Acta Materialia 54 (2006) 1995–2002 www.actamat-journals.com Yield criterion of porous materials subjected to complex stress states D.L.S. McElwain a, A.P. Roberts b, A.H. Wilkins a q b,* School of Mathematical Sciences, Queensland University of Technology, GPO Box 2434, Brisbane, Qld. 4001, Australia b Department of Mathematics, University of Queensland, St. Lucia, Brisbane, Qld. 4072, Australia Received 6 October 2005; received in revised form 12 December 2005; accepted 14 December 2005 Available online 23 February 2006 Abstract Finite-element simulations are used to obtain many thousands of yield points for porous materials with arbitrary void-volume fractions with spherical voids arranged in simple cubic, body-centred cubic and face-centred cubic three-dimensional arrays. Multi-axial stress states are explored. We show that the data may be fitted by a yield function which is similar to the Gurson–Tvergaard–Needleman (GTN) form, but which also depends on the determinant of the stress tensor, and all additional parameters may be expressed in terms of standard GTN-like parameters. The dependence of these parameters on the void-volume fraction is found. 2006 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. Keywords: Porous material; Micromechanical modeling – finite-element analysis; Mechanical properties – yield phenomena 1. Introduction The yielding and plastic flow of porous ductile materials has received much attention over the past three decades, mainly because the fracture of such materials is believed to involve nucleation, growth and coalescence of voids in the region of the crack tip [1]. Also, porous ductile materials such as foamed metals with porosities of up to 90% have recently become popular in structural applications. For these reasons it is necessary to construct accurate mechanical theories of porous ductile materials. Armed with an accurate theory of the macroscopic mechanics, scientists and engineers may easily make predictions concerning the behaviour of materials while safely ignoring the microscopic mechanics of individual voids and their interactions (see, for example [2]); the latter being computationally unfeasible when the number of voids is large. McClintock [3] and Rice and Tracey [4] first performed calculations concerning the growth of voids in ductile materials subjected to external stresses. Later, Green [5] proposed a yield function for porous materials, and later still Gurson [6] analytically derived an upper bound for the yield function for a rigid, perfectly plastic, von Mises hollow sphere subject to arbitrary external stresses. Building on early finite-element numerical work by Needleman [7], Tvergaard [8,9] studied mesoscopic stress–strain relations, the evolution of the void volume fraction and the distribution of strain and stress throughout the macroscopic porous material. Further numerical work by Tvergaard and Needleman [10] led to the famous Gurson–Tvergaard–Needleman (GTN) prediction for the yield criterion U = 0, for a ductile solid with void-volume fraction f and matrix yield stress rM: 3 2 q Rhyd =rM 1 q3 f 2 . U ¼ ðReqv =rM Þ þ 2fq1 cosh 2 2 ð1Þ q Supported by a grant from the Australian Research Council through the Discovery Grant scheme. * Corresponding author. Tel.: +61 7 3365 3266; fax: +61 7 3365 1477. E-mail addresses: [email protected] (D.L.S. McElwain), apr@ maths.uq.edu.au (A.P. Roberts), [email protected] (A.H. Wilkins). The notation used in this expression and below is as follows: Rij is the applied macroscopic stress tensor. Below we will consider arrays of voids, and if rij(x) is the Cauchy stress tensor at point x, R = Æræ, where the angled brackets 1359-6454/$30.00 2006 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. doi:10.1016/j.actamat.2005.12.028 1996 D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 indicate a volume average. The traceless part of a tensor will be denoted by a prime: R0ij ¼ Rij 13 dij trR. The macroscopic von Mises equivalent stress and hydrostatic stresses are, respectively, qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi Reqv ¼ 3R0ij R0ij =2; 1 Rhyd ¼ trR. 3 0.8 0.6 Σeqv 0.4 0.2 This paper will also use the determinant of the stress tensor, Rdet: Rdet ¼ det R. The parameters q1, q2 and q3 were introduced by Tvergaard and Needleman in order that Gurson’s bound on the yield criterion should more closely match experimental and numerical results in the initial stages of plastic flow, and many analyses use q3 ¼ q21 following the presentation of [8]. As discussed by Hom and McMeeking [11], Richmond and Smelser [12] also proposed a modified yield criterion, with q1f being replaced by f2/3, and q3f2 by f4/3. In early studies in particular, the finite-element calculations were two-dimensional, either modelling perforated sheet-like materials, or prismatic three-dimensional materials subject to plane stress. Some papers that fall into this category are [7,8,10,13,14]. The three-dimensional finite-element calculations typically involve spherical or ellipsoidal voids packed into periodic arrays (usually hexagonal or simple cubic structures). Both axisymmetric and more general macroscopic stress configurations directed along the principal axes of the material are used. Some papers that fall into this category are [15,9,16,17,11,18–21,2,22–29]. The current paper builds on this work by completing a detailed numerical study of the yield surface for almost rigid, perfectly plastic, von Mises ductile solids containing empty voids arranged in simple cubic (sc), body-centred cubic (bcc) and face-centred cubic (fcc) arrays. The results are valid for void-volume fractions ranging from f = 0% to the percolation threshold of around f = 96%. Various complicating factors are not included: the coalescence of voids; the associated or non-associated flow after yielding; the effect of large strains; and, the effect of different types of hardening. These are considered to be beyond the scope of this paper. It is hoped by the present authors and those cited above that by studying materials containing regular arrangements of voids, some insight can be gained into the mechanics of isotropic porous materials which are costly to study numerically. While this manuscript was in preparation, a recent study of the isotropic case by Wicklein and Thoma [30,31] was brought to the attention of the authors. Wicklein and Thoma simulated the behaviour of nine cubical samples (of 39 cm3) of foamed aluminium containing many voids of diameters between 8 and 10 mm, with void volume fractions ranging from f = 0.5 to f = 0.65. The elastic constants, the initial yield surface, the plastic flow and the yield-surface hardening were derived. Their initial yield 0 0 Σzz > Σxx Σzz < Σxx GTN (1.4, 1.1, 1.9) GTN (1, 1, 1) 0.2 0.4 0.6 0.8 1 Σhyd Fig. 1. Yield points for Rxx = Ryy and positive hydrostatic stress. (Crosses) Yield points for Rzz > Rxx. (Circles) Yield points for Rzz < Rxx. (Outer solid line) Gurson’s bound, q1 = q2 = q3 = 1. (Dotted line) Best-fit GTN curve with q1 = 1.4, q2 = 1.1 and q3 ¼ q21 ¼ 1:9. All data collected at f = 0.25 for voids arranged in a simple cubic pattern. These data were obtained using the numerical procedure described below. surface displays very similar characteristics to that obtained here with particular emphasis being placed on the third invariant of stress, Rdet. Despite all the investigations already mentioned, a comprehensive study of the dependence of the yield function on multiaxial stress states and void volume fractions has not been performed. The purpose of this paper is to make a comparison with the GTN proposal, quantify the effect of Rdet, and to numerically derive the dependence of the q-like parameters on f for the three structures, sc, bcc and fcc. One of the principal results of this paper is that to describe the yield surface accurately, the yield function must depend on Rdet. Hints of this may be seen in [17,19,22,23,27], where the GTN q parameters appeared to depend on the stress state used: an analogous result is found in Ref. [32]. It may be seen most dramatically in Richelsen and Tvergaard [21], and in the analysis of Zhang et al. [26], who explored several arbitrary states of stress aligned with the principal axes of a periodic voided material. It may also been seen in the data of Hom and McMeeking [11] and Goya et al. [19], where the value of stress triaxiality did not uniquely define the yield point. Fig. 1 shows data similar to that generated by [26] – axisymmetric with Rxx = Ryy, and with Rzz arbitrary, but the hydrostatic stress Rhyd P 0. The data appear to describe two distinct yield curves, meaning that yield function must depend on more variables than simply Rhyd and Reqv, in contradistinction to Eq. (1). 2. General remarks concerning the yield function 2.1. The isotropic case The yield function for an isotropic solid must depend only on Rhyd, Reqv and Rdet since these are the well-known three invariants of the rotation group. D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 Now consider the shape of the yield curve on an arbitrary octahedral planep defined ffiffiffiffiffiffiffiffi by Rhyd = h. The radial coordinate on this plane is 2=3Reqv , while the third invariant can be related to the angular coordinate, h, through 1 2 Rdet ¼ h3 R2eqv h þ R3eqv cos 3h. 3 27 ð2Þ Thus the yield curve is described by 0 = Uh(Reqv, cos 3h), which is generically a 3n-lobed shape (n is integer). The most extreme case is the equilateral triangle, shown in Fig. 2. It is most extreme in the sense that of all possible non-concave shapes, the variation of Reqv is greatest. The equilateral triangle has the property that min Rmax eqv ¼ 2Reqv . Thereby, convexity puts an upper bound on the effect of Rdet on the yield function: the value of Reqv can vary by a maximum of two for fixed Rhyd. It shall be assumed that the yield function is convex throughout this paper. While this is quite common, it is not strictly thermodynamically necessary, and non-convex forms have been used for porous materials by Wicklein and Thoma [30]. Nevertheless, the numerical data generated here suggests strongly that the yield function is convex. 2.2. Cubic symmetry For porous materials with sc, fcc and bcc arrays of voids, the yield function must be invariant under the cubic symme- 1997 try group – Oh in Schönflies notation – which is a subgroup of the group of general rotations and reflections in three dimensions [33]. Oh is finite dimensional of order 48 and consists of rotations through 90 about the x, y and z axes, reflections through the xy, xz and yz planes, and all combinations thereof. For the theory to be invariant under Oh, the arguments of the yield function must be invariant combinations of components of the stress tensor. The isotropic invariants Reqv, Rhyd and Rdet are also invariants of Oh and so we shall use these. However, there are further invariants, such as RxxRyyRzz (which does not equal Rdet for general R) or R2xy þ R2xz þ R2yz which could also be arguments of the yield function. There are six invariants in total – the yield function has six arguments – and this makes finding an analytical expression for the yield function that describes the finite element (FE) data complicated. However, here this complexity is reduced by restricting to macroscropic stress states with Rxy ¼ Rxz ¼ Ryz ¼ 0. ð3Þ Then, the independent degrees of freedom contained in the non-zero triplet (Rxx, Ryy, Rzz) are completely captured by the triplet (Reqv, Rhyd, Rdet), and the yield function has only three arguments. If this paper is considered as a precursor to a similar study of the more complicated isotropic case, this procedure should afford some insight into the type of results obtained there. 2.3. Final comments Σ III ΣI Σ II The yield function is also invariant under R ! R, since the microscopic constitutive laws, in particular the von Mises plasticity, are invariant under (R, E) ! (R, E). When Reqv = 0 the yield hypersurface degenerates to two points given by |Rhyd| = a(f). This follows because Reqv is a sum of squares, so each term must be zero, and all Oh invariant forms can be determined by Rhyd. The yield function is therefore a function of |Rhyd|. This result is evident in Fig. 1, in which the two sets of data appear to converge towards the hydrostatic axes as Reqv ! 0. In the following sections, it will be useful to write the yield function in a form which separates the contributions of Rdet from the other invariants. This is because the size of the Rdetinduced variations around the ‘‘average’’ yielding behaviour given by circles as in Fig. 2 are severely limited by the argument contained in Section 2.1, and because this ‘‘average’’ behaviour is described well by the GTN formula. This is done by writing the yield function as a power-series expansion U ¼ Uð0Þ ðReqv ; Rhyd Þ þ Uð1Þ ðReqv ; Rhyd ÞðRdet hRdet iÞ Fig. 2. Three yield curves on an octahedral plane. The most extreme nonconcave shape is the equilateral triangle (with the maximum value of Reqv attained at its vertices). The GTN form is necessarily a circle: the one shown (dashed) intersects with the triangle at cos 3h = 0. The other curve shown (in grey) is an example of a generic shape consistent with the isotropic symmetry. 2 þ Uð2Þ ðReqv ; Rhyd ÞðRdet hRdet iÞ þ ð4Þ with the following definitions. Introduce the function ÆReqv, which depends on Rhyd and solves U(0)(ÆReqvæ, Rhyd) = 0. Then define 1998 1 hRdet i R3hyd hReqv i2 Rhyd . 3 D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 ð5Þ Thus, when cos 3h = 0 and Reqv = ÆReqvæ, we have U = 0. Geometrically, U(0) is thus describing the circle in Fig. 2 – it is the ‘‘average’’ behaviour. The higher-order terms describe variations around this average behaviour, and below it will be necessary to retain only the linear term. 3. The numerical method 3.1. Description The materials studied in this paper have spherical voids arranged in sc, bcc and fcc arrays. Some examples are depicted in Fig. 3. Various void-volume fractions are considered, from 2% up to 90% which is close to the percolation threshold of the structure where the matrix is no longer connected. The voids are empty and exert no pressure on the surrounding matrix material.They have zero Young’s modulus. Because of the periodicity of the cubic structures and the stress ansatz of Eq. (3), only one-eighth of the unit cell need be considered. To stay close to the original Gurson presentation, the matrix material is chosen to be almost rigid, perfectly plastic. The Poisson ratio of the matrix is 1/3. The initial yield point rM = 7.5 · 105E, and the hardening is linear with slope 7.5 · 108E, where E is the Young’s modulus. The finite-element technique is used to generate yield points. Each unit cell, comprising of both the matrix and void material, is decomposed into n3 cubical elements as illustrated in Fig. 4. The strain rate of the one-eighth unit cell’s surfaces (which must remain planar) is held constant (but different for each simulation). That is, Eij ðtÞ ¼ diagðExx ; Eyy ; Ezz Þ t; ð6Þ where t denotes time. A quasi-static approximation is made: time is discretised and the equilibrium configuration at each small time-step is obtained iteratively by using the return-mapping algorithm described in Chapter 12 of [34] in conjunction with solving the infinitesimal elasticity problem with each different element having, in general, a different consistent tangent operator. A custom-built FORTRAN code is used, relying heavily on a customised version of the 3D infinitesimal elastic routine written and extensively bench-marked by Garboczi and collaborators [35,36]. Fig. 3. Four different unit cells. (Top left) Simple-cubic (sc) with f = 0.11. (Top right) Body-centred cubic (bcc) with f = 0.84. (Bottom) Face-centred cubic (fcc) with f = 0.45 and f = 0.83. D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 1999 However, when the triaxiality (Rhyd/Reqv) is very high, it becomes difficult to precisely ascertain when the material has ‘‘yielded’’, because the definition of ‘‘yield’’ involves finding a maximum in Reqv. The data becomes somewhat suspect and sometimes may even appear to describe a non-convex surface. This may be viewed as another sort of error which is not properly accounted for in the above analysis since it is not only related to the discretisation used. Therefore, it is prudent to omit such data from the data-fitting exercise below, although because we will demand convexity by fitting with simple three or four parameter models known to describe convex surfaces, their inclusion does not affect the result substantially because the ‘‘noise’’ due to this error cancels. 4. Results Fig. 4. A sketch of the cubical finite-element approximation to the sc unit cell (for clarity most of the cubes are not shown, and recall that only oneeighth of the unit cell is used in the simulations). The code was tested on non-porous materials and bench-marked against results found in Refs. [11,21]. The strain is increased until the ‘‘yield point’’ is reached, which is defined here following [37] as the point at which the von Mises equivalent stress reaches a maximum. The elements’ elastic and plastic strains are always small (<104) because of the matrix rigidity and because the simulations are never taken past the yield point just defined. Thus, it is safe to use the standard small-strain approximation to the mechanics. A few hundred simulations, each with randomly chosen (Exx, Eyy, Ezz) are performed for each void volume fraction giving a few hundred yield points on the yield surface. 3.2. Scaling of results with number of elements and the error 4400 yield points were generated for each of the three arrangements of voids, with f ranging from 0.02 up to 0.9 which is close to the percolation threshold of the matrix, SC BCC which is approximately 0.965 ðfperc Þ for sc, 0.994 ðfperc Þ FCC for bcc, and 0.963 ðfperc Þ for fcc. The yield points were expressed in (Reqv, Rhyd, Rdet) space and a least-squares fit with an extension of GTNs formula was found. Consider the sc case with 30% void volume fraction (f = 0.3). As is shown in Fig. 5, the average response is fitted well with GTNs formula with q1 = 1.31, q2 = 1.16 and q3 ¼ q21 . The large amount of scatter around this curve is due to the influence of Rdet. In Fig. 6 all FE data in the range 0.27 6 Rhyd 6 0.33 (approximately half-way along the hydrostatic axis in this case) is considered and a plot of ðRdet ; R2eqv Þ is made. A linear relation is evident. In fact, exploring other slices of hydrodynamic stress and f results in the conclusion that R2eqv may always be approximated as a linear function of Rdet. Moreover, the slope of this relationship is directly proportional to Rhyd. The yield point predicted depends on the value of n, and it is important to choose it large enough so that an accurate prediction is made. Numerical experiments with different n show that the predicted value of stress, Rij, at yield scales inversely with n: rij . Rij ðnÞ ¼ R1 ij þ n This is quite common [38], and can be used to derive the limiting ‘true’ value R1 ij by extrapolation, and thereby to estimate the discretisation error at each n. In the present case this gives an estimate of the relative discretisation error R ðnÞ R1 ij ij ¼ 0:02 at n ¼ 80. R1 ij The dependence on the applied strain is minimal, and this value has been obtained by averaging the results over the void volume fraction and the types of cubic structure. 0.6 0.5 Σeqv 0.4 0.3 0.2 0.1 0 0 0.1 0.2 0.3 0.4 0.5 0.6 Σhyd Fig. 5. GTN yield curve (solid) and FE data points for sc voids with 30% void volume fraction. GTN parameters are q1 = 1.31, q2 = 1.16 and q3 ¼ q21 . 2000 D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 where 0.32 A¼1þ 0.28 2 Σeqv 0.24 0.2 -0.02 -0.01 0 0.01 0.02 Σdet Fig. 6. R2eqv versus Rdet for those data points which lie in the band 0.27 6 Rhyd 6 0.33. Simple cubic voids with f = 0.3. In this way, we are led to propose an extension of the GTN yield criterion: 2 3 a2 ðf ÞRhyd =rM 1 U ¼ Reqv =rM þ 2a1 ðf Þ cosh 2 2 a1 ðf Þ sðf ÞðRhyd =rM ÞðRdet hRdet iÞ=r3M . ð7Þ Three new functions a1(f), a2(f) and s(f) have been introduced 2 here. Comparing with Eq. (5), hR2eqv =r2M i ¼ 1 þ a1 ðf Þ 3 2a1 ðf Þ cosh 2 a2 Rhyd =rM . In Eq. (7), the linear relationship between R2eqv and Rdet is evident, as is the direct proportionality between the slope of this relationship and Rhyd. The function s(f) controls the size of the term containing Rdet. When s(f) = 0, the yield function reduces to GTNs formula if a1 = q1f and a2 = q2. 4.1. Monotonicity, single-valuedness and convexity The particular forms of a1, a2 and s detailed below ensure that U is monotonic, in that increasing f always brings the yield function closer to the origin in stress space. By Eq. (2), U written above may be viewed as a cubic in Reqv, and thus it is possible that given Rhyd and h (the angle on the octahedral plane), there are up to three possible solutions for Reqv. This is a problem of single-valuedness. We address this problem by simply defining yield to occur at the smallest non-negative value of Reqv that is a root of the equation U = 0. A full set of conditions resulting from convexity are algebraically extremely complicated and beyond the scope of this paper, being largely unimportant: only the crucial points are investigated here. Finally, for some Rhyd ¼ Rmax hyd , the yield surface should degenerate to a point, irrespective of the value of h. Consider the issue of convexity in further detail. Writing Rdet in terms of h, the yield function may be expressed as 2 3 U ¼ AS þ ðReqv =rM Þ S þ ðReqv =rM Þ T ; a21 3 a2 Rhyd =rM ; 2a1 cosh 2 1 2 ð8Þ S ¼ 1 sðRhyd =rM Þ ; 3 2 T ¼ sðRhyd =rM Þ cos 3h. 27 It is immediately obvious that if S = 0 for some Rhyd < Rmax hyd then the only solution of U = 0 is Reqv = 0 which is a contradiction of the definition of Rmax hyd . Thus, if we write 2 max s ¼ 3x= Rhyd ; ð9Þ 2 1 þ a21 max Rhyd ¼ arccosh ; 3a2 2a1 the quantity x(f) 6 1 for all f. It is important that this parameterisation of s(f) in terms of Rmax hyd is not only convenient, but also strongly suggested by the FE results for the sc and bcc cases: a least-squares fit with the data at fixed volume fraction shows x(f) varies between about 0.7 for high volume fractions and unity for low volume fractions. (The FE data for the fcc case are not trilobal and hence s = 0 for fcc.) The critical point is therefore when the yield curve is an equilateral triangle for some Rhyd, for increasing Rhyd past this point may result in a non-convex curve. Some straightforward algebraic manipulation shows that triangularity is avoided if, and only if, S2 > 1 2 2 s Rhyd A; 27 ð10Þ for all Rhyd and f. The cosh factor in A means a closed-form solution cannot be found. However, by writing the pffiffiffi inequality in terms of x and using a series expansion of A, it may be checked that if 1 x1 ¼ 1 þ pffiffiffi max 3Rhyd pffiffiffi 1 1 max4 pffiffiffið4Þ 2 pffiffiffi00 A A Að0Þ þ Rmax ð0Þ þ ð0Þ þ . . . ; R 2 hyd 4! hyd ð11Þ where the RHS contains pffiffiffi a finite number of terms of the series expansion of A around Rhyd = 0, (for instance pffiffiffi00 A ð0Þ ¼ 9a1 a22 =4ð1 a1 Þr2M ), the inequality of Eq. (10) is guaranteed to hold. Any x1 greater than this will ensure convexity, however, this choice fits the FE data well. Note finally that x 6 1 as required above. 4.2. Simple cubic Applying a least-squares regression to the FE data shows that they are well-fit by SC 0:809 a1 ðf Þ ¼ ðf =fperc Þ and SC a2 ðf Þ ¼ 0:88 þ 1:27ðf =fperc Þ. ð12Þ D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 Note that, by construction, a1(f) vanishes at f = 0 and is SC unity at the percolation threshold f ¼ fperc 0:965 as required. It is of a power-law form similar to that proposed in Ref. [12], but with a different exponent. Also note that a2(f) is close, but not equal to the values of around unity proposed by a number of other authors such as [8,17,27]. The first five terms of the power series in Eq. (11) have been used. By way of example, Fig. 7 shows a slice of data from Rhyd = 0.25rM to Rhyd = 0.5rM at f = 0.25 and the fit with curves generated by the functions of Eq. (12) and x given by Eq. (11). This pattern is universal: as Rhyd is increased from zero the yield curves become more trilobal, but close to Rmax hyd the curves becomes circular again. An indication of the quality of the proposed yield function is obtained by plotting the predicted value of R2eqv (given Rhyd, Rdet and f) versus the FE result for each data point. This is shown in Fig. 8. Included is the data from [21] who calculated some yield points for a variety of different stress states (some with Rdet 6¼ 0) for voids at f = 0.04 and arranged in a simple cubic fashion inside a fairly stiff matrix (rM = 0.0033E) and Poisson’s ratio of 0.3. Data are also included from Ref. [11] in which yield points were calculated for three different stress states for voids at f = 0.0082 and f = 0.065 arranged in a simple cubic fashion inside a matrix with rM = E/200, Poisson’s ratio of 0.3, and a small power-law hardening of 0.1. In some cases data was extracted from graphs in these two papers which may have resulted in some error. Nevertheless, Fig. 8 shows good agreement with an R2 of 0.998. Σzz Σ2eqv 2001 with Σ det 0.8 0.6 0.4 0.2 0.2 0.4 0.6 0.8 FE Fig. 8. The predicted value of R2eqv versus the FE result for the 4400 yield points generated for sc with a range of void volume fractions and stress states. A regression with y = x has an R2 of 0.998. The FE results of [21] are shown as triangles and the results of [11] are shown as stars. 4.3. Body-centred cubic The FE data for the body-centred case is qualitatively very similar to the simple cubic case. Applying a leastsquares regression to the 4400 points generated shows that they are well-fit by BCC BCC BCC 1:24 a1 ðf Þ ¼ f =fperc þ 2:4ðf =fperc ðf =fperc Þ Þ; BCC Þ. a2 ðf Þ ¼ 0:85 0:22ðf =fperc ð13Þ As for the sc case, a1(f) vanishes at f = 0 and is unity at BCC f ¼ fperc 0:994. This particular function fits the data slightly better than a pure power-law. Once again, a2(f) is close, but not equal to unity. It is sufficient to keep the first five terms of the power series in Eq. (11). Similarly to the sc case, this proposal has an R2 of 0.998. 4.4. Face-centred cubic In this case, surprisingly, the 4400 data points generated show very little dependence on the determinant. Therefore, we set sðf Þ ¼ 0; Σxx Σ yy in contrast to the sc and bcc cases. Applying a least-squares regression to the FE data shows that they are well-fitted by 1:43 FCC FCC FCC a1 ðf Þ ¼ f =fperc þ 1:33 f =fperc f =fperc ; ð14Þ FCC a2 ðf Þ ¼ 0:83 0:14 f =fperc . Similarly to the sc case, this proposal has an R2 of 0.993. 5. Conclusions Fig. 7. Data at f = 0.25 with Rhyd = 0.25rM (black) through to Rhyd = 0.5rM (white) and the curves produced by Eqs. (11) and (12) projected onto the octahedral plane. For f = 0.25, Rmax hyd 0:6rM as can be seen in Fig. 1. The parameters in the latter equation are produced from a global fit to all the 4400 data points (with different f), not just those few depicted here, and that is why the fit is not perfect. The discretisation error is indicated by the size of the dots, and the almost-triangular nature of the data is evident around Rhyd = 0.5rM. Because of the role of voids in the process of ductile fracture and the fact that modern fabrication techniques can produce precisely engineered porous materials, it is desirable to gain a good understanding of the yield criterion of porous materials. We have chosen to concentrate on the simple cases where the voids are arranged in either 2002 D.L.S. McElwain et al. / Acta Materialia 54 (2006) 1995–2002 simple cubic, body-centred cubic or face-centred cubic arrays. Previous work, in particular see Refs. [11,19,21,26], has demonstrated that the celebrated Gurson–Tvergaard–Needleman yield criterion [6,8–10] is inaccurate for general stress states, and the calculations here have shown that the equivalent stress at yield can be altered by up to a factor of two by varying the determinant of the stress tensor at fixed hydrostatic stress. We used the finite-element technique employing the return-mapping algorithm described in Ref. [34] to monotonically increase arbitrarily prescribed, but diagonal, macroscopic strain to find many thousand yield points for each of the three void arrangements. A range of void volume fractions from 2% to 90% were explored, with a linearly hardening stiff matrix material with rM = 7.5 · 105E, Poisson’s ratio of 1/3 and hardening slope of 7.5 · 108E, where E is the Young’s modulus. An analysis of the relative errors incurred by the finite-resolution of the finite-element technique showed that they are ±2%. The finite-element data was fitted using least-squares to the yield function given in Eq. (7). This function’s dependence on the equivalent and hydrostatic stresses (Reqv and Rhyd) is almost identical to GTNs formula, but there is also an extra term which depends linearly on the determinant of the stress tensor, Rdet. The yield function contains three functions of void volume fraction, which are slightly different for the simple cubic, body-centred cubic and facecentred cubic cases. The first of these, a1, is well fitted by a power-law (as initially proposed in Ref. [12]), while the second, a2, is a slowly varying linear function of void volume fraction, and is numerically close to forms proposed by various other authors (such as [8,17,27]). The exact forms are given in Eqs. (12)–(14). The third, s(f), determines the strength of the contribution of Rdet. The requirement of yield-function convexity suggest a particular form for s(f) in terms of a1 and a2 – given in Eqs. (8) and (9) and the first five terms of the power series in Eq. (11) – and this compares well with the finite-element data for the simple cubic and body-centred cubic cases. Interestingly, for the face-centred cubic case, s(f) = 0, and there is no dependence on Rdet. 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