Supplement of Hydrol. Earth Syst. Sci., 18, 5255–5269, 2014 http://www.hydrol-earth-syst-sci.net/18/5255/2014/ doi:10.5194/hess-18-5255-2014-supplement © Author(s) 2014. CC Attribution 3.0 License. Supplement of Relations between macropore network characteristics and the degree of preferential solute transport M. Larsbo et al. Correspondence to: M. Larsbo ([email protected]) 1 2 3 4 Supplementary material Table S1. Column lengths and average irrigation rates at the nominal irrigation rates used in the breakthrough experiments. Standard deviations are given in parenthesis. Column Säby 1 (loam) a Säby 1 (loam) b Säby 1 (loam) c Säby 1 (loam) d Säby 1 (loam) e Säby 2 (clay) a Säby 2 (clay) b Säby 2 (clay) c Säby 2 (clay) d Säby 2 (clay) e Ultuna a Ultuna b Ultuna c Ultuna d Ultuna e Krusenberg a Krusenberg b Krusenberg c Krusenberg d Krusenberg e Average 5 Length (mm) 169 168 183 173 175 167 169 174 169 NA 170 161 170 169 NA 150 166 162 168 159 168 Average irrigation rate (mm h-1) at a nominal irrigation rate of 2 mm h-1 1.9 (0.06) 1.9 (0.06) 2.0 (0.07) 1.8 (0.11) 2.1 (0.06) 2.1 (0.05) 1.9 (0.34) 2.1 (0.28) 2.0 (0.10) NA 2.0 (0.08) 1.9 (0.05) 2.0 (0.06) 2.0 (0.06) Ponding 2.0 (0.05) 2.0 (0.02) 2.0 (0.03) 2.0 (0.09) 1.9 (0.06) 2.0 (0.09) 4 mm h-1 4.1 (0.13) 3.5 (0.33) 4.1 (0.18) 3.4 (0.58) 3.9 (0.06) 4.2 (0.07) Ponding 4.0 (0.17) 3.8 (0.00) NA 4.3 (0.25) 4.1 (0.15) 3.5 (0.53) 3.9 (0.09) Ponding 4.1 (0.08) 4.0 (0.10) 3.9 (0.13) 4.0 (0.09) 3.7 (0.21) 3.9 (0.18) 6 mm h-1 6.0 (0.04) 5.9 (0.87) 5.9 (0.16) 5.9 (0.18) 5.9 (0.32) 6.2 (0.21) Ponding Ponding 6.4 (0.38) NA 5.9 (0.06) Ponding Ponding 6.2 (0.46) Ponding 6.1 (0.08) 6.0 (0.08) 6.3 (0.42) 5.7 (0.09) 5.9 (0.32) 6.0 (0.26) 8 mm h-1 7.7 (0.18) 7.7 (NA) 7.9 (0.13) 7.8 (0.49) Ponding 8.5 (0.08) Ponding Ponding 7.3 (NA) NA 7.7 (0.61) Ponding Ponding 8.2 (0.49) Ponding 7.8 (0.77) 7.2 (NA) 8.0 (NA) 7.6 (NA) 7.8 (0.08) 7.8 (0.35) 12 mm h-1 10.6 (NA) 13.9 (NA) 14.2 (NA) 13.1 (NA) Ponding 11.1 (NA) Ponding Ponding 10.6 (NA) NA 10.9 (NA) Ponding Ponding 13.1 (NA) Ponding 12.8 (NA) 14.5 (NA) 13.6 (NA) 13.2 (NA) 12.2 (NA) 12.6 (NA) 1 Table S2. Macropore system characteristics. Column Säby 1 (loam) a Säby 1 (loam) b Säby 1 (loam) c Säby 1 (loam) d Säby 1 (loam) e Säby 2 (clay) a Säby 2 (clay) b Säby 2 (clay) c Säby 2 (clay) d Säby 2 (clay) e Ultuna a Ultuna b Ultuna c Ultuna d Ultuna e Krusenberg a Krusenberg b Krusenberg c Krusenberg d Krusenberg e 2 3 Macroporosity Hydraulic radius 0.071 0.051 0.076 0.052 0.050 0.122 0.042 0.033 0.052 Specific macropore surface area mm2 mm-3 0.061 0.039 0.064 0.040 0.037 0.079 0.032 0.019 0.037 Mean aggregate thickness mm 55 65 51 65 60 51 58 79 64 Fractal dimension Global connectivity mm 1.2 1.3 1.2 1.3 1.4 1.5 1.3 1.8 1.4 Mean pore thickness mm 1.8 1.3 1.5 1.6 1.3 3.6 1.3 2.0 1.6 2.50 2.47 2.54 2.44 2.49 2.54 2.43 2.34 2.42 1 1 1 1 1 1 0 1 1 0.065 0.049 0.037 0.078 0.052 0.039 0.027 0.069 1.2 1.2 1.4 1.1 2.1 1.4 1.3 1.8 71 79 74 47 2.43 2.38 2.36 2.52 1 1 0 1 0.075 0.073 0.072 0.092 0.086 0.056 0.060 0.060 0.075 0.064 1.3 1.2 1.2 1.2 1.3 2.0 1.6 1.7 1.9 2.5 56 49 48 47 56 2.49 2.51 2.51 2.54 2.49 1 1 1 1 1 1 2 Table S3. Characteristics of the largest cluster connecting the soil surface to the bottom of the sample. The data are for the largest non-connected cluster for cases when such a cluster did not exist (i.e. when Global connectivity = 0 in table S3). Column Säby 1 (loam) a Säby 1 (loam) b Säby 1 (loam) c Säby 1 (loam) d Säby 1 (loam) e Säby 2 (clay) a Säby 2 (clay) b Säby 2 (clay) c Säby 2 (clay) d Säby 2 (clay) e Ultuna a Ultuna b Ultuna c Ultuna d Ultuna e Krusenberg a Krusenberg b Krusenberg c Krusenberg d Krusenberg e 3 4 Fraction of macropore volume 0.91 0.87 0.91 0.81 0.83 0.92 0.79 0.79 0.78 Mean pore thickness mm 2.2 1.7 1.8 2.1 1.7 4.5 1.7 3.1 2.2 Euler number Tortuosity -24000 -21700 -27200 -21300 -21300 -16400 -18900 -14900 -19600 Critical pore diameter mm 0.77 0.48 0.73 0.24 0.59 1.7 NA 0.24 0.24 0.93 0.89 0.83 0.91 2.7 1.8 1.6 2.2 -26300 -26900 -26100 -30800 0.87 0.77 NA 1.08 1.5 2.0 NA 1.7 0.85 0.87 0.89 0.91 0.72 2.5 2.0 2.1 2.4 3.5 -23900 -29600 -28800 -31100 -24400 0.54 0.24 0.24 0.77 0.73 2.7 1.1 1.1 2.2 1.6 2.7 1.8 1.3 1.5 2.2 1.2 NA 1.4 1.2 1 Table S4. Measures of preferential transport for the irrigation rates used in the breakthrough experiments. Column Säby 1 (loam) a Säby 1 (loam) b Säby 1 (loam) c Säby 1 (loam) d Säby 1 (loam) e Säby 2 (clay) a Säby 2 (clay) b Säby 2 (clay) c Säby 2 (clay) d Säby 2 (clay) e Ultuna a Ultuna b Ultuna c Ultuna d Ultuna e Krusenberg a Krusenberg b Krusenberg c Krusenberg d Krusenberg e 2 5 % arrival time (-) at a nominal irrigation rate of 2 mm h-1 4 mm h-1 6 mm h-1 8 mm h-1 12 mm h-1 0.25 0.19 0.07 0.07 0.06 0.29 0.07 0.08 0.10 0.10 0.28 0.16 0.14 0.14 0.11 0.26 0.21 0.11 0.11 0.07 0.31 0.21 0.11 Ponding Ponding 0.38 0.33 0.34 0.27 0.26 0.24 Ponding Ponding Ponding Ponding 0.04 0.12 Ponding Ponding Ponding 0.26 0.21 0.18 0.19 0.18 Not used Not used Not used Not used Not used 0.35 0.36 0.32 0.23 0.20 0.26 0.29 Ponding Ponding Ponding 0.07 0.12 Ponding Ponding Ponding 0.34 0.32 0.36 0.33 0.34 Ponding Ponding Ponding Ponding Ponding 0.50 0.35 0.33 0.27 0.22 0.52 0.42 0.41 0.37 0.30 0.52 0.42 0.39 0.38 0.36 0.47 0.39 0.33 0.28 0.25 0.45 0.42 0.35 0.26 0.11 Apparent dispersivity (cm) at a nominal irrigation rate of 2 mm h-1 4 mm h-1 6 mm h-1 8 mm h-1 12 mm h-1 7.8 9.1 14.4 15.5 20.1 5.1 12.0 13.0 13.1 15.8 5.6 9.5 11.0 12.7 14.9 5.2 7.9 11.4 12.4 17.1 7.0 9.0 14.0 Ponding Ponding 4.8 6.6 6.3 7.7 8.4 11.8 Ponding Ponding Ponding Ponding 20.5 20.1 Ponding Ponding Ponding 12.6 12.6 13.3 14.5 16.5 Not used Not used Not used Not used Not used 7.4 8.6 9.8 13.0 14.4 13.6 13.3 Ponding Ponding Ponding 26.4 25.5 Ponding Ponding Ponding 6.5 7.2 6.7 7.8 7.6 Ponding Ponding Ponding Ponding Ponding 2.6 4.5 5.4 7.6 7.5 2.5 3.6 4.6 5.8 5.9 2.4 3.6 4.3 4.9 5.1 3.1 4.5 6.0 6.7 7.2 4.0 4.9 6.5 8.0 10.9 1 2 3 4 Figure S1. Tracer breakthrough curves for the Säby 1 (loam) soil at the different steady-state flow rates. T is dimensionless time. 1 2 3 4 5 Figure S2. Tracer breakthrough curves for the Säby 2 (clay) soil at the different steady-state flow rates. T is dimensionless time. 1 2 3 4 5 Figure S3. Tracer breakthrough curves for the Ultuna (clay) soil at the different steady-state flow rates. T is dimensionless time. 1 2 3 4 Figure S4. Tracer breakthrough curves for the Krusenberg (clay loam) soil at the different steadystate flow rates. T is dimensionless time.
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