds Figure 15: Phase function vs. scattering angle � for several wavelengths between 3.4 �m and 4.2 �m and size distribution HP1ST small and large particles which exhibit di�erent absorption characteristics caused by the photon path lengths in the crystals. As expected from the variability of the asymmetry parameter, the phase functions also show a wavelength dependence. The wavelength dependence of p��� in the 3.8-�m-channel is shown in Figs. 15 and 16: The �rst corresponds to size distribution HP1ST, the latter to HP7ST. It can be seen that the phase functions are quite similar. The main di�erences are the missing of haloes at 3.4 �m which is caused by the strong absorption, and the shift of the haloes with wavelength. The latter is caused by the changing refractive index of ice which in turn changes the refraction angles �Snell's law� of the photon paths inside the crystal and hence the position of the haloes. As a consequence of these �ndings, it seems to be necessary to use a certain number of di�erent phase functions �or g� and di�erent !0 within the 3.8-�m-channel and to interpolate for the wavelength steps used in the radiance sampling method. Similar results are found for 8.7 �m �see Figs. 17 and 18, however, less pronounced than in the previous case. The reason is obvious from inspection of nr ��� and ni ��� which do not change as strong as in the 3.8 �m region. Nonetheless, di�erent phase functions should Section 3: Scattering Properties of Ice Clouds 33 Figure 16: Same as Fig. 15, but size distribution HP7ST Figure 17: Phase function vs. scattering angle � for several wavelengths between 8.3 �m and 9.1 �m and size distribution HP1ST 34 Section 3: Scattering Properties of Ice Clouds Figure 18: Same as Fig. 17, but size distribution HP7ST be considered in this SEVIRI channel. We feel that �ve wavelengths as indicated in the �gures are su�cient to account for the moderate wavelength dependence of the scattering properties. Section 4: Comparison with Mie-Calculations 35 4 Comparison with Mie-Calculations Calculations of optical properties considering non-spherical particles require computationally expensive methods such as the ray-tracing approach which was used in this study. Application of the Lorenz-Mie-theory � which is equivalent to the assumption of spherical particles � reduces the amount of computer resources considerably however, it is expected that non-negligible errors are introduced. This is especially true for short wavelengths, whereas in the far infra-red the errors should be less signi�cant because the particles are smaller with respect to the wavelength. We have investigated the e�ect by performing �equivalent" Mie calculations for comparison. Two aspects must be considered in this context: an equivalent size and an equivalent size distribution must be found. We have assumed that spheres of equal cross sections best suit for a comparison. The size distribution has been approximated by the corresponding eight individual sizes that have been used in the KRIPO-calculations. The advantage of using the same � discrete � size distribution for the comparison has been rated higher than the smoothness of the phase function which is only provided when a quasi continuous size distribution is assumed. Again, we focus on wavelengths 0.635 �m, 3.8 �m and 8.7 �m. Analogously to Sec. 3 we have calculated phase functions of individual particles and of size distributions. For the sake of brevity only comparisons between phase functions determined from geometrical optics and Mie-theory are discussed in this Section in detail. The comparison of Mie- and KRIPO-calculations for wavelength 0.635 �m are shown in Figs. 19 and 20 for size distributions HP1ST and HP7ST, respectively. It is obvious that signi�cant di�erences occur. In the case of spherical particles the haloes disappear and the sideward scattering is lower. On the other hand the forward scattering peak is of the same order of magnitude because it is dominated by di�raction. Note that the oscillations of the Mie-phase function are caused by the small number of particle sizes considered. This result is valid for all size distributions used in this study � two are shown in the previous �gures. The corresponding comparison for 3.8 �m is shown in Figs. 21 and 22. Here, the di�erences between sphericity and non-sphericity are much less pronounced in the phase function. The general shape of p��� the phase functions is quite the same. However, no haloes are present and scattering at angles between 90� and 140� is again reduced but less signi�cant than in the visible part of the spectrum. Furthermore, backward scattering is reduced but only for angles very close to 180� . 36 Section 4: Comparison with Mie-Calculations Figure 19: Comparison of phase functions of spherical �dashed line� and non-spherical particles �full line�; size distribtion is HP1ST, ��0.635 �m. Figure 20: Same as Fig. 19, but size distribtion HP7ST Section 4: Comparison with Mie-Calculations 37 Figure 21: Comparison of phase functions of spherical �dashed line� and non-spherical particles �full line�; size distribtion is HP1ST, ��3.8 �m. Figure 22: Same as Fig. 21, but size distribtion HP7ST 38 Section 4: Comparison with Mie-Calculations Figure 23: Comparison of phase functions of spherical �dashed line� and non-spherical particles �full line�; size distribtion is HP1ST, ��8.7 �m. For even longer wavelengths the di�erences between the two phase functions remain small. The results for the third SEVIRI channel of interest � 8.7 �m � are shown in Figs. 23 and 24. The most signi�cant di�erence is the reduced scattering between ��50� and ��150� and the missing backward peak. Single scattering albedo and asymmetry parameter for size distributions assuming spherical particles are given in Tabs. 10 and 11. The values derived from the ray-tracing calculations are also included for comparison �taken from Tabs. 6 - 9�. The di�erences of the asymmetry parameters in general are small; even the sign changes with wavelength. The largest e�ect is visible for HP7ST at 8.7 �m which is consistent with the previous discussion of Fig. 24. Here, Mie calculations result in an overestimate of g by approximately 0.08. The extent to which g�0.78 and g�0.86 � equivalent to mean scattering angles of 39� and 31� , respectively � will a�ect upward radiances is discussed in Sec. 5.3.2. It is emphasized that both g and !0 change simulataneously. Note that there are wavelengths and size distributions where an increase of g and !0 coincides, but there are also cases where g increases while !0 decreases. Thus, one should beware of simple predictions of the radiative e�ect. 39 Section 4: Comparison with Mie-Calculations Figure 24: Same as Fig. 23, but size distribtion HP7ST � HP1ST Mie KRIPO 0.635 �m 0.879 0.791 3.4 �m 0.926 0.923 3.5 �m 0.891 0.905 3.6 �m 0.877 0.884 3.8 �m 0.884 0.874 4.0 �m 0.895 0.890 4.2 �m 0.913 0.902 8.3 �m 0.928 0.905 8.7 �m 0.936 0.907 9.1 �m 0.942 0.909 HP7ST Mie KRIPO 0.852 0.762 0.861 0.856 0.728 0.796 0.694 0.759 0.739 0.749 0.797 0.767 0.837 0.785 0.857 0.780 0.862 0.782 0.868 0.781 Table 10: Asymmetry parameter for size distribution HP1ST and HP7ST: Mie and KRIPO calculations. 40 Section 4: Comparison with Mie-Calculations � HP1ST Mie KRIPO 0.635 �m 1.000 1.000 3.4 �m 0.556 0.567 3.5 �m 0.581 0.596 3.6 �m 0.618 0.632 3.8 �m 0.664 0.659 4.0 �m 0.644 0.635 4.2 �m 0.631 0.616 8.3 �m 0.578 0.598 8.7 �m 0.576 0.597 9.1 �m 0.569 0.596 HP7ST Mie KRIPO 1.000 1.000 0.603 0.629 0.684 0.733 0.779 0.809 0.851 0.846 0.841 0.817 0.827 0.786 0.734 0.753 0.714 0.754 0.686 0.751 Table 11: Single scattering albedo for size distribution HP1ST and HP7ST: Mie and KRIPO calculations. In conclusion it can be said that the di�erences in the angular distribution of scattered radiation are signi�cant in the visible spectral range but decrease with wavelength. For SEVIRI channels IR 3.8 and IR 8.7 the di�erences are so small that errors in radiative transfer calculations are expected to be negligible in the infra-red region when Mie phase functions are applied a lieu of phase functions accounting for non-sphericity. Section 5: Radiative Transfer Calculations �IR Channels� 41 5 Radiative Transfer Calculations �IR-Channels� The radiance sampling method �Tjemkes and Schmetz, 1997� is to be used for the simulation of SEVIRI measurements. While the original version of the method is designed to handle absorption and emission but no scattering it must be updated with a multiple scattering module that accepts optical and thermodynamic properties of the atmosphere as pre-calculated by the radiance sampling method and the ray tracing technique. The required output from the multiple scattering module is a set of monochromatic radiances at the top of the atmosphere for speci�ed user angles that can be passed back to the radiance sampling method for convolution with the radiometer's �lter function and calculation of brightness temperatures within the radiometer's channels. 5.1 Discrete ordinate method The basis chosen here for calculating radiances in the scattering atmosphere is the discrete ordinates method �DOM� as described by Stamnes et al. �1988�. The DOM is derived from the radiative transfer equation �RTE� which is decomposed into Fourier components. The ordinate �cosine of the zenith angle� is discretized using a double Gau� quadrature and the vertically inhomogeneous atmosphere is subdivided into a set of homogeneous layers, thus, giving a set of 2N coupled ordinary di�erential equations with constant coe�cients where 2N is the number of discrete ordinates. The homogeneous equation system is solved by �nding eigenvalues and eigenvectors numerically. Subsequently, the order of the eigenvalue problem is halved by transformation of the equation system with the square of the eigenvalues and particular solutions are found for thermal and solar sources. Finally, the boundary conditions and atmospheric layers are incorporated. The combination of layers leads to an equation system of the order �2N � L� � �2N � L� where L is the number of layers. A scaling transformation is applied to remove positive exponentials from the solution in order to avoid numerical ill-conditioning. The advantages of DOM are: The solution of the RTE does not depend on the optical thickness, thus, the computing time is independent of the optical thickness. The solution is numerically stable. A disadvantage of the method is the di�cult to discretize ordinate in the case of strongly peaked or strongly varying phase functions. Therefore, the Delta-M-method of Wiscombe �1977� is incorporated in the model �cf. Sec. 5.2�. The vertical coordinate of the model is the optical depth which can be layered arbitrarily. Hence, the DOM program code can easily be incorporated in the radiance sampling method to be used for the calculation of the gaseous absorption at infrared wavelengths. For each wavenumber chosen by the radiance sampling method the DOM has to be run once for the 42 Section 5: Radiative Transfer Calculations �IR Channels� entire atmosphere. The number of quadrature angles to be used depends on the number of Legendre polynomials chosen to expand the phase function and must not be smaller than the latter. For a good �t of the sharply peaked phase function of ice crystals to be described here the number of Legendre polynomials must be at least 50 even when using the Delta-M method. Besides the optical depths the DOM requires the single scattering albedo, the phase function expressed as coe�cients of the Legendre polynomial expansion and temperature at each level. Further input is required if solar radiation is considered. In this case the intensity of the incident parallel beam at the top boundary must be entered together with the cosine of the zenith �or polar� angle of the incident beam and the azimuth angle. The output angles are independent from the computational zenith angles and can be freely chosen. The DOM returns radiances at the speci�ed user angles and user levels. Here, the upwelling radiances at the top of the atmosphere is of concern only. The monochromatic radiances are passed back to the radiance sampling program where they are convolved with the radiometer's �lter functions. 5.2 Expansion of the phase function The phase function p��� �or p�cos ��� is introduced into the radiative transfer equation in terms of coe�cients �i of a series of Legendre polynomials Pi . p�cos �� � N X i�0 �2i + 1� �i Pi �cos �� �7� The Legendre polynomials Pi �x� can be calculated recursively according to � � � 1 � P �x� Pk+2 �x� � 2kk++23 x Pk+1 �x� , kk + +2 k with P0 � 1 and P1 � x. The coe�cients �i are determined via �i � 12 Z� 0 p�cos �� Pi �cos ��d�cos �� In general, the number of coe�cients N in Eq. �7� to accurately describe a phase function increases with increasing height of the forward scattering peak. Therefore, cirrus phase functions, where p�0� � 100 quite frequently occur, require N of at least 1000. As a consequence, memory and time resources of radiative transfer calculations are extremely high and thus not very e�ective. Section 5: Radiative Transfer Calculations �IR Channels� 43 Figure 25: Phase function of size distribution HP1ST for 8.7 �m �full line� and reconstructed from a Legendre expansion with 1000 coe�cients As an example, the HP1ST phase function has been expanded in a Legendre series and reconstructed using N �1000 or N �1800 coe�cients; the results in comparison to the original phase function are shown in Figs. 25 and 26. It can be seen that applying 1800 coe�cients almost perfectly represents the original p���, N �1000 is still acceptable. The reason for this large number of terms is the magnitude of the forward scattering peak which is in the range of 200 to 600 sr,1 as has been shown in Sec. 3.4. For shorter wavelengths even larger N are required because of the increasing di�raction peak. This problem can be solved by applying the so called `Delta-Approximation' �Potter, 1970�. If most photons are scattered in forward direction scattered and unscattered photons are redistributed according to the idea that photons which are scattered exactly in forward direction or under very small scattering angles �� � �0 � cannot be distinguished from unscattered photons. Thus, forward scattered photons are added to the unscattered photons while � for compensation � the extinction coe�cient and the optical depth are reduced accordingly, and the phase function is substituted by a `truncated' one without the extreme forward scattering peak of the original phase function. As a consequence, the new `truncated' phase function requires a much smaller number of Legendre coe�cients and the radiative transfer calculation becomes much more e�ective. 44 Section 5: Radiative Transfer Calculations �IR Channels� Figure 26: Phase function of size distribution HP1ST for 8.7 �m �full line� and reconstructed from a Legendre expansion with 1800 coe�cients The truncation of the phase function is arbitrary to a certain degree. To avoid this ambiguity Wiscombe �1977� proposed a special version of this approach called the 'Delta-MMethod'. Here, the truncated fraction of the phase function and the �remaining� number M � N of Legendre coe�cients are related. In summary, the basic equations of the Delta-M-Method read as � 0 � �1 , !0 f �� for the transformation of the optical depth, !00 � 1 1,,! f f !0 0 for the single scattering albedo and p0 �cos �� � 2f��1 , cos �� + �1 , f � MX ,1 i�0 �2i + 1��i0 Pi �cos �� for the `more di�use' �truncated� phase function p0 that substitutes the original p. The advantage of p0 over p is that p0 does not require such a large number of Legendre coe�cients. Section 5: Radiative Transfer Calculations �IR Channels� 45 Figure 27: Phase function of size distribution HP1ST for 8.7 �m �dashed line� and the reconstructed �full line, Delta-M-Method, M �100�. The truncated fraction of the phase function f is set to f � �M �8� and the coe�cients �i0 are related to the previous ones according to �i0 � �1i ,, ff In contrast to the conventional Delta-Approximation the `Delta-M Method' does not explicitely require a �0 . By choosing an upper limit of the Legendre expansion, M , e.g. M �50, factor f is determined `automatically' via Eq. 8. Figs. 27 and 28 show the results when M �100 and M �50 are chosen, respectively. Though 100 coe�cients result in a much better retrieval of the original phase function we feel that 50 coe�cients are still su�cient. A corresponding sensitivity study is brei�y discussed in Sec. 5.3. It should be emphasized that in the visible spectral range M �100 will not be su�cient to describe cirrus phase functions. 46 Section 5: Radiative Transfer Calculations �IR Channels� Figure 28: Phase function of size distribution HP1ST for 8.7 �m �dashed line� and the reconstructed �full line, Delta-M-Method, M �50�. 5.3 Radiances at Top of Atmosphere The e�ect of cirrus clouds on the radiation �eld at the top of the atmosphere in the SEVIRI channels is calculated after having completed the provision of input data �mainly phase functions� and the modi�cation of the numerical tools as described in Sec. 5.1. The focus is put again on channels IR 3.8 and IR 8.7. If not otherwise stated the zenith angle of observation is assumed to be 0� . Calculations are made for di�erent phase functions �i.e., size distributions�, di�erent optical depths of the clouds, di�erent cloud heights and di�erent climatological temperatureand water vapour pro�les �from the tropics to the mid-latitudes�. Furthermore, we have studied the e�ect of the satellite's viewing angle for a limited number of cases. In all calculations following we have expressed radiances in terms of brightness temperature TB . 5.3.1 Dependence on Cloud Optical Depth The �rst examples concern the e�ect of the cirrus optical depth �c on brightness temperature. Fig. 29 shows the change of brightness temperature �TB at the top of the atmosphere Section 5: Radiative Transfer Calculations �IR Channels� 47 Figure 29: Change of brightness temperature with �c �3:8�m�; size distribution HP1ST, ��3.8 �m �dashed line�, ��8.7 �m �full line�. de�ned as �TB � TB ��c � , TB ��c � 0� for 0.01 � �c � 10. A vertical temperature and humidity pro�le from 50.0� N, 20.2� E �TIGR pro�le �469� has been taken. The cloud height is set to model-level �15, i.e., between 300 and 250 hPa �approximately 9.6-11 km�. From Fig. 29 it can be seen that the absolute value of �TB increases with optical depth. The optical depth shown is �c at 3.8 �m. For the purpose of this plot it can also be taken for ��8.7�m � the relative di�erences of the optical depth at both wavelength is between 2 and 3 �; only slightly depending on the size distribution. The larger �c, the lower is the brightness temperature TB , i.e, the stronger is the cloud e�ect. For 8.7 �m the cloud e�ect is larger than for 3.8 �m; for an optical depth of �c � 0:1, TB decreases by 1.48 K or 0.84 K, respectively, relative to the no-cloud reference case. For subvisible cirrus clouds with optical depth as low as 0.01, �TB is 0.15 K for 8.7 �m and 0.08 K for 3.8 �m. 48 Section 5: Radiative Transfer Calculations �IR Channels� Size Dist. HP1 HP1ST HP7 HP7ST ST reff 91.7 78.0 30.7 11.9 5.0 Table 12: E�ective radii for di�erent size distributions. 5.3.2 Dependence on Size Distribution The e�ect of the size distribution on �TB is relatively small. Two examples are shown here. In Fig. 30 the change in brightness temperature is shown for �ve size distributions: two realisitic including the full spectrum of small and large particles, �HP1ST and HP7ST�, two without small particles below 20 �m �HP1 and HP7� and the size distribution with only small particles �ST�. The wavelength is ��3.8 �m. For illustration, the e�ective radii of the di�erent size distributions are displayed in Tab. 12. In particular, size distributions ST consists of very small particles typical rather for contrails than for �natural" cirrus clouds. That was the reason why we did not account for the ST-size distribution in the previous sections. If size distributions HP1, HP1ST and HP7 are considered, di�erences are below 0.2 K as long as �c � 0.2. For �c�1 the di�erences are still only approximately 0.7 K, and maximum deviations occur at �c �2 with 1.2 K. Including size distributions with very small e�ective radii �HP7ST and in particular ST� the sensitivity of the irradiance to the microphysics is increasing. For optical depths of �c�0.1, the variability is about 0.3 K, for �c �1 it is up to about 3 K, and more than 6 K for �c�2. In Fig. 31 the corresponding results for ��8.7 �m are plotted. The same conclusions hold. Note, that in both �gures the cloud e�ect is interpolated between �c�2 and �c �10. An interesting question already raised in Sec. 4 is the error of the radiance at the top of the atmosphere when Mie-phase functions are applied instead of more realistic ones. The error �TB is de�ned as �TB � �TB�M � ��c� , �TB�K ���c� Section 5: Radiative Transfer Calculations �IR Channels� 49 Figure 30: Change of brightness temperature as a function of cloud optical depth for di�erent size distributions as indicated; ��3.8 �m. Figure 31: Same as Fig. 31, but ��8.7 �m. 50 Section 5: Radiative Transfer Calculations �IR Channels� Figure 32: Error in brightness temperature as a function of �c when Mie-phase functions are used; ��3.8 �m �see text�. The superscripts �K � and �M � mark brightness temperature di�erences calculated assuming KRIPO- and Mie-phase functions, respectively. Negative �TB means an underestimate of the brightness temperature in the case of spherical particles, i.e., the reduction of TB by the cloud is overestimated. From Figs. 32 and 33 it can be seen that the error is small, but not negligible. For ��3.8 �m, �TB is as large as 0.22 K �for �c � 2�, for 8.7 �m it changes sign and the absolute values reach 0.14 K. The e�ect of di�erent crystal size distributions �considering the full spectrum of small and large crystals� is so small in comparison that it can hardly be resolved in the �gures. That means that the errors caused by the assumption of spherical particles are much larger than the errors which might occur if a wrong size distribution of a natural cirrus cloud �e.g., HP1ST instead of HP7ST� is used. This conclusion might be changed if contrails are considered. 5.3.3 Dependence on Cloud Height The e�ect of the cloud height is shown in Fig. 34 ���3.8 �m� and Fig. 35 ���8.7 �m�. The optical depth of the cloud is �c�1 in both cases. The horizontal lines show the layers of the atmospheric model �TIGR �194, i.e., 1.2� N latitude, 172.6� E longitude�. Section 5: Radiative Transfer Calculations �IR Channels� 51 Figure 33: Same as Fig. 32, but ��8.7 �m. The cloud is shifted from layer �17 �200-150 hPa� to �20 �115-100 hPa�. It can be seen that the upward radiance remains almost unchanged in SEVIRI channel IR 3.8, but not in IR 8.7. At 3.8 �m, the cloud e�ect �TB is almost constant with height: �10.04 K if the cloud is in layer �17; �10.13 K for layer �20. For 8.7 �m however �TB changes by almost one degree, i.e., from �18.24 K to �19.32 K �layer �17 to �20�. 5.3.4 Dependence on Satellite Zenith Angle The dependence of the radiances at the top of the atmosphere from the zenith angle of observation was investigated between �s�0� and 60� . Results are shown in Fig. 36. A cirrus cloud is assumed in layer �15 with an optical depth of 0.1 �TIGR pro�le �469�. �TB is plotted for ��3.8 �m and ��8.7 �m. It is obvious that the in�uence of the cloud increases as the zenith angle increases. This is caused by the longer photon paths through the clouds. 5.3.5 In�uence of Phase Function Expansion We have also investigated whether 50 terms of the Legendre expansion are su�cient for describing the scattering properties of the cloud. For this purpose few runs are made with M �100. 52 Section 5: Radiative Transfer Calculations �IR Channels� Figure 34: Vertical pro�le of brightness temperature for di�erent cloud heights; ��3.8 �m. Figure 35: Vertical pro�le of brightness temperature for di�erent cloud heights; ��8.7 �m. Section 5: Radiative Transfer Calculations �IR Channels� 53 Figure 36: Change of brightness temperature with satellite zenith angle; �c�0.1. The computer time required for one run �one optical depth� is approximately 55 minutes on a DEC-Alpha-Station �128 MB RAM, 233 MHz� when the phase functions is approximated by 50 Legendre coe�cients. If M is set to 100, an Alpha-Station with 512 MB RAM and 300 MHz must be used and though the computer time increases by a factor of approximately 3. Typical radiative transfer calculations have shown that increasing the computer resources to consider more Legendre-terms is not necessary. The changes in the brightness temperature are virtually zero. 5.4 Justi�cation of scattering The strong contribution of forward scattering to the totally scattered radiation and the impossibility to distinguish photons scattered in forward direction from unscattered ones that are transmitted in the same direction might suggest to ignore the scattering completely. This is tested by comparing calculations accounting for full scattering with those where the optical depth is reduced by that of the scattering and where only absorption and emission is considered. The optical depth has been �xed to 0.1, the cloud is inserted in a topical atmosphere near 100 hPa. The test calculations show that scattering becomes increasingly important when the single 54 Section 5: Radiative Transfer Calculations �IR Channels� scattering albedo increases. At !0 � 0:6 the brightness temperature di�erences between scattering and non-scattering case at the top of the atmosphere are less than �TB � ,0:08 K. For !0 � 0:7, 0.8, 0.955 we have maximum di�erences of �TB ��0.13, �0.84, and �7.5 K, respectively. Hence, even in cases with strong forward scattering the scattering cannot be ignored when !0 exceeds values of about 0.6. 5.5 Discussion Brightness temperatures have been calculated for two SEVIRI channels in the infrared. It was found that the decrease of TB in the presence of a cloud is smaller at 3.8 �m than at 8.7 �m. The reason is primarily based on the higher single scattering albedo and lower imaginary part of the refractive index �lower absorption�emission�, respectively, at 3.8 �m. TB are virtually the same if size distributions with reff � 30 �m are considered. Largest � but still small � e�ects occur at moderate optical depths around 2. For very large �c the di�erences become smaller again as the brightness temperature approaches the thermodynamical temperature at the cloud's altitude. In case of anthropogenic cirrus clouds �contrails� the size distributions are shifted signi�cantly towards smaller particles. Only such drastical changes lead to a clearly visible e�ect in the brightness temperatures. Summarizing, if size distributions measured by Heyms�eld and Platt and extended by measurements of Strauss are accepted to be typical for natural cirrus clouds, the e�ect of size distributions on TB is small. This is in part caused by the similarity of the size distributions, i.e. they all cover the full range of sizes from a few micrometers to some millimeters. Another reason for the small di�erences is the opposite change of g and !0 when � for example � size distributions HP1ST and HP7ST are considered �see Tabs. 10 and 11�. In the spectral region between 3.4 �m and 4.2 �m, g decreases from about 0.90 to 0.78 while !0 increases from 0.62 to 0.76. Both e�ects tend to cancel out each other: the increase of !0 leads to a lower emission of the cloud and thus to a stronger contribution from atmospheric layers and the surface. Hence, there is a tendency to increase TB . On the other hand the decrease of the asymmetry parameter results in a stronger backscattering of radiation coming from below the cloud so that there is a tendency of blocking the radiation from the warm �in comparison with the cloud� surface. Both e�ects act non-linearity so that a quantitative estimate of the overall e�ect "by eye" is not possible. The radiative transfer calculations however have demonstrated that the overall e�ect indeed is small. Section 5: Radiative Transfer Calculations �IR Channels� 55 We have also compared our results with calculations performed by Betancor-Gothe and Gra�l �1993�. They have investigated the radiative in�uence of thin cirrus clouds and contrails in the 3.8 �m spectral region. Their study focussed on contrails so that they selected phase functions C1 and C5 which only consists of particles less than 20 �m and 40 �m, respectively. Furthermore, they used a HP size distribution similar to our assumptions. Phase functions determined from Mie theory and a correction scheme were used. The e�ective radii of the three phase functions �C1, C5, HP� were 4 �m, 6 �m and 100 �m, respectively. Thus, comparisons with our ST- and HP1-size distribution are possible. The general behaviour of their and our TB ��c �-curves is the same. In particular, there is a clear separation between the size distributions with very small and large e�ective radii. Furthermore, both studies show a smaller e�ect on TB in case of small particles �contrails�. Calculating �TB ��c � 2� from Betancor-Gothe and Gra�l's paper we get values of approximately �18 K for their HP cloud, and �10 K for the C1 or C5 contrail. These values agree very well with the corresponding values of our calculations �16.7 K and �10.9 K, respectively. Moreover, the decrease of the brightness temperatures relative to the no-cloud reference case is in both studies approximately �32 K for �c �3.5 �interpolated value�. Larger optical depths were not investigated by Betancor-Gothe and Gra�l �1993�. 56 Section 6: Radiative Transfer Calculations �VIS Channel� 6 Radiative Transfer Calculations �VIS-Channel� We have also calculated the e�ect of cirrus clouds in the VIS 0.6 SEVIRI channel. The concept resembles in many aspects the calculations of Sec. 5 for the IR spectral region, however, another radiative transfer code was used. It is brie�y described in the following section. 6.1 Method of Successive Order of Scattering The radiative transfer calculations for wavelength ��0.635 �m were performed with a successive order of scattering �SOS� model. The SOS is based on the monochromatic radiative transfer equation including multiple scattering. The radiances are expanded in a series of Fourier coe�cients � a typical number is 20. For each coe�cient the radiative transfer equation is solved, separately for the upward and downward looking hemispheres. The phase function is treated in the same way as described in the previous section, i.e, it is expanded in a Legendre polynomial series. Finally, a set of coupled di�erential equations is obtained which is solved iteratively. As a consequence, the contribution of each scattering order to the radiance �eld can be determined. Thus, each step of the SOS model can be attributed to a physical meaning. The iteration is stopped when the di�erence between the irradiance and the irradiance of the previous iteration step is smaller than a prescribed threshold. The convergence of the iteration slows down with increasing optical depth, however, for � � 1, approximately 10 scattering orders are su�cient. The SOS is a one-dimensional radiation code with optical depth � as variable. The vertical layers �i.e., layers of � � are de�ned in terms of height and extinction coe�cients � if optically thick layers occur they are subdivided into smaller layers. Scattering by air molecules, aerosols and clouds is considered. As already mentioned, cirrus phase functions require � caused by the pronounced forward scattering peak � the application of �a version of� the Delta-approximation. In contrast to the DOM �IR-calculations, Sec. 5.1� we apply the standard Delta-approximation. Output of the model are radiances are determined at arbitrary levels of the atmosphere as a function of azimuth and zenith angle of observation, for a �xed but arbitrary solar zenith angle. Section 6: Radiative Transfer Calculations �VIS Channel� 57 6.2 Radiances at the Top of the Atmosphere Calculations of the radiance �eld at the top of the atmosphere were performed for ��0.635�m. The surface albedo was set to 15�. In the troposphere we assume continental aerosols, in the stratosphere background aerosols. The solar zenith angle �0 is set to 30� or 60� . 31 coe�cients were considered for the radiance expansion, 181 for the truncated phase function. Results are expressed in terms of planetary albedo �pl . This is a more convenient measure than radiances if the radiative impact of di�erent clouds on the radiation �eld should be compared. On the other hand they can easily be transformed into irradiances and radiances. The conversion of planetary albedo to upward directed spectral irradiances S at the top of the atmosphere is simply performed by S � �0 �pl So with So being the extraterrestial spectral solar radiation at the selected wavelength and �o the cosine of the solar zenith angle. At ��0.635 �m So equals 1658 W m,2 �m,1 �WMO, 1986�. Spectral radiances L are determined by division through � � provided the radiation �eld is isotropic. Thus, Liso is proportional to the planetary albedo. Liso � �o ��pl So Though this is not exactly true in the case of cirrus clouds �as will be seen below� this approximation is quite useful to describe cloud e�ects and their sensitivity to microphysical properties. The reason is that the anisotropy function � ��; '� �bidirectional re�ection distribution function; � and ' being the zenith angle and azimuth angles of observation, respectively� does not change so much for a given viewing geometry in comparison to the planetary albedo. Tab. 13 gives the planetary albedo �pl for ��0.635 and a surface albedo of 15�. The cloud base height is 9.5 km, cloud top height 11 km. Listed are values for di�erent cloud optical depths and phase functions: four size distributions �namely HP1ST and HP7ST and their �counterparts" without small particles� are considered and two particle shapes �hexagonal columns, KRIPO; and spheres, Mie�. 58 Section 6: Radiative Transfer Calculations �VIS Channel� �c Mie-Theory KRIPO �GOA� HP1 HP1ST HP7 HP7ST HP1 HP1ST HP7 HP7ST 0. 16.8 0.05 16.9 17.0 16.8 17.0 17.1 17.1 17.1 17.2 0.1 17.0 17.1 17.0 17.2 17.4 17.5 17.5 17.5 0.5 18.0 18.2 18.3 19.2 19.9 20.0 20.3 20.4 1.0 19.5 19.8 19.9 21.8 23.1 23.3 23.9 24.2 Table 13: Planetary albedo in percent for a cirrus cloud �9.5 � 11 km�. ��0.635 �m, �0 �30� . In the cloudfree case, a planetary albedo of 16.8 � is derived. This corresponds to a spectral radiance of 76 W m,2 sr,1 �m,1 . It can be seen that the planetary albedo increases with cloud optical depth for all phase functions. However, the increase is di�erent for di�erent phase functions: in case of non-spherical particles �KRIPO algorithm� the radiation leaving the atmosphere is generally larger than in the case of spherical particles. The absolute di�erence is 4� for the HP7-distribution and about 2.5� for HP7ST when the cloud optical depth is 1. A 1�-albedo change is equivalent to a change in �isotropic� spectral radiance of about 4.6 W m,2 sr,1 �m,1. For thin cirrus clouds ��c � 0.1� the change of the albedo is less than 0.5 �. The variability with size distribution �HP1ST vs. HP7ST etc.� is relatively small; even for �c�1 it is less than 1� in case of KRIPO. For spherical particles the di�erences amount up to about 2�. These �ndings are in accordance with the phase functions shown in Fig. 5 � small variability of p��� with size distribution � and in Figs. 19 and 20 � large di�erences between Mie- and KRIPO-phase functions. Furthermore, the enhanced sideward and backward scattering of the non-spherical particles is obvious which corresponds to the larger planetary albedo. In case of larger solar zenith angles ��0 �60� � shown in Tab. 14, the planetary albedo is larger caused by the longer photon paths through the atmosphere, and the increase of �pl with cloud optical depth is stronger. The cloudfree planetary albedo of 19.3 � corresponds to an �isotropic� radiance of 51 W m,2 sr,1 �m,1 ; 1�-albedo to a radiance of about 2.6 W m,2 sr,1 �m,1. Again, the planetary albedo of non-spherical particles is larger than in case of spheres. That means that using Mie phase functions leads to an underestimate of �pl of 2-4� ��c �1�. Section 6: Radiative Transfer Calculations �VIS Channel� 59 �c Mie-Theory KRIPO �GOA� HP1 HP1ST HP7 HP7ST HP1 HP1ST HP7 HP7ST 0. 19.3 0.05 19.8 19.8 19.9 20.0 20.1 20.1 20.1 20.2 0.1 20.3 20.3 20.3 20.7 20.8 20.8 20.9 21.1 0.5 24.0 24.2 24.3 26.2 26.5 26.7 27.2 27.5 1.0 28.4 28.7 29.0 32.2 32.6 32.9 33.6 34.2 Table 14: Same as Tab. 13, �0 �60� . These �ndings in general agree with results � integrated over the solar spetral range � published by Kinne und Liou �1989�. As already mentioned the radiance �eld is anisotropic in case of clouds. This anisotropy must be taken into account when speci�c viewing geometries of satellite, ground pixel and sun are of interest. The angular dependence of the radiance L��; '� is described by L��; '� � � ��; '� Liso � � �0 ��pl So The bidirectional re�ection function � is derived by normalizing the radiances obtained from the SOS runs. Typical distributions of � show large values �scattering stronger than in the isotropic case� for large zenith angles of observation �. This is in particular true for small and large �forward and backward scattering� azimuth angles. Over sea surfaces a pronounced sunglint is visible ��o � �; ' � 0�. In case of clouds often a �hot spot" appears at ��o � �; ' � 180�. We have plotted four typical examples of the anisotropy function � . On one hand we show the changes of the overall pattern when the solar zenith angle changes, on the other hand we show that the pattern signi�cantly changes when spherical particles are assumed a lieu of hexagonal crystals �Mie vs. KRIPO�. Figs. 37 and 38 show the normalized angular distribution of the radiances for ��30� and ��60� , respectively. The cloud optical depth is set to unity, and size distribution HP1 is assumed. Fig. 37 shows that near zenith �� � 0� � the sky appears relatively dark while for large zenith angles of observation the sky becomes brighter. This is in particular true for forward scattering with respect to the sun �small '-angles� as expected. In backward 60 Section 6: Radiative Transfer Calculations �VIS Channel� Figure 37: Anisotropy function � ��; '� for size distribution HP1 �KRIPO model�; �o �30� . Figure 38: Same as Fig. 37, but �o �60� . Section 6: Radiative Transfer Calculations �VIS Channel� 61 Figure 39: Anisotropy function � ��; '� for size distribution HP1 �Mie calculations�; �o �30� . scattering direction at ��30� the hot spot can clearly be seen. This is a consequence of the strong backward scattering of ice crystals as has already been shown in �e.g.� Fig. 5. Similar scattering pattern are visible in Fig. 38 where the results for �o �60� are shown. In general, the dark and bright regions of the sky appear at similar angles, however, the �amplitude" of � is larger. The area of enhanced backscattering now has moved to larger zenith angles according to the position of the sun. Figs. 39 and 40 show a similar comparison, however, spherical particles have been assumed. As a �rst approximation, the normalized radiances increase with the zenith angle of observation as has been the case in the KRIPO calculations. Two main di�erences occur: �rst, a �ring" of large radiances around the position of the anti-point of the sun is visible which corresponds to the relative maximum of the phase function at � � 135� �cf. e.g. Fig. 19�. Second, the hot spot has vanished. This is caused by the reduced backscattering of spheres in comparison with hexagonal columns. The in�uence of di�erent crystal size distributions, HP1, HP1ST, HP7 and HP7ST, on the angular distribution has also been investigated. Only one example is illustrated: Fig. 41 is compared to Fig. 37, i.e., HP1 and HP7ST. It is obvious that the general pattern is very much alike. Di�erences appear in several 62 Section 6: Radiative Transfer Calculations �VIS Channel� Figure 40: Same as Fig. 39, but �o �60� . Figure 41: Anisotropy function � ��; '� for size distribution HP7ST �KRIPO model�; �o �30� . Section 6: Radiative Transfer Calculations �VIS Channel� 63 small-scale features which however are primarily based on the isoline routine of the plot program. Same results are found for the other size distributions. In summary, applying phase functions based on Mie theory introduces signi�cant errors in the calculated angular distributions of upward radiances at ��0.635 �m. The di�erences between variuos realistic cirrus particle size distributions however are very small. 64 Section 7: Summary and Conclusions 7 Summary and Conclusions Radiation scattered by cirrus clouds in�uence radiances measured at the top of the atmosphere. It was the objective of this study to develop numerical tools to describe this e�ect for three channels �at 0.635 �m and in the infrared spectral region at 3.8 �m and 8.7 �m� of SEVIRI, a radiometer which is planned to be �own as part of METEOSAT Second Generation. Since ice clouds consist of non-spherical crystals, application of the Lorentz-Mie theory to describe scattering is not adequate. Thus, more complicated models are required and the computations become more expensive. In a �rst step we have adapted a ray tracing model �KRIPO�, based on the geometric optics approach and developed by Hess, for the wavelengths of SEVIRI. KRIPO provides optical properties of individual particles, in particular, phase function and the single scattering albedo. The resulting data sets for hexagonal columns serve as input for a second program which determines phase function, asymmetry parameter g and single scattering albedo !0 for di�erent size distributions known from literature. With these two numerical tools the data base required for the radiative transfer calculations was established for several wavelengths within each SEVIRI channel under consideration. This was done to account for the spectral dependence of the optical properties of ice particles. The basis of the radiative transfer calculations was the radiance sampling method provided by EUMETSAT which, however, does not consider atmospheric scattering. As a consequence, a more general model has been developed. This task was performed by combining the discrete ordinate method and the radiance sampling technique. This approach results in 375 to 750 full multiple scattering calculations for both SEVIRI channels. Radiances at the top of the atmosphere were calculated for di�erent cirrus optical depths, di�erent crystal size distributions, di�erent cloud heights and climatological pro�les of temperature and water-vapour distributions. The e�ect of di�erent viewing geometries is also brie�y outlined. Furthermore, the errors introduced by assuming spherical particles instead of hexagonal crystals were estimated. The main results for the infrared SEVIRI channels are the following: � For the 3.8 �m channel, brightness temperatures at the top of the atmosphere are Section 7: Summary and Conclusions 65 reduced by typically �0.08 K if a cirrus cloud of optical depth �c �0.01 is present, �0.8 K and �8.2 K, if �c equals 0.1 or 1, respectively. � For the 8.7 �m channel, brightness temperatures at the top of the atmosphere are somewhat more reduced. Typical values are �0.15 K for �c �0.01, �1.5 K for �c �0.1 and �13.7 K for �c�1. � The e�ect of di�erent crystal size distributions on the radiance at the top of the atmosphere is small in the infrared if natural cirrus clouds are considered. The inclusion of contrails with a higher concentration of small particles causes greater derivations. � Assuming spherical particles instead of hexagonal columns results in errors of approximately 0.2 K in brightness temperature. For the 0.635 �m channel the main results are � The e�ect of di�erent size distributions of natural ice clouds on upwelling radiances is small. � Application of phase functions derived from Mie theory leads to a signi�cant underestimate of upward radiances and to an erroneous angular distribution of the radiation �eld. If wavelengths of the order of 10 �m are considered, the application of the geometric optics approach is critical because the basic physical concept of this method is violated in the case of small crystals. Nevertheless, GOA is an acceptable approach as was outlined in Sec.3.1. Discrete dipole approximation might become an alternative with the advent of more powerful computers in the near future. Another computational problem raises from the need to express any phase function by a series of Legendre polynomials. In the shortwave spectral range a very large number of coe�cients is required to accurately model the pronounced forward scattering peak. This causes serious problems even if the delta approximation is applied. For wavelengths between 4 and 10 �m this problem is diminished. The e�ect of di�erent size distributions on the radiation �eld at the top of the atmosphere is � according to our calculations � negligible. Consequently, the retrieval �or a �rst-order estimate� of size distribution or particle shape seems not to be possible on the basis of the two SEVIRI channels chosen. However, the discrimination of natural cirrus from contrails should be feasibile. 66 Section 7: Summary and Conclusions This conclusion is not in contradiction to other studies. One should not be confused by recent papers which publish histograms of monthly mean e�ective particle sizes of cirrus clouds with a resolution of �reff � 4 �m �Han et al., 1996�. These results are based on AVHRR measurements in the framework of ISCCP and on an inversion scheme originally developed for water clouds. Data evaluation uses a very simple cirrus cloud detection algorithm and only �ve di�erent size distributions. Thus, the discrimination of 25 distinct reff -classes is rather a mathematical consequence than a realistic retrieval of individual particle sizes. An error analysis is missing in this paper. We did not investigate the e�ect of particle shapes other than hexagonal crystals and the e�ect of horizontally aligned crystals �oriented particles�. We do not feel that the �rst will change our conclusions, however, the latter might be subject to further investigations. Such investigations would not only require even more complex models for the scattering characteristics of a particle. In addition, radiative transfer models must be extended signi�cantly: �rst, the models must be capable to deal with a much larger number of Legendre coe�cients �see above� to describe each angular pattern of the phase function, and second, the radiative transfer code must account for two-dimensional phase functions p��; '�. Present radiative transfer codes cannot treat this problem. It was beyond the scope of this project to thoroughly investigate the potential of discriminating di�erent cirrus clouds by SEVIRI measurements. For this purpose the full number of channels should be considered. We recommend to investigate more deeply the di�erences between natural and anthropogenic ice clouds. Due to their very di�erent size distributions a discrimination might be possible. A discrimination of di�erent types of natural cirrus clouds as we have done in this study seems to be critical. On one hand the e�ects on the radiation �eld are small caused by simultaneous changes of g and !0 . On the other hand spatial inhomogeneities of a cirrus cloud �eld at the scale of a pixel will lead to an averaging of di�erent cirrus size distributions which makes it di�cult to invert radiance measurements for microphysical properties. As a consequence, only mean properties can be derived, and an interpretation of very small di�erences in the received radiances is not necessary. 8 Acknowledgments The authors want to thank Dr. Michael Hess for the supply of his program `KRIPO' and many valuable comments. Section 9: References 67 9 References Auer, H.A. and D.L. Veal, 1970: The dimensions of ice crystals in natural clouds, J. Atmos. Sci., 27, 919-926. Betancor-Gothe, M. and H. 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