Ann. occup. Hyg., Vol. 48, No. 5, pp. 483–490, 2004 © 2004 British Occupational Hygiene Society Published by Oxford University Press doi:10.1093/annhyg/meh031 Particle Deposition in Industrial Duct Bends THOMAS M. PETERS and DAVID LEITH* Department of Environmental Sciences and Engineering, The University of North Carolina, Chapel Hill, NC 27599, USA Received 30 September 2003; in final form 6 January 2004; published online on 7 July 2003 A study of particle deposition in industrial duct bends is presented. Particle deposition by size was measured by comparing particle size distributions upstream and downstream of bends that had geometries and flow conditions similar to those used in industrial ventilation. As the interior surface of the duct bend was greased to prevent particle bounce, the results are applicable to liquid drops and solid particles where duct walls are sticky. Factors investigated were: (i) flow Reynolds number (Re = 203 000, 36 000); (ii) particle Reynolds number (10 < Rep∞ < 200); (iii) particle Stokes number (0.08 < Stk < 16); (iv) bend angle (θ = 45°, 90°, 180°); (v) bend curvature ratio (1.7 < R0 < 12); (vi) orientation (horizontal-to-horizontal and horizontal-tovertical); and (vii) construction technique (smooth, gored, segmented). Measured deposition was compared with models developed for bends in small diameter sampling lines (Re < 20 000; Rep∞ < 13). Whereas deposition measured in this work generally agreed with that estimated with models for particles <30 µm (Stk < 0.7), it was significantly lower than that estimated for larger particles. As the flow around larger particles became increasingly turbulent, the models progressively under-represented drag forces and over-estimated deposition. For particles >20 µm, deposition was slightly greater in the horizontal-to-horizontal orientation than in the horizontal-to-vertical orientation due to gravitational settling. Penetration was not a multiplicative function of bend angle as theory predicts, due to the developing nature of turbulent flow in bends. Deposition in a smooth bend was similar to that in a gored bend; however, a tight radius segmented bend (R0 = 1.7) exhibited much lower deposition. For more gradual bends (3 < R0 < 12), curvature ratio had negligible effect on deposition. Keywords: bend; elbow; deposition; droplet; duct; impaction; transport; ventilation that adhere to the duct walls upon impact. Deposited droplets and particles can restrict airflow in branch lines, create fire hazards, cause failure of overhead supports, and present growth media for biological contaminants (May and Berard, 1987; Gregory et al., 1991). This work focuses on particle deposition in industrial duct bends. The objectives are: (i) to measure deposition in industrial bends; and (ii) to compare these measurements with estimates from published models. INTRODUCTION Particle deposition in ducts is important in situations ranging from the pneumatic transport of materials and icing of aircraft intakes to bioterrorist attacks. In occupational hygiene, the airflow velocity required to prevent particle deposition in ducts, commonly called the criterion of minimum transport velocity, serves as the basis for exhaust system design (ACGIH, 1998). Acceptable values for this criterion are available for solid particles that bounce upon contact with duct walls and are then re-entrained into the highly turbulent airflow of an industrial exhaust system (Baliff et al., 1948; DallaValle, 1932; Rajahns and Thompkins, 1967). The criterion of minimum transport velocity is not suited for liquid particles, especially oil droplets, BACKGROUND A bend introduces several scales of curvilinear motion to duct flow. The largest of these motions occurs as the bend reorients the direction of the airflow: its radius is of the size of the bend radius, Rb. As the centrifugal force drives the central air core toward the outer wall, a smaller secondary flow *Author to whom correspondence should be addressed. Tel: +1-919-966-3851; fax: +1-919-966-7911; e-mail: [email protected] 483 484 T. M. Peters and D. Leith develops perpendicular to the main flow. The size of the secondary flow is of the size of the duct radius, a (Ito, 1987), and its strength is characterized by the Dean number, De (Berger and Talbot, 1983): De = Re/(R0)1/2, where R0 is the radius of the bend divided by the radius of the duct (R0 = Rb/a), and Re is the Reynolds number. For laminar flows (De < 370), the flow rapidly becomes fully developed with a single pair of counter-rotating vortices (Berger and Talbot, 1983). For turbulent flows (De > 370), experiments show that airflow continually develops throughout a 180° bend (Rowe, 1970; Enayet et al., 1982; Azzola et al., 1986; Anwer et al., 1989). In this flow regime, further vortical structures can develop at various locations in the bend (Boersma and Nieuwstadt, 1996). For tight bends (R0 < 3) with turbulent flow, separation can occur at the inner wall causing the replacement of the secondary flow with a single circulation pattern that switches direction at low frequency, f (Tunstall and Harvey, 1968). Rütten et al. (2001) characterized this phenomenon with the dimensionless Strouhal number: Sr = 2fDduct/U0. Several mechanisms, including Brownian diffusion, gravitational setting and electrostatic forces, can cause particles to deposit in ducts. In bends, the mechanism of inertial impaction dominates deposition for particles >10 µm (Brockmann, 2001). Given sufficient inertial force, a particle will deviate from airflow streamlines and hit the bend wall. Deposition will occur if the adhesive forces are greater than the rebound forces (Hinds, 1999). Particle deposition in bends has been characterized with the following dimensionless parameters: (i) particle Stokes number (Stk = τU0/a); (ii) particle free-stream Reynolds number (Rep∞ = DpU0/ν); (iii) flow Reynolds number (Re = DductU0/ν); (iv) De; and (5) R0 (Cheng and Wang, 1975; Pui et al., 1987). All researchers have used Stk to describe results, but use of parameters such as R0 and Re have been debated (Crane and Evans, 1977; Cheng and Wang, 1981; Pui et al., 1987). For laminar flows (De < 900; Re < 3000), Tsai and Pui (1990) claimed increased deposition with increased secondary flow strength (De high and R0 small) and used Stk, Re, De and R0 to describe their results. For moderately turbulent flows, Pui et al. (1987) used Stk alone to describe experimental measurements (R0 = 5.7; Re = 10 000 and 6000; and Rep∞ < 13) as: ηdep = (1–10–0.963 Stk) × 100%. Brockmann (1993) modified this formula to include the bend angle in radians (θ): η dep = [ 1 – exp ( – 1.412Stkθ ) ] × 100% (1) McFarland et al. (1997) used Stk, θ and R0 to describe the fraction of particles penetrating a bend. Their correlation can be rewritten in terms of deposition as: 4.61 + a m θStk - η dep = 100% – exp --------------------------------------------------------------------------------2 2 1 + b m θStk + c m θStk + d m θ Stk (2) where, am, bm, cm and dm are coefficients found using a curve-fitting program. However, an error appears in the published coefficient for the second term in the numerator of coefficient dm. Equation (13) of McFarland et al. (1997) should read: a m = – 0.9526 – 0.05686R 0 – 0.297 – 0.0174R 0 b m = -----------------------------------------------------2 1 – 0.07R 0 + 0.0171R 0 (3) 1.895 2.0 c m = – 0.306 + ------------- – ------R0 R0 2 0.131 – 0.0132R 0 + 0.000383R 0 d m = ----------------------------------------------------------------------------2 1 – 0.129R 0 + 0.0136R 0 For highly turbulent flow, Hacker et al. (1953) investigated deposition of water drops entering aircraft intakes (700 000 < Re < 3 700 000). Using a two-dimensional potential flow simulation, they demonstrated that Rep∞ strongly influenced deposition. Crane and Evans (1977) suggested that Rep∞ could affect deposition to a greater extent than R0. Their analysis estimated that for Stk = 0.7 and R0 = 4 deposition would decrease from 58% for Rep∞ of 0, to 52% for Rep∞ of 5, and to 26% for Rep∞ of 450. In industrial ventilation ducts, recommended minimum transport velocity ranges from 10 m/s for welding fumes to 30 m/s for heavy or moist dusts (Alden and Kane, 1982). Given a transport velocity of 20 m/s, the flow Re increases from 130 000 to 1 300 000 as the diameter of industrial duct increases from 0.1 m to 1 m. Typical values of R0 are between 3 and 5; cost factors generally limit the use of bends with large R0, and high pressure drop prevents widespread use of bends with small R0 (ACGIH, 1998). Given these restrictions, De in industry is ~30 000– 500 000. For droplets of unit density, Stk ranges from 0.01 to 4, and Rep∞ ranges from 1 to 300 for particles of 10–100 µm, respectively. Previous work is inadequate to describe particle behavior in industrial bends. The correlation models of Pui et al. (1987) and McFarland et al. (1997) were constructed using experimental data atypical of industry: i.e. small particles (Dp < 10 µm), small diameter tubes (Dduct < 1.6 cm), and moderately turbulent flow (Re < 19 000). The theoretical studies of Hacker et al. (1953) and Crane and Evans (1977) are useful in a qualitative sense, but are difficult to apply to a new set of conditions and have no experimental Particle deposition in industrial bends backing. Moreover, past research has been limited to bends with smooth interior walls, when, in reality, the interior of industrial bends is rarely smooth because of the manner in which they are constructed. Thus, the experiments presented in the current work are the first to be directly applicable to industrial bends. MATERIALS AND METHODS Particle deposition Particle deposition by size was measured using the methods presented by Peters and Leith (2003); a brief overview of this method is provided here. Figure 1 illustrates the experimental set-up. Upstream of the test bend, an aerosol generator introduced polydisperse glass spheres that ranged in size from 5 to 150 µm. To capture and retain particles that hit the 485 wall, the interior of the bend was coated with petroleum jelly. Circular sampling grids were cut from welded-wire mesh, coated with petroleum jelly, and alternately inserted into the duct upstream and downstream of the bend. Upstream velocity profiles were characteristic of fully developed pipe flow (Tennekes and Lumley, 1972), and particle profiles were uniform in concentration and size distribution. After sampling, the collected particles were recovered from the grids using a hexane extraction procedure and then sized using a sedimentation pipette (Silverman et al., 1971). Cumulative mass distributions were fitted with a log-normal distribution: all distributions were fit with r2 > 0.8. From these distributions, deposition was calculated for each size interval (i) as: dM i,down ηdep,i = 1 – ------------------- dM i,up where dMi,down is the downstream and dMi,up is the upstream interval mass associated with the lognormal fit. Experiments Table 1 lists the eight test conditions investigated. A base condition was selected as: Re = 203 000; R0 = 5; construction = smooth; and orientation = horizontal-to-horizontal (H–H). Re of 203 000 was achieved in a 0.152 m duct at an average velocity of 20.0 m/s. Given these conditions, Rep∞ ranged from 10 to 150, Stk ranged from 0.1 to 16, and De was 91 000. The base conditions were modified to evaluate how duct orientation, bend angle and bend Fig. 1. Experimental set-up. Table 1. Test conditions investigated θ, degrees Test description Re (De) Construction Orientation Basea 203 000 (91 000) 90 5 Smooth H–H Base + orientationa 203 000 (91 000) 90 5 Smooth H–V Base + bend angleb 203 000 (91 000) 180 5 Smooth H–H Base – bend anglec 203 000 (91 000) 45 5 Smooth H–H Base + constructiond 203 000 (91 000) 90 5 Gored H–H Base – constructione 203 000 (156 000) 90 1.7 Segmented H–H High Re, small R0f 368 000 (212 000) 90 3 Smooth H–H High Re, large R0g 368 000 (106 000) 90 12 Smooth H–H R0 Italic font identifies parameters that deviate from the base condition. aH-P Products, Louisville, OH 44641; P/N EL-602-Z. bTwo 90° bends as specified in footnote a butted together to form a 180° bend. cH-P Products; P/N EL-601-Z. dMcGill Airflow Corp., Groveport, Ohio 43125; Custom 5-piece, Gored, 6-in., 90° bend. eMcMaster-Carr, Atlanta, GA 30374 ; P/N 1766K34. fW.H. Brady, Inc., Elkton, MD 21922; P/N 90S, 8-in. diameter. gH-P Products; P/N 14–800321-Z. 486 T. M. Peters and D. Leith construction affect particle deposition. For the last two conditions in Table 1, Re was 368 000 in a 0.203 m duct with an average velocity of 27.1 m/s. All tests were conducted in a H–H orientation except for one test, where the air entered the bend horizontally and exited vertically (H–V). Deposition by size was measured three times for each test condition. Figure 2 depicts the bend construction types investigated. Smooth bends (Fig. 2a) were manufactured by bending straight tubing or fabricated by welding together two stamped halves. The gored bend (Fig. 2b) was constructed by welding sections of sheet metal together. The interior surface of the gored bend deviated from a smooth bend in that: (i) the welded seams protruded into the duct perpendicular to the main direction of airflow; and (ii) the bend’s sectional construction presented flat surfaces to the airflow. The segmented bend (Fig. 2c) was joined by interlocking sheet-metal sections. Most segmented bends have small R0; the bend tested in this work had an R0 of 1.7. Statistical analysis The combined data from the three runs for each test condition were fitted with a cumulative log-normal function (Cooper, 1982). The cutpoint (D50), or the particle size associated with 50% deposition, and the geometric standard deviation (GSD), a descriptor of the shape of the deposition curve, were estimated from the fitted function. The parameter estimates of the fitted function were used to investigate the similarity in deposition by size for different test conditions. RESULTS Table 2 provides the fit r2 value, D50 and GSD for each test condition. The cumulative log-normal distribution explained >76% of the variability in the experimental data for seven of the eight test conditions. The lowest r2 value (0.61) was observed for the test with the segmented bend. Figure 3 compares deposition by size for the base condition (H–H orientation) to H–V orientation and to model estimates from equations (1) and (2). The deposition curve was slightly steeper in the H–H orientation than in the H–V orientation (p = 0.001). The deposition curves for both H–H and H–V orientations were shallower than those estimated with either model. For particles <30 µm, the experimental Table 2. Fit results Test conditions r2 Base 0.94 D50 (µm) 18.1 GSD 2.3 0.94 20.5 2.9 0.76 12.5 2.3 0.92 105.4 24.9 0.97 18.2 2.9 Base + orientation H–V Base + bend angle θ = 180 Base – bend angle θ = 45 Base + construction Gored Base – construction 0.61 39.5 2.7 High Re; small R0 Segmented; R0=1.7 0.88 21.4 3.0 High Re; large R0 0.80 19.5 3.7 Model comparison For each test condition, experimental results were compared with deposition estimated with the Pui et al. (1987) model, equation (1), and the McFarland et al. (1997) model, equation (2). Fig. 2. Industrial bends and identification of key dimensions. Fig. 3. Deposition by size: orientation varied. Particle deposition in industrial bends Fig. 4. Deposition by size: bend angle varied. data overlapped with the Pui et al. (1987) model estimates, but measured deposition was substantially greater than that estimated with the McFarland et al. (1997) model. For larger particles, measured deposition was substantially less than that estimated with either model. Figure 4 shows deposition by size as a function of bend angle. For a given particle size, deposition increased with bend angle. For θ = 45°, deposition increased from 15% at 10 µm to 45% at 80 µm. For larger bend angles, deposition neared 100% for 100 µm particles. Figure 5 presents deposition by size for bends of different construction. Deposition in the smooth bend was similar to that in the gored bend, but was substantially and significantly higher than that in the segmented bend. The deposition cutpoint for the segmented bend (D50 = 39.5 µm) was significantly larger than that for the smooth bend (18.1 µm, p < 0.001). Figure 6 compares deposition by size measured in bends with two curvature ratios to that estimated with the models. Deposition measured in the tight bend (R0 = 3) was statistically equivalent to that in the gradual bend (R0 = 12): p = 0.53 for D50 values and p = 0.23 for GSD values. Whereas the experimental results compared favorably with the Pui et al. (1987) model estimates for particles <30 µm, measured deposition was greater than that estimated with the McFarland et al. (1997) model. For particles >30 µm, measured deposition was substantially lower than that estimated with either model. 487 Fig. 5. Deposition by size: bend construction varied. Fig. 6. Deposition by size: curvature ratio varied. DISCUSSION As shown in Figures 3 and 6, deposition by size in industrial bends was not fully described by models developed for small sampling tubes. Whereas the experimental data in this work compared favorably with the Pui et al. (1987) model estimates for particles <30 µm (Stk < 0.7), it was substantially lower than that estimated for larger particles. Moreover, the differences between measurement and models became greater when the flow Reynolds number 488 T. M. Peters and D. Leith increased from Re = 203 000 (Fig. 3) to Re = 368 000 (Fig. 6). For relatively small particles, the agreement between the deposition measured here and that estimated with the Pui et al. (1987) model illustrates the importance of Stk in estimating deposition in bends. Furthermore, the agreement suggests that deposition is dominated by large-scale curvilinear motion as opposed to the more subtle airflow features. The region where models over-estimate deposition is consistent with non-Stokesian drag effects and airflow turbulence. Some data associated with the smallest particle size (near 10 µm) had relatively large error bars and did not follow expected trends. For example, in Fig. 3, the difference in deposition between orientations should diminish as particle size becomes smaller and gravity becomes less important; this trend was observed for all but the smallest diameter particle where the error bars were large. As discussed in Peters and Leith (2003), the sedimentation pipette was optimized to size large particles, and thus, suffered from greater uncertainty for the smallest particle size measured. The analysis technique might be optimized for smaller particles, or perhaps more practical, alternative real-time, in situ methods might be used to determine deposition for particles of this size and smaller. Figure 7 compares Repr by particle size for the current experiments to that used to build the models. Repr was calculated as: Repr = DpVr/ν, where Vr is the radial velocity of the particle. Vr was estimated from a balance of outward centrifugal forces and drag forces for a particle in the centerline of the bend. Plug flow was assumed in this estimation. For the Pui et al. (1987) and McFarland et al. (1997) data, Vr was Fig. 7. Particle radial Reynolds number by size in this work and the experimental work used to develop the models of Pui (1987) and McFarland (1997). estimated from conditions they reported. For conditions in the current work where Repr was less than that of the models (i.e., Repr < 3 for particle sizes <30 µm), the models acceptably represented drag forces and experiments done here agreed with the model estimates. However, as Repr progressively became >3 (i.e. particles >30 µm), the models increasingly under-represented drag forces and overestimated deposition. Airflow turbulence might also explain some model over-estimates. Torobin and Gauvin (1961) showed that free-stream turbulence decreases the critical Reynolds number where the flow over a particle transitions from laminar to turbulent. Thus, drag forces were further under-represented in the models. Crowe et al. (1998) provided equations to account for this behavior that might be useful in future modeling efforts. As shown in Fig. 3, the deposition curve for an H– H oriented bend was steeper than that for an H–V oriented bend. When oriented H–H, gravity caused particles to settle throughout the length of the bend. As gravitational settling is proportional to the square of particle size, deposition in the H–H orientation was greater than that in the H–V orientation for particles larger than ∼20 µm. Theory predicts that particle penetration, P = 100% – ηdep, is a multiplicative function of bend angle. Thus, deposition in the 90° and 180° bends can be estimated as 100% – P452 and 100% – P454, respectively. This relationship generally holds for particles <20 µm, but not for larger particles (Fig. 4). As turbulent flow in a bend develops continuously, sufficient curvilinear motion to deposit large particles was not established by a bend angle of 45°. Better agreement was observed between deposition measured in the 180° bend and that estimated as 100% – P902, suggesting that most flow development had occurred by a bend angle of 90°. As shown in Figure 5, deposition by size was nearly identical for the smooth and gored bends; however, it was substantially lower and exhibited the greatest variability in the segmented bend. Relatively clean laboratory air might have leaked into the segmented bend through its interlocking joints, providing a clean air sheath at the bend walls that reduced deposition. As the interior of the bend was recoated with grease when sampling was switched from the upstream to the downstream position, the leaks through the interlocking joints might have changed between runs, explaining the relatively high variability in measurements for this test condition. Alternatively, the segmented bend had a very tight curvature ratio (R0 = 1.7) compared with the other bends tested (R0 > 3). As noted by Tunstall and Harvey (1968) and Rütten et al. (2001), drastically different airflow patterns are anticipated in a tight bend at these flow conditions due to flow separation Particle deposition in industrial bends at the inner wall; these differing airflow patterns may account for reduced deposition. For more gradual bends (3 < R0 < 12), deposition by particle size was relatively unaffected by curvature ratio (Fig. 6). Deposition was slightly higher in the gradual bend (R0 = 12) compared with that in the tight bend (R0 = 3). Although estimates made with the McFarland et al. (1997) model qualitatively agree with this trend, the difference in estimated deposition was greater than that observed in the experiments. The major limitation of the present work was that the inlet profiles were uniform in terms of the velocity, particle size distribution, and particle concentration. In industrial settings, deviations from such uniform conditions often occur. More work is required to evaluate how deposition changes as inlet conditions become non-uniform. CONCLUSIONS This work explored particle deposition by particle size in industrial duct bends. As the interior surface of the duct bend was greased to prevent particle bounce, the results are applicable to liquid drops and solid particles where duct walls are sticky. These experiments are the first of their kind for conditions typical of industry. As such, they should be useful to construct models appropriate for industrial conditions and to benchmark computer simulations. A new model is required to describe droplet deposition in industrial bends adequately. The high radial velocity that large droplets experience in industrial bends represents a substantial departure from conditions in small diameter sampling lines, for which the models of Pui et al. (1987) and McFarland et al. (1997) were developed. Thus, these models underrepresent drag forces and over-estimate deposition in industrial bends. Further, the current work suggests that gravitational settling causes differences in deposition with orientation. Bend angle is important in estimating deposition for particles >30 µm. In contrast, curvature ratio is relatively unimportant for R0 between 3 and 12. NOMENCLATURE a = duct radius am, bm, cm, dm = constants used in the McFarland et al. (1997) model Cc = Cunningham slip correction factor Dduct = duct diameter down = downstream measurement Dp = particle diameter Dx = the particle diameter associated with x% deposition dM = differential mass 489 2 2 ρf U0 -----------Rb Re- = ---------------De = Dean number = --------µf R0 f = frequency of switching GSD = geometric standard deviation = D 84 -------D 16 H–H = horizontal-to-horizontal orientation H–V = horizontal-to-vertical orientation i = particle size interval P = penetration Py = penetration associated with a particle of diameter y R0 = curvature ratio = Rb/a Rb = radius of bend Re = flow Reynolds number = DductU0/ν Rep∞ = free-stream particle Reynolds number = DpU0/ν Repr = radial particle Reynolds number = DpVr/ν U0 = mean axial velocity upstream of the bend up = upstream measurement Vr = particle radial velocity Sr = Strouhal number = 2fDduct/U0 Stk = particle Stokes number based on duct radius = τU0/a ηdep = percent of incoming particles that deposit µf = fluid dynamic viscosity ν = fluid kinematic viscosity θ = bend angle ρf = fluid density ρp = particle density τ = particle relaxation time = CcρpD2p/18µf Acknowledgements—This work was made possible by a gift from Ford Motor Company and the United Auto Workers to support research in air engineering at the University of North Carolina at Chapel Hill, by a Department of Education Fellowship for Interdisciplinary Training in Environmental Engineering, and by a National Institute of Occupational Safety and Health Educational Resource Center Training Grant (T42/CCT410423–09). 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