VOLUME 80, NUMBER 17 PHYSICAL REVIEW LETTERS 27 APRIL 1998 Hall Effect in SN and SNS Junctions F. Zhou* and B. Spivak Physics Department, University of Washington, Seattle, Washington 98195 (Received 17 March 1997) Hall effect in SN and SNS junctions is considered. It is shown that at low temperatures the Hall voltage is significantly suppressed as compared to its normal metal value. The time dependence of the Hall voltage in SNS junctions has a form of narrow pulses with the Josephson frequency. [S00319007(98)05980-8] PACS numbers: 74.50. + r, 05.20. – y, 82.20. – w Recent progress in microfabrication technology has rekindled the interest to low temperature proximity effect in superconductor–normal-metal (SN) junctions [1–10]. In this paper we consider the Hall effect in superconductor–normal-metal and superconductor–normal-metal– superconductor (SNS) junctions. At low temperatures T ø D, quasiparticles with energies e ø D cannot tunnel from the metal into the superconductor. Here D is the value of the gap in the superconductors. On the other hand the tunneling of electron pairs, which is known as Andreev reflection, is possible. This gives rise to a coherence between electrons and holes inside the metal, which p extends over distances of the order of Le Dye ¿ l. 1 Here D 3 yF l is the electron diffusion coefficient, l is the elastic mean free path, and yF is the Fermi velocity. Consequently, the wave packets which carry the current in the metal are coherent superpositions of electron and hole wave functions. At p T ø 1yt yF yl the packets’ size is of order LT DyT ¿ l and their effective charge is much smaller than the electron charge e. The above mentioned electron-hole coherence manifests itself in experimentally observable effects. For example, the density of states in the metal near the SN boundary nse, r$ d is significantly suppressed as compared with the bulk metal value n0 m2 yF [8–10]; the low temperature resistance of the SN junction and the electric field distribution near the SN boundary turn out to be very sensitive to the phase breaking rate in the metal [4–7]. The suppression of the effective charge should also lead to a suppression of the Hall effect. We show below that the Hall voltage in SN junctions measured with the help of leads 1,2 shown in Fig. 1(a) is indeed significantly suppressed as compared to its bulk metal value. It is worth mentioning here that at zero temperature the resistance of a long SN junction is approximately the same as the resistance of the normal segment [4–7]. Therefore the suppression of the Hall voltage is not directly connected to the suppression of the electron density of states near the SN boundary [8–10]. We also show that the Hall voltage in SNS junctions exhibits oscillations of its amplitude with Josephson frequency and with no oscillations of the sign. It is different from the behavior of supercurrent through the junction which at a given voltage oscillates both in amplitude and in sign. In this article we neglect the electron-electron interaction in metal and are interested only in effects linear in voltage applied to the junction. In the “clean limit” when Dt, Tt ¿ 1, the kinetic scheme describing Hall effect in superconductors was developed in [11,12]. In this limit, however, the above mentioned proximity effect leads only to small corrections to the value of the Hall voltage in metal. To describe the Hall effect in a metal near the SN boundary in the “dirty limit” when T ø D, 1yt we use the following set of equations analogous to that in [13,14]: J$ J$ s 1 J$ n 1 J$ H , D Z D Z J$ s n0 def0 sed Trssz fG R =G R 2 G A =G A gd, n0 de=f1 sed Trs1 2 sz G R sz G A d , J$ n 4 4 Z vc t J$ H Dn0 de e$ b 3 =f1 3 Trhs1 1 sz G R sz G R 2 G A G R 2 sz G A sz G R d sG R sz 2 G A sz dj ; 16 eFsr$ d Z def1 se, r$ dnse, r$ d, nse, r$ d 1 Trssz G R 2 G A sz d ; 2 R ehG R sz 2 sz G R j 1 D≠ ? sG R ≠G R d Iph ; (1) (2) (3) =hTrs1 2 sz G R sz G A d=f1 1 Trfsz sG R ≠G R 2 G A ≠G A dgf0 1 vc t e$ b 3 =f1 Trfs1 1 sz G R sz G R 2 G A G R 2 sz G A sz G R d sG R sz 2 sz G A dgj Trssz Iph d . 0031-9007y98y80(17)y3847(4)$15.00 © 1998 The American Physical Society (4) 3847 VOLUME 80, NUMBER 17 PHYSICAL REVIEW LETTERS Here J$ s , J$ n , J$ H are the supercurrent density, normal current density, and the Hall current density, respectively, f0 tanhsey2kT d is the Fermi distribution function, vc eHymc is the cyclotron frequency; H is the magnetic field, and e$ b is the unit vector in the direction of magnetic field; F 1y2≠t x 1 f, f, and x are the gauge invariant scalar potential, electrical potential, and phase of anomalous Green’s function, respectively; sz is the Pauli matrix, ≠X =X 2 issz X 2 Xsz dA$ is the covariant derivative, A$ is the vector potential of the magnetic field; G R,A are retarded and advanced Green’s functions which are matrices in the Nambu space µ R,A ∂ g F R,A R,A G se, r$ d , (5) 2F R,A gR,A gR,A se, r$ d and F R,A se, r$ d are normal and anomalous Green’s functions, respectively. Thus the set of equations consists of electroneutrality condition Eq. (2), the Usadel equation for retarded and advanced Green’s functions G R,A Eq. (3), and the kinetic equation Eq. (4) for the distribution function f1 se, r$ d which describes the imbalance of populations between the electron and hole branches of R ø isz tin spectrum [13,14]. The scattering integrals Iph and Trssz Iph d describe the broadening of the spectrum and the imbalance charge relaxation due to inelastic processes. In Eqs. (3),(4), we take into account that in noninteracting metal the order parameter and the supercurrent are zero. In the zeroth order approximation in the parameter vc t, these equations were derived in [13]. However, to describe the Hall effect one has to keep terms linear in vc t. The problem of the Hall effect in the mixed state of superconductors was addressed recently in [12,15,16]. We derive Eqs. (1),(3) which include the contributions linear in vc t using the same procedure as in [11,12,15,16]. Let us now consider the Hall effect in the SN junctions shown in Fig. 1(a). We assume that the magnetic field is smaller than the critical one and does not penetrate into the superconductor. Taking into account the normalization condition fgR se, r$ dg2 F2R se, r$ dF1R se, r$ d 1 1 one 27 APRIL 1998 can express gR , F R , and Eqs. (1)–(4) in the form cos use, r$ d gR se, r$ d, sin use, r$ d iF1R se, r$ d , µ ∂ D 2 1 sin used 2 = used 1 ie 2 2 tin µ ∂ D eH 2 2 x sin 2u 0 , 4 h̄c (6) (7) = ? hcosh2 u2 =f1 1 tvc e$ b 3 =f1 cos u1 cosh3 u2 j 0 , Z J$ Dn0 dehcosh2 u2 =f1 1 tvc e$ b 3 =f1 cos u1 cosh3 u2 j , (8) where u u1 1 iu2 is the complex variable. We have chosen A$ e$ y Hx. The boundary conditions for Eqs. (7),(8) have the forms [17] $ t sinfuse, 01 d 2 use, 02 dg , D n$ ? =use, Rd D cosh u22 ? =f1 tyF hf1 s02 d 2 f1 s01 dj 3 cosh u2 s01 d cosh u2 s02 d 3 cosfu1 s01 d 2 u1 s02 dg , f1 s0d 0 , f1 se, x `d 2eV ≠e f0 sed . (9) Here n$ and t are the unit vector perpendicular to the boundary and the transmission coefficient of the boundary, respectively. Indexes 1, 2 indicate two sides of the SN or NNp interface [Fig. 1(a)]. Np represents lead 1,2. Inside the superconductor use ø Dd py2 while inside the bulk metals u 0. Solving Eqs. (8),(9) in zeroth order approximation in vc t we get the expressions for the conductance GSN I0 yU0 of the junction shown in Fig. 1(a) [4–7] measured by the two probe method and the conductance Gp measured between lead 1 and lead 2. (Here I0 is the current L L D D FIG. 1. (a) Temperature dependence of Hall voltage in SN junction. a p maxh L0t , L0 j, T p minh L20 , L20 j. (b) Time dependence t of Hall voltage in SNS junctions with geometry shown in the inset, t p t0 T yEc ø t0 1y2eU0 . U0 is applied along X direction and UH is measured along Y direction in normal metals. 3848 VOLUME 80, NUMBER 17 PHYSICAL REVIEW LETTERS 27 APRIL 1998 through the junction and U0 is the voltage across the junction.) That is Z Z 1 1 de≠e f0 GSN sTd S0 s0 de≠e f0 , Gp sT d Sp sp , LS sed 2Lp sed (10) where LS sed Lp sed Z L0 1 Lt dx , 1 2 cosh u2 se, 0d sin u1 se, 0d cosh u 0 2 se, xd Z Lp Ltp 1 , dy 1 2 cosh u2 se, Ld cosh u2p se, 0d cosfu1 se, Ld 2 u1p se, 0dg se, yd cosh u2p 0 (11) S0,p are the cross sections of the sample and the leads, s0,p , D0,p are the Drude conductivities and diffusion constants in the sample and leads; Lt D0 yt0 yF , Ltp Dp ytp yF are the length characterizing SN and NNp boundaries, t0 and tp are the transmission coefficients for SN and NNp boundaries, up se, yd is the solution of Eq. (7) inside the leads. In the first order approximation in vc t we get an expression relating the Hall current IH and Hall voltage UH measured by leads 1,2 Z S p sp 1 cos u1 se, Ld d de IH Gp sT dUH sT d tvc I0 (12) ≠e f0 . GSN sT d Lp sed LS sed cosh u2 se, Ld Here d is the width of the junction (see Fig. 1). The values of u1 , u2 , and UH (as well as GSN and Gp ) depend on the processes breaking the electron-hole coherence inside the sample and in the leads. Therefore, they are very sensitive to the ratio between parameters L0 , LT , Lt , Ltp [4,5,7]. The solution of Eq. (7) in the metal for SN junctions when L0 ¿ Lt with the corresponding boundary conditions in Eq. (9) is [7] 8p p L 1L > 2 2 tL0 , Lt , L ø L0 ø Le ; > 2 <p Lt 1L L t , L ø L e ø L0 ; (13) use, Ld p2 2 s1 2 id Le , > > 2 ps11idL x e : p expf2s1 2 id g, L ø L ø L . 4Lt The most interesting results appear in the cases when the processes which break the electron-hole coherence are not effective and the value of u1 sT , Ld is close to py2. At small T and large t 8 < maxh Lt , Lt j, L ø L ø L ; UH t T L 0 LT ~ (14) : maxh L , L j, Lt ø L ø LT . UHN L0 LT Here UHN vc tdI0 yS0 s0 is the Hall voltage measured by the leads 1,2 in the absence of the proximity effect. The main feature of Eq. (14) is that UH is significantly suppressed as compared with UHN [see Fig. 1(a)]. At high temperatures when LT ø Lt or L the proximity effect gives only small corrections to UHN Ω 2 2æ UHN 2 UH LT LT (15) ~ min 2 , 2 ø 1 . UHN Lt L The above results are obtained in the limit p of low magnetic field when LH ø LT . Here LH F0 yH is the magnetic length, F0 is flux quantum. In the opposite limit one should substitute LT for LH in Eqs. (14),(15). As we have mentioned the value of UH is very sensitive to the nature of the leads. The requirement that the leads do not contribute to the breaking of the electron-hole coherence is d ø Ltp , Lt ø L0 . 2 Le e t 0 Let us now turn to the discussion of the Hall effect in SNS junctions. In this case the ac Josephson effect causes the values of usr$ , x0 d and nsr$ , x0 d to be time dependent. At small U0 these dependences adiabatically follow the corresponding time dependence of the order parameter phase difference x0 across the junction: ≠t x0 std 2eU0 . For simplicity let us consider the case of a thin junction when d ø LH when one can neglect any y dependence of x0 along the junction. It is well known that at x0 0, the energy dependence of nsed cos u1 sed cosh u2 sed exhibits a gap Eg sx0 0d , Ec DyL02 [3]. The x0 dependences of u, n, and Eg were calculated in [10,18]. It was shown that the value of the gap Eg monotonically decreases with x0 and closes at x0 p. Hence cos u1 sed 0 when e # Eg sx0 d. In two limiting cases when x0 is close to p or 0 Eg sx0 d is determined by [18] Ω s1 2 Cx02 d, x0 ø p ; Eg sx0 d Eg s0d (16) C1 sp 2 x0 d, p 2 x0 ø p . Here C and C1 are of the order of unity. It follows from Eq. (12) that the Hall voltage UH is a periodical function of time with a period 1y2eU0 . At low temperatures T ø Ec the value of UH std is exponentially small except when the gap is small Eg fx0 stdg , T . As a result UH std 3849 VOLUME 80, NUMBER 17 PHYSICAL REVIEW LETTERS consists of short pulses of duration t p , TyEc eU0 with maximums of the order of UHN [see Fig. 1(b)]. Let tn be the time when the nth maximum of UH std occurs. Then at t p ø jt 2 tn j ø 1y2eU0 , µ ∂ jt 2 tn j . (17) UH std , UHN exp 2 tp The main contribution to the Hall current averaged over the period of oscillations comes from the time intervals jt 2 tn j , t p ø 1yU0 and as a result T UHN . (18) Ec We would like to mention the difference in the temperature dependences in the SN and SNS cases. In the first p case UH , T, while in the second case UH , T. Let us note that the time dependence of the resistance of the junction exhibit peaks which are similar to the above considered peaks of the Hall voltage. In addition to the quasiparticle’s contribution to the Hall current in SNS junctions there is another contribution which can be associated with the supercurrent [15,16]. We believe, however, that in the limit when d ø LH , the supercurrent part of the Hall current does not contribute to the Hall voltage. In the case of SN junctions the supercurrent contribution to the Hall current does not exist. In this paper we considered the limit eU0 ø 1yte when it is possible to neglect nonequilibrium corrections to the quasiparticle distribution function inside the normal metal. In the opposite limit the quasiparticle distribution in the metal at e , Ec becomes nonequilibrium and as a result the duration of the pulses t p becomes of the order of seU0 d21 . The above results were obtained for the quantities averaged over realizations of random potential. We are planning to consider mesoscopic contributions in UH elsewhere. We acknowledge useful discussions with B. Altshuler, A. I. Larkin, and B. 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