What can we do to get better neutron dose equivalent measurements? David Thomas NPL Workshop 26th October 2006 What are we trying to do? Determine effective dose Effective dose, E, is the weighted sum of various organ doses, HT E = ∑wT ⋅ HT T Oesophagus Thyroid Lung Breast Bone marrow Colon Liver Stomach Bladder Gonads Skin Bone surface Remainder 2 0.05 0.05 0.12 0.05 0.12 0.12 0.05 0.12 0.05 0.20 0.01 0.01 0.05 NPL Workshop 26th October 2006 2 Conversion coefficient (pSv cm ) Effective dose conversion coefficients E(A-P) E(P-A) E(ROT) E(RLAT) E(ISO) 100 10 1 10 -9 ICRP74 10 -8 10 -7 10 -6 10 -5 10 -4 10 -3 10 -2 10 -1 10 0 10 1 10 2 Neutron energy (MeV) 3 NPL Workshop 26th October 2006 Survey instruments Ambient dose equivalent The ambient dose equivalent, H*(d), is the dose equivalent that would be produced by the corresponding expanded and aligned field, in the ICRU sphere at a depth of d mm on the radius opposing the direction of the aligned field. Expanded and aligned field • 4 ICRU sphere NPL Workshop 26th October 2006 Comparison of E and H*(10) 2 Conversion coefficient (pSv cm ) Conversion factors from ICRP Publication 74 or ICRU Report 57 for effective dose and ambient dose equivalent E (A-P) E (ROT) H*(10) 100 10 1 -9 10 -8 10 -7 10 -6 10 -5 10 -4 10 -3 10 -2 10 -1 10 0 10 1 10 2 10 Neutron energy (MeV) File ICRP74.opj 5 NPL Workshop 26th October 2006 Typical area survey instrument response functions H*(10) response Under- and over-read for samples of area survey meters 10 1 10 0 Thermal Harwell 0949 (Leake detector) Bertold LB6411 10 -1 10 -3 10 -2 10 -1 10 0 10 1 10 2 10 3 10 Neutron energy (eV) 6 4 10 5 10 6 10 7 Dosemeters.opj NPL Workshop 26th October 2006 Implications of area survey instrument response functions 1 10 Harwell 0949 (Leake detector) Berthold LB6411 3.5 3.0 2.5 1 2.0 Dose equivalent spectrum H*(10) near a transport flask Clab D 1.5 1.0 Dose equivalent response Ambient dose equivalent H*(10) 4.0 0.5 0.0 0.1 -3 10 -2 10 -1 10 0 10 1 10 2 10 3 10 Neutron energy (eV) 7 4 10 5 10 6 10 7 10 NPL Workshop 26th October 2006 Implications of area survey instrument response functions 2 Leake counter 2.0 Field types Gas cooled reactor PWR Simulated workplace Fuel cycle Transport flasks MOx fabrication Source fabrication Calibration 1.8 Reading/H*(10) 1.6 1.4 1.2 1.0 0.8 0.6 10 100 2 H*(10)/Φ (pSv cm ) 8 NPL Workshop 26th October 2006 Personal dose equivalent The personal dose equivalent, Hp(d), is the dose equivalent in soft tissue, at a depth of d mm, below a specified point on the body. • Body or slab phantom Note : in ICRU Report 47, the ICRU has considered the definition of the personal dose equivalent to include the dose equivalent at a depth, d, in a phantom having the composition of ICRU tissue. Then, Hp(10), for the calibration of personal dosemeters, is the dose equivalent at a depth of 10 mm in a phantom composed of ICRU tissue, but of the size and shape of the phantom used for calibration (a 30cm x 30cm x 15cm parallelepiped), and the conversion coefficients, hp,slab(10), are calculated for this configuration. 9 NPL Workshop 26th October 2006 Personal dose equivalent conversion coefficients Conversion coefficients, from ICRP Publication 74 or ICRU Report 57, for personal dose equivalent 2 Conversion coefficient (pSv cm ) 1000 o hp(10,0 ) o 100 hp(10,15 ) o hp(10,45 ) o hp(10,75 ) 10 1 -9 10 -8 10 -7 10 -6 10 -5 10 -4 10 -3 10 -2 10 Neutron energy (MeV) 10 -1 10 0 10 1 10 File ICRP74.opj NPL Workshop 26th October 2006 Personal dose equivalent conversion coefficients and E Conversion coefficients, from ICRP Publication 74 or ICRU Report 57, for personal dose equivalent o hp(10,0 ) and for E(A-P) 2 Conversion coefficient (pSv cm ) 1000 100 E(A-P) o hp(10,0 ) 10 1 -9 10 ICRP74 -8 10 -7 10 -6 10 -5 -4 10 10 -3 10 -2 10 -1 10 0 10 1 10 Neutron energy (MeV) 11 NPL Workshop 26th October 2006 Neutron personal dose equivalent response 100 Hp,m(10)/Hp,c(10) 10 1 0,1 0,01 -8 10 0° ALOKA PDM-313 60° ALOKA PDM-313 10 -3 10 -1 10 1 En / MeV 12 NPL Workshop 26th October 2006 Neutron personal dose equivalent response 100 0° Saphydose-n Hp,m(10)/Hp,c(10) 10 1 0,1 0,01 -8 10 10 -3 10 -1 En / MeV 13 10 1 NPL Workshop 26th October 2006 Neutron personal dose equivalent response 14 NPL Workshop 26th October 2006 Requirements • Several approaches to improving neutron dosimetry, e.g. ¾ Improved survey instruments and dosemeters ¾ Improved knowledge of workplace spectra ¾ Improved knowledge of device response functions ¾ Education of the practitioners – explaining the problems • What is the most important? 15 NPL Workshop 26th October 2006 End 16 NPL Workshop 26th October 2006 0.8 10 Ambient dose equivalent H*(10) 0.7 0.6 0.5 0.4 1 0.3 Dose equivalent spectrum H*(10) near a transport flask Clab D 241 Am-Be 0.2 Dose equivalent response Harwell 0949 (Leake detector) Berthold LB6411 0.1 0.0 0.1 -3 10 -2 10 -1 10 0 10 1 10 2 10 3 10 Neutron energy (eV) 17 4 10 5 10 6 10 7 10 NPL Workshop 26th October 2006 Neutron spectra 0.55 Neutron fluence and dose equivalent spectra outside containment for a typical gas-cooled reactor 252 compared to a Cf dose equivalent spectrum E.Φ(E) or H*(10) normalised to unity 0.50 0.45 0.40 252 Cf 0.35 0.30 0.25 0.20 Fluence H*(10) 0.15 0.10 0.05 0.00 -3 10 -2 10 -1 10 0 10 1 10 2 10 3 10 Neutron energy (eV) 18 4 10 5 10 6 10 7 10 NPL Workshop 26th October 2006 Personal dosemeters for neutrons • In general there are two mechanisms commonly used to detect neutrons in personal dosemeters – both active and passive: ¾ Detection of recoil protons from a hydrogenous layer, ¾ Detection of albedo neutrons from the body (albedo dosemeters). 19 NPL Workshop 26th October 2006 Proton recoil devices Proton recoil approach - used in etch track dosemeters, electronic dosemeters, etc. n • Converter layer p Detector By simply counting the number of recoil protons from a hydrogenous layer get a reasonable estimate of personal dose equivalent for fast (> 50 keV) neutrons 20 NPL Workshop 26th October 2006 Albedo devices Li(n,T) capture per source neutron -4 6 Albedo devices consist of 2 or more thermal neutron detectors with thermal neutron absorbing material shielding the detectors from the direct neutron field or from the backscattered neutrons. A careful choice of the combination of the signals from the detectors gives a dose equivalent response up to 1 to 10 keV. 1.6x10 6 Element 1 TLD + Li - shielded from body 6 Element 3 TLD + Li - shielded from direct -4 1.2x10 -5 8.0x10 -5 4.0x10 0.0 Combined response for: 1 x TLD element 1 and 2 X TLD element 3 -5 Body Hp(10) response Thermal shield 1.6x10 albedo neutrons Direct neutrons -5 1.2x10 -6 8.0x10 -6 4.0x10 0.0 -8 10 Thermal neutron detector -7 10 -6 10 -5 10 -4 10 -3 10 -2 10 -1 10 0 10 1 10 2 10 Neutron energy (MeV) 21 NPL Workshop 26th October 2006
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