Classification of particle effective shape ratios in cirrus clouds based on the lidar depolarization ratio Vincent Noel, Helene Chepfer, Guy Ledanois, Arnaud Delaval, and Pierre H. Flamant A shape classification technique for cirrus clouds that could be applied to future spaceborne lidars is presented. A ray-tracing code has been developed to simulate backscattered and depolarized lidar signals from cirrus clouds made of hexagonal-based crystals with various compositions and optical depth, taking into account multiple scattering. This code was used first to study the sensitivity of the linear depolarization rate to cloud optical and microphysical properties, then to classify particle shapes in cirrus clouds based on depolarization ratio measurements. As an example this technique has been applied to lidar measurements from 15 mid-latitude cirrus cloud cases taken in Palaiseau, France. Results show a majority of near-unity shape ratios as well as a strong correlation between shape ratios and temperature: The lowest temperatures lead to high shape ratios. The application of this technique to spaceborne measurements would allow a large-scale classification of shape ratios in cirrus clouds, leading to better knowledge of the vertical variability of shapes, their dependence on temperature, and the formation processes of clouds. © 2002 Optical Society of America OCIS codes: 080.2720, 010.3920, 280.3640, 010.2940, 290.5890. 1. Introduction Cirrus clouds have a strong influence on weather and climate1 because they consistently cover more than 30% of the Earth’s surface.2 To estimate their contribution to the energetic balance, a correct model of cirrus radiative properties is needed. Such a model strongly depends on the cloud’s microphysical properties, e.g., particle shape, size, and orientation. During the past two decades several intensive field experiments devoted to cirrus clouds have been conducted to document microphysical properties: the First and Second International Satellite Cloud Climatology Project 共ISCCP兲 Regional Experiment 共FIRE I and FIRE II兲,3,4 the International Cloud Experiment 共ICE兲,5,6 the European Cloud Radiation Experiment 共EUCREX兲,7–9 the Central Equatorial Pacific Experiment 共CEPEX兲,10 and the Subsonic Aircraft: Contrail and Cloud Effects Special Study 共SUCCESS兲.11 The results of these experiments confirm the strong dependence of the radiative prop- V. Noel 共[email protected]兲, H. Chepfer, G. Ledanois, A. Delaval, and P. H. Flamat are with the Laboratoire de Météorologie Dynamique, Ecole Polytechnique, 91128 Pasaiseau, France. Received 3 August 2001; revised manuscript received 4 March 2002. 0003-6935兾02兾214245-13$15.00兾0 © 2002 Optical Society of America erties of cirrus clouds on their microphysical characteristics. Among those parameters the shape of the ice crystals is one of the most difficult to study because of its temporal and spatial variability. Owing to the high altitude of such clouds, the complexity of in situ measurements makes them casual sources of information. To extend the coverage of shape retrieval, spaceborne observations have been developed: Baran et al.12 used dual-view along-track scanning radiometer 共ATSR兲 observations, Baum et al.13 or Rolland and Liou14 studied the potentiality of the moderate-resolution imaging spectrometer 共MODIS兲, and Chepfer et al.15 used the polarization and directionality of the Earth’s reflectance 共POLDER-1兲 polarization capability. Other methods must be investigated to complete the existing studies. Owing to its sensitivity to optically thin clouds, the lidar is one of the instruments most suited for retrieving cirrus properties.16 Lidars are active remotesensing devices, also referred to as laser radars. They combine a laser that sends a laser beam vertically through the atmosphere and a telescope that collects light backscattered by atmospheric components. By measuring the time elapsing between emission of the beam and reception of the signal by the telescope, the altitude of the backscattering event can be retrieved. Lidars give information on geometric properties of clouds, such as cloud thickness and altitude, as well as optical properties 共e.g., optical thickness兲. They also provide a vertical distribution 20 July 2002 兾 Vol. 41, No. 21 兾 APPLIED OPTICS 4245 of several parameters, such as the backscattering coefficient  共km⫺1 sr⫺1兲 or the extinction coefficient ␣ 共m⫺1兲.17 If the emitted light is linearly polarized in a plane referred to as the parallel plane, separating backscattered light intensity between the two polarization planes 共储 and ⬜兲 provides the depolarization ratio ⌬P: ⌬P ⫽ I⬜ , I储 (1) where I⬜ is the light backscattered in the perpendicular plane and I储 is the light backscattered in the parallel plane. The depolarization ratio is strongly dependent on the particle shape: Spherical particles lead to ⌬P ⫽ 0, whereas irregularly shaped ice particles can show values to as great as 0.6.18 As a consequence the lidar depolarization ratio can be regarded as an indicator of microphysical shape19 as well as a potential cloud-classification method. In most lidar analyses single scattering is assumed, that is, light is being scattered only once between its emission and its reception by the telescope. However, this is clearly not the case in atmospheric scattering because light can be scattered several times in the near-forward direction before it returns to the detector; this phenomenon is called multiple scattering. The importance of multiple scattering has been shown in the scattering of clouds20,21 and even more in spaceborne measurements,22,23 owing to the large volume of the receiver cone. Several studies have tried to provide an empirical global factor that corrects this effect.24,25 However, strong disparities remain among all the studies.26 To quantify the information that can be retrieved from the depolarization ratio and estimate its usefulness for spaceborne measurements, a ray-tracing code for simulating lidar measurements has been developed, taking into account multiple scattering. In this paper we present this simulation and the resulting classification of particle shapes in clouds. A selection of atmospheric settings 共clouds composition and geometry兲 and lidar configurations 共ground-based and spaceborne兲 is in Section 2. The ray-tracing code itself is presented in Section 3. Results of simulations are presented in Section 4 along with the application to 15 lidar cases collected at the ground measurement site at Palaiseau, France 关Site Instrumental Régional de Télédection Atmosphérique 共SIRTA兲兴. Finally, results are analyzed in Section 5. 2. Simulation Parameters A. Lidar Parameters In this simulation the lidar laser and telescope are both located at the origin of the coordinates. The laser has an infinitely small beamwidth, and the telescope has a field of view of FOV. Both can optionally bear the same deviation angle 0 from the vertical. Real-life lidar systems are simulated by an appropriate choice of parameters 共Table 1兲: Ground-based lidar settings are similar to the ground lidar operat4246 APPLIED OPTICS 兾 Vol. 41, No. 21 兾 20 July 2002 Table 1. Lidar Settingsa Set FOV 共mrad兲 ⌬Z 共km兲 0 共°兲 Ground-based Calipso 3.0 0.125 8.0 695.0 0° 0° a FOV, field of view; ⌬Z, range to cloud layers; 0, angle with vertical direction. ing at SIRTA 共Subsection 4.B兲, and the spaceborne settings are similar to the future Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observations lidar program27 共in the absence of a fixed value for the incidence angle, which has been taken as 0 ⫽ 0°兲. B. Atmosphere Definition The atmosphere is modeled with horizontal infinite layers, each with its own geometrical parameters 共altitude and thickness兲 and microphysical parameters 共optical depth and crystal scattering properties兲. To each layer can be assigned a free number of scatterers that modify the photon path and determine the amount of light scattered back to the detector. Scatterers can be either water droplets, atmospheric molecules, or ice crystals. Because cirrus clouds are mostly made of ice crystals, we are focusing on such crystals. They can be found in an almost infinite variety of shapes and sizes.28,29 However, since covering the full range of crystal shapes is beyond the scope of this paper and since water crystallizes naturally in a hexagonal shape, a model of hexagonally based shapes was chosen. Even if it is a fairly simple approximation, several studies show that these kinds of crystals are often found in cirrus clouds.30 They are defined by their shape ratio Q ⫽ l兾共2r兲, where l is the crystal length and r is its base radius. By browsing Q values from 0.05 to 5, we can represent ice plates and columns. Molecular scattering was approximated by adding spherical scatterers with concentrations as defined by Valley.31 A set of physical properties, noted p, is assigned to each scatterer: p 共km⫺1兲 is the photon mean free path, depending on the considered particle concentration and optical depth. It defines how often a photon will interact with particle p 共Section 3兲. • Mp共⌰兲 is the particle-scattering matrix.32 This matrix gives the Stokes vector of any light beam scattered by the particle p in direction ⌰. Computation of this matrix is a separate process that has already been addressed thoroughly.33–36 For this paper a separate specific ray-tracing code taking polarization effects into account has been internally developed, allowing computations of Mp for a wide range of particle-shape ratios. This code is based on Scattering Matrix for Oriented Crystals with optimization for the backscattering angle.37 • Cpd, CpD, and Cp␦ 共m2兲, particle cross sections for each possible interaction 共angular scattering, diffraction, and ␦-function transmission, respectively, • Table 2. Atmosphere Definitionsa Set Layers Q ␦ 1 2 3 4 5 1 1 1 2 1 0.05 1.00 2.50 0.05, 1.00 0.05, 1.00 1.0 1.0 1.0 1.0 2.0 a Q, shape factors of scatterers inside the layers; ␦, layer optical depths. Section 3兲. These cross sections are obtained as a side result of the scattering matrix computation. 3. Description of the Ray-Tracing Process The simulation begins with the emission of a single light beam into a modeled atmosphere 共Subsection 2.B兲 with an optional deviation angle 0 共Subsection 2.A兲. An associated Stokes vector I0 ⫽ 关I Q U V兴 holds all the information on beam intensity and polarization. The path and the Stokes vector of the light beam are then modified by successive interactions with atmospheric components. The probability of interaction after a progression of length l is given by P共l 兲 ⫽ exp共⫺l 兲dl, where is the mean free path of the current atmospheric layer 共Subsection 2.B兲. When the light beam encounters a particle p, an interaction is selected among angular scattering, diffraction, or ␦-function transmission, based on a random probability weighted by the relevant cross sections Cpd, CpD, and Cp␦ 共Subsection 2.B兲. In the case of angular scattering, the Stokes vector Is of the transformed beam is obtained through the scattering matrix Mp of the encountered scatterer: Is ⫽ Mp共兲 䡠 I0, where is the angle between the incoming and the transmitted beams. If diffraction occurs, the transformed beam is given by Fraunhofer formulas.38 Finally, light beams undergoing ␦-function transmission36 are regarded as not scattered at all. Eventually, some of the scattered light has to return to the detector. As in ray-tracing simulations this is an unlikely event; a technique is used in which each scattering event contributes to the recorded light. When a light beam is scattered by a particle p inside the detector field of view, no matter what direction it is following next, it contributes to detected light as the Stokes vector Ir ⫽ Mp共⌰兲 䡠 I0, where ⌰ is the angle between the incoming light beam direction and the return path to the detector. Once this contribution is recorded, the light beam follows its own course in a new direction. 4. Results A. Theoretical Analysis Simulations were conducted for both ground-based and space-based lidar configurations 共Table 1兲 and atmospheric parameters as defined in Table 2. Fig. 1. Simulated profiles for ground-based lidar: A, backscattered radiance in the parallel plane; B, backscattered radiance in normal plane; C, depolarization ratio; D, ratio between radiances in multiple and single scattering, in the parallel plane. 20 July 2002 兾 Vol. 41, No. 21 兾 APPLIED OPTICS 4247 Table 3. Increase in Depolarization Ratio Due to Multiple Scattering Set Ground-Based 共%兲 Spaceborne 共%兲 Increase 共%兲 1 2 3 4 5 ⫹53.8 ⫹16.6 ⫹14.5 ⫹54.0 ⫹56.5 ⫹53.8 ⫹13.75 ⫹12.20 ⫹36.66 ⫹58.11 ⫹0.0 ⫺1.82 0.0 ⫺20.0 ⫹1.75 1. Ground-Based Configuration Results of ground-based lidar simulations are summarized in Fig. 1: 共i兲 backscattered radiances 共Wm⫺2 sr⫺1兲 I储 共Fig. 1A兲 and I⬜ 共Fig. 1B兲, 共ii兲 depolarization ratios ⌬P 共Fig. 1C兲, 共iii兲 the ratio R of multiple-scattering radiance to single-scattering radiance for a parallel plane 共Fig. 1D兲. Singlescattering results are shown by continuous curves and multiple-scattering results by dashed curves. Figure 1 shows an increase in the depolarization ratio with in-cloud penetration depth, owing to increasing multiple scattering. For atmospheric case 1 共unity optical depth and crystals with shape factor Q ⫽ 0.05兲 the depolarization increases by 54% between the cloud base and top, whereas the increase is only 15% for the same cloud composed of columns 共case 3兲. Such coefficients for all atmospheric settings are shown in Table 3. Based on such results, it appears that multiple scattering leads to an increase in the depolarization ratio in most cases, depending on the cloud optical thickness and particle-shape ratio. Besides, the R coefficients increase strongly with in-cloud penetration, showing that the backscattered radiance in a single polarization state seems even more difficult to analyze for remote-sensing applications than the depolarization ratio. To estimate how lidar incidence angle 0 affects the results, scanning lidar measurements were simulated by modifying the incidence angle value from 0° to 45° for atmospheric set 1. Results in Fig. 2 present a very small dependence on incidence angle. For example, in both single and multiple scattering 共Figs. 2A and 2B兲 a small decrease in backscattered radiance can be observed. However, because this effect is mostly due to the increase in cloud range, I⬜ and I储 are equally influenced and the depolarization ratio is not affected 共Fig. 2C兲. However, it shows an increase of 15% on the upper right side of the cloud 共i.e., for higher ranges, Fig. 2D兲 due to the multiplescattering effect. 2. Spaceborne Configuration Results of spaceborne lidar simulations are shown in Fig. 3. They are consistent with ground-based simulations 共Fig. 1兲, except that the cloud is seen from above instead of below. Following the same approach as ground-based sim- Fig. 2. Simulated scanning lidar profiles: A, backscattered radiance for the parallel plane in single scattering; B, backscattered radiance for the parallel plane in multiple scattering; C, depolarization ratio for single scattering; D, depolarization ratio for multiple scattering. 4248 APPLIED OPTICS 兾 Vol. 41, No. 21 兾 20 July 2002 Fig. 3. Same as Fig. 1 but for spaceborne lidar. ulations, the increase in depolarization between the top and the bottom of the cloud is shown in Table 3 along with a comparison with ground-based results. It shows that the multiple-scattering effect is similar: The very narrow field of view of the spaceborne lidar, compared with the ground-based lidar compensates for its greater distance to the clouds 共Table 1兲. As a consequence the depolarization ratio holds the same amount of information for ground-based and spaceborne lidar measurements. We will therefore use ground-based measurements in the rest of the study, keeping in mind that the results will be applicable to spaceborne instruments. 3. Depolarization Ratio Study To compare lidar measurements with theoretical values, simulations were conducted for a ground-based lidar considering a single ice cloud of variable optical thickness. The depolarization ratio ⌬Psim was calculated for shape factor ratios Q ranging from 0.01 to 10 and for a cloud optical thickness ␦ ranging between 0 and 3. The resulting function, ⌬Psim ⫽ f 共Q, ␦兲, is shown in Fig. 4. The global shape of this curve is consistent with the results of Del Guasta.39 Higher depolarization ratios are associated with higher shape ratios 共columns兲 and low depolarization ratios with lower shape ratios 共plates兲. The increase in optical thickness leads to a steady increase in the depolarization ratio, which is more important for low shape ratios. Figure 4 shows that for a Q smaller than 0.05 and Q between 0.7 and 1.05, Q and ⌬P can be linked by a bijective relationship for any given value of optical depth. On the contrary, for Q between and 0.05 and 0.7 and Q greater than 1.05, several shape ratios can lead to the same depolarization ratio. Based on these statements, four classes of shape ratios were chosen: 共Q ⬍ 0.05兲, 共0.05 ⬍ Q ⬍ 0.7兲, 共0.7 ⬍ Q ⬍ 1.05兲, and 共Q ⬎ 1.05兲, noted as classes I, II, III, and IV in Fig. 4. It appears that there is a global increase in the depolarization ratio while the optical depth increases, although the class boundaries stay constant. Using Fig. 4 for a given value of cloud optical thickness, we can select a shape ratio class based on a depolarization measurement. This technique will be applied in Subsection 4.B to lidar measurements of the depolarization ratio, each vertical profile being independently processed to retrieve a value of optical thickness.20 B. Application to Experimental Measurements In this section the lidar simulation presented in Section 4 is used to derive an estimate of the ice crystal shape ratio from lidar depolarization ratio observations. The lidar data were taken by the Nd:YAG lidar located on SIRTA. The laser source, operating at a 0.532-m wavelength, is polarized in the parallel plane. Clouds limits were detected by setting a signal threshold for each lidar profile, and the depolar20 July 2002 兾 Vol. 41, No. 21 兾 APPLIED OPTICS 4249 Fig. 4. Evolution of the depolarization ratio ⌬P as a function of the shape ratio Q and the cloud optical thickness ␦ for single and multiple scattering. ization ratio ⌬Pex was defined as ⌬Pex ⫽ 共I⬜兾I储兲 共Section 1兲. This ratio was normalized to the molecular depolarization ratio 关2.79% Ref. 共40兲兲兴 in a region free of clouds and aerosols. Fifteen experimental cases were selected between 27 April 1999 and 5 December 1999, representing roughly 127 h of data. For each case, lidar profiles are averaged over 1 min, and the vertical resolution is 15 m. The characteristics of each case, including altitude, average temperature, and its standard deviation, are presented in Table 4. Temperatures were provided by radiosoundings launched at Trappes meteorological station 共15 km from Palaiseau兲. The optical depth was calculated profilewise, but as an indication the average and maximum values are provided. Table 4. Presentation of Lidar Experimental Casesa Date Time Tav Tstd zmin zmax ␦av ␦max I 共%兲 II 共%兲 III 共%兲 IV 共%兲 19990427 19990503 19990510 19990513 19990514 19990519 19990521 19990601 19990618 19991015 19991018 19991112 19991128 19991129 19991205 1195–1328 0900–1081 1115–1341 0791–1223 0828–0966 0843–1028 1210–1436 0953–1098 1273–1673 0838–1293 0715–1170 0748–1588 1125–1639 0740–1348 1751–2191 ⫺46.46 ⫺50.01 ⫺32.00 ⫺44.34 ⫺31.78 ⫺39.96 ⫺51.91 ⫺35.38 ⫺54.46 ⫺42.99 ⫺47.09 ⫺42.20 ⫺49.96 ⫺50.45 ⫺51.11 4.39 5.14 12.09 7.61 5.65 4.32 2.46 10.38 4.18 7.07 5.46 2.06 16.43 10.28 8.09 7.49 6.90 5.50 5.10 4.99 6.49 8.30 4.50 9.51 7.20 7.71 5.80 5.50 7.11 3.70 10.51 11.99 11.01 11.50 10.00 9.21 11.79 11.01 12.70 11.61 11.50 9.51 13.30 13.49 13.49 0.10 0.40 0.16 0.11 0.26 0.01 0.05 0.40 0.14 0.50 0.09 0.11 0.39 0.49 0.29 0.61 2.42 2.55 4.63 1.58 1.55 1.03 3.11 2.42 2.71 0.33 1.98 1.72 3.05 4.06 19.02 35.62 21.00 23.53 37.66 27.20 69.11 34.68 30.23 23.73 20.62 36.47 11.78 7.74 7.02 79.02 47.95 36.43 59.21 41.19 56.50 25.30 41.53 33.64 34.76 39.22 30.83 34.17 19.17 19.85 1.95 13.53 39.18 11.98 14.68 8.34 5.51 13.43 13.09 32.46 36.34 23.22 46.95 57.46 41.95 0.00 2.90 3.38 5.28 6.48 7.96 0.08 10.36 23.05 9.05 3.82 9.48 7.10 15.62 31.18 a Tav, average temperature; Tstd 共°C兲, its standard deviation; zmin, zmax 共km兲, cloud altitude boundaries; ␦av, average optical depth; ␦max, maximum optical depth, percentages of retrieved classes. 4250 APPLIED OPTICS 兾 Vol. 41, No. 21 兾 20 July 2002 Fig. 5. Experimental depolarization ratios for 5 December 1999 case. 1. 5 December 1999 Case As an example the evolution of experimental depolarization ratios as a function of time and altitude for 5 December 1999 are shown in Fig. 5. This case features a rather inhomogeneous cloud evolving from a 11-km altitude at 1800 UTC down to a 6-km altitude at 2400 UTC. This cloud shows a strong depolarization 共to as high as 0.6兲. Temperature and relative humidity profiles from radiosoundings launched at 1121 UTC are shown in Fig. 6. The Fig. 6. Temperature and humidity profiles collected at 1121 UTC. 20 July 2002 兾 Vol. 41, No. 21 兾 APPLIED OPTICS 4251 Fig. 7. Retrieved shape ratios separated in four classes from, light gray, Class I 共Q ⬍ 0.05兲, to, black, Class IV 共Q ⬎ 1.05兲. cloud temperature ranges between ⫺60 and ⫺35 °C, and the relative humidity is below 20%. The crystal shape ratio was retrieved by the classification technique presented in Subsection 4.A.3: The cloud optical depth was calculated for each lidar profile with a maximum uncertainty of ⫾0.1. Based on this value, a specific curve ⌬Psim ⫽ f 共Q, ␦兲 was selected on which the measured depolarization ratios ⌬Pex were reported. The retrieved shape ratio classes are shown in Fig. 7. The higher and colder cloud layer, between 10 and 12 km, shows a majority of shape ratios greater than 1.05 共Class IV兲. The lower cloud layer 共after 2300 UTC兲 shows a global decrease in the shape ratio that could be explained by both platelike shapes 共Q ⬍ 0.05兲 or mixed-phase crystals leading to increased sphericity and a lower average depolarization ratio in the probed cloud volume. Fig. 8. Same as Fig. 5 but for 28 November 1999. 4252 APPLIED OPTICS 兾 Vol. 41, No. 21 兾 20 July 2002 Fig. 9. Same as Fig. 6 but for 28 November 1999. 2. 28 November 1999 Case As a second example, the evolution of experimental depolarization ratios as a function of time and altitude for 28 November 1999 are shown in Fig. 8. This case features two continuous layers, one be- tween 6.5 and 8 km and another between 11 and 13 km, from 1100 to 1630 UTC. The upper layer shows strong depolarization patches, whereas the lower layer shows a wider range of depolarization values. Temperature and relative-humidity profiles are Fig. 10. Same as Fig. 7 but for 28 November 1999. 20 July 2002 兾 Vol. 41, No. 21 兾 APPLIED OPTICS 4253 shows patches of high shape ratios surrounded by low shape ratios 共Classes I and II兲. Again, this low shape ratio can be interpreted as either plates or mixed-phased crystals. Owing to the relatively high temperature of the lower layer, the mixed-phased hypothesis can be considered as the most probable. Fig. 11. Frequency of occurrence of the different effective shape classes for the 15 cases that were studied. shown in Fig. 9. For the upper layer the temperature ranges between ⫺60 and ⫺72 °C with a relative humidity of ⬃25%. For the lower one the cloud temperature ranges between ⫺35 and ⫺25 °C with a relative humidity between 25% and 55%. The retrieved shape ratios are shown in Fig. 10. The upper layer shows broken patches of high shape ratios 共Classes III and IV兲, whereas the lower layer 3. Summary of Retrievals The 15 selected cases have been processed in the same way, and a histogram of the classes of retrieved shape ratios for all cases is shown in Fig. 11. Class percentages for single cases are presented in Table 4. The upper limit for the last class has been taken as Q ⫽ 4, since almost all retrieved shape ratios are found below that value. It shows that most particle ratios can be found in Class III, that is, Q between 0.7 and 1.05 共⬃35%兲, with another peak for Class II, that is, Q between 0.05 and 0.7 共⬃32%兲. Note that these results are significant only for the mid-latitude thin cirrus cases that were studied and not applicable to all cirrus clouds. Besides, histograms of temperatures for each shape-ratio class are presented in Fig. 12, assuming that the temperature profiles stay constant during the observation. These charts show a global shift of dominant temperatures from one class ⬃ ⫺40 °C兲 for to another, from a high temperature 共T ⬃ low shape ratios 共Q ⬍ 0.05兲 to low temperatures 共T ⫺60 °C兲 for the highest shape ratios 共Q ⬎ 1.5兲. Fig. 12. Temperature histograms for each class of a shape ratio. 4254 APPLIED OPTICS 兾 Vol. 41, No. 21 兾 20 July 2002 5. Analysis When the presented results are considered, several shortcomings that could lead to bias in the results should be stressed: • The retrieval technique implies that clouds are made exclusively of pure hexagonal-based ice crystals. Occurrences of mixed-phase clouds containing water under ice and the liquid phase could lead to biased results: Near-spherical shapes lead to a low depolarization ratio and are wrongly counted as plate crystals 共i.e., low shape ratios兲. However, only the first shape ratio class is affected by this phenomenon, and its importance can be limited by a careful selec ⬍ 40°兲. tion of unambiguous cases 共T • However, in its current state the simulation focuses on hexagonal-based particle shapes. Using more complex shapes is possible, leading to potentially different depolarization ratios as long as the particle-scattering matrix Mp is known 共Subsection 2.B兲. Calculation of these matrices for a wide variety of ice crystals has been thoroughly addressed.41 • Moreover, ray-tracing by design cannot take into account particle size, where as studies42,43 have shown that the presence of small particles 共with an effective radius r ⬍ 6 m兲 could lead to strong depolarization ratios 共⌬P ⬎ 0.7兲.44 This size effect cannot be accounted for with ray-tracing models, but, since such high values were not noticed in current measurements, this phenomenon should not apply here. • Finally, until now all calculations were conducted for randomly-oriented particles. The next logical step would be to implement an anisotropic media 共i.e., particles with a preferential plane of orientation兲,45,46 which could potentially lead to higher values of ⌬Psim for low shape ratios.47 However, recent papers48,49 show that an efficient study of anisotropic media would require multiple incidence-angle measurements, which are seldomly available at this point. Furthermore spaceborne lidar measurements of this kind will not be available in the near future. 6. Conclusions We have presented a technique for retrieving information on particle shapes in ice clouds, taking advantage of the strong sensitivity of light polarization to microphysical properties. The potential application to this technique to spaceborne lidar measurements has been studied. A ray-tracing simulation of lidar backscattering and depolarization profiles has been developed, taking into account multiple scattering. Several atmospheric models were processed with different cloud microphysical and optical settings from either a ground-based or a spaceborne point of view. Lidar simulations show that the multiple-scattering effect, although strongly dependent on particle shape and optical depth, stays in the same range for either ground-based or spaceborne lidar, owing to the very narrow field of view of the spaceborne configuration. Simulated depolariza- tion ratios were used to retrieve effective shape ratios from experimental depolarization ratios. The 15 cases of lidar observations for mid-latitude cirrus clouds were studied to separate the effective shape ratios into four different classes. Results show a majority of near-unity shape ratios on average for the cases that were studied. Moreover the proportion of low temperatures is higher for high effective shape ratios 共Subsection 4.B.3兲. A comparison of such results with previous studies is difficult for the following reasons: 共i兲 The number of existing studies of particle shapes in ice clouds is very limited for the time being. 共ii兲 Passive satellite retrievals are integrated from the cloud top over a variable penetration depth, depending on the type of measurement 共wavelength, viewing direction, etc.兲, whereas the lidar provides information on the vertical distribution. 共iii兲 The existing studies do not cover seasonal variation at mid-latitude areas such as the Palaiseau ground site. Nevertheless an analysis of ATSR dual-view observations collected above tropical cirrus clouds12 led to the conclusion that near the top of such clouds, columns 共high shape ratios兲 and polycrystals are more frequent. Moreover the POLDER-1 analysis,15 in which bidirectional polarized observations were used showed that columns and polycrystals are dominant at the cloud top for mid-latitude cirrus clouds. Those results are consistent with the current study, since the higher colder particles show higher shape ratios. Note that these results could be biased owing to several assumptions that are described in detail in Section 5: 共i兲 monodisperse size distribution, 共ii兲 hexagonal particle shape, 共iii兲 randomly oriented particles. However, in the absence of large-scale climatological studies of shape factor, this retrieval method could be applied on already operational ground-based lidar measurements. Since a great number of cirrus cases are available through the globe, this method could lead to potential preliminary statistical studies of the effective shape ratios of cirrus clouds and their vertical variability. As an example, in the first step the whole cirrus lidar database of SIRTA could be used to estimate the representation of the effective shapes in cirrus clouds in northern France. In addition, the application of this retrieval method to spaceborne lidar measurements could lead to studies of shape factors at the global scale. This could allow cirrus clouds of different latitudes to be discriminated. Coupled with the vertical variability allowed by lidar measurements, several aspects of crystal shape evolution and cloud formation processes could be studied. The authors thank the Centre National d’Etudes Spatiales and the Sodern Company for financial support. Thanks are extended to Laurent Sauvage for providing the data acquisition. The authors are grateful to the anonymous reviewer for useful comments. The authors would like to thank SIRTA for providing the lidar data. 20 July 2002 兾 Vol. 41, No. 21 兾 APPLIED OPTICS 4255 References 1. K. N. Liou, “Influence of cirrus clouds on weather and climate processes: a global perspective,” J. Geophys. Res. 103, 1799 – 1805 共1986兲. 2. D. P. Wylie, W. P. Menzel, H. M. Woolf, and K. L. 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