Pure Appl. Geophys. 2016 Springer International Publishing DOI 10.1007/s00024-016-1461-2 Pure and Applied Geophysics A Stress Condition in Aquifer Rock for Detecting Anomalous Radon Decline Precursory to an Earthquake T. KUO,1 H. KUOCHEN,2 C. HO,3 and W. CHEN4 Abstract—Recurrent groundwater radon anomalous declines were observed from well measurements in the Antung hot spring area (eastern Taiwan) prior to five of six earthquakes that occurred between 2003 and 2011 (Mw range 5.0–6.8). The relationship between the detectability of radon anomalies and the first motions of P-waves was investigated. Based on the first motions of P-waves recorded near the investigated well, a precursory decrease in groundwater radon can be detected only when the first motion is compression. No precursory change in groundwater radon concentration was observed for the downward first motion of P-waves. Key words: Radon-222, Groundwater, Earthquakes, P waves, Stress. 1. Introduction Radon concentration variations (Radon-222) in groundwater have been frequently proposed as earthquake precursor (Noguchi and Wakita 1977; Shapiro et al. 1980; Wakita et al. 1980; Igarashi et al. 1995; Papastefanou 2002; Kuo et al. 2006a; Zmazek et al. 2006; Erees et al. 2007; Yalim et al. 2007; Namvaran and Negarestani 2013; Hashemi et al. 2013; Tarakçi et al. 2014; Tuccimei et al. 2015; Attanasio and Maravalle 2016). According to a worldwide survey (Hauksson 1981), more than 80% of radon anomalies measured in groundwater prior to earthquakes shows increases in radon concentration. Radon-222 is a chemically inert radioactive gas with a half-life of 3.82 days. The radon concentration in 1 Department of Mineral and Petroleum Engineering, National Cheng Kung University, Tainan, Taiwan. E-mail: [email protected] 2 Institute of Geophysics, National Central University, Jhongli, Taiwan. 3 Central Weather Bureau, Taipei, Taiwan. 4 Department of Geosciences, National Taiwan University, Taipei, Taiwan. groundwater is proportional to the uranium concentration (Uranium-238) in adjacent rocks. Because of radon’s short recoil length (3 9 10-8 cm), only atoms produced at the surface of rock grains are released to the adjacent groundwater. Therefore, the concentration of radon in groundwater is largely dependent on the surface area of adjacent rocks (Torgersen et al. 1990; Tuccimei et al. 2015). Before the occurrence of an earthquake, regional stress increases causing formation of cracks in the rocks. Thus, prior to earthquakes, both the surface area of the rocks and the radon concentration in groundwater increase (Igarashi et al. 1995; Tuccimei et al. 2015). A few anomalies measured in groundwater manifested decreases in radon concentration (Wakita et al. 1980; Shapiro et al. 1980; Kuo et al. 2006a). Anomalous decreases in radon concentration were observed in groundwater prior to the Japan 1978 IzuOshima-Kinkai earthquake of magnitude M 7.0 (Wakita et al. 1980), prior to the U. S. 1979 Malibu earthquake of magnitude M 4.6 (Shapiro et al. 1980) and prior to the Taiwan 2003 Chengkung earthquake of magnitude Mw 6.8 (Kuo et al. 2006a). The 2003 Mw 6.8 Chengkung was the strongest earthquake near the Chengkung area in eastern Taiwan since 1951. Mechanisms and geological conditions for interpreting anomalous decreases in radon prior to earthquakes are seldom discussed in the literature. The Antung hot spring is a low-porosity fractured small aquifer situated in an andesitic block and surrounded by a ductile mudstone of the Lichi mélange (Chen and Wang 1996). Regarding a physical basis that explains the anomalous decrease in radon concentration in groundwater prior to the 2003 Chengkung earthquake, a mechanism of radon volatilization was presented based on radon phase T. Kuo et al. Pure Appl. Geophys. behavior and the geological conditions of the Antung hot spring (Kuo et al. 2006b). We have studied recurrent anomalous declines in the concentration of groundwater radon at the Antung hot spring in eastern Taiwan since July 2003. The radon-monitoring well is located about 3 km southeast of the Longitudinal Valley fault (Fig. 1). The fault ruptured during two 1951 earthquakes of magnitudes M 6.2 and M 7.0 (Hsu 1962). The Longitudinal Valley fault is part of the eastern boundary of the present-day plate suture between the Eurasia and the Philippine Sea plates. Between July 2003 and December 2013, six main earthquakes occurred near the Antung hot spring (Fig. 1). Anomalous decreases in the concentration of groundwater radon were observed prior to the 2003 Chengkung Mw 6.8, 2006 Taitung Mw 6.1 and Mw 5.9, 2008 Antung Mw 5.4, and 2011 Chimei Mw 5.0 earthquakes (Kuo 2014). Nonetheless, no anomalous decline in the concentration of groundwater radon was detected at the radon-monitoring well prior to the 2013 Rueisuei Mw 6.3 earthquake. A low-porosity fractured aquifer in un-drained conditions near an active fault is a suitable geological site to detect precursory declines in groundwater radon prior to local large earthquakes (Kuo 2014). Besides, stress conditions in aquifer rock can affect the detectability of precursory radon declines. The first motion of the P-waves provides the radiation pattern of body waves at the time of the earthquake Figure 1 Map of the epicenters of the earthquakes that occurred on December 10, 2003, April 1 and 15, 2006, February 17, 2008, July 12, 2011, October 31, 2013 near the Antung hot spring. a Map of Taiwan. b Study area near the Antung hot spring (filled stars mainshocks, filled triangle radon-monitoring well, filled square seismic station HWA055) A Stress Condition in Aquifer Rock for Detecting Anomalous Radon Decline… (nearly instantaneous process). Assuming the doublecouple mechanism, the radiation pattern representing a source (for normal, thrust or strike slip fault) is described by four areas (Shearer 2009). Two areas are characterized by compression (upward first motion for P-waves at a hypothetical station within this area) and two areas are characterized by tension (downward first motion for P-waves at a hypothetical station within this area). We further assume that a similar stress pattern exists in rocks before and at the time of the earthquake. The purpose of this work is to examine the possible relationship between radon anomalies and the first motions of P-waves recorded near the radon-monitoring well for the above six main earthquakes. 2. Materials and Methods 2.1. Geological Setting The Antung area is in a unique tectonic setting located at the boundary between the Eurasian and Philippine Sea plates. Figure 2 shows the geological map and cross section near the radon-monitoring well D1 in the Antung area. The Antung hot spring is situated in an andesitic tuffaceous-sandstone block (Miocene) which is enclosed within the Paliwan Formation (Late Pliocene to Pleistocene) of alternating thin-bedded sandstone and shale. The hot spring is formed nearby an eastward-dipping, high-angle reverse fault zone which contacts between the Lichi mélange and the Paliwan Formation. Some hot springs and mud volcanoes are scattered along the fault zone, indicating a Quaternary active fault. Four stratigraphic units are present (Chen and Wang 1996). The Tuluanshan Formation consists of Miocene volcanic units such as lava and volcanic breccia, as well as tuffaceous sandstone. The Fanshuliao (Pliocene) and Paliwan (Late Pliocene to Pleistocene) Formations consist of rhythmic sandstone and mudstone turbidites. The Lichi mélange occurs as a highly deformed mudstone that is characterized by penetrative foliation visible in outcrop. Well-developed minor faults and joints are common in the tuffaceous-sandstone block displaying intensively brittle deformation. It is possible that these fractures reflect deformation and disruption by the nearby faults. Ground water flows through the fault zone and is then diffused into the block along the minor fractures. The radon-monitoring well D1 is not artesian, implying a weak recharge to a small aquifer in un-drained conditions. Hence, geological evidence suggests that the Antung hot spring at well D1 is a small low-porosity fractured aquifer in undrained conditions near an active fault. Under such geological conditions as the Antung hot spring, two physical processes, rock dilatancy and water diffusion, are likely to take place. When the regional stress increases to about half the fracture stress, rock dilatancy initiates and cracks develop in aquifer rock (Brace et al. 1966). According to the dilatancy-diffusion model (Nur 1972; Scholz et al. 1973), the development of new cracks in the aquifer rock could occur at a rate faster than the recharge of pore water. In a small aquifer with un-drained conditions, gas saturation could develop in the rock cracks. When gas phase develops in aquifer rock, the radon in groundwater volatilizes into the gas phase and the radon concentration in groundwater decreases. The above mechanism is also referred to as ‘‘in situ radon volatilization’’ (Kuo et al. 2006b). Carminati et al. (2004) analyzed the migration of seismicity on thrust and normal faults. The study reports that, in compressional regimes, fractures preferentially generate at shallow depths and propagate downward. Doglionia et al. (2011, 2013) devised a simplified two-layer model to study fault activation with a fault cross-cutting the brittle upper crust and the ductile lower crust. The study shows that, along a thrust fault, the hanging wall is over-compressed during the interseismic, and should dilate at the coseismic stage. Figure 2 shows that the Antung hot spring is situated at the hanging wall along the Yongfeng Fault and the Longitudinal Valley Fault, both of which are thrust faults. Dilatant expansion can develop in aquifer rock precursory to large earthquakes near Antung. 2.2. Seismic Data Seismic data (geographical coordinate of epicenter and depth) were taken from earthquake catalogues of Central Weather Bureau, Taiwan. Focal mechanisms and Mw (moment magnitude scale) were from T. Kuo et al. Pure Appl. Geophys. Figure 2 Geological map and cross section near the radon-monitoring well D1 in the area of Antung hot spring. (B tuffaceous andesitic blocks; filled black triangle radon-monitoring well D1; Chihshang, or, Longitudinal Valley Fault, ` Yongfeng Fault) the Global CMT catalog search. Two groups of earthquakes were selected for this study. For the first group, we selected all the mainshocks (Mw [ 6.0) that occurred near the Autng hot spring between December 10, 2003 and October 31, 2013. The 2003 Mw 6.8 Chengkung, 2006 Mw 6.1 Taitung, and 2013 Mw 6.3 Rueisuei earthquakes are the search results from the Global CMT catalog. For the second group, we selected all the mainshocks (Mw [ 5.0) that occurred between December 10, 2003 and October 31, 2013 with epicenters located on the Longitudinal Valley fault. The 2006 Mw 5.9 Taitung, 2008 Mw 5.4 A Stress Condition in Aquifer Rock for Detecting Anomalous Radon Decline… Antung, and 2011 Mw 5.0 Chimei earthquakes are the search results from the Global CMT catalog. The focal mechanisms of the above six events are shown in Fig. 1. Only event 2 (April 1, 2006) is strike-slipfaulting. All the other events are thrust-faulting. 2.3. Radon-monitoring Methods Discrete samples of groundwater were pumped and collected from the radon-monitoring well D1 located at the Antung hot spring twice per week for analysis of radon content. The production interval of the well ranges from 167 to 187 m below ground surface. Every sampling started with flushing the stagnant water in the monitoring well and in the screen zone. An insufficiently pumped volume represents a major source of error. A minimum of three well-bored volumes were purged before taking samples for radon measurements. To achieve the above criterion, a minimum of 50 min purging-time was required with a pumping rate at around 200 L/min. Water samples were collected in a 40 mL glass vial with a TEFLON-lined cap. It is important to ensure the radon not to escape during the sampling procedure and the sample transportation and preparation. After collecting a sample, the sample vial was inverted to check for air bubbles. If any bubbles were present in the vial, the sample water was discarded and sampling was repeated. The date and time of sample collection were recorded. The samples were stored and transported in a cooler. Counting radioactivity was done within 4 days. The liquid scintillation method was adopted to determine the activity concentration of radon in groundwater (Noguchi 1964). Radon was partitioned selectively into a white mineral-oil based scintillation cocktail (Perkin Elmer) immiscible with the water samples, and then assayed with a liquid scintillation counter (LSC). The results were corrected for the amount of radon decay between sampling and assay. A calibration factor for the LSC measurements of 7.1 ± 0.1 cpm/pCi was calculated using an aqueous Ra-226 calibration solution, which is in secular equilibrium with Rn-222 progeny. For a count time of 50 min and background less than 6 cpm, a detection limit below 18 pCi/L was achieved using the sample volume of 15-ml. Due to the high background noise of radon time series (Fig. 3), environmental records such as atmospheric temperature, barometric pressure, and rainfall were examined to check whether the radon anomaly could be caused by these environmental factors. Prior to the 2003 Mw = 6.8 Chengkung and 2006 Mw = 6.1 Taitung earthquakes, radon concentration in groundwater decreased from background levels of 787 ± 42 and 762 ± 57 pCi/L to minima of 326 ± 9 and 371 ± 9 pCi/L, respectively. There was no heavy rainfall responsible for the above two radon anomalies. Besides, the atmospheric temperature, barometric pressure, and rainfall are periodic in season. It is difficult to explain the above two radon anomalies by these environmental factors. 3. Results and Discussion The sequence of events for radon anomalies prior to the 2003 Chengkung Mw 6.8, 2006 Taitung Mw 6.1 and Mw 5.9, 2008 Antung Mw 5.4, and 2011 Chimei Mw 5.0 earthquakes can all be characterized into three stages (Fig. 4a–d). During stage 1, the radon concentration in groundwater is fairly stable; there is an accumulation of tectonic strain and a slow, steady increase of regional stress. Well D1 in the Antung hot spring is completed in a small low-porosity brittle aquifer surrounded by a ductile formation in undrained conditions. When the regional stress increases under these geological conditions, dilation of brittle rock masses could occur at a rate faster than the rate at which groundwater could diffuse or recharge into the newly created rock cracks (Brace et al. 1966; Nur 1972; Scholz et al. 1973). During this stage (stage 2), gas saturation and two phases (vapor and liquid) develop in the rock cracks. The radon in groundwater volatilizes into the gas phase and the radon concentration in groundwater decreases (Kuo et al. 2006b). Stage 3 starts at the point of minimum radon concentration when the water saturation in cracks and pores begins to increase again. During this stage (stage 3), the radon concentration in groundwater increases and recovers to the previous background level before the main shock. The above recurrent groundwater radon anomalies can be explained based on the dilatancy-diffusion model T. Kuo et al. Pure Appl. Geophys. 1200 1100 1000 900 222Rn (pCi/L) 800 700 600 500 400 300 1 2 6.8 6.1 200 100 Pressure (hPa) 0 1040 1020 1000 980 960 Temperature ( oC ) 940 35 30 25 20 15 10 5 Rainfall (mm) 0 600 500 400 300 200 100 0 2003/7/1 2004/7/1 2005/7/1 2006/7/1 Year/Month/Day Figure 3 Comparison of radon concentration at well D1, atmospheric temperature, barometric pressure, and rainfall data (inside open inverted triangles event number; arrows mainshocks; earthquake magnitude Mw shown beside arrows) A Stress Condition in Aquifer Rock for Detecting Anomalous Radon Decline… 2003 Mw = 6.8 Chengkung Mainshock 1 65 days 787 ± 42 pCi/L 800 600 400 200 326 ± 9 pCi/L Stage 1 0 2003/8/1 3 2 2003/9/1 Radon concentration (pCi/L) 56 days 4 700 ± 57 pCi/L 600 400 480 ± 43 pCi/L 200 Stage 1 0 2 2007/10/1 2007/11/1 2007/12/1 2008/1/1 3 2008/2/1 2 61 days 762 ± 57 pCi/L 3 600 400 200 371 ± 9 pCi/L Stage 1 2 2006/1/1 2006/2/1 3 2006/3/1 (d) 1000 5 2006/4/1 2011 Mw = 5.0 Chimei Mainshock 54 days 752 ± 24 pCi/L 800 600 400 447 ± 18 pCi/L 200 Stage 1 0 2011/3/1 2011/4/1 2 2011/5/1 2011/6/1 3 2011/7/1 2013 Mw = 6.3 Rueisuei Mainshock (e) Radon concentration (pCi/L) 800 2008 Mw = 5.4 Antung Mainshock (c) 1000 1000 0 2005/11/1 2005/12/1 2003/10/1 2003/11/1 2003/12/1 1000 800 Radon concentration (pCi/L) 1000 2006 Mw = 6.1 Taitung Mainshock (b) Radon concentration (pCi/L) Radon concentration (pCi/L) (a) R 724 ± 56 pCi/L 800 600 400 200 0 2013/6/1 2013/7/1 2013/8/1 2013/9/1 2013/10/1 Figure 4 Radon concentration data at well D1 in the Antung hot spring prior to a 2003 Chengkung, b 2006 Taitung, c 2008 Antung, d 2011 Chimei, and e 2013 Rueisuei earthquakes. Green rectangles show radon concentration between the mean radon concentration and three standard deviations below the mean. Stage 1 is buildup of elastic strain. Stage 2 is development of cracks. Stage 3 is influx of groundwater. (a), (b), (c), and (d) from Kuo (2014) (Nur 1972; Scholz et al. 1973) and the mechanism of in situ radon volatilization (Kuo et al. 2006b). Physical models relating precursory phenomena to earthquake occurrence would be useful for interpreting the above recurrent radon anomalies observed at the Antung hot spring. Based on the physical processes of rock dilatancy and water diffusion, Scholz et al. (1973) presented a model to explain a large class of earthquake precursors such as the ratio of seismic velocities vp/vs, electrical resistivity, water flow, geodetic measurements, and number of seismic events. The model is based on laboratory studies of rock dilatancy and fracture. The model assumes that dilatancy precedes the earthquake. The dilatancy- T. Kuo et al. Pure Appl. Geophys. diffusion model consists of three stages. During stage 1, the tectonic stress and strain accumulate. During stage 2, the stress becomes large enough to cause rock dilatancy at a rate faster than the rate of water diffusion. Thus, gas phase develops in the rock cracks during stage 2. During stage 3, the dilatancy rate slows down and the rate of water diffusion is faster than the rate of rock dilatancy. During stage 3, the water saturation increases and the rock cracks become saturated again. The Antung hot spring, a small low-porosity fractured aquifer near an active fault, is a suitable geological site where two physical processes, rock dilatancy and water diffusion, are likely to take place. Thus, the dilatancy-diffusion model is selected to explain groundwater radon anomalous declines recurrently observed in the Antung hot spring area. As shown in Fig. 4a–d, radon concentration of well D1 in the Antung hot spring decreased from background levels of 787 ± 42, 762 ± 57, 700 ± 57, and 752 ± 24 pCi/L to precursory minima of 326 ± 9, 371 ± 9, 480 ± 43, and 447 ± 18 pCi/ L, respectively, prior to the 2003 Chengkung Mw 6.8, 2006 Taitung Mw 6.1 and Mw 5.9, 2008 Antung Mw 5.4, and 2011 Chimei Mw 5.0 earthquakes. The observed precursory minimum in radon concentration decreases as the earthquake magnitude increases. Consequently, recognizing the v-shaped progression in three stages becomes easier as the earthquake magnitude increases (Fig. 4a, b versus c, d). Besides, we can apply standard deviation to test each radon anomaly separately. The mean radon concentration and associated standard deviation are calculated using radon data from stage 1 for each radon anomaly (787 ± 42, 762 ± 57, 700 ± 57, and 752 ± 24 pCi/ L for the 2003 Chengkung Mw 6.8, 2006 Taitung Mw 6.1 and Mw 5.9, 2008 Antung Mw 5.4, and 2011 Chimei Mw 5.0 earthquakes, respectively). An anomaly is defined as a significant deviation from the mean value, or, three standard deviations below the mean value. The green rectangles in Fig. 4 show radon concentration between the mean radon concentration and three standard deviations below the mean. The precursor times before the earthquake occurrence range from 58 to 65 days for the above radon anomalies. Anomalous radon concentrations, smaller than three standard deviations below the mean value, appeared during the precursor times as shown in Fig. 4a–d. Contrary to the above radon anomalies, the radon concentration in groundwater observed at well D1 stayed fairly steady prior to the 2013 Mw 6.3 Rueisuei earthquake that occurred on October 31. As shown in Fig. 4e, the mean radon concentration and standard deviation are calculated as 724 ± 56 pCi/L in the period from June 1, 2013 to October 31, 2013. Figure 4e also shows that no radon data are outside the green rectangle (smaller than three standard deviations below the mean value). Accordingly, no anomalous decline in groundwater radon can be defined at well D1 prior to the 2013 Mw 6.3 Rueisuei earthquake. Tarakçi et al. (2014) investigated the relationships between seismic activities and radon level in Western Turkey. The study reported that, in a compression seismic area, the radon level tended to increase before the earthquakes and decrease towards the time of earthquake occurrence. On the contrary, in a dilation area, no change in radon levels was observed. Stress conditions could affect the detectability of precursory radon declines We will compare the stress conditions near the Antung hot spring area before and at the time of the 2013 Rueisuei earthquake with those of the other five earthquakes. Figure 5 shows the radon concentration data between July 1, 2003 and October 31, 2013 at well D1 in the Antung hot spring. Anomalous radon minima of 326 ± 9, 371 ± 9, 480 ± 43, and 447 ± 18 pCi/L were observed prior to the 2003 Chengkung Mw 6.8, 2006 Taitung Mw 6.1 and Mw 5.9, 2008 Antung Mw 5.4, and 2011 Chimei Mw 5.0 earthquakes, respectively. We consider the 2006 Mw 5.9 Taitung earthquake that occurred on April 15, 2006 triggered by stress transfer in response to the 2006 Mw 6.1 Taitung earthquake that occurred on April 1, 2006. The box-and-whisker plot is used on the right-hand side in Fig. 5. It shows the median (50th percentile, 767 pCi/L) as a center bar, and the quartiles (25th and 75th percentiles, 698 and 828 pCi/ L) as a box. The whiskers (441 and 1077 pCi/L) cover all but the most extreme values in the data set. Our research effort at the Antung hot spring in eastern Taiwan since 2003 focuses on the anomalous declines in groundwater radon precursory to large 44.4 1200 40.7 1100 37.0 1000 33.3 900 29.6 800 25.9 22.2 18.5 14.8 222Rn (pCi/L) 222Rn (Bq dm-3) A Stress Condition in Aquifer Rock for Detecting Anomalous Radon Decline… 1077 828 767 698 700 600 500 441 400 11.1 300 7.4 200 3.7 100 0.0 0 7/1/2003 1 6.8 2 6.1 7/1/2005 R 3 4 5 5.9 5.4 5.0 7/1/2007 7/1/2009 7/1/2011 6.3 7/1/2013 Year/Month/Day Figure 5 Radon concentration data at well D1 in the Antung hot spring and the box-and-whisker plot (inside open inverted triangles event number; arrows mainshocks; earthquake magnitude Mw shown beside arrows) earthquakes. Based on the box-and-whisker plot, a threshold concentration (441 pCi/L) is estimated to identify radon anomalies from well D1 data. The radon minima recorded prior to the 2008 Mw = 5.4 Antung and 2011 Chimei Mw 5.0 earthquakes are close to the threshold concentration (441 pCi/L) and can be easily masked by the noisy background. On the other hand, the radon anomalous minima, recorded precursory to strong earthquakes (Mw [ 6.0), the 2003 Mw = 6.8 Chengkung and 2006 Mw = 6.1 Taitung earthquakes, are well below the threshold concentration (441 pCi/L) and can be clearly distinguished from the background noise. Unlike the 2003 Mw = 6.8 Chengkung and 2006 Mw = 6.1 Taitung earthquakes, the radon concentration prior to the 2013 Rueisuei Mw 6.3 earthquake is well above the threshold concentration (441 pCi/L). Stress conditions near the Antung hot spring area before and at the time of the earthquake could affect the detectability of precursory radon declines and the concentration of anomalous radon minima. To understand the stress conditions in aquifer rock near the Antung hot spring area during earthquakes, we chose the nearest seismic station (HWA055) of Central Weather Bureau, Taiwan. The distance between the seismic station and well D1 is 2.29 km. Figure 6 shows an upward movement of the P-wave first motion for all those events with detectable anomalous declines in groundwater radon (Events 1–5). For Event R without detectable anomalous declines in groundwater radon, the P-wave first motion is downward. The first motion of the P-waves indicates the stress condition in rocks, compression or tension, at the time of the earthquake. For the above radon anomalies observed at well D1, the precursor times before the earthquake occurrence range from 58 to 65 days. If a similar stress pattern exists in rocks before and at the time of the earthquake, the seismological observations described above suggest a possible relationship between the stress conditions in aquifer rock and the detectability of precursory radon declines. 4. Conclusions With the help of a long-term study of the radon concentration in groundwater at the Antung hot spring, suitable geological conditions to site a radonmonitoring well are recommended to detect recurrent precursory radon declines. Besides, the possible relationship between radon anomalies and stress T. Kuo et al. Pure Appl. Geophys. Figure 6 Seismic waveforms of Events 1–5 and R recorded in HWA055 station. Gray rectangular area the zoomed region of the seismic waveform of the P-wave polarity on the right panel for each event. Black arrow P-wave first motion conditions in aquifer rock are investigated in this paper. The significance of our research can be summarized as follows. grateful to Mr. C. Lin of the Antung hot spring for his kind field assistance. 1. A small low-porosity fractured aquifer in undrained conditions near an active fault is a suitable geological site to detect precursory declines in groundwater radon prior to local large earthquakes. 2. For aquifer rock under compressive conditions before and at the earthquake, a precursory anomalous decrease in the concentration of groundwater radon can be detected. 3. For aquifer rock under compressive conditions before and at the earthquake, no precursory change in the concentration of groundwater radon was observed. REFERENCES Acknowledgements Supports by the Ministry of Science and Technology Taiwan (NSC, MOST), Central Geological Surveys, Industrial Technology Research Institute (L550001060, N550003318), Radiation Monitoring Center, and Institute Earth Sciences of Academia Sinica of Taiwan are appreciated. The authors are Attanasio, A., & Maravalle, M. (2016). 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