Validation report for the inverted CO2 fluxes, v15r2 version 1.1 Issued by: CEA Date: 04/07/2016 REF.: CAMS73_2015S1_ D73.1.2_201606 Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service This document has been produced in the context of the Copernicus Atmosphere Monitoring Service (CAMS). The activities leading to these results have been contracted by the European Centre for Medium-Range Weather Forecasts, operator of CAMS on behalf of the European Union (Delegation Agreement signed on 11/11/2014). All information in this document is provided "as is" and no guarantee or warranty is given that the information is fit for any particular purpose. The user thereof uses the information at its sole risk and liability. For the avoidance of all doubts, the European Commission and the European Centre for Medium-Range Weather Forecasts has no liability in respect of this document, which is merely representing the authors view. Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2 version 1.1 CEA (Frédéric Chevallier) Date: 04/07/2016 REF.: CAMS73_2015S1_ D73.1.2_201606 Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Contents: 1 Introduction .................................................................................................... 2 2 Inversion configuration ..................................................................................... 2 3 Evaluation ....................................................................................................... 7 3.1 Benchmarking using a poor man’s inversion .................................................. 7 3.2 Fit to the assimilated measurements ............................................................ 8 3.3 Fit to the independent measurements ........................................................... 8 Appendix A: Time series of the fit to the dependent surface measurements ............. 12 Appendix B: Time series of the fit to the independent measurements ...................... 24 Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service 1 Introduction The inversion system that generates the CAMS global CO2 atmospheric inversion product is called PYVAR. It has been initiated, developed and maintained at CEA/LSCE within the series of precursor projects GEMS/MACC/MACC-II/MACC-III (Chevallier 2016, and references therein). Here, we synthesize the evaluation of version 15r2 that was released in May 2016. Section 2 describes the PYVAR-CO2 configuration that was used and Section 3 presents the evaluation synthesis. 2 Inversion configuration The transport model in PyVAR-CO2 is the global general circulation model LMDZ in its version LMDZ5A (Locatelli et al. 2015), that uses the deep convection model of Emanuel (1991). This version corresponds to the one developed and used for the fifth phase of the Coupled Model Inter-comparison Project (CMIP5). Horizontal winds are nudged to the winds analysed by ECMWF, and the transport mass fluxes are computed once and for all, before being used off-line for tracer transport. This version has a regular horizontal resolution of 3.75o in longitude and 1.875o in latitude, with 39 hybrid layers in the vertical. The inferred fluxes are estimated in each horizontal grid point of the transport model with a temporal resolution of 8 days, separately for day-time and night-time. The state vector of the inversion system is therefore made of a succession of global maps with 9,200 grid points. Per month it gathers 73,700 variables (four day-time maps and four night-time maps). It also includes a map of the total CO2 columns at the initial time step of the inversion window in order to account for the uncertainty in the initial state of CO2. The prior values of the fluxes combine estimates of (i) gridded annual anthropogenic emissions (EC-JRC/PBL EDGAR version 4.2, and CDIAC), climatological monthly ocean fluxes, (Takahashi et al. 2009), monthly biomass burning emissions (GFED 4.1s until 2014 and GFAS for 2015) and climatological 3-hourly biosphere-atmosphere fluxes taken as the 1989-2010 mean of a simulation of the ORganizing Carbon and Hydrology In Dynamic EcosystEms model (ORCHIDEE, Krinner et al. 2005), version 1.9.5.2. The mass of carbon emitted annually during specific fire events is compensated here by the same annual flux of opposite sign representing the re-growth of burnt vegetation, which is distributed regularly throughout the year. The gridded prior fluxes exhibit 3hourly variations but their inter-annual variations are only caused by anthropogenic emissions. This feature was explicitly demanded by some users who wanted the interannual signals in the inverted natural fluxes to be strictly driven by the atmospheric measurements. Over land, the errors of the prior biosphere-atmosphere fluxes are assumed to dominate the error budget and the covariances are constrained by an analysis of mismatches with in situ flux measurements (Chevallier et al. 2006, 2012): temporal correlations on daily mean Net Carbon Exchange (NEE) errors decay exponentially with a length of one month but night-time errors are assumed to be uncorrelated with daytime errors; spatial correlations decay exponentially with a length of 500 km; standard deviations are set to 0.8 times the climatological daily-varying heterotrophic respiration flux simulated by ORCHIDEE with a ceiling of 4 gC∙m-2 per day. Over a full Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service year, the total 1-sigma uncertainty for the prior land fluxes amounts to about 3.0 GtC∙yr-1. The error statistics for the open ocean correspond to a global air-sea flux uncertainty about 0.5 GtC∙yr-1 and are defined as follows: temporal correlations decay exponentially with a length of one month; unlike land, daytime and night-time flux errors are fully correlated; spatial correlations follow an e-folding length of 1000 km; standard deviations are set to 0.1 gC∙m-2 per day. Land and ocean flux errors are not correlated. Observation uncertainty in the inversion system is dominated by uncertainty in transport modelling and is represented from the variance of the high frequency variability of the de-seasonalized and de-trended CO2 time series of the measurement at a given location. Version 15r2 analysed 37 years of surface measurements, from 1979 to 2015 in a single data assimilation window. The assimilated measurements are surface air-sample measurements of the CO2 dry air mole fraction made in 133 sites over the globe. The detailed list of sites is provided in Tables 1 and 2 and their location is displayed per year in Figure 1. The irregular space-time density of the measurements implies a variable constraint on the inversion throughout the 37 years, which is documented by the associated Bayesian error statistics. Figure 1: Location of the assimilated measurements over the globe for each year in v15r2. Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Locality (indentifier) Period Source Alert, Nunavut, CA (ALT) 1988-2014 WDCGG/ EC Amsterdam Island, FR (AMS) 1981-2011 LSCE Amsterdam Island, FR (AMS) 2012-2015 ICOS/ LSCE Argyle, Maine, US (AMT) 2003-2015 NOAA/ ESRL Anmyeon-do, KR (AMY) 1999-2014 WDCGG/ KMA Barrow, Alaska, US (BRW) 1979-2015 NOAA/ ESRL Candle Lake, CA (CDL) Centro de Investigacion de la Baja Atmosfera, ES (CIB) 2002-2012 WDCGG/ EC 2009-2015 NOAA/ ESRL Monte Cimone, IT (CMN) 1996-2014 WDCGG/ IAFMS Cape Ochi-ishi, JP (COI) 1995-2002 WDCGG/ NIES Cape Point, SA (CPT) 1993-2014 WDCGG/ SAWS Egbert, CA (EGB) Estevan Point, British Columbia, CA (ESP) 2005-2014 WDCGG/ EC 2009-2014 WDCGG/ EC East Trout Lake, CA (ETL) 2005-2014 WDCGG/ EC Frasedale, CA (FSD) 1990-2014 WDCGG/ EC Hateruma, JP (HAT) Hegyhatsal tower, 115m level, HU (HUN0115) 1993-2002 WDCGG/ NIES 1994-2014 WDCGG/ HMS Ivittuut, Greenland, DK (IVI) 2011-2014 ICOS/ LSCE Tenerife, Canary Islands, ES (IZO) 1984-2015 WDCGG/ AEMET Jubany, Antartica, AR (JBN) 1994-2009 WDCGG/ ISAC IAA Jungfraujoch, CH (JFJ) 2004-2014 WDCGG/ Univ. Of Bern K-puszta, HU (KPS) 1981-1999 WDCGG/ HMS Park Falls, Wisconsin, US (LEF) 2003-2015 NOAA/ ESRL WDCGG/ EC Lac La Biche, Alberta, CA (LLB) 2007-2014 Mace Head, County Galway, IE (MHD) 1992-2009 LSCE Mace Head, County Galway, IE (MHD) 2010-2015 ICOS/ LSCE Mauna Loa, Hawaii, US (MLO) 1979-2015 NOAA/ ESRL Minamitorishima, JP (MNM) 1993-2014 WDCGG/ JMA Neuglobsow, DE (NGL) Pallas-Sammaltunturi, GAW Station, FI (PAL) 1994-2013 WDCGG/ UBA 1999-2014 WDCGG/ FMI WDCGG/ CESI RICERCA Plateau Rosa, IT (PRS) 2000-2014 Puy de Dome, FR (PUY) 2000-2010 LSCE Puy de Dome, FR (PUY) 2011-2014 ICOS/ LSCE Ryori, JP (RYO) 1987-2015 WDCGG/ JMA Tutuila, American Samoa (SMO) 1979-2015 NOAA/ ESRL Sonnblick, AU (SNB) 1999-2014 WDCGG/ EEA South Pole, Antarctica, US (SPO) 1979-2015 NOAA/ ESRL Westerland, DE (WES) 1979-2013 WDCGG/ UBA Moody, Texas, US (WKT) 2003-2015 NOAAA/ ESRL Sable Island, CA (WSA) 1992-2014 WDCGG/ EC Yonagunijima, JP (YON) 1997-2015 WDCGG/ JMA Table 1: List of the continuous sites used in v15r2 together with the period of coverage (defined as the period between the first sample and the last one), and the data source. Each station is identified by the name of the place, the corresponding country (abbreviated) and the code used in the corresponding database. Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Locality (indentifier) Period Source Alert, Nunavut, CA (ALT) 1985-2015 NOAA/ ESRL Alert, Nunavut, CA (ALT) 1979-2014 WDCGG/ EC Alert, Nunavut, CA (ALT) 1991-2014 WDCGG/ CSIRO Amsterdam Island, FR (AMS) 1979-1990 NOAA/ ESRL Amsterdam Island, FR (AMS) 2003-2015 LSCE Ascension Island, GB (ASC) 1979-2015 NOAA/ ESRL Assekrem, DZ (ASK) 1995-2015 NOAA/ ESRL St. Croix, Virgin Islands, USA (AVI) 1979-1990 NOAA/ ESRL Terceira Island, Azores, PT (AZR) 1979-2015 NOAA/ ESRL Baltic Sea, PL (BAL) 1992-2011 NOAA/ ESRL Bering Island, RU (BER) 1986-1994 WDCGG/ MGO Begur, ES (BGU) 2000-2014 LSCE/ IC·3 Baring Head, NZ (BHD) 1999-2015 NOAA/ESRL Baring Head, NZ (BHD) 1979-2014 WDCGG/ NIWA St. Davids Head, Bermuda, GB (BME) 1989-2009 NOAA/ ESRL Tudor Hill, Bermuda, GB (BMW) 1989-2015 NOAA/ ESRL Barrow, Alaska, US (BRW) 1979-2015 NOAA/ ESRL Cold Bay, Alaska, US (CBA) 1979-2015 NOAA/ ESRL Cape Ferguson, AU (CFA) 1991-2014 WDCGG/ CSIRO Cape Grim, Tasmania, AU (CGO) 1984-2015 NOAA/ ESRL Churchill, CA (CHL) Christmas Island, Republic of Kiribati (CHR) 2007-2014 WDCGG/ EC 1984-2014 NOAA/ ESRL Cape Meares, Oregon, US (CMO) 1982-1998 NOAA/ ESRL Crozet Island, FR (CRZ) 1991-2015 NOAA/ ESRL Cape St. James, CA (CSJ) 1979-1992 WDCGG/ EC Casey Station, AU (CYA) Drake Passage (DRP) 1996-2013 2003-2015 WDCGG/ CSIRO Easter Island, CL (EIC) Estevan Point, British Columbia, CA (ESP) Estevan Point, British Columbia, CA (ESP) 1994-2015 NOAA/ ESRL 1992-2014 WDCGG/ EC 1993-2001 WDCGG/ CSIRO Finokalia, Crete, GR (FIK) 1999-2015 LSCE NOAA/ ESRL Mariana Islands, Guam (GMI) 1979-2015 NOAA/ ESRL Dwejra Point, Gozo, MT (GOZ) 1993-1998 NOAA/ ESRL Halley Station, Antarctica, GB (HBA) 1983-2014 NOAA/ ESRL Hanle, IN (HLE) 2000-2013 LSCE Hohenpeissenberg, DE (HPB) 2006-2015 NOAA/ ESRL Humboldt State University, US (HSU) 2008-2014 NOAA/ ESRL Hegyhatsal, HU (HUN) 1993-2015 NOAA/ ESRL Storhofdi, Vestmannaeyjar, IS (ICE) 1992-2015 NOAA/ ESRL Grifton, North Carolina, US (ITN) 1992-1999 WDCGG/ ESRL Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Ivittuut, Greenland, DK (IVI) 2007-2014 LSCE Tenerife, Canary Islands, ES (IZO) 1991-2015 NOAA/ ESRL Key Biscayne, Florida, US (KEY) 1979-2015 NOAA/ ESRL Kotelny Island, RU (KOT) 1986-1993 WDCGG/ MGO Cape Kumukahi, Hawaii, US (KUM) 1979-2015 NOAA/ ESRL Sary Taukum, KZ (KZD) 1997-2009 NOAA/ ESRL Plateau Assy, KZ (KZM) 1997-2009 NOAA/ ESRL Lac La Biche, Alberta, CA (LLB) 2008-2014 NOAA/ ESRL Lulin, 2006-2014 NOAA/ ESRL Lampedusa, IT (LMP) TW (LLN) 2006-2015 NOAA/ ESRL Ile grande, FR (LPO) 2004-2013 LSCE Mawson, AU (MAA) 1990-2014 WDCGG/ CSIRO Mould Bay, Nunavut, CA (MBC) 1980-1997 NOAA/ ESRL High Altitude GCOC, Mexico (MEX) 2009-2015 NOAA/ ESRL Mace Head, County Galway, IE (MHD) 1991-2015 NOAA/ ESRL Mace Head, County Galway, IE (MHD) 1996-2015 LSCE Sand Island, Midway, US (MID) 1985-2015 NOAA/ ESRL Mt. Kenya, KE (MKN) 2003-2011 NOAA/ ESRL Mauna Loa, Hawaii, US (MLO) 1979-2015 NOAA/ ESRL Macquarie Island, AU (MQA) Farol De Mae Luiza Lighthouse, BR (NAT) 1990-2014 WDCGG/ CSIRO 2011-2015 NOAA/ ESRL Gobabeb, NA (NMB) 1997-2015 NOAA/ ESRL Niwot Ridge, Colorado, US (NWR) 1979-2015 NOAA/ ESRL Olympic Peninsula, WA, USA (OPW) 1984-1990 NOAA/ ESRL Ochsenkopf, DE (OXK) Pallas-Sammaltunturi, GAW Station, FI (PAL) 2003-2015 NOAA/ ESRL 2001-2015 NOAA/ ESRL Pic du Midi, FR (PDM) 2001-2015 LSCE Pacific Ocean, 0N (POC000) 1987-2015 NOAA/ ESRL Pacific Ocean, 5N (POCN05) 1987-2015 NOAA/ ESRL Pacific Ocean, 10N (POCN10) 1987-2015 NOAA/ ESRL Pacific Ocean, 15N (POCN15) 1987-2015 NOAA/ ESRL Pacific Ocean, 20N (POCN20) 1987-2015 NOAA/ ESRL Pacific Ocean, 25N (POCN25) 1987-2015 NOAA/ ESRL Pacific Ocean, 30N (POCN30) 1987-2015 NOAA/ ESRL Pacific Ocean, 5S (POCS05) 1987-2015 NOAA/ ESRL Pacific Ocean, 10S (POCS10) 1987-2015 NOAA/ ESRL Pacific Ocean, 15S (POCS15) 1987-2015 NOAA/ ESRL Pacific Ocean, 20S (POCS20) 1987-2015 NOAA/ ESRL Pacific Ocean, 25S (POCS25) 1987-2015 NOAA/ ESRL Pacific Ocean, 30S (POCS30) 1987-2015 NOAA/ ESRL Pacific Ocean, 35S (POCS35) 1987-2015 NOAA/ ESRL Palmer Station, Antarctica, US (PSA) 1979-2015 NOAA/ ESRL Point Arena, California, US (PTA) 1999-2011 NOAA/ ESRL Puy de Dome, FR (PUY) 2001-2015 LSCE Ragged Point, BB (RPB) 1987-2015 NOAA/ ESRL South China Sea, 3N (SCSN03) 1991-1998 NOAA/ ESRL Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service South China Sea, 6N (SCSN06) 1991-1998 NOAA/ ESRL South China Sea, 9N (SCSN09) 1991-1998 NOAA/ ESRL South China Sea, 12N (SCSN12) 1991-1998 NOAA/ ESRL South China Sea, 15N (SCSN15) 1991-1998 NOAA/ ESRL South China Sea, 18N (SCSN18) 1991-1998 NOAA/ ESRL South China Sea, 21N (SCSN21) 1991-1998 NOAA/ ESRL Shangdianzi, CN (SDZ) 2009-2014 NOAA/ ESRL Mahe Island, SC (SEY) Southern Great Plains, Oklahoma, US (SGP) Shemya Island, Alaska, US (SHM) Ship between Ishigaki Island and Hateruma Island, JP (SIH) 1980-2015 NOAA/ ESRL 2002-2015 NOAA/ ESRL 1985-2015 1993-2005 NOAA/ ESRL WDCGG/ Tohoku University Shetland, Scotland, GB (SIS) 1992-2003 WDCGG/ CSIRO Tutuila, American Samoa (SMO) 1979-2015 NOAA/ ESRL South Pole, Antarctica, US (SPO) 1979-2015 NOAA/ ESRL Ocean Station M, NO (STM) 1980-2009 NOAA/ ESRL Summit, GL (SUM) 1997-2015 NOAA/ ESRL Syowa Station, Antarctica, JP (SYO) 1986-2014 NOAA/ ESRL Tae-ahn Peninsula, KR (TAP) 1991-2015 NOAA/ ESRL Trinidad Head, California, US (THD) 2002-2015 NOAA/ ESRL Trainou 180m agl, FR (TR3) 2006-2015 LSCE Tromelin Island, F (TRM) 1998-2007 LSCE Tierra Del Fuego, Ushuaia, AR (USH) 1994-2015 NOAA/ ESRL Wendover, Utah, US (UTA) 1993-2015 NOAA/ ESRL Ulaan Uul, MN (UUM) 1992-2015 NOAA/ ESRL Sede Boker, Negev Desert, IL (WIS) 1995-2015 NOAA/ ESRL Mt. Waliguan, CN (WLG) 1990-2015 NOAA/ ESRL Sable Island, CA (WSA) 1979-2014 WDCGG/ EC Western Pacific Cruise (WPC) Ny-Alesund, Svalbard, Norway and Sweden (ZEP) 2004-2013 NOAA/ ESRL 1994-2015 NOAA/ ESRL Table 2: Same as Table 1 but for the flask-sampling sites. 3 Evaluation 3.1 Benchmarking using a poor man’s inversion The improvement brought by a flux inversion on the simulation of mole fractions usually looks impressive because the inversion easily corrects the growth rate of CO2. However, since the global trend can be accurately obtained from just a few marine surface sites, like MLO and SPO, it is important to assess whether inverted fluxes actually capture more information than this trend. In other words, we may wonder whether all the stations exploited here bring some constraint on the flux distribution that is superior to the global trend from MLO and SPO. For this purpose, Chevallier et al. (2009) introduced a baseline inversion that they called Poor man’s inversion, against which more sophisticated inversions can be benchmarked. In this baseline, the ocean fluxes are kept identical to Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service the prior ones. Over land, the poor man’s flux Fpm at location (x,y) and at time t is defined as: (1) Fpm (x,y,t) = Fprior (x,y,t) + k(year)·σ(x,y,t) Fprior(x,y,t) is the prior flux at the same time and location. σ(x,y,t) is its uncertainty, i.e. the standard deviation of the prior error described in Section 2. k(year) is a coefficient that varies as a function of the year only. k is chosen here so that the mean annual global totals of the poor man’s fluxes equals the mean global totals given by http://www.esrl.noaa.gov/gmd/ccgg/trends/ multiplied by a conversion factor (2.086 GtC·yr-1 per ppm, from Prather et al. 2012). In practice, this simple approach distributes the land carbon sink according to the heterotrophic respiration fluxes from the vegetation without any spatial information from the atmospheric observations, nor any temporal information within any given year. 3.2 Fit to the assimilated measurements (a) RMS (b) normalised RMS Figure 2: Statistics of the differences between LMDZ simulations and individual surface flask measurements. The LMDZ simulations use the Poor man’s fluxes (abscissa) or the posterior flux sets as boundary conditions (ordinate). One point shows (a) the RMS or (b) the RMS normalised by the observation error standard deviation for the analysis period (1979–2015) at one of the assimilated measurement site. Figure 2 shows the posterior root mean square difference (RMS) as a function of the corresponding statistics for the Poor man (except that the small bias of the Poor man is not accounted for) at each assimilated site for the assimilation period. As expected, the inversion performs at least as good as the benchmark and usually performs better. As expected too, the two inversions fit the assimilated data within the assigned standard deviation of the observation uncertainty, which the Poor man’s fluxes do not do. The time series of measurements and posterior simulation at each station are reproduced in Appendix A. 3.3 Fit to the independent measurements Comparisons are also made with independent dry air mole fraction measurements. We define five datasets. The first one is the TCCON GGG2014 archive (Wunch et al. 2011). Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service The second one is the HIPPO aircraft measurement archive (Wofsy et al. 2011). The third one is the aircraft archive built by the FP6 GEOMON project that gathers 47 campaigns (see the list in Table 3). The fourth one is the CONTRAIL aircraft archive (Machida et al. 2008, Matsueda et al. 2008, Sawa et al. 2008). The fifth one gathers the regular aircraft measurements made at South Great Plain (SGP, OK, USA) between November 2007 and December 2012 by Biraud et al. (2013). We compare the model to each individual measurement, but distinguish between the statistics above 1500 m above ground level (free troposphere, FT) and those below 1500 m (boundary layer, BL). As a simple loose quality control, aircraft measurements for which the misfits are larger than 10 ppm in absolute value are discarded. Mission Location AASE-II North Arctic, North America, Eastern Pacific ABLE_2B Amazon, Brazil ASHOE Pacific AIA North East Tasmania, Australia BIBLE-A Western Pacific BIBLE-B Western Pacific BIBLE-C Western Pacific BIK Bialystok, Poland CAR Eastern Colorado, USA CARIBIC Europe, Atlantic, Africa, Middle-East CERES Les Landes, France COBRA-2000 North America COBRA-2003 North America North America COBRA-2004 CRYSTAL Southern North America, Caribbean FTL Northern Brazil GRI Scotland, GB HAA Hawaii, USA HFM North-East United States HNG Hungary North America INTEX-NA LEF Northern Central United States ORL Orléans, France MASTUEDA North Australia to Japan Period Jan.- Mar.1992 April – May 1987 Feb. – Nov. 1994 Jun. 1991 - Sep. 2000 Sep 1998 Aug 1999 Nov 2000 Feb. 2002 – June 2007 Nov. 1992 - Dec. 2002 Nov. 1997 - Aug. 2001 May 2005 – June 2005 Jul.- Aug. 2000 May-June 2003 May-August 2004 May - Jul. 2002 Dec. 2000 - Jul. 2002 July 2001 – Sep. 2007 May. 1999 - Dec. 2002 Nov. 1999 - Nov. 2002 July-August 2004 Apr. 1998 - Dec. 2002 Apr. 1993 – March 2003 Validation report for the inverted CO2 fluxes, v15r2| Organisation Contact NASA B. Anderson Harvard Univ. S. Wofsy NASA S. Gaines, S. Hipskind CSIRO P. Steele NIES T. Machida NIES T. Machida NIES T. Machida LSCE P. Ciais NOAA P. Tans, C. Sweeney MPI-C C. A. M. Brenninkmeijer MPI-BGC C. Gerbig Harvard Univ. S. Wofsy Harvard Univ. S. Wofsy Harvard Univ. S. Wofsy Harvard Univ. S. Wofsy P. Tans, C. Sweeney NOAA LSCE NOAA P. Ciais P. Tans, C. Sweeney P. Tans, C. Sweeney LSCE P. Ciais NASA NOAA S. Vay P. Tans, C. Sweeney LSCE P. Ciais MRI H. Mastueda NOAA Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service PEM-TROP-ADC8 PEM-TROP-AP3B PEM-TROP-BDC8 PEM-TROP-BP3B PEM-WEST-A PEM-WEST-B PFA POLARIS PRE-AVE South Pacific Basin US, Central America, NorthWest South America, East Pacific South Pacific Basin South Pacific Basin Western Pacific Basin, North of Equator Western and Eastern Pacific Basin, North of Equator Alaska, United States North-West Pacific, Alaska and the Arctic North America RTA Rarotonga, South Pacific SAN Northern Brazil SOLVE-DC8 Arctic SONEX North Atlantic SPADE North-West America Western North America, North-East Pacific mid-Western USA.to North Pacific STRAT SUCCESS TOTE-VOTE TRACE-A-DC8 TRACE-P-DC8 Mid-west USA Arctic and Eastern-south Pacific North Pacific Basin TRACE-P-P3B North Pacific Basin YAK Siberia BARCA-A Amazon, Brazil BARCA-B Amazon, Brazil Sept-Oct.1996 Aug-Sept.1996 Mar-April,1999 Mar-April 1999 Sept.-Oct., 1991 Feb.-Mar., 1994 Jun. 1999 - Dec. 2002 Apr.- Sep. 1997 January 2004 Apr. 2000 - Dec. 2002 Dec. 2000 - May 2002 Nov. 1999 - March 2000 Oct.- Nov. 1997 Nov. 1992 – Oct. 1993 May.- Dec. 1995/1996 April-May 1996 Dec.- Feb. 1995/1996 Sept.- Oct., 1992 Mar-Apr 2001 Mar-Apr 2001 Apr. – Sep. 2006 Nov. 2008 May 2009 NASA S. Vay NASA B. Anderson NASA S. Vay NASA S. Vay NASA B. Anderson NASA NOAA B. Anderson P. Tans, C. Sweeney Harvard Univ. S. Wofsy Harvard Univ. NOAA S. Wofsy P. Tans, C. Sweeney P. Tans, C. Sweeney NASA S. Vay NASA B. Anderson Harvard Univ. S. Wofsy NASA S. Vay NASA B. Anderson NASA B. Anderson NASA S. Vay NASA LSCE S. Vay P. Ciais, J.-D. Paris Harvard Univ. C. Gerbig Harvard Univ. C. Gerbig NOAA Table 3: Characteristics of the 45 aircraft campaigns from the FP6 GEOMON CO2 Airborne Data Archive, and of the two BARCA campaigns that were not in the initial archive. Figure 3 shows the distribution of the statistics of the CAMS inversions and that of the corresponding Poor man’s simulation for each dataset: the five independent ones (TCCON, HIPPO, CONT, GEOM, SGP, with FT and BL separated) and a sixth one made of the assimilated measurements (SURFACE). The distribution is made of statistics for each station (TCCON, SURFACE), for each airport (CONT), or for each flight campaign: the minimum, the 25th, 50th and 75th percentiles are shown with usual boxes and whiskers. As expected, the inversion systematically performs better than the Poor man. The inversions usually fit their assimilated data, the column measurements and the aircraft free troposphere measurements within 2 ppm (the median of the RMS is usually about 1 ppm). The fits with aircraft profiles in the boundary layer are usually better than 3 ppm. The time series of aircraft measurements and posterior simulation for HIPPO and CONTRAIL flights are reproduced in Appendix B. Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Figure 3: Box and whisker plot showing the statistics of the misfits between the Poor man’s simulation and the posterior CAMS simulation for each evaluation dataset. The mean bias (standard deviation) of the posterior simulation in the free troposphere is 0.1 (1.3), 0.1 (1.0), -0.2 (1.1) ppm for GEOMON, HIPPO and SGP, respectively. Acknowledgements The author is very grateful to the many people involved in the surface and aircraft CO2 measurements and in the archiving of these data that were kindly made available to him by various means. TCCON data were obtained from the TCCON Data Archive, operated by the California Institute of Technology from the website at http://tccon.ornl.gov/. Mass fluxes for the LMDZ transport model have been provided by Y. Yin, R. Locatelli and P. Bousquet. Some of this work was performed using HPC resources of DSM-CCRT and of CCRT under the allocation t2016012201 made by GENCI (Grand Équipement National de Calcul Intensif). Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Appendix A: Time series of the fit to the dependent surface measurements The mean departure (bd, model minus observations), the associated standard deviation (σd), the mean assigned observation error standard deviation (σo) and the departure RMS normalised by σo are also indicated for each station. These statistics appear in green when RMS/σo ≤ 1 and in orange otherwise. Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Appendix B: Time series of the fit to the independent measurements The aircraft profiles are shown per day (in the form YYMMDD) and per flight, first HIPPO, then CONTRAIL. The posterior model simulation and the measurements are shown in green lines and red dots, respectively. The abscissa is both time (each dash corresponds to a day of measurements) and mole fraction (the distance beween two dashes corresponds to 10 ppm). The measurements are reported here on the 39 model levels and not at their true height. Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service References Validation report for the inverted CO2 fluxes, v15r2| Copernicus Atmosphere Monitoring Service Copernicus Atmosphere Monitoring Service Biraud, S. C., Torn, M. S., Smith, J. R., Sweeney, C., Riley, W. J., and Tans, P. P.: A multi-year record of airborne CO2 observations in the US Southern Great Plains, Atmos. Meas. Tech., 6, 751-763, doi:10.5194/amt-6-751-2013, 2013. Chevallier, F. (2016), Description of the CO2 inversion production chain. CAMS deliverable CAMS73_2015S1_ D73.1.3_201603. http://atmosphere.copernicus.eu/ Chevallier, F., N. Viovy, M. Reichstein, and P. Ciais: On the assignment of prior errors in Bayesian inversions of CO2 surface fluxes. Geophys. Res. Lett., 33, L13802, doi:10.1029/2006GL026496, 2006. Chevallier, F., R. J. Engelen, C. Carouge, T. J. Conway, P. Peylin, C. Pickett-Heaps, M. Ramonet, P. J. Rayner, and I. Xueref-Remy (2009), AIRS-based versus flask-based estimation of carbon surface fluxes, J. Geophys. Res., 114, D20303, doi:10.1029/2009JD012311. Chevallier, F., T. Wang, P. Ciais, F. Maignan, M. Bocquet, A. Arain, A. Cescatti, J.-Q. Chen, H. Dolman, B. E. Law, H. A. Margolis, L. Montagni, and E. J. 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