remote sensing Article Aerosol Retrievals from CALIPSO Lidar Ocean Surface Returns Srikanth L. Venkata and John A. Reagan * Department of Electrical and Computer Engineering, University of Arizona, Tucson, AZ 85721, USA; [email protected] * Correspondence: [email protected]; Tel.: +1-520-343-1105 Academic Editors: Raphael M. Kudela, Xiaofeng Li and Prasad S. Thenkabail Received: 3 August 2016; Accepted: 28 November 2016; Published: 9 December 2016 Abstract: This paper describes approaches to retrieve important aerosol results from the strong lidar return signals that are received by the space-borne CALIPSO lidar system after reflecting off-ocean surfaces. Relations, from which the theoretically expected values of area under ocean surface returns can be computed, are presented. A detailed description of the lidar system response to the ocean surface returns and the processes of sampling and averaging of lidar return signals are provided. An effective technique that reconstructs the lidar response to surface returns—starting from down-linked samples—and calculates the area under it, has been developed and described. The calculated area values are validated after comparing them to their theoretically predicted counterpart values. Methods to retrieve aerosol optical depths (AODs) from these calculated areas are described and retrieval results are presented, including retrieval comparison with independent AOD measurements made by an airborne High Spectral Resolution Lidar (HSRL) that yielded quite good agreement. Techniques and results are also presented on using the spectral ratios of the surface response areas to determine spectral ratios of aerosol round-trip transmission and AOD spectral difference, without need of a specific/accurate ocean-surface reflectance model. Keywords: lidar; CALIPSO; ocean surface reflectance; aerosol transmittance; aerosol optical depth 1. Introduction LIght Detection And Ranging (lidar) is an optical remote sensing technology which is very often used in the study of atmospheric aerosols. Similar in concept to radar, lidar emits highly coherent, ultra-short laser pulses at wavelengths which are comparable to the dimensions of atmospheric aerosol particles. This permits lidar pulses to physically interact fairly strongly with aerosols such as dust, pollen, smoke, etc. The inability of in situ instruments to make aerosol measurements on a global scale and the high variability of both spatial and temporal distributions of tropospheric aerosols drive the necessity for space-borne observations. Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) is a satellite lidar system that was launched by NASA on 28 April 2006 to improve our knowledge and understanding of the roles played by cloud and aerosol particles on Earth’s climate change. Being the first space-borne lidar dedicated to the study of aerosols, CALIPSO can make observations and measurements on a global scale that help provide insight into the factors that regulate Earth’s radiation budget. The principal goals of the CALIPSO mission are to provide global, vertically resolved aerosol microphysical properties and spatial distributions, perform height-resolved discrimination of aerosols into several types, to provide vertical layers of single and multi-layer transmissive clouds and to determine vertical distributions of cloud ice and water [1–3]. Laser pulses transmitted from the lidar system into the atmosphere are reflected back to the system as a result of back-scattering by various particles present in the propagation path of the Remote Sens. 2016, 8, 1006; doi:10.3390/rs8121006 www.mdpi.com/journal/remotesensing Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 1006 2 of 27 2 of 27 pulse. Backscatter hard targets targetssuch suchasasland landand andocean ocean surfaces pulse. Backscatterofofthe thelaser laserpulses pulsesalso also occurs occurs from from hard surfaces which result in what are referred to as “surface returns.” Surface returns are expected to be much which result in what are referred to as “surface returns.” Surface returns are expected to be much stronger than thethe atmospheric returns and carry in in them qualitative and quantitative stronger than atmospheric returns and carry them qualitative and quantitativefactors factorsabout aboutthe material medium presentpresent in the atmosphere throughthrough which the transmitted lidar pulses travelled. the material medium in the atmosphere which the transmitted lidar have pulses have This paper includes an in-depth analysis of surface returns from ocean surfaces and presents ways travelled. This paper includes an in-depth analysis of surface returns from ocean surfaces and to retrieve optical these returns. It is returns. a summary, somewith revisions and additions, presents ways to depths retrieve from optical depths from these It is a with summary, some revisions and additions, of the workby completed by the first author his M.S. of the work completed the first author for his M.S.for thesis [4]. thesis [4]. 2. Materials and Methods 2. Materials and Methods 2.1.2.1. Low-Pass Filter Low-Pass Filter The lidar system on board CALIPSO is calledisCloud-Aerosol LIdar with Orthogonal Polarization The lidar system on board CALIPSO called Cloud-Aerosol LIdar with Orthogonal (CALIOP). CALIOP employs a third-order Bessel filter Bessel with afilter bandwidth ~2.44 MHz, Polarization (CALIOP). CALIOP employs alow-pass third-order low-pass with a bandwidth as ~2.44 a partMHz, of its as post-detection electronics following thefollowing PMT detector for the 532 nm [5–7]. a part of its post-detection electronics the PMT detector for channel the 532 nm channel [5–7]. Similarelectronics, post-detection electronics, the same low-pass filter, the photodiode avalanche Similar post-detection with the samewith low-pass filter, follows the follows avalanche photodiode the 1064 nmimportant channel. feature A very ofimportant of filter this Bessel (APD) detector (APD) for the detector 1064 nm for channel. A very this Besselfeature low-pass (LPF) is low-pass filterreturn (LPF)signal is that(as foroccurs a pulse return signal (asreflection) occurs from a hard-target reflection) that for a pulse from a hard-target it preserves the area under itthe preserves the area under theenters pulse.this Thus, if aitsnarrow pulse enters this filter, itsthe peak amplitude is pulse. Thus, if a narrow pulse filter, peak amplitude is reduced but pulse is stretched reduced but the pulse is stretched in time so as to preserve the area under the original narrow pulse. in time so as to preserve the area under the original narrow pulse. This enables accurate capture of the This enables accurate capture of theathard target ocean surfacerate response the 10 MHz digitation rate hard target ocean surface response the 10 MHz digitation of theatdigitizers following the LPF. digitizers followingtime the input LPF. For a Dirac function timeintegral input toof the LPF, thefunction convolution Forofa the Dirac delta function to the LPF,delta the convolution the delta input integral of the the delta function input convolved with the LPFyields output-to-input transfer function yields convolved with LPF output-to-input transfer function the transient output known as the the transient output known as the Impulse Response Function (IRF). If the input is not a Impulse Response Function (IRF). If the input is not a delta function, but a short pulse compareddelta to the function, but a short pulse compared to the IRF response time, as is the case for the short-duration IRF response time, as is the case for the short-duration transmitted lidar pulse (~20 ns), the convolution transmitted lidar pulse (~20 ns), the convolution with the LPF transfer function still yields the ideal with the LPF transfer function still yields the ideal IRF to a very close approximation (simulations IRF to a very close approximation (simulations showed that the impulse response of the LPF for an showed that the impulse response of the LPF for an input pulse of duration of the transmitted lidar input pulse of duration of the transmitted lidar pulse yielded a response within ~0.1% of the ideal pulse yielded a response within ~0.1% of the ideal IRF). As with any linear time-invariant (LTI) system, IRF). As with any linear time-invariant (LTI) system, the third-order Bessel filter can be completely the third-order Bessel filter can be completely characterized by its IRF. characterized by its IRF. Impulse response measurements were made on flight hardware replicas of the CALIOP detector Impulse response measurements were made on flight hardware replicas of the CALIOP anddetector post-detection electronics electronics where the detector was exposed optical pulses of about duration and post-detection where the detector wastoexposed to optical pulses20 ofns about 20 to mimic the laser pulse transmitted by CALIOP [5]. The measured impulse response, averaged over ns duration to mimic the laser pulse transmitted by CALIOP [5]. The measured impulse response, many measurements, to unity area is shown in area Figure 1 [5]. The circles 1are digitized samples averaged over manyscaled measurements, scaled to unity is shown in Figure [5].the The circles are the (at digitized the 10 MHz sample thesample solid line is an analytical a hyperbolic samples (at rate), the 10and MHz rate), and the solidbest-fit line is using an analytical best-fittangent using afor thehyperbolic rising parttangent of the pulse a Gaussian curve the falling part [5]. for the falling part [5]. for theand rising part of the pulsefor and a Gaussian curve Figure Theimpulse impulseresponse responseas asdetermined determined by by lab Figure 1. 1. The lab measurements measurementsscaled scaledtotounity unityarea. area. As the transfer functions of Bessel filters are very well characterized, using the control system As the transfer functions of Bessel filters are very well characterized, using the control system tool-box of MATLAB, the ideal impulse response shape was generated (assuming the ~2.44 MHz tool-box of MATLAB, the ideal impulse response shape was generated (assuming the ~2.44 MHz Remote Sens. 2016, 8, 1006 3 of 27 Remote Sens. 2016, 8, 1006 3 of 27 bandwidth exhibited by the response). To compare the two responses (lab measured bandwidth exhibited bymeasured the measured response). To compare theimpulse two impulse responses (lab measured and MATLABthey generated), they to arehave scaled to same have the same area (unity) and are plotted in and MATLAB generated), are scaled the area (unity) and are plotted in Figure 2. Figure 2. It can be concluded that, within a very close approximation, the impulse response of the It can be concluded that, within a very close approximation, the impulse response of the CALIOP CALIOP receiver electronics does indeed replicate the IRF for Bessel a third-order Bessel receiver electronics does indeed replicate the theoretical IRFtheoretical for a third-order low-pass transfer low-pass transfer function (and the areas found using either impulse response curve to obtain areas function (and the areas found using either impulse response curve to obtain areas under CALIPSO under CALIPSO ocean surface returns were found to be the same within ~1%). For the work ocean surface returns were found to be the same within ~1%). For the work reported in this paper, reported in this paper, the impulse response is assumed to be the fit made to the lab measurements the impulse response is assumed to be the fit made to the lab measurements (solid curve in Figure 1). (solid curve in Figure 1). It should be noted that should subsequent investigations determine a It should be noted that shouldmodel subsequent determine a somewhat more accurate model somewhat more accurate for the investigations impulse response, the difference in determining the area for the impulse response, difference in determining themodel area under the lidar surface response (SR) under the lidar surfacethe response (SR) with the improved would only be a small, fractionally with the improved model would only be a small, fractionally fixed bias that could easily be corrected. fixed bias that could easily be corrected. 5 Impulse Response from Lab Measurements Ideal Impulse Response for a 3rd order Bessel Filter 4.5 4 Amplitude 3.5 3 2.5 2 1.5 1 0.5 0 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 Time Figure 2. Comparing the twoimpulse impulse responses. responses. Time in μsec units. Figure 2. Comparing the two Timeisismeasured measured in µsec units. 2.2. Area under Surface Return Pulse 2.2. Area under Surface Return Pulse The lidar equation for the instantaneous return signal from a distributed source such as the The lidar equation for the as instantaneous return signal from a distributed source such as the atmosphere can be expressed [8] atmosphere can be expressed as [8] V (z) = CE β (z)T (z) , z 2 (1) CEo βλ (z)Tλ (z) , (1) Vλsignal (z) =from range where Vλ represents the lidar return z2z expressed as a voltage level, z is the range from the lidar increasing downward towards the Earth’s surface, Eo represents the transmitted pulse whereenergy, Vλ represents the lidar return signal from at range z expressed as a voltage level, z −1is, the β represents the backscatter coefficient wavelength λ expressed in units of m−1·sr T (z)range from is the increasing downward the Earth’s surface, Eozrepresents the λ transmitted thelidar atmospheric round-trip pathtowards transmittance to and from range at wavelength and C is thepulse calibration constant. signalscoefficient from the atmosphere are mostly slowly varying energy, βλ represents theReturn backscatter at wavelength λ expressed in unitsand of have m−1 ·longer sr−1 , T2λ (z) durations than the impulse response of the LPF. Hence the LPF has little effect on the atmospheric is the atmospheric round-trip path transmittance to and from range z at wavelength λ and C is the returnsconstant. and the output the LPFfrom can the be well approximated by Equation However, lidar calibration Returnofsignals atmosphere are mostly slowly(1). varying andthe have longer response to surface returns Vλs, before entering the LPF, is a pulse which is a replica of the originally durations than the impulse response of the LPF. Hence the LPF has little effect on the atmospheric transmitted Gaussian-shaped lidar pulse of duration tp (tp ≈ 20 ns). As this pulse is much narrower returns and the output of the LPF can be well approximated by Equation (1). However, the lidar than the impulse response of the LPF, the output of the filter can be assumed to be the ideal impulse response to surface returns Vλs , before entering the LPF, is a pulse which is a replica of the originally response IRF of the filter itself. Hence, the time integrated output of the LPF “VλS LPF” for the surface transmitted Gaussian-shaped lidar return response “Vλs” is given by pulse of duration tp (tp ≈ 20 ns). As this pulse is much narrower than the impulse response of the LPF, the output of the filter can be assumed to be the ideal impulse response IRF of the filter itself. Hence, the time integrated output of the LPF “VλS LPF ” for the surface (2) V dt = V (t)dt , return response “Vλs ” is given by 0 where tp’ is the duration of the output impulse response duration). Defining “zs” to be p wtp of the LPFwt(the range to the surface, from Equations (1) and (2) we have VλS dt = VλS LPF (t)dt , 0 (2) 0 where tp ’ is the duration of the output of the LPF (the impulse response duration). Defining “zs ” to be range to the surface, from Equations (1) and (2) we have Remote Sens. 2016, 8, 1006 4 of 27 wtp 0 tp0 C E0 T2 (zs ) w VλS dt = λ 2 β(t)dt, zS Taking the round-trip propagation time t into account, dt can be written as wtp 0 (3) 0 z0 2E0 T2 (zs )Cλ w VλS dt = β(z)dz, cz2S 2dz c so that (4) 0 R z0 For a hard target we replace 0 β(z)dz with Rλ , the retro or backscatter reflectance (sr−1 ) of the surface. Hence, the expected surface return area, ALPF , after being normalized by the calibration constant, peak energy and range squared (just as the lidar equation, Equation (1), is normalized for the CALIPSO level 1 data product) is given by ALPF = 2T2 (zs )Rλ , c (5) The area under the surface-return response pulse thus depends on the product of the surface reflectance and total round-trip transmission. In other words, the response of the lidar receiver to ocean-surface return signals is a scaled version of the impulse response shown in Figure 1, and the magnitude of the scaling depends on the amount of atmospheric attenuation and the reflectance value of the ocean surface. With the normalizations, ALPF does not actually have the units of area, but will be referred to as an area in subsequent discussions. Also, c must be evaluated in units of km/µsec (c = 0.3 km/µsec) in Equation (5) to yield ALPF values consistent with the CALIPSO data product sample values of the surface response signals, and the ALPF inferred from the samples, per/characterized by the similarly normalized lidar equation. 2.3. Ocean Surface Reflectance Considerable effort ([9–12], to name a few) has been directed over the years to develop a model that can relate the surface reflectance to the surface wind speed (WS) and wave facet characteristics and accurately determine it. The ocean-surface reflectance model used in this paper was developed in [13]. This model is a revised and updated version of the model developed by Cox and Munk [9] and is presented below. In general, the ocean-surface backscatter reflectance, Rλ , units of sr−1 , can be modeled by Rλ = (1 − W) × Retro_Fresnel_Reflectance + W × 0.2 , (6) where “W” represents the fraction of the surface covered with whitecaps and “Retro_Fresnel_Reflectance” is the Fresnel reflectance of the ocean-surface at nadir (e.g., [14]). They are given by Whitecap Fraction = 2.95 × 10−6 × WindSpeed3.37 , (7) Fresnel Coeficient , 4πhwave_slopei2 (8) Retro_Fresnel_Reflectance = Here, as the name suggests, “WindSpeed” refers to surface wind speed (WS). The Fresnel Coefficient ($) is spectrally dependent and at 532 nm and 1064 nm has estimated values of $532 = 0.0205 and $1064 = 0.019 and hwave_slopei2 represents the variance of the distribution of wave slopes and is given by hwave_slopei2 = −0.006 + 7.95 × 10−3 × WindSpeed, (9) Thus, with known surface wind speeds (WS), the terms in Equations (7)–(9) can be calculated and the final reflectance can be determined using Equation (6). Figure 3 shows the variation of the ocean-surface reflectance at 532 nm wavelength, R532 , with surface wind speed (WS). As the reflectance Remote Sens. 2016, 8, 1006 5 of 27 Sens. at 2016, 8, 1006 5 ofdata 27 rises Remote sharply low wind speeds (WS < ~3 m/s), use of the reflectance model/input WS in estimating ALPF must be limited to higher WS, but also be cut off at too high a wind speed where the data in estimating ALPF must be limited to higher WS, but also be cut off at too high a wind speed reflectance model becomes less accurate (to be on the conservative side, analysis of CALIPSO data to where the reflectance model becomes less accurate (to be on the conservative side, analysis of retrieve ALPF presented here Ahas been limited to WS between ~4 m/s to ~8 m/s). CALIPSO data to retrieve LPF presented here has been limited to WS between ~4 m/s to ~8 m/s). 0.9 Ocean Surface Retro-Reflectance 0.8 0.7 0.6 0.5 0.4 0.3 0.2 0.1 0 1 2 3 4 5 6 7 8 9 Surface Wind Speed Figure 3. Ocean Surface Reflectance (sr−1) at 532 nm vs. Wind Speed (m/s). Figure 3. Ocean Surface Reflectance (sr−1 ) at 532 nm vs. Wind Speed (m/s). 2.4. Signal Acquisition and Post-Filtering Processing 2.4. Signal Acquisition and Post-Filtering Processing The lidar response, generated after photon detection of the received signal and post-detection The lidar response, generated after photon of the filtered. receivedThe signal and post-detection amplification, is sampled and digitized after detection being low-pass generated samples amplification, sampled and digitized afteraveraging being low-pass The generated samples undergo aiswavelength channel-specific schemefiltered. before being down-linked from undergo the satellite [6]. Thus, down-linked samples corresponding to ocean surface returns are satellite the result a wavelength channel-specific averaging scheme before being down-linked from the [6].ofThus, samplingsamples and averaging a scaled version of the LPF’sreturns impulseare response. down-linked corresponding to ocean surface the result of sampling and averaging a scaled version of the LPF’s impulse response. 2.4.1. Sampling and Generation of Down-Linked Samples 2.4.1. Sampling and Generation of of Down-Linked Samples The fundamental sampling the filter output for both wavelength channels occurs at 10 MHz frequency (consecutive samples hence separated by 0.1 μsec), insuring that samples meet the The fundamental sampling of the filter output for both wavelength channels occurs at 10 MHz sampling theorem requirement for reconstructing the sampled signal (bandwidth of the LPF is ~2.5 frequency (consecutive samples hence separated by 0.1 µsec), insuring that samples meet the sampling MHz). Sampling at this frequency essentially means that the vertical decimation of the atmosphere is theorem requirement for reconstructing the sampled signal (bandwidth of the LPF is ~2.5 MHz). performed in such a manner that the return signal is collected every 15 m along the transmission Sampling this frequency essentially meansthe that the vertical ofand thethe atmosphere is path ofatthe lidar pulse. Figure 4 below shows impulse responsedecimation (in solid blue) primary performed in such a manner that the return signal is collected every 15 m along the transmission samples (shown in black) separated by 0.1 μsec. For the 532 nm channel, every down-linked sample path is ofgenerated the lidar by pulse. Figure 4 belowprimary shows samples the impulse response them (in solid blue) andand thetheir primary pairing consecutive and averaging in both value samples by 0.1 µsec. Forfor thethe 532down-linked nm channel, every The down-linked sample time(shown instantsin toblack) obtainseparated the corresponding values sample. down-linked is generated by shown pairinginconsecutive samples and averaging themdown-linked in both value and their samples are red in Figure primary 4 and it can be observed that consecutive samples separated by 0.2 μsec, which means thatvalues the effective vertical range resolution is reduced to 30 m time are instants to obtain the corresponding for the down-linked sample. The down-linked for the 532 nm channel. samples are shown in red in Figure 4 and it can be observed that consecutive down-linked samples are 1064 which nm channel, samples are obtained after averaging consecutive separatedFor by the 0.2 µsec, meansdown-linked that the effective vertical range resolution is reduced to 30 m for primary samples in groups of four. Figure 5 describes this process by showing the original impulse the 532 nm channel. response, its primary samples and the final down-linked samples. Since the 1064 nm channel For the 1064 nm channel, down-linked samples are obtained after averaging consecutive primary requires twice the number of primary samples to be averaged to generate the down-linked sample samples in groups of four. Figure 5 describes this process by showing the original impulse response, when compared to the 532 nm channel, the total number of down-linked samples for the 1064 nm its primary samples and the final down-linked samples. Since the 1064 nm channel requires twice the channel is half that of the 532 nm channel. However, the CALIPSO data product, from where the number of primary samples to bechannels averaged generateduplicates the down-linked sample when compared to down-linked samples for both aretoretrieved, every down-linked sample of the the 532 nmnm channel, number of down-linked samples for theto1064 is half of that of 1064 channelthe andtotal stores it beside the original sample in order storenm thechannel same number the 532 nm channel. However, the CALIPSO data product, from where the down-linked samples down-linked samples for both the 1064 nm and 532 nm channels. Hence, while the 1064 nm for both channel-duplicated channels are retrieved, duplicates everyindown-linked sample ofinthe channel filtering and stores it samples are separated time by 0.2 μsec just as the1064 532 nm nm channel, beside the original sample in order to store the same number of down-linked samples for both the 1064 nm and 532 nm channels. Hence, while the 1064 nm channel-duplicated samples are separated in Remote Sens. 2016, 8, 1006 6 of 27 Remote Sens. 2016, 8, 1006 6 of 27 time by just assamples in the 532 nmbehind channel, filtering out the duplicated out0.2 theµsec duplicated leaves only the original samples (shownsamples in red inleaves Figurebehind 5) that only the original samples (shown in red in Figure 5) that are separated by 0.4 µsec which corresponds are separated by 0.4 μsec which corresponds to an effective vertical range resolution of 60 m. All to an effective vertical resolution of 60was m. done All analysis theoriginal 1064 nm channel wasout done analysis of therange 1064 nm channel data with onlyofthe samples afterdata filtering the with duplicate samples. only the original samples after filtering out the duplicate samples. 5 Impulse Response Original Samples Downlinked Samples 4.5 4 Amplitude 3.5 3 2.5 2 1.5 1 0.5 0 -0.4 -0.2 0 0.2 0.4 0.6 0.8 1 Time in usec Figure 4. Process generatingdown-linked down-linked samples thethe 532532 nmnm channel. Figure 4. Process ofof generating samplesforfor channel. 5 Impulse Response Original Samples Downlinked Samples 4.5 4 Amplitude 3.5 3 2.5 2 1.5 1 0.5 0 -0.4 -0.2 0 0.2 0.4 0.6 0.8 1 Time in usec Figure 5. Process ofof generating samplesfor for the 1064 channel. Figure 5. Process generatingdown-linked down-linked samples the 1064 nmnm channel. Effect of Sampling Delay Down-Linked Samples Samples 2.4.2.2.4.2. Effect of Sampling Delay onon Down-Linked As the primary samples are uniformly spaced with 0.1 μsec separation, the time instant of the As the primary samples are uniformly spaced with 0.1 µsec separation, the time instant of the first sample of the impulse response determines the time instances and hence the magnitudes of the first sample of the impulse response determines the time instances and hence the magnitudes of remaining samples that follow. On board CALIOP, the starting sampling instant is variable (e.g., due the remaining that follow. board CALIOP, the starting sampling is variable to digitizer samples jitter, difference in ocean On surface elevation at different locations/sea states,instant and imperfect (e.g., pointing, due to digitizer jitter, difference in ocean surface elevation at different locations/sea states, position and orbit propagation knowledge on board the satellite) [7]. Thus, different lidar and imperfect pointing, position and orbit propagation knowledge on samples board the satellite) [7].toThus, shots can have different starting sampling instances and hence surface corresponding different lidarshot shots can “delayed” have different starting instances inand hence surface samples one lidar maybe and, thus, may sampling differ in magnitudes comparison to samples obtained from another lidar shot. This process is depicted at 532 nm in Figure 6. Similarly, Figure 7 corresponding to one lidar shot maybe “delayed” and, thus, may differ in magnitudes in comparison shows the influence of sampling delay on the magnitude of the down-linked samples for the 1064 to samples obtained from another lidar shot. This process is depicted at 532 nm in Figure 6. Similarly, nm Figure 7 channel. shows the influence of sampling delay on the magnitude of the down-linked samples for the 1064 nm channel. results are shown in Figure 8. For the 532 nm channel, the remaining two samples are 0.2 μsec and 0.4 μsec away from the first sample. For the 1064 nm channel, the second sample is 0.4 μsec away from the first sample. Hence, for every lidar shot, time instances may be assigned to all the surface return samples at both wavelengths. It should be noted that, regardless of the time delay, the sum of the down-linked samples (sum value) that make up a given SR pulse is very nearly constant (within ~2%), Remote Sens. 2016, 8, 1006 7 of 27 for no noise present, and, as discussed later, can be used as a quality check to reject bad shots. Sampling Delay = 0 usec 5 Impulse Response Original Samples Downlinked Samples 4.5 4 Amplitude 3.5 3 2.5 2 1.5 1 0.5 0 -0.4 -0.2 0 0.2 0.4 0.6 0.8 1 Time in usec Sampling Delay = 0.05 usec 5 4 3 2 1 0 -0.5 Impulse Response Original Samples Downlinked Samples 4 Amplitude Amplitude Sampling Delay = 0.1 usec 5 Impulse Response Original Samples Downlinked Samples 3 2 1 0 0.5 1 0 -0.4 -0.2 Time in usec 0.4 0.6 0.8 1 Sampling Delay = 0.2 usec Sampling Delay = 0.15 usec 5 Impulse Response Original Samples Downlinked Samples 4 3 2 Impulse Response Original Samples Downlinked Samples 4 Amplitude Amplitude 0.2 Time in usec 5 3 2 1 1 0 -0.5 0 0 0.5 Time in usec 1 0 -0.5 0 0.5 Time in usec 1 Figure 6.6.Effect samplesfor forthe the532 532nm nmchannel. channel. Figure Effectofofsampling samplingdelay delay on on the the down-linked down-linked samples The effect of sampling delay on the magnitude of down-linked samples is quite evident where it can be seen that the values of the down-linked samples change relative to one another with delay. The delay must be taken into account in estimating the SR area for any given lidar shot. That is, the impulse response model used to estimate the area must be positioned under the SR samples for a given shot for the sampling delay of that shot. The delay can be estimated by the ratio of the first to second samples for a given shot. Piecewise cubic hermite (shape preserving) interpolation was performed at both wavelengths so that for every intermediate ratio, a sampling delay is assigned. The interpolation results are shown in Figure 8. For the 532 nm channel, the remaining two samples are 0.2 µsec and 0.4 µsec away from the first sample. For the 1064 nm channel, the second sample is 0.4 µsec away from the first sample. Hence, for every lidar shot, time instances may be assigned to all the surface return samples at both wavelengths. It should be noted that, regardless of the time delay, the sum of the down-linked samples (sum value) that make up a given SR pulse is very nearly constant (within ~2%), for no noise present, and, as discussed later, can be used as a quality check to reject bad shots. Remote Sens. 2016, 8, 1006 8 of 27 Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 10065 5 Amplitude 3 Impulse Response Original Samples Downlinked Samples 4 2 8 of 27 Impulse Response Original Samples Downlinked Samples Sampling Delay = 0 usec 4 Amplitude 8 of 27 Sampling Delay = 0 usec 3 1 2 0 1 -0.4 -0.2 0 0.2 0.4 0.6 0.8 1 Time in usec 0 -0.4 -0.2 0 Sampling Delay = 0.05 usec 0.2 0.4 Time in usec 5 0.6 0.8 1 Sampling Delay = 0.1 usec 5 Impulse Response Impulse Response Sampling Delay = 0.05 usecSamples Original 3 2 2 1 Sampling Delay = 0.1 usec Original Samples 54 Amplitude Amplitude Downlinked Samples Impulse Response Original Samples Downlinked Samples 4 3 Amplitude Amplitude 4 5 Downlinked Samples Impulse Response Original Samples Downlinked Samples 4 3 3 2 2 1 1 0 -0.5 0 0.5 Time in usec 0 0.5 Time in usec Sampling Delay = 0.15 usec 0 -0.5 1 1 0 -0.5 1 0 -0.5 5 5 Sampling Delay = 0.15Impulse usec Response 5 3 2 2 1 1 Impulse Response Sampling Delay = 0.2 usec Original Samples Impulse Response Downlinked Samples Original Samples Downlinked Samples 4 4 3 Amplitude Amplitude Amplitude Amplitude 4 3 0.5 Time in usec 0 0.5 Time in usec Sampling Delay = 0.2 usec 5 Original Samples Impulse Response Downlinked Samples Original Samples Downlinked Samples 4 0 3 2 2 1 1 1 1 0 -0.5 0 -0.5 0 0.5 0 Time in usec 0.5 Time in usec 0 -0.5 1 1 0 0 -0.5 0 0.5 0.5 Time in usec Time in usec 1 1 Figure 7. Effect of sampling delay on the down-linked samples for the 1064 nm channel. Figure on the thedown-linked down-linkedsamples samplesfor for the 1064 channel. Figure7.7.Effect Effectof ofsampling sampling delay on the 1064 nmnm channel. 6 5 6 532 nm channel 532 nm channel 6 6 5 4 4 44 Ratio Ratio Amplitude Amplitude 5 Ratio Amplitude Ratio Amplitude 5 3 3 2 2 1 1 0 00 0 1064 nm channel 1064 nm channel 33 22 11 0.05 0.05 0.1 0.15 0.1 0.15 SamplingDelay Delay Sampling 0.2 0.2 00 00 0.05 0.05 0.1 0.1 0.15 0.15 Sampling Delay Sampling Delay 0.20.2 Figure 8.8.Interpolation results. Sampling Sampling delayisisplotted plotted in µsec units. Figure8. Interpolationresults. results. Figure Interpolation Sampling delay delay is plottedininμsec μsecunits. units. Remote Sens. 2016, 8, 1006 9 of 27 2.4.3.Remote Down-Linked Samples Sens. 2016, 8, 1006 9 of 27 The principle data product that is down-linked from CALIPSO is the attenuated backscatter 2.4.3. Down-Linked Samples (km−1 ·sr−1 ), which for a range “z” is defined as The principle data product that is down-linked from CALIPSO is the attenuated backscatter 2 2 2 (km−1·sr−1), which for a range “z” is defined Attenuated Backscatter = (βas (10) R (z) + βa (z)) × TR (z) × Ta (z) × TOzone , AttenuatedBackscatter = β (z) + β (z) × T (z) × T (z) × T , (10) where βa and βR represent the aerosol and Rayleigh components of the backscatter coefficient and T2 a , where βa andrepresent βR represent the aerosol and Rayleigh components of the of backscatter coefficient and T2 R and T2 Ozone the aerosol, Rayleigh and ozone components the round-trip transmission, T2a, T2R and T2Ozone represent the aerosol, Rayleigh and ozone components of the round-trip respectively. It should be noted that the attenuated backscatter data product has been normalized transmission, respectively. It should be noted that the attenuated backscatter data product has been to take out the lidar calibration for each wavelength, for the given lidar orbit position, as a part normalized to take out the lidar calibration for each wavelength, for the given lidar orbit position, as of CALIPSO standard data processing. For every lidar shot, the CALIPSO data product provides a part of CALIPSO standard data processing. For every lidar shot, the CALIPSO data product the attenuated for 583 altitude at both SurfaceSurface returns can easily provides thebackscatter attenuated backscatter for 583bins altitude binswavelengths. at both wavelengths. returns can be identified (so long as the atmospheric optical depth is not too great due to clouds or optically easily be identified (so long as the atmospheric optical depth is not too great due to clouds or optically thick aerosol layers) amongst the 583 as they are stronger than atmospheric thick aerosolfrom layers) from amongst the bins 583 bins as they aresignificantly significantly stronger than thethe atmospheric returns. The ocean surface returns were observed to be made up of three down-linked returns. The ocean surface returns were observed to be made up of three down-linked samplessamples for the for the 532 and two down-linked samples the nm channel, and almost they were almost 532nm nm channel, channel, and two down-linked samples for thefor 1064 nm1064 channel, and they were always found to lieto within bins 561–565 the data in product for both channels. shows samples for both always found lie within bins in 561–565 the data product forFigure both 9channels. Figure 9 shows wavelength corresponding a typical surface signal. It should besignal. noted that the be samples for bothchannels wavelength channelstocorresponding to return a typical surface return It should scales are not the are same forthe thesame two for channels (scale for 1064 nm is twoisbin notedhorizontal that the horizontal scales not the two channels (scale fordouble, 1064 nm double, increments). two bin increments). 0.45 Downlinked Surface Samples at 532 nm 0.45 0.4 0.4 0.35 0.35 0.3 0.3 Magnitude Magnitude 0.5 0.25 0.2 Downlinked Surface Samples at 1064 nm 0.25 0.2 0.15 0.15 0.1 0.1 0.05 0.05 0 561 562 563 564 565 0 559 566 561 563 565 567 569 Altitude Bin Number Altitude Bin Number Figure 9. Typical surface return samples at 532 nm and 1064 nm found in the CALIPSO data product. Figure 9. Typical surface return samples at 532 nm and 1064 nm found in the CALIPSO data product. A useful parameter to assess the amount of aerosol loading in the atmosphere is the integral of A parameter to assess amount of aerosol in attenuated the atmosphere is the(TIAB), integral of theuseful attenuated backscatter downthe to the surface, the total loading integrated backscatter units of sr−1.backscatter Thus, if “zs” down is the range to surface, the surface the attenuated to the the total integrated attenuated backscatter (TIAB), units of sr−1 . Thus, if “zs ” is the range to the surface TIAB = TIAB = wZS β + β ×T ×T ×T dz, βAerosol + βRayleigh × T2Aerosol × T2Rayleigh × T2Ozone dz , (11) (11) From its definition,0 TIAB is expected to increase with increasing aerosol backscatter, although if βa(z) becomes too large, the corresponding impact on Ta2(z) will cause TIAB to decrease. Even as TIAB increases, Ta2(z) TIAB still decreases withto increasing a (z), causing the aerosol strength backscatter, of observed surface From its definition, is expected increaseβwith increasing although if 2 (z) will to too generally with increasing TIAB. very clear sky conditions (aerosol-free βa (z)returns becomes large, decrease the corresponding impact on TUnder cause TIAB to decrease. Even as TIAB a 2 atmosphere) for 532 nm the TIAB reduces to increases, Ta (z) still decreases with increasing βa (z), causing the strength of observed surface returns to generally decrease with increasing TIAB. Under very clear sky conditions (aerosol-free atmosphere) (12) TIAB β ×T ×T dz , for 532 nm the TIAB reduces to ( ) = TIAB(Clear sky) = wzs 0 βRayleigh × T2Rayleigh × T2Ozone dz , (12) Remote Sens. 2016, 8, 1006 10 of 27 Using the molecular and ozone density numbers provided in the CALIPSO data product, all the terms within the integral in Equation (12) can be computed and for the 532 nm channel the TIAB for clear sky conditions was calculated to be ~0.012. Thus, a TIAB threshold value of 0.0125 was set so that any 532 nm lidar shot having a TIAB value ≤0.0125 was assumed to have passed through an essentially aerosol-free atmosphere. The CALIPSO data product also provides, for every lidar shot, its eastward and westward wind component values (the wind information is provided from NASA’s Global Modeling and Assimilation Office (GMAO); the wind being estimated from an assimilation model). The total surface wind speed can be obtained by taking the vector sum of these components, from which the surface reflectance can be calculated using the model described earlier. Thus, every lidar shot can be associated with a TIAB and surface reflectance value. 2.5. Reconstruction of Impulse Response and Area Retrieval from Down-Linked Samples The low-pass filtered lidar responses to ocean-surface signal returns, which are approximated to be the scaled impulse response of the LPF, have an area that was shown to be proportional to the product of the surface reflectance and the total round-trip transmittance of the atmosphere. As the reflectance can be calculated with the knowledge of surface wind speeds, the aerosol round-trip transmission can be retrieved if the area under the scaled impulse response, ALPF , can be accurately determined. For every down-linked sample that is identified to be a part of the SR signal, by reversing this process of averaging and sampling, by using the impulse response model (shown in Figure 1), the original samples (whose average gives the down-linked sample) and the scaled impulse response from which the original samples were obtained, can be recovered and the area under it may be computed. It can be seen from Figures 6 and 7 that the surface signal is generally made up of two down-linked samples for the 1064 nm channel and three down-linked samples for the 532 nm channel, amongst which two of the three seem to be significantly stronger than the third. The first step in the reconstruction is to determine the time instances of these samples relative to the start of the impulse response (i.e., the sampling delay), which, as described earlier, can be estimated from the ratio of the first to second SR samples, using the interpolation curves shown in Figure 8. As the time instant for every down-linked sample is assigned for 532 nm, the two time instants of the original samples that upon averaging give the down-linked sample, are also known (0.05 µsec on either side of the down-linked sample). The impulse response curve based on lab measurements (solid curve in Figure 1) is varied in area until the average of the values on the curve corresponding to the two time instants is equal to the value of the down-linked sample. In this manner, area is calculated for every non-zero down-linked sample. This process is depicted by selecting an arbitrary SR non-zero sample as shown in red in Figure 10. The down-linked sample is first aligned (i.e., positioned for the sampling delay estimated for the SR sample) with the impulse response model, which is scaled initially to have a small area. The initial samples corresponding to this scaled impulse response curve are located 0.05 µsec on either side of the down-linked sample, and are shown in black. These samples are then averaged in both their value and their time instances, to produce the sample shown in green (in Figure 10). As the sample in green is clearly not equal to the down-linked sample in magnitude, the impulse response curve is scaled to have an increased area. Scaling of the area/curve is increased (an intermediate scaling is shown in Figure 11) until the average of the samples for the impulse response curve, found 0.05 µsec on either side of the down-linked sample, is equal in magnitude to the down-linked sample as shown in Figure 11. The area of the impulse response for this down-linked sample is stored. The same procedure for estimating area is used on the four-average samples for 1064 nm. The process is repeated for any other non-zero shot samples and these area estimates are also stored. The resulting areas may be averaged for the area estimate of a given shot (at 532 nm or 1064 nm) or grouped with the areas estimated for similar shots. Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 1006 0.7 Amplitude Amplitude 0.6 0.5 0.4 0.3 0.2 0.1 0.8 0.7 0.6 Area under Impulse response = 0.06 Area under Impulse response = 0.06 0.80.8 Impulse Response Impulse Response Original Sample points of the Curve Original Sample points of the Curve Downlinked Sample Point Downlinked Sample Point Area under Impulse response = 0.06 Area under Impulse response = 0.06 Impulse Response Impulse Response Original Sample points of the Curve Original Sample points of the Curve Sample resulting from Averaging original sample points Sample resulting from Averaging original sample points Downlinked Sample Point Downlinked Sample Point 0.70.7 0.60.6 0.5 0.50.5 Amplitude Amplitude 0.8 11 of 27 11 11 of of 27 27 0.4 0.40.4 0.3 0.30.3 0.2 0.20.2 0.1 0.10.1 0 0 0 0.05 0.15 0 0.05 0.15 0.4 0.4 0.6 0.6 0.8 Time Time 0.8 0 00 0 0.20.2 0.40.4 Time Time 0.60.6 0.80.8 Figure Showing time instances original samples and their average. Time is plotted in μsec in Figure 10. Showing time instances ofthe the original samples and their average. is in plotted Figure 10.10. Showing time instances of of the original samples and their average. Time is Time plotted μsec units. units. µsec units. 0.8 0.8 0.7 0.7 0.6 0.6 Area under Impulse response = 0.2130 Area under Impulse response = 0.2130 Area under Impulse response = 0.14 Area under Impulse response = 0.14 Impulse Response Impulse Response Original Sample points of the Curve 1 Original Sample points of the Curve 1 Sample resulting from Averaging original sample points Sample resulting from Averaging original sample points Downlinked Sample Point Downlinked Sample Point 0.8 0.8 Amplitude Amplitude Amplitude Amplitude 0.5 0.5 0.6 0.6 0.4 0.4 0.3 0.3 0.4 0.4 0.2 0.2 0.2 0.2 0.1 0.1 0 0 0 0 0.2 0.4 0.2 0.4 Time Time (a) (a) 0.6 0.6 0.8 0.8 0 0 0 0 0.2 0.4 0.2 0.4 Time Time (b) 0.6 0.6 (b) 0.8 0.8 Figure Process scaling area until the original impulse response down-linked sample Figure 11. Process ofof scaling inin area until the original impulse response ofthe the down-linked sample Figure 11.11. Process of scaling in area until the original impulse response of of the down-linked sample is is is recovered: (a) Area scaled too small; (b) Area scaled to fit the down-linked sample. Time is plotted recovered: scaled too toosmall; small;(b) (b)Area Areascaled scaled down-linked sample. Time is plotted recovered: (a) (a) Area Area scaled toto fit the down-linked sample. Time is plotted in in in μsec units. µsec μsecunits. units. Surface return pulses arising from surfaces having reflectance values close one another and Surface return pulses arising reflectance values close toto one another and Surface return pulses arisingfrom fromsurfaces surfaceshaving having reflectance values close to one another and havingthe thesame sameatmospheric atmosphericattenuation attenuationwill willapproximately approximatelyproduce producethe thesame sameoutput output(i.e., (i.e.,the the having having the same atmospheric attenuation will approximately produce the same output (i.e., the same same impulse response) from the LPF. the surface returns within such a group produce nearly same impulse response) the LPF. AsAs allall the surface returns within such group produce nearly impulse response) from from the LPF. As all the surface returns within such a agroup produce nearly the the same impulse response and SR area, even if each of them has a different sampling delay, they are the same impulse response and area,even evenififeach each of of them sampling delay, theythey are same impulse response and SRSR area, themhas hasa adifferent different sampling delay, are expected have approximately the same sum value (i.e., noted earlier the sum the samples expected toto have approximately the same sum value (i.e., asas noted earlier the sum ofof the SRSR samples expected to have approximately the same sum value (i.e., as noted earlier the sum of the SR samples a given nearly constant regardless sampling delay). can happen that the down-linked forfor a given SRSR is is nearly constant regardless ofof sampling delay). It It can happen that the down-linked forsamples a given corresponding SR is nearly constant regardless of sampling delay). It can happen that the down-linked some surface returns within the group will spurious (either very strong samples corresponding toto some surface returns within the group will bebe spurious (either very strong samples corresponding to to some surface returns within the group will be spurious (either verycould strong or very weak compared other samples of the group). The source of these spurious samples or very weak compared to other samples of the group). The source of these spurious samples could or very weak compared to other samples of the group). The source of these spurious samples could the result the return signal saturating the receiver, undetected abrupt changes surface windbe bebe the result ofof the return signal saturating the receiver, undetected abrupt changes inin surface wind thespeed result or of the return signal saturating the receiver, undetected abrupt changes in surface wind speed aerosolloading/aerosol loading/aerosoltype, type,orordue duetotothe thegeneral generalcorruption corruptionbybynoise noiseduring duringdata data speed or aerosol or aerosol loading/aerosol type, or due to thevalue general corruption by noise during data collection collection andsampling. sampling.The Thesample sample sum everysurface surface returnsignal signalcan canbebe usedasasa and a collection and sum value forforevery return used sampling. The sample sum value for every surface return signal can be used as a measure of quality measureofofquality qualityofofthat thatsignal. signal.ToToeliminate eliminateoutlier outliersamples, samples,the themean meanand andstandard standarddeviation deviation of measure that signal. To eliminate outlier samples, the mean and standard deviation values of the sum values valuesofofthe thesum sumvalues valuesover overallallthe thesurface surfacereturns returnsthat thatconstitute constitutethe thegroup groupare arecalculated, calculated,and and values over all the surface returns that constitute the group are calculated, and only those surface returns only those surface returns are retained whose sum values fall within two standard deviations only those surface returns are retained whose sum values fall within two standard deviations ononare retained whose sum values fall within two standard deviations onThe either side of the mean sum value eitherside sideofofthe themean mean sum value calculated the entiregroup. group. Thesame same criterion wasused usedto to either sum value calculated forforthe entire criterion was calculated for the entire group. The same criterion was used to eliminate outlier surface returns at eliminate outlier surface returns at both wavelengths. eliminate outlier surface returns at both wavelengths. both wavelengths. Thefinal finalarea areaestimate estimateofofa agroup groupis iscalculated calculatedasasthe themean meanofofthe theareas areascalculated calculatedforforallall The retained down-linked samples. The impulse response scaled to the final mean-estimated area along The final area estimate of a group is calculated as the mean of the areas calculated allalong retained retained down-linked samples. The impulse response scaled to the final mean-estimatedfor area with retained down-linked samples corresponding to an example group is shown in Figure 12. Also down-linked samples. The impulse response scaled to the final mean-estimated area along with with retained down-linked samples corresponding to an example group is shown in Figure 12. Also shown is the corresponding area standard deviation value. Similarly, for the 1064 nm channel, as the retained samples corresponding to an example group isfor shown in Figure 12. Also shown shown isdown-linked the corresponding area standard deviation value. Similarly, the 1064 nm channel, as the is the corresponding area standard deviation value. Similarly, for the 1064 nm channel, as the time Remote Sens. 2016, 8, 1006 12 of 27 Remote Sens. Sens. 2016, 2016, 8, 8, 1006 1006 Remote 12 of of 27 27 12 instant forinstant everyfor down-linked samplesample is known, the time instances of the original four samples time every down-linked down-linked is known, known, the time time instances of the the original four samplesthat time instant for every sample is the instances of original four samples uponthat averaging give the down-linked sample, are also known. The impulse response is varied in area upon averaging averaging give give the the down-linked down-linked sample, sample, are are also also known. known. The The impulse impulse response response is is varied varied that upon untilinthe average ofaverage the values the impulse response at these fourfour timetime instances is isequal area until the the of the theofvalues values of the the impulse impulse response at these these instances equalto tothe in area until average of of response at four time instances is equal to valuethe of value the down-linked sample. The area is calculated for every down-linked sample in the group the value of the down-linked sample. The area is calculated for every down-linked sample in the of the down-linked sample. The area is calculated for every down-linked sample in the in this manner and finaland areathe is final taken as the mean retained areas. Figure 13 shows group in this manner and the final area is taken taken asof thethe mean of the the calculated retained calculated calculated areas. Figure Figure group in this the manner area is as the mean of retained areas. 13 shows shows the the scatterplot of the the retained down-linked down-linked samples for an an example example 1064 nm group, group, alongthe the scatterplot of scatterplot the retained down-linked samples for an example 1064 nm1064 group, along along with 13 of retained samples for nm withresponse the impulse impulse response scaled to the final final estimated estimated area. impulse scaled to thescaled final to estimated area. with the response the area. Final Estimated Estimated Area Area == 0.1951, 0.1951, Standard Standard -- Deviation Deviation == 0.018 0.018 Final 11 Downlinked Samples Samples Downlinked Impulse Response Response Impulse Amplitude Amplitude 0.8 0.8 0.6 0.6 0.4 0.4 0.2 0.2 000 0 0.1 0.1 0.2 0.2 0.3 0.3 Time Time 0.4 0.4 0.5 0.5 0.6 0.6 0.7 0.7 Figure 12. Impulse Impulse response scaled to thefinal finalestimated estimated area area and and the down-linked samples forfor thethe Figure 12. Impulse response scaled toto the andthe thedown-linked down-linked samples Figure 12. response scaled the final estimated samples for the 532 nm channel. Time is measured in μsec units. 532 nm Time is measured in in µsec units. 532channel. nm channel. Time is measured μsec units. Final Estimated Estimated Area Area == 0.2607, 0.2607, Standard Standard -- Deviation Deviation == 0.035 0.035 Final 1.4 1.4 Downlinked Samples Samples Downlinked Impulse Response Response Impulse 1.2 1.2 Amplitude Amplitude 11 0.8 0.8 0.6 0.6 0.4 0.4 0.2 0.2 00 -0.1 -0.1 00 0.1 0.1 0.2 0.2 0.3 0.3 Time Time 0.4 0.4 0.5 0.5 0.6 0.6 0.7 0.7 0.8 0.8 Figure 13. Impulse Impulse response scaled to thefinal finalestimated estimated area area and and the down-linked samples forfor thethe Figure 13. response scaled the final estimated samples for the Figure 13. Impulse response scaled toto the andthe thedown-linked down-linked samples 1064 nm channel. Time is measured in μsec units. nm channel. Time is measured μsec units. 1064 1064 nm channel. Time is measured in in µsec units. Groups for for averaging averaging were were selected selected by by binning binning the the CALIOP CALIOP data data into into specified specified small small increments increments Groups Groups for averaging were selected by binning the CALIOP data into small increments in both wind speed (which then defines an increment in reflectance, R λ) specified and the total integrated in both wind speed (which then defines an increment in reflectance, Rλ) and the total integrated in both wind speed (which then defines increment in contain reflectance, Rλ ) and the from total spatially integrated attenuated backscatter, TIAB. While suchan groups will likely likely contain SR SR samples samples mainly from spatially attenuated backscatter, TIAB. While such groups will mainly attenuated backscatter, TIAB. While such groups will likely contain SR samples mainly from contiguous lidar shots, this is neither required nor expected as some shots may be missing due tospatially noise contiguous lidar shots, this is neither required nor expected as some shots may be missing due to noise rejection, cloud screening, abrupt spatial change in wind speed or TIAB and the like. Also, some shots contiguous lidar shots, this is neither required nor expected as some shots may be missing due to noise rejection, cloud screening, abrupt spatial change in wind speed or TIAB and the like. Also, some shots from significantly different spatial locations could have nearly the same TIAB and wind speed and be rejection, screening, abrupt spatial change in wind speedthe or same TIABTIAB and the shots from cloud significantly different spatial locations could have nearly andlike. windAlso, speedsome and be included in the same group. As presented in the next section, the averaging groups were found to be fromincluded significantly spatial locations in could havesection, nearlythe theaveraging same TIAB and were windfound speedtoand in thedifferent same group. As presented the next groups be be composed ofsame anywhere from as many as as aain few hundred lidar shots shots to as as little little as asgroups few tens tens of shots. shots. As As composed anywhere from many few lidar to aa few of included in theof group. Asas presented thehundred next section, the averaging were found to be CALIOP lidar shots occur at a surface separation of one-third of a km, the group’s spatial extents CALIOP lidar shots occur at a surface separation of one-third of a km, the group’s spatial extents composed of anywhere from as many as a few hundred lidar shots to as little as a few tens of shots. typically ranged ranged from from about about 10 10 km km up up to to 150 150 km km (could (could even even be be larger larger depending depending on on missing missing shots shots and and typically As CALIOP lidar shots occur at a surface separation of one-third of a km, the group’s spatial extents shots in in different different locations locations with with nearly nearly the the same same TIAB TIAB and and wind wind speed). speed). Grouping Grouping data data in in this this manner manner shots typically ranged from about 10 km up to 150 km (could even be larger depending on missing shots proved effective effective in in gathering gathering statistics statistics on on the the range range and and variability variability of of the the SR SR areas. areas. proved and shots in different locations with nearly the same TIAB and wind speed). Grouping data in this manner proved effective in gathering statistics on the range and variability of the SR areas. Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 1006 13 of 27 13 of 27 3. Results and Discussion 3. Results and Discussion 3.1. Regions of Study 3.1. Regions of Study Due to the absence of solar background radiation, the signals collected during the night-time Dueoftothe theorbit absence of solar background radiation, signalssamples collectedtoduring night-time portion are less noisy and provide the mostthe accurate test thethe area retrieval portion of the orbit are less noisy and provide the most accurate samples to test the area retrieval technique for estimating the area of the CALIOP ocean surface returns. Night-time down-linked technique for correspond estimating the area of the CALIOP oceancollected surface from returns. Night-time down-linked samples that to ocean surface returns were the Southern Pacific Ocean (5 samples that correspond to ocean surface returns were collected from the Southern Pacific May 2011–20 May 2011), Atlantic Ocean (1 May 2011–15 May 2011) and Indian Ocean (1 MayOcean 2011– (5 2011–20 2011), Atlantic Oceandown-linked (1 May 2011–15 andare Indian 15 May May 2011). TheMay various regions from where samplesMay were2011) collected shownOcean in the (1 May 2011–15 May 2011). The various regions from where down-linked samples were collected red rectangles (approximately 30 degrees in lat by 40 degrees in lon) of Figure 14. These regions were are shown in the red rectangles (approximately 30 degrees in lat by 40 degrees in lon) of Figure 14. chosen on the basis of providing a reasonable fraction of cloud-free situations as well as a variety of These regions were chosen on the basis of providing a reasonable fraction of cloud-free situations as aerosol-loading conditions. well as a variety of aerosol-loading conditions. Figure 14. The various ocean regions where samples were collected are shown in red, left to right, and Figure 14. The various ocean regions where samples were collected are shown in red, left to right, a typical night-time orbit (shown in black) passing through each region is included. and a typical night-time orbit (shown in black) passing through each region is included. For For each each of of the the oceanic oceanic regions, regions, aa CALIPSO CALIPSO orbit orbit passes passes over over the the region region of of study study during during night-time once every 24 h and fires approximately 5000 lidar shots during its time of flight. Thus, night-time once every 24 h and fires approximately 5000 lidar shots during its time of flight. Thus, for 15 consecutive days (as the dates suggest), ~5000 × 15 shots are fired by CALIOP over each of for 15 consecutive days (as the dates suggest), ~5000 × 15 shots are fired by CALIOP over each of the the regions of study, and surface returns corresponding to each of these lidar shots (determined to regions of study, and surface returns corresponding to each of these lidar shots (determined to be be cloud free from the CALIPSO data product) were collected in the form of down-linked samples cloud free data product) were collected in the form of down-linked samples (for (for both thefrom 532 the nm CALIPSO and 1064 nm channels). bothAs thenoted 532 nm and 1064 nm channels). at the end of Section 2.5, averaging groups were defined by binning the CALIOP data As noted at the end of Section averaging groups wereof defined by binning the TIAB CALIOP data into small increments in both wind 2.5, speed and TIAB. For each the regions of study, groups into small increments in bothSR wind speedthat andfell TIAB. For TIAB each of the regions study, were defined for the collected samples into five value ranges ofof0.012 to TIAB 0.0125,groups 0.016 were defined for0.024, the collected SR samples that fell into five value speed rangessub-groups of 0.012 tofor 0.0125, to 0.017, 0.022 to 0.028 to 0.031 and 0.034 to 0.036, units of TIAB sr−1 . Wind each −1 TIAB group were formed for samples that fell into five wind speed ranges of 3.7 to 3.9 m/s, 4.4 to 0.016 to 0.017, 0.022 to 0.024, 0.028 to 0.031 and 0.034 to 0.036, units of sr . Wind speed sub-groups 4.6 to 5.3 m/s,were 5.5 to 6.0 m/s 6.6 to that 7.1 m/s (the wind speed increments so form/s, each 5.1 TIAB group formed forand samples fell into five wind speed ranges were of 3.7selected to 3.9 m/s, that the4.6 surface by more than6.6 0.005 increment). The TIAB upper limit 4.4 to m/s, reflectance 5.1 to 5.3 did m/s,not 5.5vary to 6.0 m/s and to within 7.1 m/san(the wind speed increments were was set toso 0.036 SRsurface samplesreflectance above ~0.04 to be difficult distinguish from atmospheric selected thatasthe didwere not found vary by more than to 0.005 within an increment). The returns. As noted earlier, the lowest TIAB range of 0.012 to 0.0125 defines samples for lidar shots TIAB upper limit was set to 0.036 as SR samples above ~0.04 were found to be difficult to distinguish that passed through essentially aerosol-free atmospheres. The wind speed upper and lower limits from atmospheric returns. As noted earlier, the lowest TIAB range of 0.012 to 0.0125 defines samples (3.7 m/s and 7.1 m/s) spanned the range for which the wind speed reflectance model [13] applied to the for lidar shots that passed through essentially aerosol-free atmospheres. The wind speed upper and data was deemed reasonably applicable. Neither the TIAB or wind speed groupings are continuous; lower limits (3.7 m/s what and 7.1 m/s) spanned the range sampling for which the wind speed the reflectance model rather, they provide was deemed a sufficient to characterize continuum of [13] SR applied to the data was deemed reasonably applicable. Neither the TIAB or wind speed groupings samples occurring within the specified TIAB and wind speed limits. The defined groupings contained are continuous; rather, they provide whatinwas deemed a sufficient sampling characterize the numerous samples (see results/discussion following sub-section) that proved to quite adequate for continuum of SR samples occurring within the specified TIAB and wind speed limits. The defined statistically assessing and characterizing the effect of aerosol attenuation and ocean surface reflectance groupings contained numerous samples (see results/discussion in following sub-section) that on SR area retrievals. Remote Sens. 2016, 8, 1006 14 of 27 proved quite adequate for statistically assessing and characterizing the effect of aerosol attenuation Remote Sens. 2016, 8, 1006 14 of 27 and ocean surface reflectance on SR area retrievals. 3.2. Surface Return Area Retrieval Results 3.2. Surface Return Area Retrieval Results Example SR impulse response curve fits for data collected from the Southern Pacific Ocean Example SR impulse response curve fits for data collected from the Southern Pacific Ocean region region (see area defined in Figure 14) for the 532 nm channel are shown for several groupings in (see area defined in Figure 14) for the 532 nm channel are shown for several groupings in Figure 15. Figure 15. As described earlier in the previous section regarding Figures 12 and 13, the response As described earlier in the previous section regarding Figures 12 and 13, the response curve is the fit to curve is the fit to the mean area determined from the average of the areas of all the retained the mean area determined from the average of the areas of all the retained down-linked samples in down-linked samples in a group. For each grouping, the final estimated mean area and standard a group. For each grouping, the final estimated mean area and standard deviation, original number deviation, original number of surface returns/samples in the group and the number of surface of surface returns/samples in the group and the number of surface returns/samples retained after returns/samples retained after data screening, are also provided. The areas and standard deviations data screening, are also provided. The areas and standard deviations for all the Southern Pacific Ocean for all the Southern Pacific Ocean 532 nm data groupings are given in Table 1, and Figure 16 shows 532 nm data groupings are given in Table 1, and Figure 16 shows plots of these areas versus wind plots of these areas versus wind speed for each TIAB range. As expected, it can be seen from the speed for each TIAB range. As expected, it can be seen from the figure that the areas progressively figure that theincreasing areas progressively decrease with increasing Corresponding results the2 decrease with TIAB. Corresponding results for the TIAB. 1064 nm channel are given in for Table 1064 nm channel are given in Table 2 and Figure 17. Similarly, the results for the Atlantic Ocean data and Figure 17. Similarly, the results for the Atlantic Ocean data analysis are given in Tables 3 and 4, analysis are given in Tables and 4,data andanalysis the results theinIndian are response given in and the results for the Indian3Ocean are for given TablesOcean 5 and 6data (theanalysis SR impulse Tables 5 and (the SR impulse response fits likefor those given in Figure are not for curve fits like6those given in Figure 15 are curve not repeated the Southern Pacific 15 Ocean 1064repeated nm channel the Southern Pacific Ocean 1064 nm channel data or for the two channels for the other ocean regions data or for the two channels for the other ocean regions as they all proved similar. Also, figures as they all proved Also, figures for likethe Figures and regions 17 are not repeated the other ocean like Figures 16 andsimilar. 17 are not repeated other16 ocean as they also for all proved similar). regions as seen they in also all proved similar). As canobtained be seen in in the results obtained for As can be Figure 15 (and in the results forFigure curve15 fits(and for all ocean regions and both curve fits for all ocean regions and both wavelengths) the greatest number of available down-linked wavelengths) the greatest number of available down-linked samples/retained samples occurred at samples/retained samples occurred at the lowestoptical TIAB values (i.e., thevalues), lowest indicating aerosol optical depth the lowest TIAB values (i.e., the lowest aerosol depth (AOD) low AODs (AOD) values), indicating low AODs occurred most frequently. occurred most frequently. TIAB = 0.012 - 0.0125 1 A rea M ean = 0.2305 S td D eviation = 0.027 0.8 0.6 0.4 1 A rea M ean = 0.1940 S td D eviation = 0.017 0.8 0.6 0.4 0.2 0.2 0 0 1.2 Down-linked Samples Magnitude (Area Values) Magnitude (Area Values) 1.2 Number of Samples = 315 No. of Surface returns after screening = 86 Number of Samples= 258 0.2 0.4 0.6 0.8 Time (usec) Wind Speed = 3.7 m/s - 3.9 m/s 1.4 Original No. of Surface returns = 431 Number of Samples = 1293 No. of Surface returns after screening = 364 Number of Samples= 1092 0 0 1.2 Magnitude (Area Values) 1.4 Original No. of Surface returns = 105 1 Original No. of Surface returns = 405 Number of Samples = 1215 No. of Surface returns after screening = 342 Number of Samples= 1026 A rea M ean = 0.1330 S td D eviation = 0.013 0.8 0.6 0.4 0.2 0.2 0.4 0.6 Time (usec) Wind Speed = 4.4 m/s - 4.6 m/s Figure 15. Cont. 0 0 0.2 0.4 0.6 Time (usec) Wind Speed = 6.6 m/s - 7.1 m/s Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 1006 15 of 27 15 of 27 0.6 0.4 0.3 0.2 0.1 0 0 0.6 0.7 Original No.Aofrea Surface returns = 41 Number of Samples 123 M ean ==0. 0875 No. of Surface returns after screening = 38 S td D eviation = 0.014 Number of Samples= 114 0.5 Magnitude (Area Values) 0.5 Magnitude (Area Values) Magnitude (Area Values) 0.7 A rea M ean = 0.0875 S td D eviation = 0.014 0.5 0.4 0.3 0.4 Original No. of Surface returns = 31 A rea 0.5 Number of Samples = 93 ean = 0.0657 No. of Surface returns afterMscreening = 30 0.6 Number of Samples= 90 S td D eviation = 0.012 Original No. of Surface returns = 52 Number of Samples = 156 Down-linked Samples A rea M ean = 0.0781 S td D eviation = 0.01 0.2 0.3 0.1 0.2 0.2 0.1 0.2 0.4 Time (usec) 0 Wind Speed = 4.4 m/s 4.6 m/s 0 0.2 0.4 0.1 0 0 0.6 0.6 Time (usec) Wind Speed = 4.4 m/s - 4.6 m/s 0.6 0.2 0.4 Time (usec) 0 Wind 5.1 m/s - 5.3 0 Speed =0.2 0.4 m/s Time (usec) Wind Speed = 5.1 m/s - 5.3 m/s of 27 Original No. of Surface returns15 = 31 Number of Samples = 93 No. of Surface returns after screening = 30 Number of Samples= 90 0.7 0.6 No. of Surface returns after screening = 43 Number of Samples=A 129 rea 0.4 M ean = 0.0781 S td D eviat ion = 0.01 0.5 Down-linked Samples 0.3 0.7 Original No. of Surface returns = 52 Number of Samples = 156 No. of Surface returns after screening = 43 Number ofTIAB Samples= 129 = 0.028 - 0.031 Magnitude (Area Values) Number of Samples = 123 No. of Surface returns after screening = 38 Number of Samples= 114 Magnitude (Area Values) 0.6 TIAB = 0.028 - 0.031 0.7 Original No. 2016, of Surface returns = 41 Remote Sens. 8, 1006 Magnitude (Area Values) 0.7 0.4 0.5 0.4 0.3 0.3 A rea M ean = 0.0657 S td D eviation = 0.012 0.2 0.2 0.1 0.1 0.6 0 0 0.2 0.4 Time (usec) 0.6 0Wind Speed = 6.6 m/s - 7.1 m/s 0 0.2 0.4 0.6 Time (usec) Wind Speed = 6.6 m/s - 7.1 m/s 0.6 Figure 15. Example area values at various TIAB and and windwind speedspeed values. Also given Examplecurve curvefits fitsshowing showing area values at various TIAB values. Also is number of15.returns filtered out theby two standard deviation tests. and given is number of returns filtered out the two standard deviation tests. Figure Example curve fits by showing area values at various TIAB wind speed values. Also given is number of returns filtered out by the two standard deviation tests. Table 1. 1. Area under surface returns for various TIAB and surface wind speed values for Southern Table 1. Area Pacific Ocean, 532 under nm. surface returns for various TIAB and surface wind speed values for Southern Pacific Ocean, 532 nm. Wind Speed −1 Wind Speed TIAB (sr Wind Speed −1 ) ) −1 TIAB (sr TIAB (sr )3.7 m/s–3.9 m/s m/s–3.9 m/s 3.73.7 m/s–3.9 m/s 0.012–0.0125 ± 0.027 0.012–0.01250.2305 0.2305 ± 0.027 0.012–0.0125 0.2305 ± 0.027 0.016–0.017 ± 0.026 0.016–0.017 0.2041 0.2041 ± 0.026 0.016–0.017 0.2041 ± 0.026 0.022–0.024 ±±0.027 0.022–0.024 0.1474 0.1474 ± 0.027 0.022–0.024 0.1474 0.027 0.028–0.031 0.1174 0.019 0.028–0.031 ±±0.019 0.028–0.031 0.1174 0.1174 ± 0.019 0.034–0.036 0.0824 0.011 0.034–0.036 0.0824 0.0824 ± 0.011 0.034–0.036 ±±0.011 0.24 0.24 0.22 Magnitude (Area Values) Magnitude (Area Values) 0.22 0.2 0.2 0.18 0.18 Wind Wind Speed Wind Speed Wind Speed WindSpeed Speed Wind Speed Wind Wind Wind Speed Wind Speed Wind Speed SpeedSpeedWind Speed 4.4 m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s 6.6 m/s–7.1 m/s 4.4 m/s–5.3 m/sm/s5.5 m/s–6.0 m/s m/s 6.6 m/s–7.1 4.4m/s–4.6 m/s–4.6 m/s m/s 5.1 5.1 m/s–5.3 5.5 m/s–6.0 6.6 m/s m/s–7.1 m/s 0.1940 ± 0.017 0.1625±±0.012 0.012 0.1538 ± 0.013 0.1330 0.1330 ± 0.013 0.1940 0.1625 ± 0.013 ±0.1330 0.013 0.1940 ±±0.017 0.017 0.1625 ± 0.012 0.15380.1538 ± 0.013 ± 0.013 0.1675 ±±0.016 0.1500±±0.018 0.018 0.1358 0.1358 ± 0.016 0.1230 0.1230 ± 0.01 0.1675 0.016 0.1500 ± 0.016 ± 0.01 0.1675 ± 0.016 0.1500 ± 0.018 0.1358 ± 0.016 0.1230 ± 0.01 0.1128 0.1094 0.015 0.0960 ± 0.017 ± 0.017 0.1128±±±0.023 0.023 0.1094 ±±0.015 ± 0.017 ± 0.017 0.023 0.1094 ± 0.015 0.0960 0.0960 ± 0.0170.0990.099 0.099 ± 0.017 0.014 0.0781 ± 0.010 0.0715 0.0715 ± 0.012 ± 0.012 0.0875 0.0781 0.010 0.0715 ± 0.012 0.0657 ± 0.012 0.0875±±±0.014 0.014 0.0781 ±±0.010 ± 0.012 0.0657 ±0.0657 0.012 0.0759±±±0.008 0.008 0.0674 ± 0.006 0.0589 0.0589 ± 0.008 ± 0.003 0.0759 0.008 0.0674 ±±0.006 ± 0.008 0.0565 ±0.0565 0.003 0.0759 0.0674 0.006 0.0589 ± 0.008 0.0565 ± 0.003 TIAB Range = 0.012 - 0.0125 TIAB Range = 0.012 - 0.0125 TIAB Range = 0.016 - 0.017 TIABRange Range = 0.016 - 0.017 TIAB = 0.022 - 0.024 TIABRange Range = 0.022 - 0.024 TIAB = 0.028 - 0.031 TIABRange Range = 0.028 - 0.031 TIAB = 0.034 - 0.036 TIABArea Range = 0.034 - 0.036 Mean Values Mean Area Values 0.16 0.16 0.14 0.14 0.12 0.120.1 0.08 0.1 0.06 0.08 0.04 3 0.06 0.04 3 4 5 6 Surface Wind Speed (m/s) 4 5 6 Surface Wind Speed (m/s) 7 7 Figure 16. Plots showing variation areawith withwind windspeed speed and TIAB for Southern Pacific Figure 16. Plots showing variationofofestimated estimated area and TIAB for Southern Pacific Ocean, 532 nm. Ocean, 532 nm. Figure 16. Plots showing variation of estimated area with wind speed and TIAB for Southern Pacific Ocean, nm. 2. Area under surface returnsfor forvarious various TIAB wind speed values for Southern TableTable 2.532 Area under surface returns TIABand andsurface surface wind speed values for Southern Pacific Ocean, 1064 Pacific Ocean, 1064 nm.nm. Table 2. Area under surface returns for various TIAB and surface wind speed values for Southern Wind Speed Wind Speed Wind Speed Wind Speed Wind Speed TIABOcean, (sr−1) 1064 Pacific nm.Speed Wind Speed Wind Speed Wind m/s Speed 6.6 m/s–7.1 Wind Speed 3.7 m/s–3.9 m/s 4.4Wind m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s TIAB (sr−1 ) 0.012–0.0125 Wind 0.2846 ± 0.026 3.7 m/s–3.9 m/s Speed TIAB0.016–0.017 (sr−1) 0.2493 ± 0.04 0.012–0.0125 3.7 m/s–3.9 0.2846 ± 0.026 m/s 0.022–0.024 0.2024± ± 0.037 0.016–0.017 0.2493 0.04 0.012–0.0125 0.2846 ± 0.026 0.022–0.024 0.2024 0.028–0.031 0.1525±± 0.037 0.035 0.016–0.017 ± ±0.04 0.028–0.031 0.1525 0.034–0.036 0.2493 0.1017 ± 0.035 0.003 0.034–0.036 0.1017 ± 0.003 0.022–0.024 0.2024 ± 0.037 0.028–0.031 0.1525 ± 0.035 0.034–0.036 0.1017 ± 0.003 0.2400 ± 0.023 ±Speed 0.018m/s 4.4 m/s–4.6 m/s 0.2208 5.1 m/s–5.3 Wind Speed Wind 0.2240 ± 0.02 0.2066 ± 0.018 0.2400 ± 0.023 ± 0.018 4.4 m/s–4.6 m/s 5.1 0.2208 m/s–5.3 m/s 0.1609 0.1520 ± 0.032 0.2240±±0.03 0.02 0.2066 ± 0.018 0.2400 ± 0.023 0.2208 ± 0.018 0.1609±± 0.03 0.1520 ± 0.032 0.1135 0.014 0.096 ± 0.003 0.2240 0.2066 0.018 0.1135±±±0.02 0.014 0.096 0.003 0.0825 0.006 0.0833 ±±± 0.011 0.0825±±0.03 0.006 0.0833±± 0.011 0.1609 0.1520 0.032 0.1135 ± 0.014 0.096 ± 0.003 0.0825 ± 0.006 0.0833 ± 0.011 0.1944 0.013 ± 0.019 5.5 ±m/s–6.0 m/s0.1755 6.6 m/s–7.1 m/s Wind Speed Wind Speed 0.1766 ± 0.028 0.1683 ± 0.018 ± 0.013 ± 0.019 5.50.1944 m/s–6.0 m/s 6.60.1755 m/s–7.1 m/s 0.1219 ± 0.026 ± 0.019± 0.018 0.1766 ± 0.028 0.129 0.1683 0.1944 ± 0.013 0.1755 ± 0.019 0.1219 ± 0.026 0.0893 0.129 ± 0.019 0.0916 ± 0.016 ± 0.012 0.1766 ±±0.028 0.1683 ±±0.018 0.0916 0.016 0.0561 0.0893 0.012 0.0760 ± 0.004 ± 0.01 0.0760±±0.026 0.004 0.0561 0.01 0.1219 0.129 ±± 0.019 0.0916 ± 0.016 0.0760 ± 0.004 0.0893 ± 0.012 0.0561 ± 0.01 Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, 1006 16 of 27 16 of 27 TIAB Range = 0.012 - 0.0125 TIAB Range = 0.016 - 0.017 TIAB Range = 0.022 - 0.024 TIAB Range = 0.028 - 0.031 TIAB Range = 0.034 - 0.036 Mean Area Values Magnitude (Area Values) 0.3 0.25 0.2 0.15 0.1 0.05 3 4 5 6 Surface Wind Speed (m/s) 7 Figure Figure 17. 17. Plots Plots showing showing variation variation of of estimated estimated area area with with wind wind speed speed and and TIAB TIAB for for Southern Southern Pacific Pacific Ocean, 1064 1064 nm. nm. Ocean, Table 3. Area Areaunder undersurface surfacereturns returns various TIAB surface for Atlantic Table 3. forfor various TIAB andand surface windwind speedspeed valuesvalues for Atlantic Ocean, Ocean, 532 nm.532 nm. Wind Speed Wind Speed Wind Speed Wind Speed Wind Speed 0.2250 ± 0.009 0.2250 ± 0.009 0.1951 ± 0.018 0.1951 ± 0.018 0.1380 ± 0.018 0.1380 ± 0.018 0.0945 ± 0.009 0.0945 ± 0.009 0.0727 ± 0.009 0.0727 ± 0.009 0.2037 ± 0.021 0.2037± ± 0.021 0.1780 0.024 0.1780 ± 0.024 0.1097 ± 0.023 0.1097 ± 0.023 0.0854 ± 0.015 0.0854 ± 0.015 0.0637 0.014 0.0637± ± 0.014 0.1865 ± 0.014 0.1865± ± 0.014 0.1585 0.017 0.1585 ± 0.017 0.1085 ± 0.016 0.1085 ± 0.016 0.0810 ± 0.016 0.0810 ± 0.016 0.0600 0.009 0.0600± ± 0.009 0.1342 ± 0.012 0.1342±±0.014 0.012 0.1227 0.1227 ± 0.014 0.0895 ± 0.009 0.0895 ± 0.009 0.0683 ± 0.01 0.0683 ± 0.01 0.0540 0.0540±±0.009 0.009 0.1283 ± 0.01 0.1283± ± 0.01 0.1181 0.009 0.1181 ± 0.009 0.0870 ± 0.003 0.0870 ± 0.003 0.0607 ± 0.01 0.0607 ± 0.01 0.054 0.054±±0.008 0.008 Wind Speed Wind Speed Wind Speed Wind Speed Wind Speed TIAB (sr−1 ) 3.7 m/s–3.9 m/s 4.4 m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s 6.6 m/s–7.1 m/s 3.7 m/s–3.9 m/s 4.4 m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s 6.6 m/s–7.1 m/s TIAB (sr−1) 0.012–0.0125 0.012–0.0125 0.016–0.017 0.016–0.017 0.022–0.024 0.022–0.024 0.028–0.031 0.028–0.031 0.034–0.036 0.034–0.036 Table 4. Area under surface returns for various TIAB and surface wind speed values for Atlantic Table 4. Area under surface returns for various TIAB and surface wind speed values for Atlantic Ocean, Ocean, 1064 nm. 1064 nm. Wind Speed Wind Speed 3.7 m/s–3.9 m/s TIAB (sr−1 ) 3.7 m/s–3.9 0.012–0.0125 0.2861 ± 0.027m/s 0.016–0.017 ± 0.035 0.012–0.0125 0.2607 0.2861 ± 0.027 0.022–0.024 0.1746 0.03 0.016–0.017 0.2607± ± 0.035 0.022–0.024 0.1221 0.1746 ± 0.03 0.028–0.031 ± 0.022 0.028–0.031 0.1221± ± 0.022 0.034–0.036 0.1005 0.01 0.034–0.036 0.1005 ± 0.01 TIAB (sr−1) Wind Speed Wind Speed 4.4 m/s–4.6 m/s 4.4 m/s–4.6 0.2537 ± 0.034m/s 0.2374 0.028 0.2537± ± 0.034 0.1523 0.028 0.2374± ± 0.028 0.1523± ± 0.028 0.1083 0.013 0.1083± ± 0.013 0.0890 0.018 0.0890 ± 0.018 Wind Speed Speed 5.1 Wind m/s–5.3 m/s 5.1 m/s–5.3 m/s 0.2387 ± 0.022 0.2008 0.020 0.2387± ± 0.022 0.1443 0.028 0.2008± ± 0.020 0.1443± ± 0.028 0.0968 0.008 0.0968± ± 0.008 0.0872 0.011 0.0872 ± 0.011 Wind Speed Wind Speed Speed Speed 5.5 Wind m/s–6.0 m/s 6.6Wind m/s–7.1 m/s 5.5 m/s–6.0 m/s 0.1608 6.6 m/s–7.1 m/s 0.1820 ± 0.015 ± 0.013 0.1649 0.152 0.023 0.1820±±0.017 0.015 0.1608± ± 0.013 0.1162 0.1649 ±±0.01 0.017 0.1122 0.152 ±±0.007 0.023 0.1162± ± 0.01 0.1122±±0.016 0.007 0.0935 0.004 0.0888 0.0935±±0.008 0.004 0.0888 ±±0.01 0.016 0.0832 0.0820 0.0832 ± 0.008 0.0820 ± 0.01 Table 5. Area under surface returns for various TIAB and surface wind speed values for Indian Table 5.532 Area Ocean, nm.under surface returns for various TIAB and surface wind speed values for Indian Ocean, 532 nm. Wind Speed 3.7 m/s–3.9 m/s Wind Speed −1 ) TIAB (sr 0.012–0.0125 0.2315 ± 0.01m/s 3.7 m/s–3.9 0.016–0.017 0.2048 ± 0.018 0.012–0.0125 0.2315 ± 0.01 0.022–0.024 0.1472 ± 0.026 0.016–0.017 0.2048 ± 0.018 0.028–0.031 0.0989 0.01 0.022–0.024 0.1472± ± 0.026 0.034–0.036 0.0835 ± 0.009 0.028–0.031 0.0989 ± 0.01 0.034–0.036 0.0835 ± 0.009 TIAB (sr−1) Wind Speed 4.4 m/s–4.6 m/s Wind Speed 0.2092 ± 0.02m/s 4.4 m/s–4.6 0.1801 ± 0.022 0.2092 ± 0.02 0.1173 ± 0.021 0.1801 ± 0.022 0.0871 0.017 0.1173± ± 0.021 0.0678 ± 0.008 0.0871 ± 0.017 0.0678 ± 0.008 Wind Speed 5.1 Wind m/s–5.3 m/s Speed 0.1791 ± 0.017 5.1 m/s–5.3 m/s 0.152 ± 0.018 0.1791 ± 0.017 0.1193 ± 0.008 0.152 ± 0.018 0.0778 0.014 0.1193± ± 0.008 0.0654 ± 0.008 0.0778 ± 0.014 0.0654 ± 0.008 Wind Speed Wind Speed 5.5 Wind m/s–6.0 m/s 6.6 m/s–7.1 m/s Speed Wind Speed 0.1538 ± 0.016 ± 0.008 5.5 m/s–6.0 m/s 0.1262 6.6 m/s–7.1 m/s 0.14 ± 0.015 0.121 ± 0.007 0.1538 ± 0.016 0.1262 ± 0.008 0.1036 ± 0.021 0.0755 ± 0.011 0.14 ± 0.015 0.121 ± 0.007 0.0688 0.1036 ±±0.01 0.021 0.0554 0.0755±±0.005 0.011 0.0594 0.008 0.0493 0.0688± ± 0.01 0.0554±±0.005 0.005 0.0594 ± 0.008 0.0493 ± 0.005 Remote Sens. 2016, 8, 1006 17 of 27 Table 6. Area under surface returns for various TIAB and surface wind speed values for Indian Ocean, 1064 nm. TIAB (sr−1 ) 0.012–0.0125 0.016–0.017 0.022–0.024 0.028–0.031 0.034–0.036 Wind Speed Wind Speed Wind Speed Wind Speed Wind Speed 3.7 m/s–3.9 m/s 4.4 m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s 6.6 m/s–7.1 m/s 0.2704 ± 0.022 0.2436 ± 0.029 0.187 ± 0.032 0.1273 ± 0.019 0.1134 ± 0.012 0.248 ± 0.034 0.228 ± 0.018 0.1462 ± 0.032 0.1133 ± 0.011 0.0928 ± 0.015 0.2223 ± 0.018 0.1945 ± 0.022 0.1398 ± 0.017 0.0963 ± 0.003 0.0878 ± 0.015 0.2147 ± 0.026 0.1885 ± 0.026 0.132 ± 0.023 0.0973 ± 0.016 0.0813 ± 0.009 0.158 ± 0.009 0.152 ± 0.011 0.0938 ± 0.011 0.0813 ± 0.008 0.067 ± 0.005 From the several tables and figures, it can be seen that the data binning increments yielded tightly clustered areas for all groupings, the percent standard deviations for which ranged from a high of ~20% (one was as high as 23%) to a low of ~3%. For each channel/ocean region, the percent standard deviation of the areas was less than 12% for more than half the groupings (anywhere from 52% to 68%). The percentage of samples retained for the groupings was generally >~75%. The number of retained samples was >~100 for over 70% of the groupings, with only four groupings having <~50 samples (28 being the lowest). Thus, there were enough samples for good statistics in almost all cases. No trends of note were exhibited in the area standard deviations insofar as retained sample size, TIAB value and wind speed value. The estimated area statistics were found to be quite similar for both channels and all three ocean regions. Here it important to emphasize that the area standard deviations stem from a number contributions including (a) random signal noise; (b) temporal-spatial variability in signals assigned to a given finite size bin (recall that signals in a bin are not necessarily contiguous in space, time or stem from one aerosol type); (c) possible uncertainty in the wind speeds used to assign signals to a given bin; and (d) any error in calibration normalized out of the attenuated backscatter signals that were analyzed to obtain the areas. The fact noted above that the estimated area percent standard deviation was <12% for the majority of the groupings is relevant in that it implies the same fractional uncertainty (±0.12) for retrieving the aerosol round-trip transmittance, T2a (z), which in turn implies half that uncertainty for retrieving the Aerosol Optical Depth (AOD), or ±0.06; there will be more on this in a later sub-section. One would expect these uncertainties to be lower for a collection of contiguous/nearly contiguous shots from a localized spatial region with constant wind speed and fixed aerosol loading. To what extent such conditions may be met can be assessed by examining the statistics of areas retrieved for individual shots and running mean areas for various averaging intervals. Example retrievals along short orbit segments given later in the paper demonstrate that such averaging over fairly homogeneous aerosol regions indeed yields significantly lower uncertainties in the averaged AOD retrievals (although bias error may still be present). 3.3. Verification of Area Retrievals The SR area retrievals presented in the previous sub-section were estimated by a fitting procedure, described earlier in Section 2.5, wherein an assumed normalized impulse response curve was positioned and fitted to the down-linked SR samples for each shot, the curve fit determining the SR area for the shot. The individual estimated shot areas were grouped with areas for other shots with nearly the same TIAB and wind speed and, after screening for outliers, the retained group areas were averaged to obtain the estimated SR mean area for the group and associated standard deviation. Alternatively, SR areas may be predicted by the derived analytic relation for ALPF given in Equation (5), repeated here below with the round-trip transmission, T2λ (zs ), resolved into the aerosol, Rayleigh and ozone components as was done in Equation (10). ALPF = 2T2 (z)T2R (z)T2Ozone (z)Rλ 2T2λ (z)Rλ = a c c (13) To predict ALPF from this analytic relation requires specification of Rλ , which can be computed from the wind speed model and the wind speed data for a given shot in the CALIPSO data base, as well as T2λ (zs ). The Rayleigh and ozone round-trip transmissions are fairly constant over oceans and Remote Sens. 2016, 8, 1006 18 of 27 can be computed from the information in the CALIPSO data base, the product of which for 532 nm is to a very close approximation T2R (zs ) × T2Ozone (zs ) = 0.798 × 0.96 = 0.76. The Rayleigh and ozone attenuations for 1064 nm are quite small so that T2R (zs ) × T2Ozone (zs ) = ~1 is a reasonable approximation. T2a (zs ) is generally unknown, but by selecting data for the aerosol free, clean atmospheres (for 532 nm TIAB < 0.0125), it can be approximated as unity. Thus, for data with TIAB < 0.0125, ALPF may be approximated for 532 nm as ALPF = 2T2a × T2R × T2Ozone × R532 2 × 1 × 0.76 × R532 2T2 R532 = = c c c (14) 2 × T2a × T2R × R1064 2T2 R1064 2 × 1 × 1 × R1064 = = c c c (15) and for 1064 nm as ALPF = Computing analytically predicted areas (APA) by these relations for the various wind speed bins defined earlier (mean wind of each wind speed bin used to calculate Rλ ) and using the data-estimated areas (DEA) presented earlier (e.g., Table 1) for these wind speed bins and TIAB < 0.0125, a comparison may be made of the two sets of area determinations as shown in Table 7 for the Southern Pacific Ocean data collection. It can be seen that the ratios of DEA/APA are close to one and well within the DEA standard deviations. Similar results were found for the Atlantic and Indian Ocean ratios as shown in Table 8 (The DEA bin values are not repeated, but can be found in Tables 3–6 nor are the APA bin values as they are same for all oceans). Averaging the ratios over all wind speeds yields the results shown in Tables 9 and 10. Table 7. Comparing analytically predicted and data-estimated areas under surface returns for the Southern Pacific oceanic region for clean atmospheric conditions. Wind Speed Analytically Predicted Surface Return area APA at 532 nm Data-Estimated Area DEA at 532 nm Ratio DEA/APA for 532 nm Analytically Predicted Surface Return Area APA at 1064 nm Data-Estimated Area DEA at 1064 nm Ratio DEA/APA for 1064 nm 3.7 m/s–3.9 m/s 4.4 m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s 6.6 m/s–7.1 m/s 0.2334 0.1979 0.1747 0.1612 0.1380 0.2305 ± 0.027 0.1940 ± 0.017 0.1625 ± 0.012 0.1538 ± 0.013 0.1330 ± 0.013 0.9875 0.9802 0.9301 0.9539 0.9640 0.2891 0.2452 0.2164 0.1998 0.1710 0.2846 ± 0.026 0.2400 ± 0.023 0.2208 ± 0.018 0.1944 ± 0.013 0.1755 ± 0.019 0.9844 0.9787 1.0203 0.9729 1.026 Table 8. Ratios of analytically predicted and data-estimated areas under surface returns for the Atlantic and Indian Ocean regions for clean atmospheric conditions. Wind Speed 3.7 m/s–3.9 m/s 4.4 m/s–4.6 m/s 5.1 m/s–5.3 m/s 5.5 m/s–6.0 m/s 6.6 m/s–7.1 m/s Ratio DEA/APA for 532 nm Ratio DEA/APA for 1064 nm Ratio DEA/APA for 532 nm Ratio DEA/APA for 1064 nm (Atlantic Ocean) (Atlantic Ocean) (Indian Ocean) (Indian Ocean) 0.9640 1.0292 1.0675 0.8323 0.9299 0.9896 1.0346 1.1030 0.9109 0.9403 0.9918 1.0570 1.0251 0.9539 0.9147 0.9353 1.0114 1.0272 1.0745 0.9240 It can be seen for the 1064 nm channel that the ratios for all oceans are within 1% of unity, while the results for the 532 nm channel fall within 4% of unity, indicating perhaps a slight bias off-set to lower DEA values, although the ratios are generally within their standard deviations. Such a bias could arise due to some aerosol contamination in the 532 nm signals assumed to be aerosol free for TIAB < 0.0125, or if the impulse response assumed for the 532 nm channel was slightly different than the actual impulse response for that channel, or possible error either in the lidar calibration or the reflectance model/wind speed input to the model. No such bias is suggested for the 1064 nm channel, indicating an absence of any significant effect from lidar calibration error or the reflectance model/wind speed input to the model having caused a bias (which would also affect the 532 nm results, thereby seemingly removing these errors as the source of the 532 nm off-set). Hence, Remote Sens. 2016, 8, 1006 19 of 27 the slight deviations from unity for either wavelength, being within there standard deviations, may just stem from normally expected variability. All in all, the agreement between the data estimated and analytically predicted areas is excellent, indicating corroboration of the technique and results presented earlier for estimating the area of SR signals from the down-linked SR samples. Table 9. Mean and standard deviation of DEA/APA ratios calculated over all wind speeds for each oceanic region at 532 nm wavelength for clean atmospheric conditions. Region Mean Ratio (Overall Wind Speeds) Standard Deviation Southern Pacific Atlantic Indian 0.9631 0.9646 0.9885 0.0227 0.0915 0.0563 Table 10. Mean and standard deviation of DEA/APA ratios calculated over all wind speeds for each oceanic region at 1064 nm wavelength for clean atmospheric conditions. Region Mean Ratio (Overall Wind Speeds) Standard Deviation Southern Pacific Atlantic Indian 0.9965 0.9957 0.9945 0.0017 0.0763 0.0637 3.4. Aerosol Retrievals Rearranging Equation (13), T2a (zs ) is given by T2a (zs ) = cALPF 2Rλ T2R (zs )T2Ozone (zs ) (16) Using the approximations given earlier for T2R (zs ) × T2Ozone (zs ), Equation (16) reduces, for both wavelengths, to cALPF T2a (zs ) = (17) 2 × R532 × 0.76 T2a (zs ) = cALPF 2 × R1064 (18) In turn, the aerosol optical depth (AOD), τa , is given by τa = − loge T2a (zs ) 2 (19) By differential analysis, the fractional uncertainty in T2a due to uncertainty in ALPF is ∆ T2a ∆ ALPF = 2 ALPF Ta (20) and the corresponding uncertainty in AOD is half that, ∆τa = −0.5 × ∆ ALPF ALPF (21) Example retrievals of T2a and AOD by Equations (16) and (19) applied to the ALPF retrievals given earlier (Tables 1–6), for one wind speed bin (5.1–5.3 m/s) and two TIAB bins (0.016–0.017 and 0.028–0.031), for all three ocean regions, are given in Tables 11–13. Also given in the tables are retrievals by an alternate method, called the High/Low method. Remote Sens. 2016, 8, 1006 20 of 27 Table 11. Representative example retrievals of aerosol round-trip transmission and AOD for Southern Pacific Ocean region. TIAB (sr−1 ) 0.016–0.017 0.028–0.031 Ta 2 AOD Ta 2 AOD Ta 2 AOD Ta 2 AOD (532 nm, High/Low Method) (532 nm, High/Low Method) (532 nm, Analytic Method) (532 nm, Analytic Method) (1064 nm, High/Low Method) (1064 nm, High/Low Method) (1064 nm, Analytic Method) (1064 nm, Analytic Method) 0.9281 ± 0.131 0.4832 ± 0.071 0.037 ± 0.07 0.364 ± 0.073 0.8558 ± 0.103 0.4456 ± 0.057 0.078 ± 0.0601 0.404 ± 0.0639 0.9357 ± 0.112 0.4348 ± 0.038 0.033 ± 0.059 0.416 ± 0.043 0.9654 ± 0.084 0.4486 ± 0.014 0.018 ± 0.043 0.401 ± 0.015 Table 12. Representative example retrievals of aerosol round-trip transmission and AOD for Atlantic Ocean region. TIAB (sr−1 ) 0.016–0.017 0.028–0.031 Ta 2 AOD Ta 2 AOD Ta 2 AOD Ta 2 AOD (532 nm, High Low Method) (532 nm, High Low Method (532 nm, Analytic Method) (532 nm, Analytic Method) (1064 nm, High Low Method) (1064 nm, High Low Method (1064 nm, Analytic Method) (1064 nm, Analytic Method) 0.8500 ± 0.111 0.4343 ± 0.092 0.081 ± 0.065 0.417 ± 0.105 0.9043 ± 0.097 0.4621 ± 0.091 0.050 ± 0.053 0.386 ± 0.098 0.8412 ± 0.114 0.4055 ± 0.053 0.086 ± 0.067 0.451 ± 0.065 0.9383 ± 0.086 0.4523 ± 0.042 0.032 ± 0.045 0.397 ± 0.046 Table 13. Representative example retrievals of aerosol round-trip transmission and AOD for Indian Ocean region. TIAB (sr−1 ) 0.016–0.017 0.028–0.031 Ta 2 AOD Ta 2 AOD Ta 2 AOD Ta 2 AOD (532 nm, High Low Method) (532 nm, High Low Method (532 nm, Analytic Method) (532 nm, Analytic Method) (1064 nm, High Low Method) (1064 nm, High Low Method (1064 nm, Analytic Method) (1064 nm, Analytic Method) 0.8487 ± 0.129 0.4344 ± 0.088 0.082 ± 0.075 0.417 ± 0.101 0.8672 ± 0.102 0.4439 ± 0.080 0.071 ± 0.058 0.406 ± 0.090 0.8749 ± 0.122 0.4332 ± 0.038 0.067 ± 0.064 0.418 ± 0.043 0.9089 ± 0.103 0.4500 ± 0.014 0.048 ± 0.056 0.399 ± 0.015 Remote Sens. 2016, 8, 1006 21 of 27 As the ratio of ALPF for two different TIAB values and the same wind speed equals the corresponding ratio of T2a , the aerosol round-trip transmission for a high TIAB, T2a (high TIAB), is given by A (High TIAB) T2a (High TIAB) = LPF × T2a (Low TIAB) (22) ALPF (Low TIAB) Selecting the low TIAB to be for the clean, aerosol-free atmosphere case (TIAB < 0.0125) for which the aerosol round-trip transmission is approximated as unity, T2a (High TIAB) simply equals the ratio ALPF (High TIAB)/ALPF (Clean Atmosphere). An advantage of the High/Low method is that it eliminates the need for an accurate surface reflectance-wind speed model as the reflectance cancels in the area ratio, although the standard deviation for the retrieved aerosol round-trip transmission is generally a little higher than for the analytic method because the standard deviation of each of the areas in the ratio must be taken into account. It can be seen from the tables that the T2a retrievals for both methods agree well within their respective standard deviations (most within ~0.05) and the AODs agree within ~0.05 (most within ~0.03). This, as with the results in Tables 9 and 10, again suggests that errors in either the reflectance model/wind speed inputs to the model for determining the analytically determined AODs or lidar calibration error (which could affect the High/Low determinations) were not significant. The results for the other wind speed and TIAB bins are similar insofar as having about the same variability/uncertainty in retrieved T2a and AOD. The AOD uncertainty is comparable to the AOD retrievals for the lower TIAB (0.016 to 0.017), making it difficult to quantitatively interpret these AOD, but the higher TIAB (0.028 to 0.031) AODs generally appear good enough to be quantitatively useful. Examination of the AOD spectral ratio (532/1064) revealed that this ratio ranged from about 1.05 to 1.2, most being 1.1 or greater, which is within the range of the ratios for dust and marine aerosol models (e.g., [15]). The CALIPSO browse images for the ~15 days and regions for the observations investigated here revealed that the aerosols were mainly identified as marine aerosols. Equations (16) and (19) were used to retrieve the AOD for a sample collection of ~50 nearly contiguous lidar shots for an orbit segment over the Atlantic Ocean. These shots were for a 9 May 2011 segment between the lat-lon positions (−3.3 lat, −16.96 lon) and (−2.85 lat, −16.86 lon), which corresponds to about ~75 shots, amongst which ~50 had detectable surface returns (with 0.0125 < TIAB < 0.035). Figure 18 shows the per-shot retrievals of T2a and AOD for both wavelengths, and the TIAB times 20 (to be on scale) is also shown. The correlation of TIAB with AOD and anti-correlation with T2a is clearly evident. The mean AODs are about the same for both wavelengths (0.155 for 532 nm and 0.148 for 1064 nm, each with a standard deviation uncertainty of ±0.045). The AOD is fairly flat over the segment for 532 nm, but displays a slight rising trend for 1064 nm. As such, averaging over several shots should reduce the per-shot AOD uncertainty (~±0.05); averaging over six consecutive shots (2 km averaging) reduced the AOD uncertainty to <±0.02 for the averaged AODs. The spectral ratio (1064/532) of T2a has a mean of ~1.01, ranging from ~0.96 to ~1.12, while for AOD the mean spectral ratio is ~1.04, ranging from ~0.70 to ~1.15 (rather variable). Clearly, the mean spectral ratios are fairly neutral, and the mean AOD ratio is close to the range that applies to dust and marine aerosols (e.g., [15]). Examining the CALIPSO browse image for this segment revealed that the aerosols present were indeed mainly identified as marine aerosols. Remote Sens. 2016, 8, 1006 Remote Sens. 2016, 8, x FOR PEER REVIEW 22 of 27 22 of 27 532 nm Channel Aerosol Optical Depth Round Transmission TIAB x 20 1.2 1 Magnitude 0.8 0.6 0.4 0.2 0 -0.2 Lattitude -3.2 -3.15 -3.1 -16.90 -16.91 Longitude -16.93 -3.05 -16.89 -3 -16.88 -2.95 -16.88 -2.9 -16.87 -2.85 -16.86 1064 nm Channel Aerosol Optical Depth Round Transmission TIAB x 20 1.2 1 Magnitude 0.8 0.6 0.4 0.2 0 -0.2 Lattitude -3.25 Longitude -16.95 -3.2 -3.15 -3.1 -3.05 -16.93 -16.9 -16.89 -16.88 -3 -2.95 -2.9 -2.85 -16.87 -16.87 -16.87 -16.86 Figure 18. 18. Aerosol Aerosolround-trip round-triptransmission, transmission,AOD AOD and TIAB each retained sample point for nm 532 Figure and TIAB forfor each retained sample point for 532 nm and 1064 nm channels. and 1064 nm channels. The spectral ratio of aerosol round-trip transmission is of further interest because it can be The spectral ratio of aerosol round-trip transmission is of further interest because it can be estimated directly from the spectral ratio of the A without having to assume a particular wind estimated directly from the spectral ratio of the ALPF without having to assume a particular wind speed model, save accounting for the difference in Fresnel reflectance due to the ocean refractive speed model, save accounting for the difference in Fresnel reflectance due to the ocean refractive index index difference at the two wavelengths. From Equation (13), the spectral ratio (1064/532) of A , difference at the two wavelengths. From Equation (13), the spectral ratio (1064/532) of ALPF , using the using the numerical estimates for the round-trip Rayleigh and ozone transmittances given earlier, numerical estimates for the round-trip Rayleigh and ozone transmittances given earlier, reduces to reduces to T2T ALPF 1 1 RR A 1064 = = × ×1064 × × a2 1064 ALPF 0.76 TaT532 0.76 R532 A 532 R (23) (23) Assuming the thereflectances reflectances equal at wavelength, each wavelength, except for the refractive index Assuming areare equal at each except for the refractive index difference difference in the Fresnel reflectances, havingratio a spectral ratio(for of ~1/1.06 1064 to 532),(23) Equation in the Fresnel reflectances, having a spectral of ~1/1.06 1064 to(for 532), Equation reduces(23) to reduces to T2 T2 T2 ALPF 1064 1 R 1 1 A = R × a 1064 T = 1× 1× aT1064 = 1.241 × Ta 1064 ×1 1064 (24) (24) = ×2 = × ×2 = 1.241 ×T2 A 0.76 R× 0.76 1.06 LPF 532 0.76 532R Ta 532 0.76 1.06 TaT532 A T Ta 532 For For the the clean, clean, aerosol-free aerosol-free situation situation (TIAB (TIAB << 0.0125), 0.0125), the the aerosol aerosol transmission transmission spectral spectral ratio ratio reduces reduces to unity and the A ALPF spectral spectral ratio ratio is is simply simply 1.241. 1.241. Examining the A ALPF values values for for 1064 1064 nm nm and 532 nm given earlier in Tables 1–6, for TIAB < 0.0125 and averaging overall wind speeds and nm given earlier in Tables 1–6, for TIAB < 0.0125 and averaging overall wind speeds per per ocean region, yields spectral , of 1.281 1.283,and 1.281 andfor 1.248 ocean region, yields meanmean area area spectral ratios,ratios, A ALPF /A1064 /A,LPF of 532 1.283, 1.248 the for the Southern Pacific Ocean, Atlantic Ocean and Indian Ocean, respectively, all within ~3% of Southern Pacific Ocean, Atlantic Ocean and Indian Ocean, respectively, all within ~3% of the 1.241 the 1.241 value, substantiating theofvalidity of therelation analytic relation given in(24). Equation (24).difference, This ~3% value, substantiating the validity the analytic given in Equation This ~3% as with the ~4% difference noted regarding the 532 nm results in Table 7, could arise due to some aerosol contamination or the assumed impulse response curve for the 532 nm channel being slightly Remote Sens. 2016, 8, 1006 23 of 27 difference, as with the ~4% difference noted regarding the 532 nm results in Table 7, could arise due to some aerosol contamination or the assumed impulse response curve for the 532 nm channel being slightly different than the actual impulse response for that channel. Examining the ALPF spectral ratios for all wind speed bins and for bins with TIAB > 0.0125 in Tables 1–6, shows that ~90% of the T2a 1064 /T2a 532 ratios are >1, meaning AOD532 > AOD1064 almost always, and that these ratios are bounded by ~0.80 < T2a 1064 /T2a 532 < ~1.2 (with ~70% being between 1.0 and 1.1). Note that retrieving the spectral aerosol round-trip transmittance ratio does not yield the individual wavelength AODs, just the difference, AOD532 − AOD1064 [8]. Nevertheless, if AOD can be retrieved at only one wavelength, the other can be found knowing this difference, and knowing the difference could be a useful constraint with other techniques for retrieving AOD or identifying aerosol types. A final example of AOD retrieval along a CALIPSO orbit segment on 22 August 2010 is shown in Figure 19 from combined CALIPSO and under-orbit airborne HSRL measurements during the Caribbean Campaign [16] in August 2010. The NASA Langley airborne HSRL [17] can retrieve the AOD at 532 nm directly by the high spectral resolution lidar (HSRL) technique, providing a truth comparison with the lidar surface return AOD retrieval technique (HSRL uncertainty in AOD retrievals given in Figure 19 is estimated to be <±0.005 based on HSRL retrieval comparisons with both airborne sun-photometer and ground-based AERONET measurements [16], and this is the uncertainty obtained by averaging the HSRL retrievals over the latitude range shown in Figure 19). The shot-by-shot CALIOP AOD retrievals displayed some large spiking (8 of the ~120 shots in the segment), likely due to pre-cloud/cloud-forming effects as is typical of the Caribbean and as seen in the CALIPSO browse image for this segment (which also showed that the aerosol present was likely from an intrusion of dust), so these were screened and a 15-shot (5 km) average was formed for the CALIPSO-derived curve shown in the figure (yielding a standard deviation of ±0.015). The two retrieval curves track fairly well, and their means agree within ~0.05. As CALIPSO passed over this surface segment within seconds, while the HSRL aircraft took upwards of ~15 min to complete the segment, some spatial-temporal variation between the curves could occur (perhaps as seen in the lat region between 13.9 to 14 degrees), although results by Rogers et al. [16] indicate negligible difference should occur due to such a small temporal mismatch. This preliminary result of the lidar surface return AOD retrieval technique being capable of retrieving AOD within ~0.05 is regarded as a good start. It compares favorably with the accuracy first reported by Josset et al. [18] for their retrieval approach using combined CALIPSO and CloudSat ocean surface returns. It is also within the statistically determined difference between CALIPSO-derived AODs, using assumed aerosol models, and HSRL-determined AODs (i.e., standard deviation of CALIPSO model-derived AODs fell within the HSRL AOD determinations for 50% of the comparisons), for many comparisons [16]. However, an additional point to note regarding this comparison is that subsequent investigation of measurements made of flight hardware replicas of the CALIOP detector and post-detection electronics [5], as well as on-orbit investigations of surface return signals [6,7], when examined on a log scale revealed a slight after-pulsing tail on the measured 532 nm impulse response (such after-pulsing is not uncommon in photomultiplier tube (PMT) detectors), which, if included in the impulse response area integration, could bias ALPF higher and AOD lower. Preliminary investigations to characterize and remove the tail effect by limiting the area determination under the impulse response curve to about the first 400 nanoseconds after the pulse start yielded a higher AOD determination of 0.125 [19], an AOD increase of 0.021 (or an ALPF area decrease of 4.2%), which brings the tail-corrected AOD (0.125) to about 0.03 below the HSRL AOD retrieval of 0.158. Another possible effect which can also bias the ALPF retrieval too high is a contribution from backscattering in the water below the air-water interface. This effect was not assessed in the initially submitted manuscript, but one of the authors (J. Reagan) was made aware of this possible area contribution (by Chris Hostetler) during a visit to NASA Langley Research Center on 3 November 2016. While water is opaque to 1064 nm light, it is slightly transmissive/transparent at 532 nm, although light at this wavelength is largely extinguished within a few tens of meters below the water surface. To estimate the water backscattering area contribution, Aw , in a form directly comparable to Remote Sens. 2016, 8, 1006 24 of 27 the water reflectance contribution, ALPF , a number of effects must be taken into account. First of all, the total backscattering from the transmitted lidar pulse as it propagates downward in the water is given Remote 2016,Total 8, x FOR PEER REVIEW 24 ofz27 by theSens. water Integrated Attenuated Backscatter, TIABw , for an integration in-water distance, w, from 0 at the surface to a distance below the surface where backscattering is effectively nil (a few 10 s of distance, zw, from the 0 atwater the surface to a distance below the constant surface where backscattering is effectively meters). Treating backscatter, βw , as effectively over the short penetration distance nil (a few 10 s of meters). Treating the water backscatter, β w, as effectively constant over the short and the water extinction as Sw βw , where Sw is the water extinction-to-backscatter ratio, TIABw reduces penetration distance and the water extinction as Swβw, where Sw is the water to simply 1/2S w . As the propagation is in water, the speed of propagation is 2c/n; where n is the extinction-to-backscatter ratio, TIABwofreduces to simply 1/2Sw. Astimes the propagation is in water, water refractive index (1.33), a factor 2n/c should be multiplied TIABw , analogous to the the 2/c speed of propagation is 2c/n; where n is the water refractive index (1.33), a factor of 2n/c should be term in Equation (5) for ALPF . A transmission loss occurs as the laser pulse transmits into water and multiplied TIAB w, analogous to the 2/c term in Equation (5) for ALPF. A transmission loss backscattertimes exits the water because the air-water transmittance, Taw = (1 − R532 ), is <1, causing an 2 occurs as the laser pulse transmits into water andthe backscatter exits transmittance, the water because air-water additional loss (1 − R532 ) to be multiplied times air round-trip T2 (zsthe ). Finally, the transmittance, T aw = (1 − R532), is <1, causing an additional loss (1 − R532)2 to be multiplied times the air backscatter exiting water to air is refracted causing a beam-spreading effect that reduces the radiance 2 s). Finally, 2 . Hence, round-trip thethe backscatter exiting to water to air is lidar refracted causing a seen by thetransmittance, lidar receiver T by(z1/n Aw contribution the received signal, directly 2. Hence, the Aw beam-spreading effect that reduces the radiance seen by the lidar receiver by 1/n comparable to ALPF in Equation (5), is given by contribution to the received lidar signal, directly comparable to ALPF in Equation (5), is given by 2 2 2 2nT2 (zs ) ((1 − )( R532 )) TIABW ( T )((zs ) (1) − R532 ) AW = A = = , (25) = , (25) ncSW n2 c w. The ratio of Aw over ALPF is then simply including including the the result result that that TIAB TIABwwevaluates evaluatesto to1/2S 1/2S w . The ratio of Aw over ALPF is then simply (1 − R ) A (26) = (1 − R532 )2 AAW = 2nS R (26) ALPF 2nSW R532 Using water parameter values representative of relatively clean open ocean water as given by −1·sr−1,ocean Using[20] water representative of relatively water as R given observation site time (i.e., βw = ~3 × clean 10−4 mopen Sw = 175 sr and 532 = Churnside andparameter R532 for thevalues −4 m−1 ·sr−1 , by Churnside [20] (5) and R532a for theof observation site time (i.e., = ~3 × 10 ~0.03 sr−1), Equation yields value ~0.067 (indicating a 6.7% areaβenhancement to A LPF due to w − 1 Sw = backscatter), 175 sr and Rindicating sr AOD ), Equation yields~0.034 a value ~0.067 (indicating 6.7% area water retrieval (5) is biased toooflow. For the assumedaparameter 532 = ~0.03the enhancement to ALPF due to water backscatter), indicating the AOD retrieval is biased ~0.034 too values, the water-attenuated backscatter is reduced effectively to zero (within 0.1%) within twolow. of For the assumed parameter values, the water-attenuated backscatter is reduced effectively to zero the 532 nm down-linked samples (within 45 m below the surface), meaning the Aw contribution is (within 0.1%) withinintwo thesamples 532 nm determining down-linkedAsamples (within below surface), effectively captured the of same LPF. Adding both 45 themtail effectthe and water meaning the Aw contribution is =effectively captured in the sameAOD samples determining . Adding backscatter biases (0.021 + 0.034 0.055) yields a bias-corrected (0.104 + 0.055) of A 0.159, almost LPF both theequal tail effect and waterAOD backscatter biases (0.021Allowing + 0.034 = for 0.055) yields a bias-corrected exactly to the HSRL retrieval of 0.158. even a ±25% variation inAOD the (0.104 + 0.055) 0.159, exactly equal to the HSRL AOD retrieval of 0.158. Allowing for even estimated 0.055of bias (duealmost to some possible variation/uncertainty in the assumed parameters) yields a a ±25% variation thethe estimated some still possible in the bias-corrected AODin in range of0.055 0.145bias to (due 0.173,towhich falls variation/uncertainty within the ±0.015 standard assumed parameters) yields a bias-corrected AODfor in the 0.145 to 0.173, stillvalue falls within deviation estimated (from the 15-shot averaging) the range initialof CALIPSO AOD which retrieval (0.104 ±0.015 standard estimated (from the averaging) for the initial AOD ±the 0.015). Thus, with deviation bias correction, the HSRL and15-shot CALIPSO AOD retrievals are CALIPSO found to agree retrieval value (0.104 ± 0.015). Thus, with bias correction, the HSRL and CALIPSO AOD retrievals are within <±0.02. found to agree within <±0.02. HSRL Derived AOD = 0.158 ± 0.005 CALIPSO Derived AOD = 0.104 ± 0.015 Figure19. 19.Comparison Comparisonof ofCALIPSO CALIPSOocean oceansurface surfacereturn returnand andairborne airborneHSRL HSRLAOD AOD retrievals. retrievals. Figure 4. Conclusions A technique has been presented and applied to numerous Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO)/Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) observations for estimating from signal samples the normalized area, A , under the Remote Sens. 2016, 8, 1006 25 of 27 4. Conclusions A technique has been presented and applied to numerous Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO)/Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) observations for estimating from signal samples the normalized area, ALPF , under the received surface response from CALIOP-transmitted lidar pulses reflected from ocean surfaces. An analytic relation for ALPF has also been developed which shows that this area is proportional to the product of round-trip atmospheric transmission to the ocean surface, T2 (zs ), times the ocean surface backscatter reflectance, Rλ . The total integrated attenuated backscatter down to the ocean surface (TIAB), one of the CALIPSO data products, was demonstrated to be useful, along with ocean reflectance, for binning the ALPF estimates into sub-groups with similar properties and for demonstrating that the technique for estimating ALPF was in very good to excellent agreement with the analytic prediction for clean, aerosol-free cases, defined by TIAB values <0.0125 (indicating T2a = ~1.0). Groupings of ALPF defined by binning the areas in small increments of TIAB and wind speed (which in turn defined Rλ increments using an assumed reflectance model) yielded tightly clustered groups (majority of group ALPF having percent standard deviations within 12%) with similar statistics for both wavelength channels (532 and 1064 nm) and all three ocean regions that were investigated. Using Rλ predicted by the assumed ocean reflectance/wind speed model permitted retrieval of the aerosol round-trip transmittance, T2a , from the group ALPF values, and, in turn, the aerosol optical depth, AOD. As shown, the fractional uncertainty in the retrieved T2a due to uncertainty in ALPF equaled the fractional uncertainty in ALPF , while the AOD uncertainty equaled half that. An alternate High/Low method for retrieving T2a and AOD from ratios of ALPF for high and low TIABs, for the same wind speed, was also presented and demonstrated to be in very good agreement with results obtained by the analytic method. From the statistics for the retrieved ALPF , it was estimated that the uncertainty in AOD retrievals from the group ALPF should be less than ±0.06 in the majority of cases. Example AOD retrievals presented for two CALIPSO orbit track segments yielded similarly good results with per-shot AOD standard deviations within ±0.05. With multi-shot spatial averaging over a few km (2 to 5 km), the AOD retrieval uncertainty was reduced to <±0.02. One of the cases was concurrent with an under-orbit flight with an HSRL lidar at 532 nm that provided an independent AOD retrieval, and the means of the two 532 nm AOD retrievals were found to agree within 0.05, seemingly too high to be really useful except in cases of high AOD. However, two bias effects (PMT tail effect and underwater backscattering) were identified, both of which produce an enhancement in the data-estimated ALPF . Applying bias corrections for both of these effects yielded a bias-corrected CALIPSO AOD retrieval within 0.001 of the HSRL AOD retrieval. Allowing for reasonable uncertainty, the bias corrections still yielded a corrected AOD agreeing with the HSRL retrieval within ±0.015, which equals the uncertainty associated with the initial, uncorrected CALIPSO AOD retrieval. Thus, with bias corrections, the technique presented appears capable of retrieving AODs with an accuracy within ~±0.02 (corresponding to an error within ~±4% for the ALPF determination). It should be noted that the retrieval results were for CALIPSO observations over a limited global region (see Figure 14), and results might not be as good over other ocean regions; e.g., due to the lidar calibrations perhaps being more uncertain in regions more poleward. But it should also be noted that the analysis results for the regions investigated did not suggest any significant effect due to lidar calibration error or error in the wind speed model/wind speed input to the model. The spectral ratio of the aerosol round-trip transmission, T2a 1064 /T2a 532 , which can be determined without need of a specific wind speed–reflectance model, was also demonstrated to be useful in validating the expected ratio value for clean, aerosol-free conditions (TIAB < 0.0125), in retrieving the difference in aerosol optical depths (AOD) between the two wavelengths (AOD532 − AOD1064 ), and in providing a parameter potentially useful in aiding/constraining methods for typing aerosols. If AOD is retrieved at both wavelengths, the resulting AOD spectral ratio provides a more direct parameter for aiding aerosol typing. However, given AOD retrieved at just one wavelength, the retrieved spectral Remote Sens. 2016, 8, 1006 26 of 27 ratio of the aerosol round-trip transmission (yielding AOD532 − AOD1064 ) can be used to obtain the AOD at the other wavelength. AOD spectral ratios (532/1064) obtained for the area groups and one of the orbit track segment retrieval examples (9 May 2011) yielded ratios close to/within the range of ratios specified for marine and dust aerosol models (generally agreeing with the aerosol types identified in the CALIPSO browse images). The results of this investigation, although admittedly preliminary, argue strongly for implementing the technique presented here to retrieve atmospheric AODs from CALIOP ocean surface returns to form a CALIPSO database of global over ocean AOD at both 532 nm and 1064 nm. Such a database would be valuable in itself for monitoring changes in aerosols over time, investigating episodic aerosol events (e.g., dust and smoke layers) and in providing information useful in the development of predictive models of aerosols and their effects on climate. The surface-derived AOD retrievals at 532 nm and 1064 nm can also be used in combination with aerosol typing schemes presently used in producing CALIPSO backscatter and extinction data products to further confirm and enhance these products. The surface-derived spectral AOD information used in conjunction with CALIOP dual-wavelength atmospheric attenuated backscatter should also aid in differentiating aerosol types, or defining additional types, to obtain greater self-consistency between CALIOP profile retrievals and the surface-derived AOD product. The results presented here indicate that AOD retrievals, with bias corrections, may be accurate within ~±0.02, which is sufficient to be quite useful for most observed AODs. To confirm the capability for achieving this level of accuracy, a number of things/effects should be further investigated, particularly before using the technique to produce a CALIPSO global over-ocean data product. These include: modifying the impulse response model to remove the PMT tail effect bias; formulating a correction for the under-water backscattering bias on ALPF that is easy to implement; investigating possible improvements in the water reflectance model and wind speed estimates used in the model; formulating standard screening/saturated signal-rejection/multi-shot averaging procedures to apply to the data; using improved CALIPSO data product versions (i.e., newly issued version 4); confirming CALIPSO lidar calibration accuracies are sufficient to not significantly bias AOD retrievals in other ocean regions (or flag retrievals in regions where the calibrations are too uncertain), and testing the aforementioned on more CALIPSO data both within and outside the regions investigated in this paper. That said, the results presented here are considered very encouraging and warrant developing (along the lines suggested above) the presented AOD retrieval technique for widespread application. Acknowledgments: The authors gratefully acknowledge the support of the NASA CALIPSO Project and in particular the Algorithm Development and Data Management teams at the Langley Research Center. Discussions with and data provided by these teams, and in particular with Mark Vaughan, were a great benefit to accomplishing the work reported here. Special thanks also to William Hunt for providing information and assessments, and many useful discussions, of the results of lab tests made on flight hardware replicas of the CALIOP detector/post-detection electronics. NASA funding in support of much of this work was provided by sub-contracts through Science Systems and Applications, Inc. both to the University of Arizona and directly to the second author. Author Contributions: The results presented in this paper, in principle, constitute the thesis submitted by Srikanth Lolla Venkata (first author) as a part his master’s degree requirement at the University of Arizona. 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