`Bubble Fusion` Paper Generates A Tempest in a Beaker

NEW S
cold fusion, in which some researchers erroneously claimed to have seen fusion catalyzed by a lump of palladium metal.
It is against this backdrop that
Taleyarkhan, Richard Lahey, a nuclear engineer at Rensselaer Polytechnic Institute in
Troy, New York, and colleagues make their
case for tabletop fusion. The work relies on
a phenomenon known as acoustic cavitaThe heat from the controversy alone is kill publication of the paper.
nearly enough to trigger a nuclear reaction.
Unlike nuclear fission, fusion is very dif- tion, in which sound waves rattling through
This week in Science (p. 1868), scientists ficult to initiate. Only at extremely high pres- a fluid create tiny bubbles and then cause
led by nuclear engineer Rusi Taleyarkhan sures and temperatures can atomic nuclei them to expand and compress. Under cerof Oak Ridge National Laboratory in Ten- slam together hard enough to merge, or fuse, tain conditions, those bubbles give off tiny
nessee claim to have seen evidence for nu- releasing energy in the process. A hydrogen flashes of light as they collapse, a pheclear fusion in a beaker of organic solvent. bomb achieves those pressures by first setting nomenon known as sonoluminescence.
That stunning claim, if true, could eventu- off a small fission bomb to get the process Many scientists believe that the bubbles,
ally have important consequences for nu- going. A handful of labs are gearing up to do compressed by the acoustic waves, reach
clear proliferation and energy production. the same with enormous lasers or powerful great temperatures and pressures. Some
But other scientists, citing another Oak magnetic fields (Science, 18 August 2000, p. speculate that under the right conditions,
Ridge experiment that seems to belie the 1126; 25 January 2002, p. 602). Small-scale those bubbles might—just might—provide
claim, are likening the paper to cold fu- “tabletop” fusion reactions, meanwhile, have conditions extreme enough to trigger fusion.
Taleyarkhan and colleagues set out to
sion. Adding to the brouhaha are a series remained far out of reach. And the scientific
of exchanges in which the magazine’s edi- community is still wiping egg off its face test that idea. Starting with a small cylinder
tors say outsiders tried to revise, delay, or from the 1989 debacle involving so-called of acetone in which all the hydrogen atoms
had been replaced with deuteriVacuum pump
um (a heavy breed of hydrogen
that has an extra neutron), the
team subjected the cylinder to
0.82 MeV 2.45 MeV
acoustic waves. At the same
+
time, they zapped the deuterated
Plastic/liquid
acetone with high-speed neuHelium neutron
scintillator
trons. The neutrons, which each
Deuterium
carried about 14 million electron volts (MeV) of energy,
struck the molecules of acetone
proton
Tritium
and gave them a punch of energy. “You get vaporization on a
+
small scale,” says Taleyarkhan.
1.01 MeV 3.02 MeV
The pockets of vapor nucleate
bubbles and cause them to grow
to about 1 millimeter across—
much bigger than they would
normally get in an acoustic
field. “They grow to be mamPhotomultiplier
moths,” he says. “You can actutube
Neutron source
ally see the bubbles.”
The catastrophic collapse of
a millimeter-sized bubble to a
few nanometers across heats
Microphone
the deuterated acetone to the
Acoustic wave
point at which deuterium atoms
generator
collide and fuse, the authors argue. “I thought, doggone! I’m
depressed I hadn’t done that experiment,” says Lawrence
Crum, a sonoluminescence exChamber filled with test fluid
pert at the University of WashPop! Embattled paper suggests deuterium nuclei undergo fusion inside sonoluminescent bubbles.
ington, Seattle, who acknowlNUCLEAR FUSION
‘Bubble Fusion’ Paper Generates
A Tempest in a Beaker
1808
8 MARCH 2002
VOL 295
SCIENCE
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CREDITS: (LEFT TO RIGHT) R. TALEYARKHAN; R. LAHEY
FOCUS
edges that he reviewed the paper for
Science. (The magazine’s editors did not
reveal the identities of the paper’s reviewers to Science’s news staff.)
When deuterium fuses with deuterium,
two equally probable things can happen.
First, the two can form an atom of hydrogen3, or tritium, while the extra proton zooms
off with about 3.02 MeV (and in the apparatus would be quickly absorbed by the acetone). On the other hand, the two can make a
helium-3 nucleus, while the extra neutron
flies off with 2.45 MeV; unlike the proton, it
would escape the acetone bath. Taleyarkhan
and his colleagues claim to have detected
neutrons whose energies are consistent with
2.45-MeV emissions, and they also claim to
have seen extra tritium in the solution. Both
effects disappear when they replace deuterated acetone with acetone, turn off the acoustic waves, or change the temperature of the
bath to make it less favorable for cavitation.
Some physicists have greeted the work
with deep skepticism. “The paper’s kind of
a patchwork, technically, and each of the
patches has a hole in it,” says Mike Moran,
a physicist at Lawrence Livermore National
Laboratory in California who has performed similar experiments with deuterated
water. Moran says electromagnetic interference by an acoustic-wave generator raised
false hopes of fusion in his own lab, and he
worries that something similar may have
happened at Oak Ridge. A beaker full of
deuterated acetone, he says, should show
an increase in tritium when irradiated by
fast neutrons, even without cavitation—
whereas Taleyarkhan’s data show an enhancement only while the solution is cavitating. “It’s an inconsistency in the data,”
according to Moran.
Tougher criticism comes from Dan
Shapira and Michael Saltmarsh, two physicists who are also at Oak Ridge. Late in
May, after the lab had given Taleyarkhan
and colleagues the go-ahead to submit their
results to Science, Lee Riedinger, the lab’s
deputy director for science and technology,
asked Shapira and Saltmarsh to check the
work with a more sensitive neutron detector.
They concluded that Taleyarkhan’s results
had been an illusion.
“There’s no evidence for any neutron excess due to fusion,” Saltmarsh says. “If the
tritium results in Taleyarkhan’s paper are correct, and if you assume all the tritium is due
to d-d fusion, then you expect a 10-fold increase in the neutron signal. We see a 1% ef-
fect.” One possibility is that the extra neu- headed the Department of Energy’s science
trons are left over from the 14-MeV neutrons office for 2 years in the early 1990s, adds that
fired into the cylinder, eventually winding up he is also trying to save the scientific commuin the detector after skittering about the nity from another embarrassing fiasco. “I saw
room. To rule out that scenario, says Salt- it happen with cold fusion. If we’re really unmarsh, they timed the flashes of light from lucky, Dan Rather will talk about it on the
the bubbles and compared them with the ar- [CBS] evening news and intone how, provirival times of the extra neutrons. The effect dentially, the energy problem has been solved.
disappeared. “We didn’t see any evidence for We as a community will look stupid.”
a coincidence between neutrons, gamma
Garwin says that he was troubled by the
rays, and light emissions above background,” quality of the research. The version of the
Saltmarsh says.
Taleyarkhan and
colleagues dispute
Saltmarsh’s interpretation of the data and are
posting the details of
their objections on the
Web. Riedinger characterizes the ongoing dispute as “an active dialogue about what could
be wrong with either
set of measurements.”
At the same time, he
compliments Taleyarkhan’s abilities and calls
the work “very novel
and interesting.”
Sharper comments Deuterated duo. Rusi Taleyarkhan (left) and Richard Lahey hope others
began to pepper will soon repeat their experiment.
Science’s editors as
Taleyarkhan’s paper
neared publication. Don Kennedy, the paper he saw described how the authors
editor-in-chief of Science, says that Oak constantly adjusted the experimental setup
Ridge officials tried to withdraw their per- to keep it tuned properly—conditions ripe
mission to publish the paper. “There was for allowing unconscious bias to seep into
certainly pressure from Oak Ridge to delay, the data. Given these concerns, he says, “it
if not to kill, the paper,” says Kennedy. “I’m would be unfortunate if Science magazine
annoyed at the intervention, and I’m an- were to take any position on its correctness.”
noyed at the assumptions that nonauthors
Kennedy says that publication in Science
had the authority to tell us we couldn’t pub- certifies only that Taleyarkhan’s paper has
lish the paper.”
cleared the magazine’s own peer-review and
As knowledge of the pending paper editing process. After that, it’s up to the scispread, scientists outside Oak Ridge joined entists. “We’re not wise enough to certify
the fray. Late in February, William Happer, a that every claim will stand up to the active
physicist at Princeton University, and effort of replication,” says Kennedy.
Richard Garwin of IBM’s Thomas J. Watson
The importance of replication, apparentlaboratory in Yorktown Heights, New York, ly, is one of the few things on which everyeach wrote Kennedy a letter about the paper. body can agree. “There’s some small chance
They say they were simply encouraging that they’re right,” says Happer. “It should be
Science to publish the Shapira and Saltmarsh published. The truth always comes out.”
data as well, or at least not to hype the paper.
Taleyarkhan takes the same position, al“I like Science,” Happer says. “I’m a though he hopes for the opposite result. “I’m
member of AAAS, and I don’t want them to looking forward to helping people reproduce
shoot themselves in the foot—or some other the experiment,” he says. But until then, conbody part. All I told [Kennedy] was, for God’s fusion, not fusion, is likely to reign.
–CHARLES SEIFE
sake, don’t put it on the cover.” Happer, who
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