Module 6 - Nitrification Fundamentals

Activated Sludge
Nitrification/Denitrification
Fundamentals
by
R. Dale Richwine, P.E.
Richwine Environmental, Inc.
Session Overview
» Forms of Nitrogen
» Nitification/Denitrification Principles
» Nitrification in a WWTP
» Ammonia/Nitrogen Removal Processes
1
Nitrogen
» Total Nitrogen (TN)
» Total Kjeldahl Nitrogen (TKN)
» Organic Nitrogen (Organic-N)
» Ammonia Nitrogen (N-NH3 or N-NH4+)
» Nitrite (NO2)
» Nitrate (NO3)
» Elemental Nitrogen (N2)
Nitrogen
» TN = TKN + NO2 + NO3
» TKN = Organic-N + N-NH3
» Nitrogen Cycle
– 
– 
– 
– 
Nitrogen Fixation (N2 Ž Organic-N)
Ammonification (Organic-N Ž N-NH3)
Nitrification (N-NH3 Ž NO2 Š NO3)
Denitrification (NO3 Ž N2)
2
Nitrogen Cycle
Aerobic Respiration Oxidizes Organics
to CO2 and H2O for Energy
3
Organic Nitrogen is converted
to Ammonia
OXIDATION AND SYNTHESIS
bacteria
COHNS + nutrients ⎯⎯
⎯⎯→ CO2 + NH3 + C5H7NO2 + other end products
ENDOGENOUS RESPIRATION
bacteria
C5H7NO2 + O2 ⎯⎯
⎯⎯→ 5CO2 + 2H 2O + NH3 + energy
Ammonification
4
Biological Nitrification
» 2-step process
» Step 1 – Ammonia converted to Nitrite
» Step 2 – Nitrite converted to Nitrate
Nitrification
5
Biological Nitrification
Step 1: Ammonia oxidized to Nitrite. Hydrogens are released
resulting in the reduction of alkalinity.
Nitroso - bacteria
2NH + 3O ⎯⎯ ⎯ ⎯ ⎯ ⎯ ⎯ ⎯
⎯→ 2NO − + 2H O + 4H+
4
2
2
2
Step 2: Nitrite is oxidized to Nitrate
Nitro − bacteria
2NO − + O ⎯⎯ ⎯ ⎯ ⎯ ⎯ ⎯⎯→ 2NO −
2
2
3
Total Oxidation Reaction
NH+ + 2O ⎯⎯⎯⎯→ NO- + 2H+ + H O
4
2
3
2
Ammonium Oxidation Bacteria
Nitroso - bacteria
2NH + 3O ⎯⎯ ⎯ ⎯ ⎯ ⎯ ⎯ ⎯
⎯→ 2NO − + 2H O + 4H+
4
2
2
2
Ammonia Oxidizing Bacteria
•  Nitrosomonas
•  Nitrosospira
•  Nitrosococcus
•  Nitrosolobus
•  Nitosorobrio
6
Nitrite Oxidation Bacteria
Nitro − bacteria
2NO2− + O2 ⎯⎯ ⎯ ⎯ ⎯ ⎯ ⎯⎯→ 2NO3−
Nitrite Oxidizing Bacteria
•  Nitrobacter
•  Nitrococcus
•  Nitrospina
•  Nitrospira
•  Nitroeystis
Rates of Nitrification by
Various Bacteria
Organism
Substrate
Product
Rate of
Formation
Max. Product
Accumulation
Arthrobacter
NH4+
Nitrite
375 – 9,000
0.2 – 1
Arthrobacter
NH4+
Nitrate
250 – 650
2 – 4.5
Aspergillis
NH4+
Nitrate
1,350
75
Nitrosomonas
NH4+
Nitrite
1 – 30 million
2,000 – 4,000
Nitrobacter
NH2-
Nitrate
5 – 70 Million
2,000 – 4,000
7
Alkalinity Requirements
NH+ + 2HCO− + 2O ⎯⎯→ NO− + 2CO + 3H O
4
3
2
3
2
2
For each gram of ammonia nitrogen (as N) converted
7.14 grams of alkalinity as CaCO3 is required.
Biological Denitrification
Carbon Source Required as Electron Donor
− ⎯⎯→ NO ⎯⎯→ N O ⎯⎯→ N
NO3
2
2
Wastewater
C H O N + 10NO− ⎯⎯→ 5N + 10CO + 3H O + NH + 10OH−
10 19 3
2
2
2
2
3
Methanol
5CH OH + 6NO− ⎯⎯→ 3N + 5CO + 7H O + 6OH−
3
3
2
2
2
8
Denitrification
Nitrification in the WWTP
Org-N
Ammonification
Org - N → NH4 - N
Influent
TKN
Nitrogen Gas
NH4 - N
Nitrification
NH4 - N → NO3 - N
Aerobic
Denitrification
NO3 - N → N2 (g)
Anaerobic
9
Processes Used for
Nitrogen Removal
Nitrification Processes
» Preanoxic
– 
– 
– 
– 
– 
– 
Ludzack-Ettinger
Modified Ludzack-Ettinger (MLE)
Step Feed
Sequencing Batch Reactor (SBR)
Bio-denitro
Nitrox
10
Nitrification Processes
» Post-anoxic
– 
– 
– 
– 
Single-sludge
Bardenpho (4-stage)
Oxidation Ditch
Two-stage (two-sludge)
» Simultaneous Nitification/Denitrification
–  Low DO Oxidation Ditch
–  Orbal Oxidation Ditch
Ludzack-Ettinger
Secondary
Clarifier
Influent
Anoxic
Aerobic
Effluent
Return activated sludge
Sludge
11
Modified Ludzack-Ettinger (MLE)
Internal recycle
Secondary
Clarifier
Influent
Anoxic
Effluent
Aerobic
Return activated sludge
Sludge
Step Feed
Influent
Secondary
Clarifier
Anoxic Aerobic Anoxic Aerobic Anoxic Aerobic Anoxic Aerobic
Effluent
Return activated sludge
Sludge
12
Sequencing Batch Reactor (SBR)
Influent
Air
Effluent
Fill
Fill
anoxic/anaerobic
mix
React/aeration
Settle
Decant
Idle
Bio-denitro
Secondary
Clarifier
Aerobic
Anoxic
Effluent
Influent
Aerobic
Aerobic
Return activated sludge
Return activated sludge
Sludge
Sludge
Phase B
Phase A
Aerobic
Aerobic
Effluent
Influent
Effluent
Influent
Aerobic
Anoxic
Return activated sludge
Return activated sludge
Sludge
Sludge
Phase C
Effluent
Influent
Phase D
13
Nitrox
Aerator and
mixer control
PLC
Aerator
DO
ORP
Secondary
Clarifier
Effluent
Mixer
Return activated sludge
Sludge
Influent
Single-Sludge
Secondary
Clarifier
Influent
Aerobic
Anoxic
Effluent
Return activated sludge
Sludge
14
Bardenpho (4-stage)
Mixed-liquor return
Secondary
Clarifier
Influent
Anoxic
Aerobic
Anoxic
Aerobic
Effluent
Return activated sludge
Sludge
Oxidation Ditch
Aerators
Anoxic
Aerobic
Secondary
Clarifier
Effluent
Return activated sludge
Influent
Sludge
15
Two-Stage (two-sludge)
Air
Air
Methanol
Primary
Clarifier
Nitrification
Clarifier
Secondary
Clarifier
Effluent
Influent
Nitrification tank
Denitrification tank
Return activated sludge
Return activated sludge
Sludge
Sludge
Sludge
Low DO Oxidation Ditch
Aerators
Influent
Secondary
Clarifier
Effluent
DO probe
NADH probe
(Sym-BioTM process)
Return
activated
sludge
Sludge
16
Orbal
Aerobic
First
channel
Second
channel
Third
channel
Anoxic
Secondary
Clarifier
Anaerobic
Effluent
Influent
Internal recycle (optional)
Return activated sludge
First channel
Sludge
Second channel
Third channel
Influent
Effluent
Session Summary
» Forms of Nitrogen
» Nitification/Denitrification Principles
» Nitrification in a WWTP
» Ammonia/Nitrogen Removal Processes
17