Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5. RADIONUCLIDE DATA U.S. Department of Energy 201 Varick Street, 5th Floor New York, NY 10014-4811 Environmental Measurements Laboratory U.S. Department of Energy 5-i Table of Contents, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Page 5. Radionuclide Data 5.1 Overview 5.2 Alpha . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.1-1 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.1-1 . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.2-1 5.2.1 Scope . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.2-1 5.3 Beta . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.3-1 5.3.1 Scope . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.3-1 5.4 Gamma . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.4-1 5.4.1 Scope . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.4-1 5.5 X-Ray . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.5-1 5.5.1 Scope . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.5-1 5.6 Natural Decay Series . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.6-1 5.6.1 Scope . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5.6-1 Environmental Measurements Laboratory U.S. Department of Energy 5 - ii Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5. RADIONUCLIDE DATA 5.1 OVERVIEW This section describes current radionuclide measurement techniques in use at EML and their associated data. A radionuclide is identified by its three principal characteristics: half-life, type of emission, and energy of the emission. Sometimes overlooked in the process are progeny radionuclides with their own particular characteristics. In the 1960s, routine measurements were being performed at EML for ", $, and ( radionuclides. Measurements in both the Frisch grid ion chamber and the solid-state surface barrier detection systems were used to identify " energies in sources in properly calibrated systems. Contained in this section is a table of " emitters by energy, especially linked to the charts of the naturally occurring radionuclides, which assists in radionuclide identification in separated samples and in radionuclide purity checks. Routine measurement of $ emitters is performed on counters designed at EML. These counters have a very low background count rate due to anticoincidence counting techniques. The overall counting efficiencies are comparable to proportional counters. Radiochemical purity is typically assessed by decay measurements. Use of NaI(T1) ( spectrometry detection systems provides poorly resolved spectra compared with the Ge(Li) and intrinsic Ge systems presently in use. The resolution of these present systems require sophisticated computer algorithms to identify energies associated with particular radionuclides. It is most important that the energies and the branching ratios used at any facility be documented and a table of ( emitters in the environment is included. Contained in the natural decay series are charts of three natural radionuclide series and the man-made americium series. Pertinent data are included in these charts. Environmental Measurements Laboratory U.S. Department of Energy 5.1 - 1 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5.2 ALPHA Contact Person(s) : Isabel M. Fisenne 5.2.1 SCOPE The tables on " emitters by atomic number and by energy have been developed for internal use at EML. The present tables are revisions compiled from the data given in Table of Radioactive Isotopes by Browne et al. (1986). REFERENCE Browne, E., R. B. Firestone and V. S. Shirley (Editors) Table of Radioactive Isotopes John Wiley and Sons, Inc., New York (1986) Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 1 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 ALPHA EMITTERS BY ATOMIC NUMBER Most short-lived nuclides are included as principal members of the natural decay series (see Section 5.6) t1/2 Isotopic Abundance (%) 60 144Nd 2.1 x 1015 y 23.8 62 147Sm 1.03 x 108 y Radionuclide 62 147 Sm 64 148Gd 11 1.06 x 10 y " Emission (when not 100%) EMeV 1.83 2.46 15.0 2.233 75.3 y 3.183 64 152Gd 1.79 x 106 y 64 152Gd 1.08 x 1014 y 66 154Dy 2.9 x 106 y 0.20 2.14 2.872 174 Hf 2.0 x 10 y 0.162 2.50 76 186Os 2.0 x 1015 y 1.58 2.80 78 190Pt 6.0 x 1011 y <0.02 3.175 83 210mBi 3.00 x 106 y 72 15 2.726 83 211Bi(AcC) 2.14 m 83 212Bi(ThC') 1.0092 h 84 206Po 8.83 d 84 208Po 2.898 y 84 209Po 84 210 Po (RaF) 84 212Po (ThC)' 84 213Po 84 214Po(RaC)' 84 215Po(AcC) 84 216 4.946(55.5%), 4.908(38.8%), 4.569(3.8%) 6.623(84%), 6.279(16%) 39.54% 5.45% 6.090(26.8%), 6.051(70.2%), 5.768(1.7%), 5.707(1.1%) 5.223 5.116 102.0 y 4.866 138.376 d 5.305 298.0 ns 8.784 4.28 µs 8.375 163.69 µs 7.687 1.780 ms 7.386 Po(ThA) 150.0 ms 6.779 84 218Po(RaA) 3.05 m 6.003 Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 2 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 ALPHA EMITTERS BY ATOMIC NUMBER (Cont'd) Radionuclide t1/2 85 211At 85 Isotopic Abundance (%) 7.215 h 217 At 41.7% 32.3 ms 86 219Rn(219Em) EMeV 5.868 7.067 3.96 s 86 220Rn(220Em, Tn) " Emission (when not 100%) 6.819(80.9%), 6.553(12.2%), 6.425(7.5%) 55.6 s 6.288 86 222Rn(222Em, Rn) 3.825 d 5.490 87 221Fr 4.9 m 6.341(83.4%), 6.243(1.3%), 6.127(15.1%) 88 223Ra(AcX) 11.43 d 5.747(9.5%), 5.716(52.5%), 5.607(24.2%), 5.540(9.2%), others 88 224Ra(ThX) 3.66 d 5.686(95.1%), 5.449(4.9%) 88 226Ra 89 1600.0 y 225 Ac 4.784(94.5%), 4.601(5.6%) 10.0 d 5.829(51.6%), 5.793(18.1%), 5.791(8.6%), 5.731(10%), 5.637(4.5%), others 90 227Th(Rd Ac) 18.718 d 6.038%(24.5%), 5.978(23.4%), 5.757(20.3%), 5.714(4.9%), 5.710(8.2%), others 90 228Th(Rd Th) 1.913 y 5.423(72.7%), 5.341(26.7%) 90 229Th 7340.0 y 5.050(5.2%), 4.968(6.0%), 4.901(10.2%), 4.845(56.2%), 4.814(9.3%), others 90 230Th(Io) 7.54 x 104 y 4.688(76.3%), 4.621(23.4%) 90 232Th(Th) 1.405 x 1010 y 91 231Pa(Pa) 3.276 x 104 y 100. 4.010(77%), 3.952(23%) 5.059(11%), 5.029(20%), 5.013(25.4%), 4.951(22.8%), 4.734(8.4%), others 92 230U 20.8 d 5.889(67.4%), 5.818(32%), others 92 232U 68.9 y 5.320(68.6%), 5.264(31.2%) 92 233U 92 234 U(UII) 1.592 x 105 y 5 2.454 x 10 y 0.0055 4.825(84.4%), 4.783(13.2%), others 4.776(72.5%), 4.724(27.5%) Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 3 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 ALPHA EMITTERS BY ATOMIC NUMBER (Cont'd) Radionuclide Isotopic Abundance (%) t1/2 92 235U(AcU) 7.037 x 108 y 92 236U 2.342 x 107 y EMeV 4.597(5%), 4.556(4.2%), 4.395(55%), 4.364(~11%), 4.218(5.7%), others 4.494(74%), 4.445(26%) 238 4.468 x 10 y 93 237Np 2.14 x 106 y 4.873(2.6%), 4.988(47%), 4.772(25%), 4.766(8%), 4.640(6.2%), others 94 236Pu 2.851 y 5.768(68.1%), 5.721(31.7%) 92 U(UI) 94 238Pu 94 239 Pu 94 240Pu 94 242 94 244 Pu Pu 9 0.7200 " Emission (when not 100%) 87.74 y 99.2745 4.196(77%), 4.147(23%) 5.499(71.6%), 5.456(28.3%) 4 2.411 x 10 y 6563.0 y 5.156(73.2%), 5.143(15.1%), 5.105(10.6%) 5.168(73.5%), 5.124(26.4%) 5 3.763 x 10 y 4.901(78%), 4.856(22.4%) 8.26 x 107 y 4.589(80.5%),4.546(19.4%) 95 241Am 432.7 y 95 243Am 7380.0 y 96 240Cm 27.0 d 96 242Cm 162.94 d 96 243Cm 28.5 y 6.067(1.5%), 6.059(5%), 5.992(6.5%), 5.786(73.3%), 5.742(10.6%), others 96 244Cm 18.11 y 5.805(76.4%), 5.763(23.6%), others 5.486(85.2%), 5.443(12.8%), 5.388(1.4%) 5.277(88%), 5.234(11%), 5.180(1.1%) 6.291(70.6%), 6.248(28.8%) 6.113(74%), 6.070(25%) 96 245Cm 8500.0 y 5.362(93.2%), 5.304(5.0%), others 96 246Cm 4730.0 y 5.386(79%), 5.343(21%) 96 247Cm 1.56 x 107 y 5.266(13.8%), 5.210(5.7%), 4.869(71%), 4.818(4.7%), others Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 4 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 ALPHA EMITTERS BY ATOMIC NUMBER (Cont'd) Radionuclide 96 248Cm* 97 247 Bk t1/2 Isotopic Abundance (%) 3.40 x 105 y " Emission (when not 100%) 91.7% 1380.0 y 98 246Cf EMeV 5.078(81.9%), 5.035(18%) 5.795(5.5%), 5.712(17%), 5.687(13%), 5.532(45%), 5.501(7%), others 1.487 d 6.750(78.0%), 6.709(21.8%) 98 248Cf 334.0 d 6.262(83.0%), 6.220(17.0%) 98 249Cf 350.6 y 6.194(2.2%), 6.140(1.1%), 5.945(4%), 5.903(2.8%), 5.812(84.4%), others 98 250Cf 98 251Cf 13.09 y 6.031(84.5%), 5.989(15.1%) 898.0 y 6.074(2.7%), 6.014(11.6%), 5.851(27%), 5.812(4.2%), 5.677(35%), others 98 252Cf* 2.646 y 96.9% 6.118(84%), 6.076(15.8%) 252 1.291 y 76.4% 6.632(79.8%), 6.562(13.5%), 6.483(2.2%), others 99 Es* 99 253Es 20.4 d 6.633(89.8%), 6.592(6.6%), others 99 254Es 275.7 d 6.427(93.1%), 6.416(1.8%), 6.357(2.6%) 99 255Es* 39.8 d 100 52Fm 1.058 d 100 253Fm* 3.00 d 100 255 Fm 20.07 h 100 257Fm 100.5 d 101 258Md 55.4 d 8.0% 6.300(87.5%), 6.260(10.0%), 6.213(2.5%) 7.04(~85%), 6.999(~15%) 12.0% 7.024(6.7%), 6.943(42.7%), 6.901(9.8%), 6.847(8.5%), 6.674(23.3%), others 7.022(93.4%), 6.963(5.0%), others 6.696(3.4%), 6.519(93.5%), 6.441(2.0%) 6.790(28%), 6.716(72%) *Relative "-intensity normalized to 100 "-decays. Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 5 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 ALPHA EMITTERS BY ENERGY (MeV)* 3.8-4.0 4.0-4.2 4.2-4.4 4.4-4.6 4.6-4.8 4.8-5.0 5.0-5.2 5.2-5.4 5.4-5.6 5.6-5.8 5.8-6.0 6.0-6.2 6.2-6.4 Uranium Series: 238 234 U 210 U Po 222 Rn 228 Th 212 Ra 224 218 Po Bi 220 Rn Th 227 230 Th 226 Ra Thorium Series: 232 Th 232 228 Th Th 224 Bi 212 Ra Actinium Series: 235 U 235 U 231 Pa 231 Pa 231 223 Pa Ra 227 Th 227 Th Americium Series: 237 Np 233 U 233 241 Am 241 Am 225 Ac 225 Ac 221 Fr 221 Fr U 229 Th 229 Th All Emitters: 232 Th 232 Th 235 U 238 U 210m 235 Bi 226 Ra 209 Th 210m Pa 229 U 231 U U 230 236 U 231 244 233 Pu 234 237 Np Po 206 Po 222 Rn 212 Bi 211 At 212 Bi 211 Bi 229 Th 210 Po 223 Ra 223 Ra 225 Ac 218 Po 220 Rn Th 231 Pa 228 Th 224 Ra 224 Ra 227 Th 221 Fr 221 Fr Pa 239 Pu 232 U 228 Th 225 Ac 230 U 227 Th 240 Cm 233 U 240 Pu 241 Am 238 Pu 227 Th 243 Cm 242 Cm 248 Cf 237 Np 243 Am 243 Am 241 Am 236 Pu 244 Cm 243 Cm 254 Es Pu 248 Cm 245 Cm 247 Bk 243 Cm 249 Cf 249 Cf 255 Es 246 Cm 244 Cm 250 Cf 250 Cf Cm 247 Bk 251 Cf 251 Cf Po Bi 242 247 Cm 208 247 251 Cf 252 Cf *A listing may denote more than one energy. Environmental Measurements Laboratory U5.S. Department of Energy 5.2 - 6 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5 ALPHA EMITTERS BY ENERGY (MeV) -- (Cont'd) 6.4-6.6 6.6-.68 6.8-7.0 7.0-7.2 7.2-7.4 7.4-7.6 7.6-7.8 7.8-8.0 8.0-8.2 8.2-8.4 8.4-.86 8.6-8.8 Uranium Series:: 214 Po Thorium Series: 216 212 Po Actinium Series: 211 Rn Bi 219 219 215 Rn Po Po Americium Series: 217 All Emmitters: 219 Rn 252 Es 253 Es 254 Es 257 Fm 211 Bi Po 246 Cf 252 Es 253 Es 253 Fm 257 Fm 258 Md 216 219 Rn Fm 253 Fm 255 Fm 252 213 217 At At Fm 253 Fm 255 Fm 215 Po 214 Po 213 Po Po 212 Po 252 Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 7 Section 5, Vol. I HASL-300, 28th Edition SPECIFIC ACTIVITY OF SELECTED ALPHA EMITTERS (in order of ascending atomic numbers) Nuclide t1/2 (y) 210m 3.00 x 106 208 2.898 Bi Po 209 102 226 1600 Po Ra 228 Th 229 Th 1.913 7340 mCi mg-1 5.7 x 10-4 MBq mg-1 2.11 x 10-2 593.1 2.19 x 104 16.8 6.22 x 102 0.989 819.6 3.66 x 101 3.03 x 104 0.213 7.88 230 7.54 x 104 2.062 x 10-2 7.63 x 10-1 232 1.405 x 1010 1.0969 x 10-7 4.06 x 10-6 231 3.276 x 104 4.724 x 10-2 1.75 Th Th Pa 232 U 68.9 22.4 8.29 x 102 233 1.592 x 105 9.64 x 10-3 3.57 x 10-1 234 2.454 x 105 6.225 x 10-3 2.30 x 10-1 235 7.037 x 108 1.922 x 10-6 7.11 x 10-5 236 2.342 x 107 6.508 x 10-5 2.41 x 10-3 238 4.468 x 109 3.36237 x 10-7 1.24 x 10-5 237 2.140 x 106 7.05 x 10-4 2.61 x 10-2 236 2.851 U U U U U Np Pu 238 Pu 239 Pu 240 Pu 87.74 2.411 x 104 6563 531.3 17.119 1.97 x 104 6.33 x 102 6.204 x 10-2 2.30 0.22696 8.40 Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 8 Section 5, Vol. I HASL-300, 28th Edition SPECIFIC ACTIVITY OF SELECTED ALPHA EMITTERS (Cont'd) (in order of ascending atomic numbers) Nuclide 242 Pu 241 Am 243 Am 242 Cm t1/2 (y) 3.763 x 105 mCi mg-1 MBq mg-1 3.962 x 10-3 1.45 x 10-1 432.7 3.428 1.27 x 102 7380 0.1993 7.37 4.461 x 10-1 3311.4 1.23 x 105 243 28.5 51.6 1.91 x 103 244 18.11 80.90 2.99 x 103 Cm Cm 245 Cm 248 Cm 247 Bk 248 Cf 249 Cf 250 Cf 251 Cf 8500 3.40 x 105 1380 9.1444 x 10-1 350.6 13.08 898 0.1717 6.35 4.24 x 10-3 1.57 x 10-1 1.05 3.89 x 101 1579 4.095 109.3 1.59 5.84 x 104 1.52 x 102 4.04 x 103 5.88 x 101 252 2.645 536.3 1.98 x 104 252 1.291 1098 4.06 x 104 254 7.54825 x 10-1 1865 6.90 x 104 Cf Es Es Environmental Measurements Laboratory U.S. Department of Energy 5.2 - 9 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5.3 BETA Contact Person(s) : Isabel M. Fisenne 5.3.1 SCOPE The table of $ emitters presented here is useful in identifying unknown $ emitters whose energies and possibly half-lives have been determined by standard laboratory techniques, including the Harley-Hallden method (see Procedure A-01-R). It is also a handy guide to $ emitting isotopes for applications requiring specific half-lives and/or energies. The original table was developed by Hallden (1955). Since that time there have been three revisions based on "current" published compilations. The present table was compiled from the Table of Isotopes (Lederer and Shirley, 1978). The emitter energy listings are the maximum $ energy (Emax). Isotopes decaying the emission of $ particles of different energies are listed in the energy group corresponding to each Emax, provided that the branch contributes > 5% of the total $ emission. Isotopes with longer-lived parents are also listed under the parent half-life. In the case of multiple long-lived parents, the nuclide is listed under the half-life of the nearest long-lived parent, as well as its own half-life. REFERENCES Hallden, N. A. "Beta Emitters by Energy and Half-life" Nucleonics, 13, 78-79 (1955) Lederer, C. and V. S. Shirley (Editors) Table of Isotopes - Seventh Edition John Wiley and Sons, New York, NY (1978) Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 1 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) T1/2 6-12 h <0.1 0.1-0.3 234 Pa 0.3-0.5 0.5-0.7 1.3-1.5 1.5-1.7 1.7-1.9 1.9-2.1 2.1-2.3 62 52 91 163 73 208 152m 77 91 77 135 184 77 212 208 212 Sm Ac 244 Am Zn Sr 135 152m 101 Pd 171 Er 171 127 Te 245 212 156 Sm 245 228 173 Tm 234 173 Tm 234 180m 43 Eu Pa Pa Mg 64 43 K 64 96 119 197 Pt 236 Np 240 U I 135 Ac Nb Ge Sr Rb Pb 28 Fe 82m I Er Pd 1.1-1.3 212 Pb 112 09.-1.1 156 228 12 h-1 d 0.7-0.9 Cu Cu Te 130 159 Gd 187 W 228 Ge Bi 163 Tb Am 184 Ta Eu Ge Tl 228 Sr Pu Ac Tl 91 I K 55 Zn 109 Pd 90 Nb 130 I Nb 157 Eu 159 Gd 197 187 240m W Tl 135 69 187 W Ta 208 Se 228 Sb 91 Sr 2.7-2.9 93 Y 2.9-3.1 62 Cu >3.1 66 Ga Bi 228 Ac K 142 Pr Zr 188 Ac 128 2.5-2.7 Ac Ta 96 I Xe Tb 2.3-2.5 Co 150 Eu 157 Eu 159 Gd 86 Y 24 Nb 133 157 97 Na 55 Co 76 Br 42 97 Eu 86 112 187 I 72 Ga W 240m Np Y Ag 90 Nb 240m Np 152 Tb 188 Re Re 194 Ir 240m Np 72 Ga 28 Al 152 Tb 42 K 72 Ga 76 Br 112 Ag 112 Ag 194 Ir Pt Np 197 Pt 200m Au 236 Np 240m Np 242 Am 242 Am 248 Bk Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 2 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont’d) T1/2 1-3 d <0.1 231 Th 0.1-0.3 0.3-0.5 0.5-0.7 0.7-0.9 66 67 48 57 72 67 Cu 67 Cu 71 72 Zn 77 As 143 Br 79 Kr 149 Ni Zn 105 Rh 172 Er 172 Tm 231 Th Cu 82 99 Mo 121 Sn Sc 105 115 231 131m 231 151 140 238 172 143 238 172 151 238 232 Pa 153 239 Np 239 Th Th Np Np Np Te Pm Er Tm Np 239 Np 245m Ni 151 Cd 151 131m Te 151 143 Ce 69 Ge 149 Pm 83 Ce 151 Pm 99 Pm 189 Re 115 As Rh 0.9-1.1 1.1-1.3 1.3-1.5 Pm 198 Au Sb Sr 131 Te Mo 140 La 143 Ce 140 La 1.7-1.9 1.9-2.1 2.1-2.3 66 Cu 76 72 Ga 166 131 166 140 131 140 Cd Pm Pm 122 1.5-1.7 Te La As Ho Ho 122 Sb 90 Y 2.3-2.5 76 As 2.5-2.7 66 Cu Te 72 Ga La 72 As 2.7-2.9 2.9-3.1 76 As >3.1 72 Ga 72 As 172 Tm 172 Tm 143 Ce La 153 Sm 151 Ce 153 Sm 151 Pm 172 Tm 193 Sm 189 Re 226 193 Os 193 Os 193 Os 226 Ac 239 Np Pm Pm Os Ac 238 Np 245m Es Es Note: Where the symbol for a nuclide appears more than once in any grouping it indicates emission of more than one energy. Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 3 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont’d) T1/2 3-5 d <0.1 175 Yb 0.1-0.3 0.3-0.5 0.5-0.7 0.7-0.9 0.9-1.1 1.1-1.3 1.3-1.5 1.5-1.7 1.7-1.9 1.9-2.1 2.1-2.3 2.3-2.5 2.5-2.7 2.7-2.9 2.9-3.1 132 199 199 5-10 d 237 U 177 196 237 Te 47 Au 166 Au 166 Sc Sc 127 Zr Dy Yb 214 199 Au 214 Bi Lu 131 I 52 Au 133 Xe 111 Ag U 161 Tb 131 I Er 161 Tb Lu 161 Tb 183 Ta Ba 140 La 140 Nd 209 Pb 147 Pu 211 Pu 140 147 246 13-15 d 89 175 177 246 Dy 47 Ca 127 169 10-13 d 47 126 I 136 Cs 225 Ra Environmental Measurements Laboratory U.S. Department of Energy Te 132 Pb 214 I 127 Re 132 Sb 186 I 186 Pb 214 111 Ag Mn 136 132 Ba Sb 126 I 166 Ho Bi Sb Re 132 I 214 Bi 214 Bi 148 Pm 140 Ba 143 124 210 140 Pr 126 127 I Ho La I 47 Ca 148 Bi Nd I Sb 166 Pb Cs 127 140 La 140 207 Tl 246 211 Pb 213 Bi 246 Am 126 La Am 32 124 I 132 I Pm Sb 140 La 246 Am 140 Pr 134 125 Sn 72 148 Pm La As >3.1 214 72 Bi As P 5.3 - 4 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont’d) T1/2 15-20 d 20-30 d <0.1 0.10.3 0.5-0.7 0.7-0.9 0.91.1 1.1-1.3 1.3-1.5 74 As 156 Eu 74 86 Rb 234 Pa 191 Os 156 Eu 48 253 Cf 156 Eu 230 Pa 233 Pa Pa 33 P 233 30-40 d 0.3-0.5 V Pa 234 233 Pa 234 Pa 234 Th 234 Th 234 Pa 141 Ce 95 Nb 103 Ru 103 Ru 141 Ce 84 Rb 74 As 129 Te 1.5-1.7 1.7-1.9 86 As Rb 1.9-2.1 2.1-2.3 2.3-2.5 156 2.5-2.7 2.7-2.9 2.9-3.1 >3.1 Eu 82 129 Te 84 Rb Rb 129m Te Note: Where the symbol for a nuclide appears more than once in any grouping it indicates emission of more than one energy. Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 5 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont'd) T1/2 <0.1 0.1-0.3 0.3-0.5 0.5-0.7 0.7-0.9 0.9-1.1 1.1-1.3 1.3-1.5 1.5-1.7 1.7-1.9 1.9-2.1 2.1-2.3 2.3-2.5 2.5.-2.7 2.7-2.9 2.9-3.1 59 40-50 d Fe 203 Hg 59 Fe 148m 181 35 50-100 d 95 S 46 Nb 58 124 160 192 253 45 148m Pm Sc 124 Tb Sb Co Sb Zr 192 Ir Tb 95 Zr 192 Ir Ir 160 Tb Cf 185 W 188 W 182 Ta 127 Te 182 Ta 177 115m 160 Tb 56 Sb 170 Tm 170 110m Ag 144 106 Rh 171 Tm Co 91 Sr 124 123 Tm Y Sb 114 In 188 Re 188 Re 124 Sb Sn Lu Lu 102 249 1-2 y 124 89 200-250 d 250 d-1 y Cd Hf 95 Ca 177 Pm 160 100-150 d 150-200 d Pm 148m >3.1 Ce 144 Ce Bk Environmental Measurements Laboratory U.S. Department of Energy 110m Ag 250 Bk Rh 68 144 Ga 250 Pr Bk 106 Rh 106 Rh 106 Rh 5.3 - 6 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont'd) T1/2 2-3 y <0.1 134 Cs 0.1-0.3 0.3-0.5 0.5-0.7 0.7-0.9 0.9-1.1 1.1-1.3 1.3-1.5 1.5-1.7 1.7-1.9 1.9-2.1 2.1-2.3 2.3-2.5 2.5-2.7 2.7-2.9 2.9-3.1 125 Sb 125 Pm 125 147 Sb 22 Sb 125 >3.1 Na Sb 134 Cs 155 3-5 y Eu 155 Eu 5-10 y 194 Os 228 Ra 154 Eu 60 Co 228 Ac 228 Ra 204 Tl 154 Eu 146 Pm 228 Ac 154 Eu 228 Ac 154 Eu 228 Ac 228 Ac 194 Ir 194 Ir 228 Ac Note: Where the symbol for a nuclide appears more than once in any grouping it indicates emission of more than one energy. Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 7 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont'd) T1/2 10-20 y <0.1 3 0.1-0.3 0.3-0.5 0.5-0.7 0.7-0.9 0.9-1.1 1.1-1.3 1.3-1.5 1.5-1.7 1.7-1.9 1.9-2.1 2.1-2.3 2.3-2.5 2.5-2.7 2.7-2.9 2.9-3.1 85 H 241 113 Pu 152 Kr Eu 154 >3.1 Eu Cd 152 Eu 154 Eu 20-30 y 210 90 Pb Sr 210 Bi 137 Cs 90 Y 210 Pb 227 Ac 137 30-50 y 50-100 y 151 >100 y 63 121m Sm Ni 14 C 94 93 Zr 32 Si 98 107 79 Se 115 166m 87 Rb 182 187 99 225 227 Cs Nb 10 Tc 39 Be 36 Ar 158 In Lu Ta 182 Ta Ra 233 Pa 126 242 Am 228 129 242 Am 228 135 231 138 Ho Re Ac Ra Ra Th Tc Sn I Sc 40 K Sn 176 Pd 44 Cl Tb 26 Al 238 32 P 126 Sb 234m Pa Np Cs La 231 Th 231 Th BETA EMITTERS BY HALF-LIFE AND ENERGY (EMAX IN MeV) - (Cont'd) Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 8 Section 5, Vol. I HASL-300, 28th Edition T1/2 <0.1 Rev. 0 February 1997 0.1-0.3 0.3-0.5 0.5-0.7 0.7-0.9 0.9-1.1 1.1-1.3 1.3-1.5 1.5-1.7 1.7-1.9 1.9-2.1 2.1-2.3 2.3-2.5 2.5-2.7 2.7-2.9 2.9-3.1 >3.1 231 Th 233 Pa 233 Pa 234 Th 234 Th Note: Where the symbol for a nuclide appears more than once in any grouping it indicates emission of more than one energy. Environmental Measurements Laboratory U.S. Department of Energy 5.3 - 9 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5.4 GAMMA Contact Person(s) : Colin G. Sanderson 5.4.1 SCOPE Presented here is a tabulation of ( rays and nuclides that are common to environmental analyses. These data may be useful for interpreting either field or laboratory measurements. As an aid in verifying nuclide identifications, two additional (-ray lines are included when possible as E2 and E3. The following special notations are used in the table: Symbol Meaning % ratio of (-rays to disintegrations. X indicates X-ray. KX, LX sum of K or L X-rays. D T indicates a doublet. indicates a triplet. * indicates annihilation radiation. Long in half-life column is used for all members of the primordial series, % refers to U or Th decays REFERENCE Browne, E., R. B. Firestone and V. S. Shirley (Editors) Table of Radioactive Isotopes John Wiley and Sons, Inc., New York (1986) Environmental Measurements Laboratory U.S. Department of Energy 5.4 - 1 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES Energy 14.4 26.3 30.0 39.6 39.9 40.6 46.5 49.8 53.2 59.5 59.5 60.0 61.5 63.3 66.9 74.8X 74.8X 75.0X 77.1X 77.1X 79.6 80.1 80.2 81.0 81.0 84.3X 86.4 86.5 87.2X 87.2X 88.0 90.0X 91.1 92.6D 93.4X 97.1 99.6 Nuclide 57 Co Am 140 Ba 129 I 212 Bi 99 Mo 210 Pb 132 Te 133 Ba 237 U 241 Am 155 Eu 239 Np 234 Th 136 Cs 214 Pb 212 Pb 208 Tl 214 Pb 212 Pb 133 Ba 144 Ce 131 I 133 Ba 133 Xe 228 Th 136 Cs 155 Eu 214 Pb 212 Pb 109 Cd 228 Ac 147 Nd 234 Th 228 Ac 237 U 228 Ac 241 % 9.5 2.4 13.6 7.5 1.1 1.1 4.1 14.4 2.2 32.8 35.7 1.1 1.0 3.8 12.5 6.5 10.5 3.6 11.0 17.7 3.2 1.1 2.6 34.2 37.0 1.2 6.3 34.0 3.9 6.3 3.6 3.4 28.0 5.4 5.6 16.0 1.3 T1/2 272D 433Y 12.8D 1.6E7 Long 65.9H 22.3Y 78.2H 10.5Y 6.75D 433Y 4.96Y 2.36D Long 13.2D Long Long Long Long Long 10.5Y 285D 8.04D 10.5Y 5.25D 1.91Y 13.2D 4.96Y Long Long 463D Long 11.0D Long Long 6.75D Long Environmental Measurements Laboratory U.S. Department of Energy E2 % E3 % Origin 122.1 59.5 162.7 30.0KX 727.3 18.3X 85.5 35.7 6.2 70.8 6.7 3.2 136.5 17.0LX 304.9 10.7 38.7 4.3 30.0KX 81.0 101.1 26.3 86.5 14.3LX 92.6D 34.0KX 77.1X 77.1X 72.8X 74.8X 74.8X 53.2 133.5 364.5 276.4 79.6 12.3X 66.9 105.3 77.1X 238.6 23.0KX 93.4X 38.5KX 63.3 90.0X 101.0 129.0 70.9 34.2 26.0 2.4 30.4 56.1 5.4 17.6 11.0 17.7 2.1 6.5 10.5 2.2 11.1 81.2 7.3 0.2 3.1 12.5 20.6 11.0 43.6 99.8 5.6 37.4 3.8 3.4 26.0 2.9 Activation 241 Pu Fallout Fission 232 Th Fallout 238 U Fallout Activation Fallout 241 Pu Fallout Fallout 238 U Fission 238 U 232 Th 232 Th 238 U 232 Th Activation Fallout Fission Activation Fission 232 Th Fission Fallout 238 U 232 Th Activation 232 Th Fallout 238 U 232 Th Fallout 232 Th 1620.7 140.5 111.9 31.0KX 208.0 17.0LX 105.3 101.0KX 1.5 3.5 1.9 101.3 22.0 38.7 20.6 38.9 86.4 87.3X 87.2X 84.8X 87.2X 87.2X 6.3 3.9 6.3 1.3 3.9 6.3 696.5 284.3 79.6 31.0KX 1.3 6.1 3.2 40.1 153.3 60.0 241.9 77.1X 7.5 1.1 7.5 17.7 99.6 319.4 1.3 2.0 99.6 208.0 209.4 1.3 22.0 4.1 5.4 - 2 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % E3 % Origin 208.0 60.0 129.0 117.0KX 143.8 116.4 208.0 228.3 244.7 14.4 591.8 325.2 209.4 80.1 14.4 462.8 181.1 20.6X 163.4 22.0 1.1 2.9 11.6 10.5 1.9 22.0 88.2 7.5 9.5 4.8 13.4 4.1 1.1 9.5 30.7 6.1 1.2 4.7 164.0 258.4 30.0 185.7 176.6 4.6 31.5 13.6 53.0 13.6 362.3 380.4 273.7 366.4 205.3 2.3 1.5 12.7 1.2 4.7 101.1 105.3 105.4X 106.1 109.2 111.9 113.9 116.3 121.8 122.1 123.1 127.2 129.0 133.5 136.5 138.0 140.5 140.5 143.8 145.4 151.2 153.3 153.9 162.7 163.4 164.0 165.9 166.0 176.3 176.6 181.1 185.7 186.1 192.3 196.3 198.0 237 U Eu 228 Ac 239 Np 235 U 132 Te 237 U 132 Te 152 Eu 57 Co 154 Eu 101 Rh 228 Ac 144 Ce 57 Co 138 Cs 99 Mo 99m Tc 235 U 141 C 85m Kr 136 Cs 138 Xe 140 Ba 235 U 136 Cs 139 Ce 88 Kr 125 Sb 136 Cs 99 Mo 235 U 226 Ra 59 Fe 88 Kr 101 Rh 26.0 20.6 2.0 22.7 1.5 1.9 25.0 1.9 28.4 85.5 40.5 73.0 2.9 11.1 10.7 1.5 3.5 87.2 10.5 48.4 75.2 7.5 6.0 6.2 4.7 4.6 79.9 3.1 6.8 13.6 6.1 53.0 3.3 3.1 26.0 70.8 6.75D 4.96Y Long 2.36D 70E7Y 78.2H 6.75D 78.2H 13.3Y 273D 8.8Y 3.3Y Long 285D 272D 32.2M 65.9H 6.01H 70E7Y 32.5D 4.48H 13.2D 14.1M 12.8D 70E7Y 13.2D 138D 2.84H 2.73Y 13.2D 65.9H 70E7Y 1600Y 44.5D 2.84H 3.3Y 1099.3 362.3 127.2 56.5 2.3 73.0 1291.6 166.0 325.2 43.2 3.1 13.4 Fallout Fallout 232 Th Fallout Natural Fallout Fallout Fallout Fallout Activation Fallout Fallout 232 Th Fallout Activation 138 Xe Fallout 99 Mo Natural Fission Fission Fission Fission Fallout Natural Fission Activation Fission Fallout Fission Fallout Natural Natural Activation Fission Fallout 205.3 208.0 235 4.7 22.0 70E7Y 6.75D 185.7 59.5 53.0 32.8 143.8 101.1 10.5 26.0 Natural Fallout 155 U U 237 Environmental Measurements Laboratory U.S. Department of Energy 59.5 86.5 99.6 61.5 93.4KX 49.8 101.1 111.9 344.3 136.5 248.0 198.0 99.6 696.5 122.1 227.7 40.6 18.4X 109.2 37.0KX 304.9 86.4 242.7 304.9 143.8 153.3 34.0KX 196.3 427.9 164.0 140.5 143.8 32.8 34.0 1.3 1.0 5.5 14.4 26.0 1.9 26.6 10.7 6.6 70.8 1.3 1.3 85.5 1.5 1.1 6.1 1.5 17.4 13.7 6.3 3.5 4.3 10.5 7.5 79.5 26.0 29.4 4.6 3.5 10.5 5.4 - 3 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 209.4 227.7 228.2 228.3 233.2 238.6 240.8 241.9 242.7 244.7 248.0 249.8 258.4 262.8 270.3 273.7 276.4 277.3 277.6 279.2 284.3 295.1 228 Ac Cs 239 Np 132 Te 133m Xe 212 Pb 224 Ra 214 Pb 138 Xe 152 Eu 154 Eu 135 Xe 138 Xe 132 I 228 Ac 136 Cs 133 Ba 208 Tl 239 Np 203 Hg 131 I 214 Pb 4.1 1.5 10.7 88.2 10.3 43.6 3.9 7.5 3.5 7.5 6.6 90.0 31.5 1.4 3.8 12.7 7.1 2.4 14.2 81.5 6.1 19.2 Long 32.2M 2.36D 78.2H 2.19D Long Long Long 14.1M 13.3Y 8.8Y 9.10H 14.1M 2.28H Long 13.2D 10.5Y Long 2.36D 46.6D 8.04D Long 300.0 302.9 304.9 304.9 315.9 319.4 320.1 325.2 328.0 328.8 334.3 338.4 340.6 344.3 352.0 356.0 212 3.3 18.4 4.3 13.7 1.6 2.0 9.8 13.4 3.5 20.7 2.1 12.4 48.6 26.6 37.1 62.2 Long 10.5Y 12.8D 4.48H 2.36D 11.0D 27.7D 3.3Y Long 40.3H 2.36D Long 13.2D 13.3Y Long 10.5Y 138 Pb 133 Ba 140 Ba 85m Kr 239 Np 147 Nd 51 Cr 101 Rh 228 Ac 140 La 239 Np 228 Ac 136 Cs 152 Eu 214 Pb 133 Ba Environmental Measurements Laboratory U.S. Department of Energy E2 % E3 % 129.0 138.0 106.1 116.4 30.0KX 300.0 2.9 1.5 22.7 1.9 56.3 3.3 270.3 409.0 277.6 111.9 3.8 4.7 14.2 1.9 295.1 153.9 121.8 123.1 608.2 242.7 505.9 209.4 176.6 302.9 510.6 228.2 74.6X 364.5 351.9 19.2 6.0 28.4 40.5 2.9 3.5 5.0 4.1 13.6 18.4 7.8 10.7 12.9 81.2 37.1 352.0 258.4 344.3 591.8 31.0KX 396.6 522.7 328.0 340.6 81.0 583.0 315.9 37.1 31.5 26.6 4.8 5.2 6.3 16.1 3.5 48.6 34.2 30.9 1.6 238.6 276.4 162.7 151.2 277.6 439.9 43.6 7.1 6.2 75.1 14.2 1.2 127.2 270.3 432.5 315.9 328.0 273.7 244.7 241.9 302.9 73.0 3.8 3.0 1.6 3.5 12.7 7.5 7.5 18.4 80.2 241.9 2.6 7.5 Origin 232 Th Xe Fallout Fallout Fission 232 Th 232 Th 238 U Fission Fallout Fallout Fission Fission 132 Te 232 Th Fission Activation 232 Th Fallout Fallout Fission 238 U 138 232 356.0 423.7 62.2 3.1 334.3 91.1 2.1 28.0 198.0 338.4 487.0 61.5 409.6 818.6 411.1 295.1 383.8 70.8 12.4 45.9 1.0 2.2 99.8 2.2 19.2 8.9 Th Activation Fallout Fission Fallout Fallout Activation Fallout 232 Th Fallout Fallout 232Th Fission Fallout 238 U Activation 5.4 - 4 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % E3 % Origin 362.3 364.5 366.4 380.4 383.8 396.6 88 Kr I 99 Mo 125 Sb 133 Ba 138 Xe 2.3 81.2 1.2 1.5 8.9 6.3 2.84H 8.04D 65.9H 2.73Y 10.5Y 14.1M 196.3 637.0 181.1 176.3 356.0 258.4 26.0 7.3 6.1 6.8 62.2 31.5 834.9 284.3 739.5 427.9 302.9 401.5 13.0 6.1 12.1 29.4 18.4 2.2 Fission Fission Fallout Fallout Activation Fission 401.5 402.6 409.0 409.6 411.1 415.3 418.5 420.4 423.7 427.9 432.5 434.6 437.6 439.9 444.0D 446.8 462.8 463.1 463.4 468.7 475.1 475.1 475.4 477.6 487.1 497.1 138 Xe Kr 138 Cs 228 Ac 152 Eu 102 Rh 102 Rh 102 Rh 140 Ba 125 Sb 140 La 138 Xe 140 Ba 147 Nd 152 Eu 110m Ag 138 Cs 228 Ac 125 Sb 102m Rh 102m Rh 102 Rh 134 Cs 7 Be 140 La 103 Ru 2.2 49.6 4.7 2.2 2.2 2.1 10.6 3.2 3.1 29.4 3.0 20.3 1.9 1.2 3.1 3.8 30.7 4.6 10.5 2.9 46.0 95.0 1.5 10.3 45.5 89.5 14.1M 76.3M 32.2M Long 13.3Y 2.89Y 2.89Y 2.89Y 12.8D 2.73Y 40.3H 14.1M 12.8D 11.0D 13.3Y 250D 32.2M Long 2.73Y 207D 207D 2.89Y 2.06Y 53.2D 40.2H 39.6D 434.6 845.5 227.7 338.4 344.3 418.5 415.3 418.5 437.6 380.4 487.0 401.5 537.3 319.4 411.1 657.8 547.0 409.6 427.9 475.1 468.7 628.1 563.2 20.3 7.3 1.5 12.4 26.6 10.6 2.1 10.6 1.9 1.5 45.9 2.2 24.4 2.0 2.2 94.6 10.8 2.2 29.4 46.0 2.9 8.5 8.4 396.6 673.9 462.8 463.1 444.0D 420.4 420.4 475.1 304.9 463.4 328.8 1114.3 423.7 531.0 778.9 620.4 409.0 755.3 600.5 556.6 556.6 420.5 569.3 6.3 1.9 30.7 4.6 3.1 3.2 3.2 95.0 4.3 10.5 20.7 1.5 3.1 13.1 13.0 2.8 4.7 1.3 17.8 1.9 1.9 3.2 15.4 751.9 610.3 4.3 5.6 432.6 2.9 Fission Fission 138 Xe 232 Th Fallout Fallout Fallout Fallout Fallout Fallout Fallout Fission Fallout Fallout Fallout Activation 138 Xe 232 Th Fallout Fallout Fallout Fallout Fission Cosmic Fallout Fallout 505.9 510.6 511.0 511.0 132 5.0 7.8 2.9 30.0 2.28H Long 244D 70.9D 262.8 277.3 1115.5 810.8 1.4 2.4 50.8 99.5 522.7 583.0 16.1 30.9 131 87 I Tl 65 Zn 58 Co 208 Environmental Measurements Laboratory U.S. Department of Energy 132 Te Th Activation Activation 232 5.4 - 5 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide 511.0 511.9 514.0 522.7 526.6 531.0 537.3 547.0 547.0 556.6 563.2 569.3 569.2 583.0 591.8 22 600.5 602.7 604.7 606.6 608.2 609.3 610.3 620.4 621.2 621.9 628.1 628.1 630.3 631.3 635.9 637.0 645.9 650.6 657.8 661.7 665.4 667.7 125 Na Ru 85 Sr 132 I 135m Xe 147 Nd 140 Ba 138 Cs 132 I 102m Rh 134 Cs 134 Cs 207 Bi 208 Tl 154 Eu 106 Sb Sb 134 Cs 125 Sb 135 Xe 214 Bi 103 Ru 110m Ag 132 I 106 Ru 102m Rh 102 Rh 132 I 102 Rh 125 Sb 131 I 124 Sb 132 I 110m Ag 137 Cs 214 Bi 132 I 124 % T1/2 E2 % 180.8 20.7 99.3 16.1 81.2 13.1 24.4 10.8 1.3 1.9 8.4 15.4 97.8 30.9 4.8 2.60Y 372D 64.8D 2.28H 15.7M 11.0D 12.8D 32.2M 2.28H 207D 2.06Y 2.06Y 32.2Y Long 8.8Y 1274.5 1050.4 13.4KX 505.9 30.0KX 439.9 437.6 462.8 522.7 475.1 475.4 563.2 1063.1 510.6 248.0 99.9 1.5 50.6 5.0 14.0 1.2 1.9 30.7 16.1 46.0 1.5 8.4 74.9 7.8 6.6 17.8 97.8 97.6 5.0 2.9 46.1 5.6 2.8 ~2.0 9.8 5.5 8.5 13.8 56.0 11.3 7.3 7.4 2.7 94.6 85.2 1.6 98.7 2.73Y 60.2D 2.06Y 2.73Y 9.10H Long 39.3D 250D 2.28H 372D 207D ~2.9Y 2.28H ~2.9Y 2.73Y 8.04D 60.2D 2.28H 250D 30.0Y Long 2.28H 463.4 645.9 795.9 600.5 249.8 665.4 497.1 657.8 547.1 511.9 556.6 475.1 621.2 628.1 606.6 364.5 602.7 630.3 620.4 33.0KX 609.3 650.6 10.5 7.4 85.4 17.8 90.0 1.6 88.7 94.6 1.3 20.7 1.9 95.0 ~2.0 8.5 5.0 81.2 97.8 13.8 2.8 7.1 46.1 2.7 Environmental Measurements Laboratory U.S. Department of Energy E3 621.9 15.0KX 547.0 319.4 423.7 871.7 621.2 628.1 569.3 604.7 1769.7 860.3 692.5 606.6 709.3 569.3 635.9 31.6KX 768.4 % 9.8 8.7 1.3 2.0 3.1 5.1 ~2.0 5.5 15.4 97.6 6.9 4.3 1.7 5.0 1.4 15.4 11.3 5.2 4.9 446.8 630.3 1050.4 1103.2 631.3 650.6 692.4 671.4 722.9 709.3 667.7 677.6 3.8 13.8 1.5 2.9 56.0 2.7 1.8 1.8 1.8 1.4 98.7 10.4 768.4 669.9 4.9 4.9 Origin Cosmic Fallout Activation 132 Te Fission Fallout Fallout 138 Xe 132Te Fallout Fission Fission Fallout 232 Th Fallout Fallout Fallout Fission Fallout Fission 238 U Fallout Activation 132 Te Fallout Fallout Fallout 132 Te Fallout Fallout Fission Fallout 132 Te Activation Fallout 238 U 132 Te 5.4 - 6 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % E3 % Origin 669.9 671.4 671.6 673.9 677.6 687.0 692.4 692.5 695.6 696.5 697.6 132 I Sb 132 I 87 Kr 110m Ag 110m Ag 102 Rh 154 Eu 102 Rh 144 Ce 102 Rh 4.9 1.8 5.2 1.9 10.4 6.4 1.8 1.7 2.7 1.3 45.7 2.28H 2.73Y 2.28H 76.3M 250D 250D ~2.9Y 8.8Y ~2.9Y 285D ~2.9Y 667.7 635.9 669.9 845.5 657.8 677.6 631.3 591.8 692.4 133.5 766.9 98.7 11.3 4.9 7.3 94.6 10.4 56.0 4.8 1.8 11.1 34.0 671.6 606.6 727.D 402.6 687.0 706.7 695.6 723.4 697.6 80.1 695.6 5.2 5.0 5.4 49.6 6.4 16.4 2.7 19.7 45.7 1.1 2.7 132 706.7 709.3 713.8 722.8 722.9 723.4 724.2 727.0D 727.3 728.7 739.5 744.3 751.7 755.3 756.7 756.8 763.1 763.9 765.8 766.9 768.4 772.3 772.7 777.9 778.9 780.1 110m 16.4 1.4 2.3 10.9 1.8 19.7 44.1 5.4 6.7 1.1 12.1 4.7 4.3 1.3 54.5 4.3 0.6 22.3 99.8 34.0 5.0 1.1 76.2 4.4 13.0 1.2 250D 60.2D 60.2D 60.2D 8.04D 8.8Y 64.0D 2.28H Long 2.28H 65.9H 250D 40.3H Long 64.0D 8.8Y Long 250D 35.0D ~2.9Y Long Long 2.28H 65.9H 13.3Y 2.28H 687.0 645.9 709.3 713.8 364.5 692.5 756.7 671.6 39.9 727.0D 366.4 706.7 487.0 463.1 724.2 723.4 583.0 744.3 6.4 7.4 1.4 2.3 81.2 1.7 54.5 5.2 1.1 5.4 1.2 16.4 45.9 4.6 44.1 19.7 30.9 4.7 744.3 713.8 722.8 968.2 637.0 756.8 4.7 2.3 10.9 1.9 7.3 4.3 728.7 1620.7 772.7 777.9 763.9 815.8 772.3 1.1 1.5 76.2 4.4 22.3 23.6 1.1 873.2 860.3 818.0 11.5 4.3 7.3 697.6 665.6 755.3 728.7 739.5 444.0D 772.7 45.7 1.6 1.3 1.1 12.1 3.1 76.2 1046.6 786.4D 794.8 780.1 366.4 867.4 809.8 34.0 0.3 4.6 1.2 1.2 4.2 2.9 Activation Fallout Fallout Fallout Fission Fallout Fallout 132 Te 232 Th 132 Te Fallout Activation Fallout 232 Th Fallout Fallout 232 Th Activation Fallout Fallout 238 U 232 Th 132 Te Fallout Fallout 132 Te 125 Ag Sb 124 Sb 124 Sb 131 I 154 Eu 95 Zr 132 I 212 Bi 132 I 99 Mo 110m Ag 140 La 228 Ac 95 Zr 154 Eu 208 Tl 110m Ag 95 Nb 102 Rh 214 Bi 228 Ac 132 I 99 Mo 152 Eu 132 I 124 Environmental Measurements Laboratory U.S. Department of Energy Te Fallout 132 Te Fission Activation Activation Fallout Fallout Fallout Fallout Fallout 5.4 - 7 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide 785.5 786.4 794.8 795.8 212 802.0 806.2 809.8 810.8 812.3 815.8 818.0 818.6 830.6 834.8 834.9 835.6 840.4 845.5 860.3 867.4 867.8 871.7 873.2 877.2 884.7 898.1 898.0 134 904.3 911.2 919.6 925.2 934.0 937.5 954.6 964.1 964.6 968.2 228 Bi Bi 228 Ac 134 Cs 214 Cs Bi 132 I 58 Co 132 I 140 La 110m Ag 136 Cs 228 Ac 54 Mn 88 Kr 228 Ac 228 Ac 87 Kr 208 Tl 152 Eu 140 La 138 Cs 154 Eu 132 I 110m Ag 88 Y 88 Rb 214 Ac Ac 140 La 140 La 214 Bi 110m Ag 132 I 152 Eu 228 Ac 124 Sb 228 % T1/2 E2 % 1.1 0.3 4.6 85.4 Long Long Long 2.06Y 727.3 768.4 772.3 604.7 6.7 4.9 1.1 97.8 1620.7 806.2 830.6 801.9 1.5 1.2 0.6 8.7 232 8.7 1.2 2.9 99.5 5.6 23.6 7.3 99.8 0.6 100.0 13.0 1.7 0.9 7.3 4.3 4.2 5.6 5.1 11.5 1.1 72.7 92.7 14.1 2.06Y Long 2.28H 70.9D 2.28H 40.3H 250D 13.2D Long 312.2D 2.84H Long Long 76.3M Long 13.3Y 40.3H 32.2M 8.8Y 2.28H 250D 107D 17.8M 795.9 786.4 780.1 511.0 809.8 751.7 763.9 340.6 794.8 85.4 0.3 1.2 30.0 2.9 4.3 22.3 48.6 4.6 1038.6 934.0 812.3 1.0 3.2 5.6 877.2 867.8 884.7 1048.1 835.6 1.1 5.6 72.7 79.7 1.7 362.3 830.6 835.6 673.9 2614.4 778.9 815.8 547.0 756.8 812.3 818.0 1836.1 1836.1 2.3 0.6 1.7 1.9 35.8 13.0 23.6 10.8 4.3 5.6 7.3 99.4 21.4 985.8D 840.4 904.3 1175.5 583.0 964.1 919.6 1009.8 996.3 954.6 937.5 1.3 0.9 0.9 1.1 30.9 14.5 2.7 29.8 10.3 18.1 34.4 2677.9 2.0 Fission 238 U 132 Te Activation 132 Te Fallout Activation Fission 232 Th Fallout Fission 232 Th 232 Th Fission 232 Th Fallout Fallout 138 Xe Fallout 132 Te Activation Activation 88 Kr 0.9 29.0 2.7 7.1 3.2 34.4 18.1 14.5 5.8 1.9 Long Long 40.3H 40.3H Long 250D 2.28H 13.3Y Long 60.2D 840.4 966.0D 867.8 487.0 1120.3 1384.3 877.2 1085.9 969.0 1045.1 0.9 23.2 5.6 45.9 15.0 24.3 1.1 9.9 17.4 1.9 911.2 840.4 925.2 919.6 806.2 884.7 1136.2 867.4 911.2 722.8 29.0 0.9 7.0 2.7 1.2 72.7 3.0 4.2 29.0 10.9 Environmental Measurements Laboratory U.S. Department of Energy E3 % Origin Th U 232 Th Fission 238 232 Th Th Fallout Fallout 238 U Activation 132 Te Fallout 232 Th Fallout 232 5.4 - 8 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % E3 % 969.0 985.8 996.3 1001.0 1004.8 1009.8 1038.6 1045.1 1046.6 1048.1 1050.4 1063.1 1085.9 1099.3 1103.2 1103.2 1112.1 1112.9 1114.3 1115.5 1120.3 1136.2 1141.4 1143.6 1147.3 1155.2 1167.9 1173.2 1173.3 1175.5 228 Ac Kr 154 Eu 234m Pa 154 Eu 138 Cs 134 Cs 124 Sb 102 Rh 136 Cs 106 Ru 207 Bi 152 Eu 59 Fe 102m Rh 102 Rh 152 Eu 102 Rh 138 Xe 65 Zn 214 Bi 132 I 88 Kr 132 I 138 Cs 214 Bi 134 Cs 60 Co 132 I 87 Kr 17.4 1.3 10.3 0.7 17.9 29.8 1.0 1.9 33.0 79.7 1.5 74.9 9.9 56.5 2.9 4.4 13.6 18. 1.5 50.8 15.0 3.0 1.3 1.4 1.2 1.7 1.8 99.9 1.1 1.1 Long 2.84H 8.8Y Long 8.8Y 32.2M 2.06Y 60.2D 2.9Y 13.2D 372D 32.2Y 13.3Y 44.5D 207D 2.9Y 13.3Y 2.9Y 14.1M 244D Long 2.28H 2.84H 2.28H 32.2M Long 2.06Y 5.27Y 2.28H 76.3M 911.2 1141.4 1004.8 766.4 1274.5 1147.3 1167.9 1325.5 1103.2 818.6 511.9 569.2 1112.1 1291.6 556.6 1046.6 1085.9 1046.6 1768.4 511.0 1155.2 954.6 1369.4 1136.2 1009.8 1238.1 1038.6 1332.5 1143.6 1740.6 29.0 1.3 17.9 0.2 35.5 1.2 1.8 1.6 4.4 99.8 20.7 97.8 13.6 43.2 1.9 33.0 9.9 33.0 16.7 2.9 1.7 18.1 1.5 3.0 29.8 5.9 1.0 100.0 1.4 2.0 1459.2 834.9 873.2 742.8 996.3 871.7 802.0 968.2 766.9 1235.4 621.9 1769.7 964.1 192.3 628.1 1112.9 1212.9 1103.2 434.6 1.1 13.0 11.5 0.1 10.3 5.1 8.7 1.9 34.0 19.8 9.8 6.9 14. 3.1 5.5 18.9 1.4 4.4 20.3 934.0 1143.6 985.8D 1173.3 1343.6 1120.3 1365.2 3.2 1.4 1.3 1.1 1.1 15.0 3.0 1290.8 845.5 1.1 7.3 1212.9 1235.4 1238.1 1274.5 1274.5 1281.0 1290.8 1291.6 152 1.4 19.8 5.9 99.9 35.5 1.5 1.1 43.2 13.3Y 13.2D Long 2.60Y 8.8Y Long 2.28H 44.5D 1112.1 818.6 1155.2 511.0 1004.8 1238.1 1173.3 1099.3 13.6 99.8 1.7 181.0 17.9 5.9 1.1 56.5 1299.2 1048.1 1281.0 1.6 79.7 1.5 1596.6 1377.7 1295.4 192.3 1.8 4.0 2.0 3.1 88 Eu Cs 214 Bi 22 Na 154 Eu 214 Bi 132 I 59 Fe 136 Environmental Measurements Laboratory U.S. Department of Energy Origin 232 Th Fission Fallout 238 U Fallout 138 Xe Fission Fallout Fallout Fission Fallout Fallout Fallout Fallout Fallout Fallout Fallout Fallout Fission Activation 238 U 132 Te Fission 132 Te 138 Xe 238 U Fission Activation 132 Te Fission Fallout Fission 238 U Cosmic Fallout 238 U 132 Te Activation 5.4 - 9 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % % Origin 99.2 2.0 1.6 1.83H 2.28H 13.3Y 1290.8 1212.9 1.1 1.4 1372.1 1408.0 2.5 20.8 Activation 132 Te Fallout 1.6 100.0 1.1 3.0 2.7 100.0 1.5 2.5 4.0 24.3 7.1 1.4 2.5 20.8 76.3 1.3 1.4 1.1 10.7 4.0 1.6 60.2D 5.27Y 32.2M 2.06Y 60.2D 14.7H 2.84H 2.28H Long 250D 2.28H Long Long 13.3Y 32.2M 60.2D 2.28H Long 1.3E9 250D Long 1045.1 1173.2 1147.3 1167.9 1325.5 2754.1 1141.4 1295.4 1281.0 1475.8 1372.1 1377.7 1401.5 1299.2 1343.6 1368.2 1398.6 1499.0D 1.9 99.9 1.2 1.8 1.6 99.9 1.3 2.0 1.5 4.0 2.5 4.0 1.4 1.6 1.1 2.7 7.1 1.6 1368.2 2.7 1435.8 1038.6 1436.7 76.3 1.0 1.3 1518.4 1398.6 1401.5 937.5 1442.5 1408.0 1509.2 1212.9 2218.0 1691.0 1921.1 969.0 2.2 7.1 1.4 34.4 1.4 2.5 2.2 1.4 15.2 47.1 1.2 17.4 1384.3 1459.2 24.3 1.1 1505.0 1588.2 13.0 3.6 Fallout Activation 138 Xe Fission Fallout Activation Fission 132 Te 238 U Activation 132 Te 238 U 238 U Fallout 138 Xe Fallout 132 Te 232 Th Natural Activation 232 Th 4.0 2.5 1.5 2.2 1.6 45.9 35.5 1562.3 1661.3 1529.8 2029.9 1630.5 2521.7 1004.8 1.0 1.2 10.9 4.5 2.0 3.4 17.9 Activation 238 U Fission Fission 232 Th Fallout Fallout 1293.6 1295.4 1299.2 41 1325.5 1332.5 1343.6 1365.2 1368.2 1368.6 1369.4 1372.1 1377.7 1384.3 1398.6 1401.5 1408.0 1408.0 1435.8 1436.6 1442.5 1459.2 1460.8 1475.8 1499.0D 124 1505.0 1509.2 1518.4 1529.8 1588.2 1596.5 1596.6 110m Ag Bi 88 Kr 88 Kr 228 Ac 140 La 154 Eu 13.0 2.2 2.2 10.9 3.6 95.4 1.7 250D Long 2.84H 2.84H Long 40.3H 8.8Y 1475.8 1408.0 1369.4 1518.4 1499.0D 487.0 1274.5 1620.7 1630.5 1661.3 1691.0 212 1.5 2.0 1.2 47.1 Long Long Long 60.2D 727.3 1588.2 1509.2 2090.9 Ar I 152 Eu 132 Sb Co 138 Cs 134 Cs 124 Sb 24 Na 88 Kr 132 I 214 Bi 110m Ag 132 I 214 Bi 214 Bi 152 Eu 138 Cs 124 Sb 132 I 228 Ac 40 K 110m Ag 228 Ac 60 214 Bi Ac 214 Bi 124 Sb 228 Environmental Measurements Laboratory U.S. Department of Energy 6.7 3.6 2.2 5.5 E3 785.5 1499.0D 1729.6 1436.7 1.1 1.6 3.1 1.3 232 Th Th 238 U Fallout 232 5.4 - 10 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % E3 % Origin 1729.6 1740.6 1764.5 1768.4 1769.7 214 Bi Kr 214 Bi 138 Xe 207Bi 3.1 2.0 15.9 16.7 6.9 Long 76.3M Long 14.1M 32.2Y 1764.5 1175.5 1729.6 1114.3 1063.1 15.9 1.1 3.1 1.5 74.9 1661.3 2011.9 1847.4 1850.9 569.2 1.2 2.9 2.1 1.4 97.8 238 1836.1 1836.1 1847.4 1850.9 88 21.4 99.4 2.1 1.4 17.8M 107D Long 14.1M 2677.9 898.1 1764.5 1768.4 2.0 92.7 15.9 16.7 898.1 14.1 88 2118.5 2004.8 1.2 5.4 1921.1 132 1.2 2.28H 1442.5 1.4 2002.4 1.1 132 2002.4 2004.8 2011.9 2015.9 2029.9 2035.5 2079.3 2090.9 132 I Xe 87 Kr 138 Xe 88 Kr 88 Kr 138 Xe 124 Sb 1.1 5.4 2.9 12.3 4.5 3.7 1.4 5.5 2.28H 14.1M 76.3M 14.1M 2.84H 2.84H 14.1M 60.2D 1921.1 1850.9 1740.6 2004.8 1529.8 2029.9 2015.9 1436.6 1.2 1.4 2.0 5.4 10.9 4.5 12.3 1.3 1.4 12.3 13.1 1.4 3.7 13.2 2.3 47.1 132 2118.5 2195.8 214 1.2 13.2 Long 2.84H 1847.4 2035.5 2.1 3.7 2204.1 2231.8 5.0 3.4 238 2204.1 2217.8 2231.8 2252.3 214 Bi Cs 88 Kr 138 Xe 5.0 15.2 3.4 2.3 Long 32.2M 2.84H 14.1M 2447.7 1435.8 2195.8 2079.3 1.6 76.3 13.2 1.4 2118.5 2639.4 2392.1 2015.9 1.2 7.6 34.6 12.3 238 2392.1 88 34.6 2.84H 2231.8 3.4 2195.8 13.2 Fission 2447.7 214 1.6 Long 2204.1 5.0 2118.5 1.2 2521.7 2556D 140 3.4 13.1 40.3H 76.3M 1596.5 2011.9 96.4 2.9 487.0 1740.6 45.9 2.0 Fallout Fission 2614.4 2639.4 208 35.8 7.6 Long 32.2M 860.3 2217.8 4.3 15.2 583.0 1435.8 30.9 76. 232 87 Rb Y 214 Bi 138 Xe 88 I 138 Bi Kr 88 138 Kr Bi La Kr 87 Tl 138 Cs Environmental Measurements Laboratory U.S. Department of Energy 1442.5 2015.9 2556.0D 2079.3 2035.5 2195.8 2252.3 1691.0 U Fission 238 U Fission Fallout Kr Other 238 U Fission Te Te Fission Fission Fission Fission Fission Fission Fallout U Fission U Xe Fission Fission 138 238 U Th Xe 138 5.4 - 11 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 TABLE OF ( RAYS AND NUCLIDES COMMON TO ENVIRONMENTAL ANALYSES (Cont'd) Energy Nuclide % T1/2 E2 % E3 % Origin 2677.9 88 2.0 17.8M 1836.1 21.4 2754.0 24 99.9 14.7H 1368.6 100.0 6129.2 16 68.8 7.13S 7115.2 4.7 Other 7115.2 16 4.7 7.13S 6129.2 68.8 Other Rb Na N N Environmental Measurements Laboratory U. S. Department of Energy 898.1 14.1 88 Kr Activation 5.4 - 12 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5.5 X-RAY Contact Person(s) : Colin G. Sanderson 5.5.1 SCOPE This section presents a table of X-ray energies which are useful for radiochemical analyses. A number of nuclides emit X-rays as part of their decay scheme. These X-rays may be counted with Ar proportional counters with Ge planar or n-type Ge co-axial detectors or with thin crystal NaI(Tl) scintillation counters. In both cases, spectral measurements can be made and both qualitative and quantitative information obtained on the sample. K Shell vacancies are filled by a higher shell election. In the process an energy Ek - Ex is liberated either as an X-ray or an Auger electron. The most important X-ray transitions are designated as, K"1 = K - LIII K"2 = K - LII Kß1 = K - MIII Kß2 = K - NIII Kß3 = K - MII Kß4 = K - NII Kß5 = K - MIV Environmental Measurements Laboratory U. S. Department of Energy 5.5 - 1 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 With moderate resolution only Kß1' and Kß2' can be resolved, Kß1' = Kß1 + Kß3 + Kß5 Kß2' = Kß2 + Kß4 The same is true for K" K" = K"1 + K"2 The present table lists the values for K", Kß1' and Kß2'. Electron binding energies used in this table were based on the tabulations of Wapstra et al. (1959) and Siegbahn (1965). REFERENCES Browne, E. and R. B. Firestone Table of Radioactive Isotopes Shirley, V. S. (Editor) John Wiley and Sons, Inc., New York (1986) Siegbahn, K. Alpha, Beta, and Gamma Ray Spectroscopy North-Holland Publishing, Co., Amsterdam (1965) Wapstra, A. H., G. J. Nijgh and R. Van Lieshout Nuclear Spectroscopy Tables North-Holland Publishing, Co., Amsterdam (1959) Environmental Measurements Laboratory U. S. Department of Energy 5.5 - 2 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Energy (keV) Kß1' Z Element K"- 3 4 5 Li Be B 0.05 0.11 0.18 6 7 8 C N O 0.28 0.40 0.53 9 10 11 F Ne Na 0.68 0.85 1.04 12 13 14 Mg Al Si 1.25 1.49 1.74 15 16 17 P S C1 2.01 2.31 2.62 18 19 20 Ar K Ca 2.96 3.31 3.69 3.19 3.59 4.01 21 22 23 Sc Ti V 4.09 4.51 4.95 4.46 4.93 5.43 24 25 26 Cr Mn Fe 5.42 5.90 6.40 5.95 6.49 7.06 27 28 29 Co Ni Cu 6.93 7.47 8.03 7.65 8.26 8.91 30 31 32 Zn Ga Ge 8.63 9.24 9.88 9.57 10.3 11.1 Environmental Measurements Laboratory U. S. Department of Energy Kß2' 5.5 - 3 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Z Element K"- Energy (keV) Kß1- 33 34 35 As Si Br 10.5 11.2 11.9 11.7 12.5 13.3 36 37 38 Kr Rb Sr 12.6 13.4 14.1 14.1 15.0 15.8 16.1 39 40 41 Y Zr Nb 14.9 15.7 16.6 16.7 17.7 18.6 17.0 18.0 19.0 42 43 44 Mo Te Ru 17.4 18.3 19.2 19.6 20.6 21.6 20.0 21.0 22.1 45 46 47 Rh Pd Ag 20.2 21.1 22.1 22.7 23.8 24.9 23.2 24.3 25.5 48 49 50 Cd In Sn 23.1 24.1 25.1 26.1 27.3 28.4 26.6 27.9 29.1 51 52 53 Sb Te I 26.3 27.3 28.5 29.7 31.0 32.3 30.4 31.7 33.0 54 55 56 Xe Cs Ba 29.6 30.8 32.0 33.6 34.9 36.4 34.4 35.8 37.2 57 58 59 La Ce Pr 33.3 34.5 35.9 37.8 39.3 40.7 38.7 40.2 41.8 60 61 62 Nd Pm Sm 37.2 38.5 39.8 42.3 43.8 45.4 43.3 44.9 46.6 Environmental Measurements Laboratory U. S. Department of Energy Kß2' 5.5 - 4 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 K"- Energy (keV) Kß1- Kß2' Z Element 63 64 65 Eu Cd Tb 41.3 42.7 44.1 47.0 48.7 50.4 48.2 49.9 51.7 66 67 68 Dy Ho Er 45.6 47.1 48.7 52.1 53.8 55.6 53.4 55.3 57.1 69 70 71 Tm Yb Lu 50.3 51.9 53.5 57.5 59.4 61.3 59.0 60.9 62.9 72 73 74 Hf Ta W 55.2 57.1 58.8 63.2 65.2 67.2 64.9 67.0 69.1 75 76 77 Re Os Ir 60.6 62.4 64.3 69.3 71.4 73.6 71.2 73.4 75.6 78 79 80 Pt Au Hg 66.2 68.2 70.1 75.7 78.0 80.1 77.8 80.1 82.5 81 82 83 Tl Pb Bi 72.1 74.2 76.3 82.4 84.7 87.1 84.9 87.3 89.8 84 85 86 Po At Rn 78.4 80.5 82.8 89.6 92.7 94.7 92.3 95.0 97.5 87 88 89 Fr Ra Ac 85.0 87.3 89.7 97.3 99.9 102.6 100.2 103.0 105.7 Environmental Measurements Laboratory U. S. Department of Energy 5.5 - 5 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Element K"- Energy (keV) Kß1- 90 91 92 Th Pa U 92.1 94.5 97.0 105.3 108.1 111.0 108.6 111.4 114.5 93 94 95 Np Pu Am 99.5 102.1 104.7 113.9 116.9 119.9 117.5 120.5 123.6 96 97 98 Cm Bk Cf 107.5 110.2 113.0 123.0 126.2 129.4 126.9 130.2 133.5 99 100 101 Es Fm Md 115.9 118.8 122.8 132.7 136.0 139.4 136.9 140.4 144.9 102 103 104 No Lw 124.8 127.9 130.5 142.7 146.2 149.7 147.5 151.2 154.5 Z Environmental Measurements Laboratory U. S. Department of Energy Kß2' 5.5 - 6 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 5.6 NATURAL DECAY SERIES Contact Person(s) : Isabel M. Fisenne 5.6.1 SCOPE Charts of the four heavy element series are given in this section. These are the three natural series and the artificial Am series. Data for half-lives and energies have been taken from Browne et al. (1986). Energies are given in order of abundance and include only the major emissions. Branching in the chains that amount to one percent or less are also omitted. REFERENCE Browne, E. and R. B. Firestone Table of Radioactive Isotopes Shirley, V. S. (Editor) John Wiley and Sons, Inc. (1986) Environmental Measurements Laboratory U. S. Department of Energy 5.6 - 1 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Principal Members of the Uranium Series 238 U (UI) 4.47 x 109 y 4.2 MeV U (UII) 2.45 x 105 y 4.7 MeV 234 9 234 234 Th (UX1) 24.1 d 0.2, 0.1 MeV _ _ 9 Pa (UX2) 1.17 min 2.3 MeV 230 Th (Io) 7.54 x 104 4.6 MeV 9 226 Ra (Ra) 1600 y 4.8 MeV 9 222 Rn (Rn) 3.825 d 5.5 MeV 9 218 9 Alpha Decay Beta Deca 214 _ 9 214 Environmental Measurements Laboratory U. S. Department of Energy _ 210 Pb (RaF) 138.376 d 5.3 MeV 210 Bi (RaC) 19.9 m 0.4-3.3 MeV _ Pb (RaB) 26.8 m 0.7, 1.0 MeV Po (RaCN) 1.64 x 10-4 s 7.7 MeV 214 Po (RaA) 3.05 m 6.0 MeV 9 210 _ Pb (RaD) 22.3 y 0.02, 0.06 MeV _ Bi (RaE) 5.013 d 1.2 MeV 9 206 Pb (RaG) Stable 5.6 - 2 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Principal Members of the Thorium Series 232 228 Th (Th) 1.405 x 1010 y 4.0 MeV 9 228 228 _ Ac (Ms Th II) 6.13 h 0.4-2.2 MeV Ra (Ms Th I) 5.75 y 0.01, 0.04 MeV _ Th (Rd Th) 1.91 y 5.3, 5.4 MeV 9 224 Ra (ThX) 3.66 d 5.4, 5.7 MeV 9 220 Rn (Tn) 55.6 s 6.3 MeV 9 216 Po (ThA) 0.15 s 6.8 MeV 9 218 212 Pb (ThB) 10.64 h 0.3, 0.6 MeV 9 Alpha Decay Beta Decay 9 _ Environmental Measurements Laboratory U. S. Department of Energy 212 Pb (ThB) 10.64 h 0.3, 0.6 MeV _ 212 _ Po (ThCN) 2.98 x 10-7 8.8 MeV 9 Bi (ThC) 60.6 min 6.1 MeV ", 2.2 MeV $ 208 Pb (ThD) 9 208 1/3 TI (ThCO) 3.053 min 1.0-1.8 MeV _ Stable 5.6 - 3 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Principal Members of the Actinium Series 235 U (AcU) 7.037 x 108 y 4.4-4.6 MeV 231 9 231 Th (UY) 1.063 d 0.09-0.30 MeV _ Pa 3.276 x 104 y 4.7-5.1 MeV 9 227 Ac 21.77 y 0.05 MeV 227 Th (Rd Ac) 18.718 d 5.7-6.0 MeV _ 9 223 Ra (AcX) 11.43 d 5.5-5.7 MeV 9 219 Rn (An) 3.96 s 6.4-6.8 MeV 9 215 Po (AcA) 1.78 x 10-3 s 7.4 MeV 9 Alpha Decay Beta Decay 9 _ 211 Pb (AcB) 36.1 min 0.5-1.4 MeV 211 _ Bi (AcC) 2.14 min 6.3, 6.6 MeV 207 Pb 9 207 Ti (AcC'') 4.77 m 1.43 MeV Environmental Measurements Laboratory U. S. Department of Energy Stable _ 5.6 - 4 Section 5, Vol. I HASL-300, 28th Edition Rev. 0 February 1997 Principal Members of the Americium Series 241 Am 432.7 y 5.4-5.5 MeV 241 Pu 14.4 y 0.02 MeV 9 9 237 Np 2.14 x 106 y 4.6-4.8 MeV _ 237 U 6.75 d 0.09, 0.25 MeV 9 233 9 233 _ Pa 27.0 d 0.15-0.57 MeV 233 Th 22.3 min 1.23 MeV _ U 1.592 x 105 y 4.8 MeV 9 229 Th 7340 y 4.8-5.1 MeV 9 225 Ra 14.8 d 0.32 MeV _ 225 Ac 10.0 d 5.8 MeV 9 221 Fr 4.9 min 6.1-6.3 MeV 9 217 At 0.032 s 7.1 MeV 9 Alpha Decay 9 _ 213 Bi 45.59 min 1.0-1.4 MeV 213 _ Po 4.2 x 10-6 s 8.4 MeV 9 Beta Decay 209 Pb 3.253 h 0.64 MeV Environmental Measurements Laboratory U. S. Department of Energy 209 Bi Stable _ 5.6 - 5
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