Bull Volcanol DOI 10.1007/s00445-010-0393-4 RESEARCH ARTICLE Volcanic lightning: global observations and constraints on source mechanisms Stephen R. McNutt & Earle R. Williams Received: 2 June 2008 / Accepted: 4 June 2010 # Springer-Verlag 2010 Abstract Lightning and electrification at volcanoes are important because they represent a hazard in their own right, they are a component of the global electrical circuit, and because they contribute to ash particle aggregation and modification within ash plumes. The role of water substance (water in all forms) in particular has not been well studied. Here data are presented from a comprehensive global database of volcanic lightning. Lightning has been documented at 80 volcanoes in association with 212 eruptions. The Volcanic Explosivity Index (VEI) could be determined for 177 eruptions. Eight percent of VEI=3–5 eruptions have reported lightning, and 10% of VEI=6, but less than 2% of those with VEI=1–2. These findings suggest consistent reporting for larger eruptions but either less lightning or possible under-reporting for small eruptions. Ash plume heights (142 observations) show a bimodal distribution with main peaks at 7–12 km and 1– 4 km. The former are similar to heights of typical thunderstorms and suggest involvement of water substance, whereas the latter suggest other factors contributing to electrical behavior closer to the vent. Reporting of lightning is more common at night (56%) and less common in daylight (44%). Reporting also varied substantially from year to year, suggesting that a more systematic observational strategy is needed. Several weak trends in lightning occurrence based on magma composition were found. The bimodal ash plume heights are obvious only for andesite to dacite; basalt and basaltic-andesite evenly span the range of heights; and rhyolites are poorly represented. The distributions of the latitudes of volcanoes with lightning and eruptions with lightning roughly mimic the distribution of all volcanoes, which is generally flat with latitude. Meteorological lightning, on the other hand, is common in the tropics and decreases markedly with increasing latitude as the ability of the atmosphere to hold water decreases poleward. This finding supports the idea that if lightning in large (deep) eruptions depends on water substance, then the origin of the water is primarily magma and not entrainment from the surrounding atmosphere. Seasonal effects show that more eruptions with lightning were reported in winter (bounded by the respective autumnal and vernal equinoxes) than in summer. This result also runs counter to the expectations based on entrainment of local water vapor. Editorial responsibility: JC Phillips Keywords Volcanoes . Lightning . Electrification . Ash plumes . Water Electronic supplementary material The online version of this article (doi:10.1007/s00445-010-0393-4) contains supplementary material, which is available to authorized users. S. R. McNutt (*) Geophysical Institute, University of Alaska Fairbanks, 903 Koyukuk Drive, P.O. Box 757320, Fairbanks, AK 99775, USA e-mail: [email protected] E. R. Williams Massachusetts Institute of Technology 48-211, Parsons Laboratory, Cambridge, MA 02139, USA Introduction Electrical discharge in volcanic eruptions (i.e., volcanic lightning) is fairly common yet relatively understudied. Lightning is reported at only a few of the 55–70 volcanoes that erupt each year (Simkin 1993), so it appears that either there are systematic problems with reporting, or some special set of circumstances must prevail to favor the Bull Volcanol production of lightning, or both. Lightning and electrification at volcanoes are important because they represent a hazard in their own right (people were killed by volcanic lightning at Paricutin and Rabaul; see McNutt and Davis 2000, p. 45–47), they are a component of the global electrical circuit, and because they contribute to ash particle aggregation and modification within ash columns (Lane and Gilbert 1992; Gilbert and Lane 1994a, b; James et al. 2003; Textor et al. 2005a, b; Mather and Harrison 2006; James et al. 2008). Conventional thinking has been that interactions between dry silicate ash particles, such as collisions and fractures, have been dominant processes causing electrification, while the role of water is secondary. This is in contrast to early studies of Surtsey, Iceland, in which seawater played a prominent role (Blanchard 1964; Anderson et al. 1965; Blanchard and Björnsson 1967). Further, the existence and role of ice particles in ash plumes, now recognized as a fundamental aspect of thundercloud electrification, has been noted in only a few studies at volcanoes (e.g. Thorarinsson 1966; Rose et al. 1995a, b, 2000; Hoblitt 2000; Thompson 2000). In this report, the expansion of steam and its subsequent condensation and freezing are emphasized as primary processes whose magnitude and effects have been understudied with respect to volcanic lightning. Despite the frequent occurrence of volcanic lightning, and many spectacular photographs, only two systematic compilations of basic lightning facts have been published (McNutt and Davis 2000; Mather and Harrison 2006). Here we present results of a more comprehensive literature search on the occurrence of volcanic lightning and attempt to summarize the effects of observed parameters such as height of plume, volume of tephra and gases (mainly water vapor), and magma composition. We also discuss reporting parameters because these affect the historical record of lightning occurrence. Few instrumental studies of volcanic lightning have been undertaken (Hoblitt 1994; McNutt and Davis 2000; Paskievitch et al. 1995; Thomas et al. 2007, 2010), but this study is complementary to all of them. Accordingly, some recommendations are included regarding desirable electrical studies that will be necessarily aimed at constraining mechanisms for volcanic lightning. Data and methods The main information source for this study is a comprehensive literature compilation that was carried out over a period of about 10 years. A standard bibliography keyword search yielded only a handful of studies, so instead the literature was searched systematically, colleagues were polled, photographs were collected, and information from newspapers and other sources, such as poster displays and videos, was also compiled. The bulk of this work was completed before modern computer search engines, such as Google™, were in common use. Key references included the Bulletin of Volcanology, the Journal of Volcanology and Geothermal Research, the Smithsonian Institution’s Scientific Event Alert Network and Global Volcanism Network Bulletins, and the books by McClelland et al. (1989), Taylor (1958), and Newhall and Punongbayan (1996), amongst others. We note that books published after about 1984 had better indexes than older works, probably a result of the increased use of electronic word processing and the ease of making searches by keywords. Information that was collected included the name of the volcano, the date (and time, where noted), the Volcanic Explosivity Index (VEI; Newhall and Self 1982; Simkin and Siebert 1994) of the eruption, the plume height maximum, the magma composition, whether it was day or night, any significant ancillary observations, and references (Appendix). Latitudes and longitudes for volcanoes are available from Volcanoes of the World (Simkin and Siebert 1994). VEI values were generally taken from Simkin and Siebert (1994) after checking that the date of the lightning observations coincided with the date of an eruption that was assigned a VEI. We also estimated many VEI values ourselves based mainly on reports of tephra volumes and plume heights. Analyses and results Reporting problems We first discuss reporting problems because these must be understood before other features of the data can be interpreted. Considerations of the detectability of volcanic lightning over the full range of sunlight conditions must be determined. Of the 131 eruptions for which the time of day was known, we found that 44% occurred during daylight hours and 56% at night (Appendix). This suggests that lightning is more easily seen against a dark background and may be missed during bright daytime conditions. As a specific example of this effect, the eruption of Mount Spurr, Alaska, on September 17, 1992, occurred at night and had dramatic displays of lightning readily noted by people on the ground. However, the amount of lightning for this eruption (7 flashes recorded instrumentally) was nearly an order of magnitude less than for the other two 1992 eruptions (61 and 57 flashes, also recorded instrumentally), which were of similar size but occurred during the day, when ground observations of lightning were lacking (McNutt and Davis 2000). All three Spurr eruptions used the same instrumental data to determine the number of flashes; details are given in McNutt and Davis (2000). Bull Volcanol An additional reporting problem with regard to daytime observations has to do with the fact that many volcanoes are located in tropical areas where lightning is common from thunderstorms. Thus volcanic lightning may not be noticed if an observer is not aware of an eruption, because the lightning would be dismissed as being due to normal weather patterns. Conversely, thunderstorm lightning that happens to occur near an erupting volcano might be associated with the eruption even if it is not caused by the eruption, depending on the interpretation of the observer. For some regions, such as the Alaska/Aleutian arc, lightning is not common (J. Painter, National Weather Service, pers. comm., 1997; D. Dissing, pers. comm., 2003). During a rare thunderstorm near Augustine Volcano in 1998, several local citizens called the Alaska Volcano Observatory to ask if Augustine was erupting, because they remembered that the 1976 and 1986 eruptions had been accompanied by vigorous lightning (Kienle and Swanson 1985; J. Kienle pers. comm. 1992). The volcano was not erupting at the time of the 1998 thunderstorm. In contrast, Augustine’s 2006 eruptions were accompanied by abundant lightning (Thomas et al. 2007, 2010). We determined the number of eruptions with reported lightning versus year (Table 1). Considerable variation is noted, with values ranging from 0 to 19. The peak year was 1979. Given that between 55 and 70 volcanoes erupt per year (Simkin and Siebert 1994) this suggests that up to 27– 35% of erupting volcanoes can produce lightning. Another way to view this is that volcanic lightning is generally under-reported. It is not clear why the reporting varies so much from year to year. There is a rough tendency for the number of reports to be higher following famous eruptions. For example, 1951 is the only year from 1950 to 1978 to have more than 10 eruptions reported with lightning. Ten of 11 reports were from Lamington volcano, which had a large explosive eruption that year. In other years with high numbers of cases generally one volcano contributed most of the cases. The large number of reports for 1979 (19) includes many reports for Aso and Sakurajima; apparently some sort of systematic study of lightning/electrical activity was under way in Japan. Lightning occurrence and volcanic explosivity index We found that lightning has occurred in association with 212 eruptions at 80 volcanoes (Appendix). These are significantly higher numbers than the 55 volcanoes cited in McNutt and Davis (2000) or 58 cited in Mather and Harrison (2006) and reflect our additional work since then. VEI values were known or could be estimated for 177 eruptions, and a histogram of these events is shown in Fig. 1 (bottom). Note that heights are estimated above the vent for eruptions with VEI=2 and smaller, but above sea level for eruptions with VEI=3 and larger following the standard conventions (Simkin and Siebert 1994). For comparison, a histogram of all known VEI is shown in Fig. 1 (top). There are many more small eruptions than large ones, so the numbers increase from right to left. The drop off for VEI=1 is likely due to under reporting (Simkin and Siebert 1994). The number of occurrences of volcanic lightning at various VEI values is also shown in Table 2 along with all known VEI and percent of cases showing lightning versus all VEI. The percent of eruptions with lightning is nearly the same for VEI=3, 4, and 5. This suggests a standard reporting efficiency. The percentage of VEI=6 eruptions is somewhat higher. Such large eruptions attract attention and are generally well reported. We also note the common observation that large eruptions create local darkness because of the dense ash plumes, a condition under which lightning can be more easily seen. Further, the heights of the ash plumes are >15 km for this range of VEI, so these are taller than most thunderclouds (also referred to as deep convection by atmospheric scientists) and we infer that similar water based charge generation or separation mechanisms may be acting (see Discussion section below). The percentage of eruptions with recorded lightning with VEI=2 and smaller drops off sharply. This behavior suggests either a systematic reporting problem, or that lightning is simply less common in these smaller eruptions, or both. Bimodality of eruption plume heights Eruptions with VEI=3 have ash plume heights of 3–15 km (Simkin and Siebert 1994); these straddle typical thunderstorm heights, and we find many cases with lightning and also many without. For VEI=1 and 2 eruptions there are relatively fewer cases, but these are important because the ash plume heights are <5 km, less than summertime thunderclouds (tops at 7 to 20 km a.s.l.; Byers and Braham 1949; Williams 1985), and they suggest that some other lightning producing mechanisms may be acting. A histogram of ash plume heights is shown in Fig. 2a for the 142 cases for which we have data. The histogram shows a bimodal distribution with one peak in the range of 7 to 12 km and another peak in the range of 1 to 4 km. The higher altitude peak represents the typical heights of ordinary thunderstorms. The low altitude peak, however, is significantly lower than thunderstorm values. No comprehensive or extensive compilation of plume heights is known to us, based on numerous searches and discussions with colleagues. We expect plume heights, which are a component of VEI, to have a similar distribution to the VEI data in Fig. 1 (top). Restated, a histogram of all plume heights would be expected to have Bull Volcanol Table 1 Number of eruptions with lightning per year Prior to 1960 only years with eruptions are listed Prior to 1900, the year 1707 is the only year with more than one report of lightning Year No. Eruptions Year 2009 2008 2007 2006 2005 2004 2003 2002 2001 2000 1999 1998 1997 1996 1995 6 6 2 15 13 5 0 0 0 3 1 1 1 3 2 1972 1971 1970 1969 1968 1967 1966 1965 1964 1963 1962 1961 1960 0 1 0 0 2 0 1956 1 1994 1993 1992 1991 1990 1989 1988 1987 1986 1985 1984 1983 1982 1981 1980 1979 1978 1977 2 1 4 9 12 1 2 1 4 1 1 1 13 2 3 19 7 1 1953 1952 1951 1950 1949 1948 1947 1946 1945 1944 1943 1937 1933 1931 1929 1924 1914 1912 1 1 11 1 1 1 1 1 1 2 1 1 1 1 1 1 2 1 1976 1975 1974 1973 5 1 1 2 1911 1906 1902 1 1 3 1707 2 Augustine (14) Colima (11) Redoubt (12) Galunggung (6) Aso (7), Sakurajima (8) smoothly increasing numbers moving to smaller heights. Because no compilation exists, we created a synthetic distribution of heights as follows. We used VEI data to generate a plot of number of plumes at each km of altitude by assuming all heights for a given VEI were at the midpoint of the altitude range. For example, the height range for VEI=2 is 1–5 km so we assumed 3 km as the mean height. For VEI=5 we used 25 km and for VEI=6 we used 31 km. We then computed a linear regression for the VEI values from 2 to 6 (heights of 3 to 31 km) and used the No. Eruptions 1 2 1 1 0 0 Lamington (10) linear relation to estimate the number of plume heights for each km. Data were then renormalized so the total number of eruptions was the same as the starting values. This procedure gives us estimates of the total number of eruptions for each km of plume height. We then can plot the number of eruption plumes with lightning for each height as a percentage of all eruptions, as shown in Fig. 2b. Here we observe that all the values for heights of 1–6 km are 0.3% or less (mean 0.018%), whereas those between 7 and 13 km are 0.3% or greater (mean 0.07%). This Bull Volcanol Fig. 1 Histogram of Volcanic Explosivity Index (VEI) for all eruptions in Volcanoes of the World, by Simkin and Siebert, 1994 (a) and for eruptions accompanied by lightning (b) using data from the Appendix. Note that the eruptions accompanied by lightning are skewed towards higher VEI values. The plume heights for VEI 3 and larger are similar to the heights of thunderclouds difference of more than a factor of 3 suggests that eruptions with ash plume heights of 7 to 13 km, the same range as thunderstorms, are more efficient at producing lightning than smaller eruptions. Additional reasons for this systematic difference are given in the discussion section. Recent instrumental data from Augustine volcano in Alaska may also shed some light on this issue. The eruption on January 28, 2006 at 05:31 UT had an ash plume 10.5 km high (a.s.l.), similar to thunderstorms. It had abundant lightning in the plume, with over 300 lightning flashes starting about 5 min after the onset of the main phase of the eruption (Thomas et al. 2007, 2010). Most of these events were intracloud flashes with durations of 30–600 ms, typical of values for thunderstorms. Measurements of duration were made using Lightning Mapping Array (LMA) data (Thomas et al. 2004). In contrast, a smaller eruption at 08:37 UT January 28 had an ash plume only Table 2 Number and percent of occurrences of volcanic lightning at various VEI values VEI 1 2 3 4 5 6 7 8 No. cases with Lightning No. cases all eruptions 7 61 81 22 7 4 0 0 845 3477 869 278 84 39 4 0 percent 0.83 1.75 9.32 7.91 8.33 10.26 0.00 – 3.8 km high and this was accompanied by only a single lightning flash. The latter flash showed a duration of about 10 ms, substantially shorter than typical thunderstorm lightning (Thomas et al. 2010). Thus the available instrumental data, although sparse, do suggest a systematic difference in lightning between large plumes and small ones. The study of photographs of volcanic lightning also supports a systematic difference. Photos of small plumes (1–3 km), typically time exposures, show lightning with few branches and typical lengths of a few tens to hundreds of meters (e.g. National Geographic Sept. 2007, p. 14–15). Some photos from larger eruptions, on the other hand, show lightning with many branches and lengths of several km (e.g. Galunggung; Katili and Sudrajat 1984). We note that the dozen or so photos we examined are suggestive but not definitive. A more comprehensive study of this topic is warranted. Magma composition The chemical composition of erupting magma is of interest in studies of volcanic lightning because this characteristic is known to influence the dissolved water content in the magma (with important effects on electrification in its own right), with important consequences for the style of the eruption (i.e., Strombolian, Plinean, etc.). The broad categorization for chemical composition in eruptions ranges from basalt to andesite to dacite to rhyolite (48–77% SiO2), with a systematic decline in equilibrium magma temperature from about 1,200°C to 800°C over this range. Water contents range from about 0.1 to 6.5 weight percent, and are systematically higher with increasing silica content Bull Volcanol Fig. 2 a Histogram of ash plume heights for eruptions accompanied by volcanic lightning. The broad peak >7 km includes heights of similar dimension and larger than typical thunderclouds. This suggests that similar mechanisms may be acting. Also note the second peak from 1 to 4 km. These heights are significantly smaller than thunderclouds and suggest a possible second mechanism or mechanisms. b Histogram of ash plume heights for eruptions accompanied by volcanic lightning plotted as percentages of the numbers of all eruptions for given ash column heights (Wallace and Anderson 2000). In an ideal case we would have eruptions of identical size (plume height and volume, etc.) with only the composition (SiO2 percent) varying. Unfortunately the tests enabled here with real-world observations fall short of this mark. To address this issue we compiled information concerning the magma composition for as many of the cases in the Appendix as possible. Some of the cases were compiled previously (Mather and Harrison 2006) and we added 30 or so new cases to that list. One problem is that information on a volcano is often given based on study of geological samples over a long time span, rather than for a specific eruption that produced lightning. Hence we were constrained to choose representative values for magma composition based on published data. All identified eruptions with lightning as functions of plume height and magma composition are listed in Table 3. Basaltic eruptions span the range from 1 to 21 km, with no clear groupings as a function of plume height. The same is true for the basaltic-andesite cases, which range from 0 to 19 km. Andesite cases, which were the most numerous, give the first indication of two groups of plume heights as also seen in Fig. 2. They also span the largest range from 0 to 21 km. Andesitic-dacite cases form a single group between 7 and 13 km plume height. Dacite cases range from 4 to 33 km (Pinatubo at the maximum) with no obvious grouping. Four of the six rhyolite cases were associated with small eruptions from 0 to 2 km plume height; the high value is for Chaiten, May 2008. This is too small a sample to be able to generalize. Thus the overall data do not appear to display any simple compositiondependent trends. The number of cases in Table 3 is fairly high and supports the general conclusions given here, however, we suspect that the sample is not uniform. This topic will benefit from better data from future eruptions. Ideally, future cases of instrumental recording of lightning will also include the supporting information on magma composition for each individual eruption. Latitude effects The current data set on volcanic lightning (Appendix) is now sufficiently extensive to explore the variation of events with latitude, with results that serve to constrain source mechanisms for the lightning. Figure 3 (top) shows the number of volcanoes with at least one eruption with lightning, binned in 5° increments of latitude and normalized for surface area within these increments, and summed for northern and southern latitudes. Figure 3 (bottom), constructed in similar fashion for sake of contrast, shows the latitudinal distribution of all volcanoes in the Holocene record (Smithsonian Institution 2009; Simkin and Siebert 1994). Figure 3 (middle) shows the latitudinal variation of all eruptions known to produce lightning. Despite a notable gap in all the distributions in Fig. 3 in the 20°–30° range, attributable to a deficit in island arc length in this region, the overall distributions are decidedly flat with latitude. Indeed, the percentage of all historical volcanoes with documented lightning (Fig. 4, top) is largely independent of latitude. If the entrainment of meteorological water was significant, then the tropical values should be significantly higher. As a check, the percentage of eruptions with lightning is also plotted versus latitude (Fig. 4, bottom). Here several volcanoes contribute heavily Bull Volcanol Table 3 Volcanic Lightning occurrence, magma composition, and ash plume height Plume Height km 0–1 1–2 2–3 3–4 4–5 5–6 6–7 7–8 8–9 9–10 10–11 11–12 12–13 13–14 14–15 Repeated letters indicate multiple observations B basalt; BA basaltic-andesite; A andesite; AD andesitic dacite; D dacite; R rhyolite 15–16 16–17 17–18 18–19 19–20 20–21 21–22 22–23 33 B B,B B B,B BA A BA BA A,A A,A,A,A A,A,A,A,A A,A AD B D R A BA,BA BA BA A,A,A A,A,A A,A,A,A A,A B B B R R,R R,R BA B D BA,BA BA AD AD AD,AD,AD AD,AD,AD,AD D AD,AD D,D D A A B BA,BA R B to specific latitude bins, but overall the distribution is still flat with no significant increase for the tropics. These observations suggest that magmatic water already brings volcanic plumes above the threshold needed to produce lightning, hence the role of meteoric water is secondary. In marked contrast with the latitudinal behavior of volcanic lightning, Fig. 5 shows the latitudinal distribution of natural (meteorological) lightning after Williams (1992). A pronounced decline with increasing latitude is evident. Similar findings are evident in the classical study of thunder days for the globe (Brooks 1925). These trends are generally attributable to the temperature dependence of saturation water vapor embodied in the Clausius-Clapeyron relation (Williams 1995, 2005). For a rough doubling of saturation water vapor mixing ratio for every 10°C of temperature change in the latter relation, this can amount to an order-of-magnitude effect between equatorial and polar regions. For thunderstorms the water substance is responsible for generating and moving charges between water droplets, ice, and graupel. Hence more water in tropical air means more lightning there. Water substance is fundamentally important for volcanic lightning, according to at least one idea (Williams and McNutt 2005). If this water is derived from the magma rising in the eruption, one does not expect a latitudinal A D,D D D dependence in the available water, because geochemistry— and water content—is independent of latitude. If, on the other hand, the water is derived by entrainment of water vapor from the local atmosphere (e.g., Rose et al. 1995a, b; Sparks et al. 1997; Carey and Bursik 2000; Textor et al. 2003), then a pronounced latitudinal dependence in volcanic lightning is expected. The latter expectation is not supported by the available observations in Figs. 3 and 4. Some water vapor is added to ash columns via entrainment, but our data suggest this is not in sufficient amounts to alter the electrical activity. In other words, there may be a threshold of water substance concentration required in a plume for lightning to occur, but this appears to be a function of the large amount of water in the magma and not the smaller amount in the entrained air. Seasonal effects A second test of these ideas pertaining to water substance involves the comparison of volcanic lightning in the winter and in the summer, on account of the pronounced differences in surface temperature between these two seasons. For purposes of this comparison, only extra-tropical volcanoes (with latitudes greater than 23° in both hemispheres) were considered. ‘Winter’ eruptions were consid- Bull Volcanol Fig. 3 a Number of volcanoes with lightning versus latitude; b number of eruptions with lightning versus latitude; and c number of volcanoes versus latitude. The three plots show basically the same trend: the distribution of volcanoes, eruptions, and volcanoes at which lightning is observed occur rather uniformly from 5 to 20 and from 35 to 65° latitude, with a conspicuous gap from 25 to 30°. This plot is very different from the plot of thundercloud lightning versus latitude shown in Fig. 5. The numbers for volcanoes and eruptions are normalized for the total area within each 5° interval of latitude ered bounded by the autumnal and vernal equinoxes, and ‘summer’ eruptions, vice versa. With these definitions, 44 eruptions from the Appendix are wintertime, in contrast with only 36 in summer. This result runs counter to the expectations based on the entrainment of local water vapor, whereas geochemistry is seasonally independent. The greater number of eruptions in winter may find an explanation in the temperature structure of the local atmosphere, a circumstance that assures that more of the magma-derived water substance is transformed to ice during the eruption. Note that the results found here do not mean that entrainment of water vapor does not occur; it Fig. 4 a Percent of volcanoes with lightning versus latitude. b Percent of eruptions with lightning versus latitude. High values in (b) between 30–35 and 60–65° represent observations from Japan and Alaska. These distributions are essentially flat, suggesting that entrainment of meteorological water does not play a major role in volcanic lightning occurrence does indeed occur. The available evidence, however, suggests that it is not an important effect in terms of increasing the water content of volcanic plumes. Previous calculations (Williams and McNutt 2005) show that the magma-derived water content in volcanic plumes is already considerably higher than that of thunderstorms. An additional effect must be noted here. We had assumed in the previous paragraph that eruptions were evenly distributed by season. However, Mason et al. (2004) demonstrate seasonality of eruptions with higher numbers occurring in boreal winter. Thus it is possible that the greater number of eruptions with lightning in winter may be Bull Volcanol observations from the constellation of US DoD satellites (Moore and Rice 1984; Pack et al. 2000). Ash plume heights Fig. 5 Latitudinal distribution of lightning from space (i.e. global ISS-b satellite observations) showing a dominant contribution from the tropics (+23°). This strong decline with latitude is attributable to the distribution of water in the atmosphere. Dominant signals are from thunderstorms, not volcanoes. Note the differences between this figure and volcanic lightning data in Figs. 3 and 4, particularly between 25– 30° and >50°. Figure from Williams (1992) based on data from Orville and Henderson (1986) a function of more eruptions in that season, and the relative ease of forming ice at colder winter conditions. Discussion Lightning occurrence Our compilation shows that volcanic lightning is quite common, having occurred at 212 eruptions from 80 volcanoes (Appendix). However, Simkin (1993) estimates that 55–70 volcanoes erupt worldwide each year. From Table 1 we find the year with the greatest number of lightning reports is 1979 with 19 cases. This suggests that only 27–35% of eruptions are accompanied by lightning, assuming one eruption per volcano per year. These must be over-estimates because most volcanoes erupt more than once per episode. There are several reasons that such low percentages of eruptions are accompanied by lightning. First, our table may be incomplete; we did our best, but we cannot guarantee completeness. Second, specialized conditions may be necessary, and these may occur during only a small percentage of eruptions. Third are reporting problems mentioned above, such as daylight or tropical environments and the need for alert observers in areas where the general population may be very sparse. To improve reporting and to remove possible bias, we recommend that a representative suite of volcanoes be instrumented and a systematic reporting scheme be set up. A more comprehensive documentation of eruptions worldwide (with and without lightning) could also be achieved through greater exploitation of continuously available The bimodal ash plume height distributions of Fig. 2 (top; and normalized version in Fig. 2 (bottom)) suggest that two broad classes of charging mechanisms may be acting. It is important to distinguish what we actually measured— plume heights—from the lengths of lightning flashes which can be much smaller. First, note that the ash plume heights are for the tops of the plumes. Lightning occurs within the ash plume at various azimuths (not necessarily vertical) and flashes typically have smaller dimensions. For the higher ash plume peak from 7 to 12 km, and including all reports greater than 7 km, the mechanism is plausibly the same as for ordinary thunderstorms. The concentration of water in eruption plumes is likely greater than for typical thunderstorms (Williams and McNutt 2005), so the stage is set for efficient charge separation via the mixed phase microphysics of water substance (Williams 1995). Indeed, the expected abundance of water may lead to an ice coating of the ash particles that interferes with a charge separation mechanism based on the collisions of dry silicate particles, but it is suggested here that tall (>7 km) volcanic ash plumes are essentially dirty thunderstorms. Further evidence for this point of view may be found in Williams and McNutt (2005). A recent study by Durant et al. (2008) concluded that volcanic plumes are “overseeded” with ice particles compared with thunderstorms, and have higher concentrations of ice particles of smaller average size. This lab based finding agrees with our inferences based on lightning distribution. Modeling studies by Textor et al. (2005a, b) also discuss formation of ice and water droplets. Durant et al. (2008) noted that ice formation occurs on ash particles at temperatures of 250 to 260 K (−10 to −20 C); these temperatures are found at heights of several km depending on the atmospheric model, latitude, and time of year. Plumes may be somewhat warmer than the surrounding ambient air, so heights of ice formation would be a bit higher. We suggest that the formation of ice particles within plumes larger than 7 km is the reason for the systematic increase in lightning percent shown in Fig. 2 (bottom). Once ice particles exist, the processes separating charges operate efficiently as in ordinary thunderstorms. The charge distribution in thunderstorms as a function of height and temperature is shown by Krehbiel (1986) and lightning initiation is common at heights of 5–6 km where temperatures are −10 to −20 C and ice particles form. This is the same range of temperatures found by Durant et al. (2008) for ice formation on ash particles. The data of Fig. 2 (bottom) suggest that this process—involving water and ice—is about 3 times more Bull Volcanol efficient than the process or processes dominant at altitudes of 6 km and below. The secondary peak of Fig. 2 (top), from 1 to 4 km, suggests that a second process or suite of processes is acting. The ash plume heights for these eruptions are smaller than those for thunderstorms and the near-vent temperatures are likely quite elevated, both effects casting doubt on any significant ice phase. Accordingly, a mechanism similar to thunderstorms seems unlikely. We suggest that several mechanisms are operating simultaneously. The first is ash particle collisions, which have been shown to generate reasonable charges in laboratory experiments (James et al. 2000). A second related mechanism consists of fracturing particles, so called fracto-emission (James et al. 2000; Gilbert and Lane 1994b). A possible third mechanism involves moving insulating bodies relative to ionizing fluids (also called streaming potential; e.g. Morgan et al. 1989). A familiar example of this is gasoline moving through hoses. (This is why gas stations have signs requiring containers to be placed on the ground for filling.) This effect requires an electrical double layer at the contact between the fluid and wall or pipe. This effect, if it occurs, may be most likely for basalt because basalt is the most fluid lava. Alternatively, gases separating from the magma or groundwater may be involved. With the cases we have for study, however, we cannot verify or quantify this mechanism. It is mentioned for the sake of completeness. Boiling of seawater, as discussed by Blanchard (1964), Blanchard and Björnsson (1967) and James et al. (2008) is a very efficient charge generating mechanism. However, the number of cases in the Appendix that involve seawater is very small, so we infer this to be a special case rather than the more ubiquitous general case involving ash. Recent instrumental observations The 2006 eruptions of Augustine (Power et al. 2006) provide some clues about charging mechanisms (Thomas et al. 2007; Thomas et al. 2010). The explosive eruption on January 28, 2006 at Augustine 08:37 UT produced significant nearly continuous radio frequency electrical discharge activity (vent discharges; 1–2 ms, 10 s of m scale length) for the 20 s during which the tephra and gases were exiting the vent (Thomas et al. 2010; these were similar to the continuous charges as shown in Fig. 1a of Thomas et al. 2007). The 08:37 UT eruption had the highest pressure amplitude (105 Pa) of the 13 explosive eruptions as measured on an infrasound sensor 3 km from the vent (Petersen et al. 2006). From this we infer relatively higher gas content and high ejection rates. However, the ash plume was only about 3.8 km high, and this eruption produced only a single lightning flash (near vent lightning; 10–30 ms, 100 m to km scale length). This behavior contrasts with the subsequent eruptions at 11:04 UT and 16:42 UT, which had ash plumes 7.2 and 7.0 km high. Each of these produced a weaker (but longer lasting) vent discharge signal at the time of the eruption, and correspondingly weaker pressure amplitudes on the infrasound sensor (Petersen et al. 2006), but each had more near vent lightning flashes, 28 for the 11:04 UT eruption and 6 for the 16:42 UT eruption. To summarize, the continuous electrical signals at the time of the eruptions (vent discharges) were positively correlated with pressure amplitudes, but negatively correlated with the number of lightning flashes. We can reconcile these observations by noting that the eruptions with longer durations produced more lightning flashes (McNutt et al. 2010). This suggests that efficient charge producing mechanisms (high pressure amplitudes at the vent) alone are not enough to produce lightning; there must also be a sufficiently large amount of tephra to carry the electric charge and redistribute it in space to produce conditions favorable for lightning generation. A later phase of sustained eruptions at Augustine (in the interval January 29-February 2, 2006) showed lightning only in association with four stronger pulses (Thomas et al. 2010), even though the ash columns were persistently 5 km or more in height. The ash plume height was 3.8–7.2 km for each of the four pulses (Thomas et al. 2010). However, the pressure amplitudes were low (all less than 13 Pa at 3 km distance), so even though abundant tephra was available, the charging mechanisms were only sufficiently vigorous for lightning production when the stronger pulses occurred. We infer that virtually all the visual observations of lightning in the Appendix are either near vent lightning or plume lightning; the vent discharges (continuous signals during eruption) have only been observed instrumentally and there are not yet any corroborating visual observations. From a theoretical point of view, the maximum electric field at the surface of a uniformly charged spherical volume of radius R is E ¼ rR=3"o where ρ is the space charge density (C/m3) and εo is the permittivity of free space. The maximum field between two uniformly charged spherical volumes of opposite polarity is twice this value, by superposition. These simple calculations show that dielectric breakdown can be achieved in clouds of small size only if the space charge density is very large. Typical values of ρ for thunderstorms are 1 nC/m3 which requires R of several km to produce lightning. For some observed volcanic lightning, the scale length is a few hundred meters, which suggests space charge densities about one order of magnitude larger. Dielectric breakdown initiated in the high field region is sufficient to produce VHF radiation, but subsequent thermalization of the streamer channel is required to form lightning flashes. Bull Volcanol (Thermalization is movement of the channel towards thermal equilibrium, a transition in the state from high electron energy alone to high energy for all constituents (Gallimberti et al. 2002)). Small volumes of space charge may not provide sufficient charge (and current) for thermalization, if laboratory studies are a guide (Boschung et al. 1977). These considerations suggest that the nearly continuous electrical activity—vent discharges—in the high pressure emission at Augustine on January 28, 2006 at 08:37 UT was caused by a mechanism generating large space charge density in a relatively compact cloud (3.8 km height) that produced discharges with durations much shorter than typical lightning flashes in thunderclouds. The larger, deeper clouds (7.0–7.2 km) in the 11:04 UT and 16:42 UT eruptions plausibly involved an in situ mechanism, possibly involving ice particle collisions, which allowed for both dielectric breakdown and sufficient charge to thermalize channels and provide for discharges with durations more typical of those in thunderclouds. In the later January 29-February 2, 2006 Augustine eruption phase, involving smaller clouds (<~5km) and also low ejection rates, again, only four episodes of near vent lightning activity were present. The behavior during most of the continuous phase is plausibly explained by the absence of high space charge density and by a cloud radius R insufficient for either dielectric breakdown or channel thermalization. Other meteorological phenomena Electrical charge separation is known to occur in two other meteorological phenomena that are distinct from thunderclouds: dusty gust fronts (Williams et al. 2009) and dust devils (Freier 1960; Crozier 1964; Ette 1971). These involve lofting of silicate minerals into the boundary layer by strong winds by an entirely dry process. Though the detailed physical process for charge separation is still poorly understood at the particle scale, the observations support a selective charging of the smaller dust particles with negative electricity. This polarity is opposite to the behavior of ordinary thunderclouds and the few volcano clouds that have been documented electrically (Cobb 1980; Hobbs and Lyons 1993; Lane and Gilbert 1992; Gilbert and Lane 1994b; Hoblitt 1994; McNutt and Davis 2000). Miura et al. (2002) showed cases with both positive and negative charge in fine particles from eruptions of Sakurajima. Furthermore, dusty gust fronts and dust devils occur in dry environments, whereas even ‘dry’ volcanic eruptions contain a significant quantity of water. These considerations and comparisons cast doubt on the gust front/dust devil process alone in accounting for volcano electricity. To better constrain these ideas, instrumental data are needed. For example we need to know particle velocities and electric field intensities as functions of time. Are particles already charged and simply hoisted into the air by eruptions? Or does the eruption process itself produce the charges? Previous works by Gilbert and Lane (1994b) and James et al. (2000) investigated charging mechanisms and rates but not with respect to lightning per se. If particle collisions are needed, then we would expect greater concentration of fines in ash columns with greater charge, and textural evidence of collisions in the particles that fall to the ground. We are not aware of studies that looked for these features in particular with respect to volcanic lightning production, and we suggest that such studies are needed. Information is also needed on the distribution of electric charge carried by tephra particles over the full range of particle sizes. Some work on charge versus size has been documented by Miura et al. (2002) but the eruptions studied did not produce lightning. In ordinary thunderclouds, the ability to access such information is difficult. In volcanic eruptions, the access is extraordinarily difficult. Practical considerations A certain concentration or density of charge is needed to cause lightning, so there ought to be a relation between ash particle concentration and lightning occurrence if indeed the ash particles are the charge carriers. This suggests that lightning may be used as a real-time predictor of charge density, hence ash particle density. The occurrence of lightning would then add information of value to determine ash hazards to aviation. Lightning could thus improve the ability to verify when significant ash clouds are being produced, and by identifying the different types or regimes of lightning, such as near-vent or plume lightning, also improve estimates of the sizes of eruptions. This would be especially true for volcanoes where lightning detection systems are in place, which could provide information in poor weather or darkness. Better instrumental data are needed, including specific experiments for individual eruptions as well as better utilization of existing resources. For example, there is a need for a systematic search for volcanic lightning in the Lightning Imaging Sensor (LIS) and Optical Transient Detector (OTD) satellite data (Christian et al. 2003). Volcanic lightning presents many interesting research opportunities, which are complementary to both atmospheric sciences and volcanology. It is hoped that future research with better data will further illuminate the trends identified in this work. Conclusions Data from a comprehensive global database show that lightning has been documented at 80 volcanoes in Bull Volcanol association with 212 eruptions. Eight percent of VEI=3–5 eruptions have reported lightning, and 10% of VEI=6, but less than 2% of those with VEI=1–2. These findings suggest consistent reporting for larger eruptions but either less lightning, a different mechanism, or possible underreporting for small eruptions. Ash plume heights show a bimodal distribution with main peaks at 7–12 km and 1– 4 km. The former are similar to heights of typical thunderstorms and suggest involvement of water substance, whereas the latter suggest other factors contributing to electrical behavior closer to the vent. Reporting of lightning is more common at night (56%) and less common in daylight (44%). Reporting also varied substantially from year to year. Several weak trends in lightning occurrence based on magma composition were found. The bimodal ash plume heights are obvious only for andesite to dacite; basalt and basaltic-andesite evenly span the range of heights; and rhyolites are poorly represented. The distributions of the latitudes of volcanoes with lightning and eruptions with lightning roughly mimic the distribution of all volcanoes, which is generally flat with latitude. Meteorological lightning, on the other hand, is common in the tropics and decreases markedly with increasing latitude. This finding supports the idea that lightning in large (deep) eruptions depends on water substance, and the origin of the water is primarily magma and not entrainment from the surrounding atmosphere. Seasonal effects show that more eruptions with lightning were reported in winter (bounded by the respective autumnal and vernal equinoxes) than in summer, again suggesting that the water is primarily from magma. The small number of modern instrumental observations from Augustine Volcano shows features that are complementary to the data from the global compilation. 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