Earth and Planetary Science Letters 237 (2005) 45 – 55 www.elsevier.com/locate/epsl Stepwise expansion of desert environment across northern China in the past 3.5 Ma and implications for monsoon evolution Z.L. Ding a,*, E. Derbyshire b, S.L. Yang a, J.M. Sun a, T.S. Liu a a Institute of Geology and Geophysics, Chinese Academy of Sciences, Beijing 100029, China Department of Geography, Royal Holloway (University of London), Egham, Surrey TW20 0EX, UK b Received 20 January 2005; received in revised form 26 May 2005; accepted 8 June 2005 Available online 19 July 2005 Editor: E. Boyle Abstract A systematic study of the last glacial cycle along three transects across the Chinese Loess Plateau shows that sand-sized particle content within loess decreases rapidly from north to south, and that markedly high sand particle contents in loess horizons occur only in the northern part of the Plateau. This suggests that variation in the sand-sized particle fraction within loess near the desert margin is closely linked to migration of the southern desert border in northern China where sand grains move mainly in saltation or modified saltation mode near the ground surface. As desert margin shift is essentially controlled by the amount of monsoon precipitation, the sand-sized particle content within loess near desert margin is regarded as a new and readily applied proxy for variations in the strength of the East-Asian summer monsoon. A continuous record of sand content in loess along the loess–desert transitional zone shows that the Mu Us Desert migrated southward at 2.6, 1.2, 0.7 and 0.2 Ma, suggesting a stepwise weakening of the East-Asian summer monsoon during the past 3.5 Ma. This evolutionary pattern is significantly different from that previously inferred from loess magnetic susceptibility records, a widely used monsoon proxy. Our results further suggest that changes in global ice volume may have been an essential factor in controlling Plio–Pleistocene monsoon evolution, and that the anticipated future melting of polar ice cover may lead to a northward migration of the monsoon rainfall belt in northern China. D 2005 Elsevier B.V. All rights reserved. Keywords: East-Asian summer monsoon; loess–red clay sequence; Mu Us desert; sand content of loess; Plio–Pleistocene 1. Introduction * Corresponding author. Tel.: +86 10 62008111; fax: +86 10 62010846. E-mail address: [email protected] (Z.L. Ding). 0012-821X/$ - see front matter D 2005 Elsevier B.V. All rights reserved. doi:10.1016/j.epsl.2005.06.036 Formation and evolution of deserts can be regarded as a result of interactions between the atmosphere, hydrosphere, biosphere and lithosphere [1–4]. Changes in desert environment can, in turn, exert a significant 46 Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 influence on the climate system by altering surface albedo feedback and by supplying to the atmosphere and oceans variable quantities of mineral aerosols that have the potential to affect the radiative balance of the atmosphere and the global carbon cycle [5–7]. The deserts of northern China, covering an area of about 1.5 106 km2, together make up the worldTs largest mid-latitude, temperate, continental interior desert. The location of this desert zone is thought to be closely associated with the uplift of the Tibetan Plateau during the late Cenozoic, a process that progressively hindered northward penetration of moisture-laden air from the Indian Ocean [8]. Another forcing mechanism leading to dryland environmental change is the variation in the strength of the East-Asian summer monsoon. A compilation of paleo-data from within the North China deserts has demonstrated that the southern desert margin migrated several hundred kilometers north of its last glacial maximum (LGM, ~20 ka BP) limit in response to increased monsoon rainfall during the Holocene Optimum (~8–4 ka BP) [9]. The long-term evolution of the deserts of northern China remains poorly understood because of the sparseness of directly extractable geological evidence of suitable type and quality to be found within them. Given that the loess deposits making up the Loess Plateau of China lie immediately south and southeast of these deserts, and so are largely a product of winds from these dryland sources [10–12], it is considered that well-dated, semi-continuous loess records may provide valuable insights into the recent history of the deserts and their margins. In this study, three loess transects covering the last glacial cycle, from Hongde (HD) to Yangling (YAL), Zichang (ZC) to Lantian (LAT), and Yulin (YL) to Weinan (WN), were sampled and analyzed, together with a thick eolian loess–red clay sequence at Jingbian near the Mu Us desert (Fig. 1). The aim was to use spatial changes in loess particle size to establish a semi-quantitative relation between particle size and desert margin location, and to reconstruct shifts in desert margins since the late Pliocene. The linkage between desert Fig. 1. The sampling localities and annual precipitation isopleths (mm) in the Loess Plateau. The southern border of the Mu Us Desert during the LGM lay in a location similar to that of the present [9]. The three loess transects studied here stretch from YL to WN, ZC to LAT and HD to YAL. Within the loess–desert transitional zone, few loess sections with complete last glacial loess deposits have been found. Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 changes in northern China and East-Asian monsoon evolution is also briefly addressed. 2. Spatial variation in grain size of late Pleistocene loess Fig. 2 shows the down-section changes in median grain size and content of sand particles (N 63 Am%) 47 for the three transects. The HD–YAL (upper panel), YL–WN (middle panel) and ZC–LAT (lower panel) transects consist of 12, 8, and 7 sections, respectively. All sections include the S1–S0 stratigraphic units. The S1 soil formed in the last interglacial period, and has a brownish or reddish color. In the northernmost part of the transects, this soil consists of three discrete pedogenic units and two intercalated loess horizons. Loess unit L1, which accumulated in the last glacial, can be Fig. 2. Changes in median grain size and sand-grade particle (N63 Am%) content for the HD–YAL (upper panel), YL–WN (middle panel) [15] and ZC–LAT (lower panel) transects. The left curve in each pair is median grain size and the right curve is sand-grade particle content. The shaded zones indicate interglacials. The loess sections were sampled at 5–10 cm intervals. 48 Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 subdivided into 5 loess layers, namely L1-1, L1-2, L13, L1-4 and L1-5. Chronological studies have shown that the L1-2, L1-3 and L1-4 units together accumulated in marine isotope stage 3 (MIS 3), and that L1-1 and L1-5 formed in MIS 2 and MIS 4, respectively [13–15]. In the YL section, the L1-1, L1-3 and L1-5 horizons are composed of medium sand particles, indicating southward advance of paleo-desert during these times [14]. The S0 soil, developed in the Holocene, has a darkish color because of relatively high organic matter. In some sections of the northern Loess Plateau, e.g. at ZC, the S0 soil has been partly or totally eroded (Fig. 2). Across the Loess Plateau, there is a consistent northward decrease both in present-day mean annual temperatures (from ~13 to ~8 8C) and mean annual precipitation (from ~600 to below 400 mm) (Fig. 1). The northward increase in aridity is essentially controlled by the systematic decrease in summer rainfall derived from the East-Asian summer monsoon over the Loess Plateau. The stratigraphy of the sections is correlative in the field, suggesting quasi continuous dust accumulation during the last glacial cycle. Particle size was determined for all samples taken at 5–10 cm intervals downsection, using the method described in Ding et al. [16]. The following features are clearly evident in Fig. 2. (1) Thickness, median size and sand particle percentage all decrease consistently from north to south, indicating strong spatial differentiation of dust during subaerial transport. (2) Loess units L1-1 and L1-5 are characterized by much coarser median grain sizes and higher sand contents than soils S0 and S1 and the middle part of L1 in each section. (3) Markedly high sand particle contents in the glacial loess (L1-1 and L1-5) occur only in the northern part of the Plateau, a time when the desert margin was close by [9]. In order to demonstrate further the spatial differentiation of eolian sediments, changes in sand particle content (N 63 Am%) with increasing distance southward of the present Mu Us Desert margin (Fig. 1) are shown for L1-1, L1-4, L1-5 and S1 (Fig. 3). All horizons exhibit a consistent southward decrease in the sand particle content, the rate of decrease for L1-1 and L1-5 being more rapid than that for L1-4 and S1. Both the L1-1 and L1-5 records show an abrupt decrease near the desert margin and a gradual decrease beyond. According to the reconstruction of Sun et al. [9], the southern border of the Mu Us Desert during Fig. 3. Changes in the content of sand-sized particles southward from the southern border of the Mu Us Desert (Fig. 1) for L1-1, L14, L1-5 and S1. The values for each horizon in each section were averaged from between 4 and 20 samples (depending on estimated sedimentation rates) from the portions with coarsest (L1-1 and L15) or finest (L1-4 and S1) median grain size. Changes in these values are assumed to represent an approximately synchronous differentiation of sand-sized particles on a millennial-scale average. the cold-dry LGM (L1-1) was broadly similar to that of today, whereas it retreated several hundred kilometers to the north during the warm-humid Holocene Optimum. This implies that this desert margin experienced wide-ranging advance–retreat cycles in response to climatic oscillations at orbital time scales. It is clear that significant increase in sand percentages in L1-1 and L1-5 relative to S1 and L1-4 were con- Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 trolled at the first order by the desert advance during their accumulation. Using the sand content–distance relation of L1-1 (Fig. 3), it is therefore inferred that sand particle contents of ~30% and ~15% within the loess indicate a distance from the desert margin of ~100 and ~200 km, respectively. In general, loess particles are transported by winds from the source area to the depositional area in two modes, namely saltation and suspension. Theoretical and experimental studies by Pye [17] and Tsoar and Pye [18] concluded that, during low-level atmospheric dust storms, sand-sized particles are usually transported by saltation or modified saltation near the desert surface, and that any sand particles transported in suspension quickly settle back on the ground surface. Our observations show that significant volumes of sand particles are present within the wind-blown loess only near the desert margin during glacial periods, which is consistent with the Tsoar and Pye model. Moreover, our data suggest a statistical relationship from which may be derived a semi-quantitative estimation of the distance between dust sources and depositional areas. Of course, as previously suggested [11], other factors such as wind velocity play a part in sand particle transport. It is widely accepted that the Chinese loess was transported mainly by winter monsoon winds driven by the Siberian–Mongolian high pressure system [11,19]. The mean and maximum velocities of winter monsoon winds during the LGM may well have been higher than during other intervals of the last glacial cycle, because of the likely intensification of the Siberian High associated with expanded polar ice sheets and a more extensive sea ice cover [20]. It follows from this that source-to-sink estimates for loess horizons other than L1-1, based on the N 63 Am% to distance relationship provided by L1-1 (Fig. 3), should be regarded as upper limits. 3. Desert migrations during the past 3.5 Ma The Jingbian section (37840V54W N, 108831V15W E), at 1370 m above sea level, lies on the summit of the Baiyu Mountains. It is located only ~12 km south of the present margin of the Mu Us Desert. No local sources of sand, such as river channels, are present in this area. The section is composed of a ~252 m thick Pleistocene loess-soil sequence resting on a ~30 m 49 Pliocene red clay deposit, making a total thickness of ~282 m. A previous magnetic polarity study showed that this sequence has a basal age of 3.5 Ma [21]. Field observations have demonstrated that the development of the paleosols within both the Pleistocene and Pliocene eolian deposits is much weaker at Jingbian than in the main body of the Loess Plateau series, and that the Pleistocene loess-soil stratigraphy correlates well with the classic loess sections. To the best of our knowledge, the Jingbian section is the only desert margin eolian sequence known to cover the whole Pleistocene and the late Pliocene. Its proximity to the dust source region makes it ideal for the study of long-term desert changes. In the field, samples were taken at 5–10 cm intervals, making up a total of 3440 samples. The magnetic susceptibility and median grain-size records at Jingbian are shown in Fig. 4. As seen in other loess sections, the magnetic susceptibility values are 2–4 times higher in paleosols than in loess horizons, and grain sizes are much coarser in loess than in soils. Both the susceptibility and grain-size records further support our field observation that this eolian sequence is a well preserved and almost complete record, making it possible to develop a time scale for this sequence by correlating its loess-soil unit succession to the Chinese Loess Particle Time Scale (Chiloparts) [22]. The Chiloparts record was developed by stacking five individual loess grain-size records that were tuned to the obliquity and precession records of the EarthTs orbits. The Jingbian magnetic susceptibility and grain-size records, plotted on the Chiloparts time scale, are shown in Fig. 5, together with a composite marine oxygen isotope record [23–25]. The N 63 and N125 Am% records (Fig. 5C and D) at Jingbian show four stepped increases in sand-sized particle content. The late Pliocene red clay (below L33) contains few sand particles, indicating that the dust was transported in suspension, mainly from a remote source. From ~2.6 to ~1.2 Ma, sand content in interglacial soils remains low, whereas it varies generally between 18% and 25% in glacial loess except for the case of L15 and L16. This suggests that, during glacial periods, the desert environment advanced to a location no more than 200 km from the present northern margin of the Loess Plateau. In the part of the section deposited between ~1.2 and ~0.7 Ma, sand content increases to ~12% in soils and to ~43% in loess with a sub- 50 Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 Fig. 4. The magnetic susceptibility and median grain-size records of the Jingbian section, located in the northernmost part of the Loess Plateau (Fig. 1). The Pleistocene loess (above L33) at Jingbian is ~252 m thick, and the Pliocene red clay ~30 m thick. The red clay accumulated during the time interval ~3.5–2.6 Ma, as suggested by magnetic polarity studies [21]. The Jingbian section was sampled at 5–10 cm intervals. The major loess-paleosol units are labeled for the section. stantial increase in N125 Am particles, implying a large-scale advance of the desert margin during both glacial and interglacial times. Throughout material deposited in the interval ~0.7–0.2 Ma, N 63 Am particles range from ~30% in soils and ~55% in loess units, with the N 125 Am particles exceeding 8%. This suggests that the distance between the Loess Plateau and the present desert margin was less than 100 km. During the last two glacial periods, eolian sand was directly deposited at Jingbian, indicating a further southward desert shift. 4. Discussion and conclusions In previous studies, two factors have been proposed as controls on grain-size variations within the Chinese loess, namely strength of the transporting winds, specifically those associated with the winter monsoon [11,19], and the location of the desert margin [15,22]. If the source-to-sink distance remains unchanged, an increase in the winter monsoon intensity will result in the deposition of coarser dust particles. On the other hand, if the desert margin advances southwards, the loess deposited at a specific site on the Plateau will also be coarser. In this study, we show that loess particle size is much coarser during glacial periods than during interglacials. This may have resulted from either or both desert margin advance and wind intensity increase due to cold-dry climatic conditions. However, a significant sand content within glacial loess horizons is present only in the northern part of the Loess Plateau, i.e. near desert margins where saltation or modified saltation may be the Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 51 Fig. 5. Changes in magnetic susceptibility (A) and grain-size data (B, C, D) at Jingbian, and correlation with a stacked marine d 18O record (E) [23–25]. The time scale of the Jingbian section was developed by correlating the loess-soil units with the Chiloparts record [22]. dominant mode of transport. It is conceivable that, regardless of the wind intensity, loess deposited close to desert margins will contain a high sand-sized particle fraction, and that this fraction will rapidly decrease with distance from the margins, as shown in Fig. 3. It is thus concluded that changes in the sandsized particle fraction within loess can be used as an indicator of advance–retreat cycles along desert–loess transition zones. Humidity is the most important factor affecting desert margin shift, since desert margin advance can occur only when the vegetation cover there is destroyed with a critical reduction of humidity. In the loess–desert transitional region of northern China, about 80% of rainfall is attributable to the East-Asian summer monsoon. When this summer frontal rainfall belt penetrates farther to the north, the desert margins show a corresponding northward 52 Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 shift, as in the case of the Holocene Optimum [9]. In this context, the sand-sized fraction in the loess near desert margin can be regarded as a proxy of summer monsoon intensity. In most previous studies, loess magnetic susceptibility [26,27] and various chemical element ratios [28] of the Chinese loess-paleosol series have been used as summer monsoon proxies, a practice based, respectively, on the recognition that the susceptibility values of interglacial paleosols are 2–4 times greater than those found in the loess units laid down in glacials, and that paleosols show much more advanced chemical weathering than is seen in adjacent loess. However, the processes and factors affecting variations in loess-paleosol susceptibility remain controversial [29– 32]. Recent studies have shown that increased magnetic susceptibility in paleosols may not result solely from intensified pedogenic processes arising from increased monsoonal precipitation [31,32]. Here, we propose that changes in elemental concentrations within loess-paleosol sequences may be determined largely by three factors: chemical weathering in source regions, grain-size distribution, and post-depositional weathering. It is only the signature resulting from post-depositional weathering that can be linked to summer monsoon intensity. Unfortunately, the detailed studies required to distinguish the major controlling factors in loess element ratios are still pending. The East-Asian summer monsoon affects vast areas of the continent. Essentially, monsoon precipitation is a product of the interaction between warm-moist southerly airmasses and cold northerly airflows from middle and high latitudes. Generally, the more northerly the penetration of the frontal rainfall belt the greater is the intensity of the summer monsoon [33]. It follows that desert margin retreat in northern China is consistent with a stronger summer monsoon. Thus, the linkage described above between the sand-sized particle fraction within loess, desert margin location and summer monsoon intensity forms the basis of a novel, and readily applied monsoon proxy. As desert margin shift is a geographical phenomenon, the sandsized particle content in loess near desert margin should be regarded as a more direct and sensitive proxy for monsoon strength than either loess magnetic susceptibility or elemental ratios derived from physical and chemical characteristics of loess, respectively. The Jingbian sand-sized particle record clearly demonstrates that, superimposed on the glacial–interglacial oscillations, the deserts in northern China experienced significant expansion at ~2.6, ~1.2, ~0.7 and ~0.2 Ma, directly implying a stepwise southward retreat of the monsoon rainfall belt, associated with a complementary reduction in summer monsoon strength, in the past 3.5 Ma. This evolutionary pattern conflicts with current understanding based on loess magnetic susceptibility records, which show a significant increase in susceptibility values in sediments from early to late Pleistocene in age [26,34], thus implying a progressively enhanced monsoon precipitation. This suggests that factors affecting variations in loess magnetic susceptibility require further investigation. Two forcing factors may have driven the long-term evolution of the East-Asian monsoon, namely changes in the elevation of the Tibet Plateau [3,35] and changing global ice volumes [20,34]. Both meteorological observations [33,36] and numerical model experiments [35,37,38] indicate that uplift of the Tibet Plateau plays a critical role in initiation and maintenance of the Asian monsoon system. Geological studies show that the main body of the Plateau had reached its highest elevation by ~14 Ma [39] or ~8 Ma [40], although a late phase (~3.6 Ma) of uplift of its northern parts may have occurred [41]. This implies that Tibetan tectonic changes were not a significant influence on Plio–Pleistocene monsoon evolution. In addition, any substantial uplift of the Plateau, if such occurred during the past 3.5 Ma, would be expected to have caused an increase in monsoon strength. The Jingbian record shows that this was not the case. The main causal factor in the stepwise weakening of the summer monsoon, therefore, was probably the increase in global ice volume. The marine oxygen isotope record [23–25] shows a gradual, oscillatory increase in global ice volume from the late Pliocene until replaced by a dstationaryT fluctuation at around 0.8 Ma (Fig. 5E); this is broadly consistent with the trend in East-Asian monsoon evolution (Fig. 5C). Numerical modeling results also suggest that Pleistocene glaciation should lead to a substantial weakening of the East-Asian summer monsoon [35]. Here, we propose that the global ice volume signatures were transferred into the monsoon system by means of Z.L. Ding et al. / Earth and Planetary Science Letters 237 (2005) 45–55 three well-known mechanisms. (1) Development and expansion of polar ice sheets and sea ice cover would lead to increased temperature and atmospheric pressure gradients between the polar regions and the middle-low latitudes, thereby impeding northward movement of moisture-laden monsoon airflows. (2) Ice accumulation on continents would cause sea-level lowering and exposure of vast continental shelves in the Pacific marginal seas [42], thus resulting in enhanced continentality (increased distances to ocean moisture sources, affecting monsoon rainfall belt migration towards the inland desert margins). Given the steep monsoon precipitation gradients, particularly over northern China (Fig. 1), such changes would have the effect of weakening the summer monsoon. (3) The expansion of polar ice sheets and sea ice cover would result in the intensification of the northerly winter monsoon winds, imposing a downstream cooling on the low-latitude oceans. This would thereby lead to weakened oceanic water evaporation and a decreased summer monsoon season via delayed onset. The abruptness of desert margin shift (Fig. 5C and D) also suggests that threshold mechanisms should be recognized as fundamental factors in assessment of long-term monsoon evolution. By generating a multiple-proxy data set, Clemens et al. [43] found that the growth of ice sheets in the Northern Hemisphere over the past 3.5 Ma has weakened the Indian summer monsoon and increased the aridity of subtropical Asia and eastern Africa. With respect to long-term evolution, the phase of summer monsoon maxima relative to global ice volume maxima has changed significantly over both the precession and obliquity bands, with major changes occurring at about 2.6, 1.2 and 0.6 Ma. This would lead us to expect a similar evolutionary history for closely coupled though discrete East-Asian and Indian monsoons, although such abruptness of events shown here for China is not evident in the Indian monsoon records. The Indian subsystem has a north–south land–ocean configuration with a latent heat source in the southern hemisphere part of the Indian Ocean. In contrast, the East-Asian subsystem has a significant east–west land–ocean configuration with a major Pacific Ocean latent heat source (e.g. [44]). The close coupling between the Indian and East-Asian monsoon subsystems indicates that the common mechanism driving the long-term evolution of these subsystems 53 lies within the Asian continent, rather than within the oceans, providing further support for a link between northern hemisphere ice volume and monsoon strength, as argued here. The close linkage between the East-Asian monsoon and global ice volume, on both long and glacial cycle time scales, may have important implications for assessing the consequences of human-induced global warming for ecosystems in the semi-arid regions in northern China, where devastating desertification now threatens. 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