This article was downloaded by: [Universita Degli Studi di Cagliari] On: 12 November 2014, At: 03:15 Publisher: Taylor & Francis Informa Ltd Registered in England and Wales Registered Number: 1072954 Registered office: Mortimer House, 37-41 Mortimer Street, London W1T 3JH, UK International Journal of Mining, Reclamation and Environment Publication details, including instructions for authors and subscription information: http://www.tandfonline.com/loi/nsme20 Dust dispersion from haul roads in complex terrain: the case of a mineral reclamation site located in Sardinia (Italy) a a a Letizia Piras , Valentina Dentoni , Giorgio Massacci & Ian S. Lowndes b a Department of Civil and Environmental Engineering and Architecture (DICAAR), University of Cagliari, Cagliari, Italy b Faculty of Engineering, Process and Environmental Research Division, University of Nottingham, UK Published online: 06 Mar 2014. To cite this article: Letizia Piras, Valentina Dentoni, Giorgio Massacci & Ian S. Lowndes (2014) Dust dispersion from haul roads in complex terrain: the case of a mineral reclamation site located in Sardinia (Italy), International Journal of Mining, Reclamation and Environment, 28:5, 323-341, DOI: 10.1080/17480930.2014.884269 To link to this article: http://dx.doi.org/10.1080/17480930.2014.884269 PLEASE SCROLL DOWN FOR ARTICLE Taylor & Francis makes every effort to ensure the accuracy of all the information (the “Content”) contained in the publications on our platform. However, Taylor & Francis, our agents, and our licensors make no representations or warranties whatsoever as to the accuracy, completeness, or suitability for any purpose of the Content. Any opinions and views expressed in this publication are the opinions and views of the authors, and are not the views of or endorsed by Taylor & Francis. The accuracy of the Content should not be relied upon and should be independently verified with primary sources of information. 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Terms & Conditions of access and use can be found at http://www.tandfonline.com/page/termsand-conditions International Journal of Mining, Reclamation and Environment, 2014 Vol. 28, No. 5, 323–341, http://dx.doi.org/10.1080/17480930.2014.884269 Dust dispersion from haul roads in complex terrain: the case of a mineral reclamation site located in Sardinia (Italy) Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 Letizia Pirasa, Valentina Dentonia*, Giorgio Massaccia and Ian S. Lowndesb a Department of Civil and Environmental Engineering and Architecture (DICAAR), University of Cagliari, Cagliari, Italy; bFaculty of Engineering, Process and Environmental Research Division, University of Nottingham, UK (Received 20 December 2013; accepted 13 January 2014) In recent years, there has been significant research effort to investigate the use of plume dispersion models to assess the environmental impact of fugitive dust emissions from surface mining operations. In particular, the results of these studies have identified challenges to the use of traditional Gaussian plume dispersion models to satisfactorily reproduce fugitive dust dispersion and deposition experienced from low elevation release heights within complex topography. This paper presents a discussion of the results of a preliminary series of modelling studies that have employed the UK-Atmospheric Dispersion Modelling System (ADMS) model to investigate the dust dispersion and deposition from a former mining site currently undergoing remediation. The remediation site is located within a valley in south-western Sardinia that may be considered an aerodynamically complex terrain. A series of field measurement surveys were conducted along the length of an unpaved surface haul truck roadway to measure the PM2.5 and PM10 dust fractions within the emitted plumes. To investigate the potential effects that the surrounding topography may have on the atmospheric dispersion and deposition experienced a series of UK-ADMS dispersion models were solved for a range of meteorological stability conditions typical of the area under investigation. A preliminary analysis of the results of these simulations concludes that there was a strong influence of the surrounding terrain on the dispersion and deposition phenomena predicted. Keywords: mine reclamation; unpaved roads; fugitive dust; emission factors; atmospheric dispersion Introduction Mining and mineral site remediation activities can represent a significant contribution to particulate matter (PM) emissions from a range of sources which may include: overburden removal, drilling, blasting, loading, transit along unpaved roads, materials handling and wind erosion from exposed surfaces [1]. These potential emission sources are classified as fugitive dust sources by the US Environmental Protection Agency, since they emit dust in the form of a non-confined flow stream [2]. National and International regulations to specify air quality standards have established statutory exposure limit levels for airborne dust concentrations, and in particular for the PM10 and PM2.5 size fractions, deemed potentially hazardous to human *Corresponding author. Email: [email protected] © 2014 Taylor & Francis Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 324 L. Piras et al. health. In particular, since 2005 Annex XI (Limit values for the protection of Human Health) of the European Directive on ambient air quality [3] established a daily PM10 exposure limit of 50 μg/m3, and that a daily exposure of 40 μg/m3 should not be exceeded more than 35 times in a calendar year. As regards PM2.5, Annex XIV (National exposure reduction target, target value and limit value for PM2.5) of the Directive establishes an exposure-level limit value of 25 μg/m3 per calendar year to be achieved by 2015, followed by a 20 μg/m3 limit value to be met by 2020. A series of recent research studies have highlighted that Gaussian plume models may not satisfactorily predict the atmospheric dispersion and deposition of fugitive dust emitted from sources within mining and mine remediation operations. It was concluded that this may be due to a number of factors including: the typically low release heights of the fugitive dust sources and the complexity of the surrounding topography. Recently, Cole and Zapert [4] employed the ISC3 Gaussian plume model to investigate the dispersion of dust from a number of fugitive sources located within three stone quarries in the state of Georgia, USA. The results of these studies demonstrated that the model overpredicted the actual measured PM10 ground-level deposition experienced by a factor of 5. It was concluded that this overprediction was due to both an overestimation of the actual fugitive dust emission by the US EPA AP42 dust emission factor equations used to estimate the source emissions, and to the inherent limitations of the Gaussian plume model to predict the particulate dispersion and deposition within areas of complex terrain. Other research studies have confirmed the need to develop more representative emission factors to be employed with Gaussian plume dispersion models in order to more satisfactorily predict the environmental impact of surface mining operations [5,6]. Several recent research studies were performed to investigate the performance of the UK-Atmospheric Dispersion Modelling System (ADMS) model [7] against other Gaussian plume dispersion models [8–11]. The UK-ADMS code uses a modified Gaussian dispersion model to simulate pollutant dispersion within the atmospheric boundary layer. The ADMS code was developed to model the dispersion of buoyant or neutrally buoyant particles and gases [10,12]. A recent study [13] employed the ADMS code to develop a simulation strategy to investigate the fugitive dust emissions from in-pit quarry extraction and processing activities. The model was used to replicate the fugitive dust emissions, dispersion and deposition observed at a working quarry during the blasting, loading and haulage of the mineral. The study concluded that the observed dust dispersion is strongly affected by the local meteorological conditions and by the in-pit and surrounding terrains. A further investigation [14] was carried out at the same quarry site to verify the reliability of the predicted ADMS model simulations. The modelled monthly dust deposition rates arising from the routine blasting, loading and haul road operations were compared against the dust deposition data collected by a network of British Standard Frisbee deposition gauges. A comparative analysis of this data concluded that the ADMS models overpredicted the observed dust deposition rates; the discrepancy was attributed to the use of non-site-specific emission factors and to the inherent limits of the flow field model to simulate the in-pit turbulent flow fields [15]. This paper presents the results of a series of parametric modelling studies conducted to investigate the predicted atmospheric dispersion of fugitive dust emissions measured along an unpaved haul road of a mineral remediation site in the south‐west of Sardinia. The UK-ADMS models were solved for a range of typical meteorological conditions (wind speed, wind direction and atmospheric stability class). The results of these International Journal of Mining, Reclamation and Environment 325 Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 simulation results were analysed to identify the effects that the surrounding topography may have on the predicted dust dispersion and deposition. The dust emissions simulated were validated against a series of PM10 and PM2.5 dust measurements collected along the near upwind and downwind lengths of an unpaved haul road travelled by mineral haulage trucks [16]. The resultant fugitive dust emission rates were used to determine emission factors that were used to represent the fugitive dust sources within the UK-ADMS models. The case study This paper presents the results of a series of modelling studies to investigate the predicted dust dispersion and deposition experienced from the unpaved haul roads within a former mineral property undergoing remediation in south-western Sardinia. There are a significant number of former mining and mineral sites currently undergoing remediation in this region, which was an important former mining area in Italy for lead, zinc and silver extraction. These mining activities ceased towards the end of the 1980s. Since this time, an intensive remediation plan has been promoted by both the local and national authorities to reclaim many of these former mining and mineral sites. Figure 1 shows a photograph of one of the major remediation sites in the province of Carbonia–Iglesias (Monteponi): the remaining surface structures of the former mineral plant are visible behind the red mud tailings bank that has been covered with a geotextile fabric. The principal reclamation activities conducted at the former mineral property are the limestone capping of the abandoned tailings dumps, which are part of a wider hydraulic management project to prevent the potential emission of acid leachate from the residual ore remaining within the tailings dumps. The emplacement of the limestone cap involves the following stages: the crushed limestone rock is loaded from stock piles into haulage trucks by wheeled loaders and then transported along unpaved haul roads to the emplacement sites on top of the former tailings dumps; the limestone material is then unloaded from haulage trucks and spread over the surface of the tailings dump by a shovel excavator. A schematic representation of these activities is shown in Figure 2. Table 1 summarises the operational capacities of the vehicles. A preliminary estimation of the fugitive dust emission rates associated with these activities concluded that the total emissions inventory was dominated by that generated by the transit of the haulage trucks along the unpaved roads. Figure 1. The former mining and mineral site of Monteponi (Carbonia–Iglesias) illustrating the red mud tailings dump in the foreground that is undergoing remediation. 326 L. Piras et al. material loading material transport material unloading material spreading empty dumper travel Figure 2. process. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 Table 1. Flow diagram of the various stages of operational activities involved in the reclamation Main operational characteristics of the vehicles used during the reclamation activities. Vehicle No. of wheels Weight [t] Capacity [m3] 4 6 tracked 18.2 13.8 23.0 3.0 12.5 1.2 Wheeled loader Haulage truck Excavator As regards material spreading, it was concluded that the release height of this potential source was very close to the ground and therefore the major dust deposition occurred at short distances from the emission point. Therefore, the contribution of this activity to the overall emission was not included during the subsequent modelling studies. With reference to the loading and unloading operations, the emission factors were estimated by employing Equation 1, proposed by US EPA for mineral drop operations [17]: U 1=3 E ¼ k 0:0016 2:21=4 M (1) 2 where E = emission factor in terms of mass of emitted dust per mass of handled material [kg/Mg]; U = mean wind speed [m/s]; M = material moisture content [%]; and k = numerical coefficient depending on the particulate size. As shown above, the emission generated depends on the near-surface wind speed; therefore, different emission factors were obtained for a range of different meteorological conditions and release heights, typical to the mineral operations under consideration. For the atmospheric conditions simulated, the wind speeds at the release heights of loading and unloading (4 m and 1.5 m, respectively) were estimated [18]. The crushed Table 2. TSP emission factors and TSP emission rates for the material handling operations. Dust source Material loading Material unloading Meteorological conditions Class Class Class Class Class Class A D F A D F TSP emission factor [kg/Mg] 0.17 1.25 0.24 0.16 1.03 0.12 × × × × × × 10−2 10−2 10−2 10−2 10−2 10−2 TSP emission rate [g/s] 7.36 54.25 10.24 6.74 44.81 5.08 × × × × × × 10−2 10−2 10−2 10−2 10−2 10−2 International Journal of Mining, Reclamation and Environment 327 limestone was assumed to have a moisture content of 0.7% [17]. The total suspended particulate (TSP) emission factors and the corresponding emission rates determined for the material loading and unloading operations are reported in Table 2. A comparison of the computed emission rates for the material loading and unloading, and the truck haulage operations concluded that the contributions of the dust emissions due to material loading and unloading were assumed negligible. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 Field measurements Dust emission from unpaved roads The transit of the loaded and unloaded vehicles along the unpaved haul roads crushes the surface road material into finer particles due to the force applied by the haulage truck wheels. These generated fine particles which are then subsequently lifted up by the action of the rolling wheels, to be potentially transported by the background wind flows across large distances. Following the initial suspension of the fine dust by the wheels of the trucks, the turbulent wake generated around and left behind by the passage of the vehicles can continue to act on the surface material of the road, and thus potentially generating further particulate emissions [19]. Unpaved haul roads are classified as fugitive dust sources by the US Environmental Protection Agency, as they emit fugitive dust in the form of an unconfined flow stream. The sampling of the dust plume arising from a vehicle travelling on a road is complex and traditional sampling techniques cannot be used as they are designed for application to confined flow streams. There are currently two accepted sampling methods suitable to estimate the emissions from fugitive dust sources: either the upwind–downwind method or the exposure-profiling method [20]. With reference to the case study under examination, a series of field measurements were performed to measure the PM2.5 and PM10 dust emissions generated by the transit of haulage trucks along the unpaved roads. The exposure-profiling method [16] was used to estimate the dust emission factors. A detailed description of the sampling procedures and the measurement instruments used is reported below. Materials and methods The PM2.5 and PM10 dust fractions generated by the transit of the haulage trucks along an unpaved haul road within the remediation site were sampled using Respicone multistage Virtual Impactors. The dust samplers have three sampling stages in which different size fractions are collected on fibreglass filters. The samplers combine traditional inertial classification with a photometric detection system which analyses the variability of dust concentration over time for each collected dust fraction. The two pictures in Figure 3 illustrate the classification mechanism and stages employed by the collectors. A total airflow of 3.10 l/min (Q) is pulled through each sampler delivering the total inhalable fraction (IF). This total airflow is subsequently divided into three airflow streams which exit the instrument at each of the three collection stages (where Q1 = 2.66 l/min, Q2 = 0.33 l/min, Q3 = 0.11 l/min). The following three PM fractions are captured in each of the three sampling stages, listing from top to bottom the finest fraction PM2.5 (cut-off diameter 2.5 μm), the PM10 fraction (cut-off diameter 10 μm) deprived of the PM2.5 fraction and the coarser IF deprived of the PM10 fraction. The mass deposited on each of the three fibreglass filters enables the Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 328 L. Piras et al. Figure 3. Schematic representations of the Respicone multistage Virtual Impactor dust sampler illustrating the 3 size fraction sampling and collection stages. determination of the mean dust concentration for each fraction. The photometric measurement system analyses the variability of dust concentration collected over time by each size collection stage. The time histories of the collected dust concentration for each of the three size fractions were recorded by a digital data logger connected to the samplers. The dust measurements were carried out in accordance with the protocols defined within the US EPA approved exposure-profiling method for unpaved roads [20]. Three Respicone multistage Virtual Impactors were mounted on a dust sampling tower located 5 m downwind of the haul road, to sample the dust concentration at three different heights above the haul road surface (0.75, 1.5 and 3 m above the tower base). A fourth Virtual Impactor was installed at a height of 1.5 m above the ground level on a second tower located upwind of the same road to measure the upwind background dust concentration. A weather station connected to a portable PC was also mounted on the upwind tower to record the wind speed and direction, the temperature and the relative humidity of the air. The wind speeds at the corresponding dust sampling heights were determined from the average wind speed recorded by the weather station and the application of a power law equation used to estimate the wind profile over a defined height range [18]. A schematic representation of the location of the dust samplers is shown in Figure 4. The dust measurements were collected on a sunny day under convective stable atmospheric conditions. The haulage trucks travelled along a dry unpaved road surface, which were the environmental conditions experienced on a typical working day during the spring and summer seasons. A number of road surface dirt samples were collected for subsequent analysis to determine the moisture content and the silt percentage. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 International Journal of Mining, Reclamation and Environment 329 Figure 4. A schematic of the relative locations of the upwind and downwind dust samplers and weather station to comply with the sampling protocol of the exposure-profiling method. Table 3. Truck haulage transit data recorded during the field dust survey collection programmes. Haul truck (loaded) Haul truck (empty) No. of transits Min speed [km/h] Max speed [km/h] 38 18 7.3 9.0 21.8 21.2 Table 3 indicates the number of sampled truck transits and the average vehicle speeds recorded during the sampling periods. Elaboration of emission factors The PM10 and PM2.5 emission factors were determined for each truck transit according to Equation (2) [21]. ( ) M N X X E¼ Dt cos hj uij Cij Dzi (2) j¼1 i¼1 where E = PM emission in grams per vehicle kilometre travelled [g/VKT]; Δt = sampling period of dust sampler (Δt = 1 s); θj = angle between the mean wind direction and the perpendicular to the road centreline; uij = average wind speed at time tj at i‐th 330 L. Piras et al. Table 4. The average dust emission factors determined from an analysis of the collected field dust measurements [16]. Vehicle No. of transits PM2.5 E [g/VKT] PM10 E [g/VKT] 34 13 158 100 1560 812 Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 Dump truck (loaded) Dump truck (empty) sampler position on the downwind tower [m/s]; Cij = PM concentration at time tj as measured by the i‐th sampler [mg/m3]; Δzi = vertical interval represented by the i‐th sampler [m]; M = number of Δt included in the event; and N = number of samplers on the downwind tower (N = 3). The emission factors for the haul road under investigation were determined for the transit of a fully loaded and an empty truck. Table 4 reports the mean value of the dust emission factors determined for a truck travelling at different speeds. According to the US EPA AP42 dust emission model guidelines for truck haulage on unpaved roads [22], the transits that took place when the angle between the wind direction and the perpendicular to the road centre line exceeded 45° were excluded from the calculation of the average emission factors. The ratio of the PM2.5 and PM10 emission factors (EFPM2.5/EFPM10) determined from the field measurements collected was computed to be approximately 0.1 for both the loaded and unloaded truck conditions, which is within the accepted range for the US EPA method [23]. Comparison of measured and estimated emission factors The emission factors determined from an analysis of the field measurements were compared to the emission factors estimated by the use of Equation (3), which represents the latest version of the US EPA AP-42 haul road fugitive dust emissions estimate [22]: s a W b E¼k (3) 12 3 where E = size-specific emission factor in grams per vehicle kilometre travelled [g/VKT]; s = road surface material silt content [%]; W = mean vehicle weight [tons]; and a, b = parameters dependant on the particulate size range. The emission factors derived from the field measurements (Measured E) and the emission factors estimated on the basis of the EPA Equation (3) (Estimated E) are reported in Table 5. A comparative analysis of the two sets of values concluded that the computational model overestimates the measured values by a factor of between 1.08 and 1.25. Modelling methodology Representation of mobile sources A number of different modelling methodologies have been proposed to represent the fugitive dust emission sources within atmospheric dispersion models. The simplest method is to represent the source as a continuous line source, the total emission being Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 International Journal of Mining, Reclamation and Environment 331 uniformly distributed along the length of the road centreline and determined by the speed, tonnage and frequency of the haul trucks [11]. The emission factor may be either estimated from measurements taken on-site or in accordance with the haul road dust emission models defined by US EPA AP-42 manual [22]. Organisiak and Reed [24] carried out field studies at a limestone quarry and coal preparation plant, to quantify the fugitive dust emission and dispersion experienced from the transit of haulage trucks along unpaved roads. The results of these studies support the representation of these mobile sources as an area or volume-distributed sources [25] and suggest the definition of an adjusted road width given by the actual road width plus 6 m, to represent the horizontal extent of the wake arising from the transit along the road. Reed and Westman [6] developed a modified emission model to improve the reliability of the use of the Gaussian model ISC3 (Industrial Source Complex model) to replicate the observed total fugitive dust emission arising from an unpaved road. The emission is represented as a set of equidistant spaced point sources distributed along the length of the road. The results of a recent modelling study carried out by Joseph [26], to investigate the use of the UK-ADMS Gaussian plume dispersion model, concluded that the use of a series of non-overlapping point emission sources appeared to best replicate the haul road emissions and dispersion experienced at a surveyed quarry under variable meteorological conditions and downwind terrain conditions. Adopting the modelling strategy proposed by Joseph, the haul road under investigation was modelled as a series of non-overlapping point sources with a 5 m diameter, which corresponds to the width of the trailing truck plumes observed during field measurements. The total haul road distance travelled by the haulage trucks on a single trip from the crushed limestone source pile to the tailings dump was approximately 1200 m. Consequently, a series of 240 equidistant emission point sources were distributed along the linear length of the unpaved haulage road within the UK-ADMS model solution domain. Each individual fugitive dust source release point was set 1.5 m above the road surface, which corresponds to the mid height of the actual observed emission plumes during the vehicle transits. Emission rates In accordance with the US EPA fugitive dust emission guidance notes on dust sampling, a ratio of the PM10 to TSP emission factors, (EPM10/ETSP) of 0.3, was used to estimate the TSP emission factors associated with the transits of both the empty and fully loaded haulage trucks: ETSP (empty haulage truck) = 2707 [g/VKT ] and ETSP (fully loaded haulage truck) = 5200 [g/VKT]. The consistency of such an assumption is confirmed by the results of the field study carried out by Organisiak and Reed [24], who found that the majority of Table 5. Measured and estimated emission factors for the three PM fractions. Load condition Size fraction Empty dumper PM2.5 PM10 TSP PM2.5 PM10 TSP Loaded dumper Measured E [g/VKT] Estimated E [g/VKT] 100 812 na 158 1560 na 109 1092 3399 176 1759 5475 332 L. Piras et al. Table 6. TSP emission factors and TSP emission rates determined from the survey of the unpaved haul road. Dust source Working condition Haul road empty haulage truck loaded haulage truck TSP emission factor [g/VKT] 2707 5200 TSP emission rate [g/s] 5.46 10.49 Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 dust generated from unpaved and untreated haulage roads is non-respirable and at least 80% of the airborne dust has an aerodynamic diameter size larger than 10 μm. The TSP emission rates determined for the unpaved road on the mineral remediation site are reported in Table 6. Topography The former mine reclamation site is located within a valley at an elevation of between 50 and 425 m above the sea level. The area may be considered as an aerodynamically complex terrain, where the slopes of the valley sides in close vicinity to the haul road have a gradient of between 25 and 75%. To investigate the effect that the surrounding topography may have on the predicted dust plume dispersion, a number of UK-ADMS model simulations were performed. To define the solution domain for the models requires the specification of the surface terrain in terms of the spatial variation in elevation. A digital elevation model of the actual topography (with a spatial resolution of 10 m) was obtained from the Regione Sardegna. A preliminary series of grid size solution sensitivity exercises were performed to ensure that the predicted dispersion and deposition solutions obtained were grid size independent [27]. Figure 5 shows a representative contour relief map of the area and indicates the positions of the surveyed haul road (bold black line), the limestone stockpile (location A) and the tailings dump emplacement site (location B). Meteorological data The meteorological data for surveyed region over the previous 30 years were analysed to determine the statistical frequency distributions of the predominant seasonal wind speeds and directions. The analysis confirmed that most frequent wind direction for this region was from the north-west direction (315° measured clockwise from the North) which corresponds to the dominant regional wind called the maestrale. This predominant wind system was prevalent during the dust sampling survey period and was therefore used to simulate the predicted plume dispersion and deposition within the UK-ADMS model valleys. To investigate the potential dust plume dispersion that may be experienced transversely across the same valley, model simulations were subsequently performed employing a cross-valley 45° wind direction. A series of parametric modelling studies were performed to predict the dispersion of the observed dust plumes for both the identified principal wind directions under unstable, neutral and stable atmospheric stability conditions. Table 7 summarises the meteorological input parameters used to conduct the UK-ADMS model simulations. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 International Journal of Mining, Reclamation and Environment 333 Figure 5. Contour relief map of the area indicating the positions of the surveyed haul road (bold black line), the limestone stock piles (location A) and the tailings dump emplacement site (location B). Simulation results Preliminary modelling across flat terrain Preliminary benchmark model simulation studies were performed across a flat terrain to investigate the plume dispersion arising from the haul road under different meteorological conditions in the absence of the influence of any surrounding complex topography. As was expected, under convective atmospheric conditions (stability class A), the horizontal plume dispersion is constrained and the maximum value of dust Table 7. Meteorological input data used for the ADMS simulation models that correspond to the unstable (A), neutral (D) and stable (F) Pasquill atmospheric stability classes [11]. Wind direction [°] 315 315 315 45 45 45 Wind speed [m/ s] Surface heat flux [W/m2] 1 5 2 1 5 2 113 0 −6 113 0 −6 Boundary layer height [m] 1300 800 100 1300 800 100 Stability class A D F A D F Figure 6. Predicted hourly averaged TSP particulate concentrations across a flat terrain under convective (Class A), neutral (Class D) and stable (Class F) atmospheric stability conditions under the influence of a 315° wind direction. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 334 L. Piras et al. International Journal of Mining, Reclamation and Environment 335 Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 concentration is observed very close to the source. Larger downwind plume transport distances are predicted under neutral stability conditions, which are also accompanied by a wider predicted areal dispersion and deposition. The maximum plume advection is found for very stable conditions (stability class F) for a low boundary layer height (100 m above the ground) which suppresses the vertical rise of the plume. Figure 6 shows the hourly averaged TSP concentrations predicted across a flat terrain subject to a 315° wind direction under representative unstable, neutral and stable atmospheric conditions. Influence of topography A further series of model simulations were performed to study the influence of the surrounding complex topography on the predicted plume dispersion across the range of atmospheric stability conditions described in Table 7. The UK-ADMS simulation model calculates the plume dispersion over a given terrain by first determining the flow field generated by the defined wind direction and speed by using a calculation sub-model called FLOWSTAR. The FLOWSTAR model computes the near-surface flow fields over terrains with gradients up to 1:3. Validation studies performed by Carruthers et al. [7] confirmed that the FLOWSTAR model simulations are reliable over ranges of between tens of metres to several kilometres, for gradients up to 1:3 in hill wakes and up to 1:2 for upwind slopes and hill summits [10]. The simulation of the plume dispersion predicted along the length of the valley, which corresponds to the most frequently experienced scenario, has been analysed using the actual topography together subject to the predominant north-westerly wind direction. As shown in Figure 7, the simulation of the three different stability conditions produces significantly different behaviour in the predicted plume dispersions. The relative confinement of the plume in the near vicinity of the source under the influence of the highly convective unstable Class A stability conditions does not indicate a strong influence of the topography. However, the higher wind speeds used to simulate neutral stability conditions (class D) result in a distinct channelling of the plume path by the confining valley sides. However, the downwind travel length and lateral spread achieved by the predicted plume were found to be dependent on the resolution scale of the flow field. The FLOWSTAR sub-model permits the use of different grid resolutions to model the flow field, whilst maintaining the same terrain file. An analysis of the flow grid resolution studies concluded that for higher grid resolutions, the plumes were predicted to penetrate further along the valley. It was concluded that under stable atmospheric condition (class F), the downwind travel of the predicted plume trajectory is arrested by the influence of a local flow reversal (recirculation) experienced at the base of the hill slope. Figure 8 shows the predicted plume dispersion across the valley subject to a 45° wind direction under unstable, neutral and stable atmospheric conditions. Under the highly convective unstable (Class A) conditions, the path of the plume is observed to be channelled by the valleys slopes, with the maximum concentrations of the plume being confined near to the source of emission. Under neutral atmospheric conditions (class D), the path of the predicted plume is observed to be strongly channelled by the combined influences of the higher surface wind flows and the confinement of the local topography. Under stable atmospheric conditions (Class F), the areal extent of the predicted dust dispersion is confined by the slopes of the surrounding valley. The Figure 7. Hourly averaged TSP dust concentrations simulated within the actual field terrain under convective (Class A), neutral (Class D) and stable (Class F) atmospheric stability conditions under the influence of a 315° wind direction. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 336 L. Piras et al. Figure 8. The predicted hourly averaged TSP plume concentrations for the actual terrain under convective (Class A), neutral (Class D) and stable (Class F) atmospheric conditions subject to a 45° wind direction. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 International Journal of Mining, Reclamation and Environment 337 338 L. Piras et al. Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 lateral confinement of the plume is much greater than that predicted for the highly convective stability class A. The inclusion of the actual topography creates a reversal of the local flow field within a 30 m height above the ground at the base of the rising slope of the adjacent main hill. A comparative analysis of the predicted plume concentrations at different heights (0 m, 25 m, 50 m, 75 m, 100 m) above the ground level concluded that under the same meteorological conditions, the vertical rise of the simulated plumes over the actual terrain was higher than those predicted. Figure 9. Deposition rates simulated for the flat and the actual complex real terrain under stable conditions and 45° wind direction. Dry deposition The predicted dry deposition rates were determined for all the simulation scenarios described above. The results predicted for 45° and 315° wind directions under both the unstable convective (class A) and neutral (Class D) atmospheric stability conditions were as expected. However, under the simulated stable (Class F) atmospheric conditions, the predicted deposition rates were higher than expected for both the flat and real complex topographies. For cross-valley plume dispersion under stable conditions (class F), the comparison between the simulations performed with flat and real topography produced a surprisingly higher rate of deposition over the flat terrain (Figure 9). An examination of the calculation method used by UK-ADMS to model dry deposition may explain the differences in these predicted deposition rates. The dry deposition rate is defined as equal to the product of the particle deposition velocity and the ground-level concentration, Equation (4) [11]. Consequently, the lower predicted ground-level dust concentrations determined for cross-valley dispersion under stable atmospheric conditions will necessarily lead to lower deposition rates. F ¼ vd Cðx; y; 0Þ 2 (4) where F = rate of deposition per unit area [μg/ s·m ]; vd=particle deposition velocity [m/s]; and C (x, y, 0) = ground-level concentration at the point (x, y). International Journal of Mining, Reclamation and Environment 339 Downloaded by [Universita Degli Studi di Cagliari] at 03:15 12 November 2014 Conclusions In recent years, there has been significant research effort to investigate the use of plume dispersion models to assess the environmental impact of fugitive dust emissions from surface mining operations. In particular, the results of these studies have identified challenges to the use of traditional Gaussian plume dispersion models to satisfactorily reproduce fugitive dust dispersion and deposition experienced from low elevation release heights within complex topography. Recent studies have highlighted the need to more accurately define and assess the fugitive dust emission factors used with predictive atmospheric dispersion models. This paper discusses the results of an application of the UK-ADMS model to predict the fugitive dust plume dispersion and deposition experienced at a former mining site currently undergoing remediation. The UK-ADMS model employs a sub-model FLOWSTAR to compute the near-surface flow field over complex terrains. Previous research studies have confirmed the reliability of this sub-model to replicate these flows over ranges of between tens of metres to several kilometres from the dust emission source, and across surfaces possessing gradients of up to 1:3 for hill wakes and of up to 1:2 for upwind slopes and hill summits. This paper summarises the results of a PM10 and PM2.5 dust sampling survey that was conducted along the length of an unpaved haul road at a former mineral property that is being remediated. The results of this survey were used to compute the actual dust emission factors for the truck haulage activities conducted along this road. Unpaved road haulage truck dust emission factors were also computed using the revised AP42 emission models proposed by the US EPA. A comparative analysis of the values produced by both methods showed satisfactory agreement. To investigate the effect that surrounding topography may have on the dispersion of generated dust plumes, a series of UK-ADMS models were solved for a number of different meteorological and atmospheric stability conditions. An analysis of the results of these studies concludes that the surrounding complex topography can have a strong influence on the dispersion and deposition of the dust plumes generated from the haul road. However, the results of this preliminary study need to be further investigated and validated against further dust dispersion and deposition data collected in the field. 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